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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 397 records · Page 22
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Effects of temperature inversion on densification in chemical vapor infiltration

In a classical chemical vapor infiltration (CVI) process, the competing effects of chemical kinetics and reagent gas transport lead to non–uniform depositions such that outer layers of a preform densify faster leaving the core highly porous. Currently, CVI must be performed at a sufficiently low temperature to achieve good densification quality which leads to high processing time and cost. Volumetric heating of the preform, especially through microwaves, can create temperature inversion such that the core is hotter than the outer surface and potentially, overcome the challenges associated with isothermal CVI. Direct numerical simulations (DNS) of densification under various such temperature distributions indicate that microwave heating in CVI processing can lead to better (uniform) densification of porous preforms. Here the role of key parameters describing the temperature distributions on the densification behavior is investigated. Strategic temporal control of the temperature distribution shows that processing times can be reduced by almost half while maintaining a good densification quality similar to that of low–temperature isothermal processing. Inside–out densification due to the inverted temperature profile is a key distinguishing characteristic of microwave assisted CVI.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1992

Statistical analysis of stratospheric temperature and ozone profile data for trends and model comparison

Work performed during the project period July 1, 1990 to June 30, 1992 on the statistical analysis of stratospheric temperature data, rawinsonde temperature data, and ozone profile data for the detection of trends is described. Our principal topics of research are trend analysis of NOAA stratospheric temperature data over the period 1978-1989; trend analysis of rawinsonde temperature data for the period 1964-1988; trend analysis of Umkehr ozone profile data for the period 1977-1991; and comparison of observed ozone and temperature trends in the lower stratosphere. Analysis of NOAA stratospheric temperature data indicates the existence of large negative trends at 0.4 mb level, with magnitudes increasing with latitudes away from the equator. Trend analysis of rawinsonde temperature data over 184 stations shows significant positive trends about 0.2 C per decade at surface to 500 mb range, decreasing to negative trends about -0.3 C at 100 to 50 mb range, and increasing slightly at 30 mb level. There is little evidence of seasonal variation in trends. Analysis of Umkehr ozone data for 12 northern hemispheric stations shows significant negative trends about -.5 percent per year in Umkehr layers 7-9 and layer 3, but somewhat less negative trends in layers 4-6. There is no pronounced seasonal variation in trends, especially in layers 4-9. A comparison was made of empirical temperature trends from rawinsonde data in the lower stratosphere with temperature changes determined from a one-dimensional radiative transfer calculation that prescribed a given ozone change over the altitude region, surface to 50 km, obtained from trend analysis of ozonsonde and Umkehr profile data. The empirical and calculated temperature trends are found in substantive agreement in profile shape and magnitude.

Tiao, G. C.↗
NASA NTRS1979

Full-scale aircraft simulation with cryogenic tunnels and status of the National Transonic Facility

The effect of thermal and caloric imperfections in cryogenic nitrogen on boundary layers was determined to indicate that in order to simulate nonadiabatic laminar or turbulent boundary layers in a cryogenic nitrogen wind tunnel, the flight enthalpy ratio, rather than the temperature ratio, should be reproduced. The absence of significant real gas effects on both viscous and inviscid flows makes it unlikely that there will be large real gas effects on the cryogenic tunnel simulation of shock boundary layer interactions or other complex flow conditions encountered in flight. Condensation effects were studied to determine the minimum usable temperature and indicated that under most circumstances free stream Mach number rather than maximum local Mach number determines the onset of condensation effects.

Kilgore, R. A.↗
NASA NTRS1995

Solar coronal hole simulations compared with interpretations of Yohkoh SXT observations

Recent observations of coronal holes made with the soft X-ray telescope aboard Yohkoh have indicated a temperature of 1.8 approximately 2.1 x 10(exp 6) K and an emission measure of 10(exp 25.7 approximately 26.2) cm (exp -5). This is almost the same as in quiet regions of the Sun. Numerical simulations of the temperature density and velocity structure in a coronal hole. using a parameterized heating distribution have been used for a comparison with the Yohkoh observations. Models are obtained which fit the observed temperature and emission measure. with heating fluxes which are consistent with other measurements. However, the final velocity of the solar wind is very slow which indicates the necessity of another acceleration mechanism such as alfven waves.

Tziotziou, K.↗
NASA NTRS2006

Carbon-rich Chondritic Clast PV1 from the Plainview H-chondrite Regolith Formation from H3 Chondrite Material by Possible Cometary Impact

Chondritic clast PV1 from the Plainview H-chondrite regolith breccia is a subrounded, 5-mm diameter unequilibrated chondritic fragment that contains 13 wt% C occurring mainly within irregularly shaped 30-400-micron-size opaque patches. The clast formed from H3 chondrite material as indicated by the mean apparent chondrule diameter (310 micron vs. approximately 300 micron in H3 chondrites), the mean Mg-normalized refractory lithophile abundance ratio (1.00 +/- 0.09 XH), the previously determined 0-isotopic composition (Delta O-17 = 0.66% vs. 0.68 +/- 0.04%0 in H3 chondrites and 0.73 +/- 0.09% in H4-6 chondrites), the heterogeneous olivine compositions in grain cores (with a minimum range of Fal-19), and the presence of glass in some chondrules. Although the clast lacks the fine-grained, ferroan silicate matrix material present in type 3 ordinary chondrites, PV1 contains objects that appear to be recrystallized clumps of matrix material. Similarly, the apparent dearth of radial pyroxene and cryptocrystalline chondrules in PV1 is accounted for by the presence of some recrystallized fragments of these chondrule textural types. All of the chondrules in PV1 are interfused indicating that temperatures must have briefly reached approximately 1100C (the approximate solidus temperature of H-chondrite silicate). The most likely source of this heating was by an impact. Some metal was lost during impact heating as indicated by the moderately low abundance of metallic Fe-Ni in PV1 (approximately 14 wt%) compared to that in mean H chondrites (approximately 18 wt%). The carbon enrichment of the clast may have resulted from a second impact event, one involving a cometary projectile, possibly a Jupiter-family comet. As the clast cooled, it experienced hydrothermal alteration at low water/rock ratios as evidenced by the thick rims of ferroan olivine around low-FeO olivine cores. The C-rich chondritic clast was later incorporated into the H-chondrite parent-body regolith and extensively fractured and faulted.

Rubin, Alan E.↗
NASA NTRS1981

Preliminary results of an assessment of FGGE 'special effort' data and its impact on GLAS model analyses and forecasts

Attempts to improve the handling of satellite temperature and cloud-derived data during the FGGE experiment are compared with results gained during the trials. The satellite data were edited by assigning quality indicators to temperature soundings by means of the IR TV camera on the Tiros-N spacecraft, and to cloud-tracked wind data from GEO satellites. The data quality were assayed on the basis of horizontal, vertical, and temporal consistency of observed synoptic conditions. The data interpreter-operator retrieved all available data for an area, determined which regions were data-sparse, then used data-rich areas nearby to supply smoothed gradients into the zones with insufficient data. Results are presented for measurements taken during Jan.-Feb., and May 1979 over Alaska. It was found that enhanced and operational IR soundings were mostly equivalent. Some improvements were implemented in the 1000-300 mb layer thickness and intensification of atmospheric thermal gradients. Interactive processing was concluded to be an aid to processing Tiros-N data. The data-improvements treatment was found to significantly modify large scale analyses.

Atlas, R.↗
NASA NTRS1975

Reaction of sulfur dioxide with modified 440C, studied by Auger electron spectroscopy and depth profiling

Auger electron spectroscopy and sputtering were used to study the interaction of SO2 with modified 440C, which is a nominally 77-wt%-Fe, 14-wt%-Cr, and 4-wt%-Mo bearing steel with C, S, Si, Ni, V, P, and Mn making up the balance. The sample was polycrystalline. Three temperatures were used: room temperature, 500 C, and 600 C. The reaction time was varied from 30 minutes to 2 hours. A surface cleaned of oxides was the starting point for each reaction. For reactions at 500 C, the major constituents Cr, O, Fe, and S were present in the surface film. At 600 C, the principal constituents of the film were Cr, O, and S with no Fe present. Therefore, a transition in film composition occurred between 500 and 600 C. Oxides were the primary constituents of the films at both temperatures. Room-temperature reactions indicated that SO2 adsorbed dissociatively, with approximately equal quantities of S and O on the surface. For the same reaction time (1 hr) and pressure, a strong temperature dependence of film thickness was observed. The film formed at 600 C was approximately seven times thicker than that formed at 500 C.

Ferrante, J.↗
NASA NTRS1985

The Hadley and Rossby regimes in a spherical atmosphere

The properties of the steady Hadley and Rossby regimes for a thermally forced rotating fluid on a sphere are studied. The two layer modified geostrophic model is employed which allows for thermal advection by the divergent wind and time dependent static stability. Heating processes are parameterized using the Newtonian approximation and Rayleigh friction is accounted for. The equations are transformed to spectral form using spherical harmonics and then truncated retaining a simple axisymmetric state and initial, one wave. A time independent Hadley circulation is obtained which is neutral to axisymmetric disturbances but unstable to wave like perturbations for intermediate values of the meridional temperature gradient, indicating the existence of both an upper and lower symmetric Hadley regime. An analytical solution for the steady Rossby circulation is determined for values of the meridional temperature gradient where the Hadley regime is unstable. Linear perturbation theory is used to show that within the steady Rossby regime two or more waves cannot exist simultaneously.

Feldstein, S. B.↗
NASA NTRS2009

The Seasonal Response of Titan's Troposphere and Stratosphere

The radiative response of Titan's atmosphere varies by several orders of magnitude with altitude. This presents an interesting situation in which most of the stratosphere----at least that part above 100km is characterized by radiative relaxation times that are short compared to the length of a Titan season, and the troposphere and tropopause region by times that are larger than seasonal timescales. Consistent with this, Cassini CIRS spectra indicate stratospheric temperatures at 100-170 kin that are 20-30 K cooler at high northern latitudes in winter than those at equatorial and southern latitudes. Given the expectation that the situation will largely reverse in southern winter, the observed large meridional contrast is likely indicative of the expected seasonal variation at polar latitudes in both hemispheres. CIRS spectra do not as easily yield temperatures below 100 km in the lower stratosphere and tropopause region, because of the contribution of heterogeneously distributed aerosols and condensates to the infrared opacity. However, Cassini radio occultations probe both the stratosphere and troposphere, and below 80 km they show the thermal contrast with latitude to be muted, e.g,, approx.5 K near the tropopause at 40-50 km and approx.3 K just above the surface. This is consistent with the large radiative relaxation times at these altitudes and with efficient meridional heat transport. What is curious is the manner in which temperatures in the north winter polar atmosphere make the transition between the troposphere and lower stratosphere, where seasonal variations are relatively small, and higher altitudes, where they are large. Temperatures at all latitudes sounded by the radio occultations exhibit similar behavior in the lower stratosphere, increasing with altitude. Between 80 and 100 kin, however, the temperatures at high northern latitudes exhibit a sudden drop with increasing altitude, producing the meridional contrast in the upper stratosphere described above. While the radiative relaxation time associated with infrared gaseous coolants decreases with altitude in the stratosphere, it is not likely to account for the abrupt transition observed. Possible mechanisms for this transition are discussed, including the presence of an optically thick. cloud at thermal-infrared wavelengths.

Flasar, F. M.↗
DOE OSTI2025

Unraveling the depth-dependent causal dynamics of methanogenesis and methanotrophy in a high-latitude fen peatland

The dynamics of methane (CH 4 ) cycling in high-latitude peatlands through different pathways of methanogenesis and methanotrophy are still poorly understood due to the spatiotemporal complexity of microbial activities and biogeochemical processes. Additionally, long-term in situ measurements within soil columns are limited and associated with large uncertainties in microbial substrates (e.g. dissolved organic carbon, acetate, hydrogen). To better understand CH 4 cycling dynamics, we first applied an advanced biogeochemical model, ecosys , to explicitly simulate methanogenesis, methanotrophy, and CH 4 transport in a high-latitude fen (within the Stordalen Mire, northern Sweden). Next, to explore the vertical heterogeneity in CH 4 cycling, we applied the PCMCI/PCMCI+ causal detection framework with a bootstrap aggregation method to the modeling results, characterizing causal relationships among regulating factors (e.g. temperature, microbial biomass, soil substrate concentrations) through acetoclastic methanogenesis, hydrogenotrophic methanogenesis, and methanotrophy, across three depth intervals (0–10 cm, 10–20 cm, 20–30 cm). Our results indicate that temperature, microbial biomass, and methanogenesis and methanotrophy substrates exhibit significant vertical variations within the soil column. Soil temperature demonstrates strong causal relationships with both biomass and substrate concentrations at the shallower depth (0–10 cm), while these causal relationships decrease significantly at the deeper depth within the two methanogenesis pathways. In contrast, soil substrate concentrations show significantly greater causal relationships with depth, suggesting the substantial influence of substrates on CH 4 cycling. CH 4 production is found to peak in August, while CH 4 oxidation peaks predominantly in October, showing a lag response between production and oxidation. Overall, this research provides important insights into the causal mechanisms modulating CH 4 cycling across different depths, which will improve carbon cycling predictions, and guide the future field measurement strategies.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Temperature Effect on Photoelectrochemical Water Splitting: A Model Study Based on BiVO 4 Photoanodes

Photoelectrochemical (PEC) water splitting is typically studied at room temperature. In this work, the temperature effect on PEC water splitting is studied using crystalline BiVO4 thin film photoanode as a model system. Systematic temperature-dependent electrochemical study demonstrates that the PEC activity is boosted at elevated electrolyte temperatures and indicates that thermal energy plays a main role in improving charge carrier transport in the bulk of BiVO 4 . Irreversible surface reconstruction is observed after PEC reactions at elevated temperature in the presence of hole scavengers, with regularly spaced stripes emerging on BiVO4 grains. The surface-reconstructed photoanode exhibits up to 40% improvement in photocurrent densities and ~0.25 V shift of photocurrent onset to favorable direction. Detailed investigation shows the formation of amorphous layer without stoichiometric change at the reconstructed surface. Furthermore, this work provides insights of temperature effect on photoelectrode in solar water splitting and reveals the non-negligible effect of hole scavengers in photoelectrochemical measurement.

36 MATERIALS SCIENCE↗
NASA NTRS1987

Fiber-Optic Temperature Sensor

Proposed sensor measures temperatures over wide range, from cryogenic liquids to burning gases. Made in part of optical fibers, sensor lighter in weight than thermocouple and immune to electromagnetic interference. Device does not respond to temperatures elsewhere than at sensing tip. Thermal expansion and contraction of distance between fiber end and mirror alters interference between light reflected from those two surfaces, thereby giving interferometric indication of temperatures.

Maram, Jonathan M.↗
NASA NTRS2002

Variability of Winter Air Temperature in Mid-Latitude Europe

The aim of this paper is to report extreme winter/early-spring air temperature (hereinafter temperature) anomalies in mid-latitude Europe, and to discuss the underlying forcing to these interannual fluctuations. Warm advection from the North Atlantic in late winter controls the surface-air temperature, as indicated by the substantial correlation between the speed of the surface southwesterlies over the eastern North Atlantic (quantified by a specific Index Ina) and the 2-meter level air temperatures (hereinafter Ts) over Europe, 45-60 deg N, in winter. In mid-March and subsequently, the correlation drops drastically (quite often it is negative). This change in the relationship between Ts and Ina marks a transition in the control of the surface-air temperature: absorption of insolation replaces the warm advection as the dominant control. This forcing by maritime-air advection in winter was demonstrated in a previous publication, and is re-examined here in conjunction with extreme fluctuations of temperatures in Europe. We analyze here the interannual variability at its extreme by comparing warm-winter/early-spring of 1989/90 with the opposite scenario in 1995/96. For these two December-to-March periods the differences in the monthly mean temperature in Warsaw and Torun, Poland, range above 10 C. Short-term (shorter than a month) fluctuations of the temperature are likewise very strong. We conduct pentad-by-pentad analysis of the surface-maximum air temperature (hereinafter Tmax), in a selected location, examining the dependence on Ina. The increased cloudiness and higher amounts of total precipitable water, corollary effects to the warm low-level advection. in the 1989/90 winter, enhance the positive temperature anomalies. The analysis of the ocean surface winds is based on the Special Sensor Microwave/Imager (SSM/I) dataset; ascent rates, and over land wind data are from the European Centre for Medium-Range Weather Forecasts (ECMWF); maps of 2-m temperature, cloud cover and precipitable water are from the National Centers for Environmental Prediction (NCEP) Reanalysis.

Otterman, J.↗
DOE OSTI2020

Hydrogen desorption from the surface and subsurface of cobalt

The influence of coverage on the diffusion of hydrogen into the subsurface of cobalt was studied using density functional theory (DFT) and temperature programmed desorption (TPD). DFT calculations show that as the hydrogen coverage on Co(0001) increases, the barrier for hydrogen diffusion into the bulk decreases by 20%. Additionally, subsurface hydrogen on a hydrogen covered surface was found to be more stable when compared to a clean cobalt surface. To test these theoretical findings experimentally, excited hydrogen was used in an ultra-high vacuum environment to access higher hydrogen coverages. Here, our TPD studies showed that at high hydrogen coverages, a sharp low temperature feature appeared, indicating the stabilization of subsurface hydrogen. Further DFT calculations indicate that this sharp low temperature feature results from associative hydrogen desorption from a hydrogen saturated surface with a population of subsurface hydrogen. Microkinetic modelling was used to model the TPD spectra for hydrogen desporption from cobalt with and without subsurface hydrogen, showing reasonable agreement with experiment.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Subharmonic Shapiro steps in depinning dynamics of a two-dimensional solid dusty plasma modulated by one-dimensional nonlinear deformed periodic substrates

Langevin dynamical simulations are performed to investigate the depinning dynamics of a two-dimensional (2D) solid dusty plasma, which is modulated by one-dimensional (1D) nonlinear deformed periodic substrates, and also driven by the combination of the DC and AC forces. As the DC driving force increases gradually, pronounced subharmonic and harmonic Shapiro steps are discovered under the combined modulation of the deformed substrate and the external AC drive. Here, these observed subharmonic and harmonic Shapiro steps are attributed to the dynamic mode locking. The data analysis results indicate that the nonlinear deformed substrate strongly influences these subharmonic Shapiro steps, which can be accurately diagnosed using the fraction of sixfold coordinated particles. Furthermore, the diagnostic of the kinetic temperature clearly indicates the difference between harmonic and subharmonic Shapiro steps, i.e., the particle motion is slightly less synchronized at subharmonic Shapiro steps, caused by the unstable locations of the deformed substrate.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Study of Elastic and Structural Properties of BaFe2As2 Ultrathin Film Using Picosecond Ultrasonics

We obtain the through-thickness elastic stiffness coefficient (C33) in nominal 9 nm and 60 nm BaFe2As2 (Ba-122) thin films by using picosecond ultrasonics. Particularly, we reveal the increase in elastic stiffness as film thickness decreases from bulk value down to 9 nm, which we attribute to the increase in intrinsic strain near the film-substrate interface. Our density functional theory (DFT) calculations reproduce the observed acoustic oscillation frequencies well. In addition, temperature dependence of longitudinal acoustic (LA) phonon mode frequency for 9 nm Ba-122 thin film is reported. The frequency change is attributed to the change in Ba-122 orthorhombicity (a−b)/(a+b). This conclusion can be corroborated by our previous ultrafast ellipticity measurements in 9 nm Ba-122 thin film, which exhibit strong temperature dependence and indicate the structural phase transition temperature Ts.

36 MATERIALS SCIENCE↗
NASA NTRS1977

On coronal Fe abundances and temperatures from XUV emission lines

Data obtained by the OSO-7 spectroheliograph on strong XUV lines of five different Fe ions from the outer equatorial corona are presented. Interpretation of the data with a spherically symmetric model atmosphere gives average ion abundances for lines of sight at 0.3 solar radii from the limb. Fe XVI is usually more abundant than Fe XV, XIV, XII and IX, but there are times when Fe XII is more abundant than the other ions. The deviation of measured relative abundances of Fe XII, XIV, and XVI from predictions of ionization equilibrium at one temperature seems to indicate that there are appreciable temperature variations along lines of sight. Element abundances are very uncertain since they appear to depend so heavily on likely but unknown density irregularities along lines of sight.

Nakada, M. P.↗
NASA NTRS1985

Coronal Temperatures

The solid state spectrometer (SSS) on the Einstein Observatory (HEAO 2) was sensitive in the energy range 0.5 to 4.5 keV to fluxes as low as 4x10 to the 12th power ergs/cu cm/s. Good spectra were obtained for 19 stars, including Algol, 7 RS CVn systems, 2 dMe stars, 2 W UMa binaries, 1 GV single star, and 3 0B supergiants, 2 BV stars and 1 07 binary. This is a very incomplete survey of stellar coronae, but it does include coverage of several late and early types and usually more than 1 sample of the class. The results for these stars suggest two generalizations despite the small numbers: (1) there is a broad variety of X-ray spectra of stellar coronae; and (2) there probably are X-ray spectral types (X-ray coronae of stars of similar other properties have similar temperatures). Evidence indicating that some emission distributions are bimodal is discussed. Finally, some remarks are made concerning the spectra of the early type stars and constraints on the presence of very high temperatures.

Swank, J. H.↗