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NASA NTRSDate not supplied

First Optical Constants from 0.4 to 1.6 µm of Titan Aerosol Analogs Produced in the NASA Ames COSmIC Facility and Their Use in a New Analysis of Cassini VIMS Observations

We have determined the real and imaginary refractive indices (n and k, respectively), from the visible to the near infrared (0.4 to 1.6 μm), of five laboratory-generated organic refractory materials produced from gas-phase chemistry with the NASA Ames COSmIC facility. The solid samples were produced using a plasma discharge in the stream of a 200-K supersonic jet-cooled expansion of different gas mixtures to study the impact of the molecular precursors on the solid sample optical properties. Three samples were produced from N2:CH4 (95:5) gas mixtures using three different high voltages (700V, 800V and 1000V) to vary the energy in the plasma discharge. One sample was produced from a N2:CH4:C2H2 (94:5:5:0.5) gas mixture, with a high voltage of 1000 V. The fifth sample was produced in an Ar:CH4 (95:5) gas mixture with a high voltage of 1000 V to produce a nitrogen-free hydrocarbon sample. The optical constants, n and k, of these five samples were determined using spectral reflectance measurements. They appear to be positively correlated with the nitrogen content in the solid sample, i.e., a sample with larger nitrogen content exhibits higher n and k values. We have used these refractive indices as input parameters in a radiative transfer model to analyze Cassini Visible Infrared Mapping Spectrometer (VIMS) observations of Titan’s atmosphere. The results show that using the tholin samples with higher n and k values (higher nitrogen content) provides a better fit to the observational data than using the samples with lower n and k values (lower nitrogen content). The Titan tholins with higher nitrogen content therefore appear to be more representative of the Titan aerosols observed by VIMS.

Titan Aerosol Analogs↗

NASA NTRS1998

Stellar Occultation Probe of Triton's Atmosphere

The goals of this research were (i) to better characterize Triton's atmospheric structure by probing a region not well investigated by Voyager and (ii) to begin acquiring baseline data for an investigation of the time evolution of the atmosphere which will set limits on the thermal conductivity of the surface and the total mass of N2 in the atmosphere. Our approach was to use observations (with the Kuiper Airborne Observatory) of a stellar occultation by Triton that was predicted to occur on 1993 July 10. As described in the attached reprint, we achieved these objectives through observation of this occultation and a subsequent one with the KAO in 1995. We found new results about Triton's atmospheric structure from the analysis of the two occultations observed with the KAO and ground-based data. These stellar occultation observations made both in the visible and infrared, have good spatial coverage of Triton including the first Triton central-flash observations, and are the first data to probe the 20-100 km altitude level on Triton. The small-planet light curve model of Elliot and Young (AJ 103, 991-1015) was generalized to include stellar flux refracted by the far limb, and then fitted to the data. Values of the pressure, derived from separate immersion and emersion chords, show no significant trends with latitude indicating that Triton's atmosphere is spherically symmetric at approximately 50 km altitude to within the error of the measurements. However, asymmetry observed in the central flash indicates the atmosphere is not homogeneous at the lowest levels probed (approximately 20 km altitude). From the average of the 1995 occultation data, the equivalent-isothermal temperature of the atmosphere is 47 +/- 1 K and the atmospheric pressure at 1400 km radius (approximately 50 km altitude) is 1.4 +/- 0.1 microbar. Both of these are not consistent with a model based on Voyager UVS and RSS observations in 1989 (Strobel et al, Icarus 120, 266-289). The atmospheric temperature from the occultation is 5 K colder than that predicted by the model and the observed pressure is a factor of 1.8 greater than the model.

Elliot, James L.↗

NASA NTRS1979

The investigation of advanced remote sensing techniques for the measurement of aerosol characteristics

Advanced remote sensing techniques and inversion methods for the measurement of characteristics of aerosol and gaseous species in the atmosphere were investigated. Of particular interest were the physical and chemical properties of aerosols, such as their size distribution, number concentration, and complex refractive index, and the vertical distribution of these properties on a local as well as global scale. Remote sensing techniques for monitoring of tropospheric aerosols were developed as well as satellite monitoring of upper tropospheric and stratospheric aerosols. Computer programs were developed for solving multiple scattering and radiative transfer problems, as well as inversion/retrieval problems. A necessary aspect of these efforts was to develop models of aerosol properties.

Deepak, A.↗

NASA NTRS2018

Remote Sensing of the Ocean Surface Refractive Index via Short-Wave Infrared Polarimetry

The linear polarization of sunlight reflected by ocean surfaces in the shortwave infrared (SWIR), at geometries where specular reflection dominates the signal, is a direct function of the refractive index of the surface microlayer(SML). This simple physical concept is at the base of a novel technique presented in this study. We invert observations obtained by the airborne Research Scanning Polarimeter (RSP) in the sun glint region, where each pixel's radiance is dominated by the signal originating from the wave slopes oriented precisely to cause specular reflection. The SWIR wavelength ensures minimization of aerosol interference when radiance travels through the atmosphere; strong absorption by the water body then limits the penetration depth to the first micrometer or so, effectively probing the SML. The resulting Degree of Linear Polarization (DoLP) is then governed by the refractive index via the Fresnel law for the specfic pixel geometry, independently of the wind speed. The selected dataset concerns several field deployments from both low- and high-altitude aircraft, including total reflectance measurements with the sole purpose of accounting for the residual aerosol effect.Stable retrievals from transects above pure seawater yielded values of refractive index that match the values published in the literature within an accuracy of 5 x 10 [superscript 4]. Flying over the oil spill caused by the explosion of the Deepwater Horizon platform, detected variations were found compatible with the presence of an oil slick. The robustness of the results, guaranteedby the high RSP polarimetric accuracy (less than or equal to 0:2%), opens the possibility for remote-sensing detection of other entities that similarly affect the refractive index including whitecaps, microplastics, biological gels, seaweed and grass mats.

Surface Microlayer↗

NASA NTRS1986

Laboratory evaluation and application of microwave absorption properties under simulated conditions for planetary atmospheres

The recognition of the need to make laboratory measurements of simulated planetary atmospheres over a range of temperatures and pressure which correspond to the altitudes probed by radio occultation experiments, and over a range of frequencies which correspond to both radio occultation experiments and radio astronomical observations, has led to the development of a facility at Georgia Tech which is capable of making such measurements. Construction was completed of the outer planets simulator and measurements were conducted of the microwave absorption and refraction from nitrogen under simulated Titan conditions. The results of these and previous laboratory measurements were applied to a wide range of microwave opacity measurements, in order to derive constituent densities and distributions in planetary atmospheres such as Venus.

Steffes, P. G.↗

NASA NTRS1972

Effects of atmospheric irregularities on sonic-boom propagation.

A review is given of information obtained in recent years concerning the effects on sonic-boom signatures of departures of the atmosphere from a perfectly stratified time invariant model. These effects include the observed random variations in boom overpressures from those expected for a stratified atmosphere, the anomalously large and variable rise times, and the occurrence of spiked or rounded waveforms rather than the characteristic N waves. The extent of the variability in data recorded during actual flight tests is summarized in the form of histograms, representing experimentally obtained probability density functions. The physical mechanisms believed to be responsible for the variations and the anomalous features in the signatures are described. These include refraction and subsequent wavefront rippling by turbulence, the possible focusing or defocusing of rays, the formation of caustics, and the phenomenon of wavefront folding, diffraction, and scattering. Recent statistical theories of shock propagation through a turbulent atmosphere proposed by Crow, George and Plotkin, Pierce, Horning, and others are reviewed.

Pierce, A. D.↗

NASA NTRS1998

Raman Lidar Measurements of Aerosol Extinction and Backscattering: Derivation of Aerosol Real Refractive Index, Single-Scattering Albedo, and Humidification Factor using Raman Lidar and Aircraft Size Distribution - Report 2

Aerosol backscattering and extinction profiles measured by the NASA Goddard Space Flight Center Scanning Raman Lidar (SRL) during the remote cloud sensing (RCS) intensive operations period (IOP) at the Department of Energy Atmospheric Radiation Measurement (ARM) southern Great Plains (SGP) site during two nights in April 1994 are discussed. These profiles are shown to be consistent with the simultaneous aerosol size distribution measurements made by a PCASP (Passive Cavity Aerosol Spectrometer Probe) optical particle counter flown on the University of North Dakota Citation aircraft. We describe a technique which uses both lidar and PCASP measurements to derive the dependence of particle size on relative humidity, the aerosol real refractive index n, and estimate the effective single-scattering albedo Omega(sub 0). Values of n ranged between 1.4-1.5 (dry) and 1.37-1.47 (wet); Omega(sub 0) varied between 0.7 and 1.0. The single-scattering albedo derived from this technique is sensitive to the manner in which absorbing particles are represented in the aerosol mixture; representing the absorbing particles as an internal mixture rather than the external mixture assumed here results in generally higher values of Omega(sub 0). The lidar measurements indicate that the change in particle size with relative humidity as measured by the PCASP can be represented in the form discussed by Hattel with the exponent gamma = 0.3 + or - 0.05. The variations in aerosol optical and physical characteristics captured in the lidar and aircraft size distribution measurements are discussed in the context of the meteorological conditions observed during the experiment.

Ferrare, R. A.↗

NASA NTRS1983

High altitude Venus haze from Pioneer Venus limb scans

High-resolution limb scans of Venus made with the Orbiter Cloud Photopolarimeter aboard Pioneer Venus have been used to observe the high altitude Venus haze and its variation over almost one half a Venusian year. A model for a spherical atmosphere with tangential viewing geometry was used to analyze the observations and derive the haze properties. Values are found for the particle size and refractive index, particle number density and scale height, and eddy diffusion coefficient. Single scattering computations show good agreement with observed intensities for particles smaller than 0.3 micron radius and refractive index less than 1.7, consistent with, but not limited to, concentrated sulfuric acid. Particle scale height in the 0.5 to 2 mbar pressure regions varies between 1 and 3 km over the season, latitude, and local time ranges of the observations. Detached layers of haze are sometimes present. An average particle scale height of 2.2 km at 84 km altitude yields an eddy diffusion coefficient of 130,000 sq cm/sec.

Lane, W. A.↗

NASA NTRS1993

Temperature dependence of nu3 and nu4 bandwidths and complex refractive indices for crystalline methane

Infrared spectra of thin films of pure CH4 have been measured for a range of temperatures from 22 to 68 K. The bandwidth for the fundamental nu3 near 3000/cm varies from 12.7 to 33.2/cm, while that for nu4 near 1300/cm varies from 6.2 to 16.0/cm. The real and imaginary parts of the index of refraction also exhibit significant dependence on temperature. These broadband measurements at low temperatures are useful for an understanding of clouds and hazes in the atmosphere of Uranus, clouds and ices in the atmosphere of Titan, and ices on the surfaces of Pluto and Triton.

Ngoh, M. A.↗

NASA NTRS1997

Comparison of Modeled Backscatter using Measured Aerosol Microphysics with Focused CW Lidar Data over Pacific

During NASA's GLObal Backscatter Experiment (GLOBE) II flight mission over the Pacific Ocean in May-June 1990, extensive aerosol backscatter data sets from two continuous wave, focused CO2 Doppler lidars and an aerosol microphysics data set from a laser optical particle counter (LOPC) were obtained. Changes in aerosol loading in various air masses with associated changes in chemical composition, from sulfuric acid and sulfates to dustlike crustal material, significantly affected aerosol backscatter, causing variation of about 3 to 4 orders of magnitude. Some of the significant backscatter features encountered in different air masses were the low backscatter in subtropical air with even lower values in the tropics near the Intertropical Convergence Zone (ITCZ), highly variable backscatter in the ITCZ, mid-tropospheric aerosol backscatter background mode, and high backscatter in an Asian dust plume off the Japanese coast. Differences in aerosol composition and backscatter for northern and southern hemisphere also were observed. Using the LOPC measurements of physical and chemical aerosol properties, we determined the complex refractive index from three different aerosol mixture models to calculate backscatter. These values provided a well-defined envelope of modeled backscatter for various atmospheric conditions, giving good agreement with the lidar data over a horizontal sampling of approximately 18000 km in the mid-troposphere.

Srivastava, Vandana↗

NASA NTRS2021

Quantifying the range of the dust direct radiative effect due to source mineralogy uncertainty

The large uncertainty in the mineral dust direct radiative effect (DRE) hinders projections of future climate change due to anthropogenic activity. Resolving modeled dust mineral speciation allows for spatially and temporally varying refractive indices consistent with dust aerosol composition. Here, for the first time, we quantify the range in dust DRE at the top of the atmosphere (TOA) due to current uncertainties in the surface soil mineralogical content using a dust mineral-resolving climate model. We propagate observed uncertainties in soil mineral abundances from two soil mineralogy atlases along with the optical properties of each mineral into the DRE and compare the resultant range with other sources of uncertainty across six climate models. The shortwave DRE responds region-specifically to the dust burden depending on the mineral speciation and underlying shortwave surface albedo: positively when the regionally averaged annual surface albedo is larger than 0.28 and negatively otherwise. Among all minerals examined, the shortwave TOA DRE and single scattering albedo at the 0.44–0.63 µm band are most sensitive to the fractional contribution of iron oxides to the total dust composition. The global net (shortwave plus longwave) TOA DRE is estimated to be within −0.23 to +0.35 W/sq. m. Approximately 97 % of this range relates to uncertainty in the soil abundance of iron oxides. Representing iron oxide with solely hematite optical properties leads to an overestimation of shortwave DRE by +0.10 W/sq. m at the TOA, as goethite is not as absorbing as hematite in the shortwave spectrum range. Our study highlights the importance of iron oxides to the shortwave DRE: they have a disproportionally large impact on climate considering their small atmospheric mineral mass fractional burden (∼2 %). An improved description of iron oxides, such as those planned in the Earth Surface Mineral Dust Source Investigation (EMIT), is thus essential for more accurate estimates of the dust DRE.

mineral dust↗

NASA NTRSDate not supplied

Use of three-cornered hat error estimates in MERRA-2 to guide an improved reanalysis-Part 1

The three-cornered hat (3CH) method estimates the uncertainties of three different co-located model or observational data sets (Anthes and Rieckh, 2018; Sjoberg et al., 2021). Rieckh et al. (2021) used the 3CH method to compare the random error statistics of different global forecast and reanalysis models, as well as radio occultation (RO) and radiosonde observations. That study showed that the MERRA-2 reanalysis, while having smaller errors in the stratosphere than its predecessor MERRA, had larger errors in the troposphere than many of the other data sets analyzed. The MERRA-2 errors were particularly large in the tropics. In a collaborative effort between UCAR’s COSMIC (Constellation Observing System for Meteorology, Ionosphere and Meteorology) program and NASA’s Global Modeling and Assimilation Office (GMAO), we carried out further 3CH error diagnostics to help isolate the causes of these larger errors and help guide the development of an improved reanalysis. This presentation summarizes random error statistics associated with MERRA-2, ECMWF’s ERA5 reanalysis, and COSMIC-2 (C2) RO observations. We compute 3CH error variance estimates of refractivity, as well as temperature and specific humidity using UCAR’s COSMIC Data Analysis and Archive Center (CDAAC) improved 1D-variational (1D-Var) retrieval (wetPf2) over 15 latitude bands from 45S to 45N. The 1D-Var retrievals of specific humidity and temperature for C2 use NCEP’s Global Forecast System (GFS) as the background. Anthes et al. (2021) showed that it gives accurate estimates of temperature and specific humidity in the tropics and subtropics, even in the challenging environment of intense Hurricane Dorian (2019). This presentation confirms the previous results that MERRA-2 has significantly larger errors in the tropics and subtropics than either C2 or ERA5. Its errors are larger between 30S and 30N compared to 30-45 N-S latitudes, and are also larger over land compared to oceans. Most of the MERRA-2 refractivity errors come from specific humidity, except over land below 3 km where temperature errors are large. These results suggest that moist convection and atmospheric boundary layer physics in MERRA-2 may be responsible for a significant part of the higher uncertainties. These results are being used to guide GMAO in developing an improved next-generation reanalysis, as shown in a companion presentation submitted to this conference (El Akkraoui et al., 2021), which extends this study and describes improvements to MERRA-2 leading to the next GMAO reanalysis.

Jeremiah Sjoberg↗

NASA NTRS2015

Systematic Relationships Between Lidar Observables and Sizes And Mineral Composition Of Dust Aerosols

The physical and chemical properties of soil dust aerosol particles fundamentally affect their interaction with climate, including shortwave absorption and radiative forcing, nucleation of cloud droplets and ice crystals, heterogeneous formation of sulfates and nitrates on the surface of dust particles, and atmospheric processing of iron into bioavailable forms that increase the productivity of marine phytoplankton. Lidar measurements, such as extinction-to-backscatter, color and depolarization ratios, are frequently used to distinguish between aerosol types with different physical and chemical properties. The chemical composition of aerosol particles determines their complex refractive index, hence affecting their backscattering properties. Here we present a study on how dust aerosol backscattering and depolarization properties at wavelengths of 355, 532 and 1064 nm are related to size and complex refractive index, which varies with the mineral composition of the dust. Dust aerosols are represented by collections of spheroids with a range of prolate and oblate aspect ratios and their optical properties are obtained using T-matrix calculations. We find simple, systematic relationships between lidar observables and the dust size and complex refractive index that may aid the use of space-based or airborne lidars for direct retrieval of dust properties or for the evaluation of chemical transport models using forward simulated lidar variables. In addition, we present first results on the spatial variation of forward-simulated lidar variables based on a dust model that accounts for the atmospheric cycle of eight different mineral types plus internal mixtures of seven mineral types with iron oxides, which was recently implemented in the NASA GISS Earth System ModelE2.

Dust↗

NASA NTRS1998

The Atmospheric Structure of Triton and Pluto

The goal of this research was to better determine the atmospheric structures of Triton and Pluto through further analysis of three occultation data sets obtained with the Kuiper Airborne Observatory (KAO.) As the research progressed, we concentrated our efforts on the Triton data, as this appeared to be the most fruitful. Three papers have been prepared as a result of this research. The first paper presents new results about Triton's atmospheric structure from the analysis of all ground-based stellar occultation data recorded to date, including one single-chord occultation recorded on 1993 July 10 and nine occultation lightcurves from the double-star event on 1995 August 14. These stellar occultation observations made both in the visible and in the infrared have good spatial coverage of Triton, including the first Triton central-flash observations, and are the first data to probe the altitude level 20-100 km on Triton. The small-planet lightcurve model of J. L. Elliot and L. A. Young was generalized to include stellar flux refracted by the far limb, and then fitted to the data. Values of the pressure, derived from separate immersion and emersion chords, show no significant trends with latitude, indicating that Triton's atmosphere is spherically symmetric at approximately 50 km altitude to within the error of the measurements; however, asymmetry observed in the central flash indicates the atmosphere is not homogenous at the lowest levels probed (approximately 20 km altitude). From the average of the 1995 occultation data, the equivalent isothermal temperature of the atmosphere is 47 plus or minus 1 K and the atmospheric pressure at 1400 km radius (approximately 50 km altitude) is 1.4 plus or minus 0.1 microbar. Both of these are not consistent with a model based on Voyager UVS and RSS observations in 1989. The atmospheric temperature from the occultation is 5 K colder than that predicted by the model and the observed pressure is a factor of 1.8 greater than the model. In our opinion, the disagreement in temperature and pressure is probably due to modeling problems at the microbar level, since measurements at this level have not previously been made. Alternatively, the difference could be due to seasonal change in Triton's atmospheric structure. The second paper reports observations of a recent stellar occultation by Triton which, when combined with earlier results, show that Triton has undergone a period of global warming since 1989. The most conservative estimates of the rate of temperature and surface-pressure increase during this period imply that the atmosphere is doubling in bulk every 10 years -- significantly faster than predicted by published frost model for Triton. Our results suggests that permanent polar caps on Triton play a dominant role in regulating seasonal atmospheric changes. Similar processes should also be active on Pluto. A third paper 'Global Warming on Triton' will appear in a the January 1999 issue of Sky and Telescope.

Elliot, James L.↗

NASA NTRS1979

Atmospheric effects on coherent laser systems

Effects of the truncation of the gaussian beam by the telescope on the signal to noise ratio were studied. Finite and infinite beams were also considered, along with the refractive index structure constant.

Murty, S. S. R.↗

NASA NTRS1978

Martian atmosphere modeling between 0.4 and 3.5 microns - Comparison of theory and experiment

A model of the lower atmosphere of Mars has been constructed that combines aerosol absorption and scattering with a line-by-line analysis of CO2 and H2O in a multilayer radiative transfer program. Aerosol composition previously inferred from the NASA Lear Jet Observatory data was used to measure the optical complex indices of refraction of appropriate Martian analogs from 0.4 to 2.5 microns. The aerosol vertical particle density scale was deduced using the Viking camera observations of the soil and sky intensities between 0.4 and 1.0 microns in comparison with those modeled using a multilayer Mie scattering program. A comparison of observed Mars atmospheric absorptions was made with those obtained using Lorentz, Voigt, and Doppler line profiles in a multilayer model of the CO2 and H2O. The Voigt line profile of CO2 absorption at approximately 4976 kaysers was then combined in a multilayer aerosol model of the Martian atmosphere. An evaluation of the effect on the line shape was made using several aerosol loadings.

Egan, W. G.↗

NASA NTRS1983

Interpretation of MST radar returns from clear air

The nature of the scattering and reflection mechanisms that give rise to the MST radar echoes from the clear air is essential in the correct interpretation of the data about winds, waves, turbulence and stability in the atmosphere. There are two main aspects: the nature of the targets the radar sees and their generation mechanisms; and the signatures of the radar signals returned from the different targets. Volume scatterings from isotropic or anisotropic turbulence, and partial reflections from horizontally stratified, sharp refractive index gradients are believed the main contributors to radar echoes. Combined effects from all the mechanisms probably produce the observed data. The signature of the echo signals for these different scatterers under realistic experimental conditions should be studied. It is hoped from these studies, the nature of the targets can be better understood, and related to atmospheric dynamic processes.

Liu, C. H.↗

NASA NTRS1974

Scattering and absorption from poly-dispersed aerosols

Results from numerical computations of the diffuse sky radiances and degree of polarization are given. These results were obtained by solving the equation of radiative transfer in the formulation of Eschelbach. In these computations, multiple scattering and absorption by aerosol particles were considered. In addition, results from experimental measurements of the complex refractive index of aerosol samples at different relative humidities are presented. From the radiation flux divergences which were computed based on the determined properties of atmospheric aerosol particles, atmospheric heating rates were derived which were found to be comparable to the heating rates by water vapor.

Bullrich, K.↗