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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 433 records · Page 24
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Exclusive $|V_{ub}|$ determinations using Padé Approximants

We determine the CKM parameter |V ub | from the exclusive semileptonic decays B→πℓν ℓ and B s →Kℓν ℓ , employing Lattice QCD theoretical information on the form factors in combination with experimental measurements of the differential branching ratio distributions. Using Pad\'{e} approximants to the participating form factors we obtain |V ub |=3.86(11)x10 -3 and |V ub |=3.58(9)x10 -3 from the analyses of the individual decay channels, respectively, and |V ub |=3.68(5)x10 -3 from a simultaneous analysis of both decays. Our results highlight the importance of the decay B s →Kμν μ in complementing the traditional B→πℓν ℓ one in the exclusive determination of |V ub | , and strengthens the case for precise measurements of the differential B s →Kℓν ℓ decay rate with a finer resolution of the q 2 bins, as it would definitely allow achieving more conclusive results for |V ub | .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Excited-State Dynamics of All the Mono-cis and the Major Di-cis Isomers of β-Apo-8′-Carotenal as Revealed by Femtosecond Time-Resolved Transient Absorption Spectroscopy

Cis isomers of carotenoids play important roles in light harvesting and photoprotection in photosynthetic bacteria, such as the reaction center in purple bacteria and the photosynthetic apparatus in cyanobacteria. Carotenoids containing carbonyl groups are involved in efficient energy transfer to chlorophyll in light-harvesting complexes, and their intramolecular charge–transfer (ICT) excited states are known to be important for this process. Previous studies, using ultrafast laser spectroscopy, have focused on the central-cis isomer of carbonyl-containing carotenoids, revealing that the ICT excited state is stabilized in polar environments. However, the relationship between the cis isomer structure and the ICT excited state has remained unresolved. In this study, we performed steady-state absorption and femtosecond time-resolved absorption spectroscopy on nine geometric isomers (7-cis, 9-cis, 13-cis, 15-cis, 13′-cis, 9,13′-cis, 9,13-cis, 13,13′-cis, and all-trans) of β-apo-8′-carotenal, whose structures are well-defined, and discovered correlations between the decay rate constant of the S1 excited state and the S0−S1 energy gap, as well as between the position of the cis-bend and the degree of stabilization of the ICT excited state. Our results demonstrate that the ICT excited state is stabilized in polar environments in cis isomers of carbonyl-containing carotenoids and suggest that the position of the cis-bend plays an important role in the stabilization of the excited state.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Effect of Random Nanostructured Metallic Environments on Spontaneous Emission of HITC Dye

We have studied emission kinetics of HITC laser dye on top of glass, smooth Au films, and randomly structured porous Au nanofoams. The observed concentration quenching of luminescence of highly concentrated dye on top of glass (energy transfer to acceptors) and the inhibition of the concentration quenching in vicinity of smooth Au films were in accord with our recent findings. Intriguingly, the emission kinetics recorded in different local spots of the Au nanofoam samples had a spread of the decay rates, which was large at low dye concentrations and became narrower with increase of the dye concentration. We infer that in different subvolumes of Au nanofoams, HITC molecules are coupled to the nanofoams weaker or stronger. The inhibition of the concentration quenching in Au nanofoams was stronger than on top of smooth Au films. This was true for all weakly and strongly coupled subvolumes contributing to the spread of the emission kinetics. The experimental observations were explained using theoretical model accounting for change in the Förster radius caused by the strong energy transfer to metal.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Ozone Gas: Scientific Justification and Practical Guidelines for Improvised Disinfection using Consumer-Grade Ozone Generators and Plastic Storage Boxes

Here, we describe direct measurements of ozone concentration achievable in small enclosed containers (plastic storage boxes) for use as improvised decontamination systems for small articles such as disposable PPE (N95 masks, nitrile gloves, etc.), clothing, mail and small packages, food, and other miscellaneous articles. The emphasis is on the reliable and sustained generation of ozone gas concentrations of sufficient concentration and duration to create an effective virucidal environment to achieve more than 95% to 99% viral inactivation, based upon the data already published in the peer-review literature on this topic. The suggestion that ozone be used to inactivate virus is certainly not a new idea. Our objective in this report is to make clear that the necessary levels of ozone can be improvised using simple, easy-to-use, inexpensive, and widely available supplies, and that there is every theoretical and experimental reason to believe that this approach is as highly effective in viral inactivation by ozone as are the far more expensive, complex, cumbersome, and less available equivalent ozone (and other) disinfectant systems that have themselves become unavailable during times of pandemic crisis. Using multiple types of readily available commercial ozone generators, concentration in the tested improvised enclosure is tracked over time to assess ozone charging and decay rates, and the ozone quenching effects of items placed in the box. Generator performance is compared against published ozone dosage values for virucidal and antimicrobial activity. Bubbler and box-fan-type ozone generators were found to be effective at achieving and maintaining target concentrations of 10ppm ozone or higher, whereas automotive cigarette lighter and universal serial bus type plug in “air freshener” ozone generators could not achieve the target concentrations in these experiments. Calculations and practical guidelines for assembly and effective use of an ozone box for improvised decontamination are offered. The majority of this report is directed toward the scientific justification and rationale for this approach. The end of the document summarizes the findings and offers simplified designs for the construction and use of ozone boxes as an improvised method of disinfection.

60 APPLIED LIFE SCIENCES↗
DOE OSTI2024

Artificial Intelligence Assisted Inversion (AIAI): Quantifying the Spectral Features of 56 Ni of Type Ia Supernovae

Abstract Following our previous study of Artificial Intelligence Assisted Inversion (AIAI) of supernova analyses, we train a set of deep neural networks based on the 1D radiative transfer code TARDIS to simulate the optical spectra of Type Ia supernovae (SNe Ia) between 10 and 40 days after the explosion. The neural networks are applied to derive the mass of 56 Ni in velocity ranges above the photosphere for a sample of 124 well-observed SNe Ia in the TARDIS model context. A subset of the SNe have multi-epoch observations for which the decay of the radioactive 56 Ni can be used to test the AIAI quantitatively. The 56 Ni mass derived from AIAI using the observed spectra as inputs for this subset agrees with the radioactive decay rate of 56 Ni. AIAI reveals that a spectral signature near 3890 Å is related to the Niii4067Å line, and the 56 Ni mass deduced from AIAI is found to be correlated with the light-curve shapes of SNe Ia, with SNe Ia with broader light curves showing larger 56 Ni mass in the envelope above the photosphere. AIAI enables spectral data of SNe to be quantitatively analyzed under theoretical frameworks based on well-defined physical assumptions.

Astronomy & Astrophysics↗
DOE OSTI2024

Impact of Systematic Modeling Uncertainties on Kilonova Property Estimation

The precise atomic structure and therefore the wavelength-dependent opacities of lanthanides are highly uncertain. This uncertainty introduces systematic errors in modeling transients like kilonovae and estimating key properties such as mass, characteristic velocity, and heavy metal content. Here, we quantify how atomic data from across the literature as well as choices of thermalization efficiency of r-process radioactive decay heating impact the light curve and spectra of kilonovae. Specifically, we analyze the spectra of a grid of models produced by the radiative transfer code Sedona that span the expected range of kilonova properties to identify regions with the highest systematic uncertainty. Our findings indicate that differences in atomic data have a substantial impact on estimates of lanthanide mass fraction, spanning approximately 1 order of magnitude for lanthanide-rich ejecta, and demonstrate the difficulty in precisely measuring the lanthanide fraction in lanthanide-poor ejecta. Mass estimates vary typically by 25%–40% for differing atomic data. Similarly, the choice of thermalization efficiency can affect mass estimates by 20%–50%. Observational properties such as color and decay rate are highly model dependent. Velocity estimation, when fitting solely based on the light curve, can have a typical error of ∼100%. Atomic data of light r-process elements can strongly affect blue emission. Even for well-observed events like GW170817, the total lanthanide production estimated using different atomic data sets can vary by a factor of ∼6.

Gravitational wave sources↗
DOE OSTI2025

Nonthermal Ionization of Kilonova Ejecta: Observable Impacts

The characteristic rapid rise and decline at optical wavelengths of a kilonova is the product of the low ejecta mass (≲0.05 M ⊙ ) and high ejecta velocity (≳0.1c). We show that, even at very early times (≲2 days), regions of ejecta fall below critical density and temperature thresholds at which nonlocal thermodynamic equilibrium (NLTE) effects become important. Here, we present an approximate method for calculating the ionization state of the ejecta that accounts for the NLTE impact of high-energy electrons produced in the beta decay of freshly synthesized r-process elements. We find that incorporating ionization from high-energy electrons produces an “inverted” and “blended” ionization structure, where the most highly ionized species are located in the fastest moving homologous ejecta, and multiple ionization states coexist. In radiation transport calculations, the higher degree of ionization reduces line blanketing in optical bands, leading to improved agreement with the light-curve properties of AT 2017gfo, such as the duration, decay rates, brightness, and colors. Our quasi-NLTE implementation helps to alleviate tensions in kilonova modeling: for high-velocity (∼0.3 c) ejecta components, our models require less mass for a given peak brightness in optical bands, by as much as a factor of 3; our models can explain the presence of observed features associated to Sr II, W III, Se III, and Te III under conditions where LTE models would predict only neutral species; and we naturally predict the coexistence of species like Sr II and Ce III without the need for fine-tuning of the ejecta properties.

High energy astrophysics↗
DOE OSTI2025

XRISM Constraints on Unidentified X-Ray Emission Lines, Including the 3.5 keV Line, in the Stacked Spectrum of 10 Galaxy Clusters

We stack 3.75 Ms of early XRISM Resolve observations of 10 galaxy clusters to search for unidentified spectral lines in the E = 2.5–15 keV band (rest frame), including the E = 3.5 keV line reported in earlier low spectral resolution studies of cluster samples. Such an emission line may originate from the decay of the sterile neutrino, a warm dark matter (DM) candidate. No unidentified lines are detected in our stacked cluster spectrum, with the 3σ upper limit on the m s ∼ 7.1 keV DM particle decay rate (which corresponds to an E = 3.55 keV emission line) of Γ ∼ 1.0 × 10 −27 s −1 . This upper limit is 3–4 times lower than the one derived by Hitomi Collaboration from the Perseus observation but still 5 times higher than the XMM-Newton detection reported by E. Bulbul et al. in the stacked cluster sample. XRISM Resolve, with its high spectral resolution but small field of view, may reach the sensitivity needed to test the XMM-Newton cluster sample detection by combining several years worth of future cluster observations.

Astronomy and AstroPhysics↗
NASA NTRS1963

THE MAIN PHASE OF GREAT MAGNETIC STORMS

Demonstration that the main phase of great geomagnetic storms is composed of two parts, characterized by different decay rates of the ring current field

MAGNETIC STORM↗
NASA NTRS1969

Radiative effects in semiclassical theory.

Unquantized field calculations extended to include atomic field effect on atom, predicting spontaneous decay rate from excited state and light frequency time dependence

Crisp, M. D.↗