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At least 415 records · Page 23

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NASA NTRS1992

Remote sensing of aerosols with the Earth Observing Scanning Polarimeter

Tropospheric aerosols have potential climate forcing roles through both the direct effect on solar radiation scattered and absorbed and the indirect effect as condensation nuclei for cloud particles. Present capabilities for characterizing the global aerosol climatology are limited by the existing satellite remote sensing measurements, making a quantitative determination of the climate forcing effects of aerosols rather difficult and uncertain. The Earth Observing Scanning Polarimeter (EOSP) instrument under consideration for Earth Observing System (EOS) mission platforms and for a proposed Climsat Earth Probe mission is intended to provide global mapping with multispectral photopolarimetry, which can be exploited for the more pronounced aerosol signature in the polarization of the scattered light as compared to the radiance. We describe the essential features and performance specifications of the EOSP instrument and discuss approaches for retrieving tropospheric aerosol properties from multispectral photopolarimetry.

Travis, Larry D.↗

NASA NTRS1993

Investigation of passive atmospheric sounding using millimeter and submillimeter wavelength channels

Progress by investigators at the Georgia Institute of Technology in the development of techniques for passive microwave retrieval of water vapor, cloud, and precipitation parameters using millimeter- and sub-millimeter wavelength channels is reviewed. Channels of particular interest are in the tropospheric transmission windows at 90, 166, 220, 340, and 410 GHz and centered around the water vapor lines at 183 and 325 GHz. Collectively, these channels have potential application in high-resolution mapping (e.g., from geosynchronous orbit), remote sensing of cloud and precipitation parameters, and retrieval of water vapor profiles. During the period from 1 Jan. 1993 through 30 Jun. 1993 the Millimeter-wave Imaging Radiometer (MIR) completed data flights during a two-month long deployment in conjunction with TOGA/COARE. Coincident data was collected from several other ground-based, airborne, and satellite sensors, including the NASA/MSFC AMPR, MIT MTS, DMSP SSM/T-2 satellite, collocated radiosondes, ground- and aircraft-based radiometers and cloud lidars, airborne infrared imagers, solar flux probes, and airborne cloud particle sampling probes.

Gasiewski, A. J.↗

NASA NTRS1990

New findings and instrumentation from the NASA Lewis Microgravity Facility

The study of fundamental combustion and fluid physics phenomena in microgravity enables a new range of experiments to be performed since buoyancy-type flows are nearly eliminated, normally obscured forces and flows may be isolated, gravitational settling or sedimentation is nearly eliminated, and larger time or length scales in experiments become permissible. Some new phenomena found through ground-based microgravity research at NASA facilities is reviewed along with the instrumentation and drop tower facilities used in the research. Experiments are described in the areas of premixed gas combustion, droplet combustion, particle cloud combustion, liquid reorientation, and two-phase flow patterns. Future plans for instrumentation development are also outlined.

Ross, Howard D.↗

NASA NTRS1994

Cometary dust: A thermal criterion to identify cometary samples among the collected interplanetary dust

The relative proportions of the cometary and the asteroidal contributions to the interplanetary dust have not yet been definitively established. These proportions may vary with time as a result of major catastrophic disruptions in the main belt or the appearance of fresh, active comets. Dermott et al. and Reach suggest the debris from catastrophic collisions in the main belt can account for most of the zodiacal cloud particles. Earth collection of these asteroidal particles is strongly favored by near-Earth gravitational enhancement. However, comets are observed to produce interplanetary dust particles (IDP's), and the identification of cometary IDP's would allow inferences of the compositions, mineralogies, and physical properties of the comets. The peak temperatures reached by IDP's on atmospheric entry indicate the distribution of IDP velocities. Each IDP contains many internal thermometers: minerals that transform above certain temperatures, volatile elements that are lost sequentially with increasing temperatures, solar flare tracks that anneal at different temperatures in different minerals, and solar-implanted noble gases that outgas progressively with temperature. Thus, limits on the peak temperature reached by each IDP on Earth atmospheric entry can be set. Other aspects of this investigation are covered.

Flynn, George J.↗

NASA NTRS1993

Use of stratospheric aerosol properties as diagnostics of Antarctic vortex processes

Physical properties of the stratospheric aerosol population are inferred from cloud-free SAGE II multiwavelength extinction measurements in the Antarctic during late summer (February/March) and spring (September/October, November). Seasonal changes in these properties are used to infer physical processes occurring in the Antarctic stratosphere over the course of the winter. The analysis suggests that the apparent springtime cleansing of the Antarctic stratosphere is the result of aerosol redistribution through subsidence of the polar vortex air mass and sedimentation of large polar stratospheric cloud particles. The analysis also suggests that vortex processes are responsible for a significant downward transport of aerosol through the tropopause.

Thomason, Larry W.↗

NASA NTRS1995

HCl Vapour Pressures and Reaction Probabilities for ClONO2 + HCl on Liquid H2SO4-HNO3-HCl-H20 Solutions

Henry's Law solubility constants for HCl have been measured for liquid H2SO4-HNO3-HCl-H2O solutions; the results are in good agreement with predictions from published semiempirical models. The ClONO2 + HCl reaction on the surfaces of such solutions with compositions simulating those of stratospheric aerosols has been investigated; as the composition changes following the temperature drop characteristic of the high-latitude stratosphere the reaction probability gamma increases rapidly. Furthermore, the gamma values remain essentially unchanged when HN03 uptake is neglected; the controlling factor appears to be the solubility of HCl. These results corroborate our earlier suggestion that supercooled liquid sulfate aerosols promote chlorine activation at low temperatures as efficiently as solid polar stratospheric cloud particles.

Elrod, M. J.↗

NASA NTRS1994

Heterogeneous Interactions of ClONO2 and HCl with Sulfuric Acid Tetrahydrate: Implications for the Stratosphere

The reaction probabilities for ClONO2+H2O- HOCl + HNO3 and ClONO2+ HCl Cl2 +HNO3 have been investigated on sulfuric acid tetrahydrate (SAT, H2SO4-4H2O)surfaces at temperatures between 190 and 230 K and at reactant concentrations that are typical in the lower stratosphere, using a fast-flow reactor coupled to a quadrupole mass spectrometer. The results indicate that the reaction probabilities as well as HCl uptake depend strongly on the thermodynamic state of SAT surface: they decrease significantly with decreasing H2O partial pressure at a given temperature, and decrease with increasing temperature at a given H2O partial pressure, as the SAT changes from the H2O-rich form to the H2SO4-rich form. For H2O-rich SAT at 195 K gamma(sub 1) approx. = -0.01 and gamma(sub 2) greater or equal to 0.1, whereas the values for H2SO4-rich SAT decrease by more than 2 orders of magnitude. At low concentrations of HCl, close to those found in the stratosphere, the amount of HCl taken up by H2O-rich SAT films corresponds to a coverage of the order of a tenth of a monolayer (approx. = 10(exp 14) molecules/sq cm); H2SO4-rich SAT films take up 2 orders of magnitude less HCl (les than 10(exp 12) molecules/sq cm). Substantial HCl uptake at high HCl concentrations is also observed, as a result of surface melting. The data reveal that frozen stratospheric sulfate aerosols may play an important role in chlorine activation in the winter polar stratosphere via processes similar to those occurring on the surfaces of polar stratospheric cloud particles.

Zhang, Renyi↗

NASA NTRS1999

Land-Ocean Differences in LIS and OTD Tropical Lightning Observations

Significant differences are known to exist on a global scale between continental and oceanic total lightning regional flash rates, suggesting differences in the properties of convective storms in these regimes. Lightning properties observed by the Optical Transient Detector (OTD) and Lightning Imaging Sensor (LIS) over land and ocean are compared, limited to analysis over the tropics in order to simplify physical interpretation. We find that the mean flash rates of individual storms over tropical land only exceed those over ocean by a factor of 2 (far less than the observed differences in regional flash rates). However, the average nearest neighbor distance of continental thunderstorms in half that over oceans. Cloud-top lightning optical radiance in oceanic storms is also twice as large as over land, suggesting either more energetic flashes over the oceans or less intervening cloud particles.

Boccippio, Dennis J.↗

NASA NTRS1999

Land-Ocean Differences in LIS and OTD Tropical Lightning Observations

Significant differences are known to exist on a global scale between continental and oceanic total lightning regional flash rates, suggesting differences in the properties of convective storms in these regimes. Lightning properties observed by the Optical Transient Detector (OTD) and Lightning Imaging Sensor (LIS) over land and ocean are compared, limited to analysis over the tropics in order to simplify physical interpretation. We find that the mean flash rates of individual storms over tropical land only exceed those over ocean by a factor of 2 (far less than the observed differences in regional flash rates). However, the average nearest neighbor distance of continental thunderstorms is half that over oceans. Cloud-top lightning optical radiance in oceanic storms is also twice as large as over land, suggesting either more energetic flashes over the oceans or less intervening cloud particles.

Boccippio, D. J.↗

NASA NTRS1999

The Infrared Spectral Imaging Radiometer and Laser Altimeter on STS-85 (an Aircraft Style Experiment Flown in Space)

Improvements in the remote sensing of clouds from space in the future will come from instruments with higher spatial and spectral resolution on more platforms and supported by active sounding. The space shuttle hitchhiker system allows new measurements to be prototyped in space with costs, operating flexibility and data volumes similar to aircraft experiments. The Infrared Spectral Imaging Radiometer and Shuttle Laser Altimeter hitchhiker experiment was flown in 1997. The experiment tested the use of uncooled thermal infrared imaging, laser cloud altitude measurements and high spatial resolution, tri-spectral sensing of cloud particle size and phase. A 1/4 km resolution, fifty orbit data set was obtained from STS-85. The presentation will focus on the use of the shuttle as an experiment platform and cover possible transition to the space station in the future.

Spinhirne, James D.↗

NASA NTRS1995

Freezing Behavior of Stratospheric Sulfate Aerosols Inferred from Trajectory Studies

Temperature histories based on 10-day back growth trajectories for six ER-2 flights during AASE I (1989) and AAOE (1987) are presented. These trajectories along with the properties of the observed PSC (polar stratospheric cloud) particles are used here to infer the physical state of the pre-existing sulfuric acid aerosols. Of all the ER-2 flights described here, only the PSCs observed on the flights of January 24 and 25, 1989 are consistent with the thermodynamics of liquid ternary solutions of H2SO4/HNO3/H2O Ib PSCs). For these two days, back trajectories indicate that the air mass was exposed to SAT (sulfuric acid tetrahydrate) melting temperatures about 24 hours prior to being sampled by the ER-2. For the remaining ER-2 flights (January, 16, 19, and 20 for the AASE I campaign and August 17 for the AAOE campaign), the observed PSCs were probably composed of amorphous solid solutions of HNO3 and H2O (Type Ic PSCs). Formation of such Type Ic PSCs requires the presence of solid H2SO4 aerosols since liquid aerosols yield ternary solutions. The 10-day back trajectories of these flights indicate that the air mass was not exposed to SAT melting temperatures during the past week and had experienced cooling/warming cycles prior to being sampled by the ER-2. These temperature histories, recent laboratory measurements and the properties of glassy solids suggest that stratospheric H2SO4 aerosols may undergo a phase transition to SAT upon warming at approximately 198 K after going through a cooling cycle to about 194 K or lower.

Tabazadeh, A.↗

NASA NTRS1999

Water Ice Cloud Opacities and Temperatures Derived from the Viking IRTM Data Set

The degree to which water ice clouds play a role in the Mars climate is unknown. Latent heating of water ice clouds is small and since most hazes appeared to be thin (tau less than or = 1) their radiative effects have been neglected. Condensation likely limits the vertical extent of water vapor in the water column and a lowering of the condensation altitude, as seen in the northern spring and summer, could increase the seasonal exchange of water between the atmosphere and the surface. It has been suggested that water ice cloud formation is more frequent and widespread in the aphelic hemisphere (currently the northern). This may limit water to the northern hemisphere through greater exchange with the regolith and through restricted southward transport of water vapor by the Mars Hadley circulation. In addition, it has been suggested that water ice cloud formation also controls the vertical distribution of atmospheric dust in some seasons. This scavenging of dust may Continuing from the IRTM cloud maps, derived cloud opacities and cloud temperatures for several locations and seasons will be presented. Sensitivities to cloud particle sizes, surface temperature, and dust opacity will be discussed.

TamppariL. K.↗

NASA NTRS2000

What Controls the Temperature of the Arctic Stratosphere during the Spring?

Understanding the mechanisms that control the temperature of the polar lower stratosphere during spring is key to understanding ozone loss in the Arctic polar vortex. Spring ozone loss rates are directly tied to polar stratospheric temperatures by the formation of polar stratospheric clouds, and the conversion of chlorine species to reactive forms on these cloud particle surfaces. In this paper, we study those factors that control temperatures in the polar lower stratosphere. We use the National Centers for Environmental Prediction (NCEP)/NCAR reanalysis data covering the last two decades to investigate how planetary wave driving of the stratosphere is connected to polar temperatures. In particular, we show that planetary waves forced in the troposphere in mid- to late winter (January-February) are principally responsible for the mean polar temperature during the March period. These planetary waves are forced by both thermal and orographic processes in the troposphere, and propagate into the stratosphere in the mid and high latitudes. Strong mid-winter planetary wave forcing leads to a warmer Arctic lower stratosphere in early spring, while weak mid-winter forcing leads to cooler Arctic temperatures.

Newman, Paul A.↗

NASA NTRS2001

HO(x) Measurements in PEM Tropics B with the Airborne Tropospheric Hydrogen Oxides Sensor (ATHOS)

The primary objective of PEM Tropics B was to study the processes responsible for the production and loss of tropospheric ozone over the tropical Pacific. This region of the globe contains very clean air as well as aged, polluted air that was advected from both the Asian and American continents. Understanding ozone requires understanding of HO(x) (HO(x) = OH + HO2) chemistry, since the reaction between H02 and NO leads to ozone production and the production of OH often requires ozone loss. In addition, OH is the atmosphere's primary oxidant. Since most atmospheric oxidation is thought to occur in the tropical lower troposphere, measurements during PEM Tropics B should provide an important test of the OH abundances and distributions. Thus, understanding and thoroughly testing HO(x) processes was an important objective of PEM Tropics B. Several issues need to be tested, One is HO, production rates and sources, since HO,, production directly affects ozone production and loss. Another is HO(x) behavior in and around clouds, since HO(x) is lost to cloud particles, but convection may bring HO(x) precursors from near the surface to the upper troposphere. A third is the rise and fall of HO(x) at sunrise and sunset, since these variations give strong indications of the important sources and sinks of HO(x). Making and interpreting high-quality OH and H02 measurements from the NASA DC-8 during PEM Tropics B is the objective of this research effort.

Brune, William H.↗

NASA NTRS2001

Volcanoes, Polar Clouds and Arctic Ozone

Satellite observations and model calculations show 5 to 10% local column ozone loss in some tropical and mid latitude locations, following El Chichon and Mount Pinatubo eruptions. The rapid deepening of the Antarctic ozone hole in the early 1980s has also been partially attributed to chemistry on volcanic aerosols from a number of large eruptions. Here the effects of volcanoes on Arctic polar processes are explored. Large polar stratospheric cloud particles that cause denitrification cannot form in a volcanically perturbed environment. Denitrification can increase Arctic ozone loss by up to 30% in a future colder climate. However, we show that enhanced chemical processing on volcanic aerosols can increase Arctic ozone loss in a cold year by about 60% independent of denitrification. A coupled chemistry-microphysics model is used to show that widespread distribution of volcanic aerosols in 2000 could have caused severe springtime ozone depletion in the Arctic stratosphere. While, volcanic aerosols can strongly affect the current Arctic column ozone abundance in a cold year, denitrification effects on ozone can only become important in a much colder lower stratosphere.

Tabazadeh, Azadeh↗

NASA NTRS2000

An NOy Algorithm for Arctic Winter 2000

NOy, total reactive nitrogen, and the long-lived tracer N2O, nitrous oxide, were measured by both in situ and remote sensing instruments during the Arctic winter 1999-2000 SAGE III Ozone Loss and Validation Experiment (SOLVE). The correlation function NOy:N2O observed before the winter Arctic vortex forms, which is known as NOy(sup), is an important reference relationship for conditions in the evolving vortex. NOy(sup) can, with suitable care, be used to quantify vortex denitrification by sedimentation of polar stratospheric cloud particles when NOy data is taken throughout the winter. Observed NOy values less than the reference value can be interpreted in terms of semi-permanent removal of active nitrogen by condensation and sedimentation processes. In this paper we present a segmented function representing NOy(sup) applicable over the full range of altitudes sampled during SOLVE. We also assess the range of application of this function and some of its limitations.

Loewenstein, M.↗

NASA NTRS2002

Microphysics and Radiative Properties of Cirrus: Instrumentation and Analysis

Work under this grant has involved further development of a new aircraft instrument (the cloudscope) for real time characterization of atmospheric particulates together with field observations of such particulates, both in the form of ice and also as nuclei responsible for nucleation of both ice and water cloud particles. Part of the work involving assessment of the frequency of ice crystal shapes has been carried out in collaboration with the Meteorological Service of Canada; part of the work in a field program with the NCAR C-130. Part of the work has been interpreted in terms of laboratory simulation of ice crystal growth under a wide variety of conditions carried out under a grant from Physical Meteorology Program, National Science Foundation.

Hallett, John↗

NASA NTRS2003

Modeling Aerosol Nucleation

The goal of this work has been to understand how nitric acid condenses on cirrus ice cloud particles by analyzing data obtained during the SAGE III Ozone Loss and Validation Experiment (SOLVE) research mission based out of Kiruna, Sweden. Ms. Gamblin simultaneously analyzed gas phase nitric acid data along with particulate NO, data, particulate, vapor and gas-phase water data from several different instruments, particle size data, which included surface area and volume measurements, ozone concentration data as well as temperature, pressure and GPS coordinates of the sampled air parcel. All parameters where held constant with only one allowed to vary in order to determine what controls the extent to which nitric acid will condensation on ice. In addition, this data was compared to theoretical values of nitric acid condensation on ice based upon recent laboratory data. Comparison of these two data sets shows the field data does not agree with what is expected in the laboratory at comparable temperatures and nitric acid pressures. The most significant difference is that surface coverages in the atmosphere were found to be elevated relative to surface coverages measured in the laboratory. The results of this study were accepted for publication by Geophysical Research Letters.

Toon, Owen B.↗