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DOE OSTI2024

Understanding aerosol–cloud interactions using a single-column model for a cold-air outbreak case during the ACTIVATE campaign

Marine boundary layer clouds play a critical role in Earth's energy balance. Their microphysical and radiative properties are highly impacted by ambient aerosols and dynamic forcings. In this study, we evaluate the representation of these clouds and related aerosol–cloud interaction processes in the single-column version of the E3SM climate model (SCM) against field measurements collected during the NASA ACTIVATE campaign over the western North Atlantic, as well as intercompare results with high-resolution process level models. We show that E3SM SCM reproduces the macrophysical properties of post-frontal boundary layer clouds in a cold-air outbreak (CAO) case well. However, it generates fewer but larger cloud droplets compared to aircraft measurements. Further sensitivity tests show that the underestimation of both aerosol number concentration and vertical velocity variance contributes to this bias. Aerosol–cloud interactions are examined by perturbing prescribed aerosol properties in E3SM SCM with fixed dynamics. Higher aerosol number concentration or hygroscopicity leads to more numerous but smaller cloud droplets, resulting in a stronger cooling via shortwave cloud forcing. This apparent Twomey effect is consistent with prior climate model studies. The cloud liquid water path shows a weakly positive relation with cloud droplet number concentration due to precipitation suppression. This weak aerosol effect on cloud macrophysics may be attributed to the dominant impact of strong dynamical forcing associated with the CAO. Our findings indicate that the SCM framework is a key tool to bridge the gap between climate models, process level models, and field observations to facilitate process level understanding.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2006

Model Intercomparison of Indirect Aerosol Effects

Modeled differences in predicted effects are increasingly used to help quantify the uncertainty of these effects. Here, we examine modeled differences in the aerosol indirect effect in a series of experiments that help to quantify how and why model-predicted aerosol indirect forcing varies between models. The experiments start with an experiment in which aerosol concentrations, the parameterization of droplet concentrations and the autoconversion scheme are all specified and end with an experiment that examines the predicted aerosol indirect forcing when only aerosol sources are specified. Although there are large differences in the predicted liquid water path among the models, the predicted aerosol first indirect effect for the first experiment is rather similar, about -0.6 W/sq m to -0.7 W/sq m. Changes to the autoconversion scheme can lead to large changes in the liquid water path of the models and to the response of the liquid water path to changes in aerosols. Adding an autoconversion scheme that depends on the droplet concentration caused a larger (negative) change in net outgoing shortwave radiation compared to the 1st indirect effect, and the increase varied from only 22% to more than a factor of three. The change in net shortwave forcing in the models due to varying the autoconversion scheme depends on the liquid water content of the clouds as well as their predicted droplet concentrations, and both increases and decreases in the net shortwave forcing can occur when autoconversion schemes are changed. The parameterization of cloud fraction within models is not sensitive to the aerosol concentration, and, therefore, the response of the modeled cloud fraction within the present models appears to be smaller than that which would be associated with model "noise". The prediction of aerosol concentrations, given a fixed set of sources, leads to some of the largest differences in the predicted aerosol indirect radiative forcing among the models, with values of cloud forcing ranging from -0.3 W/sq m to -1.4W/sq m. Thus, this aspect of modeling requires significant improvement in order to improve the prediction of aerosol indirect effects.

Penner, J. E.↗

NASA NTRS1996

Study of the Radiative Properties of Inhomogeneous Stratocumulus Clouds

Clouds play an important role in the radiation budget of the atmosphere. A good understanding of how clouds interact with solar radiation is necessary when considering their effects in both general circulation models and climate models. This study examined the radiative properties of clouds in both an inhomogeneous cloud system, and a simplified cloud system through the use of a Monte Carlo model. The purpose was to become more familiar with the radiative properties of clouds, especially absorption, and to investigate the excess absorption of solar radiation from observations over that calculated from theory. The first cloud system indicated that the absorptance actually decreased as the cloud's inhomogeneity increased, and that cloud forcing does not indicate any changes. The simplified cloud system looked at two different cases of absorption of solar radiation in the cloud. The absorptances calculated from the Monte Carlo is compared to a correction method for calculating absorptances and found that the method can over or underestimate absorptances at cloud edges. Also the cloud edge effects due to solar radiation points to a possibility of overestimating the retrieved optical depth at the edge, and indicates a possible way to correct for it. The effective cloud fraction (Ne) for a long time has been calculated from a cloud's reflectance. From the reflectance it has been observed that the N, for most cloud geometries is greater than the actual cloud fraction (Nc) making a cloud appear wider than it is optically. Recent studies we have performed used a Monte Carlo model to calculate the N, of a cloud using not only the reflectance but also the absorptance. The derived Ne's from the absorptance in some of the Monte Carlo runs did not give the same results as derived from the reflectance. This study also examined the inhomogeneity of clouds to find a relationship between larger and smaller scales, or wavelengths, of the cloud. Both Fourier transforms and wavelet transforms were used to analyze the liquid water content of marine stratocumulus clouds taken during the ASTEX project. From the analysis it was found that the energy in the cloud is not uniformly distributed but is greater at the larger scales than at the smaller scales. This was determined by examining the slope of the power spectrum, and by comparing the variability at two scales from a wavelet analysis.

Batey, Michael↗

NASA NTRS2006

Atmospheric Teleconnection over Eurasia Induced by Aerosol Radiative Forcing during Boreal Spring

The direct effects of aerosols on global and regional climate during boreal spring are investigated based on numerical simulations with the NASA Global Modeling and Assimilation Office finite-volume general circulation model (fvGCM) with Microphyics of Clouds with the Relaxed Arakawa Schubert Scheme (McRAS), using aerosol forcing functions derived from the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The authors find that anomalous atmospheric heat sources induced by absorbing aerosols (dust and black carbon) excite a planetary-scale teleconnection pattern in sea level pressure, temperature, and geopotential height spanning North Africa through Eurasia to the North Pacific. Surface cooling due to direct effects of aerosols is found in the vicinity and downstream of the aerosol source regions, that is, South Asia, East Asia, and northern and western Africa. Significant atmospheric heating is found in regions with large loading of dust (over northern Africa and the Middle East) and black carbon (over Southeast Asia). Paradoxically, the most pronounced feature in aerosol-induced surface temperature is an east west dipole anomaly with strong cooling over the Caspian Sea and warming over central and northeastern Asia, where aerosol concentrations are low. Analyses of circulation anomalies show that the dipole anomaly is a part of an atmospheric teleconnection pattern driven by atmospheric heating anomalies induced by absorbing aerosols in the source regions, but the influence was conveyed globally through barotropic energy dispersion and sustained by feedback processes associated with the regional circulations. The surface temperature signature associated with the aerosol-induced teleconnection bears striking resemblance to the spatial pattern of observed long-term trend in surface temperature over Eurasia. Additionally, the boreal spring wave train pattern is similar to that reported by Fukutomi et al. associated with the boreal summer precipitation seesaw between eastern and western Siberia. The results of this study raise the possibility that global aerosol forcing during boreal spring may play an important role in spawning atmospheric teleconnections that affect regional and global climates.

Kim, Maeng-Ki↗

NASA NTRS2024

Substantial Cooling Effect From Aerosol-Induced Increase in Tropical Marine Cloud Cover

With global warming currently standing at approximately +1.2 °C since preindustrial times, climate change is a pressing global issue. Marine cloud brightening is one proposed method to tackle warming through injecting aerosols into marine clouds to enhance their reflectivity and thereby planetary albedo. However, because it is unclear how aerosols influence clouds, especially cloud cover, both climate projections and the effectiveness of marine cloud brightening remain uncertain. Here, we use satellite observations of volcanic eruptions in Hawaii to quantify the aerosol fingerprint on tropical marine clouds. We observe a large enhancement in reflected sunlight, mainly due to an aerosol-induced increase in cloud cover. This observed strong negative aerosol forcing suggests that the current level of global warming is driven by a weaker net radiative forcing than previously thought, arising from the competing effects of greenhouse gases and aerosols. This implies a greater sensitivity of Earth’s climate to radiative forcing and therefore a larger warming response to both rising greenhouse gas concentrations and reductions in atmospheric aerosols due to air quality measures. However, our findings also indicate that mitigation of global warming via marine cloud brightening is plausible and is most effective in humid and stable conditions in the tropics where solar radiation is strong.

Atmospheric science↗

NASA NTRS2004

Clouds and Aerosols in the Climate System

Remote sensing of cloud and aerosol properties from space is reviewed for present and planned international satellite sensors. Techniques that are being used to enhance our ability to characterize the global distribution of cloud and aerosol properties include well-calibrated multispectral radiometers that rely on visible, near-infrared, and thermal infrared channels, sometimes including polarization as well. The availability of thermal channels to aid in cloud screening for aerosol properties is an important additional piece of information that has not always been incorporated into sensor designs. In this paper, we describe the radiative properties of clouds as currently determined from satellites (cloud fraction, optical thickness, cloud top pressure, and cloud effective radius), and highlight the global and regional cloud microphysical properties currently available for assessing climate variability and forcing. In addition, we will frustrate the radiative and microphysical properties of aerosol particles that are currently available from space-based observations, as well as enhancements to aerosol remote sensing over bright-reflecting surfaces that is anticipated in the next couple of years. Finally, we will describe the aerosol optical and radiative properties available from the globally distributed AERONET network of ground-based sun-sky radiometers.

King, Michael D.↗

DOE OSTI2026

Substantial Diel Changes of Cloud Adjustments to Aerosols in Ship‐Tracks

Clouds adjust their albedo, amount and liquid water path to anthropogenic aerosols, and produce a climate forcing. Such cloud adjustments are complex functions of both environmental conditions and interaction time. However, direct observations of temporal changes in cloud adjustments are limited. Here, we develop a method to show observational evidence of substantial diel changes in cloud adjustments within ship-tracks. Polluted clouds experiencing extended nighttime exposure exhibit higher increases in cloud fraction while liquid-water path adjustments follow a non-monotonic evolution. The higher cloud fraction increase persists through daytime. Such diel variations likely stem from diel changes in solar heating and background cloud precipitation, and are important because nighttime changes persist and affect solar radiation during the day. Accounting for diel variations produces a stronger aerosol forcing, by −0.1 ∼−0.4 W⁢m −2 . Our approach reveals how the temporal evolution of cloud adjustments can have important implications for aerosol-cloud interactions.

Yuan, Tianle [NASA Goddard Space Flight Center (GS↗

NASA NTRS2010

Changes in Stratiform Clouds of Mesoscale Convective Complex Introduced by Dust Aerosols

Aerosols influence the earth s climate through direct, indirect, and semi-direct effects. There are large uncertainties in quantifying these effects due to limited measurements and observations of aerosol-cloud-precipitation interactions. As a major terrestrial source of atmospheric aerosols, dusts may serve as a significant climate forcing for the changing climate because of its effect on solar and thermal radiation as well as on clouds and precipitation processes. Latest satellites measurements enable us to determine dust aerosol loadings and cloud distributions and can potentially be used to reduce the uncertainties in the estimations of aerosol effects on climate. This study uses sensors on various satellites to investigate the impact of mineral dust on cloud microphysical and precipitation processes in mesoscale convective complex (MCC). A trans-Atlantic dust outbreak of Saharan origin occurring in early March 2004 is considered. For the observed MCCs under a given convective strength, small hydrometeors were found more prevalent in the dusty stratiform regions than in those regions that were dust free. Evidence of abundant cloud ice particles in the dust regions, particularly at altitudes where heterogeneous nucleation of mineral dust prevails, further supports the observed changes of clouds and precipitation. The consequences of the microphysical effects of the dust aerosols were to shift the size spectrum of precipitation-sized hydrometeors from heavy precipitation to light precipitation and ultimately to suppress precipitation and increase the lifecycle of cloud systems, especially over stratiform areas.

Lin, B.↗

NASA NTRS2016

Aerosol Complexity and Implications for Predictability and Short-Term Forecasting

There are clear NWP and climate impacts from including aerosol radiative and cloud interactions. Changes in dynamics and cloud fields affect aerosol lifecycle, plume height, long-range transport, overall forcing of the climate system, etc. Inclusion of aerosols in NWP systems has benefit to surface field biases (e.g., T2m, U10m). Including aerosol affects has impact on analysis increments and can have statistically significant impacts on, e.g., tropical cyclogenesis. Above points are made especially with respect to aerosol radiative interactions, but aerosol-cloud interaction is a bigger signal on the global system. Many of these impacts are realized even in models with relatively simple (bulk) aerosol schemes (approx.10 -20 tracers). Simple schemes though imply simple representation of aerosol absorption and importantly for aerosol-cloud interaction particle-size distribution. Even so, more complex schemes exhibit a lot of diversity between different models, with issues such as size selection both for emitted particles and for modes. Prospects for complex sectional schemes to tune modal (and even bulk) schemes toward better selection of size representation. I think this is a ripe topic for more research -Systematic documentation of benefits of no vs. climatological vs. interactive (direct and then direct+indirect) aerosols. Document aerosol impact on analysis increments, inclusion in NWP data assimilation operator -Further refinement of baseline assumptions in model design (e.g., absorption, particle size distribution). Did not get into model resolution and interplay of other physical processes with aerosols (e.g., moist physics, obviously important), chemistry

Predictability↗

NASA NTRSDate not supplied

Impacts of aerosol size-dependent below-cloud scavenging on tropospheric aerosol in the NASA GEOS model

Cloud scavenging is the major sink for a suite of tropospheric aerosols, and thus largely affects the global distribution and lifetime of aerosols as well as the formation of clouds. Simplified model parameterizations of cloud scavenging of aerosols substantially contribute to large uncertainties in the simulated aerosol burdens, spatial distributions, lifetimes, as well as aerosol radiative forcing. Here we evaluate the wet scavenging scheme in the current NASA GEOS model, develop more physically-based parameterizations of below-cloud scavenging, and assess the impacts of the new scavenging parameterizations on the GEOS simulations of aerosols. The current below-cloud scavenging (BCS; washout) scheme uses a first-order removal with a constant scavenging coefficient. We replaced the current scheme with a size-dependent parameterization of Croft et al.(Atmos. Chem. Phys., 2009; hereafter referred to as C09). The C09 BCS parameterizations calculate aerosol below-cloud scavenging coefficients based on a size-dependent collision efficiency between aerosol particles and raindrops (or snow crystals). A look-up table of compiled collision efficiencies provides values for sixty aerosol sizes and nine rain flux rates. Snow-aerosol collision efficiencies are a function of the sixty aerosol sizes only. We assume a log-normal size distribution for aerosols (bulk) in GOCART. The collision efficiencies are then calculated online using a bilinear interpolation from the look-up table for the given aerosol sizes and precipitation flux rates in the model.

aerosols↗

NASA NTRSDate not supplied

TPSAS-NF1676L-10947-DND

There are large uncertainties in quantifying dust effects on the climate because of the limitations on the measurements and observations of dust-cloud-precipitation-dynamics interactions. As a major terrestrial source of atmospheric aerosols, dusts may serve as a significant climate forcing for the changing climate due to its effect on solar and thermal radiation as well as on clouds and precipitation processes. Latest satellites measurements enable us to determine dust loadings and cloud distributions and can potentially be used to reduce the uncertainties in the estimations of aerosol effects on climate. This study uses sensors on various satellites to investigate the impact of mineral dust on cloud microphysical and precipitation processes in convective systems. A trans-Atlantic dust outbreak of Saharan origin occurring in early March 2004 is considered. For the observed convective systems under a given convective strength, small hydrometeors were found more prevalent in the dusty stratiform regions than in those regions that were dust free. Evidence of abundant cloud ice particles in the dust regions, particularly at altitudes where heterogeneous nucleation of mineral dust prevails, further supports the observed changes of clouds and precipitation. These microphysical effects of the dusts on clouds are to shift the size spectrum of precipitation-sized hydrometeors from heavy precipitation to light precipitation and ultimately to suppress precipitation and increase the lifecycle of cloud systems, especially for stratiform clouds.

B Lin↗

DOE OSTI2022

Near‐Cloud Aerosol Retrieval Using Machine Learning Techniques, and Implied Direct Radiative Effects

Abstract There is a lack of satellite‐based aerosol retrievals in the vicinity of low‐topped clouds, mainly because reflectance from aerosols is overwhelmed by three‐dimensional cloud radiative effects. To account for cloud radiative effects on reflectance observations, we develop a Convolutional Neural Network and retrieve aerosol optical depth (AOD) with 100–500 m horizontal resolution for all cloud‐free regions regardless of their distances to clouds. The retrieval uncertainty is 0.01 + 5%AOD, and the mean bias is approximately −2%. In an application to satellite observations, aerosol hygroscopic growth due to humidification near clouds enhances AOD by 100% in regions within 1 km of cloud edges. The humidification effect leads to an overall 55% increase in the clear‐sky aerosol direct radiative effect. Although this increase is based on a case study, it highlights the importance of aerosol retrievals in near‐cloud regions, and the need to incorporate the humidification effect in radiative forcing estimates.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

CMIP7 Data Request: atmosphere priorities and opportunities

This paper presents a comprehensive overview of the Coupled Model Intercomparison Project Phase 7 (CMIP7) request for data unlocking key research avenues in atmospheric science and provides justification for the resources needed to produce this data. Topics within the CMIP7 Atmosphere Theme centre around processes and feedbacks in atmospheric science such as clouds, aerosols and atmospheric chemistry, atmospheric circulation, temperature variability and extremes, radiative forcings, and Earth system model evaluation. These topics are summarised in this paper as scientific “opportunities” which will be realised through CMIP7 experiments and Earth system model outputs. These opportunities were submitted by a thematic group of atmospheric science community representatives combined with an extended consultation process. The production of these variables will close key gaps and uncertainties identified during previous rounds of CMIP, and will be broadly used by scientific, policy, governmental, industry, and other communities that rely on climate model projections for research and decision making, including supporting the 7th Intergovernmental Panel on Climate Change Assessment Report (AR7). As an author group, we also reflect on the process used to collate this data request and make recommendations to future CMIP governance on implementing a consultation on this scale in the future.

58 GEOSCIENCES↗

NASA NTRS1994

Spatial organization and time dependence of Jupiter's tropospheric temperatures, 1980-1993

The spatial organization and time dependence of Jupiter's temperature near 250-millibar pressure were measured through a jovian year by imaging thermal emission at 18 micrometers. The temperature field is influenced by seasonal radiative forcing, and its banded organization is closely correlated with the visible cloud field. Evidence was found for a quasi-periodic oscillation of temperatures in the Equatorial Zone, a correlation between tropospheric and stratospheric waves in the North Equatorial Belt, and slowly moving thermal features in the North and South Equatorial Belts. There appears to be no common relation between temporal changes of temperature and changes in the visual albedo of the various axisymmetric bands.

Orton, Glenn S.↗

NASA NTRS1996

Solar Absorption in Cloudy Atmospheres

The theoretical computations used to compute spectral absorption of solar radiation are discussed. Radiative properties relevant to the cloud absorption problem are presented and placed in the context of radiative forcing. Implications for future measuring programs and the effect of horizontal inhomogeneities are discussed.

Harshvardhan↗

NASA NTRS2002

The Radiative Impact of Smoke Aerosols on Clouds in Southeast Asia

The impact of smoke aerosols generated from biomass burning activities in Southeast Asia on the total (direct and indirect) reflected solar radiation from clouds was investigated using satellite data. Narrowband measurements from UV to near-infrared wavelengths (from SeaWiFS and TOMS) were combined with broadband radiation measurements (from CERES). Using this information, we quantified how smoke aerosols change the cloud forcing spectrally and as a whole in the Southeast Asia region. In this region our results show that smoke is present over large areas of cloud-covered regions, and that the frequency of such occurrences is high in the boreal spring. Depending on the thickness of the smoke aerosol, the reflected solar radiation from clouds could he reduced by as much as 100 Watt/sq m, on average over the March 2000 data. We also found that the reduction in the reflectance of the clouds at 670 nm is large enough to lead to significant errors in cloud optical thickness retrievals from satellites such as AVHRR and MODIS.

Hsu, N. Christina↗

NASA NTRS2017

Exploring the Elevated Water Vapor Signal Associated with Biomass Burning Aerosol over the Southeast Atlantic Ocean

The quantification of radiative forcing due to the cumulative effects of aerosols, both directly and on cloud properties, remains the biggest source of uncertainty in our understanding of the physical climate. How the magnitude of these effects may be modified by meteorological conditions is an important aspect of this question. The Southeast Atlantic Ocean (SEA), with seasonal biomass burning (BB) smoke plumes overlying a persistent stratocumulus cloud deck, offers a perfect natural observatory in which to study the complexities of aerosol-cloud interactions. The NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) campaign consists of three field deployments over three years (2016-2018) with the goal of gaining a better understanding of the complex processes (direct and indirect) by which BB aerosols affect clouds. We present results from the first ORACLES field deployment, which took place in September 2016 out of Walvis Bay, Namibia. Two NASA aircraft were flown with a suite of aerosol, cloud, radiation, and meteorological instruments for remote-sensing and in-situ observations. A strong correlation was observed between the aircraft-measured pollution indicators (carbon monoxide and aerosol properties) and atmospheric water vapor content, at all altitudes. Atmospheric reanalysis indicates that convective dynamics over the continent, near likely contribute to this elevated signal. Understanding the mechanisms by which water vapor covaries with plume strength is important to quantifying the magnitude of the aerosol direct and semi-direct effects in the region.

Pistone, Kristina↗

NASA NTRS1992

Climate forcing by anthropogenic aerosols

Although long considered to be of marginal importance to global climate change, tropospheric aerosol contributes substantially to radiative forcing, and anthropogenic sulfate aerosol, in particular, has imposed a major perturbation to this forcing. Both the direct scattering of short-wavelength solar radiation and the modification of the shortwave reflective properties of clouds by sulfate aerosol particles increase planetary albedo, thereby exerting a cooling influence on the planet. Current climate forcing due to anthropogenic sulfate is estimated to be -1 to -2 watts per square meter, globally averaged. This perturbation is comparable in magnitude to current anthropogenic greenhouse gas forcing but opposite in sign. Thus, the aerosol forcing has likely offset global greenhouse warming to a substantial degree. However, differences in geographical and seasonal distributions of these forcings preclude any simple compensation. Aerosol effects must be taken into account in evaluating anthropogenic influences on past, current, and projected future climate and in formulating policy regarding controls on emission of greenhouse gases and sulfur dioxide. Resolution of such policy issues requires integrated research on the magnitude and geographical distribution of aerosol climate forcing and on the controlling chemical and physical processes.

Charlson, R. J.↗