Search NASA⌕ Search

SEARCH · Search NASA

Results for “Ice cloud”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 415 records · Page 23
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Model-observation discrepancies in Arctic moisture intrusions: causes and pathways for improved simulation

Arctic moisture intrusions (MIs), narrow filaments of strong moisture transport, are key drivers of poleward moisture flux and Arctic weather extremes, yet their representation in climate models is poorly understood. Using a new Arctic MI detection algorithm, we document persistent biases across three CMIP generations (CMIP3–CMIP6): models overestimate MI occurrence over the Pacific sector and underestimate it over the Atlantic sector. These errors stem from misrepresented midlatitude westerly jets, with an equatorward North Atlantic jet associated with too few Atlantic MIs, and a poleward, weakened North Pacific jet linked to too many Pacific MIs. Experiments that correct sea surface temperature and sea ice concentration biases and increase atmospheric resolution improve jet structure and MI statistics, while a cloud-locking simulation indicates that better high-frequency cloud–radiation–circulation interactions can yield further gains. Our results clarify pathways to reducing long-standing MI and jet biases, providing guidance for improving simulations of Arctic and midlatitude climate.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Polarimetric Radar Characteristics of Simulated and Observed Intense Convective Cores for a Midlatitude Continental and Tropical Maritime Environment

This study contrasts midlatitude continental and tropical maritime deep convective cores using polarimetric radar observables and retrievals from selected deep convection episodes during the MC3E and TWPICE field campaigns. The continental convective cores produce stronger radar reflectivities throughout the profiles, while maritime convective cores produce more positive differential reflectivity Z dr and larger specific differential phase K dp above the melting level. Hydrometeor identification retrievals revealed the presence of large fractions of rimed ice particles (snow aggregates) in the continental (maritime) convective cores, consistent with the Z dr and K dp observations. The regional cloud-resolving model simulations with bulk and size-resolved bin microphysics are conducted for the selected cases, and the simulation outputs are converted into polarimetric radar signals and retrievals identical to the observational composites. Both the bulk and the bin microphysics reproduce realistic land and ocean (L-O) contrasts in reflectivity, polarimetric variables of rain drops, and hydrometeor profiles, but there are still large uncertainties in describing Z dr and K dp of ice crystals associated with the ice particle shapes/orientation assumptions. Sensitivity experiments are conducted by swapping background aerosols between the continental and maritime environments, revealing that background aerosols play a role in shaping the distinct L-O contrasts in radar reflectivity associated with raindrop sizes, in addition to the dominant role of background thermodynamics.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Long-Term Trends for Marine Sulfur Aerosol in the Alaskan Arctic and Relationships With Temperature

Marine aerosol plays a vital role in cloud-aerosol interactions during summer in the Arctic. The recent rise in temperature and decrease in sea ice extent have the potential to impact marine biogenic sources. Compounds like methanesulfonic acid (MSA) and non-sea-salt sulfate (nss-SO 4 2- ), oxidation products of dimethyl sulfide (DMS) emitted by marine primary producers, are likely to increase in concentration. Long-term studies are vital to understand these changes in marine sulfur aerosol and potential interactions with Arctic climate. Samples were collected over three summers at two coastal sites on the North Slope of Alaska (Utqiagvik and Oliktok Point). MSA concentrations followed previously reported seasonal trends, with evidence of high marine primary productivity influencing both sites. When added to an additional data set collected at Utqiagvik, an increase in MSA concentration of + 2.5% per year and an increase in nss-SO 4 2- of + 2.1% per year are observed for the summer season over the 20-year record (1998–2017). This study identifies ambient air temperature as a strong factor for MSA, likely related to a combination of interrelated factors including warmer sea surface temperature, reduced sea ice, and temperature-dependent chemical reactions. Analysis of individual particles at Oliktok Point, within the North Slope of Alaska oil fields, showed evidence of condensation of MSA onto anthropogenic particles, highlighting the connection between marine and oil field emissions and secondary organic aerosol. Finally, this study shows the continued importance of understanding MSA in the Arctic while highlighting the need for further research into its seasonal relationship with organic carbon.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

A review of coarse mineral dust in the Earth system

Mineral dust particles suspended in the atmosphere span more than three orders of magnitude in diameter, from <0.1 µm to more than 100 µm. This wide size range makes dust a unique aerosol species with the ability to interact with many aspects of the Earth system, including radiation, clouds, hydrology, atmospheric chemistry, and biogeochemistry. This review focuses on coarse and super-coarse dust aerosols, which we respectively define as dust particles with a diameter of 2.5–10 µm and 10–62.5 µm. We review several lines of observational evidence indicating that coarse and super-coarse dust particles are transported farther than previously expected and that the abundance of these particles is substantially underestimated in current global models. We synthesize previous studies that used observations, theories, and model simulations to highlight the impacts of coarse and super-coarse dust aerosols on the Earth system, including their effects on dust-radiation interactions, dust-cloud interactions, atmospheric chemistry, and biogeochemistry. Specifically, coarse and super-coarse dust aerosols produce a net positive direct radiative effect (warming) at the top of the atmosphere and can modify temperature and water vapor profiles, influencing the distribution of clouds and precipitation. In addition, coarse and super-coarse dust aerosols contribute a substantial fraction of ice-nucleating particles, especially at temperatures above –23 °C. They also contribute a substantial fraction to the available reactive surfaces for atmospheric processing and the dust deposition flux that impacts land and ocean biogeochemistry by supplying important nutrients such as iron and phosphorus. Furthermore, we examine several limitations in the representation of coarse and super-coarse dust aerosols in current model simulations and remote-sensing retrievals. Because these limitations substantially contribute to the uncertainties in simulating the abundance and impacts of coarse and super-coarse dust aerosols, we offer some recommendations to facilitate future studies. Overall, we conclude that an accurate representation of coarse and super-coarse properties is critical in understanding the impacts of dust aerosols on the Earth system.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Predictive Proxies of Present and Future Lightning in a Superparameterized Model

Abstract A superparameterized climate model is used to assess the global performance of several previously proposed proxies for lightning. In particular, predictors incorporating hydrometeor (ice, graupel) profiles and convective vertical velocities are compared to observations, then used to estimate changes in flash rates with global warming. The choice of microphysics parameterization is also investigated, with all predictors showing higher correlations with Lightning Imaging Sensor/Optical Transient Detector observations when using a 2‐moment scheme compared to a 1‐moment representation. All proxies generally agree in their response to warming over tropical land, with notable decreases in Africa, the Middle East, and northern South America, but disagree over oceans and the midlatitudes. The product of convective available potential energy and precipitation predicts increases over these latter areas, as do the 2‐moment ice‐based proxies, while those of the 1‐moment model tend to show decreases, highlighting the importance of cloud microphysics when using climate models to simulate lightning.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Cloud radiative effect dominates variabilities of surface energy budget in the dark Arctic

Climate models simulate a wide range of temperatures in the Arctic. Here we investigate one of the main drivers of changes in surface temperature: the net surface heat flux in the models. We show that in the winter months of the dark Arctic, there is a more than two-fold difference in the net surface heat fluxes among the models, and this difference is dominated by the downward infrared radiation from clouds. Owing to the small amount of water vapor in the winter Arctic, infrared radiation from clouds transmits more easily to the surface in the Arctic than at other latitudes, resulting in large cloud radiative effect at the surface. The dominant role of the cloud effect is also found in the transient variability of the net surface heat flux. Results demonstrate that accurate simulation of clouds is crucial for determining the net surface heat flux, which in turn affects surface temperature and sea ice properties in the Arctic.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Seasonal Variation of Dust Aerosol Vertical Distribution in Arctic Based on Polarized Micropulse Lidar Measurement

This study investigates the seasonal variation of dust aerosol vertical distribution using polarized Micropulse lidar (MPL) measurements at the Atmospheric Radiation Measurement (ARM) North Slope of Alaska (NSA) observatory from January 2013 to September 2017. For the first time, multi-year aerosol backscatter coefficients are retrieved at the ARM NSA site from MPL measurements and are consistent with co-located high spectral resolution lidar (HSRL) measurements. The high-quality aerosol backscatter coefficient retrievals are used to derive the particle depolarization ratio (PDR) at the wavelength of 532 nm, which is used to identify the presence of dust aerosols. The annual cycles of the vertical distributions of dust backscatter coefficient and PDR and dust aerosol optical depth (DAOD) show that aerosol loading has a maximum in late winter and early spring but a minimum in late summer and early autumn. Vertically, dust aerosol occurs in the entire troposphere in spring and winter and in the low and middle troposphere in summer and autumn. Because dust aerosols are effective ice nuclei, the seasonality of dust aerosol vertical distribution has important implications for the Arctic climate through aerosol–cloud–radiation interactions, primarily through impacting mixed-phase cloud processes.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Stochastic nucleation processes and substrate abundance explain time-dependent freezing in supercooled droplets

Atmospheric immersion freezing (IF), a heterogeneous ice nucleation process where an ice nucleating particle (INP) is immersed in supercooled water, is a dominant ice formation pathway impacting the hydrological cycle and climate. Implementation of IF derived from field and laboratory data in cloud and climate models is difficult due to the high variability in spatio-temporal scales, INP composition, and morphological complexity. We demonstrate that IF can be consistently described by a stochastic nucleation process accounting for uncertainties in the INP surface area. This approach accounts for time-dependent freezing, a wide range of surface areas and challenges phenomenological descriptions typically used to interpret IF. The results have an immediate impact on the current description, interpretation, and experiments of IF and its implementation in models. The findings are in accord with nucleation theory, and thus should hold for any supercooled liquid material that nucleates in contact with a substrate.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Characterization of Orography-Influenced Riming and Secondary Ice Production and Their Effects on Precipitation Rates Using Radar Polarimetry and Doppler Spectra (CORSIPP-SAIL)

The Characterization of Orography-Influenced Riming and Secondary Ice Production and Their Effects on Precipitation Rates Using Radar Polarimetry and Doppler Spectra (CORSIPP) project was conducted to help improve the understanding of precipitation formation in orographically influenced terrain. Special focus is put on the two processes of riming and secondary ice production and their external drivers. Two instruments, a polarimetric W-band simultaneous transmission simultaneous reception (STSR) Doppler cloud radar manufactured by Radiometer Physics GmbH (RPG, instrument type RPG-FMCW-94-DP), from now on named LIMRAD94, and the video in situ snowfall sensor (VISSS), were deployed at the U. S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility’s Surface Atmosphere Integrated Field Laboratory (SAIL) site in Gothic, Colorado between November 2022 and June 2023 during the second SAIL winter. Note that the exact dates of data availability differ between the instruments. Both instruments arrived at Gothic on November 2, 2022, 09:20 local time. VISSS, described by Maahn et al., is equipped with two camera systems with telecentric lenses. The two cameras are at a 90° angle to each other. This configuration allows for size-independent measurements by capturing images of hydrometeors from two sides at a high frame rate of 250 Hz. With a minimum detection size of 200 μm, VISSS provides valuable insights into particle size, number, shape, complexity, and fall velocity. The VISSS was deployed on the grassland next to the ARM facility with the amazing help of the ARM employees on site. The setup started on November 2, 2022, and was finished on November 5, 2022, without major problems. VISSS measurements were started on November 6, 2022. LIMRAD94 was installed on a scaffolding platform near Orehouse (Gothic) on November 9, 2022, with the great help of RMBL staff. LIMRAD94 was mounted on a cold temperature scanner prototype. After a short test of the setup on November 9, 2022, the digital control of the scanner elevation stopped working for (at that time) unknown reasons. All attempts to resolve the problem failed. This malfunction made it impossible to operate LIMRAD94 in scanning mode. The scanner was then manually moved to zenith pointing mode and between November 10 and November 15, 2022, vertical observations for polarimetric calibration were performed. On November 15, 2022, after the polarimetric calibration was applied, the scanner was manually moved to 40° elevation with azimuthal view towards the Ka-band ARM Zenith Radar (KAZR) and measurements were continued at constant elevation. Investigation of the scanner malfunction on February 6, 2023, by Benn Schmatz revealed a disengagement between the cogwheel of the elevation motor and the cogwheel moving the scanner in elevation. This mechanical issue was temporarily solved by re-engaging the cogwheels. This made the scanner operational again for about four weeks, until mechanical force disengaged the cogwheels again on March 15, 2023. This repeated scanner failure remained undetected for about three weeks until April 8, 2023; during this time the scanner was stuck at 72° elevation. However, the radar software continued to produce data files falsely indicating that the scanner was still operational. After the scanner failure was noticed, scanning was stopped again, and we returned to constant elevation measurements. On May 15, 2023, the cogwheels of the elevation motor were secured with additional screws sent by the manufacturer. At some point in May, the cogwheels of the azimuth motor were also disengaged by mechanical force, which still allowed for range height indicator (RHI) but no plan position indicator (PPI) scans in the last weeks of the campaign. The azimuth motor was repaired in Germany after the end of the campaign. Throughout the campaign, RMBL and ARM staff kept the radar and the VISSS free of snow.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Nudging allows direct evaluation of coupled climate models with in situ observations: a case study from the MOSAiC expedition

Comparing the output of general circulation models to observations is essential for assessing and improving the quality of models. While numerical weather prediction models are routinely assessed against a large array of observations, comparing climate models and observations usually requires long time series to build robust statistics. Here, we show that by nudging the large-scale atmospheric circulation in coupled climate models, model output can be compared to local observations for individual days. We illustrate this for three climate models during a period in April 2020 when a warm air intrusion reached the MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition in the central Arctic. Radiosondes, cloud remote sensing and surface flux observations from the MOSAiC expedition serve as reference observations. The climate models AWI-CM1/ECHAM and AWI-CM3/IFS miss the diurnal cycle of surface temperature in spring, likely because both models assume the snowpack on ice to have a uniform temperature. CAM6, a model that uses three layers to represent snow temperature, represents the diurnal cycle more realistically. During a cold and dry period with pervasive thin mixed-phase clouds, AWI-CM1/ECHAM only produces partial cloud cover and overestimates downwelling shortwave radiation at the surface. AWI-CM3/IFS produces a closed cloud cover but misses cloud liquid water. Our results show that nudging the large-scale circulation to the observed state allows a meaningful comparison of climate model output even to short-term observational campaigns. We suggest that nudging can simplify and accelerate the pathway from observations to climate model improvements and substantially extends the range of observations suitable for model evaluation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Radar Retrieval Evaluation and Investigation of Dendritic Growth Layer Polarimetric Signatures in a Winter Storm

Abstract This study evaluates ice particle size distribution and aspect ratio φ Multi-Radar Multi-Sensor (MRMS) dual-polarization radar retrievals through a direct comparison with two legs of observational aircraft data obtained during a winter storm case from the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) campaign. In situ cloud probes, satellite, and MRMS observations illustrate that the often-observed K dp and Z DR enhancement regions in the dendritic growth layer can either indicate a local number concentration increase of dry ice particles or the presence of ice particles mixed with a significant number of supercooled liquid droplets. Relative to in situ measurements, MRMS retrievals on average underestimated mean volume diameters by 50% and overestimated number concentrations by over 100%. IWC retrievals using Z DR and K dp within the dendritic growth layer were minimally biased relative to in situ calculations where retrievals yielded −2% median relative error for the entire aircraft leg. Incorporating φ retrievals decreased both the magnitude and spread of polarimetric retrievals below the dendritic growth layer. While φ radar retrievals suggest that observed dendritic growth layer particles were nonspherical (0.1 ≤ φ ≤ 0.2), in situ projected aspect ratios, idealized numerical simulations, and habit classifications from cloud probe images suggest that the population mean φ was generally much higher. Coordinated aircraft radar reflectivity with in situ observations suggests that the MRMS systematically underestimated reflectivity and could not resolve local peaks in mean volume diameter sizes. These results highlight the need to consider particle assumptions and radar limitations when performing retrievals. significance statement Developing snow is often detectable using weather radars. Meteorologists combine these radar measurements with mathematical equations to study how snow forms in order to determine how much snow will fall. This study evaluates current methods for estimating the total number and mass, sizes, and shapes of snowflakes from radar using images of individual snowflakes taken during two aircraft legs. Radar estimates of snowflake properties were most consistent with aircraft data inside regions with prominent radar signatures. However, radar estimates of snowflake shapes were not consistent with observed shapes estimated from the snowflake images. Although additional research is needed, these results bolster understanding of snow-growth physics and uncertainties between radar measurements and snow production that can improve future snowfall forecasting.

Meteorology & Atmospheric Sciences↗
DOE OSTI2021

Multifrequency radar observations of clouds and precipitation including the G-band

Abstract. Observations collected during the 25 February 2020 deployment of the Vapor In-Cloud Profiling Radar at the Stony Brook Radar Observatory clearly demonstrate the potential of G-band radars for cloud and precipitation research, something that until now was only discussed in theory. The field experiment, which coordinated an X-, Ka-, W- and G-band radar, revealed that the Ka–G pairing can generate differential reflectivity signal several decibels larger than the traditional Ka–W pairing underpinning an increased sensitivity to smaller amounts of liquid and ice water mass and sizes. The observations also showed that G-band signals experience non-Rayleigh scattering in regions where Ka- and W-band signal do not, thus demonstrating the potential of G-band radars for sizing sub-millimeter ice crystals and droplets. Observed peculiar radar reflectivity patterns also suggest that G-band radars could be used to gain insight into the melting behavior of small ice crystals. G-band signal interpretation is challenging, because attenuation and non-Rayleigh effects are typically intertwined. An ideal liquid-free period allowed us to use triple-frequency Ka–W–G observations to test existing ice scattering libraries, and the results raise questions on their comprehensiveness. Overall, this work reinforces the importance of deploying radars (1) with sensitivity sufficient enough to detect small Rayleigh scatters at cloud top in order to derive estimates of path-integrated hydrometeor attenuation, a key constraint for microphysical retrievals; (2) with sensitivity sufficient enough to overcome liquid attenuation, to reveal the larger differential signals generated from using the G-band as part of a multifrequency deployment; and (3) capable of monitoring atmospheric gases to reduce related uncertainty.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Simulating Mixed‐Phase Open Cellular Clouds Observed During COMBLE: Evaluation of Parameterized Turbulence Closure

Marine cold-air outbreaks, or CAOs, are airmass transformations whereby relatively cold boundary layer (BL) air is transported over relatively warm water. To more deeply understand BL and mixed-phase cloud properties during CAO conditions, the Cold-Air Outbreaks in the Marine Boundary Layer Experiment (COMBLE) took place from late 2019 into early 2020. During COMBLE, the U.S. Department of Energy's first Atmospheric Radiation Measurement Mobile Facility (AMF1) was deployed to Andenes, Norway, far downstream (~1,000 km) from the Arctic pack ice. This study examines the two most intense CAOs sampled at the AMF1 site. The observed BL structures are open cellular with high (~3–5 km) and cold (–30 to –50 °C) cloud tops, and they often have pockets of high liquid water paths (LWPs; up to ~1,000 g m –2 ) associated with strong updrafts and enhanced turbulence. We use a high-resolution mesoscale model to explore how well four turbulence closure methods represent open cellular clouds. After applying a radar simulator to model outputs for direct evaluation, cloud top properties agree well with AMF1 observations (within ~10%), but radar reflectivity and LWP agreement is more variable. Results suggest that the turbulent Prandtl number may play an important role for the simulated BL and cloud properties. All simulations produce enhanced precipitation rates that are well-correlated with a cloud transition. Finally, the eddy-diffusivity/mass-flux approach produces the deepest cloud layer and therefore the largest and most coherent cellular structures. Furthermore, we recommend the use of a non-local turbulence closure approach to better capture turbulent processes in intense CAOs.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Tropical Cirrus in Global Storm-Resolving Models. Part II: Cirrus Life Cycle and Top-of-Atmosphere Radiative Fluxes

Cirrus clouds of various thicknesses and radiative characteristics extend over much of the tropics, especially around deep convection. They are difficult to observe due to their high altitude and sometimes small optical depths. They are also difficult to simulate in conventional global climate models, which have coarse grid spacings and simplified parameterizations of deep convection and cirrus formation. We investigate the representation of tropical cirrus in global storm-resolving models (GSRMs), which have higher spatial resolution and explicit convection and could more accurately represent cirrus cloud processes. This study uses GSRMs from the DYnamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains (DYAMOND) project. The aggregate life cycle of tropical cirrus is analyzed using joint albedo and outgoing longwave radiation (OLR) histograms to assess the fidelity of models in capturing the observed cirrus cloud populations over representative tropical ocean and land regions. The proportions of optically-thick deep convection, anvils, and cirrus vary across models and are portrayed in the vertical distribution of cloud cover and top-of-atmosphere radiative fluxes. Model differences in cirrus populations, likely driven by subgrid processes such as ice microphysics, dominate over regional differences between convectively-active tropical land and ocean locations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Sensitivity of deep convection and cross-tropopause water transport to microphysical parameterizations in WRF

Deep convective storms can overshoot the tropopause, thus altering the composition of the stratosphere by vertically transporting tropospheric air. The transport of water vapor and ice particles into a sub-saturated environment can hydrate the stratosphere, with implications for radiative forcing and ozone chemistry. Cloud-resolved models, if employed at high spatial resolutions, are used to probe process-level questions about cross-tropopause deep convective hydration and its controls. There is considerable diversity in model representations of processes associated with water transport and transformation, and the choice of a microphysics scheme affects model skill in simulating deep convective events. This motivates our evaluation of state-of-the-art, as well as widely used standard schemes, in a high spatial- and temporal-resolution framework. Six bulk microphysics schemes were employed in a WRF-LES setup, initialized with a sounding profile representative of a tropopause-overshooting storm. Here, we used an idealized framework to isolate the effect of microphysics on the dominant processes that control the reach of deep convection and stratospheric hydration. All schemes produced the highest reaching updrafts 8-12 hours into the simulation but the strength and persistence of updrafts varied across the schemes; maximum storm heights ranged 9.1-12.6 km across the schemes. Varying microphysics produced large differences in the vertical extent and horizontal aggregation of convection, and an order of magnitude spread in above-tropopause water vapor concentrations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Overview of the MOSAiC expedition—Atmosphere

With the Arctic rapidly changing, the needs to observe, understand, and model the changes are essential. To support these needs, an annual cycle of observations of atmospheric properties, processes, and interactions were made while drifting with the sea ice across the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from October 2019 to September 2020. An international team designed and implemented the comprehensive program to document and characterize all aspects of the Arctic atmospheric system in unprecedented detail, using a variety of approaches, and across multiple scales. These measurements were coordinated with other observational teams to explore cross-cutting and coupled interactions with the Arctic Ocean, sea ice, and ecosystem through a variety of physical and biogeochemical processes. This overview outlines the breadth and complexity of the atmospheric research program, which was organized into 4 subgroups: atmospheric state, clouds and precipitation, gases and aerosols, and energy budgets. Atmospheric variability over the annual cycle revealed important influences from a persistent large-scale winter circulation pattern, leading to some storms with pressure and winds that were outside the interquartile range of past conditions suggested by long-term reanalysis. Similarly, the MOSAiC location was warmer and wetter in summer than the reanalysis climatology, in part due to its close proximity to the sea ice edge. The comprehensiveness of the observational program for characterizing and analyzing atmospheric phenomena is demonstrated via a winter case study examining air mass transitions and a summer case study examining vertical atmospheric evolution. Overall, the MOSAiC atmospheric program successfully met its objectives and was the most comprehensive atmospheric measurement program to date conducted over the Arctic sea ice. The obtained data will support a broad range of coupled-system scientific research and provide an important foundation for advancing multiscale modeling capabilities in the Arctic.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea

The Arctic is rapidly transforming due to sea ice loss, increasing shipping activity, and oil and gas development. Associated marine and combustion emissions influence atmospheric aerosol composition, impacting complex aerosol–cloud–climate feedbacks. To improve understanding of the sources and processes determining Arctic aerosol composition, atmospheric particles were collected aboard the Korean icebreaker R/V Araon cruising within the Bering Strait and Chukchi Sea during August 2016. Offline analyses of individual particles by microspectroscopic techniques, including scanning electron microscopy with energy dispersive X-ray spectroscopy and atomic force microscopy with infrared spectroscopy, provided information on particle size, morphology, and chemical composition. The most commonly observed particle types were sea spray aerosol (SSA), comprising ~60–90%, by number, of supermicron particles, and organic aerosol (OA), comprising ~50–90%, by number, of submicron particles. Sulfate and nitrate were internally mixed within both SSA and OA particles, consistent with particle multiphase reactions during atmospheric transport. Within the Bering Strait, SSA and OA particles were more aged, with greater number fractions of particles containing sulfate and/or nitrate, compared to particles collected over the Chukchi Sea. This is indicative of greater pollution influence within the Bering Strait from coastal and inland sources, while the Chukchi Sea is primarily influenced by marine sources.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

The Two Arctic Wintertime Boundary Layer States: Disentangling the Role of Cloud and Wind Regimes in Reanalysis and Observations During MOSAiC

The wintertime central Arctic atmosphere comprises a radiatively clear and a radiatively opaque state, which are linked to synoptic forcing and mixed-phase clouds. Weather and climate models often lack process representations surrounding these states, but prior work mostly treated the problem as an aggregate of synoptic conditions, resulting in partially overlapping biases. Here, we disaggregate the Arctic states and confront ERA5 reanalysis with observations from the MOSAiC campaign over the central Arctic sea ice during winter 2019/2020. Low-level winds and liquid water path (LWP) are combined to derive different synoptic classes. Results show that the clear state is primarily formed by weak/moderate winds and the absence of liquid-bearing clouds, while strong winds and enhanced LWP primarily form the radiatively opaque state. ERA5 struggles to reproduce these basic statistics, shows too weak sensitivity of thermal radiation to synoptic forcing, and overestimates thermal radiation for similar LWP amounts. The latter is caused by a warm bias, which has a pronounced inversion structure and is largest in clear and calm conditions. Under strong synoptic forcing, the warm bias is constant with height and discrepancies in mixed-phase cloud altitude appear. Separating synoptic conditions is regarded as useful for process-oriented evaluation of the Arctic troposphere in models.

54 ENVIRONMENTAL SCIENCES↗