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NASA NTRS1995

Clouds and the Earth's Radiant Energy System (CERES) algorithm theoretical basis document: Overviews (subsystem 0) - Volume 1

The theoretical bases for the Release 1 algorithms that will be used to process satellite data for investigation of the Clouds and the Earth's Radiant Energy System (CERES) are described. The architecture for software implementation of the methodologies is outlined. Volume 1 provides both summarized and detailed overviews of the CERES Release 1 data analysis system. CERES will produce global top-of-the-atmosphere shortwave and longwave radiative fluxes at the top of the atmosphere, at the surface, and within the atmosphere by using the combination of a large variety of measurements and models. The CERES processing system includes radiance observations from CERES scanning radiometers, cloud properties derived from coincident satellite imaging radiometers, temperature and humidity fields from meteorological analysis models, and high-temporal-resolution geostationary satellite radiances to account for unobserved times. CERES will provide a continuation of the ERBE record and the lowest error climatology of consistent cloud properties and radiation fields. CERES will also substantially improve our knowledge of the Earth's surface radiation budget.

Wielicki, Bruce A.↗

NASA NTRS2015

Snowfall Rate Retrieval Using Passive Microwave Measurements and Its Applications in Weather Forecast and Hydrology

(AMSU), Microwave Humidity Sounder (MHS) and Advance Technology Microwave Sounder (ATMS). ATMS is the follow‐on sensor to AMSU and MHS. Currently, an AMSU and MHS based land snowfall rate (SFR) product is running operationally at NOAA/NESDIS. Based on the AMSU/MHS SFR, an ATMS SFR algorithm has also been developed. The algorithm performs retrieval in three steps: snowfall detection, retrieval of cloud properties, and estimation of snow particle terminal velocity and snowfall rate. The snowfall detection component utilizes principal component analysis and a logistic regression model. It employs a combination of temperature and water vapor sounding channels to detect the scattering signal from falling snow and derives the probability of snowfall. Cloud properties are retrieved using an inversion method with an iteration algorithm and a two‐stream radiative transfer model. A method adopted to calculate snow particle terminal velocity. Finally, snowfall rate is computed by numerically solving a complex integral. The SFR products are being used mainly in two communities: hydrology and weather forecast. Global blended precipitation products traditionally do not include snowfall derived from satellites because such products were not available operationally in the past. The ATMS and AMSU/MHS SFR now provide the winter precipitation information for these blended precipitation products. Weather forecasters mainly rely on radar and station observations for snowfall forecast. The SFR products can fill in gaps where no conventional snowfall data are available to forecasters. The products can also be used to confirm radar and gauge snowfall data and increase forecasters' confidence in their prediction.

Meng, Huan↗

NASA NTRS2023

Updated Observations of Clouds By MODIS for Global Model Assessment

This paper describes a new global dataset of cloud properties observed by MODIS relying on the current (collection 6.1) processing of MODIS data and produced to facilitate comparison with results from the MODIS observational proxy used in climate models. The dataset merges observations from the two MODIS instruments into a single netCDF file. Statistics (mean, standard deviation, and number of observations) are accumulated over daily and monthly timescales on an equal-angle grid for viewing and illumination geometry, cloud detection, cloud-top pressure, and cloud properties (optical thickness, effective particle size, and water path) partitioned by thermodynamic phase and an assessment as to whether the underlying observations come from fully or partly cloudy pixels. Similarly partitioned joint histograms are available for (1) optical thickness and cloud-top pressure, (2) optical thickness and particle size, and (3) cloud water path and particle size. Differences with standard data products, caveats for data use, and guidelines for comparison to the MODIS simulator are described.

Robert Pincus↗

NASA NTRS2008

High Vertically Resolved Atmospheric and Surface/Cloud Parameters Retrieved with Infrared Atmospheric Sounding Interferometer (IASI)

The Joint Airborne IASI Validation Experiment (JAIVEx) was conducted during April 2007 mainly for validation of the IASI on the MetOp satellite. IASI possesses an ultra-spectral resolution of 0.25/cm and a spectral coverage from 645 to 2760/cm. Ultra-spectral resolution infrared spectral radiance obtained from near nadir observations provide atmospheric, surface, and cloud property information. An advanced retrieval algorithm with a fast radiative transfer model, including cloud effects, is used for atmospheric profile and cloud parameter retrieval. This physical inversion scheme has been developed, dealing with cloudy as well as cloud-free radiance observed with ultraspectral infrared sounders, to simultaneously retrieve surface, atmospheric thermodynamic, and cloud microphysical parameters. A fast radiative transfer model, which applies to the cloud-free and/or clouded atmosphere, is used for atmospheric profile and cloud parameter retrieval. A one-dimensional (1-d) variational multi-variable inversion solution is used to improve an iterative background state defined by an eigenvector-regression-retrieval. The solution is iterated in order to account for non-linearity in the 1-d variational solution. It is shown that relatively accurate temperature and moisture retrievals are achieved below optically thin clouds. For optically thick clouds, accurate temperature and moisture profiles down to cloud top level are obtained. For both optically thin and thick cloud situations, the cloud top height can be retrieved with relatively high accuracy (i.e., error < 1 km). Preliminary retrievals of atmospheric soundings, surface properties, and cloud optical/microphysical properties with the IASI observations are obtained and presented. These retrievals will be further inter-compared with those obtained from airborne FTS system, such as the NPOESS Airborne Sounder Testbed - Interferometer (NAST-I), dedicated dropsondes, radiosondes, and ground based Raman Lidar. The capabilities of satellite ultra-spectral sounder such as the IASI are investigated indicating a high vertical structure of atmosphere is retrieved.

Zhou, Daniel K.↗

NASA NTRSDate not supplied

Assessing the Variability of Radiation, Water and Energy in the Deep Tropics Over the Last 3 Decades

Global surface energy closure and its variability depends heavily upon the surface radiative energy budget in the deep tropics. A key process observed is the change in convection regimes from disorganized convection to organized deep convection. During these periods an imbalance is observed between energy and water fluxes in terms of energy closure in some atmospheric reanalysis systems, implying that processes are not simulated well. A recent paper by Hsaio et al (2023, pre-published version) found that the transition process has wind shear and longwave cloud radiative feedback signatures. In this presentation, we assess the surface radiative budget in the deep tropics by comparing multiple data products (GEWEX SRB Rel4IP, CERES Ed4.1, ISSCP FH, etc.) and describing the variability across the deep tropics for the period from 1988 to near present. We assess this variability of the radiative flux anomalies (including the net TOA, surface and the atmospheric divergence fluxes) against water vapor divergence, cloud properties (include ISCCP “Weather States, Tselioudis et al. 2021) and larger scale wind shear. We include further analysis contrasting 6 key tropical oceanic regions (Indian Ocean east and west, tropical western, central and eastern Pacific Ocean, and Tropical Atlantic Ocean) and the sensitivity of the fluxes as a function of fluctuations in cloud types in response to various larger scale atmospheric processes (e.g. El Niño, Indian Ocean Dipole). These are contrasted against the modeled radiative fluxes from ERA-5 and MERRA-2. Ocean buoy measurements of radiative fluxes are utilized to help assess data radiative flux uncertainty over the nearly 40 year period. In general, the variability for overlap periods of these various data products agrees well, but there are significant differences in the net fluxes that vary according to the rendering of surface, atmospheric, aerosol and cloud properties. We conclude with recommendations for continuing work.

Radiation budget↗

NASA NTRS2002

Parameterization of Cloud Optical Properties for a Mixture of Ice Particles for use in Atmospheric Models

Based on the single-scattering optical properties that are pre-computed using an improve geometric optics method, the bulk mass absorption coefficient, single-scattering albedo, and asymmetry factor of ice particles have been parameterized as a function of the mean effective particle size of a mixture of ice habits. The parameterization has been applied to compute fluxes for sample clouds with various particle size distributions and assumed mixtures of particle habits. Compared to the parameterization for a single habit of hexagonal column, the solar heating of clouds computed with the parameterization for a mixture of habits is smaller due to a smaller cosingle-scattering albedo. Whereas the net downward fluxes at the TOA and surface are larger due to a larger asymmetry factor. The maximum difference in the cloud heating rate is approx. 0.2 C per day, which occurs in clouds with an optical thickness greater than 3 and the solar zenith angle less than 45 degrees. Flux difference is less than 10 W per square meters for the optical thickness ranging from 0.6 to 10 and the entire range of the solar zenith angle. The maximum flux difference is approximately 3%, which occurs around an optical thickness of 1 and at high solar zenith angles.

Chou, Ming-Dah↗

NASA NTRS2024

Mapping Cloud Microphysical Properties to Triple-Wavelength Airborne Lidar Measurements in Winter Storms: Results from the IMPACTS Field Campaign

Ice production and growth inmixed-phase cloudsgive a complicated picture of the radiative and mass characteristics due to the heterogeneity of particle shapes and sizes. Collocated airborne lidar and microphysics datasets from a recent winter storm field study are used to evaluate the effect of ice and liquid hydrometeors,observed in situ,on the multiple-wavelength backscatter coefficientvalues measured by the NASA Cloud Physics Lidarover the course of three winter deployments in the Midwestand Northeast United States.

Joseph A. Finlon↗

NASA NTRS2002

Parameterization of Shortwave Cloud Optical Properties for a Mixture of Ice Particle Habits for use in Atmospheric Models

Based on the single-scattering optical properties pre-computed with an improved geometric optics method, the bulk absorption coefficient, single-scattering albedo, and asymmetry factor of ice particles have been parameterized as a function of the effective particle size of a mixture of ice habits, the ice water amount, and spectral band. The parameterization has been applied to computing fluxes for sample clouds with various particle size distributions and assumed mixtures of particle habits. It is found that flux calculations are not overly sensitive to the assumed particle habits if the definition of the effective particle size is consistent with the particle habits that the parameterization is based. Otherwise, the error in the flux calculations could reach a magnitude unacceptable for climate studies. Different from many previous studies, the parameterization requires only an effective particle size representing all ice habits in a cloud layer, but not the effective size of individual ice habits.

Chou, Ming-Dah↗

NASA NTRSDate not supplied

TPSAS-NF1676L-10737-DND

The Clouds and the Earth's Radiant Energy System (CERES) project provides the community a quality climate TOA and surface fluxes and cloud properties and are key elements in evaluating the ability of climate models to predict both past and future climate states. One important aspect of successful climate monitoring is satellite calibration. The CERES instantaneous broadband calibration radiance stability is 0.1% per year, whereas the accuracy of the longwave (LW) and shortwave (SW) is better than 0.5% and 1% respectively. CERES uses the 3-hourly GEO fluxes and clouds to provide diurnally averaged daily and monthly TOA flux means from the CERES measurements onboard the Terra (10:30 AM local equator crossing time) and Aqua (13:30 PM) sun-synchronous satellites. The GEO radiances are calibrated against MODIS as a reference to provide consistent GEO retrieved cloud properties and derived broadband fluxes. These fluxes are then carefully normalized against the well-calibrated CERES fluxes to ensure climate quality fluxes, free of GEO artifacts. With the upcoming release of Edition3 products, CERES has just recalibrated all the CERES instruments to ensure that both Terra and Aqua fluxes are on the same radiometric scale and the removal of all known instrument trends. CERES will also recalibrate all GEO satellites using the entire GEO time record. CERES employs collocated, coincident ray-matched GEO/MODIS radiances as its primary technique, calibrating GEO radiances beginning in the year 2000. The advantage of the ray-matching technique is that it provides a full dynamic range of radiances to check the linearity of the GEO visible instrument. CERES uses deep convective clouds and invariant desert sites to validate the primary technique. All three methods can assess the stability of the GEO visible instrument. Examples of the CERES GEO calibration techniques and validation efforts will be shown at the conference. Special emphasis will be given to the newly incorporated desert site methodology.

R. Bhatt↗

DOE OSTI2025

Developing a Lagrangian Frame Transformation on Satellite Data to Study Cloud Microphysical Transitions in Arctic Marine Cold Air Outbreaks

Abstract Arctic marine cold air outbreaks (CAOs) generate distinct and dynamic cloud regimes due to intense air‐sea interactions. To understand the temporal evolution of CAO cloud properties and compare different CAO events, a Lagrangian perspective is particularly useful. We developed a novel technique that enables the conversion of inherently Eulerian satellite data into a Lagrangian framework, combining the broad spatiotemporal coverage of satellite observations with the advantages of Lagrangian tracking. This technique was applied to eight CAO cases associated with a recent field campaign. Our results reveal a striking contrast among the cases in terms of cloud‐top phase transitions, providing new insights into the evolution of CAO cloud properties.

Lagrangian analysis↗

NASA NTRS2014

Snowfall Rate Retrieval using NPP ATMS Passive Microwave Measurements

Passive microwave measurements at certain high frequencies are sensitive to the scattering effect of snow particles and can be utilized to retrieve snowfall properties. Some of the microwave sensors with snowfall sensitive channels are Advanced Microwave Sounding Unit (AMSU), Microwave Humidity Sounder (MHS) and Advance Technology Microwave Sounder (ATMS). ATMS is the follow‐on sensor to AMSU and MHS. Currently, an AMSU and MHS based land snowfall rate (SFR) product is running operationally at NOAA/NESDIS. Based on the AMSU/MHS SFR, an ATMS SFR algorithm has been developed recently. The algorithm performs retrieval in three steps: snowfall detection, retrieval of cloud properties, and estimation of snow particle terminal velocity and snowfall rate. The snowfall detection component utilizes principal component analysis and a logistic regression model. The model employs a combination of temperature and water vapor sounding channels to detect the scattering signal from falling snow and derive the probability of snowfall (Kongoli et al., 2014). In addition, a set of NWP model based filters is also employed to improve the accuracy of snowfall detection. Cloud properties are retrieved using an inversion method with an iteration algorithm and a two‐stream radiative transfer model (Yan et al., 2008). A method developed by Heymsfield and Westbrook (2010) is adopted to calculate snow particle terminal velocity. Finally, snowfall rate is computed by numerically solving a complex integral. The ATMS SFR product is validated against radar and gauge snowfall data and shows that the ATMS algorithm outperforms the AMSU/MHS SFR.

Meng, Huan↗

NASA NTRS2015

NPP ATMS Snowfall Rate Product

Passive microwave measurements at certain high frequencies are sensitive to the scattering effect of snow particles and can be utilized to retrieve snowfall properties. Some of the microwave sensors with snowfall sensitive channels are Advanced Microwave Sounding Unit (AMSU), Microwave Humidity Sounder (MHS) and Advance Technology Microwave Sounder (ATMS). ATMS is the follow‐on sensor to AMSU and MHS. Currently, an AMSU and MHS based land snowfall rate (SFR) product is running operationally at NOAA/NESDIS. Based on the AMSU/MHS SFR, an ATMS SFR algorithm has been developed recently. The algorithm performs retrieval in three steps: snowfall detection, retrieval of cloud properties, and estimation of snow particle terminal velocity and snowfall rate. The snowfall detection component utilizes principal component analysis and a logistic regression model. The model employs a combination of temperature and water vapor sounding channels to detect the scattering signal from falling snow and derive the probability of snowfall (Kongoli et al., 2015). In addition, a set of NWP model based filters is also employed to improve the accuracy of snowfall detection. Cloud properties are retrieved using an inversion method with an iteration algorithm and a two‐stream radiative transfer model (Yan et al., 2008). A method developed by Heymsfield and Westbrook (2010) is adopted to calculate snow particle terminal velocity. Finally, snowfall rate is computed by numerically solving a complex integral. NCEP CMORPH analysis has shown that integration of ATMS SFR has improved the performance of CMORPH‐Snow. The ATMS SFR product is also being assessed at several NWS Weather Forecast Offices for its usefulness in weather forecast.

Forecasting↗

NASA NTRS1990

The 27-28 October 1986 FIRE IFO cirrus case study - Cloud optical properties determined by High Spectral Resolution Lidar

The High Spectral Resolution Lidar (HSRL) was operated from a roof-top site in Madison, Wisconsin. The transmitter configuration used to acquire the case study data produces about 50 mW of ouput power and achieved eye-safe, direct optical depth, and backscatter cross section measurements with 10 min averaging times. A new continuously pumped, injection seeded, frequency doubled Nd:YAG laser transmitter reduces time-averaging constraints by a factor of about 10, while improving the aerosol-molecular signal separation capabilities and wavelength stability of the instrument. The cirrus cloud backscatter-phase functions have been determined for the October 27-28, 1986 segment of the HSRL FIRE dataset. Features exhibiting backscatter cross sections ranging over four orders of magnitude have been observed within this 33 h period. During this period, cirrus clouds were observed with optical thickness ranging from 0.01 to 1.4. The altitude relationship between cloud top and bottom boundaries and the optical center of the cloud is influenced by the type of formation observed.

Grund, C. J.↗

NASA NTRS1990

A GCM parameterization for the shortwave radiative properties of water clouds

A new parameterization was developed for predicting the shortwave radiative properties of water clouds, suitable for inclusion in general circulation models (GCMs). The parameterization makes use of the simple relationships found by Slingo and Schrecker, giving the three input parameters required to calculate the cloud radiative properties (the optical depth, single scatter albedo and asymmetry parameter) in terms of the liquid water path and equivalent radius of the drop size distribution. The input parameters are then used to derive the cloud radiative properties, using standard two-stream equations for a single layer. The relationships were originally derived for fairly narrow spectral bands but it was found that it is possible to average the coefficients so as to use a much smaller number of bands, without sacrificing accuracy in calculating the cloud radiative properties. This makes the parameterization fast enough to be included in GCMs. The parameterization was programmed into the radiation scheme used in the U.K. Meteorological Office GCM. This scheme and the 24 band Slingo/Schrecker scheme were compared with each other and with observations, using a variety of published datasets. There is good agreement between the two schemes for both cloud albedo and absorption, even when only four spectral bands are employed in the GCM.

Slingo, A.↗

DOE OSTI2024

Simulating Mixed‐Phase Open Cellular Clouds Observed During COMBLE: Evaluation of Parameterized Turbulence Closure

Marine cold-air outbreaks, or CAOs, are airmass transformations whereby relatively cold boundary layer (BL) air is transported over relatively warm water. To more deeply understand BL and mixed-phase cloud properties during CAO conditions, the Cold-Air Outbreaks in the Marine Boundary Layer Experiment (COMBLE) took place from late 2019 into early 2020. During COMBLE, the U.S. Department of Energy's first Atmospheric Radiation Measurement Mobile Facility (AMF1) was deployed to Andenes, Norway, far downstream (~1,000 km) from the Arctic pack ice. This study examines the two most intense CAOs sampled at the AMF1 site. The observed BL structures are open cellular with high (~3–5 km) and cold (–30 to –50 °C) cloud tops, and they often have pockets of high liquid water paths (LWPs; up to ~1,000 g m –2 ) associated with strong updrafts and enhanced turbulence. We use a high-resolution mesoscale model to explore how well four turbulence closure methods represent open cellular clouds. After applying a radar simulator to model outputs for direct evaluation, cloud top properties agree well with AMF1 observations (within ~10%), but radar reflectivity and LWP agreement is more variable. Results suggest that the turbulent Prandtl number may play an important role for the simulated BL and cloud properties. All simulations produce enhanced precipitation rates that are well-correlated with a cloud transition. Finally, the eddy-diffusivity/mass-flux approach produces the deepest cloud layer and therefore the largest and most coherent cellular structures. Furthermore, we recommend the use of a non-local turbulence closure approach to better capture turbulent processes in intense CAOs.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

Characterization of carbonaceous aerosols during TRACER-CAT

Absorbing aerosols (AA) have an important impact on the global radiation budget and cloud properties. The composition and properties of AA can vary substantially throughout the atmosphere, depending on the particle source and the influence of chemical aging. Uncertainties associated with the radiative effects of AA remain substantial. A key contributor to this uncertainty is understanding the extent to which coatings in general, and water uptake especially, alters absorption by AA particles and how this depends on particle composition. We deployed new and existing experimental tools during the Tracking Aerosol Convection Interactions Experiment (TRACER) campaign in Houston, TX as part of the Carbonaceous Aerosols Thrust (CAT) to provide detailed characterization of aerosol optical, chemical, and physical properties. Our TRACER-CAT measurements complemented and expanded on the planned TRACER instrumentation, allowing for more detailed characterization of aerosol properties of relevance to cloud development (a core focus of TRACER), such as the composition of particles that can act as cloud condensation nuclei, than would otherwise be available. Our measurements have allowed for assessment of the relationship(s) between AA optical properties (with a focus on absorption) and the chemical and physical characteristics (including the mixing state of black carbon (BC) containing particles). These field observations occurred in collaboration with Los Alamos National Laboratory in summer 2022 during the TRACER intensive operating period. The instrumentation we co-deployed provided for measurement of (i) multi-wavelength dry aerosol absorption, scattering, and extinction, (ii) the size-dependent composition and abundance of sub-micron aerosol, differentiating between those particles that do and do not contain BC, (iii) BC-specific concentrations and size distributions, (iv) particle size, and (v) the first field measurements at an ARM site of the influence of RH on multi-wavelength absorption by ambient AA. We have leveraged the natural variability of the atmosphere and of aerosol sources in the Houston region to (i) specifically disentangle contributions to light absorption from BC, absorbing organic carbon (brown carbon), and coatings on BC, (ii) characterize the mixing state of BC and assess the factors that give rise to compositional differences between BC-containing and BC-free aerosol, and (iii) establish how water uptake influences absorption and how any such effect depends on particle composition and BC mixing state. Overall, our study contributed to the mission of the Atmospheric System Research program in multiple ways. Through the deployment of complementary, advanced instrumentation for characterization of a wide range of aerosol properties our work helped to maximize the scientific impact of the TRACER campaign. Our work also allowed for development of new insights into the relationship(s) between aerosol composition, hygroscopicity, and the mixing state of BC with aerosol optical properties. Through this, our work has provided knowledge that can improve understanding and model representation of aerosol processes as they affect the Earth’s radiation budget.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2020

Uncertainties in CERES Top-of-Atmosphere Fluxes Caused by Changes in Accompanying Imager

The Clouds and the Earth’s Radiant Energy System (CERES) project provides observations of Earth’s radiation budget using measurements from CERES instruments on board the Terra, Aqua, Suomi National Polar-orbiting Partnership (S-NPP), and NOAA-20 satellites. The CERES top-of-atmosphere (TOA) fluxes are produced by converting radiance measurements using empirical angular distribution models, which are functions of cloud properties that are retrieved from imagers flying with the CERES instruments. As the objective is to create a long-term climate data record, not only calibration consistency of the six CERES instruments needs to be maintained for the entire time period, it is also important to maintain the consistency of other input data sets used to produce this climate data record. In this paper, we address aspects that could potentially affect the CERES TOA flux data quality. Discontinuities in imager calibration can affect cloud retrieval which can lead to erroneous flux trends. When imposing an artificial 0.6 per decade decreasing trend to cloud optical depth, which is similar to the trend difference between CERES Edition 2 and Edition 4 cloud retrievals, the decadal SW flux trend changed from −0.3 5 ± 0.18 Wm −2 to 0.61 ± 0.18 Wm −2 . This indicates that a 13% change in cloud optical depth results in about 1% change in the SW flux. Furthermore, different CERES instruments provide valid fluxes at different viewing zenith angle ranges, and including fluxes derived at the most oblique angels unique to S-NPP (>66 ∘ ) can lead to differences of 0.8 Wm −2 and 0.3 Wm −2 in global monthly mean instantaneous SW flux and LW flux. To ensure continuity, the viewing zenith angle ranges common to all CERES instruments (<66 ∘ ) are used to produce the long-term Earth’s radiation budget climate data record. The consistency of cloud properties retrieved from different imagers also needs to be maintained to ensure the TOA flux consistency.

Wenying Su↗

NASA NTRS2019

A Large Source of Cloud Condensation Nuclei from New Particle Formation in the Tropics

Cloud condensation nuclei (CCN) can affect cloud properties and therefore the Earth’s radiative balance. New particle formation (NPF) from condensable vapours in the free troposphere has been suggested to contribute to CCN, especially in remote, pristine atmospheric regions, but direct evidence is sparse, and the magnitude of this contribution is uncertain. Here we use in-situ aircraft measurements of vertical profiles of aerosol size distributions to present a global-scale survey of NPF occurrence. We observed intense NPF occurring at high altitude in tropical convective regions over both the Pacific and Atlantic Oceans. Together with the results of chemical-transport models, our findings indicate that NPF persists at all longitudes as a global-scale band in the tropical upper troposphere, covering about 40% of the Earth’s surface. Furthermore, we find that this NPF in the tropical upper troposphere is a globally important source of CCN in the lower troposphere, where they can affect cloud properties. Our findings suggest that the production of CCN, as these new particles descend towards the surface, is currently not adequately captured in global models, because they tend to underestimate both the magnitude of tropical upper tropospheric NPF and the subsequent growth to CCN sizes. This has potential implications for cloud albedo and the global radiative balance.

Atmospheric chemistry↗