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NASA NTRS2016

Model Sensitivity Studies of the Decrease in Atmospheric Carbon Tetrachloride

Carbon tetrachloride (CCl4) is an ozone-depleting substance, which is controlled by the Montreal Protocol and for which the atmospheric abundance is decreasing. However, the current observed rate of this decrease is known to be slower than expected based on reported CCl4 emissions and its estimated overall atmospheric lifetime. Here we use a three-dimensional (3-D) chemical transport model to investigate the impact on its predicted decay of uncertainties in the rates at which CCl4 is removed from the atmosphere by photolysis, by ocean uptake and by degradation in soils. The largest sink is atmospheric photolysis (74% of total), but a reported 10% uncertainty in its combined photolysis cross section and quantum yield has only a modest impact on the modelled rate of CCl4 decay. This is partly due to the limiting effect of the rate of transport of CCl4 from the main tropospheric reservoir to the stratosphere, where photolytic loss occurs. The model suggests large interannual variability in the magnitude of this stratospheric photolysis sink caused by variations in transport. The impact of uncertainty in the minor soil sink (9%of total) is also relatively small. In contrast, the model shows that uncertainty in ocean loss (17%of total) has the largest impact on modelled CCl4 decay due to its sizeable contribution to CCl4 loss and large lifetime uncertainty range (147 to 241 years). With an assumed CCl4 emission rate of 39 Gg year(exp -1), the reference simulation with the best estimate of loss processes still underestimates the observed CCl4 (overestimates the decay) over the past 2 decades but to a smaller extent than previous studies. Changes to the rate of CCl4 loss processes, in line with known uncertainties, could bring the model into agreement with in situ surface and remote-sensing measurements, as could an increase in emissions to around 47 Gg year(exp -1). Further progress in constraining the CCl4 budget is partly limited by systematic biases between observational datasets. For example, surface observations from the National Oceanic and Atmospheric Administration (NOAA) network are larger than from the Advanced Global Atmospheric Gases Experiment (AGAGE) network but have shown a steeper decreasing trend over the past 2 decades. These differences imply a difference in emissions which is significant relative to uncertainties in the magnitudes of the CCl4 sinks.

Carbon Trechloride↗

DOE OSTI2026

Shower Reconstruction for Cross-Section Measurements with Photon(s) in the Final State at SBND

The Short-Baseline Near Detector (SBND) is a 112-ton liquid argon time projection chamber operating in the Booster Neutrino Beam at Fermilab as part of the Short-Baseline Neutrino Program. Precise reconstruction of electromagnetic showers from photons and electrons is essential for searches for neutrino oscillations, cross-section measurements, and rare-process studies in liquid argon. In this poster, we present a unified set of SBND analyses enabled by the SPINE (Scalable Particle Imaging with Neural Embeddings) end-to-end machine-learning–based reconstruction framework, highlighting charged-current neutral pion (CC π⁰) production and neutral-current (NC) Δ radiative decay as complementary physics cases. Charged-current π⁰ interactions provide a high-statistics benchmark for validating photon reconstruction, constraining the electromagnetic energy scale, and modeling backgrounds to other cross-section measurements and BSM searches with one or more photons in the final state. We summarize progress toward the ongoing development of a CC π⁰ selection in SBND and, report on the current status of a search for NC resonant Δ production followed by radiative decay (Δ→Nγ) in SBND. This rare process, previously investigated in MicroBooNE, provides a stringent test of photon-only final-state reconstruction and is of interest in the context of the MiniBooNE low-energy excess. Together, these analyses demonstrate how modern machine-learning–based shower reconstruction enables a diverse and scalable physics program at SBND.

Chung, Seokju [Nevis Labs, Columbia U.]↗

DOE OSTI2024

Elucidating the Radiation-Induced Redox Chemistry of Plutonium Under Used Nuclear Fuel Reprocessing Conditions

Plutonium plays a critical role in the development of sustainable nuclear fuel cycles, and yet, our fundamental understanding of this element’s inherent radiation-induced redox chemistry and associated impacts on nuclear fuel cycle technologies is limited. Unanticipated changes in oxidation state distribution can influence the speciation and transport of plutonium in a given process. Control of these parameters is especially important for used nuclear fuel reprocessing technologies, wherein the separation and recovery of plutonium is typically achieved by the selective formation, maintenance, and complexation of specific oxidation states. Furthermore, plutonium’s inherent radiation-induced redox chemistry has the capacity to influence the radiolytic behavior of its complexes, the longevity of which are critical in the design of efficient and cost-effective advanced reprocessing technologies. These radiation-induced processes are unavoidable under fuel cycle conditions owing to the inherency of ionizing radiation fields to the decay of plutonium’s isotopes and to the various other radioisotopes generated by nuclear fission and neutron-capture process and the subsequent radioactive decay of their products. As such, mechanistically understanding the response of plutonium’s multiple oxidation states to multi-component ionizing radiation fields is essential for predicting the behavior of this critical element under used nuclear fuel reprocessing conditions. Here, through a combination of time-resolved (electron pulse) and steady-state (alpha and gamma) irradiation experiments complemented by quantitative, multiscale modeling calculations, we present advances in our understanding of radiation-induced plutonium redox chemistry!

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1989

Nonlinear evolution of high frequency R-mode waves excited by water group ions near comets - Computer experiments

An ion beam resonates with R-mode waves at a high-frequency RH mode and a low-frequency RL mode. The nonlinear evolution of ion beam-generated RH waves is studied here by one-dimensional hybrid computer experiments. Both wave-particle and subsequent wave-wave interactions are examined. The competing process among coexisting RH and RL mode beam instabilities and repeated decay instabilities triggered by the beam-excited RH mode waves is clarified. It is found that the quenching of the RH instability is not caused by a thermal spreading of the ion beam, but by the nonlinear wave-wave coupling process. The growing RH waves become unstable against the decay instability. This instability involves a backward-traveling RH electromagnetic wave and a forward-traveling longitudinal sound wave. The inverse cascading process is found to occur faster than the growth of the RL mode. Wave spectra decaying from the RH waves weaken as time elapses and the RL mode waves become dominant at the end of the computer experiment.

Kojima, H.↗

DOE OSTI2024

Unveiling the properties of the dimuonium at the energies available at the Large Hadron Collider at CERN

We study the production of dimuonium (also known as true muonium) in two- and three-photon fusion processes in nucleus–nucleus collisions at the CERN Large Hadron Collider (LHC). A new formalism is introduced for the production process, and valuable new information is extracted, which will be helpful in proposals of future experiments. We explore the phase space constraints, the reaction mechanisms, and how dimuonium decay observables might be jeopardized by other physical processes. Here, we show that the energies available at the Large Hadron Collider at CERN might lead to the first identification of dimuonium in a terrestrial laboratory.

Bertulani, Carlos A.↗

NASA NTRS1987

Radiation characteristics of low resistivity float zone silicon solar cells

The effects of 1-MeV electron irradiation on silicon solar cells with AM0 efficiencies ranging from 17 to 17.7 percent are described. These cells were processed on low-resistivity FZ substrates using techniques recently developed for high-efficiency terrestrial silicon solar cells. Results indicate that these cells are more susceptible to radiation damage. However, they do maintain a greater overall power output than conventional cells to which they were compared. These cells do not demonstrate post-electron-irradiation photon decay as has been described for cells processed on 1-10 ohm-cm FZ silicon.

Crotty, G. T.↗

DOE OSTI2025

PHOTOPRODUCTION OF np^0 BY DOUBLE-REGGE EXCHANGE

The GlueX experiment is a photoproduction experiment based at Jeferson Lab in Newport News, Virginia. A major aim of GlueX is to look for hybrid mesons, which are a quark and an anti-quark bound by an excited gluonic field that contributes to the quantum numbers. The reaction ¿p ¿ ¿e0p is of particular interest since ¿e is a potential decay mode of states with exotic quantum numbers JPC =1¿+, which are forbidden in the constituent quark model. Finding such a resonance would be a clear sign of non-quark model physics. In concert with the Joint Physics Analysis Center we have developed a model for double-Regge interactions in this channel. These non-resonant processes generate asymmetries in the distributions of decay angles, which could be falsely attributed to the interference between exotic odd partial waves and even partial waves. In previous searches for light exotics we have seen evidence for the necessity of accounting for the presence of these non-resonant productions. We present a double-Regge model for photoproduction of ¿e0 and the application of it by measuring the asymmetry of ¿e0 production in the double Regge limit, as well as a comparison of the measured results to current theoretical predictions.

Barsotti, Rebecca [Indiana Univ. Southeast, New Al↗

DOE OSTI2025

Search for B 0 → K *0 𝜏 + ⁢𝜏 − Decays at the Belle II Experiment

We present a search for the rare flavor-changing neutral-current decay 𝐵 0 →𝐾 *0 ⁢𝜏 + ⁢𝜏 − with data collected by the Belle II experiment at the SuperKEKB electron-positron collider. The analysis uses a 365 fb −1 data sample recorded at the center-of-mass energy of the ϒ⁡(4⁢𝑆) resonance. One of the 𝐵 mesons produced in the ϒ⁡(4⁢𝑆)→𝐵 0 $⁢\overline{𝐵}$ 0 process is fully reconstructed in a hadronic decay mode, while its companion 𝐵 meson is required to decay into a 𝐾 *0 and two 𝜏 leptons of opposite charge. The 𝜏 leptons are reconstructed in final states with a single electron, muon, charged pion or charged 𝜌 meson, and additional neutrinos. We set an upper limit on the branching fraction of ℬ⁡(𝐵 0 →𝐾 *0 ⁢𝜏 + ⁢𝜏 − )<1.8×10 −3 at the 90% confidence level, which is the most stringent constraint reported to date.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Electron-positron, parton-parton, and photon-photon production of τ -lepton pairs: Anomalous magnetic and electric dipole moments spin effects

Anomalous contributions to the electric and magnetic dipole moments of the τ lepton from new physics scenarios have brought renewed interest in the development of new charge-parity violating signatures in τ -pair production at Belle II energies, and also at higher energies of the Large Hadron Collider and the Future Circular Collider. In this paper, we discuss the effects of spin correlations, including transverse degrees of freedom, in the τ -pair production and decay. These studies include calculating analytical formulas, obtaining numerical results, and building semirealistic observables sensitive to the transverse spin correlations induced by the dipole moments of the τ lepton. The effects of such anomalous contributions to the dipole moments are introduced on top of precision simulations of e − e + → τ − τ + , q q ¯ → τ − τ + and γ γ → τ − τ + processes, involving multibody final states. The τ decays are simulated along with radiative corrections, in particular electroweak box contributions of W W and Z Z exchanges are taken into account. Respective extensions of the Standard Model amplitudes and the reweighting algorithms are implemented into the Monte Carlo, which is used to simulate τ -pair production in e − e + collisions, and the aupinner program, which is used to reweight events with τ pair produced in p p collisions. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

Spatially resolved photoluminescence brightening in individual single-walled carbon nanotubes

Single-molecule microscopy was used to image photoluminescence (PL) brightening of individual sodium-dodecyl-sulfate (SDS)-wrapped single-walled carbon nanotubes (SWCNTs) upon the addition of dithiothreitol (DTT). PL enhancement varied for each nanotube (NT), with some brightening by 16% and others by a factor of about 7. Interestingly, NTs that displayed lower initial QY values showed the largest increases in PL enhancement. SDS-SWCNTs longer than the diffraction limit were studied in order to spatially resolve the brightening phenomenon. Quite unexpectedly, a uniform, single-step PL brightening along the NT was consistently observed, suggesting that the PL enhancement is the result of a non-localized process. Furthermore, the even PL brightening seen over SWCNTs that are micrometers long implies that single point defect sites, which are known to be largely responsible for exciton nonradiative decay, play no significant role in the brightening process. Interestingly, affixing the SWCNT strongly to the substrate surface mitigated the PL brightening response, consistent with a hypothesis that surfactant reorganization upon the addition of DTT is responsible for exciton PL brightening.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

NASA NTRS2002

On the Exit Boundary Condition for One-Dimensional Calculations of Pulsed Detonation Engine Performance

In one-dimensional calculations of pulsed detonation engine (PDE) performance, the exit boundary condition is frequently taken to be a constant static pressure. In reality, for an isolated detonation tube, after the detonation wave arrives at the exit plane, there will be a region of high pressure, which will gradually return to ambient pressure as an almost spherical shock wave expands away from the exit, and weakens. Initially, the flow is supersonic, unaffected by external pressure, but later becomes subsonic. Previous authors have accounted for this situation either by assuming the subsonic pressure decay to be a relaxation phenomenon, or by running a two-dimensional calculation first, including a domain external to the detonation tube, and using the resulting exit pressure temporal distribution as the boundary condition for one-dimensional calculations. These calculations show that the increased pressure does affect the PDE performance. In the present work, a simple model of the exit process is used to estimate the pressure decay time. The planar shock wave emerging from the tube is assumed to transform into a spherical shock wave. The initial strength of the spherical shock wave is determined from comparison with experimental results. Its subsequent propagation, and resulting pressure at the tube exit, is given by a numerical blast wave calculation. The model agrees reasonably well with other, limited, results. Finally, the model was used as the exit boundary condition for a one-dimensional calculation of PDE performance to obtain the thrust wall pressure for a hydrogen-air detonation in tubes of length to diameter ratio (L/D) of 4, and 10, as well as for the original, constant pressure boundary condition. The modified boundary condition had no performance impact for values of L/D > 10, and moderate impact for L/D = 4.

Wilson, Jack↗

DOE OSTI2020

MeV Gamma Rays from Fission: A Distinct Signature of Actinide Production in Neutron Star Mergers

Neutron star mergers (NSMs) are the first verified sites of rapid neutron capture (r-process) nucleosynthesis, and could emit gamma rays from the radioactive isotopes synthesized in the neutron-rich ejecta. These MeV gamma rays may provide a unique and direct probe of the NSM environment as well as insight into the nature of the r process, just as observed gammas from the 56 Ni radioactive decay chain provide a window into supernova nucleosynthesis. In this work, we include the photons from fission processes for the first time in estimates of the MeV gamma-ray signal expected from an NSM event. We consider NSM ejecta compositions with a range of neutron richness and find a dramatic difference in the predicted signal depending on whether or not fissioning nuclei are produced. The difference is most striking at photon energies above ~3.5 MeV and at a relatively late time, several days after the merger event, when the ejecta is optically thin. We estimate that a Galactic NSM could be detectable by a next generation gamma-ray detector such as AMEGO in the MeV range, up to ~104 days after the merger, if fissioning nuclei are robustly produced in the event.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1978

An instability of finite amplitude circularly polarized Alfven waves

A demonstration is presented that a finite-amplitude circularly-polarized Alfven wave is generally unstable in a MHD fluid. The wave decays by a four-wave coupling process in which the daughter waves are forward propagating random density and magnetic fluctuations and a backward-propagating magnetic wave. For parameters typical of the solar corona and the solar wind (thermal to magnetic energy density ratios between 0.1 and 1, and values between 0.1 and 0.9 for the ratio of magnetic energy density of the initial Alfven wave to that of the background magnetic field), large decay rates are found.

Goldstein, M. L.↗

DOE OSTI2021

Measurements of WH and ZH production in the $$H \rightarrow b\bar{b}$$ decay channel in pp collisions at $$13\,\text {Te}\text {V}$$ with the ATLAS detector

Measurements of the Standard Model Higgs boson decaying into a $$b\bar{b}$$ b b ¯ pair and produced in association with a W or Z boson decaying into leptons, using proton–proton collision data collected between 2015 and 2018 by the ATLAS detector, are presented. The measurements use collisions produced by the Large Hadron Collider at a centre-of-mass energy of $$\sqrt{s} = 13\,\text {Te}\text {V}$$ s = 13 Te , corresponding to an integrated luminosity of $$139\,\mathrm {fb}^{-1}$$ 139 fb - 1 . The production of a Higgs boson in association with a W or Z boson is established with observed (expected) significances of 4.0 (4.1) and 5.3 (5.1) standard deviations, respectively. Cross-sections of associated production of a Higgs boson decaying into bottom quark pairs with an electroweak gauge boson, W or Z , decaying into leptons are measured as a function of the gauge boson transverse momentum in kinematic fiducial volumes. The cross-section measurements are all consistent with the Standard Model expectations, and the total uncertainties vary from 30% in the high gauge boson transverse momentum regions to 85% in the low regions. Limits are subsequently set on the parameters of an effective Lagrangian sensitive to modifications of the WH and ZH processes as well as the Higgs boson decay into $$b\bar{b}$$ b b ¯ .

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS1973

Re-187, recycling r-process elements through stars, and the age of the Galaxy.

The enhanced beta-decay rate of ionized Re-187 in stars has been studied within the context of a detailed numerical model of the production of r-process elements and their recycling through stars during the course of galactic evolution. It is concluded that the enhanced decay rate does not significantly reduce the Re-Os chronometer age for the Galaxy. Consequently, the Re-187 beta-decay half-life and the Os-186/Os-187 neutron cross-section ratio remain as the significant uncertainties in this chronology. Unlike the uncertainties in other chronologies, both are amenable to laboratory measurements.

Talbot, R. J., Jr.↗

NASA NTRS1985

The cancellation of magnetic flux. II - In a decaying active region

H-alpha filtergrams and videomagnetograms are used to study an active region during its period of decay on August 3-8, 1984; the decay had been initiated by a fragmentation process in which very small knots of magnetic flux separated from larger concentration of flux. The disappearance of magnetic flux was always observed when the small fragments of flux encountered other small fragments or concentrations of flux of opposite polarity. Such 'cancellations' are shared by both polarities of magnetic field, and it is deduced that the disappearance of flux occurred either at or within 5 arcsec of the apparent dividing line between the opposite polarities. All of the 22 flares observed during the decay of this region were initiated around sites where magnetic flux was cancelling or was deduced to be cancelling during the flares. It is hypothesized that cancellation was one of the necessary conditions for flaring in this active region.

Martin, S. F.↗

DOE OSTI2023

Bentonite buffer under high temperature: laboratory experiments and coupled process modeling

Abstract. Bentonite buffer in a geological repository will be simultaneously heated from decaying radioactive waste and hydrated from the surrounding host rock, triggering complex and coupled THMC (thermal–hydrological–mechanical–chemical) processes. Understanding the THMC behavior of bentonite-based engineered barrier system (EBS) is key to the evaluation and prediction of its long-term performance. Studies on the THMC process have been focused on conditions under 100 ∘C, as most design concepts impose a thermal limit of 100 ∘C in bentonite. Recently, studies under high-temperature conditions have been conducted to evaluate the possibility of raising the thermal limit and expanding the data/knowledge base to increase the confidence level. In this abstract, we present a series of bench-scale laboratory experiments at high temperatures (up to 200 ∘C) and the corresponding modeling work. Two sets of column tests were conducted, and each set consisted of two test columns: a control column undergoing only hydration (non-heated) and an experiment column experiencing both heating and hydration (heated). During the experiment, frequent X-ray computed tomography (CT) images were collected to provide a 3D visualization of the density distribution and present the spatiotemporal evolution of (1) hydration/dehydration, (2) clay swelling/shrinkage, (3) displacement, and (4) mineral precipitation. The two sets of tests differ with respect to several experimental conditions, such as bentonite type, compacted density and water content, water chemistry, and hydration pressure, but the important difference is that the first set used bentonite powder with a dry density of 1.28 g cm−3, whereas the second set used granulated bentonite (mixture of pellets and powder) with a dry density of 1.45–1.5 g cm−3. In both sets of experiments, a comprehensive post-dismantling characterization of bentonite samples was carried out after the column tests had been running for 1.5 years. Comparing non-heated and heated columns, the temperature gradient led to lower degree of homogenization of bentonite after bentonite became fully saturated; comparing the first and second sets, granulated and powdered bentonite exhibited drastically different hydration behavior. A THM model with a 2D axisymmetric grid system was used to interpret the data from the first set of tests. The model considers the combined impact of saturation, fluid pressure, and porosity change due to swelling/compression on the spatiotemporal distribution of bulk density and movement of the thermocouple modules. Observations from the tests help us understand the early perturbation of bentonite buffer under high temperature, and data from these tests improve the calibration of key constitutive hydrological and mechanical models and, therefore, enhance the modeling capability with respect to calculating the long-term evolution of bentonite buffer.

Zheng, Liange↗

DOE OSTI2020

Improved Limit on Neutrinoless Double-Beta Decay in Te 130 with CUORE

We report new results from the search for neutrinoless double-beta decay in $^{130}$Te with the CUORE detector. This search benefits from a four-fold increase in exposure, lower trigger thresholds and analysis improvements relative to our previous results. We observe a background of $(1.38\pm0.07)\cdot10^{-2}$ counts$/($keV$\cdot$kg$\cdot$yr$)$ in the $0\nu\beta\beta$ decay region of interest and, with a total exposure of 372.5 kg$\cdot$yr, we attain a median exclusion sensitivity of $1.7\cdot10^{25}$ yr. We find no evidence for $0\nu\beta\beta$ decay and set a $90\%$ CI Bayesian lower limit of $3.2\cdot10^{25}$ yr on the $^{130}$Te half-life for this process. In the hypothesis that $0\nu\beta\beta$ decay is mediated by light Majorana neutrinos, this results in an upper limit on the effective Majorana mass of 75-350 meV, depending on the nuclear matrix elements used.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗