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At least 397 records · Page 22

Eclipse mapping of the accreting magnetic white dwarf in DP Leonis with HST

We present time-resolved ultraviolet spectrophotometry of the AM Her system DP Leo (E1114+182), obtained with the Faint Object Spectrograph on the Hubble Space Telescope (HST) in 1991 October. During this period, the binary was in a low-activity state. Complementary optical spectrophotometry and spectopolarimetry were obtained in 1991 October and December, as well as in 1992 April when the object had entered a high-accretion state. The HST spectrophotometry reveals two UV-emitting components-a hot 'spot' (T approximately 50,000 K, very approximately) near the magnetic pole into which most material is accreted, and the white dwarf photosphere (T approximately 16,000 K), which dominates when the spot is not in view. Both components appear as rapid and gradual components in the ingress and egress of secondary eclipse, the latter indicating a normal white dwarf radius of 0.8 x 10(exp 9) cm. The fractional area of the spot (f approximately 0.006) implied by the eclipse data is consistent with the observed UV flux and a minimum distance of 380 pc is similar to those found in other AM Her systems. The nearly identical eclipse light curves from the HST and earlier optical observations imply that the UV-emitting reprocessing area is not more extended than the cyclotron source of optical radiation in the accretion funnel. The timing of the onset of the bright phase indicated that the spot leads the secondary in orbital azimuth by approximately 3 deg.

Stockman, H. S.↗

Assessment of SNPP VIIRS RSB detector-to-detector differences using deep convective clouds and deserts

An accurate on-orbit characterization of the Visible Infrared Imaging Radiometer Suite (VIIRS) onboard the Suomi National Polar-orbiting Partnership satellite is essential to satisfy the requirements from NOAA, NASA, and the general research community for high-quality operational and research products. NASA’s Land Science Investigator-led Processing System (LSIPS) sensor data records (SDRs) are utilized to assess the stability of the calibrated top of atmosphere reflectance over the deep convective clouds (DCCs) and over the Libya-4desert site. The results from DCCs and desert show detector-to-detector (D2D) reflectance differences in the VIIRS reflective solar bands, 10 moderate-resolution bands (M-bands, M1to M5, M7 to M11), and three imagery resolution bands (I-bands, I1-I3). More importantly, the D2D differences exhibit an increase in magnitude over time for bands M1 to M5 and I1to I2, which induces noticeable striping and higher uncertainties in the downstream data products. The largest D2D difference is observed in bands M1 and M2, with magnitudes greater than1.8% in trends among the 16 detectors and standard deviations less than 0.12% over time. TheD2D stability assessment results over DCCs are consistent with those observed over the Libya-4desert site. To improve the quality of the calibrated SDR reflectance data, NASA’s VIIRS characterization support team has improved the calibration algorithm to incorporate corrections based on these DCC measurements to mitigate the striping (detector differences) observed in the current version of the SDR. These improvements are planned to be included in the next mission reprocessing of the LSIPS land products.

SNPP VIIRS↗

Heading Toward Launch with the Integrated Multi-Satellite Retrievals for GPM (IMERG)

The Day-l algorithm for computing combined precipitation estimates in GPM is the Integrated Multi-satellitE Retrievals for GPM (IMERG). We plan for the period of record to encompass both the TRMM and GPM eras, and the coverage to extend to fully global as experience is gained in the difficult high-latitude environment. IMERG is being developed as a unified U.S. algorithm that takes advantage of strengths in the three groups that are contributing expertise: 1) the TRMM Multi-satellite Precipitation Analysis (TMPA), which addresses inter-satellite calibration of precipitation estimates and monthly scale combination of satellite and gauge analyses; 2) the CPC Morphing algorithm with Kalman Filtering (KF-CMORPH), which provides quality-weighted time interpolation of precipitation patterns following cloud motion; and 3) the Precipitation Estimation from Remotely Sensed Information using Artificial Neural Networks using a Cloud Classification System (PERSIANN-CCS), which provides a neural-network-based scheme for generating microwave-calibrated precipitation estimates from geosynchronous infrared brightness temperatures. In this talk we summarize the major building blocks and important design issues driven by user needs and practical data issues. One concept being pioneered by the IMERG team is that the code system should produce estimates for the same time period but at different latencies to support the requirements of different groups of users. Another user requirement is that all these runs must be reprocessed as new IMERG versions are introduced. IMERG's status at meeting time will be summarized, and the processing scenario in the transition from TRMM to GPM will be laid out. Initially, IMERG will be run with TRMM-based calibration, and then a conversion to a GPM-based calibration will be employed after the GPM sensor products are validated. A complete reprocessing will be computed, which will complete the transition from TMPA.

Huffman, George J.↗

Fault Detection in the Solvent Extraction Process with Non-traditional Sensors

Solvent extraction is used to separate metals or other complexes into two different immiscible liquids and is an essential component of the PUREX Process. Improvements to the solvent extraction process can directly contribute to an organization’s ability to ensure the purity and recovery of special nuclear materials from spent nuclear fuel. Such improvements can benefit nuclear reprocessing efforts, increase fuel reutilization, and limit the concentration of actinides in nuclear waste repositories.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

'Spherical' disks: Moving toward a unified source model for L1551

To predict the effects of a disk on the spectral energy distribution of a deeply embedded protostar, we construct disk models with power-law temperature distributions T is proportional to r(exp -q). We then use the spherically averaged disk emission as the central source for a spherical envelope, hence the term, 'spherical' disk. We then calculate the predicted spectral energy distribution of the disk and envelope, using a spherically symmetric radiative transport code. Applying this procedure to L1551 IRS 5, we find that the predicted far-infrared flux is not very sensitive to the nature of the central source. The best source model is consistent with the far-infrared emission arising from the infalling region in an 'inside-out' collapse model, independent of the nature of the central source. Disk models are superior to the star-only model when we try to match millimeter interferometer data. While disks with various q can reproduce the observed 2.7 mm interferometer flux, only an active disk (q = 0.5) can produce enough emission in a region small enough to match the observed 2.7 mm visibilities. However, if the disk is backwarmed by the envelope, even purely reprocessing disks can meet this constraint. All types of backwarmed disks are virtually in distinguishable in their millimeter properties. We find that all reasonable envelope models are sufficiently opaque in the mid-infrared to attenuate any disk model to a level well below the observations, unless the ratio of the mid-infrared to far-infrared dust opacities is similar to that of the dust opacities advocated by Mathis, Mezger, & Panagia (1983).

Butner, Harold M.↗

Predicting the X-Ray Spectra of Stellar-mass Black Holes from Simulations

We describe results from a new technique for the prediction of complete, self-consistent X-ray spectra from three-dimensional general relativistic magnetohydrodynamic (GRMHD) simulations of black hole accretion flows. Density and cooling rate data from a harm3d GRMHD simulation are post-processed by an improved version of the Monte Carlo radiation transport code pandurata (in the corona) and the Feautrier solver PTRANSX (in the disk), with xstar subroutines. The codes are run in a sequential, iterative fashion to achieve globally energy-conserving and self-consistent radiation fields, temperature maps, and photoionization equilibria. The output is the X-ray spectrum as seen by a distant observer, including features, such as the Fe Kα emission line and corresponding K-edge absorption trough, due to disk reprocessing of coronal power. For the example cases we consider—a non-rotating 10 M(sub ⊙) black hole with solar abundances, accreting at 0.01, 0.03, 0.1, or 0.3 Eddington—we find spectra resembling actual observations of stellar-mass black holes in the soft or steep power-law state: broad thermal peaks (at 1–3 keV), steep power laws extending to high energy (Γ = 2.7–4.5), and prominent, asymmetric Fe Kα emission lines with equivalent widths in the range 40–400 eV (larger EW at lower accretion rates). By starting with simulation data, we obviate the need for parameterized descriptions of the accretion flow geometry—no a priori specification of the corona's shape or flux, or the disk temperature or density, etc., is needed. Instead, we apply the relevant physical principles to simulation output using appropriate numerical techniques; this procedure allows us to calculate inclination-dependent spectra after choosing only a small number of physically meaningful parameters: black hole mass and spin, accretion rate, and elemental abundances.

Kinch, Brooks E.↗

Status and Plans for the WCRP/GEWEX Global Precipitation Climatology Project (GPCP)

The Global Precipitation Climatology Project (GPCP) is an international project under the auspices of the World Climate Research Program (WCRP) and GEWEX (Global Water and Energy Experiment). The GPCP group consists of scientists from agencies and universities in various countries that work together to produce a set of global precipitation analyses at time scales of monthly, pentad, and daily. The status of the current products will be briefly summarized, focusing on the monthly analysis. Global and large regional rainfall variations and possible long-term changes are examined using the 27-year (1 979-2005) monthly dataset. In addition to global patterns associated with phenomena such as ENSO, the data set is explored for evidence of long-term change. Although the global change of precipitation in the data set is near zero, the data set does indicate a small upward change in the Tropics (25s-25N) during the period,. especially over ocean. Techniques are derived to isolate and eliminate variations due to ENS0 and major volcanic eruptions and the significance of the linear change is examined. Plans for a GPCP reprocessing for a Version 3 of products, potentially including a fine-time resolution product will be discussed. Current and future links to IPWG will also be addressed.

Adler, Robert F.↗

X-ray Absorption Spectroscopy Investigation of Iodine Capture by Silver-Exchanged Mordenite

Capture of radioactive iodine is a significant consideration during reprocessing of spent nuclear fuel and disposal of legacy wastes. While silver-exchanged mordenite (AgZ) is widely regarded as a benchmark material for assessing iodine adsorption performance, previous research efforts have largely focused on bulk material properties rather than the underpinning molecular interactions that achieve effective iodine capture. As a result, the fundamental understanding necessary to identify and mitigate deactivation pathways for the recycle of AgZ is not available. In this paper, we applied X-ray Absorption Fine Structure (XAFS) spectroscopy to investigate AgZ following activation, adsorption of iodine, regeneration, and recycle, observing no appreciable degradation in performance due to the highly controlled conditions under which the AgZ was maintained. Fits of the extended XAFS (EXAFS) data reveal complete formation of Ag 0 nanoparticles upon treatment with H 2 , and confirm the formation of α-AgI within the mordenite channels in addition to surface γ/β-AgI nanoparticles following iodine exposure. Analysis of the nanoparticle size and fractional composition of α-AgI to γ/β-AgI supports ripening of surface nanoparticles as a function of recycle. Finally, this work provides a foundation for future investigation of AgZ deactivation under conditions relevant to spent nuclear fuel reprocessing.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A Decade of MWC 758 Disk Images: Where are the Spiral-Arm-Driving Planets?

Large-scale spiral arms have been revealed in scattered light images of a few protoplanetary disks. Theoretical models suggest that such arms may be driven by and corotate with giant planets, which has called for remarkable observational efforts to look for them. By examining the rotation of the spiral arms for the MWC 758 system over a 10 year timescale, we are able to provide dynamical constraints on the locations of their perturbers. We present reprocessed Hubble Space Telescope (HST)/NICMOS F110W observations of the target in 2005, and the new Keck/NIRC2 L'-band observations in 2017. MWC 758's two well-known spiral arms are revealed in the NICMOS archive at the earliest observational epoch. With additional Very Large Telescope (VLT)/SPHERE data, our joint analysis leads to a pattern speed of 0.°6(sup +3.°3, sub -0.°6)/yr at 3σ for the two major spiral arms. If the two arms are induced by a perturber on a near-circular orbit, its best-fit orbit is at 89 au (0."59), with a 3σ lower limit of 30 au (0."20). This finding is consistent with the simulation prediction of the location of an arm-driving planet for the two major arms in the system.

MWC 758↗

Retrievals of Aerosol Optical Depth and Spectral Absorption from DSCOVR EPIC

A new algorithm is described for joint retrievals of the aerosol optical depth and spectral absorption from EPIC observations in the UV—Vis spectral range. The retrievals are illustrated on examples of the wildfire smoke events over North America, and dust storms over greater Sahara region in 2018. An initial evaluation of single scattering albedo (SSA) at 443 nm over these regions shows a good agreement with AERONET data, generally within the uncertainty of AERONET SSA of ± 0.03. A particularly good agreement is achieved for dust with R∼0.62, rmse∼0.02, negligible bias, and 85% points within the expected error. This new capability is part of version 2 MAIAC EPIC algorithm. The v2 algorithm has recently completed reprocessing of the EPIC record covering the period of 2015–2020.

EPIC↗

A search for evolutionary changes in planetary nuclei: A continuation

This report summarizes the final results of an IUE investigation to search for signs of evolutionary changes in high-mass central stars of planetary nuclei, as evidenced by UV-optical fading over the lifetime of the satellite. The program is a continuation of an earlier investigation, expanding the target list to include more types of hot central stars and to obtain more spectra of previously observed stars. In order to compare the IUE fluxes of a central star obtained over a more-than-ten-year timespan, several steps were necessary, including reprocessing of very early spectra and correction for the sensitivity degradation of the SWP camera over time. The results indicate that while a few stars appear to have diminished UV fluxes compared to earlier IUE observations, the evidence for this is less than overwhelming due to the sparseness of the data. Those stars which emerge from this study as viable candidates for having faded are the cooler Of-type stars (O6f-O7f), i.e., those for which the change in spectral energy with increasing temperature is greatest. The report describes the data analysis steps and discusses the uncertainties in both the data and in the resulting fading rates. Estimates of stellar mass based on theoretical evolutionary rates are also provided.

Altner, Bruce↗

Climate and Lightning: An updated TRMM-LIS Analysis

The TRMM Lightning Imaging Sensor (LIS) has sampled global tropical and sub-tropical lightning flash densities for approximately 11 years. These data were originally processed and results presented by the authors in the 3rd AMS MALD Conference held in 2007 using both pre and post TRMM-boost lightning data. These data were normalized for the orbit boost by scaling the pre-boost data by a fixed constant based on the different swath areas for the pre and post-boost years (post-boost after 2001). Inevitably, one must question this simple approach to accounting for the orbit boost when sampling such a noisy quantity. Hence we are in the process of reprocessing the entire 11-year TRMM LIS dataset to reduce the orbit swath of the post-boost era to that of the pre-boost in order to eliminate sampling bias in the dataset. Study of the diurnal/seasonal/annual sampling suggests that those biases are already minimal and should not contribute to error in examination of annual trends. We will present new analysis of the 11-year annual trends in total lightning flash density for all latitudinal belts and select regions/regimes of the tropics as related to conventional climate signals and precipitation contents in the same period. The results should enable us to address, in some fashion, the sensitivity of the lightning flash density to subtle changes in climate.

Petersen, Walter A.↗

The calculation of light element impurity (α, n) yield curves in a PuO 2 matrix and associated specific yield coefficients: Influence of the reaction cross sections

Most of the Pu separated from irradiated commercial nuclear fuel is stored as PuO 2 . The primary quantitative nondestructive measurement technique used to verify the amount of Pu in storage containers is passive neutron correlation counting. An important physical property of the oxide material is the ratio, α, of the rate of (α, n) neutrons produced inside the item to the rate of neutrons produced by spontaneous fission. This ratio influences the precision of the correlated counting method and affects the interpretation of the data because of how it changes both the primary total neutron production rate and the rate of induced fission events taking place inside the item. In addition to the main O(α, n) contribution, additional contributions come from α-particle interactions with light element impurities that are inevitably present. In this work, we calculate specific (α, n) yield coefficients, expressed in units of neutrons per second per gram of α-emitting nuclide per part per million by mass of the specified impurity element distributed in a pure PuO 2 matrix, for some key α-emitting actinides commonly present in reprocessed Pu ( 238–242 Pu+ 241 Am). These coefficients are directly applicable to nuclear safeguards verification work in which the α ratio is often calculated from the Pu-isotopic composition and chemical information obtained by other means. Further, they also provide a convenient up-to-date reference set against which values generated by other methods can be compared. Results are presented for impurities with atomic number from 3 to 17 inclusive, plus K and Fe. In most cases, these coefficients are not expected to change by more than 5%–10% at any time in the future. However, as new data become available, changes as large as 20% may be needed for some targets (e.g., F). The present yield calculations are limited by the general shortage of quality experimental total (α, n) reaction cross section data, which, together with unexplained variation between determinations, means that an objective and coherent evaluation is not possible. The situation is even less satisfactory for the partial differential cross section needed to calculate neutron spectra.

(𝛼, n) reactions↗

Spectroscopic Characterization of Aqua [ fac -Tc(CO) 3 ] + Complexes at High Ionic Strength

Understanding fundamental Tc chemistry is important to both the remediation of nuclear waste and the reprocessing of nuclear fuel; however, current knowledge of the electronic structure and spectral signatures of low-valent Tc compounds significantly lags behind the remainder of the d-block elements. In particular, identification and treatment of Tc speciation in legacy nuclear waste is challenging due to the lack of reference data especially for Tc compounds in the less common oxidation states (I–VI). In an effort to establish a spectroscopic library corresponding to the relevant conditions of extremely high ionic strength typical for the legacy nuclear waste, compounds with the general formula of [ fac -Tc(CO) 3 (OH 2 ) 3– n (OH) n ] 1– n (where n = 0–3) were examined by a range of spectroscopic techniques including 99 Tc/ 13 C NMR, IR, XPS, and XAS. In the series of monomeric aqua species, stepwise hydrolysis results in the increase of the Tc metal center electron density and corresponding progressive decrease of the Tc–C bond distances, Tc electron binding energies, and carbonyl stretching frequencies in the order [ fac -Tc(CO) 3 (OH 2 ) 3 ] > [ fac -Tc(CO) 3 (OH 2 ) 2 (OH)] > [ fac -Tc(CO) 3 (OH 2 )(OH) 2 ] – . These results correlate with established trends of the 99 Tc upfield chemical shift and carbonyl 13 C downfield chemical shift. The lone exception is [ fac -Tc(CO) 3 (OH)] 4 which exhibits a comparatively low electron density at the metal center attributed to the μ 3 -bridging nature of the –OH ligands causing less σ-donation and no π-donation. As a result, this work also reports the first observations of these compounds by XPS and [ fac -Tc(CO) 3 Cl 3 ] 2– by XAS. The unique and distinguishable spectral features of the aqua [ fac -Tc(CO) 3 ] + complexes lay the foundation for their identification in the complex aqueous matrixes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Fe kα profiles from simulations of accreting black holes

We present the first results from a new technique for the prediction of Fe Kα profiles directly from general relativistic magnetohydrodynamic (GRMHD) simulations. Data from a GRMHD simulation are processed by a Monte Carlo global radiation transport code, which determines the X-ray flux irradiating the disk surface and the coronal electron temperature self-consistently. With that irradiating flux and the disk’s density structure drawn from the simulation, we determine the reprocessed Fe Kα emission from photoionization equilibrium and solution of the radiation transfer equation. We produce maps of the surface brightness of Fe Kα emission over the disk surface, which—for our example of a 10M{sub ⊙} Schwarzschild black hole accreting at 1% the Eddington value—rises steeply one gravitational radius outside the radius of the innermost stable circular orbit and then falls ∝r {sup −2} at larger radii. We explain these features of the Fe Kα radial surface brightness profile as consequences of the disk’s ionization structure and an extended coronal geometry, respectively. We also present the corresponding Fe Kα line profiles as would be seen by distant observers at several inclinations. Both the shapes of the line profiles and the equivalent widths of our predicted Kα lines are qualitatively similar to those typically observed from accreting black holes. Most importantly, this work represents a direct link between theory and observation: in a fully self-consistent way, we produce observable results—iron fluorescence line profiles—from the theory of black hole accretion with almost no phenomenological assumptions.

79 ASTRONOMY AND ASTROPHYSICS↗

Development of an Operational Land Water Mask for MODIS Collection 6, and Influence on Downstream Data Products

Data from the Moderate Resolution Imaging Spectro-radiometer (MODIS)on-board the Earth Observing System Terra and Aqua satellites are processed using a land water mask to determine when an algorithm no longer needs to be run or when an algorithm needs to follow a different pathway. Entering the fourth reprocessing (Collection 6 (C6)) the MODIS team replaced the 1 km water mask with a 500 m water mask for improved representation of the continental surfaces. The new water mask represents more small water bodies for an overall increase in water surface from 1 to 2 of the continental surface. While this is still a small fraction of the overall global surface area the increase is more dramatic in certain areas such as the Arctic and Boreal regions where there are dramatic increases in water surface area in the new mask. MODIS products generated by the on-going C6 reprocessing using the new land water mask show significant impact in areas with high concentrations of change in the land water mask. Here differences between the Collection 5 (C5) and C6 water masks and the impact of these differences on the MOD04 aerosol product and the MOD11 land surface temperature product are shown.

Carroll, M. L.↗

Partial defect verification of spent fuel assemblies by PDET: Principle and field testing in Interim Spent fuel Storage Facility (CLAB) in Sweden

Here, the need for the development of a credible method and instrument for partial defect verification of spent fuel has been emphasized over a few decades in the safeguards communities as the diverted spent fuel pins can be the source of nuclear terrorism or devices. The need is increasingly more important and even urgent as many countries have started to transfer spent fuel to so called "difficult-to-access" areas such as dry storage casks, reprocessing or geological repositories. Partial defect verification is required by IAEA before spent fuel is placed into "difficult-to-access" areas. Earlier, Lawrence Livermore National Laboratory (LLNL) has reported the successful development of a new, credible partial defect verification method for pressurized water reactor (PWR) spent fuel assemblies without use of operator data, and further reported the validation experiments using commercial spent fuel assemblies with some missing fuel pins. The method was found to be robust as the method is relatively invariant to the characteristic variations of spent fuel assemblies such as initial fuel enrichment, cooling time, and burn-up. Since then, the PDET system has been designed and prototyped for 17×17 PWR spent fuel assemblies, complete with data acquisition software and acquisition electronics. In this paper, a summary description of the PDET development followed by results of the first successful field testing using the integrated PDET system and actual spent fuel assemblies performed in a commercial spent fuel storage site, known as Central Interim Spent fuel Storage Facility (CLAB) in Sweden will be presented. In addition to partial defect detection initial studies have determined that the tool can be used to verify the operator declared average burnup of the assembly as well as intra-assembly bunrup levels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Assembly and Testing of a Tritium and Iodine Removal System for Use with Advanced Tritium Pretreatment

US regulations will require the removal of iodine and tritium, along with other volatile and semivolatile radionuclides, from the off-gas streams of nuclear fuel reprocessing plants. Tritium pretreatment is a head-end operation that could be incorporated within nuclear fuel reprocessing plants for the upfront removal and trapping of these volatiles species. Quantitative, up-front removal in a single compact system is of significant advantage because otherwise tritium and iodine distributes to other unit operations, each of which have associated off-gas streams also requiring treatment. Oak Ridge National Laboratory is presently developing an advanced tritium pretreatment process based on the oxidation of used nuclear fuel at low temperature using NO 2 /O 2 mixtures, which produces a fine powder. This process can result in the quantitative volatilization of both tritium and iodine. The powder product can be selected to be U 3 O 8 , UO 3 , or a nitrate by adjusting the processing conditions and the process can be readily interfaced to either conventional aqueous-based or advanced pyrochemical–based reprocessing plants. In preparation for a planned kilogram-scale hot cell demonstration of the advanced tritium pretreatment process with used nuclear fuel (UNF), an integrated iodine and tritium capture system was designed and assembled. Three experimental runs of this system were completed successfully. All the samples were submitted for analysis. The results and data analysis will be covered in a subsequent report to be issued by the Off-Gas Sigma Team. Several additional tests should be undertaken to provide additional information on the system’s performance. The objectives for the additional tests and test conditions are presented in this report.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗