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DOE OSTI2022

Subsurface Hydrogen and Natural Gas Storage (State of Knowledge and Research Recommendations Report)

Global efforts to decrease carbon dioxide (CO 2 ) emissions will result in increased reliance on renewable energy sources. One of the most significant obstacles to implementing this transition is the need for energy storage to compensate for varying, and sometimes intermittent, production rates and ever-increasing demand. An attractive solution is to use surplus energy to produce hydrogen gas (H 2 ), which can then be used to produce energy on demand without emitting CO 2 . This approach would require a vast H 2 network linking generators with consumers via transmission systems. Additionally, H 2 storage would be needed to support immediate needs, but larger storage reserves also will be required to ensure energy reliability and mitigate the impact of the mismatch between variable production rates and demand. Large-scale storage of H 2 may be achieved by using underground resources similar to how natural gas (NG) has been stored for the past century. While there is much experience in underground NG storage (UGS), significant technical challenges must be addressed to economically and safely store H 2 at the commercial scale. The purpose of this report is to assess the current state of knowledge and to identify technical research needs to facilitate deployment of large-scale underground hydrogen storage (UHS).

03 NATURAL GAS↗

DOE OSTI2020

Sensor Enabled Coatings for Methane Release Mitigation

Methane as a greenhouse gas is as much as 30 times more efficient than carbon dioxide. Given the increasing reliance on natural gas, methane release mitigation has become an increasingly important issue to address. In this investigation, PPG, RTI, and GTI focused on the exploration of resonant frequency identification (RFID) sensors embedded in natural gas pipeline coatings and their ability to detect coating damage at an early stage. Various coating formulations and their respective physical properties were examined to determine their effect on sensor performance in various accelerated aging environments. Overall, it was found that the RFID sensor responses could not be correlated to the coating properties and formulation variables examined in this investigation.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2022

SOFIA: Spectrometer Optimized for Facility Integrated Applications

Los Alamos National Laboratory researchers developed the Spectrometer Optimized for Facility Integrated Applications (SOFIA) for new capabilities in non-destructive nuclear material analysis, nuclear data measurements, and actinide science. SOFIA is the first ultra-high resolution gamma spectrometer technology based on low-temperature microcalorimeter designs. By precisely measuring the gamma rays passively emitted from radioactive and nuclear materials, SOFIA provides rapid, completely nondestructive analysis to improve the economics and timeliness of nuclear material analysis by reducing reliance on costly sampling and destructive analysis. By developing the first compact instrument based on ultrahigh resolution microcalorimeter gamma spectroscopy, the researchers intended to bring this technology into practical use in nuclear facilities and analytical laboratories.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2022

The Demand for a Domestic Offshore Wind Energy Supply Chain

In March of 2021, the Biden-Harris Administration established a National Offshore Wind Target to install 30 GW by 2030. This ambitious goal was not only intended to help reduce dependencies on fossil fuels, but also represents an opportunity to establish a new and sustainable industry in the United States. The announcement referenced the potential benefits of establishing a domestic supply chain, including the opportunity for existing suppliers to produce thousands of components while creating tens of thousands of jobs over the course of the decade. This vision by the Biden-Harris Administration aligns with the perspective of the offshore wind industry. At a Leadership 100 event hosted by the Business Network for Offshore wind in 2019, offshore wind developers and manufacturers identified the need for a roadmap outlining a pathway to a domestic supply chain as the top priority facing the industry. Building up domestic manufacturing capabilities will not only energize local industries but can potentially de-risk individual project by reducing reliance on importing resources from European or Asian markets. Although establishing a domestic supply chain will require significant investment, it has the potential to create substantial benefits throughout the industry and, by extension, on the decarbonization goals of the United States. This study characterizes the challenges and opportunities facing the growth of a domestic supply chain industry and evaluates the potential benefits that could be achieved through the creation of the supply chain. This report is the first of a two-part series which will describe the full supply chain roadmap and the associated benefits; the current report focuses on the high-level deployment, workforce, and component requirements that need to be met to achieve the National Offshore Wind Target. We will present: 1. A deployment pipeline that demonstrates the pathway to 30 GW, the associated demand for major fixed-bottom and floating offshore wind components (turbines, foundations, cables, substations), and the vessel and port requirements to support these installation activities. 2. A series of sensitivity analyses showing how the demand for components, ports, and vessels changes for different technology pathways and availability of the global supply chain. 3. An estimate of the total number of jobs that would be required to support these deployment scenarios under varying levels of assumed domestic content. 4. A comprehensive list of the Tier 1, 2, and 3 components (finished components, subassemblies, and subcomponents) required to construct fixed-bottom and floating offshore wind projects. 5. A discussion of critical path components that represent a significant challenge, bottleneck, or risk for a future domestic supply chain.

17 WIND ENERGY↗

DOE OSTI2022

Geothermal Energy and Resilience in Arctic Countries

The eight Arctic countries - Iceland, Canada, Denmark (Greenland and the Faroe Islands) Norway, Sweden, Finland, Russia, and the United States (Alaska) - have diverse energy systems, but can be split into two distinct groups based on energy characteristics. The first group includes systems in Europe (Finland, Norway, Sweden, and Iceland), which are heavily grid-connected. The second group includes the United States (Alaska), Canada, Russia, and Greenland, which have grid-connected energy systems in their more densely populated southern regions, but are also defined by the prevalence of remote microgrids. Energy sources for heat and power vary across grid-connected communities in the Arctic nations. The primary energy source for remote communities, on the other hand, is almost exclusively diesel. This is true for both heat and power. Despite these and other key distinctions, Arctic countries share many commonalities with regard to their energy systems. One is a fundamental need for heat. Heat and electric energy are linked in most communities - remote, rural, and urban - and those linked systems are increasingly vulnerable to disruptions. Several of the Arctic countries use baseload renewable energy resources for heat and power. Iceland uses geothermal and hydroelectric; Canada, the United States, Sweden, Norway, and Finland use hydroelectric. Utilization of baseload renewable energy resources on-site for combined heat and power appears to enhance the resilience of communities in Arctic countries with high penetration of those resources. On the other hand, reliance on diesel by remote communities in other Arctic countries may be amplifying vulnerabilities. Although geothermal energy is currently used in all eight Arctic countries, resources are poorly mapped, and details can be difficult to come by. Despite this, geothermal energy provides heat and sometimes electricity at both utility scales and at the microgrid scale. Geothermal electricity is produced in Iceland, Russia, and the United States (Alaska). Direct use of geothermal heat is used in Iceland, Russia, United States, Canada, and Norway. Geo-exchange is used in Sweden, Finland, Norway, Canada, and the United States. In this paper, we reframe geothermal heat and power systems as integrated energy systems, asking the question: are integrated geothermal energy systems - where available and economic - resilient solutions for communities in Arctic countries? We identify resilience attributes of integrated geothermal energy systems, with a focus on microgrids and small-scale applications. Based on the high-level, qualitative analysis presented in this paper, the answer appears to be yes. Further work should prioritize refining our understanding of geothermal resources in Arctic countries, because development of the most economic geothermal resources in Arctic countries has the potential to enhance the energy resilience of its residents, whether in a grid-connected or remote off-grid context.

15 GEOTHERMAL ENERGY↗

DOE OSTI2022

Fine Gradient Electrode and Micro Porous Layer Structures for Improved Heavy Duty Fuel Cells (Final Report)

The commercial deployment of Heavy Duty Fuel Cells(HDFC) for applications such as large trucks (for example, Class 8 capable of carrying 50,000 lb. loads) depends vitally on achieving high efficiency and durability at reasonable costs. Furthermore, the HDFC must operate under practical conditions such as with fuel and air impurities, multiple stop-start cycles, and under the extremes of climate our planet offers – from hot and cold to dry and wet. These conditions place a premium on the stability and utilization of the materials comprising the membrane electrode assemblies (MEAs) powering the fuel cell. and the current catalysts, MicroPorous Layers, and Electrode structures and additives are insufficient for these needs. In Phase I Pajarito and Advent will develop durable electrocatalysts, MicroPorous Layer and electrode additives, and electrode structures for heavy duty fuel cells designed for zero-emission long-haul trucking. The electrocatalyst products are designed to solve the challenging durability and performance needs of fuel cells designed for long life and high efficiency through a combination of uniquely structured designed catalysts as well as new MicroPorous Layers (MPLs) and electrode structure additives. These improved materials will provide Pajarito both an expanded commercial opportunity in electrocatalysts, as well as new markets for MPL and electrode additives. The resulting public benefits include improved economics of fuel cells, a leading zero-emission technology for mobility, as well as reduced reliance on the critical minerals and metals used in the heavy-duty trucks industry. Possible follow-up Phase II and III projects would add full MEA products based on the Phase I efforts catalysts and additives, with full system validation by leading Fuel Cell Truck developers.

08 HYDROGEN↗

DOE OSTI2021

Codes and Standards Assessment for Hydrogen Blends into the Natural Gas Infrastructure

Energy utilities are evaluating emerging energy technologies to reduce reliance on carbon as an energy carrier. Hydrogen has been identified as a potential substitute for carbon-based fuels that can be blended into other gaseous energy carriers, such as natural gas. However, hydrogen blending into natural gas has important implications on safety which need to be evaluated. Designers and installers of systems that utilize hydrogen gas blending into natural gas distribution systems need to adhere to local building codes and engage with the authority having jurisdiction (AHJ) for safety and permitting approvals. These codes and standards must be considered to understand where safety gaps might be apparent when injecting hydrogen into the natural gas infrastructure. This report generates a list of relevant codes and standards for hydrogen blending on existing, upgraded, or new pipelines. Additionally, a preliminary assessment was made to identify the codes and standards that need to be modified to enable this technology as well as potential gaps due to the unique nature and safety concerns of gaseous hydrogen.

03 NATURAL GAS↗

DOE OSTI2022

Electric Vehicle and Infrastructure Systems Modeling in Washington D.C. and Baltimore

This report documents the Argonne-Exelon effort to develop and utilize an agent-based model (ATEAM) of charging demand and infrastructure expansion applicable to the Washington, DC–Baltimore, MD consolidated metropolitan area. This study extends the ATEAM model time horizon to 10 years (from 2020 to 2030), expands agent behavior modeling capabilities, incorporates more granular and extensive empirical data on charging behavior, and analyzes charging needs for a much larger population of PEVs, in keeping with regional goals for significant adoption of ZEVs. With given targets for annual BEV adoption, five scenarios were developed to examine public infrastructure needs and resulting charging load, considering different home charging availabilities, as well as different PEV consumer profiles and public charging infrastructure deployment strategies. Scenario results show that if new chargers (both L2 and DCFC) are spread more widely (as with ubiquitous deployment strategies), there will be less variation in the number of chargers added to each census tract in the study area. More importantly, widespread public charging infrastructure with ubiquitous deployment strategies reduces unmet charging demand and improves charging success, even with heavy reliance on public charging. About 80 percent of BEV drivers can charge on their first attempt in scenarios with ubiquitous deployment strategies. Moreover, widespread public charging infrastructure better meets the demand for more charging, and in return, increases BEV adoption. Low home charging availability produces higher charging loads in public locations, especially during the early morning (around 8:00 a.m.) and late afternoon (around 6:00 p.m.). The evening peak load indicates that drivers are taking advantage of public charging before heading home. Study results also indicate that even with 20 percent home charging availability in 2030, just 20 percent of drivers attempt to charge on a given day. With their relatively high electric range (200+ miles), the BEVs expected to be on the road in 2030 can handle daily commutes without re-charging for a couple of days.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2021

Dual Purpose Canister Reactivity and Groundwater Absorption Analyses (Rev. 7)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2022

Risk-Informed Initiating Events and Accident Response

Emerging nuclear technologies and advanced reactor developments have brought proposed changes to the regulatory framework which can be leveraged to improve safety implementation and regulatory oversight processes at existing operating nuclear power plants. Specifically, opportunities exist to make plants’ regulatory compliance processes more efficient. This can be done by decreasing reliance on purely deterministic and prescriptive approaches and expansion of the use of risk informed and performance-based approaches to demonstrate reactor safety while achieving economic gains and efficiencies. In this report, we researched possibilities of economic benefits potentially available from the application of concepts associated with a modernized regulatory framework developed for advanced reactors to the existing light water reactors. We used timing factors to demonstrate the complexity of the existing risk assessments and described how these complexities affect regulatory compliance activities at the plants. We also investigated regulatory framework for both existing and new reactors and provided an overview of potential improvements. Lastly, we evaluated various areas of existing plant operations where modernization of compliance activities can offer substantial benefits.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2022

Compensation for Long-Duration Energy Storage

Rapidly changing power system conditions, driven by decarbonization goals, are leading to significant growth in renewable energy sources, which can be both variable and uncertain. This has been accompanied with increased reliance on and rapid growth in deployment of energy storage technologies. Currently, approximately 90% of installed, utility-scale energy storage capacity in the United States comes from pumped storage hydropower (PSH). However, development of new PSH has been limited and all recent growth in energy storage has come from batteries, , especially as technology costs have decreased over the years. Most of the current deployment still remains in the form of short-duration (<6 hours) energy storage technologies; the average duration of new storage was 3.7 hours for projects deployed in the first half of 2021 (Wood Mackenzie and Energy Storage Association 2021).

25 ENERGY STORAGE↗

DOE OSTI2022

Dual Purpose Canister Reactivity and Groundwater Absorption Analyses

The current spent nuclear fuel (SNF) management strategy includes reliance on dry storage. Utilities are meeting their interim storage needs on an individual basis with use of large-capacity dry storage casks, with a current focus on meeting existing storage and transportation requirements, as disposal requirements are not currently available. These casks are commonly known as dual-purpose (i.e., storage and transportation) canisters (DPCs). However, a small percentage of single-purpose (storage only) systems is also being used to meet storage needs. These are included under the “DPC” heading. This report investigates the postclosure criticality safety aspects of DPCs. Placing large, heavy waste packages containing DPCs into a repository for direct disposal has not yet been implemented domestically or internationally. Therefore, direct disposal of DPCs represents new engineering and scientific challenges. Some of the engineering challenges that have already been addressed include handling and placement, use of ramps vs. shafts, use of hoists, use of transport equipment, and thermal management. Additionally, some studies have been conducted in the past regarding the feasibility of direct disposal from a criticality analysis perspective and have concluded that while possible, demonstrating subcriticality over the disposal time period is a challenge. The alternative to direct disposal of DPCs into a repository is to repackage the SNF into different canisters. The direct disposal of DPCs without cutting them open and repackaging is appealing because it could be more cost-effective, reduce the complexity of fuel management operations both in and outside reactor facilities, and result in less cumulative worker dose during interim storage and handling before eventual disposal in a deep geologic repository.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2023

Fort Erie On-Demand Transit Case Study

Rural and smaller-sized communities in North America face unique mobility challenges due to their low population density, lower public transit spending per capita compared to major cities, and a high reliance on private vehicles. In recent years, communities such as Fort Erie, Ontario have restructured or advanced their public transit systems using on-demand services. Fort Erie is a relatively sparsely populated region of 32,901 residents, spread across a land area of 166 square kilometers (64 square miles), for an average population density of 193 residents per square kilometer (500 per square mile). In October 2021, the town implemented a mobility-on-demand system integrated with smartphone software to replace its fixed-route community bus system, which consisted of four buses with three routes, each with a roughly one-hour, one way loop. The new service utilizes a fleet of six minivans, two of which are retrofitted with wheelchair-accessible ramps. The system may require that a passenger requesting a standard van walk up to 400 meters (a quarter mile) to their pickup location to optimize vehicle routing while providing origin-to-destination service. The on-demand system proved effective in providing service, eclipsing pre-pandemic ridership by 40%, decreasing greenhouse gas emissions per ride by 63%, and decreasing the cost per ride to the town by 29%. This report documents both the previous system and the new system in terms of routes, ridership, costs, fuel, and other notable system parameters. This work is part of an ongoing series of case studies on providing small communities with on-demand, right-sized vehicle service coupled with a smartphone application.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

DOE OSTI2022

A Comprehensive Economic Coal Transition in South Asia

Many countries are considering accelerating their coal transition. A coal transition refers to an energy sector’s shift from a reliance on coal toward an energy mix largely based on cleaner fuels and renewable energy sources. Such a transition is not just related to greenhouse gas emissions, but also encompasses a range of benefits, recognizing that global energy costs and options are changing. Since 2015, proposed new coal power capacity has dropped by three-quarters globally, leaving only a few countries that develop coal-fired power plants at scale (Littlecott et al., 2021). Historic steps were taken at the United Nations Climate Change 26th Conference of Parties (COP26) in Glasgow, as countries pledged to stop new coal builds, end international coal financing, phase down and phase out unabated coal use, and transition to clean energy. In South Asia, there have been several indicators suggesting that countries may be open to moving toward a coal transition. For example, the number of coal power plants under development across South Asia has decreased by 87% since 2015 (Littlecott et al., 2021). However, the challenges of assuring a just transition are substantial. Because coal plays a critical role in the energy and economic systems in South Asia, especially India, moving away from coal means realizing a broader country-wide economic and social transition. A comprehensive, integrated transition strategy for each state is thus needed urgently. This report briefly reviews the current trends and policies on coal in South Asian countries, develops a framework for a comprehensive economic coal transition, and assesses the opportunities and challenges of the transition in key countries. Several important findings emerge from the analysis. First, a coal transition can support overall economic growth and stability. Financial advantages to a well-planned coal transition include mitigating the risk of stranded assets and taking advantage of low-cost renewables. As a global coal transition proceeds, funds are being diverted from new unabated coal power plants, and utilization rates are declining. The likelihood that coal assets will become stranded is increasing, and the potential for future losses therefore increases as well. Second, coal imports in South Asia are rising. Of the coal consumed in Bangladesh, India, Nepal, and Sri Lanka, 32% is imported; this number increases to 94% when excluding India (International Energy Agency [IEA], 2021d). This illustrates a serious energy security risk. One example is the recent increase in coal prices in South Asia, to be discussed in Section 2.2.1. A diverse energy portfolio that incorporates local renewable energy can provide resilience in the face of changing commodity prices and availability. Third, the social benefits of a coal transition include positive health impacts and broader economic improvements in job creation, although assuring a just transition may be a challenge. Phasing out or phasing down coal can significantly reduce air pollutant emissions and therefore minimize associated premature mortality and improve life expectancy. Additional societal benefits of a coal transition include the high economy-wide potential for job creation, although it creates challenges in terms of reintegration and resettlement for coal miners and their communities.

01 COAL, LIGNITE, AND PEAT↗

DOE OSTI2023

Understanding and Predictability of Integrated Mountain Hydroclimate (Workshop Report)

Mountainous systems cover approximately 23% of Earth’s land and are distributed across all continents. They can capture and store atmospheric moisture that is then cycled through the terrestrial surface and subsurface system, released to downstream communities, and cycled back to the atmosphere. Mountain hydroclimate—characterized by steep gradients, geological, ecological, and biogeochemical diversity—is influenced by topographic forcing and elevated warming and susceptible to large subseasonal to multidecadal variability and rapid changes. Terrestrial hydrological and biogeochemical cycles also experience cascading effects from global warming impacts, such as multidecadal declines in mountain snowpack, longer growing seasons, and increased frequency and severity of extreme events like droughts and wildfires. However, little is known about the effects of these impacts and their feedbacks on climate systems and surface-subsurface compartments. Also unknown are the full implications of changing hydroclimate and extreme events on hydro biogeochemical cycles across atmosphere, terrestrial, and human systems in mountain regions and beyond. This knowledge gap is critical, given human reliance on mountain systems for stable water supply and quality. Mountain systems’ increasing vulnerability to climate change and human perturbations motivates the need to improve understanding of integrated mountain hydroclimate (IMHC) systems and their feedbacks and impacts on humans across scales. However, due to large heterogeneity and strong gradients, coupled natural-human processes in mountain regions present significant challenges for observations, modeling, predictions, and projections. Motivated by gaps in mountain hydroclimate understanding, observations, and modeling and the need for credible projections of future changes, the U.S. Department of Energy’s (DOE) Biological and Environmental Research (BER) program organized a virtual workshop on “Understanding and Predictability of Integrated Mountain Hydroclimate.” Sponsored by BER’s Earth and Environmental Systems Sciences Division (EESSD), the workshop aimed to inform and catalyze EESSD’s growing interests in enhancing predictive understanding of IMHC. Organizers structured the workshop to identify (1) knowledge gaps, (2) observational and modeling challenges, (3) short-term (1 to 3 years) and long-term (10 years and beyond) research opportunities, and (4) strategies for fostering collaboration and coordination. To address the outstanding challenges of IMHC, the workshop included two sessions organized by disciplinary, cross-disciplinary, and crosscutting science topics. The disciplinary and cross-disciplinary topics focused on essential IMHC elements: atmosphere, terrestrial, and human systems and their interactions. Breakout sessions on disciplinary and cross-disciplinary topics facilitated identification of crosscutting topics and central emerging themes. Session 1 focused on connecting existing DOE investments to accelerate progress related to scientific challenges in understanding mountain hydroclimate. In Session 2, participants further explored key Session 1 takeaways through the lens of multiagency collaborations and coordination.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2023

Multi-Sourced Collaboration for the Production and Refining of Rare Elements and Critical Metals (Final Technical Report)

The project objective was to develop a feasible and cost-effective method for recovering rare earth elements (REEs) and critical materials (CMs) from coal and coal byproducts, resulting in high-purity individually separated REEs and CMs. The targeted REEs included Y, Pr, Nd, Gd, Dy, and Sm, with a purity of over 99.5%, while the CMs included Co, Mn, Ga, Sr, Li, Ni, Zn, and Ge, with a purity of over 90%. The project aimed to design a prototype facility capable of producing 1-3 tonnes/day of high-purity REO mixes. The work was divided into four designated circuits: 1) REE extraction and concentration, 2) REE separation and purification, 3) RE metal production, and 4) CM production. To achieve these goals, the project involved 11 tasks, including technology reviews, research, process flow diagram development, mass balance estimation, and preliminary technical-economic analysis. The project team included researchers from the University of Kentucky, University of Alabama and Virginia Tech as well as process specialists from Argonne National Laboratory. MP Materials provided technical support regarding rare earth markets and processing while Alliance Coal performed resource assessment. The project included a market analysis for Nd/Pr, Tb, Dy, Gd, Y, Co, Mn, Li, Sr, Ga, Ni, Zn, and Ge. These analyses provided insights into the supply and demand trends as well as historic and future projections of market price relative to purity requirements for these elements. Two coal resources were selected for the project: the West Kentucky No. 13 (Baker) Seam and an undisclosed lignite resource in the Illinois coal basin. The estimated quantities of REEs in these resources were calculated based on production samples and drilling data. It was estimated that there is adequate supply for an operation producing one metric ton daily of higher purity mixed rare earth oxides (MREO) for approximately 20 years at a site located in western Kentucky. In Circuit 1, project data was obtained from a pilot heap leach and REE concentration facility. It was concluded that the existing circuit, which generated a MREO concentrate, two types of CM mixed products, and Li- and Sr-containing waters, would be suitable feed for circuits 2-4. Data from the first-of-its-kind coal coarse refuse heap leach pilot pad played a crucial role in estimating reliable elemental concentrations of the pregnant leaching solution (PLS). The average total REE concentration in the PLS was found to be 28.6 ppm. In Circuit 2, several concepts were explored including a novel process referred to as solvent-assisted chromatography (SAC). This concept involved a novel columnar reactor that incorporated multiple mixer/settlers, thereby enabling the operation of counter-flowing aqueous and organic phases. Unfortunately, due to project time constraints, a complete fundamental modeling analysis could not be completed to fully evaluate the technology. Molten salt electrowinning was considered as an alternative for circuit 3 following circuit 2 purification circuit utilizing the novel SAC process. A mass and energy balance of Nd reduction to metal in a fluoride containing molten salt electrolyte was conducted. Comparisons were made with the current state of Asian molten salt electrorefining, and potential improvements in siphoning rare earth metals (REM) from the reactor were presented. A cost estimate was performed for the production of 1 tonne per day, which yielded a total of $2.29 million for the nine electrowinning (EW) cells required. The selected option for circuits 2 and 3 was a plasma distillation process, which initially separates rare earth elements (REEs) from other elements. This is followed by selective electrowinning in various ionic liquids. The selection was made on the basis of thermodynamic modeling and experimental data previously published by a project partner. The combination offers an innovative approach to integrated refining and RE metal production. For Circuit 4, an extensive literature review was conducted for the processing of the CMs. The ultimate decision was to utilize a combined plasma and ionic liquid process as well to produce individual high-purity concentrates of Zn, Ni, Co, Mn, and Mg. A separate flowsheet for Li and Sr was recommended, which would yield carbonates of these elements. Due to the lack of suitable experimental data at this time, a process recommendation could not be provided but several methods have been proposed for consideration. Lastly, a techno-economic analysis (TEA) was conducted to assess the effectiveness of the proposed process for further investigation. The TEA results revealed a capital expense (CapEx) of $737 million and an annual operational expense (OpEx) of $220 million. Due to the selected elements, the hypothetical heap leach pad can produce 1 metric tonne per day of REO equivalent, but a conscious decision was made to only treat targeted REEs, resulting in the production of 0.4 metric tonne of REM. An estimated annual revenue of $90.87 million was projected based on standard market pricing information provided by the funding agency. During the TEA, ten different modules were evaluated for costing purposes. The precipitation circuit was identified as the largest single operational expense, followed by the Mg/Mn process due to the amount of treated metal. In terms of capital expenditures, the heap leach process incurred the highest cost, followed by the Mg/Mn process. The scalability of the plasma process is a crucial consideration since the reactors cannot be scaled beyond the largest demonstrated size due to their reliance on surface area of the slag and vapor phase. The purity estimate for the REEs are generally 98%±2% to produce a metal. The purity level being lower than the project objective was due to the lack of specific experimental data needed to tighten the tolerance of the estimates. Based on literature and previous experience, the CMs are estimated as follows; Ga (95%+, metal), Sr (95%+, carbonate), Li (95%+, carbonate), Ni (98%±2%, metal), Zn (95%+, metal sponge), Ge (95%+, metal), Co (98%±2%, metal), and Mn (98%±2%, metal).

01 COAL, LIGNITE, AND PEAT↗

DOE OSTI2022

Valuing Resilience for Microgrids: Challenges, Innovative Approaches, and State Needs

The United States depends on the delivery of reliable, affordable, clean, and safe electricity. Electric utilities invest billions of dollars each year in generation, transmission, and distribution assets to meet this need. However, experiences with recent natural disasters of increasing frequency and duration demonstrate the shortcomings of this approach in the face of modern threats. Further, as customers rely on electricity for a broader range of important needs, such as transportation, as well as critical life-saving services and mission critical facilities such as water treatment, medical care, shelters, telecommunications, and more, the need to minimize the likelihood and impacts of outages grows. Against this backdrop, resilience has emerged as a key consideration to guide electricity spending, whether from utilities, customers, or taxpayers. Although reliability has been defined and measured for decades with broadly accepted metrics that measure how many customers lose power and at what frequency and duration, resilience considers the electricity system’s response to a disruption and its subsequent impacts on customers. Developing tools and methods to accurately assess the costs and benefits of resilience investments is a critical step toward the goal of mitigating the impacts of outages on customers and society. Today, electric system resilience is largely treated as an externality due to challenges estimating the costs of long-duration outages, impacts of outages on society, and increasing reliance on electricity for a growing set of interdependent services. These interdependencies include the water, wastewater, telecommunications, natural gas, and health sectors. Without knowing how much a given resilience investment will benefit customers or society more broadly, investors, policymakers, and regulators are less likely to make or approve such investments, and less able to prioritize those investments. State Energy Offices and public utility commissions (PUCs) lead the development of state-level energy policy and utility regulation, respectively, and each has interests in encouraging appropriate public and private investments in resilience. To this end, the National Association of State Energy Officials (NASEO) and National Association of Regulatory Utility Commissioners (NARUC), with the support of the U.S. Department of Energy (DOE) Office of Electricity (OE), formed a joint Microgrids State Working Group to explore the costs and benefits of microgrids, barriers to broader deployment of microgrids to meet resilience and other objectives, and policy and regulatory strategies to optimize investments in resilience, including but not limited to microgrids. Although no universally accepted valuation tool for resilience exists, National Laboratories, utilities, researchers, and state and federal agencies have collaborated to develop, apply, and improve a number of approaches to quantify resilience, several of which are still in progress at the time this report is published. This report seeks to share these important advances by discussing current definitions of resilience (Section 1), how microgrids are defined and used to meet resilience objectives (Section 2), new approaches to valuing resilience (Section 3), steps State Energy Offices and PUCs have taken to further resilience valuation efforts (Section 4), and finally, considerations and suggested next steps for State Energy Offices and PUCs (Section 5). Relevant examples of specific microgrid projects and resilience valuation efforts are included throughout the report. While this report is written specifically for NASEO and NARUC members, it may be useful for utilities, local governments, and individual customers interested in improving the way public and private dollars are spent to achieve resilience outcomes.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2023

A Fission-like Neutron Spectrum Shaping Assembly based on D-T Generator

For nearly five decades, 252 Cf sources have been used for testing and calibration over a wide range of neutron detection devices used for nuclear safety and radiation protection. However, the vastly increased cost of 252 Cf sources, its short half-life, and concerns about future shortage have prompted nuclear facilities and radiological calibration laboratories that rely on high-intensity neutron sources to seek alternatives. While there appear to be no other radionuclide neutron sources that would match the 252 Cf performance characteristics, all of them, including 252 Cf, present similar concerns in terms of hazards, safety, and security. As a possible solution to this issue, the Pacific Northwest National Laboratory (PNNL) developed a low-risk, cost-efficient alternative to produce fission-like spectra based on commercially available deuterium-tritium (D-T) neutron generators. The alternative of producing a fission-like neutron spectrum without any fissionable materials or beryllium would enable the nuclear facilities across the entire complex to eliminate their reliance on high intensity 252 Cf sources for nuclear safety and radiation protection applications, substantially reducing risks and associated costs. This report describes efforts of designing the spectrum shaping assembly, its construction and characterization of the neutron field produced. Performance of this newly developed D-T generator based neutron field is demonstrated via calibration of a criticality detector, neutron survey instruments, and personal dosimeters verified against current standardized fields produced by 252 Cf spontaneous fission sources.

42 ENGINEERING↗