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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 397 records · Page 22
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Laser-induced fluorescence of filament-produced plasmas

Self-guided ultrafast laser filaments are a promising method for laser beam delivery and plasma generation for standoff and remote detection of elements and isotopes via filament-induced breakdown spectroscopy (FIBS). Yet, there are several challenges associated with the practical application of FIBS, including delivery of sufficient laser energy at the target for generating plasma with a copious amount of emission signals for obtaining a high signal-to-noise ratio. Here, in this study, we use laser-induced fluorescence (LIF) to boost the emission signal and reduce self-reversal in the spectral profiles. Ultrafast laser filaments were used to produce plasmas from an Al 6061 alloy target at various standoff distances from 1 to 10 m. For LIF emission enhancement, a narrow linewidth continuous-wave laser was used in resonance with a 394.40 nm Al I resonant transition, and the emission signal was monitored from the directly coupled transition at 396.15 nm. Emission signal features of Al I are significantly enhanced by resonant excitation. In addition, LIF of filament ablation plumes reduces the self-reversal features seen in the thermally excited spectral profiles. Time-resolved two-dimensional fluorescence spectroscopy was performed for evaluating the optical saturation effects, which are found to be non-negligible due to high Al atomic densities in the filament-produced plasmas.

47 OTHER INSTRUMENTATION↗
DOE OSTI2026

FLASH-therapy suitable single-pulse proton generation using TiH 2 under nanosecond laser irradiation

We investigated proton emission from titanium hydride (TiH 2 ) targets irradiated in vacuum by a 6-ns, 1064-nm Nd:YAG laser. Time-of-flight measurements with a Faraday cup and an electrostatic ion analyzer resolved distinct proton peaks at high pulse energies, with yields on the order of 10 9 protons per shot. Systematic scans over pulse energy and up to 1000 repeated shots showed that, while the peak amplitude gradually decreased, the integrated proton number remained nearly constant. This behavior is consistent with surface-induced broadening of the plasma expansion while bulk hydrogen is replenished by diffusion and repeated ablation of fresh TiH 2 layers. Using the measured proton numbers and pulse widths, a simple direct-plasma-injection-style scaling indicates peak currents of ∼100 mA and sub-microsecond pulse durations. The pulse structure and yield satisfy key ultra-high-dose-rate criteria and, together with sustained output over 1000 shots, support TiH 2 -based laser ion sources as practical candidates for FLASH-therapy (ultra-high-dose-rate)-oriented studies and injector development using direct plasma injection.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Development of a directly driven multi-shell platform: Laser drive energetics

Simulations predict that directly driven multi-shell targets can provide a robust alternative to conventional high-convergence implosion concepts by coupling two to three times more energy into the final igniting thermonuclear fuel assembly than indirect-drive concepts. The three-shell directly driven Revolver concept [K. Molvig, M. J. Schmitt, B. J. Albright, E.S. Dodd, N.M. Hoffman, G.H. McCall, and S.D. Ramsey, Phys. Rev. Lett. 116, 255003 (2016)] utilizes a design that maximizes laser energy conversion into inward kinetic energy of the outermost ablator shell (~9%) while minimizing the DT fuel convergence (~9) to reduce the mixing of material from the innermost shell into the fuel. Inherent in this design concept is the use of 192 narrow beams (with a 1/e laser beam-to-capsule diameter ratio of 0.33) from the National Ignition Facility laser pointed in a polar direct drive laser configuration. In this paper, we demonstrate that low average laser intensity at the capsule surface (≤300 TW/cm 2 ) limits the measured laser backscatter, indicating that a greater amount of laser energy is coupled into the target. Omega experiments have been performed to determine the coupling of laser energy to the outermost shell of a scaled Revolver target (i.e., the ablator shell) by measuring capsule implosion trajectories and scattered-light fractions for two different drive configurations. Comparisons of simulated shell trajectory and velocity profiles with experimental data obtained from self-emission images show good agreement and are consistent with measured scattered light data. Furthermore, the low levels of scattered light measured are consistent with post-shot simulation results that show high hydro-coupling efficiency. These results strengthen the case for using narrow beams at low intensity to drive large ablator capsules for future direct-drive, multi-shell ignition concepts.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Symmetry requirements for double shell capsules with aluminum ablators

Double shell targets present a promising avenue to obtain robust neutron yield on current laser facilities. The nature of the target, like current single shell designs, requires a symmetric implosion of an outer ablator to obtain a symmetric fuel volume that will lead to alpha heating and thermonuclear burn. Due to using aluminum as an ablator material and requiring different convergence than single shell symmetry studies at various energies are required. This paper moves forward from previous experiments conducted at 1MJ to show implosion symmetry at 1.25 and 1.5MJ. Symmetry in these experiments is sufficient to merit experiments using double shells to study the platform further. Additional studies are carried out on the outer shell symmetry impacts, showing that mitigating mode growth on the outer ablator is of great importance.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Low mode implosion symmetry sensitivity in low gas-fill NIF cylindrical hohlraums

Achieving an efficient capsule implosion in National Ignition Facility indirect-drive target experiments requires symmetric hohlraum x-ray drive for the duration of the laser pulse. This is commonly achieved using two-sided two-cone laser irradiation of cylindrical hohlraums that, in principle, can zero the time average of all spherical harmonic asymmetry modes <6 as well as the time dependence of the usually dominant mode 2. In practice, experimental evidence indicates that maintaining symmetric drive becomes limited late in the pulse due to the inward expansion of the hohlraum wall and outward expansion of the capsule ablator plasmas impairing the propagation of the inner-cone laser beams. This effect is enhanced in hohlraums employing low gas-fill, now used almost exclusively as these provide the highest performing implosions and reduce Stimulated Brillouin and Raman backscatter losses, since the gas plasma provides less back pressure to limit blow-in of the hohlraum wall and capsule ablator plasmas. In order to understand this dynamic behavior, we combined multi-keV X-ray imaging of the wall and imploded fuel plasmas as we changed a single parameter at a time: hohlraum gas-fill, laser outer cone picket energy, radius of high density carbon capsules used, and laser beam polar and azimuthal pointing geometry. In this work, we developed a physics-based multi-parameter experimental scaling to explain the results that extend prior scalings and compare those to radiation hydrodynamic simulations to develop a more complete picture of how hohlraum, capsule, and laser parameters affect pole vs equator drive symmetry.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Two-dimensional Thomson scattering measurements of misaligned electron density and temperature gradients and associated Biermann battery produced fields

We present optical Thomson scattering measurements of electron density and temperature in high Mach number laser-driven blast waves in homogeneous gases. Taylor–Sedov blast waves are launched in nitrogen (N2) or helium (He) at pressures between 0.4 mTorr and 10 Torr by ablating a solid plastic target with a high energy laser pulse (10 J, 1012 W/cm2). Experiments are performed at high repetition rate (1 Hz), which allows one-dimensional and two-dimensional Thomson scattering measurements over an area of several cm2 by automatically translating the scattering volume between shots. Electron temperature and density in the blast wave fronts were seen to increase with increasing background gas pressure. Measured electron density and temperature gradients were used to calculate ∂B/∂t∝∇Te×∇ne. The experimentally measured ∂B/∂t showed agreement with the magnetic field probe (B-dot) measurements, revealing that magnetic fields are generated in the observed blast waves via the Biermann battery effect. The results are compared to numerical three-dimensional collisional magnetohydrodynamic simulations performed with FLASH, and are discussed in the context of spontaneous magnetic field generation via the Biermann battery effect.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Hot Electron Scaling and Energy Coupling In Nonlinear Laser Plasma Interactions

Energy conversion from high power lasers to energetic hot electrons is a fundamental phenomenon in laser-plasma interactions. At laser intensities above a few times 10 14 W/cm 2 , nonlinear laser-plasma interactions lead to the generation of hot electrons with a broad energy distribution at typical temperatures of 10’s – 100’s kilo-electron-volt (keV). The fraction of laser energy transferred to hot electrons, their energy distribution and energy coupling efficiency to the targets are strongly affected by the laser intensity, wavelength and the plasma condition. Most investigations to date that are related to the fusion of high-energy-density laboratory plasmas (HEDLP) are carried out with relatively moderate laser intensity and lower laser wavelength to minimize hot electron generation, as electron preheating can degrade the fuel assembly. An alternative fusion scheme known as shock ignition (SI) has been proposed, requiring a high intensity spike pulse at the end of a fuel assembly phase to generate a strong shock to ignite the fuel. An initial shock pressure of 0.3 Gbar is required for ignition-scale targets using the SI scheme, requiring a relatively high on-target laser intensity of 5-10X10 15 W/cm 2 for the spike pulse. At such intensities, copious hot electrons can be produced by laser-plasma-instabilities (LPI), e.g., Stimulated Raman Scattering (SRS) and Two-Plasmon Decay (TPD). While very energetic electrons (>200 keV) could preheat the fuel, electrons with moderate energies may actually be beneficial for the SI scheme. Electrons in the 50-100 keV range can be stopped in the compressed high-density outer ablator layer leading to an increase in the ignitor shock strength and therefore enhancing overall efficiency in the SI scheme. Considering this importance of total energy and temperature of hot electrons, it is necessary to understand the LPI in the SI high intensity regime. Characterizing the hot electron source and energy coupling is key to investigating the viability of the SI concept. The overall goal of the HEDLP award was to perform a detailed study of the scaling of hot electron generation and energy coupling on high power laser systems, with intensity, wavelength, and target ablator material relevant to the nonlinear laser-plasma interaction at SI relevant conditions. This was a collaborative project between the Center for Energy Research at the University of California, San Diego (UCSD) and General Atomics. The experiment was performed at the Omega Laser Facility at the Laboratory for Laser Energetics (LLE) in the University of Rochester. Specific objectives of the work were to: understand the basic physics of laser-plasma interactions and instabilities at high laser intensities (up to 10 17 W/cm 2 ) and the effects of low-Z ablator materials and laser wavelengths (IR pulse at 1.054 µm versus UV pulse at 0.351 µm) and intensity scaling, fully characterize the resultant hot electron energy distribution, validate hot electron energy deposition via collisional and kinetic processes in the target and the induced shocks in support of electron-assisted SI concept.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Property Variations in Modern REBCO Coated Conductors from Multiple Manufacturers

The complex, multilayer structure of REBCO Coated Conductor (CC) poses significant challenges in the fabrication of high magnetic field devices where large stresses may initiate various forms of damage. Our goal is to peer below the cartoon representations of CC so that, amongst other things, we might better understand whether a CC from one manufacturer is interchangeable with that from another. This involves knowledge of a broad range of electromagnetic, geometric, microstructural, and J c (θ,B,T) properties, and their variations that collectively pose challenges for the fault tolerance of REBCO CC devices. Accordingly, comparative measurements of J c , visualization of flux penetration with Magneto-Optical Imaging (MOI), tape geometry from Scanning Electron Microscopy (SEM) of polished cross-sections, and extensive optical microscopy was performed on recently purchased samples from multiple manufacturers. Our analyses reveal many deviations from or characteristics absent from manufacturers’ specifications, while a comparison of different manufacturers’ mechanically and laser slit tapes shows a diverse array of slitting characteristics amongst the manufacturers and variation in properties those made to the same specification. Laser slit tapes from several manufacturers reveal ablated edges with damaged regions extending up to 50 μm, comparable to the damaged region found in the mechanically slit CC of this study. Overall, the aim of this study is to flesh out appropriate ways to understand the real conductor below the manufacturers’ cartoons to avoid surprises in our REBCO CC coil development program. The goal of this work was to perform a broad array of characterizations of the type needed for validation of purpose for making high field magnets: to our surprise we found a wide range of properties which greatly impact the mechanical strength and electromagnetic performance of solenoids composed of these conductors and reinforced the need for a broad characterization program for each conductor prior to its implementation.

Bradford, G.↗
DOE OSTI2022

Hot-electron preheat and mitigation in polar-direct-drive experiments at the National Ignition Facility

Target preheat by superthermal electrons from laser–plasma instabilities is a major obstacle to achieving thermonuclear ignition via direct-drive inertial confinement fusion at the National Ignition Facility (NIF). Polar-direct-drive surrogate plastic implosion experiments were performed on the NIF to quantify preheat levels at ignition-relevant scale and develop mitigation strategies. Here, the experiments were used to infer the hot-electron temperature, energy fraction, divergence, and to directly measure the spatial hot-electron energy deposition profile inside the imploding shell. Silicon layers buried in the ablator are shown to mitigate the growth of laser–plasma instabilities and reduce preheat, providing a promising path forward for ignition designs at an on-target intensity of about 10 15 W/cm 2 .

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Mitigation of hot-electron preheat from the two-plasmon-decay instability using silicon-doped plastic shells in direct-drive implosions on OMEGA

Hot electrons generated by the two-plasmon-decay (TPD) instability in laser-direct-drive implosions preheat the fuel and degrade performance. The mitigation of preheat using silicon-doped ablators (i.e., preheat is reduced by a factor of 1.40 ± 0.04) while decreasing the ratio of the laser spot diameter to the target diameter (⁠R b /R t⁠ ) to mitigate cross-beam energy transfer has been demonstrated on the OMEGA laser for quarter-critical laser intensities of 4.1 x 10 14 W/cm 2 ⁠, equivalent to an incident laser intensity of 8.3 x 10 14 W/cm 2 ⁠. The silicon dopant increases the electron temperature of the ablation plasma, which raises the intensity threshold for the onset of the TPD instability. These results show that implosion designs utilizing higher drive intensities can be used to achieve higher shell velocities, which are currently inaccessible with plastic ablators due to excessive preheat.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Hot-electron generation at direct-drive ignition-relevant plasma conditions at the National Ignition Facility

Laser–plasma interaction instabilities can be detrimental for direct-drive inertial confinement fusion by generating high-energy electrons that preheat the target. Moreover, an experimental platform has been developed and fielded on the National Ignition Facility to investigate hot-electron production from laser–plasma instabilities at direct-drive ignition-relevant conditions. The radiation-hydrodynamic code DRACO has been used to design planar-target experiments that generate plasma and interaction conditions comparable to direct-drive ignition designs: I L ~10 15 W/cm 2 , T e > 3 keV, and density-gradient scale lengths of L n ~ 600 μ m in the quarter-critical density region. The hot-electron properties were inferred by comparing the experimentally observed hard x-ray spectra to Monte Carlo simulations of hard x-ray emission from hot electrons depositing energy in the target. Hot-electron temperatures of ~40 keV to 60 keV and the fraction of laser energy converted to hot electrons of ~0.5% to 5% were inferred in plastic targets for laser intensities at the quarter-critical density surface of (~4 to 14) × 10 14 W/cm 2 . The use of silicon ablators was found to mitigate the hot-electron preheat by increasing the threshold laser intensity for hot-electron generation from ~3.5 × 10 14 W/cm 2 in plastic to ~6 × 10 14 W/cm 2 in silicon. The overall hot-electron production is further reduced in silicon ablators when the intensity threshold is exceeded.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Atmospheric clearing of solid-particle debris using femtosecond filaments

Through nonlinear self-focusing, femtosecond pulses can propagate several kilometers beyond diffraction limits, forming an ionization channel in air known as a laser filaments. It has been demonstrated that in the wake of the filament, aerosols can be effectively cleared to improve the transmission of subsequent laser pulses or secondary light sources, pertinent to applications in atmospheric sensing. However, the current understanding of aerosol clearing is founded on interactions with droplets to simulate fogs and clouds and thus does not extend to solid particles or atmospheric debris. Using optical trapping, we isolate both graphite and silica microparticles and directly measure the subsequent displacement caused by the filament using time-resolved shadowgraphy. The shock wave from the filament is demonstrated to propel particles away from the filament, directly contributing to atmospheric debris clearing. Particles exposed to the laser light in either the intense filament core or the surrounding energy reservoir are axially displaced along the beam path. Furthermore, it is found that the optomechanical properties of the particle largely influence the axial displacement induced by laser exposure through mechanisms such as radiation pressure, mass ejection from ablation or optical damage, and particle deagglomeration.

42 ENGINEERING↗
DOE OSTI2020

Destruction of absorbing metal films during laser printing with gel microdroplets

The degree of destruction and evaporation of metal films (Au and Ti, thickness ∼50 nm) with a gel layer during laser transfer of small volumes of a gel substrate is estimated depending on the laser fluence value. The dynamics of these processes for dry films and films with a gel layer at fluences close to threshold values is investigated using a probe beam of a He – Ne laser. It is shown that the presence of a gel leads to an increase in the ablation threshold, but the time during which the process of structural changes in the film material is completed does not change significantly. The results obtained can be used to improve the laser bioprinting technology. (interaction of laser radiation with matter)

36 MATERIALS SCIENCE↗
DOE OSTI2024

Excitation of optically trapped single particles using femtosecond pulses

Excitation from optically trapped particles is examined through laser-induced breakdown spectroscopy following interactions with mJ-level fs pulses. Optical emissions from sub-ng ablation of precisely positioned cupric oxide microparticles are used as a method to spatially resolve laser–particle interactions resulting in excitation. External focusing lenses are often used to change the dynamics of nonlinear self-focusing of fs pulses to form laser filaments or, alternatively, to form very intense air plasmas. Given the significant implications external focusing has on laser propagation and plasma conditions, single-particle emissions are studied with focusing lenses ranging from 50 to 300 mm. It is shown that, while single particles are less excited at longer focal lengths due to limited energy transfer through laser–particle interactions, the cooler plasma results in a lower thermal background to reveal resolved single-shot emission peaks. Furthermore, by developing an understanding in the fundamental interaction that occurs between single particles and fs pulses and filaments, practical improvements can be made for atmospheric remote sensing of low-concentration aerosols.

42 ENGINEERING↗
DOE OSTI2025

Laser wavelength dependence of laser imprint

In laser direct-drive inertial confinement fusion, laser imprint is one of the major causes of degradation in target performance through its seeding of hydrodynamic instabilities. Early experiments and simulations have shown that laser imprint could be mitigated with a longer laser wavelength because of its lower critical density and longer conduction zone. Building upon this work, we explore a scenario where the laser wavelength during the picket pulse differs from that of the main pulse in order to gain the benefit of reduced imprint, while avoiding losses in drive coupling efficiency or an increase in laser-plasma instabilities. A series of 2D radiation-hydrodynamic simulations, which test three different laser wavelengths for the picket pulse, has been performed, where the intensity of the picket pulse is adjusted in order to maintain the same implosion adiabat. A detailed analysis of the growth of the mass density modulations at the ablation front over a large range of mode numbers confirms that the laser imprint can be mitigated with a picket pulse operating at a longer wavelength than the main pulse because of the longer conduction zone and enhanced thermal smoothing. The amplitude of the ablation front modulations is found to be lower for all mode numbers, which reduces the seeding of the Rayleigh–Taylor instability without affecting the mode growth rates.

Fourier analysis↗
DOE OSTI2020

Remote Detection of Uranium Using Self-Focusing Intense Femtosecond Laser Pulses

Optical measurement techniques can address certain important challenges associated with nuclear safety and security. Detection of uranium over long distances presents one such challenge that is difficult to realize with traditional ionizing radiation detection, but may benefit from the use of techniques based on intense femtosecond laser pulses. When a high-power laser pulse propagates in air, it experiences collapse and confinement into filaments over an extended distance even without external focusing. In our experiments, we varied the initial pulse chirp to optimize the emission signal from the laser-produced uranium plasma at an extended distance. While the ablation efficiency of filaments formed by self-focusing is known to be significantly lower when compared to filaments produced by external focusing, we show that filaments formed by self-focusing can still generate luminous spectroscopic signatures of uranium detectable within seconds over a 10-m range. The intensity of uranium emission varies periodically with laser chirp, which is attributed to the interplay among self-focusing, defocusing, and multi-filament fragmentation along the beam propagation axis. Grouping of multi-filaments incident on target is found to be correlated with the uranium emission intensity. The results show promise towards long-range detection, advancing the diagnostics and analytical capabilities in ultrafast laser-based spectroscopy of high-Z elements.

42 ENGINEERING↗
DOE OSTI2023

Nanoscale reshaping of resonant dielectric microstructures by light-driven explosions

Femtosecond-laser-assisted material restructuring employs extreme optical intensities to localize the ablation regions. To overcome the minimum feature size limit set by the wave nature of photons, there is a need for new approaches to tailored material processing at the nanoscale. Here, we report the formation of deeply-subwavelength features in silicon, enabled by localized laser-induced phase explosions in prefabricated silicon resonators. Using short trains of mid-infrared laser pulses, we demonstrate the controllable formation of high aspect ratio (>10:1) nanotrenches as narrow as ~ $λ / 80$. The trench geometry is shown to be scalable with wavelength, and controlled by multiple parameters of the laser pulse train, such as the intensity and polarization of each laser pulse and their total number. Particle-in-cell simulations reveal localized heating of silicon beyond its boiling point and suggest its subsequent phase explosion on the nanoscale commensurate with the experimental data. The observed femtosecond-laser assisted nanostructuring of engineered microstructures (FLANEM) expands the nanofabrication toolbox and opens exciting opportunities for high-throughput optical methods of nanoscale structuring of solid materials.

42 ENGINEERING↗
DOE OSTI2021

Reducing Direct Drive Preheat with Dopants

Preheat in laser-driven experiments can have negative impacts on inertial confinement fusion (ICF) and hydrodynamic experiments. While many groups employ the use of dopants to reduce or block preheat, direct quantification has not previously been explored. We developed a planar platform and a series of ablator targets to measure the electron and x-ray spectra generated by laser-plasma interactions with a direct drive using OMEGA-60. By comparing both thin ablators (75 μm) and thick ablators (270 μm) that were either pure CH, 3% Si doped or 3% I doped, we were able to measure differences in electron and x-ray spectra. In addition, we observed the preheat growth of tracer layers and observed reductions in the growth with different materials. We find that iodine or a thin gold layer is the best at tamping the direct-drive preheat at OMEGA, but that the growth is still significant.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗