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At least 379 records · Page 21

Latest D0 results on exotic hadrons produced in $p\bar p $ collision

Prompt and nonprompt productions of exotic multiquark states are studied using the $\sim$10.4~fb$^{-1}$ data sample collected by the D0 experiment in Tevatron $p\bar{p}$ collisions at $\sqrt{s}$ = 1.96 TeV. The recent D0 results on the prompt and nonprompt production of the $X(3872)$ and $Z_c^+(3900)$ states and the $P_c$ pentaquarks at the 4450~MeV region are reported. Signals corresponding to these states are found in the nonprompt production, whereas only the $X(3872)$ state is seen in the prompt production. The ratio of prompt to nonprompt $X(3872)$ production is about three times larger in the D0 measurement than that obtained by the ATLAS experiment at 8 TeV. Theoretically, the production, formation, coalescence, and disassociation processes are expected to be quite different for conventional mesons with a spatial size of (0.4-0.8) fm, compact multiquark states such as tetraquarks with a size of a few fm, and spatially extended molecular states with a size of (4-10) fm. They can be differently affected in prompt hadron-hadron collisions where there are many additional particles emitted from the interaction point. Consequently, the prompt to nonprompt production ratio of spatially extended exotic states can be suppressed at LHC comparing with the Tevatron conditions, because of large difference in the hadron-hadron collisions particle multiplicity. The prompt production studies provide an opportunity to better understand the nature of exotic states.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Uses of Multi-Objective Flux Analysis for Optimization of Microbial Production of Secondary Metabolites

Secondary metabolites are not essential for the growth of microorganisms, but they play a critical role in how microbes interact with their surroundings. In addition to this important ecological role, secondary metabolites also have a variety of agricultural, medicinal, and industrial uses, and thus the examination of secondary metabolism of plants and microbes is a growing scientific field. While the chemical production of certain secondary metabolites is possible, industrial-scale microbial production is a green and economically attractive alternative. This is even more true, given the advances in bioengineering that allow us to alter the workings of microbes in order to increase their production of compounds of interest. This type of engineering requires detailed knowledge of the “chassis” organism’s metabolism. Since the resources and the catalytic capacity of enzymes in microbes is finite, it is important to examine the tradeoffs between various bioprocesses in an engineered system and alter its working in a manner that minimally perturbs the robustness of the system while allowing for the maximum production of a product of interest. The in silico multi-objective analysis of metabolism using genome-scale models is an ideal method for such examinations.

59 BASIC BIOLOGICAL SCIENCES↗

Data Release 1 of the Dark Energy Spectroscopic Instrument

In 2021 May the Dark Energy Spectroscopic Instrument (DESI) collaboration began a 5 yr spectroscopic redshift survey to produce a detailed map of the evolving three-dimensional structure of the Universe between z = 0 and z ≈ 4. DESI’s principal scientific objectives are to place precise constraints on the equation of state of dark energy, the gravitationally driven growth of large-scale structure, and the sum of the neutrino masses, and to explore the observational signatures of primordial inflation. We present DESI DR1, which consists of all data acquired during the first 13 months of the DESI main survey, as well as a uniform reprocessing of the DESI Survey Validation data, which were previously made public in the DESI Early Data Release. The DR1 main survey includes high-confidence redshifts for 18.7M objects, of which 13.1M are spectroscopically classified as galaxies, 1.6M as quasars, and 4M as stars, making DR1 the largest sample of extragalactic redshifts ever assembled. We summarize the DR1 observations, the spectroscopic data-reduction pipeline and data products, large-scale structure catalogs, value-added catalogs, and describe how to access and interact with the data. In addition to fulfilling its core cosmological objectives with unprecedented precision, we expect DR1 to enable a wide range of transformational astrophysical studies and discoveries.

79 ASTRONOMY AND ASTROPHYSICS↗

Background optimization of powder electron diffraction for implementation of the e-PDF technique and study of the local structure of iron oxide nanocrystals

The local structural characterization of iron oxide nanoparticles is explored using a total scattering analysis method known as pair distribution function (PDF) (also known as reduced density function) analysis. The PDF profiles are derived from background-corrected powder electron diffraction patterns (the e-PDF technique). Due to the strong Coulombic interaction between the electron beam and the sample, electron diffraction generally leads to multiple scattering, causing redistribution of intensities towards higher scattering angles and an increased background in the diffraction profile. In addition to this, the electron–specimen interaction gives rise to an undesirable inelastic scattering signal that contributes primarily to the background. The present work demonstrates the efficacy of a pre-treatment of the underlying complex background function, which is a combination of both incoherent multiple and inelastic scatterings that cannot be identical for different electron beam energies. Therefore, two different background subtraction approaches are proposed for the electron diffraction patterns acquired at 80 kV and 300 kV beam energies. From the least-square refinement (small-box modelling), both approaches are found to be very promising, leading to a successful implementation of the e-PDF technique to study the local structure of the considered nanomaterial.

36 MATERIALS SCIENCE↗

Out-of-pile and postirradiated examination of lanthanide and lanthanide-palladium interactions for metallic fuel

Palladium is being investigated as a fuel additive to bind with and potentially immobilize lanthanide fission products. A primary cause of fuel-cladding chemical interaction (FCCI) is the lanthanide fission products migrating to the fuel periphery and interacting with the cladding. This interaction will lead to wastage of the cladding and eventually to a cladding breach. Palladium has previously been identified as a promising additive used to prevent or decrease FCCI by reacting with the lanthanide fission products. In the current study, an alloy cast from the four highest abundant lanthanides found in irradiated metallic fuel, Nd, Ce, Pr, and La, with and without Pd, has been characterized using neutron diffraction, scanning electron microscopy, and electron probe microanalysis. In the lanthanide-Pd intermetallic compounds, all of the constituent compounds, i.e. Nd-Pd, Ce-Pd, La-Pd and Pr-Pd are known. There is very good agreement, both structurally and compositionally, between the out-of-pile lanthanide alloy and lanthanide fission products characterized in irradiated fuels. In both cases, the lanthanide elements form a solid solution in a hexagonal crystal structure. The out-of-pile lanthanide alloy follows Vegard's Law, with the measured and calculated (weighted average of constituents) lattice parameters being within 1% for both the a and c parameters. Pd bonds with the lanthanides (Ln) forming the phases LnPd and Ln7Pd3. The results indicate the properties of lanthanide compounds in irradiated metallic fuel can be reliably simulated in out-of-pile experiments.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Controlling process instability for defect lean metal additive manufacturing

The process instabilities intrinsic to the localized laser-powder bed interaction cause the formation of various defects in laser powder bed fusion (LPBF) additive manufacturing process. Particularly, the stochastic formation of large spatters leads to unpredictable defects in the as-printed parts. Here we report the elimination of large spatters through controlling laser-powder bed interaction instabilities by using nanoparticles. The elimination of large spatters results in 3D printing of defect lean sample with good consistency and enhanced properties. We reveal that two mechanisms work synergistically to eliminate all types of large spatters: (1) nanoparticle-enabled control of molten pool fluctuation eliminates the liquid breakup induced large spatters; (2) nanoparticle-enabled control of the liquid droplet coalescence eliminates liquid droplet colliding induced large spatters. The nanoparticle-enabled simultaneous stabilization of molten pool fluctuation and prevention of liquid droplet coalescence discovered here provide a potential way to achieve defect lean metal additive manufacturing.

36 MATERIALS SCIENCE↗

Scalable Pattern Matching in Metadata Graphs via Constraint Checking

Pattern matching is a fundamental tool for answering complex graph queries. Unfortunately, existing solutions have limited capabilities: They do not scale to process large graphs and/or support only a restricted set of search templates or usage scenarios. Moreover, the algorithms at the core of the existing techniques are not suitable for today’s graph processing infrastructures relying on horizontal scalability and shared-nothing clusters, as most of these algorithms are inherently sequential and difficult to parallelize. In this article we present an algorithmic pipeline that bases pattern matching on constraint checking. The key intuition is that each vertex and edge participating in a match has to meet a set of constraints implicitly specified by the search template. These constraints can be verified independently and typically are less expensive to compute than searching the full template. The pipeline we propose generates these constraints and iterates over them to eliminate all the vertices and edges that do not participate in any match, thus reducing the background graph to a subgraph that is the union of all template matches—the complete set of all vertices and edges that participate in at least one match. Additional analysis can be performed on this annotated, reduced graph, such as full match enumeration, match counting, or computing vertex/edge centrality. Furthermore, a vertex-centric formulation for constraint checking algorithms exists, and this makes it possible to harness existing high-performance, vertex-centric graph processing frameworks. This technique (i) enables highly scalable pattern matching in metadata (labeled) graphs; (ii) supports arbitrary patterns with 100% precision; (iii) enables tradeoffs between precision and time-to-solution, while always selects all vertices and edges that participate in matches, thus offering 100% recall; and (iv) supports a set of popular data analytics scenarios. We implement our approach on top of HavoqGT, an open-source asynchronous graph processing framework, and demonstrate its advantages through strong and weak scaling experiments on massive scale real-world (up to 257 billion edges) and synthetic (up to 4.4 trillion edges) labeled graphs, respectively, and at scales (1,024 nodes / 36,864 cores), orders of magnitude larger than used in the past for similar problems. This article serves two purposes: First, it synthesises the knowledge accumulated during a long-term project. Second, it presents new system features, usage scenarios, optimizations, and comparisons with related work that strengthen the confidence that pattern matching based on iterative pruning via constraint checking is an effective and scalable approach in practice. The new contributions include the following: (i) We demonstrate the ability of the constraint checking approach to efficiently support two additional search scenarios that often emerge in practice, interactive incremental search and exploratory search. (ii) We empirically compare our solution with two additional state-of-the-art systems, Arabsque and TriAD. (iii) We show the ability of our solution to accommodate a more diverse range of datasets with varying properties, e.g., scale, skewness, label distribution, and match frequency. (iv) We introduce or extend a number of system features (e.g., work aggregation, load balancing, and the ability to cap the generated traffic) and design optimizations and demonstrate their advantages with respect to improving performance and scalability. (v) We present bottleneck analysis and insights into artifacts that influence performance. (vi) We present a theoretical complexity argument that motivates the performance gains we observe.

97 MATHEMATICS AND COMPUTING↗

Addressing Uncertainty in MultiSector Dynamics Research

MultiSector Dynamics (MSD) research explores the dynamics and co-evolutionary pathways of human and Earth systems and the emerging interdependent sectors of energy, water, agriculture, and transportation among others. The interactions between these sectors are central to MSD science, as they capture how processes and feedbacks across Earth, environmental, infrastructure, and societal systems shape transitions, socioeconomic risks, and the provision of services. By definition, MSD research requires deep integration across diverse scientific disciplines, ranging from the natural to the social sciences and engineering. All these disciplines apply a variety of numerical simulation models to study and understand their underlying systems of focus. The utility of these models hinges on the fidelity with which they represent the real systems and their ability to produce novel insights about systems and their interactions. The coupled human-natural systems typically represented are shaped by a multitude of interdependent human and natural processes which, when modeled, translate to highly complex, non-linear, interacting behaviors. This ever-increasing complexity massively expands the uncertainty space of a model and can be found in model inputs, processes and parameters. This is further amplified when several models are combined to answer multisectoral questions, as additional uncertainty regarding coupling relationships and interactions is introduced.

IM3, Uncertainty and Sensitivity Analysis, multise↗

Alkane Dehydrogenation and H/D Exchange by a Cationic Pincer-Ir(III) Hydride: Cooperative C–H Addition and β -H Elimination Modes Induce Anomalous Selectivity

We report that the cationic iridium complex ( iPr PCP)IrH + catalyzes the transfer-dehydrogenation of alkanes to give alkenes and hydrogen isotope exchange (HIE) of alkanes and arenes. Contrary to established selectivity trends found for C–H activation by transition metal complexes, strained cycloalkanes, including cyclopentane, cycloheptane, and cyclooctane, undergo C–H addition much more readily than n-alkanes, which in turn are much more reactive than cyclohexane. Aromatic C–H bonds also undergo H/D exchange much less rapidly than those of the strained cycloalkanes, but much more favorably than cyclohexane. The order of reactivity toward dehydrogenation correlates qualitatively with the reaction thermodynamics, but the magnitude is much greater than can be explained by thermodynamics. Accordingly, the cycloalkenes corresponding to the strained cycloalkanes undergo hydrogenation much more readily than cyclohexene, despite the less favorable thermodynamics of such hydrogenations. Here, computational (DFT) studies allow rationalization of the origin of reactivity and the unusual selectivity. Specifically, the initial C–H addition is strongly assisted by β-agostic interactions, which are particularly favorable for the strained cycloalkanes. Subsequent to α-C–H addition, the H atom of the β-agostic C–H bond is transferred directly to the hydride ligand of ( iPr PCP)IrH + to give a dihydrogen ligand.

02 PETROLEUM↗

A temporal analysis and response to nitrate availability of 3D root system architecture in diverse pennycress (Thlaspi arvense L.) accessions

Introduction Roots have a central role in plant resource capture and are the interface between the plant and the soil that affect multiple ecosystem processes. Field pennycress ( Thlaspi arvense L.) is a diploid annual cover crop species that has potential utility for reducing soil erosion and nutrient losses; and has rich seeds (30-35% oil) amenable to biofuel production and as a protein animal feed. The objective of this research was to (1) precisely characterize root system architecture and development, (2) understand plastic responses of pennycress roots to nitrate nutrition, (3) and determine genotypic variance available in root development and nitrate plasticity. Methods Using a root imaging and analysis pipeline, the 4D architecture of the pennycress root system was characterized under four nitrate regimes, ranging from zero to high nitrate concentrations. These measurements were taken at four time points (days 5, 9, 13, and 17 after sowing). Results Significant nitrate condition response and genotype interactions were identified for many root traits, with the greatest impact observed on lateral root traits. In trace nitrate conditions, a greater lateral root count, length, density, and a steeper lateral root angle was observed compared to high nitrate conditions. Additionally, genotype-by-nitrate condition interaction was observed for root width, width:depth ratio, mean lateral root length, and lateral root density. Discussion These findings illustrate root trait variance among pennycress accessions. These traits could serve as targets for breeding programs aimed at developing improved cover crops that are responsive to nitrate, leading to enhanced productivity, resilience, and ecosystem service.

59 BASIC BIOLOGICAL SCIENCES↗

A Study of Wake Characteristics of Marine Turbine Arrays: Preprint

As the marine energy industry continues to develop and installations grow from single turbines to small arrays and larger farms, understanding and predicting wake behavior using modeling tools is necessary for array design and optimization. The wake characteristics of upstream turbines, including velocity deficit, wake swirling, tip vortices, wake shape and direction, and flow recovery, influence the inflow conditions experienced by downstream turbines in an array and, subsequently, affect the individual turbine loading and power generated by the array. These wake characteristics are influenced by many factors, including site geography, inflow shear profile, turbulence, waves, the strength of the current resource, gravitational forces, storm surges, and seasonal effects like temperature and wind conditions. Efficient array modeling tools that capture these wake effects and resulting turbine-to-turbine interactions need to be developed to optimize farm layouts and design individual turbines for operation within arrays. Unlike the wind industry, the marine energy research community is largely limited to the use of either numerical tools or tank/flume testing to understand marine turbine wake interactions. This paper will investigate recent advances in numerical and experimental marine turbine wake modeling, with a focus on recent publications and on both axial-flow and cross-flow marine turbines. A summary of recent research on these topics is provided. Additionally, a demonstration of turbine wake interactions using computational fluid dynamics is presented.

marine hydrokinetic turbine↗

MeV Scale Physics in MicroBooNE

This thesis presents the reconstruction and measurement of low-energy electromagnetic activity with beam neutrino interactions within the MicroBooNE Liquid Argon Time Projection Chamber (LArTPC). LArTPCs have proven to be excellent detectors to measure neutrino interaction cross sections and are being used to perform precision measurements of neutrino oscillation parameters. The work presented in this thesis has demonstrated unprecedentedly low, sub-MeV energy thresholds that have increased sensitivity of LArTPCs to detect neutrino interactions from core collapse supernovae and Muon Decay at Rest (µDAR). In addition, such low thresholds have also increased measurement sensitivity for interactions from Beyond the Standard Model (BSM) candidates such as millicharged particles and nuclear and electron recoils from dark matter candidate particles. On the reconstruction side, this work has established an energy resolution of 6.3% for electromagnetic activity i the 0-5 MeV energy range within the MicroBooNE LArTPC. Additionally this work presents the quantitative analysis of the low-energy activity emanating from G-10 support ribs in MicroBooNE and discusses how such activity could be a problematic source of background for low-energy physics analyses in future neutrino detectors such as the Deep Underground Neutrino Experiment (DUNE).

Bhat, Avinay↗

Impact of Resonator-Assisted ZZ Cancellation on Cross-Resonance Gate Performance

Strong coupling in superconducting processors enables fast two-qubit gates but also produces static ZZ interactions that degrade performance. Flux-tunable couplers can suppress ZZ but introduce flux noise and additional hardware complexity. A driven-resonator RIP interaction offers a simple method to dynamically cancel ZZ [1]. Using this RIP-based cancellation scheme in a fixed-frequency transmon system, we compare cross-resonance gate behavior with and without ZZ suppression. Idling errors improve substantially when ZZ is cancelled, while CR calibration reveals clear tradeoffs in Hamiltonian composition and achievable gate speed. [1]: Huang, Z. et al. (2024). Physical Review Applied, 22(3), 034007.

Heidler, Paul [Fermilab]↗

Deep learning approaches for instantaneous laser absorptance prediction in additive manufacturing

Abstract The quantification of absorbed light is essential for understanding laser-material interactions and melt pool dynamics in order to minimize defects in additively manufactured metal components. The geometry of a vapor depression formed during laser melting is closely related to laser energy absorption. This relationship has been observed by the state-of-the-art in situ high-speed synchrotron X-ray visualization and integrating sphere radiometry. These two techniques create a temporally resolved dataset consisting of vapor depression images and corresponding laser absorptance. In this work, we propose two different approaches to predict instantaneous laser absorptance. The end-to-end approach uses deep convolutional neural networks to learn implicit features of X-ray images automatically and predict the laser energy absorptance. The two-stage approach uses a semantic segmentation model to engineer geometric features and predict absorptance using classical regression models. While having distinct advantages, both approaches achieved a consistently low mean absolute error of less than 3.3%.

Chemistry↗

Constraints on hadron resonance gas interactions via first-principles Lattice QCD susceptibilities

We investigate extensions of the Hadron Resonance Gas (HRG) Model beyond the ideal case by incorporating both attractive and repulsive interactions into the model. When considering additional states exceeding those measured with high confidence by the Particle Data Group, attractive corrections to the overall pressure in the HRG model are imposed. On the other hand, we also apply excluded-volume corrections, which ensure there is no overlap of baryons by turning on repulsive (anti)baryon-(anti)baryon interactions. We emphasize the complementary nature of these two extensions and identify combinations of conserved charge susceptibilities that allow us to constrain them separately. In particular, we find interesting ratios of susceptibilities that are sensitive to one correction and not the other. This allows us to constrain the excluded volume and particle spectrum effects separately. Analysis of the available lattice results suggests the presence of both the extra states in the baryonstrangeness sector and the repulsive baryonic interaction, with indications that hyperons have a smaller repulsive core than non-strange baryons. We note that these results are interesting for heavy-ion-collision systems at both the LHC and RHIC.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

High Temperature Polymer Electrolyte Membrane Fuel Cells with High Phosphoric Acid Retention

Phosphoric acid loss poses immense hurdles for the durability of high-temperature polymer electrolyte membrane fuel cells (HT-PEMFCs). Here we report quaternary ammonium-biphosphate ion-pair HT-PEMFCs that do not lose phosphoric acids under normal and accelerated stress conditions. Additionally, our energetics study explains the acid loss behavior of the conventional phosphoric acid-polybenzimidazole (PA-PBI) system by two mechanisms. If PA loss occurs via acid evaporation, the acid loss is constant over time. On the other hand, when water activity in the PA-PBI system is high, exponential decay of PA loss occurs via the water replacement mechanism. Combined 31 P NMR and computational studies show that the proposed ion-pair system has six times higher interaction energy, which allows for containing all PAs in the membrane electrode assemblies under a broad range of operating conditions. In addition, polar interactions between the phosphonic acid ionomer and phosphoric acid explain acid retention in the electrodes of the ion-pair HT-PEMFCs.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗