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At least 397 records · Page 22

High-resolution lidar system for measuring the spatial and temporal structure of the mesospheric sodium layer

The design of a high-resolution tunable-dye laser-based lidar system for the study of the mesospheric sodium layer is presented and results of sodium measurements are indicated. The lidar system comprises a tunable flashlamp-pumped dye laser operating at the sodium D2 resonance line at 589.0 nm with a pulse width of 2 microsec FWHM and pulse frequency of 10 Hz and a telescope with a 1.22=m diameter Fresnel lens. Sodium profiles are obtained from the integration of 100 to 250 laser shots, with spatial and temporal resolution enhanced by two-dimensional filtering techniques. Measurements obtained over a 9-hour nighttime period illustrate the highly dynamic nature of the sodium layer, which was observed with a spatial resolution of 2 km and temporal resolution of 30 min. Observations made with a steerable apparatus have confirmed a presunrise enhancement of over 100 percent in sodium column abundance.

Gardner, C. S.↗

Generation of 369.4 nm Radiation by Efficient Doubling of a Diode Laser

The trapped ytterbium ion frequency standard under development at JPL is designed to supply ultra-stable reference signals to be used in spacecraft tests of general relativity and other science experiments. Only diode lasers meet the requirements of low power comsumption and small size for use aboard spacecraft, but diode lasers are not currently available at 369.4 nm wavelength. It is therefore necessary to employ frequency doubling methods to reach this frequency with diode lasers. Here we present the characteristics of the resonant cavity doubling system we have designed and preliminary UV conversion results.

ultra-stable↗

The OH + HBr reaction revisited

Variable-temperature measurements of the rate coefficient /k(1)/ for the reaction OH + HBr yield Br + H2O are presented. The measurements are verified by two techniques: one involved a 266-nm pulsed-laser photolysis of O3/H2O/HBr/He mixtures in conjunction with time-resolved resonance fluorescence detection of OH, the second comprised pulsed laser-induced fluorescence detection of OH following 248-nm pulsed-laser photolysis of H2O2/HBr/Ar mixtures. It is reported that k(1) = (11.9 + or -1.4 x 10 to the -12th (cu cm)/(molecule)(s) independent of temperature. The measurements are compared with other available results.

Ravishankara, A. R.↗

Time-resolved photoelectron imaging of complex resonances in molecular nitrogen

We have used the FERMI free-electron laser to perform time-resolved photoelectron imaging experiments on a complex group of resonances near 15.38 eV in the absorption spectrum of molecular nitrogen, N-2, under jet-cooled conditions. The new data complement and extend the earlier work of Fushitani et al. [Opt. Express 27, 19702-19711 (2019)], who recorded time-resolved photoelectron spectra for this same group of resonances. Time-dependent oscillations are observed in both the photoelectron yields and the photoelectron angular distributions, providing insight into the interactions among the resonant intermediate states. In addition, for most states, we observe an exponential decay of the photoelectron yield that depends on the ionic final state. This observation can be rationalized by the different lifetimes for the intermediate states contributing to a particular ionization channel. Finally, although there are nine resonances within the group, we show that by detecting individual photoelectron final states and their angular dependence, we can identify and differentiate quantum pathways within this complex system.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Single-frequency diode-pumped lasers for free-space optical communication

Recent advances in laser technology for intersatellite optical communication systems are reviewed and illustrated with graphs and diagrams. Topics addressed include (1) single-frequency diode-pumped Nd:YAG lasers of monolithic ring configuration (yielding 368-384 mW output power with 1-W pumping), (2) injection chaining of up to 10 monolithic resonators to achieve redundancy and/or higher output power, (3) 2-kHz-linewidth 5-mW versions of (1) which are tunable over a 30-MHz range for use as local oscillators in coherent communication, (4) resonant external modulation and doubling or resonant phase modulation of diode-pumped lasers, and (5) wavelength multiplexing.

Kane, Thomas J.↗

Resonant x-ray absorption of strong-field-ionized CF 3 Br

We report on an experimental and theoretical study of strong-field laser ionization of CF 3 Br followed by resonant x-ray absorption at the Br K-edge. Distinct 1s -> 4p, 5p Rydberg transitions of Br q+ (q = 1-4) atomic ions are observed and identified with Hartree-Fock-Slater and relativistic configuration interaction calculations. Time-dependent density functional theory and ab initio molecular dynamics calculations were performed to simulate the dissociative ionization process and the molecular orbitals for the q = 1-4 charge states. Measurements were made with both parallel and perpendicular linear polarizations of the laser and x-rays, but dichroism was not observed, indicating negligible alignment by the laser ionization process. This result is explained by calculations on atomic Br and the molecular simulation.

74 ATOMIC AND MOLECULAR PHYSICS↗

Lidar Measurements of Metallic Species in Mesopause Region

Sodium density distributions were measured over more than 20 nights since Jul. 1991 at Tokyo Metropolitan University. Our sodium lidar specifications are shown. The lidar consists of a dye laser that is pumped by a pulsed Nd:YAG laser. The dye laser is tuned to the D2 resonant absorption line of Na at the wavelength of 589 nm. A small fraction of the output beam is directed to a hollow-cathode lamp. The precise tuning of the Na D2 line is accomplished by monitoring the signal obtained from the hollow-cathode lamp and controlling the grating in the dye laser oscillator cavity. The raw data for each profile were obtained by firing the laser 5000 times for approximately 8.5 minutes. We have observed the sporadic sodium layers three times during the observation period. Recently, lidar measurements of iron atoms were also performed. Other aspects of this investigation are presented.

Nagasawa, Chikao↗

Electric-optic resonant phase modulator

An electro-optic resonant cavity is used to achieve phase modulation with lower driving voltages. Laser damage thresholds are inherently higher than with previously used integrated optics due to the utilization of bulk optics. Phase modulation is achieved at higher speeds with lower driving voltages than previously obtained with non-resonant electro-optic phase modulators. The instant scheme uses a data locking dither approach as opposed to the conventional sinusoidal locking schemes. In accordance with a disclosed embodiment, a resonant cavity modulator has been designed to operate at a data rate in excess of 100 Mbps. By carefully choosing the cavity finesse and its dimension, it is possible to control the pulse switching time to within 4 ns and to limit the required switching voltage to within 10 V. Experimentally, the resonant cavity can be maintained on resonance with respect to the input laser signal by monitoring the fluctuation of output intensity as the cavity is switched. This cavity locking scheme can be applied by using only the random data sequence, and without the need of additional dithering of the cavity. Compared to waveguide modulators, the resonant cavity has a comparable modulating voltage requirement. Because of its bulk geometry, resonant cavity modulator has the potential of accommodating higher throughput power. Furthermore, mode matching into a bulk device is easier and typically can be achieved with higher efficiency. On the other hand, unlike waveguide modulators which are essentially traveling wave devices, the resonant cavity modulator requires that the cavity be maintained in resonance with respect to the incoming laser signal. An additional control loop is incorporated into the modulator to maintain the cavity on resonance.

Chen, Chien-Chung↗

Ultra-narrow-linewidth hybrid-integrated self-injection locked laser at 780 nm

Narrow-linewidth lasers are essential across a wide range of applications, including classical and quantum sensing, trapped ion systems, position/navigation/timing systems, optical clocks, and microwave frequency synthesizers. In the visible and near-visible spectrum, low-noise lasers are particularly important for laser trapping and cooling techniques, which are vital for trapped ion quantum computing, sensing, and atomic clocks. In this context, our work showcases a hybrid-integrated narrow-linewidth laser that operates at 780 nm, achieving a self-heterodyne linewidth of 105 Hz. To validate the experimental results, we performed a numerical analysis that combines insights from a many-body theory applied to the gain region with a travelling-wave model to capture the laser dynamics. Our investigation further delves into how the linewidth of the self-injection locked lasers is influenced by the parameters of micro-ring resonators, aiming to assess the potential for achieving Hz-level integrated laser linewidths at 780 nm. This work not only demonstrates the technical feasibility of Hz-level narrow-linewidth lasers but also lays the groundwork for future explorations in the field.

Prokoshin, Artem (ORCID:0009000699760238)↗

Compact Dielectric-Rod White-Light Delay Lines

Optical delay lines of a proposed type would be made from rods of such dielectric materials as calcium fluoride, fused silica, or sapphire. These would offer advantages over prior optical delay lines, as summarized below. Optical delay lines are key components of opto-electronic microwave oscillators, narrow-band opto-electronic microwave filters, evanescent-field optical biochemical detectors, and some Fourier-Transform spectrum analyzers. Heretofore, optical delay lines used in such applications have been of two types: resonators and coiled long optical fibers, both of which have disadvantages: Resonators are compact, but excitation must be provided by narrow-band lasers. Wide-band (including noisy) laser light cannot be coupled efficiently to narrow-band resonators. When light is coupled into a narrowband resonator from a source of reasonably high power, a significant amount of optical energy circulates within the resonator, causing nonlinear loss and significant noise. Typically, a coil-type optical delay line is made of fused-silica fiber, which exhibits fundamental loss. To overcome the limit imposed by the optical loss in fused silica, it would be necessary to use fibers having crystalline cores. Although space is saved by winding fibers into coils, fiber-coil delay lines are still inconveniently bulky. The proposed compact dielectric-rod delay lines would exploit the special class of non-diffracting light beams that are denoted Bessel beams because their amplitudes are proportional to Bessel functions of the radii from their central axes. High-order Bessel beams can have large values of angular momentum. They can be generated with the help of whispering-gallery-mode optical resonators, as described, for example, in "Simplified Generation of High-Angular-Momentum Light Beams" (NPO-42965) NASA Tech Briefs, Vol. 31, No. 3 (March 2007), page 8a. In a delay line according to the proposal, the dielectric rod would be dimensioned to function as a multimode waveguide. Suitably chosen high-angular-momentum modes in such a waveguide exhibit low group velocity (hence, long delay) and no resonance. Such a delay line could perform well at any wavelength or range of wavelengths within the transparency wavelength band of the dielectric material, and the maximum possible group delay achievable through suitable design would be limited only by the optical loss in the rod material.

Maleki, Lute↗

Ponderomotive recoil for electromagnetic waves

When waves damp or amplify on resonant particles in a plasma, nonresonant particles experience a recoil force that conserves the total momentum between particles and electromagnetic fields. This force is important to understand, as it can completely negate current drive and rotation drive mechanisms that are predicted on the basis of only resonant particles. Here, the existing electrostatic theory of this recoil force is extended to electromagnetic waves. While the result bears close similarity to historical fluid theories of laser–plasma interactions, it now incorporates both resonant and nonresonant particles, allowing momentum conservation to be self-consistently proven. Furthermore, the result is shown to be generally valid for kinetic plasmas, which is verified through single-particle hot-plasma simulations. Here, the new form of the force provides physical insight into the nature of the generalized Minkowski (plasmon) momentum of geometrical optics, which is shown to correspond to the momentum gained by the field and nonresonant particles as the wave is self-consistently ramped up from vanishing amplitude.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Low temperature operation of an S2 laser using radio frequency simmer discharges

Technological problems stemming from high temperature operation of the sulfur resonator have hindered its development as a tunable, efficient, discharge pumped laser. The use of RF simmer discharges is shown to reduce previous temperature constraints by dissociating polyatomic sulfur molecules into the dimer, such that lasing is achieved when pumped by an XeCl excimer laser. The peak power output of the S2 laser and the transmission spectra through sulfur discharges are used to infer the effectiveness of the discharge in dissociating the vapor.

Killeen, K. P.↗

Nonequilibrium phonon tuning and mapping in few-layer graphene with infrared nanoscopy

Electron-phonon interactions are fundamentally important physical processes responsible for many key discoveries in condensed matter physics and material sciences. Herein, by exploiting the scattering-type scanning near-field optical microscope (s-SNOM) excited with a femtosecond infrared (IR) laser, we explored the strong coupling between IR phonons in few-layer graphene (FLG) with ultrahot electrons, which are heated up by the intense laser field enhanced by the s-SNOM tip. More specifically, we found that the intensity of the phonon resonance can be tuned systematically by varying the laser power that controls the electron temperature. Furthermore, the high spatial resolution of s-SNOM allows us to map the local phonon characteristics at sharp boundaries and nanostructures. Our results offer insights into the intriguing physics behind the electron-phonon interactions in nonequilibrium conditions and open a pathway for manipulating phonons with optical means.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Open-Access, Low-Magnetic-Field MRI System for Lung Research

An open-access magnetic resonance imaging (MRI) system is being developed for use in research on orientational/gravitational effects on lung physiology and function. The open-access geometry enables study of human subjects in diverse orientations. This system operates at a magnetic flux density, considerably smaller than the flux densities of typical other MRI systems, that can be generated by resistive electromagnet coils (instead of the more-expensive superconducting coils of the other systems). The human subject inhales air containing He-3 or Xe-129 atoms, the nuclear spins of which have been polarized by use of a laser beam to obtain a magnetic resonance that enables high-resolution gas space imaging at the low applied magnetic field. The system includes a bi-planar, constant-current, four-coil electromagnet assembly and associated electronic circuitry to apply a static magnetic field of 6.5 mT throughout the lung volume; planar coils and associated circuitry to apply a pulsed magnetic-field-gradient for each spatial dimension; a single, detachable radio-frequency coil and associated circuitry for inducing and detecting MRI signals; a table for supporting a horizontal subject; and electromagnetic shielding surrounding the electromagnet coils.

Mair, Ross W.↗

Diode laser 87Rb optical pumping in an evacuated wall-coated cell

The evacuated wall coated sealed cell coupled with diode laser optical pumping offers a number of attractive potential advantages for use in Rb or Cs atomic frequency standards. An investigation of systematic effects is required to explore possible limitations of the technique. The use of diode laser optical pumping of 87 Rb in an evacuated wall coated sealed cell is presented. Experimental results/discussion to be presented include the signal strength and line broadening of the 0 - 0 hyperfine resonance as a function of light intensity for the D1 optical transitions (F - F prime) - (2 1 prime) and (2 - 2 prime), shift of the 0 - 0 hyperfine frequency as a function of laser intensity and de-tuning from optical resonance, and diode laser frequency stabilization techniques.

Lee, W. K.↗

Modeling of THz Lasers Based on Intersubband Transitions in Semiconductor Quantum Wells

In semiconductor quantum well structures, the intersubband energy separation can be adjusted to the terahertz (THz) frequency range by changing the well width and material combinations. The electronic and optical properties of these nanostructures can also be controlled by an applied dc electric field. These unique features lead to a large frequency tunability of the quantum well devices. In the on-going project of modeling of the THz lasers, we investigate the possibility of using optical pumping to generate THz radiation based on intersubband transitions in semiconductor quantum wells. We choose the optical pumping because in the electric current injection it is difficult to realize population inversion in the THz frequency range due to the small intersubband separation (4-40 meV). We considered both small conduction band offset (GaAs/AlGaAs) and large band offset (InGaAs/AlAsSb) quantum well structures. For GaAs/AlGaAs quantum wells, mid-infrared C02 lasers are used as pumping sources. For InGaAs/AlAsSb quantum wells, the resonant intersubband transitions can be excited by the near-infrared diode lasers. For three- and four-subband quantum wells, we solve the pumpfield-induced nonequilibrium distribution function for each subband of the quantum well system from a set of rate equations that include both intrasubband and intersubband relaxation processes. Taking into account the coherent interactions between pump and THz (signal) waves, we calculate the optical gain for the THz field. The gain arising from population inversion and stimulated Raman processes is calculated in a unified manner. A graph shows the calculated THz gain spectra for three-subband GaAs/AlGaAs quantum wells. We see that the coherent pump and signal wave interactions contribute significantly to the gain. The pump intensity dependence of the THz gain is also studied. The calculated results are shown. Because of the optical Stark effect and pump-induced population redistribution, the maximum THz gain saturates at larger pump intensities.

Liu, Ansheng↗

Resonance ionization of zirconium

Abstract Measuring the isotopic composition of trace Zr in presolar stardust grains allows us to study the environment of slow neutron-capture nucleosynthesis in asymptotic giant branch stars. Here, we present a newly characterized Zr resonance ionization scheme that can be saturated with state-of-the-art titanium-sapphire lasers and yields a useful yield of (5.4 ± 0.4)%. Resonance ionization is achieved in two steps: after first being excited with a photon at 319.215 nm, neutral Zr atoms are then ionized with a photon at 388.988 nm, where both wavelengths are reported as in vacuum.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗