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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 415 records · Page 23
All sourcesNASA NTRSDOE OSTI
DOE OSTI2017

Advanced Fuel Cycle Cost Basis – 2017 Edition

This report, commissioned by the U.S. Department of Energy (DOE) Office of Nuclear Energy (NE), provides a comprehensive set of cost data supporting a cost analysis for the relative economic comparison of options for use in the DOE Nuclear Technology Research and Development (NTRD) Program (previously the Fuel Cycle Research and Development (FCRD) and the Advanced Fuel Cycle Initiative (AFCI)). The report describes the NTRD cost basis development process, reference information on NTRD cost modules, a procedure for estimating fuel cycle costs, economic evaluation guidelines, and a discussion on the integration of cost data into economic computer models. This report contains reference cost data for numerous fuel cycle cost modules (modules A-O) as well as cost modules for a number of reactor types (R modules). The fuel cycle cost modules were developed in the areas of natural uranium mining and milling, thorium mining and milling, conversion, enrichment, depleted uranium disposition, fuel fabrication, interim spent fuel storage, reprocessing, waste conditioning, spent nuclear fuel (SNF) packaging, long-term monitored retrievable storage, managed decay storage, recycled product storage, near surface disposal of low-level waste (LLW), geologic repository and other disposal concepts, and transportation processes for nuclear fuel, LLW, SNF, transuranic, and high-level waste. Since its inception, this report has been periodically updated. The last such internal document was published in August 2015 while the last external edition was published in December of 2009 as INL/EXT-07-12107 and is available on the Web at URL: www.inl.gov/technicalpublications/Documents/4536700.pdf. This current report (Sept 2017) is planned to be reviewed for external release, at which time it will replace the 2009 report as an external publication. This information is used in the ongoing evaluation of nuclear fuel cycles by the NE NTRD program.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2021

Single-component-at-a-time variation study for glass-ceramic waste forms

Here, a 51-sample composition variation study was performed on glass-ceramic waste forms for a raffinate waste stream from aqueous reprocessing of used nuclear fuel containing high fractions of Mo, alkalis, alkaline earths (AEs), and rare earths (REs). The study was designed with a single-component-at-a-time variation approach off a centroid composition. The components that were varied included Al, B, Ca, Li, Mo, Na, REs, Si, Zr, and Others (containing minor components). Data analysis included crystallization curves, microstructure, and phase compositions. A number of components (i.e., Li 2 O, B 2 O 3 , REO x , MoO 3 , Na 2 O, and ZrO 2 ) significantly impacted the concentration and chemistry of phases, especially the primary phases of oxyapatite [i.e., Ca 2 RE 8 (SiO 4 ) 6 O 2 ] and powellite (i.e., AEMoO 4 ), precipitated in the slow-cool heat-treated waste forms; minor phases included cerianite [i.e., Ce x Zr (1-x) O 2 ], Ba-molybdate [i.e., Ba(Gd 0.67 Mo 0.33 O 3 ], noble metals, pollucite (i.e., CsAlSiO 4 ), and RE-borosilicate (i.e., RE 3 BSi 2 O 10 ).

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
NASA NTRS1990

Rapid variability of the iron fluorescence line from the Seyfert 1 galaxy NGC6814

NGC6814, one of the faster X-ray-variable AGN, has been observed with the Large Area Counters aboard the Ginga satellite in order to obtain data on the variability of the iron fluorescence line and thus to constrain the distribution of cold gas from which the line originates. A positive correlation measured between the variability of the iron-line flux and the continuum emission suggests an upper limit of 10 to the 14th cm for the size of the ion reprocessing region.

Kunieda, Hideyo↗
NASA NTRS2006

Satellite Estimates of Surface Short-wave Fluxes: Issues of Implementation

Surface solar radiation reaching the Earth's surface is the primary forcing function of the land surface energy and water cycle. Therefore, there is a need for information on this parameter, preferably, at global scale. Satellite based estimates are now available at accuracies that meet the demands of many scientific objectives. Selection of an approach to estimate such fluxes requires consideration of trade-offs between the use of multi-spectral observations of cloud optical properties that are more difficult to implement at large scales, and methods that are simplified but easier to implement. In this study, an evaluation of such trade-offs will be performed. The University of Maryland Surface Radiation Model (UMD/SRB) has been used to reprocess five years of GOES-8 satellite observations over the United States to ensure updated calibration and improved cloud detection over snow. The UMD/SRB model was subsequently modified to allow input of information on aerosol and cloud optical depth with information from independent satellite sources. Specifically, the cloud properties from the Atmospheric Radiation Measurement (ARM) Satellite Data Analysis Program (Minnis et al., 1995) are used to drive the modified version of the model to estimate surface short-wave fluxes over the Southern Great Plain ARM sites for a twelve month period. The auxiliary data needed as model inputs such as aerosol optical depth, spectral surface albedo, water vapor and total column ozone amount were kept the same for both versions of the model. The estimated shortwave fluxes are evaluated against ground observations at the ARM Central Facility and four satellite ARM sites. During summer, the estimated fluxes based on cloud properties derived from the multi-spectral approach were in better agreement with ground measurements than those derived from the UMD/SRB model. However, in winter, the fluxes derived with the UMD/SRB model were in better agreement with ground observations than those estimated from cloud properties provided by the ARM Satellite Data Analysis Program. During the transition periods, the results were comparable.

Wang, H.↗
NASA NTRS2012

Calibration Adjustments to the MODIS Aqua Ocean Color Bands

After the end of the SeaWiFS mission in 2010 and the MERIS mission in 2012, the ocean color products of the MODIS on Aqua are the only remaining source to continue the ocean color climate data record until the VIIRS ocean color products become operational (expected for summer 2013). The MODIS on Aqua is well beyond its expected lifetime, and the calibration accuracy of the short wavelengths (412nm and 443nm) has deteriorated in recent years_ Initially, SeaWiFS data were used to improve the MODIS Aqua calibration, but this solution was not applicable after the end of the SeaWiFS mission_ In 2012, a new calibration methodology was applied by the MODIS calibration and support team using desert sites to improve the degradation trending_ This presentation presents further improvements to this new approach. The 2012 reprocessing of the MODIS Aqua ocean color products is based on the new methodology.

Meister, Gerhard↗
NASA NTRS1999

RXTE Observation of Cygnus X-1: III. Implications for Compton Corona and ADAF Models: Implications for Compton Corona and ADAF Models - Report 3

We have recently shown that a 'sphere + disk' geometry Compton corona model provides a good description of Rossi X-ray Timing Explorer (RXTE) observations of the hard/low state of Cygnus X-1. Separately, we have analyzed the temporal data provided by RXTE. In this paper we consider the implications of this timing analysis for our best-fit 'sphere + disk' Comptonization models. We focus our attention on the observed Fourier frequency-dependent time delays between hard and soft photons. We consider whether the observed time delays are: created in the disk but are merely reprocessed by the corona; created by differences between the hard and soft photon diffusion times in coronae with extremely large radii; or are due to 'propagation' of disturbances through the corona. We find that the time delays are most likely created directly within the corona; however, it is currently uncertain which specific model is the most likely explanation. Models that posit a large coronal radius [or equivalently, a large Advection Dominated Accretion Flow (ADAF) region] do not fully address all the details of the observed spectrum. The Compton corona models that do address the full spectrum do not contain dynamical information. We show, however, that simple phenomenological propagation models for the observed time delays for these latter models imply extremely slow characteristic propagation speeds within the coronal region.

Nowak, Michael A.↗
DOE OSTI2016

Adsorption of iodine on hydrogen-reduced silver-exchanged mordenite: Experiments and modeling

The adsorption process of iodine, a major volatile radionuclide in the off-gas streams of spent nuclear fuel reprocessing, on hydrogen-reduced silver-exchanged mordenite (Ag 0 Z) was studied at the micro-scale. The gas-solid mass transfer and reaction involved in the adsorption process were investigated and evaluated with appropriate models. Optimal conditions for reducing the silver-exchanged mordenite (AgZ) in a hydrogen stream were determined. Kinetic and equilibrium data of iodine adsorption on Ag 0 Z were obtained by performing single-layer adsorption experiments with experimental systems of high precision at 373–473 K over various iodine concentrations. Results indicate approximately 91% to 97% of the iodine adsorption was through the silver-iodine reaction. The effect of temperature on the iodine loading capacity of Ag 0 Z was discussed. In conclusion, the Shrinking Core model describes the data well, and the primary rate controlling mechanisms were macro-pore diffusion and silver-iodine reaction. © 2016 American Institute of Chemical Engineers AIChE J, 2016

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
NASA NTRS2019

MODIS Aqua Reflective Solar Bands Calibration for NASA's R2018 Ocean Color Products

Remote sensing ocean color products have stringent requirements on radiometric calibration stability. To address a calibration deficiency in MODIS Aqua in recent years, the NASA Ocean Biological Processing Group (OBPG) developed a new calibration for the reflective solar bands. Prior to the reprocessing of NASA's ocean color products for 2018 (R2018), the OBPG MODIS products had been based on calibration provided by the MODIS Calibration Support Team (MCST). Several modifications were made to the MCST calibration approach to improve the calibration accuracy for ocean color products. These include: 1) apply 936nm detector normalization to solar diffuser stability monitor (SDSM) data to reduce coherent noise; 2) modeling solar diffuser (SD) degradation wavelength dependency to determine SD degradation in near-infrared and shortwave infrared wavelength; 3) detector gains are computed using SD screen-closed data to better match ocean radiance levels in all bands; 4) a simple atmospheric correction is performed to reduce bidirectional reflectance distribution function (BRDF) effects in desert trends; 5) modulated relative spectral response (RSR) impact on ocean data is estimated and used to adjust the calibration coefficients. 6) smoothing is used to characterize the temporal change in calibration, and response versus scan angle (RVS) changes are characterized using 2nd order polynomials to improve spatial/temporal calibration stability. Relative to the previous R2014 ocean color products, the R2018 calibration removed the suspect late-mission global trends in blue-band water-leaving reflectance, and some anomalously large short-term variability (spikes) in the temporal trend of chlorophyll concentration. This paper will describe the OBPG calibration with a focus on the differences between the MCST and OBPG approaches.

calibration↗
DOE OSTI2020

Zinc-in-titania waste form for immobilizing lanthanide fission products from electrochemical reprocessing

This paper provides microstructural, microchemical, and bulk X-ray diffraction information for a zinc-in-titania waste form for immobilizing rare-earth oxide (REOx) fission products recovered through precipitation from electrochemical salt wastes. This waste form can be used to immobilize REOx at loadings as high as 40 mass% in a chemically durable matrix consisting of glass-bonded minerals including Zn2TiO4 as well as RE-containing phases of REOx, RE2Ti2O7, and REPO4 (monazite). Chemical durability data is also provided, and comparisons are drawn between this waste form and one made using a similar process with half the REOx loading.

rare earth, rare earth waste form, electrochemical↗
DOE OSTI2024

Assessment of uranium nitride interatomic potentials

Uranium mononitride (UN) is a promising nuclear fuel due to its high fissile density, high thermal conductivity, and suitability for reprocessing. In this study, two uranium nitride interatomic potentials are assessed: Tseplyaev and Starikov's angular-dependent potential and Kocevski et al.'s embedded atom model potential. Predictions of the thermophysical and elastic properties of UN, UN 2 , and α- and β-U 2 N 3 computed using both potentials are assessed and compared to available experimental data. Notably, the Tseplyaev potential performs better with the energetic aspects of UN, e.g., specific heat capacity and point defect formation energies, whereas the Kocevski potential performs better with the structural aspects of UN, e.g., thermal expansion as well as with the elastic properties. The reasons why the Kocevski potential underestimates the UN specific heat are explained by examining the UN phonon properties modeled using both potentials. The Kocevski potential shows better identification of the mechanical stability ranges of UN, UN 2 , and α- and β-U 2 N 3 , reasonably predicting the melting point of UN and predicting stable structures for UN 2 and α- and β-U 2 N 3 . On the other hand, the Tseplyaev potential predicts a premature phase change of both UN and UN 2 and cannot stabilize α- nor β-U 2 N 3 . However, the Kocevski potential cannot predict a stable α-U phase and is thus not suitable for the calculation of formation energies for non-stoichiometric point defects.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
NASA NTRS1989

Gamma ray bursts from magnetospheric plasma oscillations

Neutron star Magnetospheric Plasma Oscillations (MPO), can account for the energetics, decay time scale, and spectra of typical Gamma Ray Bursts (GRBs). The soft photon source is likely to be due to backwarming of the reprocessing boundary by the incipient gamma rays. It is shown that the observed fraction of bursts displaying low energy absorption features may be understood in the context of an MPO model. Moreover, it is found that GRB spectra should display these cyclotron lines about 18 percent of the time, which is consistent with the KONUS and Ginga sets of data.

Melia, Fulvio↗
NASA NTRS2007

Comparison of TWP-ICE Satellite and Field Campaign Aircraft Derived Cloud Properties

Cloud and radiation products derived from the MTSAT-1R satellite have been developed for TWP-ICE. These include pixel-level, gridded, and ground site and aircraft matched. These products are available from the Langley website and the ARM data center. As shown in Figs 2, and 4-6, these products compare favorably with in-situ ground and aircraft based measurements. With additional quantitative validation these products can provide valuable information about tropical convection and its impact on the radiation budget and climate. As new algorithm improvements, such as multi-layer cloud detection, are implemented these products will be reprocessed and updated.

Ayers, J. K.↗
DOE OSTI2024

Adsorption of molecular iodine and alkyl iodides from spent-nuclear-fuel-reprocessing off-gas using reduced silver mordenite

Radioactive iodine is a hazardous byproduct of spent-nuclear-fuel reprocessing that must be removed from the off-gas stream before it can be discharged. Reduced silver mordenite (Ag 0 Z) is currently the baseline material for iodine capture in the U.S. Although the performance characteristics and capture mechanisms of I 2 and CH 3 I have been established, similar investigations into long-chain organic iodides have yet to be performed. In this study, thin beds of Ag 0 Z were loaded with I 2 , CH 3 I, C 4 H 9 I, and C 12 H 25 I (5 ppm to 50 ppm) carried in a dry air stream at 150°C. The maximum iodine capacity was 105 ± 5 mg I/g Ag 0 Z for all species. Saturated Ag 0 Z samples were characterized using scanning electron microscopy, X-ray fluorescence, X-ray photoelectron spectroscopy, diffuse reflectance UV–visible spectroscopy, pair distribution function analysis, and thermogravimetric analysis. Further, near-complete Ag utilization and similar physical/chemical properties were observed for all samples. Through a comparison with previous studies and an investigation of aged Ag 0 Z, we propose that iodine species react with Ag + at exchange sites, forming α-AgI within the mordenite channels, and with surface Ag 0 nanoparticles, yielding β-/γ-AgI. The available Ag sites in the interior (Ag + ) and exterior (Ag 0 ) of mordenite determine the adsorption capacity since α-AgI formation is limited by the total pore volume. Potential iodine uptake routes were summarized for aging and non-aging environments. A scalable predictive model was implemented for deep-bed iodine removal, and predictions were in good agreement with experimental data. Sensitivity analysis suggests that iodine uptake kinetics is governed by pore diffusion.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2016

IC 3639—a new bona fide compton-thick AGN unveiled by NuSTAR

We analyze high-quality NuSTAR observations of the local (z = 0.011) Seyfert 2 active galactic nucleus (AGN) IC 3639, in conjunction with archival Suzaku and Chandra data. This provides the first broadband X-ray spectral analysis of the source, spanning nearly two decades in energy (0.5–30 keV). Previous X-ray observations of the source below 10 keV indicated strong reflection/obscuration on the basis of a pronounced iron fluorescence line at 6.4 keV. The hard X-ray energy coverage of NuSTAR, together with self-consistent toroidal reprocessing models, enables direct broadband constraints on the obscuring column density of the source. We find the source to be heavily Compton-thick (CTK) with an obscuring column in excess of 3.6×10{sup 24} cm{sup −2}, unconstrained at the upper end. We further find an intrinsic 2–10 keV luminosity of log{sub 10}(L{sub 2--10keV} [erg s{sup −1}])=43.4{sub −1.1}{sup +0.6} to 90% confidence, almost 400 times the observed flux, and consistent with various multiwavelength diagnostics. Such a high ratio of intrinsic to observed flux, in addition to an Fe-Kα fluorescence line equivalent width exceeding 2 keV, is extreme among known bona fide CTK AGNs, which we suggest are both due to the high level of obscuration present around IC 3639. Our study demonstrates that broadband spectroscopic modeling with NuSTAR enables large corrections for obscuration to be carried out robustly and emphasizes the need for improved modeling of AGN tori showing intense iron fluorescence.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2016

IC 3639 - A New Bona Fide Compton-Thick AGN Unveiled By NuSTAR

We analyze high-quality NuSTAR observations of the local (z = 0.011) Seyfert 2 active galactic nucleus (AGN) IC 3639, in conjunction with archival Suzaku and Chandra data. This provides the first broadband X-ray spectral analysis of the source, spanning nearly two decades in energy (0.5-30 keV). Previous X-ray observations of the source below 10 keV indicated strong reflection/obscuration on the basis of a pronounced iron fluorescence line at 6.4 keV. The hard X-ray energy coverage of NuSTAR, together with self-consistent toroidal reprocessing models, enables direct broadband constraints on the obscuring column density of the source. We find the source to be heavily Compton-thick (CTK) with an obscuring column in excess of 3.6 x 10(exp 24) cm(exp −2), unconstrained at the upper end. We further find an intrinsic 2-10 keV luminosity of log(sub 10) (L(sub 2-10 keV) [erg s(exp -1)])= 43.4(+0.6/-1.1) to 90% confidence, almost 400 times the observed flux, and consistent with various multiwavelength diagnostics. Such a high ratio of intrinsic to observed flux, in addition to an Fe-K(alpha) fluorescence line equivalent width exceeding 2 keV, is extreme among known bona fide CTK AGNs, which we suggest are both due to the high level of obscuration present around IC 3639. Our study demonstrates that broadband spectroscopic modeling with NuSTAR enables large corrections for obscuration to be carried out robustly and emphasizes the need for improved modeling of AGN tori showing intense iron fluorescence.

galaxies: active – galaxies: nuclei – galaxies↗
DOE OSTI2023

Enabling Recycling of Composites: Understanding the Impacts of Multiple Thermal Processing Cycles

When considering the utilization of recycled short carbon fiber feedstock materials for advanced manufacturing, understanding the material degradation behavior is essential in determining how many times a composite material can be effectively reprocessed and remanufactured. This study characterizes the degradation behavior of short carbon fiber acrylonitrile butadiene (CF-ABS) that has been reprocessed five times with twin screw extrusion. Parallel plate rheology was completed to observe the degradation in complex viscosity of the recycled feedstock materials. Gel permeation chromatography (GPC) was utilized to characterize the changes in molecular weight distribution of the recycled materials as a result of thermal and mechanical degradation during the re-processing steps. Rheological characterization, GPC, and twin-screw processing data help inform the process optimizations required to process the recycled feedstock material. Successful characterization of the degradation behavior of short fiber composite feedstock materials aids in increased understanding of the lifespan of high value carbon fiber composite materials and aids in process optimization of recycled composite materials.

Walker, Roo↗
DOE OSTI2016

Magnox Reprocessing TDN Reactors: Utilising 3D Printing and X-Ray Imaging to Re-Design and Test Fluidising Air Nozzles - 16402

One of the key final steps in reprocessing spent nuclear fuel is the conversion of highly concentrated uranyl nitrate hexahydrate liquor [> 1000 gU/litre] into uranium trioxide (UO{sub 3}) powder by thermal decomposition using Thermal Denitration (TDN) reactors. The TDN reactors in the Magnesium non-oxidising (Magnox) fuel reprocessing plant are high aspect ratio fluidising beds, which suffer from poor fluidization and UO{sub 3} powder blockages. It is widely understood that these issues arise from the inadequate design of the fluidising air distributors (nozzles), which are located around the base of the TDN reactors. A non-active test rig was constructed at the National Nuclear Laboratory (NNL) experimental facility in Workington, Cumbria (UK) which used compressed air at ambient temperature to assess the performance of the current fluidising air nozzle designs (datum) against a range of new nozzle designs. Full-scale nozzle designs were manufactured using a 3-Dimensional (3D) printer and tested to obtain data of both quantitative and qualitative nature. NNL then collaborated with the Chemical Engineering Department at University College London (UCL) to further assess the fluidising potential of the new nozzle designs. Images of inside the fluidized bed were taken utilising a unique X-Ray facility. The results from this study will allow new nozzle designs to be recommended, manufactured and installed, which will ensure improved fluidization of the TDN reactor bed and prevent blockages with UO{sub 3} powder. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
NASA NTRS2004

X-Ray Reprocessing in Active Galactic Nuclei

This is the final report for research entitled "X-ray reprocessing in active galactic nuclei," into X-ray absorption and emission in various classes of active galaxy via X-ray spectral signatures. The fundamental goal of the research was to use these signatures as probes of the central engine structure and circumnuclear environment of active galactic nuclei. The most important accomplishment supported by this grant involved the detailed analysis and interpretation of the XMM data for the bright Seyfert 1 galaxy MCG-6-30-15. This work was performed by Drs. Christopher Reynolds and Mitchell Begelman in collaboration with Dr. Jorn Wilms (University of Tubingen, Germany; PI of the XMM observation) and other European scientists. With XMM we obtained medium resolution X-ray spectra of unprecedented quality for this Seyfert galaxy. Modeling the X-ray spectrum within the framework of accretion disk reflection models produced the first evidence for energy extraction from the spin of a black hole. Specifically, we found that the extreme gravitational redshifts required to explain the X-ray spectrum suggests that the bulk of the energy dissipation is concentrated very close to the black hole, in contrast with the expectations of any pure accretion disk model. In a second paper we addressed the low- energy spectral complexity and used RXTE specta to pin down the high-energy spectral index, thus firming up our initial interpretation. Additionally, we carried out detailed spectral and variability analyses of a number of Seyfert and radio galaxies (e.g., NGC 5548 and 3C 111) and developed general techniques that will be useful in performing X-ray reverberation mapping of accretion disks in AGN, once adequate data becomes available. A list of papers supported by this research is included.

Begelman, Mitchell C.↗