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NASA NTRS1972

Thyroid and adrenal cortical rhythmicity during bed rest.

The effects of prolonged bed rest on adrenocortical and thyroid function were assessed in eight healthy males, aged 20-40 years, who were submitted to bed rest for 56 days on a 14L:10D regimen (lights-on, 9:00 AM). Four of these subjects exercised three times daily throughout the experiment. Circulating cortisol, triiodothyronine, and thyroxine, concentrations were determined in blood samples drawn at four hourly intervals for 48-hr periods before, 10, 20, 30, 42, and 54 days during, and 10 days post-bed rest. Significant fluctuations in the circulating levels of all three hormones occurred with peaks at 7:30 AM. The suggestion is advanced that thyroid rhythms may be posture dependent.

Vernikos-Danellis, J.↗

NASA NTRS1998

Modeling the Variability of the BL Lacertae Object PKS 2155-304

The bright X-ray-selected BL Lacertae object PKS 2155-304 has been the target of two intense multi-wavelength campaigns in 1991 November and in 1994 May. Although the spectral energy distributions at both epochs were quite similar, the source exhibited two very distinct variability patterns that cannot be easily reconciled with homogeneous one-zone C7 jet models. During the first epoch the variability was almost achromatic in amplitude, with a time lag between X-rays and ultraviolet radiation (UV) of approximately three hours, while during the second epoch the variability amplitude increased as a function of wavelength with the EUV flare peaking approximately one day after the X-ray flare. We model the source using a time-dependent inhomogeneous accelerating jet model. We reproduce the general characteristics of the different variability signatures by assuming that plasma disturbances with different physical properties propagate downstream in an underlying jet characterized by the same set of physical parameters at both epochs. A time delay of approximately one day between the hardening of the UV spectral index and the UV flux present at both epochs is modeled with stochastic fluctuations in the particle acceleration manifested through small variations of the maximum energy of the injected electrons. We predict that similar time delays will be present in future observations even in the absence of strong variability event. We stress the importance of observations at neighboring frequencies as a diagnostic tool for the structure of the quiescent jet in blazars especially in the seemingly dull case in which strong variability is absent.

Georganopuolos, Markos↗

DOE OSTI2020

Standoff Detection of Chemical Plumes Using Swept-ECQCL Remote Detection Technology: Results from EMRTC Complex Terrain Dual Tracer Experiment

As part of the Complex Terrain Dual Tracer Experiments performed in support of the LYNM program, a swept-wavelength external cavity quantum cascade laser (swept-ECQCL) remote detection system was deployed to measure chemical plume propagation with high temporal resolution. The swept-ECQCL remote detection technology was initially developed at PNNL, and is now under further development at Opticslah, LLC under SBIR funding from DOE (DOE SBIR Phase I Project DE-SC0019855, Remote Detection Technologies, Program Manager Chris Ramos). The swept-ECQCL technology provides a single-frequency infrared laser source which is rapidly scanned over a large wavelength range to measure the infrared absorption of gases, liquids, or solids. Analysis of the measured infrared absorption spectrum is used to detect, identify, and quantify the chemical species which are present. While most previous laser-based techniques used small wavelength tuning ranges to measure only a few isolated spectral lines of a few species, the swept-ECQCL provides the large tuning range needed to measure multiple species simultaneously, and to detect broad absorption features from large molecules or condensed phase materials. In addition, the swept-ECQCL systems have high enough spectral resolution and sensitivity to measure narrow lines of small molecules and determine isotope ratios. The remote detection system for gas plumes is based on the swept-ECQCL technology, and consists of a swept-ECQCL source, infrared detector, control electronics, and beam transmitting and alignment optics. The remote detection system directs the infrared output of the swept-ECQCL to a target retro reflector typically located at ~10-10,000 m distance. The swept-ECQCL wavelength is varied continuously over a large wavelength range (>1000 nm) at rates up to 1000 Hz. The swept ECQCL light reflected from the remote target is collected and focused onto an infrared photodetector. By measuring the detector signal continuously as the swept-ECQCL wavelength is varied, a time-series of absorption spectra are measured for the gases along the beam line of-sight. Based on analysis and fitting of the measured absorption spectra, the time-dependent chemical concentrations of species are determined. Multiple species and mixtures can be detected simultaneously, for all species with absorption features above the sensor noise floor. The sensor output is thus a continuous, high-speed record of identified chemicals along with their concentrations and isotope ratios of interest. The high-speed operation enables low-noise operation in conditions of atmospheric turbulence and allows tracking of fluctuating concentrations in transient chemical plumes as needed for reliable remote detection applications. All components operate with minimal cooling requirements and no cryogens are needed. In addition, the output infrared light is invisible with an intensity below the maximum permissible exposure (MPE) threshold of 100 mW/cm2 for these infrared wavelengths and thus eye safe. The measurement concept for plume detection using the swept-ECQCL remote detection system is as follows. The ECQCL beam is directed toward a remote retro-reflector, which reflects the beam back to the ECQCL system where it is focused onto an infrared photodetector. The line-of-sight from the ECQCL system to the retro-reflector defines the measurement path. The detected infrared signal is recorded continuously and detects the absorption of molecular species along the measurement path. Before a plume release, the system measures absorption from atmospheric constituents, which in this LWIR band consist primarily of lines from H 2 O and CO 2 , with additional weaker absorption from N 2 O, NH 3 , and O 3 possibly contributing. The system then measures any changes in absorption due to the tracer compounds when they enter the measurement path. The shape of absorption features is used to distinguish and identify the different tracer compounds, and the strength of the absorption is used to determine the path-integrated concentration – also called the column density.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1986

Helicopter tail rotor noise analyses

A study was made of helicopter tail rotor noise, particularly that due to interactions with the main rotor tip vortices, and with the fuselage separation mean wake. The tail rotor blade-main rotor tip vortex interaction is modelled as an airfoil of infinite span cutting through a moving vortex. The vortex and the geometry information required by the analyses are obtained through a free wake geometry analysis of the main rotor. The acoustic pressure-time histories for the tail rotor blade-vortex interactions are then calculated. These acoustic results are compared to tail rotor loading and thickness noise, and are found to be significant to the overall tail rotor noise generation. Under most helicopter operating conditions, large acoustic pressure fluctuations can be generated due to a series of skewed main rotor tip vortices passing through the tail rotor disk. The noise generation depends strongly upon the helicopter operating conditions and the location of the tail rotor relative to the main rotor.

George, A. R.↗

NASA NTRS1986

Helicopter tail rotor noise

Chou, S.-T.↗

NASA NTRS2000

Towards LES Models of Jets and Plumes

As pointed out by Rodi standard integral solutions for jets and plumes developed for discharge into infinite, quiescent ambient are difficult to extend to complex situations, particularly in the presence of boundaries such as the sea floor or ocean surface. In such cases the assumption of similarity breaks down and it is impossible to find a suitable entrainment coefficient. The models are also incapable of describing any but the most slowly varying unsteady motions. There is therefore a need for full time-dependent modeling of the flow field for which there are three main approaches: (1) Reynolds averaged numerical simulation (RANS), (2) large eddy simulation (LES), and (3) direct numerical simulation (DNS). Rodi applied RANS modeling to both jets and plumes with considerable success, the test being a match with experimental data for time-averaged velocity and temperature profiles as well as turbulent kinetic energy and rms axial turbulent velocity fluctuations. This model still relies on empirical constants, some eleven in the case of the buoyant jet, and so would not be applicable to a partly laminar plume, may have limited use in the presence of boundaries, and would also be unsuitable if one is after details of the unsteady component of the flow (the turbulent eddies). At the other end of the scale DNS modeling includes all motions down to the viscous scales. Boersma et al. have built such a model for the non-buoyant case which also compares well with measured data for mean and turbulent velocity components. The model demonstrates its versatility by application to a laminar flow case. As its name implies, DNS directly models the Navier-Stokes equations without recourse to subgrid modeling so for flows with a broad spectrum of motions (high Re) the cost can be prohibitive - the number of required grid points scaling with Re(exp 9/4) and the number of time steps with Re(exp 3/4). The middle road is provided by LES whereby the Navier-Stokes equations are formally filtered with the filter chosen to only exclude the smallest turbulent motions. If successful, LES should provide much of the detail available to DNS but at more bearable cost. Fatica et al. in comparing LES with DNS for a low Reynolds number jet showed that the LES could simulate the temporally evolving behavior including growth of the jet thickness. It is the intention of this report to explore the application of an LES model to jets and plumes. As always, before tackling complex situations, the model must be tested for the simplest of cases and so we address only two, a non-buoyant axisymmetric jet issuing steadily from an orifice into a semi-infinite stationary environment and a buoyant jet in the same environment. The work is a continuation of Basu and Mansour.

Webb, A. T.↗

NASA NTRS2003

Unified Models of Turbulence and Nonlinear Wave Evolution in the Extended Solar Corona and Solar Wind

The PI (Cranmer) and Co-I (A. van Ballegooijen) made significant progress toward the goal of building a "unified model" of the dominant physical processes responsible for the acceleration of the solar wind. The approach outlined in the original proposal comprised two complementary pieces: (1) to further investigate individual physical processes under realistic coronal and solar wind conditions, and (2) to extract the dominant physical effects from simulations and apply them to a one-dimensional and time-independent model of plasma heating and acceleration. The accomplishments in the report period are thus divided into these two categories: 1a. Focused Study of Kinetic MHD Turbulence. We have developed a model of magnetohydrodynamic (MHD) turbulence in the extended solar corona that contains the effects of collisionless dissipation and anisotropic particle heating. A turbulent cascade is one possible way of generating small-scale fluctuations (easy to dissipate/heat) from a pre-existing population of low-frequency Alfven waves (difficult to dissipate/heat). We modeled the cascade as a combination of advection and diffusion in wavenumber space. The dominant spectral transfer occurs in the direction perpendicular to the background magnetic field. As expected from earlier models, this leads to a highly anisotropic fluctuation spectrum with a rapidly decaying tail in the parallel wavenumber direction. The wave power that decays to high enough frequencies to become ion cyclotron resonant depends on the relative strengths of advection and diffusion in the cascade. For the most realistic values of these parameters, though, there is insufficient power to heat protons and heavy ions. The dominant oblique waves undergo Landau damping, which implies strong parallel electron heating. We thus investigated the nonlinear evolution of the electron velocity distributions (VDFs) into parallel beams and discrete phase-space holes (similar to those seen in the terrestrial magnetosphere) which are an alternate means of heating protons via stochastic interactions similar to particle-particle collisions. 1b. Focused Study of the Multi-Mode Detailed Balance Formalism. The PI began to explore the feasibility of using the "weak turbulence," or detailed-balance theory of Tsytovich, Melrose, and others to encompass the relevant physics of the solar wind. This study did not go far, however, because if the "strong" MHD turbulence discussed above is a dominant player in the wind's acceleration region, this formalism is inherently not applicable to the corona. We will continue to study the various published approaches to the weak turbulence formalism, especially with an eye on ways to parameterize nonlinear wave reflection rates. 2. Building the Unified Model Code Architecture. We have begun developing the computational model of a time-steady open flux tube in the extended corona. The model will be "unified" in the sense that it will include (simultaneously for the first time) as many of the various proposed physical processes as possible, all on equal footing. To retain this generality, we have formulated the problem in two interconnected parts: a completely kinetic model for the particles, using the Monte Carlo approach, and a finite-difference approach for the self-consistent fluctuation spectra. The two codes are run sequentially and iteratively until complete consistency is achieved. The current version of the Monte Carlo code incorporates gravity, the zero-current electric field, magnetic mirroring, and collisions. The fluctuation code incorporates WKJ3 wave action conservation and the cascade/dissipation processes discussed above. The codes are being run for various test problems with known solutions. Planned additions to the codes include prescriptions for nonlinear wave steepening, kinetic velocity-space diffusion, and multi-mode coupling (including reflection and refraction).

Cranmer, Steven R.↗

DOE OSTI2020

Examination of synthetic gas puff imaging diagnostic data from a gyrokinetic turbulence code

A synthetic gas puff imaging (GPI) diagnostic has been developed for the purpose of validating the three-dimensional gyrokinetic turbulence code XGC. The synthetic diagnostic is described and applied to XGC simulations of two Alcator C-Mod discharges. The turbulence characteristics deduced from the resulting simulated GPI frames, using analysis techniques similar to those applied to experimental data, are compared with locally derived characteristics extracted directly from the XGC output. The comparison of the two is shown to be potentially impacted by misalignment between the GPI view and the magnetic field, the dependence of the light emission on the electron density and temperature, and spatial and temporal variations in the neutral gas cloud induced by the turbulent plasma fluctuations. We conclude that quantitative and, in some cases even qualitative, validation of turbulence simulations need to account for these effects. While we cannot directly compare our results with experimental data due to the absence of high quality GPI data from the shots and times simulated by XGC, we do relate the overall characteristics obtained from the synthetic GPI analysis to published Alcator C-Mod GPI data.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

Dynamical instability in multi-orbiter systems with gas friction

ABSTRACT Closely packed multiplanet systems are known to experience dynamical instability if the spacings between the planets are too small. Such instability can be tempered by the frictional forces acting on the planets from gaseous discs. A similar situation applies to stellar-mass black holes embedded in active galactic nuclei discs around supermassive black holes. We use N-body integrations to evaluate how the frictional damping of orbital eccentricity affects the growth of dynamical instability for a wide range of K (the difference in the planetary semimajor axes in units of the mutual Hill radius) and (unequal) planet masses. We find that, in general, the stable region (large K) and unstable region (small K) are separated by a “grey zone”, where the (in)stability is not guaranteed. We report the numerical values of the critical spacing for stability Kcrit and the “grey zone” range in different systems, and provide fitting formulae for arbitrary frictional forcing strength. We show that the stability of a system depends on the damping time-scale τ relative to the zero-friction instability growth time-scale tinst: two-planet systems are stable if tinst ≳ τ; three-planet systems require tinst ≳ 10τ−100τ. When K is sufficiently small, tinst can be less than the synodic period between the planets, which makes frictional stabilization unlikely to occur. As K increases, tinst tends to grow exponentially, but can also fluctuate by a few orders of magnitude. We also devise a linear map to analyse the dynamical instability of the “planet + test mass” system, and find qualitative agreement with N-body simulations.

Li, Jiaru (ORCID:0000000155507421)↗

NASA NTRS1975

UV stars and the interstellar medium - A statistical time-dependent model

A statistical time-dependent model for the effects on the interstellar gas of the ionizing radiation from UV stars is presented. The radiation from the stars is assumed to be emitted as monochromatic bursts at random times and locations. The thermal and ionization history of the gas is followed in a Monte Carlo simulation. Probability densities as well as mean values for the ionization fraction, temperature, and other observable quantities are derived. The fluctuations in observed quantities due to the stochastic nature of the model are estimated. Models of the interstellar medium perpendicular to the galactic plane are developed and compared with observations. The action of the UV stars can explain the bulk properties of the interstellar gas toward the galactic poles and is consistent with the Copernicus satellite observations toward lambda Scorpii.

Lyon, J.↗

NASA NTRS1973

Time dependent worldwide distribution of atmospheric neutrons and of their products. I, II, III.

Review of the experimental results obtained in a series of measurements of the fast neutron cosmic ray spectrum by means of high-altitude balloons and aircraft. These results serve as a basis for checking a Monte Carlo calculation of the entire neutron distribution and its products. A calculation of neutron production and transport in the earth's atmosphere is then discussed for the purpose of providing a detailed description of the morphology of secondary neutron components. Finally, an analysis of neutron observations during solar particle events is presented. The Monte Carlo output is used to estimate the contribution of flare particles to fluctuations in the steady state neutron distributions.

Merker, M.↗

NASA NTRS1992

A numerical study of two-dimensional vortex shedding from rectangular cylinders

An efficient time-marching, non-iterative calculation method is used to analyze time-dependent flows around rectangular cylinders. The turbulent flow in the wake region of a square section cylinder is analyzed using an anisotropic k-epsilon model. Initiation and subsequent development of the vortex shedding phenomenon is naturally captured once a perturbation is introduced in the flow. Transient calculations using standard eddy-viscosity and an anisotropic k-epsilon model averaged over an integral number of cycles to get the fluctuating energy (organized and turbulent) are compared with experimental data. It is shown that the anisotropic k-epsilon model resolves the anisotropy of the Reynolds stresses and gives mean energy distribution closer to the experiment than the standard k-epsilon model.

Hadid, A. H.↗

NASA NTRS1995

Statistical studies of impulsive events at high latitudes

A statistical study has been made of the high-latitude impulsive events that were observed during the 1985-1986 South Pole Balloon Campaign. The events were selected by searching for unipolar pulses greater than or equal to 10 nT above background in the vertical component of the magnetic field on the ground and/or pedestal or 'W' shaped horizontal electric field perturbations greater than or equal to 10 mV/m in amplitude and accompanied by perturbations in the vertical electric field at balloon altitude. A main event list comprising 112 events was compiled from the 468 hours of data available. Three aspects of the events were examined: the solar wind conditions prior to the event, local time of observation, and intrinsic properties of the events. The local time distribution was obtained from the 112 entry main event list and was found to be nearly uniform across the dayside, with no midday gap. The event rate found using our low-amplitude selection criteria was 0.7 event/hr, comparable to expectations based on in situ studies of the magnetopause. A total of 42 events were found for which data were available from Interplanetary Monitoring Platform (IMP) 8. Of these events, 12 occurred when the Z(sub GSM) component (B(sub Z)) of the interplanetary magnetic field (IMF) was northward and 30 occurred when B(sub Z) was southward or fluctuating. Only three of the B(sub Z) northward cases and only five of the B(sub Z) southward cases were preceded by pressure pulses greater than 0.4 nPa in amplitude. Ten of the events were studied in detail by means of a model-fitting method discussed elsewhere. This method infers values of several parameters, including the total current flowing in a coaxial or monopole system and a two-dimensional dipole system. The intrinsic properties of the events showed that only approximately 10% of the total current contributed to momentum transfer to the high-latitude ionosphere, that the direction of the motion depended more on local time of observation than IMF B(sub y), and that events were usually several hundred kilometers in size. The observed B(sub z) control found in the 42 event list and the prevalence of coaxial current dominated events are inconsistent with the predictions of the pressure pulse model.

Lin, Z. M.↗

NASA NTRS2005

Solar Wind Fluctuations and Their Consequences on the Magnetosphere

Efforts have been made to extract the physical meaning of each term in our prediction model of the Dst index using the solar wind as the only input. The work has been published Journal of Geophysical Research (Temerin and Li, 21002). We found different terms in the model representing different current in the magnetospheric system and each current has different rise and decay times, with the symmetric ring current the slowest, then the partial ring current, then the tail current. We also have been trying to understand the physical meaning of the diffusion coefficient used in our prediction model of relativistic electron fluxes at geostationary orbit. The model reproduced the observations of MeV electron flux variations well, the diffusion coefficient had be assumed only die to local magnetic field fluctuations, leading to its 10th power dependence on the L. We have studied the theoretical derivation of the diffusion coefficient and we believe that the effect electric field fluctuations at smaller L could become more significant. We have expanded our previous radiation belt electron prediction model, which predicted MeV electron geosynchronous orbit based on solar wind measurements, to predict MeV electrons inside geosynchronous orbit. The model results are compared with measurements from Polar/CEPPAD. Prediction efficiencies of 0.56 and 0.54, respectively, at L=6 and L=4, have been achieved over the entire year of 1998. This work wa reported at 2003 Fall AGU and has been accepted for publication in Space Weather (Barker et al., 2005). We also have used simultaneous measurements of the upstream solar wind and of energetic electrons at geosynchronous orbit to analyze the response of electrons over a very wide energy range, 50 keV-6MeV, to solar wind variations. Enhancements of energetic electron fluxes over this whole energy range are modulated by the solar wind speed and the polarity of the interplanetary magnetic field (IMF). The solar wind speed seems to be a dominant controlling parameter for electrons of all energy. This work has been published in Space Weather (Li et al., 2005).

Li, Xin-Lin↗

DOE OSTI2022

Turbulent flow characteristics in an 84-pin rod bundle for typical and damaged spacer grids

Hexagonal rod bundles arranged in a tightly packed triangular lattice are extensively used for heat transfer and energy generation applications. Staggered spacer grids are used to maintain the structural integrity of gas-cooled fast reactor (GFR) fuel assemblies, while inducing localized turbulence in flow. Damage to these spacer grids results in a disruption of flow fields within these hexagonal fuel bundles. Experimental flow visualizations are critical to identify the differences in local flow properties that the structural damage may cause. This experimental research investigates the flow-field characteristics at a near-wall and center plane in a prototypical 84-pin GFR fuel assembly. Newly installed typical spacers and spacers subject to naturally occurring damage due to material degradation over prolonged experimentation were investigated. Velocity fields were acquired by utilizing the matched-index-of-refraction method to obtain time-resolved particle image velocimetry measurements for a Reynolds number of 12 000. Reynolds decomposition statistical results divulged differences in the time-averaged velocity, velocity fluctuations, flow anisotropy, and Reynolds stress distributions. Galilean decomposition demarcated the influence of spacer grid damage on the velocity fields. To extract turbulent structures and elucidate mechanisms of flow instabilities, proper orthogonal decomposition analysis was employed. Reduced order flow reconstructions enabled the application of vortex identification algorithms to determine the spatial and statistical characteristics of vortices generated. This research work provides unique experimental data on the spacer grid condition-dependent flow. The results offer a deeper understanding of fluid dynamics behavior to support GFR rod bundle design efforts and computational fluid dynamics model validation.

36 MATERIALS SCIENCE↗

NASA NTRS2003

Presumed PDF Modeling of Early Flame Propagation in Moderate to Intense Turbulence Environments

The present paper describes the results obtained from a one-dimensional time dependent numerical technique that simulates early flame propagation in a moderate to intense turbulent environment. Attention is focused on the development of a spark-ignited, premixed, lean methane/air mixture with the unsteady spherical flame propagating in homogeneous and isotropic turbulence. A Monte-Carlo particle tracking method, based upon the method of fractional steps, is utilized to simulate the phenomena represented by a probability density function (PDF) transport equation. Gaussian distributions of fluctuating velocity and fuel concentration are prescribed. Attention is focused on three primary parameters that influence the initial flame kernel growth: the detailed ignition system characteristics, the mixture composition, and the nature of the flow field. The computational results of moderate and intense isotropic turbulence suggests that flames within the distributed reaction zone are not as vulnerable, as traditionally believed, to the adverse effects of increased turbulence intensity. It is also shown that the magnitude of the flame front thickness significantly impacts the turbulent consumption flame speed. Flame conditions studied have fuel equivalence ratio s in the range phi = 0.6 to 0.9 at standard temperature and pressure.

Carmen, Christina↗

DOE OSTI2022

Deep modelling of plasma and neutral fluctuations from gas puff turbulence imaging

The role of turbulence in setting boundary plasma conditions is presently a key uncertainty in projecting to fusion energy reactors. To robustly diagnose edge turbulence, we develop and demonstrate a technique to translate brightness measurements of HeI line radiation into local plasma fluctuations via a novel integrated deep learning framework that combines neutral transport physics and collisional radiative theory for the $3^3 D - 2^3 P$ transition in atomic helium. The tenets for experimental validity are reviewed, illustrating that this turbulence analysis for ionized gases is transferable to both magnetized and unmagnetized environments with arbitrary geometries. Based upon fast camera data on the Alcator C-Mod tokamak, we present the first 2-dimensional time-dependent experimental measurements of the turbulent electron density, electron temperature, and neutral density revealing shadowing effects in a fusion plasma using a single spectral line.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2020

Atomic fluctuations in electronic materials revealed by dephasing

The microscopic origin and timescale of the fluctuations of the energies of electronic states has a significant impact on the properties of interest of electronic materials, with implication in fields ranging from photovoltaic devices to quantum information processing. Spectroscopic investigations of coherent dynamics provide a direct measurement of electronic fluctuations. Modern multidimensional spectroscopy techniques allow the mapping of coherent processes along multiple time or frequency axes and thus allow unprecedented discrimination between different sources of electronic dephasing. Exploiting modern abilities in coherence mapping in both amplitude and phase, we unravel dissipative processes of electronic coherences in the model system of CdSe quantum dots (QDs). The method allows the assignment of the nature of the observed coherence as vibrational or electronic. The expected coherence maps are obtained for the coherent longitudinal optical (LO) phonon, which serves as an internal standard and confirms the sensitivity of the technique. Fast dephasing is observed between the first two exciton states, despite their shared electron state and common environment. This result is contrary to predictions of the standard effective mass model for these materials, in which the exciton levels are strongly correlated through a common size dependence. In contrast, the experiment is in agreement with ab initio molecular dynamics of a single QD. Electronic dephasing in these materials is thus dominated by the realistic electronic structure arising from fluctuations at the atomic level rather than static size distribution. The analysis of electronic dephasing thereby uniquely enables the study of electronic fluctuations in complex materials.

36 MATERIALS SCIENCE↗