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At least 415 records · Page 23

Simulated Disruptions of the Quasi-Biennial Oscillation

The Quasi-Biennial Oscillation has exhibited remarkable stability over the observational record—until a well-documented 2015/16 disruption and an emerging disruption in 2020/21. The possibility that disruptions are more frequent in a changing climate is important to consider, as the QBO affects predictability, stratospheric composition, and surface weather. However, this possibility is challenging to assess for a variety of reasons. For instance, the 2015/16 disruption has been attributed to anomalous easterly momentum flux from extratropical waves. By comparison, the 2020/21 disruption involves anomalous westerly forcing, less likely to originate from the same mechanism. We present a rich variety of QBO disruptions that spontaneously arise in integrations of the hightop NASA GISS Model E2.2. The disruptions loosely fall into several categories, some of which are analogous to the 2015/16 disruption and the 2020 disruption, as well as a previously undocumented possible disruption in 1988. Several factors appear to influence QBO disruptions in the model: natural variability, climate change, tropical SSTs, volcanic eruptions, and model physics/tuning. Although QBO representation is an ongoing challenge for models, the results point to a model-independent framework for assessment of disruptions.

Quasi-Biennial Oscillation↗

Tropical African wildfire aerosols trigger teleconnections over mid-to-high latitudes of Northern Hemisphere in January

This study investigates the impacts of African wildfire aerosols (primary organic carbon, black carbon and sulfate) on the Northern Hemispheric in January. We found that wildfire aerosols emitted from equatorial Africa result in two mid-to-high latitudes atmospheric Rossby wave trains. One is from subtropical Atlantic propagating northeastward across Europe to Siberia, and the other one propagates eastward from Middle East across Asia to Pacific Northwest. The maximum positive geopotential height anomaly locates in Europe, concurrent with a greater-than-2 K land surface warming. These Rossby wave trains are excited by the atmospheric heating that caused by the wildfire aerosols in equatorial Africa and propagate into extratropics with the help of the westerly jet. Based on the diabatic heat budget analysis, the Rossby wave source is primarily from the solar absorption of black carbon of African wildfire. The present study emphasizes that wildfire aerosols, especial the absorbing aerosols, would have profound climate effects on remote regions and thus need more attentions.

54 ENVIRONMENTAL SCIENCES↗

Sensing Clouds via Spacecraft Radio Occultation Observations

The presence of clouds dramatically alters the opacity and radiative transfer within Earth's atmosphere at both short and long wavelengths. Knowledge of cloud top and base is needed to estimate the Outgoing Long wave Radiation (OLR) to space and the net radiation at the surface from a given atmospheric profile. Satellite observations are required to provide the global perspective needed for climate. Cloud top pressure can be determined to some accuracy from spaceborne radiance measurements when cloud opacities are sufficiently large and cloud top temperatures are sufficiently low to readily them from the surface. Cloud base is particularly difficult to determine from space. The relatively small sensitivity of long wavelengths must be used to penetrate the clouds while at the same time providing sufficient sensitivity to detect the cloud base. We are studying the indirect sensitivity of radio occultation observations to clouds through their impact on the refractivity structure. The tradewind inversion is an excellent example where a very sharp refractivity structure coincides with the top of the tradewind cumulus and stratus clouds. In general, any cloud with sufficient IR opacity will have large transmissivity gradient at cloud top (base) which will result in large cooling (heating) which will create a thermal inversion at cloud top (base). Both liquid and ice clouds can reach this critical opacity. The thermal inversion and sharp change in specific humidity will cause a sharp change in the refractivity gradient which can be identified in the radio occultation results, particularly the signal amplitude. The occultations yield very accurate information on the height of such features. The heating at cloud base drives convection causing the air to follow a moist adiabat within the Cloud which further helps constrain the interpretation of the observations. The upward expansion of such opaque clouds due to convection may be an important mechanism supplying moisture into the upper troposphere. We will present simulations using high resolution radiosondes from field campaigns representing the expected signatures of such features. We will also present initial results of comparisons between GPS observations and GOES-derived cloud tops to assess the utility of this concept.

Kursinski, E. R.↗

The 1998-2000 SHADOZ (Southern Hemisphere ADditional OZonesondes) Tropical Ozone Climatology: Stratospheric and Tropospheric Ozone Variability and the Zonal Wave-One - 2

This is the second 'reference' or 'archival' paper for the SHADOZ (Southern Hemisphere Additional Ozonesondes) network and is a follow-on to the recently accepted paper with similar first part of title. The latter paper compared SHADOZ total ozone with satellite and ground-based instruments and showed that the equatorial wave-one in total ozone is in the troposphere. The current paper presents details of the wave-one structure and the first overview of tropospheric ozone variability over the southern Atlantic, Pacific and Indian Ocean basins. The principal new result is that signals of climate effects, convection and offsets between biomass burning seasonality and tropospheric ozone maxima suggest that dynamical factors are perhaps more important than pollution in determining the tropical distribution of tropospheric ozone. The SHADOZ data at ( ) are setting records in website visits and are the first time that the zonal view of tropical ozone structure has been recorded - thanks to the distribution of the 10 sites that make up this validation network.

Thompson, Anne M.↗

Living with a Star: New Opportunities in Sun-Climate Research

Living With a Star is a NASA initiative employing the combination of dedicated spacecraft with targeted research and modeling efforts to improve what we know of solar effects of all kinds on the Earth and its surrounding space environment, with particular emphasis on those that have significant practical impacts on life and society. The highest priority among these concerns is the subject of this report: the potential effects of solar variability on regional and global climate, including the extent to which solar variability has contributed to the well-documented warming of the Earth in the last 100 years. Understanding how the climate system reacts to external forcing from the Sun will also greatly improve our knowledge of how climate will respond to other climate drivers, including those of anthropogenic origin. A parallel element of the LWS program addresses solar effects on space weather : the impulsive emissions of charged particles, short-wave electromagnetic radiation and magnetic disturbances in the upper atmosphere and near-Earth environment that also affect life and society. These include a wide variety of solar impacts on aeronautics, astronautics, electric power transmission, and national defense. Specific examples are (1) the impacts of potentially- damaging high energy radiation and atomic particles of solar origin on satellites and satellite operations, spacecraft electronics systems and components, electronic communications, electric power distribution grids, navigational and GPS systems, and high altitude aircraft; and (2) the threat of sporadic, high-energy solar radiation to astronauts and high altitude aircraft passengers and crews. Elements of the LWS program include an array of dedicated spacecraft in near- Earth and near-Sun orbits that will closely study and observe both the Sun itself and the impacts of its variations on the Earth's radiation belts and magnetosphere, the upper atmosphere, and ionosphere. These spacecraft, positioned to study and monitor changing conditions in the Sun-Earth neighborhood, will also serve as sentinels of solar storms and impulsive events.

Source record↗

Cloud-System Resolving Models: Status and Prospects

Cloud-system resolving models (CRM), which are based on the nonhydrostatic equations of motion and typically have a grid-spacing of about a kilometer, originated as cloud-process models in the 1970s. This paper reviews the status and prospects of CRMs across a wide range of issues, such as microphysics and precipitation; interaction between clouds and radiation; and the effects of boundary-layer and surface-processes on cloud systems. Since CRMs resolve organized convection, tropical waves and the large-scale circulation, there is the prospect for several advances in both basic knowledge of scale-interaction requisite to parameterizing mesoscale processes in climate models. In superparameterization, CRMs represent convection, explicitly replacing many of the assumptions necessary in contemporary parameterization. Global CRMs have been run on an experimental basis, giving prospect to a new generation of climate weather prediction in a decade, and climate models due course. CRMs play a major role in the retrieval of surface-rain and latent heating from satellite measurements. Finally, enormous wide dynamic ranges of CRM simulations present new challenges for model validation against observations.

Tao, Wei-Kuo↗

A Quantum Annealing Computer Team Addresses Climate Change Predictability

The near confluence of the successful launch of the Orbiting Carbon Observatory2 on July 2, 2014 and the acceptance on August 20, 2015 by Google, NASA Ames Research Center and USRA of a 1152 qubit D-Wave 2X Quantum Annealing Computer (QAC), offered an exceptional opportunity to explore the potential of this technology to address the scientific prediction of global annual carbon uptake by land surface processes. At UMBC,we have collected and processed 20 months of global Level 2 light CO2 data as well as fluorescence data. In addition we have collected ARM data at 2sites in the US and Ameriflux data at more than 20 stations. J. Dorband has developed and implemented a multi-hidden layer Boltzmann Machine (BM) algorithm on the QAC. Employing the BM, we are calculating CO2 fluxes by training collocated OCO-2 level 2 CO2 data with ARM ground station tower data to infer to infer measured CO2 flux data. We generate CO2 fluxes with a regression analysis using these BM derived weights on the level 2 CO2 data for three Ameriflux sites distinct from the ARM stations. P. Gentine has negotiated for the access of K34 Ameriflux data in the Amazon and is applying a neural net to infer the CO2 fluxes. N. Talik validated the accuracy of the BM performance on the QAC against a restricted BM implementation on the IBM Softlayer Cloud with the Nvidia co-processors utilizing the same data sets. G. Nearing and K. Harrison have extended the GSFC LIS model with the NCAR Noah photosynthetic parameterization and have run a 10 year global prediction of the net ecosystem exchange. C. Pellisier is preparing a BM implementation of the Kalman filter data assimilation of CO2 fluxes. At UMBC, R. Prouty is conducting OSSE experiments with the LISNoah model on the IBM iDataPlex to simulate the impact of CO2 fluxes to improve the prediction of global annual carbon uptake. J. LeMoigne and D. Simpson have developed a neural net image registration system that will be used for MODIS ENVI and will be converted to a BM algorithm implementation on the QAC. The first integer adder has been implemented on the D-Wave 2X by A. Shehab that will perform HAAR wavelets for image compression of MODIS scenes. Finally, based on the next generations of QACs, we are preparing a 5-year performance road map on the scalability of the current QAC algorithms.

Science Data Processing↗

Observing Ice Phase Clouds and Precipitation with Millimeter- and Submillimeter-wave Radiometry during the IMPACTS field campaign: Algorithm Development for the Emerging Class of Microwave Radiometers

Millimeter- and submillimeter-wave (mmWave, submm) radiometers provide significant information content on atmospheric water in liquid, ice, and vapor phases. Recent sensors, such as the Global Precipitation Measurement (GPM) or the Temporal Experiment for Storms and Tropical Systems Technology – Demonstration (TEMPEST-D), use mmWave bands to improve estimation of ice-phase precipitation, and future missions, such as the Atmosphere Observing System (AOS), will extend to submm to provide additional information on thinner ice clouds, linking clouds and precipitation and therefore elucidating the links between weather, climate, and the water cycle. To support the expanded use of mmWave/submm radiometry and exploit the available information content on condensed water mass, we demonstrate ice and liquid water path retrievals for NASA Goddard Space Flight Center's airborne radiometers the Conical Scanning Millimeter-wave Imaging Radiometer (CoSMIR) and the Configurable Scanning Submillimeter-wave Instrument/Radiometer (CoSSIR, formerly the Compact Scanning Submillimeter Imaging Radiometer). The analysis is based on data collected during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS) field campaign. A simulation study compares and contrasts retrievals for CoSMIR and CoSSIR, with CoSSIR demonstrating higher skill in ice retrievals, particularly for thin clouds, and the CoSMIR frequencies performing better for liquid. Additionally, we look at dual-polarized radiances observed by CoSMIR during the first two IMPACTS deployments to understand the polarization signatures induced by oriented hydrometeors. Results will be presented in the context of upcoming missions and sensors including AOS and the Ice Cloud Imager (ICI). We will describe the objectives for the expected first flight of the newly upgraded CoSSIR during the final IMPACTS deployment, and we will share novel science investigations we plan to undertake with CoSSIR's new capabilities. Popular Summary: Ice in clouds and falling snow is an important component of weather, climate, and water resources. To better use a new class of sensors that provide information on atmospheric ice, we developed an approach to measure ice clouds and falling snow using airborne data taken during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS), a field campaign to study winter storms. We look at the results for two similar instruments to understand how those differences affect these measurements of clouds and snow, and we further investigate the information the sensors can provide on properties of the clouds and snow.

Ian S Adams↗

Observing Ice Phase Clouds and Precipitation with Millimeter- and Submillimeter-wave Radiometry during the IMPACTS field campaign: Algorithm Development for the Emerging Class of Microwave Radiometers

Millimeter- and submillimeter-wave (mmWave, submm) radiometers provide significant information content on atmospheric water in liquid, ice, and vapor phases. Recent sensors, such as the Global Precipitation Measurement (GPM) or the Temporal Experiment for Storms and Tropical Systems Technology – Demonstration (TEMPEST-D), use mmWave bands to improve estimation of ice-phase precipitation, and future missions, such as the Atmosphere Observing System (AOS), will extend to submm to provide additional information on thinner ice clouds, linking clouds and precipitation and therefore elucidating the links between weather, climate, and the water cycle. To support the expanded use of mmWave/submm radiometry and exploit the available information content on condensed water mass, we demonstrate ice and liquid water path retrievals for NASA Goddard Space Flight Center's airborne radiometers the Conical Scanning Millimeter-wave Imaging Radiometer (CoSMIR) and the Configurable Scanning Submillimeter-wave Instrument/Radiometer (CoSSIR, formerly the Compact Scanning Submillimeter Imaging Radiometer). The analysis is based on data collected during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS) field campaign. A simulation study compares and contrasts retrievals for CoSMIR and CoSSIR, with CoSSIR demonstrating higher skill in ice retrievals, particularly for thin clouds, and the CoSMIR frequencies performing better for liquid. Additionally, we look at dual-polarized radiances observed by CoSMIR during the first two IMPACTS deployments to understand the polarization signatures induced by oriented hydrometeors. Results will be presented in the context of upcoming missions and sensors including AOS and the Ice Cloud Imager (ICI). We will describe the objectives for the expected first flight of the newly upgraded CoSSIR during the final IMPACTS deployment, and we will share novel science investigations we plan to undertake with CoSSIR's new capabilities. Popular Summary: Ice in clouds and falling snow is an important component of weather, climate, and water resources. To better use a new class of sensors that provide information on atmospheric ice, we developed an approach to measure ice clouds and falling snow using airborne data taken during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS), a field campaign to study winter storms. We look at the results for two similar instruments to understand how those differences affect these measurements of clouds and snow, and we further investigate the information the sensors can provide on properties of the clouds and snow.

Ian S Adams↗

Differences Between ERBE and CERES Tropical Means Fluxes: ENSO, Climate Change of Calibration?

Verner E. Soumi was the father of radiation budget measurements from space. He directed the team at the University of Wisconsin that developed the first radiation budget measurements on the Iota (Explorer VII) coverage) spacecraft in 1959. The first data published was from hand calculations of night-time long-wave fluxes, with absolute accuracy estimated as better than 10 percent, and the data shown as hand drawn maps with lines of equal "long-wave radiation loss, in Langleys per minute X 10(exp -3) (isolangleys)". The first comparisons of the new radiation data with nephanalyses showed that clouds dominated the radiation patterns. Soumi immediately proposed using the radiation fields to help understand the atmospheric heat sources necessary to drive the atmospheric circulation. This early work already pointed to the relationship between the outgoing longwave radiation at the top of the atmosphere and the vertical flux divergence of infrared radiation within the atmosphere. In the next 30 years, global satellite observations of the radiation balance of the planet have advanced both in accuracy, stability, and in their ability to address cause and effect in the climate system. The purpose of the present paper is to examine early results of the new Clouds and the Earth's Radiant Energy System (CERES) data on Tropical Rainfall Measuring System (TRMM) which started data collection in January, 1998. CERES is a direct descendant of the legacy of Soumi's foresight on understanding the global energetics using satellite observations of broadband radiation.

Wielicki, Bruce A.↗

Differences between ERBE and CERES Tropical Mean Fluxes: ENSO, Climate Change or Calibration?

Verner E. Soumi was the father of radiation budget measurements from space. He directed the team at the University of Wisconsin that developed the first radiation budget measurements on the Iota (Explorer VII) coverage) spacecraft in 1959. The first data published was from hand calculations of night-time long-wave fluxes, with absolute accuracy estimated as better than 10 percent, and the data shown as hand drawn maps with lines of equal "long-wave radiation loss, in Langleys per minute X 10(exp -3) (isolangleys)". The first comparisons of the new radiation data with nephanalyses showed that clouds dominated the radiation patterns. Soumi immediately proposed using the radiation fields to help understand the atmospheric heat sources necessary to drive the atmospheric circulation. This early work already pointed to the relationship between the outgoing longwave radiation at the top of the atmosphere and the vertical flux divergence of infrared radiation within the atmosphere. In the next 30 years, global satellite observations of the radiation balance of the planet have advanced both in accuracy, stability, and in their ability to address cause and effect in the climate system. The purpose of the present paper is to examine early results of the new Clouds and the Earth's Radiant Energy System (CERES) data on Tropical Rainfall Measuring System (TRMM) which started data collection in January, 1998. CERES is a direct descendant of the legacy of Soumi's foresight on understanding the global energetics using satellite observations of broadband radiation.

Wielicki, Bruce A.↗

Cool rooms for indoor heat resilience: Evaluating affordable cooling strategies in heat-stressed California homes

Extreme heat conditions pose significant indoor survivability challenges for resource-constrained communities, which often lack access to cooling, have poorly insulated homes, and face compounding socioeconomic vulnerabilities. Moreover, concurrent power outages worsen health risks and heat-related illnesses. It is therefore crucial to develop innovative and affordable cooling approaches to protect vulnerable populations. This study assesses the efficacy of “cool rooms”– a designated space within a home equipped with passive and low-power active cooling measures to maintain safe indoor temperatures during extreme heat events and power disruptions. Using a physics-based building energy modeling approach, we evaluate the efficacy of various retrofit packages in maintaining thermal safety within the cool room under recent extreme heat conditions. The results indicate that passive measures can reduce 64% of hours with unmet standard effective temperatures, while the combination of passive and low-power active measures with built-in batteries further cuts this to 86%. Nevertheless, these strategies remain insufficient to maintain indoor thermal safety during extended outages. In contrast, integrating a solar-powered mini-split heat pump, whose technical potential was evaluated in this study, reduces indoor air temperatures below the 28 °C overheating threshold and significantly improves indoor habitability. The localized cool room strategy also offers potential for grid resilience by reducing peak electricity demand by up to 70% compared to whole house cooling during heat waves. The findings can inform the development of actionable heat mitigation plans and retrofit policies for residential communities with relatively low adoption of air conditioning such as warm marine climates.

Cool room↗

DiffESM: Conditional Emulation of Temperature and Precipitation in Earth System Models With 3D Diffusion Models

Earth system models (ESMs) are essential for understanding the interaction between human activities and the Earth's climate. However, the computational demands of ESMs often limit the number of simulations that can be run, hindering the robust analysis of risks associated with extreme weather events. While low-cost climate emulators have emerged as an alternative to emulate ESMs and enable rapid analysis of future climate, many of these emulators only provide output on at most a monthly frequency. This temporal resolution is insufficient for analyzing events that require daily characterization, such as heat waves or heavy precipitation. We propose using diffusion models, a class of generative deep learning models, to effectively downscale ESM output from a monthly to a daily frequency. Trained on a handful of ESM realizations, reflecting a wide range of radiative forcings, our DiffESM model takes monthly mean precipitation or temperature as input, and is capable of producing daily values with statistical characteristics close to ESM output. Combined with a low-cost emulator providing monthly means, this approach requires only a small fraction of the computational resources needed to run a large ensemble. We evaluate model behavior using a number of extreme metrics, showing that DiffESM closely matches the spatio-temporal behavior of the ESM output it emulates in terms of the frequency and spatial characteristics of phenomena such as heat waves, dry spells, or rainfall intensity.

54 ENVIRONMENTAL SCIENCES↗

A three-dimensional simulation of the equatorial quasi-biennial oscillation

A simulation of the equatorial quasi-biennial oscillation (QBO) has been obtained using a three-dimensional mechanistic model of the stratosphere. The model is a simplified form of the NCAR CCM (Community Climate Model) in which the troposphere has been replaced with a specified geopotential distribution near the tropical tropopause and most of the physical parameterizations have been removed. A Kelvin wave and a Rossby-gravity wave are forced at the bottom boundary as in previous one- and two-dimensional models. The model reproduces most of the principal features of the observed QBO, as do previous models with lower dimensionality. The principal difference between the present model and previous QBO models is that the wave propagation is explicitly represented, allowing wave-wave interactions to take place. It is found that these interactions significantly affect the simulated oscillation. The interaction of the Rossby-gravity waves with the Kelvin waves results in about twice as much easterly compared to westerly forcing being required in order to obtain a QBO.

Takahashi, M.↗

Powering the Blue Economy: Foundational Research and Development

With increased use of the oceans for transportation, extraction of food, fibre, and minerals, recreation and tourism, and other blue economy industries, there is a need for additional power at sea. In the face of climate change, the increased power must come from renewable sources; often marine energy is the most energy-dense power source available. But we have little experience with adapting wave and tidal devices from large scale grid power to the specialized and small devices needed to power blue economy applications, nor the engineering solutions to support codesign of emerging marine industries. As directed by the U.S. Department of Energy (DOE), two DOE national laboratories have developed foundational research and development projects to replace conventional power or batteries at sea (ocean observation platforms), emerging industry power needs (offshore aquaculture operations), as well as examining common challenges for using marine power (efficient power systems, minimizing interference, optimizing materials and manufacturing).

marine energy↗

The Response of Lower Atmospheric Ozone to ENSO in Aura Measurements and a Chemistry-Climate Simulation

The El Nino-Southern Oscillation (ENSO) is the dominant mode of tropical variability on interannual time scales. ENSO appears to extend its influence into the chemical composition of the tropical troposphere. Recent work has revealed an ENSO-induced wave-1 anomaly in observed tropical tropospheric column ozone. This results in a dipole over the western and eastern tropical Pacific, whereby differencing the two regions produces an ozone anomaly with an extremely high correlation to the Nino 3.4 Index. We have successfully reproduced this feature using the Goddard Earth Observing System Version 5 (GEOS-5) general circulation model coupled to a comprehensive stratospheric and tropospheric chemical mechanism forced with observed sea surface temperatures over the past 25 years. An examination of the modeled ozone field reveals the vertical contributions of tropospheric ozone to the column over the western and eastern Pacific region. We will show composition sensitivity in observations from NASA s Aura satellite Microwave Limb Sounder (MLS) and the Tropospheric Emissions Spectrometer (TES) and a simulation to provide insight into the vertical structure of these ENSO-induced ozone changes. The ozone changes due to the Quasi-Biennial Oscillation (QBO) in the extra-polar upper troposphere and lower stratosphere in MLS measurements will also be discussed.

Oman, L. D.↗

Wintertime Arctic Oscillation and North Atlantic Oscillation and their impacts on the Northern Hemisphere climate in E3SM

The characteristics of the wintertime Arctic Oscillation (AO) and North Atlantic Oscillation (NAO) and their impacts on climate variability over the Northern Hemisphere are important metrics for evaluating a climate system model. Observational analyses reveal that the horizontal and vertical structures in the AO and NAO exhibit a meridional dipole and a large-scale barotropic pattern between the Arctic and mid-latitudes. Historical model simulations from the Energy Exascale Earth System Model (E3SM-HIST) are used to identify how well it captures these major climate modes. It is found that the simulated AO and NAO modes have spatial structures similar to the observed features. In addition, the observed frequency bands in the AO and NAO-related time variability are captured well in the E3SM-HIST simulation. Associated with the positive phase in wintertime AO and NAO, zonal flow and warm advection in mid-latitude continents are enhanced, along with stronger cold flow from enhanced northerly winds over high latitudes. These features are linked to the atmospheric circulation pattern reflected by lower SLP anomalies over the Arctic and higher SLP anomalies over the mid-latitudes. In E3SM-HIST, these spatial associations and main structural features are analogous to those in observations. In the time-height evolution related to winter AO and NAO modes, it can also be seen that the simulations reproduce the downward propagating patterns in observations. Nevertheless, the vertical structures associated with AO and NAO in E3SM-HIST exhibit substantial biases in the lower stratosphere. The cause of these stratospheric biases is investigated using the strength of climatological stratospheric polar vortex (SPV) and wave activity fluxes. The results herein suggest that E3SM-HIST has a reasonable skill in reproducing the observed characteristics related to the winter AO and NAO, although there exist systematic biases in the associated climate variability.

54 ENVIRONMENTAL SCIENCES↗

Polar primary aerosols across the ocean-sea ice-snow-atmosphere interface: From sources to impacts

Primary aerosols play a critical role in polar climate systems, influencing cloud formation, precipitation, radiative balance, and surface energy budgets. This paper provides a comprehensive synthesis of primary aerosol sources, transformation and removal processes, and broader atmospheric impacts in polar regions, emphasizing their links to ocean and sea ice biogeochemistry. These aerosols (including sea salt, primary organic aerosol, and primary biological aerosol particles) originate from marine and cryospheric environments and are emitted through physical processes, such as wave breaking, bubble bursting, and blowing snow. Emission sources include seawater, sea ice, snow, and freshwater from river discharge and glacial runoff. Once airborne, these particles can serve as a chemical reservoir, influencing atmospheric composition and reactivity, and as seeds for cloud droplet and ice crystal formation, influencing cloud microphysics and polar climate. Despite their importance, many of the processes governing primary aerosol emissions and transformations remain poorly constrained. The most pressing knowledge gaps pertain to emission processes, limited spatiotemporal observational coverage, instrumentation constraints, parameterization development, and the integration of interdisciplinary expertise. To improve our understanding of primary aerosol drivers and their response to climate, future research efforts should prioritize strategically coordinated and cross-disciplinary process studies, advancements in measurement technologies and coverage, and close collaboration between modelers and observational scientists to inform and refine model parameterizations. As polar regions continue to undergo profound changes marked by increased precipitation, reduced sea and land ice, freshening oceans, and shifting ecosystem dynamics, characterizing present-day primary aerosol populations is vital. Improved understanding will be essential for anticipating future changes in aerosol-radiation and aerosol-cloud interactions and their implications for polar and global climate systems.

Aerosol-cloud↗