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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 397 records · Page 22
All sourcesNASA NTRSDOE OSTI
NASA NTRS2016

The Mapping X-Ray Fluorescence Spectrometer (MAPX)

MapX will provide elemental imaging at ≤100 micron spatial resolution over 2.5 X 2.5 centimeter areas, yielding elemental chemistry at or below the scale length where many relict physical, chemical, and biological features can be imaged and interpreted in ancient rocks. MapX is a full-frame spectroscopic imager positioned on soil or regolith with touch sensors. During an analysis, an X-ray source (tube or radioisotope) bombards the sample surface with X-rays or αlpha-particles / gamma rays, resulting in sample X-ray Fluorescence (XRF). Fluoresced X-rays pass through an X-ray lens (X-ray μ-Pore Optic, "MPO") that projects a spatially resolved image of the X-rays onto a CCD. The CCD is operated in single photon counting mode so that the positions and energies of individual photons are retained. In a single analysis, several thousand frames are stored and processed. A MapX experiment provides elemental maps having a spatial resolution of ≤100 micron and quantitative XRF spectra from Regions of Interest (ROI) 2 centimers ≤ x ≤ 100 micron. ROI are compared with known rock and mineral compositions to extrapolate the data to rock types and putative mineralogies. The MapX geometry is being refined with ray-tracing simulations and with synchrotron experiments at SLAC. Source requirements are being determined through Monte Carlo modeling and experiment using XMIMSIM [1], GEANT4 [2] and PyMca [3] and a dedicated XRF test fixture. A flow-down of requirements for both tube and radioisotope sources is being developed from these experiments. In addition to Mars lander and rover missions, MapX could be used for landed science on other airless bodies (Phobos/Deimos, Comet nucleus, asteroids, the Earth's moon, and the icy satellites of the outer planets, including Europa.

Blake, David↗
DOE OSTI2023

Laser Characterization of Optically Smooth BREAD parts

The Broadband Reflector Experiment for Axion Detection is a dish antenna experiment probing the axion and dark photon parameter space in the [1 μeV, 1 eV] mass range, or [.02, 200] THz frequency range. In the pilot design for the InfraBREAD model, the dish antenna includes an optically smooth coaxial parabolic reflector to focus incoming photons in the near Infrared spectrum, created by the spontaneous photoconversion of axions and dark photons, onto a Superconducting Nanowire Single Photon Detector at the focus point of the reflector. As the pilot begins as a dark photon detector, sensitivity estimates hypothesize that it could cover unprobed parameter space in the search for the dark photon. Because of this, it is of critical importance that the reflector and SNSPD be placed at the correct points in the dish antenna, as previous work has shown that in addition to the focal spot of the photons being smeared to an area larger than the SNSPD, detection efficiency is s ensitive to shifts on the millimeter scale. In order to constrain this barrier to efficiency, the reflector had its focal spot, roughness, and length of surface waves measured by lasers in an optical bench setup. Results show the focal point diverging slightly from its theorized position in the antenna, while uncertainty in the height at which the detector should be placed was constrained to 10s of microns, the uncertainty in radial position could not be constrained to smaller than the detector given the methods used. Results for the roughness and surface wavelength show that the reflector was uniformly machined in a diamond-turning process used to fabricate optically smooth parts, as well as support a roughly 90% detection efficiency, reinforcing the sensitivity estimates presented.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Sub-threshold ultrafast one-photon photoemission from a Cu(111) photocathode

Single-photon photoemission of electrons for incident photon energies below the surface work function is reported for a single-crystal Cu(111) photocathode. Spectral characterization of the quantum efficiency and mean transverse energy of the emitted electrons is shown to be consistent with emission from a thermalized hot electron distribution photoexcited on sub-picosecond time scales into an upper conduction band at the L-point of the Brillouin zone of copper. To our knowledge, this is the first time that such excited-state thermionic emission has been observed from a planar metal photocathode, and then from a commonly used photocathode material. The results, therefore, indicate the potential importance of such band structure dependent sub-threshold photoemission mechanisms on the performance of photocathodes employed for the generation of short electron pulses using sub-picosecond laser pulses. Consequently, the combined experimental and theoretical work presented in this paper contributes to solid-state photocathode-based research aimed at our understanding and selection (or discovery) of high brightness photo-electron sources required for many electron-based diffraction, imaging, and accelerator applications.

43 PARTICLE ACCELERATORS↗
NASA NTRS2019

Real Time Photon-Counting Receiver for High Photon Efficiency Optical Communications

We present a scalable design for a photon-counting ground receiver based on superconducting nanowire single photon detectors (SNSPDs) and field programmable gate array (FPGA) real-time processing for applications to space-to-ground photon starved links, such as the Orion EM-2 Optical Communication Demonstration (O2O), and future deep space or low transmitter power missions. The receiver is designed to receive a serially concatenated pulse position modulation (SCPPM) waveform, which follows the Consultative Committee for Space Data Systems (CCSDS) Optical Communications Coding and Synchronization Red Book standard. The receiver design uses multiple individually fiber coupled, 80% detection efficiency commercial SNSPDs in parallel to scale to a required data rate, and is capable of achieving data rates up to 528 Mbps. For efficient fiber coupling from the telescope to the array of parallel detectors that can be scaled both to telescope aperture size and the number of detectors, we use either a single mode fiber (SMF) photonic lantern or a few-mode fiber (FMF) photonic lantern. In this paper we give an overview of the receiver system design, the characteristics of the photonic lanterns, the performance of the SNSPDs, and system level tests. We show that 40 Mbps can be received using a single SNSPD, and discuss aspects for scaling to higher data rates.

Vyhnalek, Brian E.↗
NASA NTRS2019

Real Time Photon-Counting Receiver for High Photon Efficiency Optical Communications

We present a scalable design for a photon-counting ground receiver based on superconducting nanowire single photon detectors (SNSPDs) and field programmable gate array (FPGA) real-time processing for applications to space-to-ground photon starved links, such as the Orion EM-2 Optical Communication Demonstration (O2O), and future deep space or low transmitter power missions. The receiver is designed to receive a serially concatenated pulse position modulation (SCPPM) waveform, which follows the Consultative Committee for Space Data Systems (CCSDS) Optical Communications Coding and Synchronization Red Book standard. The receiver design uses multiple individually fiber coupled, 80% detection efficiency commercial SNSPDs in parallel to scale to a required data rate, and is capable of achieving data rates up to 528 Mbps. For efficient fiber coupling from the telescope to the array of parallel detectors that can be scaled both to telescope aperture size and the number of detectors, we use either a single mode fiber (SMF) photonic lantern or a few-mode fiber (FMF) photonic lantern. In this paper we give an overview of the receiver system design, the characteristics of the photonic lanterns, the performance of the SNSPDs, and system level tests. We show that 40 Mbps can be received using a single SNSPD, and discuss aspects for scaling to higher data rates.

Vyhnalek, Brian E.↗
DOE OSTI2021

Enhanced Emission from Bright Excitons in Asymmetrically Strained Colloidal CdSe/Cd x Zn 1– x Se Quantum Dots

Colloidal CdSe quantum dots (QDs) designed with a high degree of asymmetric internal strain have recently been shown to host a number of desirable optical properties including subthermal room-temperature line widths, suppressed spectral diffusion, and high photoluminescence (PL) quantum yields. It remains an open question, however, whether they are well-suited for applications requiring emission of identical single photons. Here we measure the low-temperature PL dynamics and the polarization-resolved fluorescence line narrowing spectra from ensembles of these strained QDs. Our spectroscopy reveals the radiative recombination rates of bright and dark excitons, the relaxation rate between the two, and the energy spectra of the quantized acoustic phonons in the QDs that can contribute to relaxation processes. In comparison to conventional colloidal CdSe/ZnS core/shell QDs, we find that in asymmetrically strained CdSe QDs over six times more light is emitted directly by the bright exciton. Furthermore, these results are therefore encouraging for the prospects of chemically synthesized colloidal QDs as emitters of single indistinguishable photons.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Designing high-power, octave spanning entangled photon sources for quantum spectroscopy

Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and temporal-frequency resolutions, increased cross sections for multiphoton and nonlinear measurements, and new abilities in inducing or measuring quantum correlations. A critical step in enabling entangled photon spectroscopies is the creation of high-flux entangled sources that can use conventional detectors as well as provide redundancy for the losses in realistic samples. Here, we report a periodically poled, chirped, lithium tantalate platform that generates entangled photon pairs with ~10 -7 efficiency. For a near watt level diode laser, this results in a near μW-level flux. The single photon per mode limit that is necessary to maintain non-classical photon behavior is still satisfied by distributing this power over up to an octave-spanning bandwidth. The spectral–temporal photon correlations are observed via a Michelson-type interferometer that measures the broadband Hong–Ou–Mandel two-photon interference. A coherence time of 245 fs for a 10 nm bandwidth in the collinear case and a coherence time of 62 fs for a 125 nm bandwidth in the non-collinear case are measured using a CW pump laser and, essentially, collecting the full photon cone. We outline in detail the numerical methods used for designing and tailoring the entangled photons source, such as changing center wavelength or bandwidth, with the ultimate aim of increasing the availability of high-flux UV–Vis entangled photon sources in the optical spectroscopy community.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Photonic Curing of Nickel Oxide Transport Layer and Perovskite Active Layer for Flexible Perovskite Solar Cells: A Path Towards High-Throughput Manufacturing

High-throughput roll-to-roll (R2R) manufacturing of perovskite solar cells (PSCs) is currently limited by thermal processes that take tens of minutes each, translating to impractically long annealing tools at high web speeds. In addition, PSCs are usually made with metal oxide transport layer materials that require high temperatures for thermal annealing. Here, we demonstrate the fabrication of PSCs using photonic curing, instead of thermal annealing, to convert NiO x directly from sol-gel precursors for hole transport layers and to crystallize methylammonium lead iodide (MAPbI 3 ) active layers on flexible Willow ® Glass substrates. Photonic curing uses short, intense pulses of light to process materials at a high speed, hence it is compatible with R2R manufacturing. We achieved power conversion efficiencies (PCEs) of 11.7% in forward-scan and 10.9% in reverse-scan for PSCs made with photonic cured NiO x and MAPbI 3 films. Furthermore, both NiO x and MAPbI 3 films could be processed with a single photonic curing pulse, with a web speed of 5.7 m/min, and still produce PCEs comparable to thermally annealed control samples. Based on the single-pulse photonic curing condition for each film, we project a web speed of 26 m/min, laying a pathway to high-throughput production of perovskite solar modules.

14 SOLAR ENERGY↗
NASA NTRSDate not supplied

A Photon Counting Ground Receiver for Free-Space Optical Communications

The National Aeronautics and Space Administration is developing a photon counting ground receiver for free-space optical communications. The receiver consists of a fiber interconnect, superconducting nanowire single photon counting detectors (SNSPDs), and a field programmable gate array (FPGA) based receive modem. This receiver is compliant with the Consultative Committee for Space Data Systems (CCSDS) Optical Communications High Photon Efficiency standard, which is used in the low photon flux communications regime, including on the upcoming Optical Artemis-2 Orion communications demonstration. The receiver architecture is modular, can be scaled for data rate, and is designed with primarily commercial-off-the-shelf technology. Two fiber interconnect and detector architectures are being prototyped. The first uses a few-mode-fiber coupled to a 16-channel SNSPD array and the second architecture uses a photonic lantern coupled to 7 single-pixel SNSPDs. Photon counting, symbol timing recovery, demodulation and decoding is done using several FPGA cards. This presentation describes the unique features of the ground receiver, performance test results, and challenges with using commercial SNSPDs in free-space optical communications.

Jennifer N Downey↗
NASA NTRS2009

Negative Avalanche Feedback Detectors for Photon-Counting Optical Communications

Negative Avalanche Feedback photon counting detectors with near-infrared spectral sensitivity offer an alternative to conventional Geiger mode avalanche photodiode or phototube detectors for free space communications links at 1 and 1.55 microns. These devices demonstrate linear mode photon counting without requiring any external reset circuitry and may even be operated at room temperature. We have now characterized the detection efficiency, dark count rate, after-pulsing, and single photon jitter for three variants of this new detector class, as well as operated these uniquely simple to use devices in actual photon starved free space optical communications links.

single photon detector↗
DOE OSTI2023

Axial vs equatorial: Capturing the intramolecular charge transfer state geometry in conformational polymorphic crystals of a donor–bridge–acceptor dyad in nanosecond-time-scale

Two conformational polymorphs of a donor–bridge–acceptor (D-B-A) dyad, p-(CH 3 ) 2 N-C 6 H 4 -(CH 2 ) 2 -(1-pyrenyl)/PyCHDMA, were studied, where the electron donor (D) moiety p-(CH 3 ) 2 N-C 6 H 4 /DMA is connected through a bridging group (B), –CH 2 –CH 2 –, to the electron acceptor (A) moiety pyrene. Though molecular dyads like PyCHDMA have the potential to change solar energy into electrical current through the process of photoinduced intramolecular charge transfer (ICT), the major challenge is the real-time investigation of the photoinduced ICT process in crystals, necessary to design solid-state optoelectronic materials. The time-correlated single photon counting (TCSPC) measurements with the single crystals showed that the ICT state lifetime of the thermodynamic form, PyCHDMA1 (pyrene and DMA: axial), is ~3 ns, whereas, for the kinetic form, PyCHDMA20 (pyrene and DMA: equatorial), it is ~7 ns, while photoexcited with 375 nm radiation. The polymorphic crystals were photo-excited and subsequently probed with a pink Laue x-ray beam in time-resolved x-ray diffraction (TRXRD) measurements. The TRXRD results suggest that in the ICT state, due to electron transfer from the tertiary N-atom in DMA moiety to the bridging group and pyrene moiety, a decreased repulsion between the lone-pair and the bond-pair at N-atom induces planarity in the C–N–(CH 3 ) 2 moiety, in both polymorphs. The Natural Bond Orbital calculations and partial atomic charge analysis by Hirshfeld partitioning also corroborated the same. Although the interfragment charge transfer (IFCT) analysis using the TDDFT results showed that for the charge transfer excitation in both conformers, the electrons were transferred from the DMA moiety to mostly the pyrene moiety, the bridging group has little role to play in that.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Heralded Multiplexed High-Efficiency Cascaded Source of Dual-Rail Entangled Photon Pairs Using Spontaneous Parametric Down-Conversion

Deterministic sources of high-fidelity entangled qubit pairs encoded in the dual-rail photonic basis, i.e., presence of a single photon in one of two orthogonal modes, are a key enabling technology of many applications of quantum information processing, including high-rate, high-fidelity quantum communications over long distances. The most popular and mature sources of such photonic entanglement, e.g., those that leverage spontaneous parametric down-conversion (SPDC) or spontaneous four-wave mixing, generate an entangled (so-called continuous-variable) quantum state that contains contributions from high-order photon terms that lie outside the span of the dual-rail basis, which is detrimental to most applications. One often uses low pump power to mitigate the effects of those high-order terms. However, that reduces the pair generation rate, and the source becomes inherently probabilistic. We investigate a cascaded source that performs a linear-optical entanglement swap between two SPDC sources, to generate a heralded photonic entangled state that has a higher fidelity (to the ideal Bell state) compared to a free-running SPDC source. Furthermore, with the Bell swap providing a heralding trigger, we show how to build a multiplexed source, which despite reasonable switching losses and detector loss and noise, yields a fidelity versus success probability trade-off of a high-efficiency source of high-fidelity dual-rail photonic entanglement. We find, however, that there is a threshold of 1.5 dB of loss per switch, beyond which multiplexing hurts the fidelity versus success probability trade-off.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1969

Electrodynamics of vector mesons.

Renormalization of second order self energy part of photon and lowest order corrections to single photon vertex using Lagrange vector meson density

Grant, C. T.↗
NASA NTRS2011

Polarimetric, Two-Color, Photon-Counting Laser Altimeter Measurements of Forest Canopy Structure

Laser altimeter measurements of forest stands with distinct structures and compositions have been acquired at 532 nm (green) and 1064 nm (near-infrared) wavelengths and parallel and perpendicular polarization states using the Slope Imaging Multi-polarization Photon Counting Lidar (SIMPL). The micropulse, single photon ranging measurement approach employed by SIMPL provides canopy structure measurements with high vertical and spatial resolution. Using a height distribution analysis method adapted from conventional, 1064 nm, full-waveform lidar remote sensing, the sensitivity of two parameters commonly used for above-ground biomass estimation are compared as a function of wavelength. The results for the height of median energy (HOME) and canopy cover are for the most part very similar, indicating biomass estimations using lidars operating at green and near-infrared wavelengths will yield comparable estimates. The expected detection of increasing depolarization with depth into the canopies due to volume multiple-scattering was not observed, possibly due to the small laser footprint and the small detector field of view used in the SIMPL instrument. The results of this work provide pathfinder information for NASA's ICESat-2 mission that will employ a 532 nm, micropulse, photon counting laser altimeter.

Harding, David J.↗
DOE OSTI2025

Third-order photon correlations extract single-nanocrystal multiexciton properties in solution

Colloidal semiconductor nanocrystals are considered promising materials for high-flux optical applications, including lasing, light-emitting diodes, biological imaging, and quantum optics. In high-flux applications, multiexcitons can significantly contribute to emission, influencing its brightness, spectral purity, and kinetics. As a result, understanding and controlling multiexciton emission in colloidal nanocrystal materials is of the utmost importance. In the past, single-nanocrystal photon correlation methods have been applied to understand biexciton and triexciton efficiencies, lifetimes, and spectra. While powerful, such methods suffer from user selection bias and require stable emission from single nanocrystals. To compensate for this shortcoming, second-order correlation methods were developed to extract sample-averaged biexciton properties from a solution of nanocrystals. Until now, however, the analogous third-order solution photon correlation methods remained unexplored. In this work, we present a pair of third-order photon correlation techniques to obtain the sample-averaged single-nanocrystal triexciton quantum yield and lifetime in a solution-phase experiment. These techniques derive from the relationship between the Poisson probability of nanocrystal photon absorption and the intrinsic probability of nanocrystal photon emission. We validate the theoretical background of these techniques by creating a numerical model to simulate the diffusion and emission of many nanocrystals in solution. Our simulations confirm that the average triexciton quantum yield and triexciton lifetime can be extracted from a solution of nanocrystals. These techniques will enable researchers to gain a better understanding of the fundamental multiexciton properties of colloidal nanocrystals.

Horowitz, Jonah R. [Massachusetts Institute of Tec↗
NASA NTRSDate not supplied

Testing of A Photon-Counting Optical Ground Receiver With Emulated Space-to-Ground Link Effects

The National Aeronautics and Space Administration (NASA) Glenn Research Center (GRC) developed and previously characterized a photon-counting optical ground receiver system. The receiver is compliant with the Consultative Committee for Space Data Systems (CCSDS) Optical Communications Coding and Synchronization High Photon Efficiency (HPE) Standard. The standard will be used on the Optical Artemis-2 Orion (O2O) communications demonstration and the Deep Space Optical Communication (DSOC) project aboard the Psyche spacecraft. The receiver system consists of a fiber interconnect, up to sixteen superconducting nanowire single-photon detectors (SNSPDs), and a field programmable gate array (FPGA) based receive modem. Previously, the receiver system architecture was described and test results without emulated link effects were presented. SNSPD device properties, which impact detection jitter and time delay, can limit the receiver dynamic range, especially when operating with varying flux rates (>10 dB) between detectors. Codeword error-rate curves with and without simulated clock drifts attributed to Doppler shift and space transmitter clock differences are presented. Results with ±66 ppm clock differences show minimal performance impact (<0.2 dB). Test results show that the receiver dynamic range (>28 dB) is limited by changing SNSPD detection delays at high photon flux rates.

optical communications↗
NASA NTRSDate not supplied

Testing of A Photon-Counting Optical Ground Receiver With Emulated Space-to-Ground Link Effects

The National Aeronautics and Space Administration (NASA) Glenn Research Center (GRC) developed and previously characterized a photon-counting optical ground receiver system. The receiver is compliant with the Consultative Committee for Space Data Systems (CCSDS) Optical Communications Coding and Synchronization High Photon Efficiency (HPE) Standard. The standard will be used on the Optical Artemis-2 Orion (O2O) communications demonstration and the Deep Space Optical Communication (DSOC) project aboard the Psyche spacecraft. The receiver system consists of a fiber interconnect, up to sixteen superconducting nanowire single-photon detectors (SNSPDs), and a field programmable gate array (FPGA) based receive modem. Previously, the receiver system architecture was described and test results without emulated link effects were presented. SNSPD device properties, which impact detection jitter and time delay, can limit the receiver dynamic range, especially when operating with varying flux rates (>10 dB) between detectors. Codeword error-rate curves with and without simulated clock drifts attributed to Doppler shift and space transmitter clock differences are presented. Results with ±66 ppm clock differences show minimal performance impact (<0.2 dB). Test results show that the receiver dynamic range (>28 dB) is limited by changing SNSPD detection delays at high photon flux rates.

optical communications↗