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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 433 records · Page 24

Raman Laser-Induced Structural Modification in CVD-Grown Monolayer MoS 2 for Multi-Purposed Nanofabrication

Molybdenum disulfide (MoS 2 ) has been extensively explored to be utilized as an electronic material in a variety of device applications. In particular, the tunability of MoS 2 enhances its electrical properties making it an intriguing candidate for field-effect transistors (FETs), while also extending beyond electrical properties to structural phase engineering. Laser-induced modifications, particularly with Raman lasers, offer a straightforward method to modulate materials via thermal processes with precise patterning control and energy-level flexibility. However, most studies on the modification of MoS 2 have focused on multilayered structures or have been conducted under low-power laser conditions, leaving the feasibility of structural modifications in monolayer MoS 2 elusive. In this study, we fundamentally elucidated the effects of high-power Raman laser irradiation on the surface of chemical vapor deposition (CVD)-grown monolayer MoS 2 under ambient conditions and uncovered the underlying mechanisms of laser-induced modifications by applying intense photon energy with highly interactive reactions. Our results revealed both etching and deposition phenomena in two discernible regions, and it can be demonstrated by intensity regimes based on the spatial distribution of laser irradiance within the laser-irradiated spot. Furthermore, phase transition was found to be inhibited due to the promoted oxidation and the deposition of hydrogenated amorphous carbon (a-C:H), and p-type doping was observed, likely occurring in the region beneath the a-C:H deposition as substitutional doping on the 2H phase of MoS 2 . To compare the thermal effects, MoS 2 modifications were further analyzed using simplified heat transfer estimations. In conclusion, these findings deepen our understanding of how Raman laser irradiation modifies MoS 2 under ambient conditions, providing guidelines for optimizing its modification processes.

36 MATERIALS SCIENCE↗

Efficient backward x-ray emission in a finite-length plasma irradiated by a laser pulse of picosecond duration

Motivated by experiments employing picosecond-long, kilojoule laser pulses, we examined x-ray emission in a finite-length underdense plasma irradiated by such a pulse using two-dimensional particle-in-cell simulations. We found that, in addition to the expected forward emission, the plasma also efficiently emits in the backward direction. Our simulations reveal that the backward emission occurs when the laser exits the plasma. The longitudinal plasma electric field generated by the laser at the density down-ramp turns around some of the laser-accelerated electrons and re-accelerates them in the backward direction. As the electrons collide with the laser, they emit hard x rays. The energy conversion efficiency is comparable to that for the forward emission, but the effective source size is smaller. We show that the picosecond laser duration is required for achieving a spatial overlap between the laser and the backward energetic electrons. At peak laser intensity of 1.4×1020 W/cm2, backward-emitted photons (energies above 100 keV and 10° divergence angle) account for 2×10−5 of the incident laser energy. This conversion efficiency is three times higher than that for similarly selected forward-emitted photons. The source size of the backward photons (5 μm) is three times smaller than the source size of the forward photons.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Pointing stabilization of a 1 Hz high-power laser via machine learning

Abstract High-power lasers are vital for particle acceleration, imaging, fusion and materials processing, requiring precise control and high-energy delivery. Laser plasma accelerators (LPAs) demand laser positional stability at focus to ensure consistent electron beams in applications such as X-ray free-electron lasers and high-energy colliders. Achieving this stability is especially challenging for the low-repetition-rate lasers in current LPAs. We present a machine learning method that predicts and corrects laser pointing instabilities in real-time using a high-frequency pilot beam. By preemptively adjusting a correction mirror, this approach overcomes traditional feedback limits. Demonstrated on the BELLA petawatt laser operating at the terawatt level (30 mJ amplification), our method achieved root mean square pointing stabilization of 0.34 and 0.59 $\unicode{x3bc} \mathrm{rad}$ in the x and y directions, reducing jitter by 65% and 47%, respectively. This is the first successful application of predictive control for shot-to-shot stabilization in low-repetition-rate laser systems, paving the way for full-energy petawatt lasers and transformative advances across science, industry and security.

Amodio, Alessio↗

Path to a single-stage, 100-GeV electron beam via a flying-focus-driven laser-plasma accelerator

Dephasingless laser wakefield acceleration (DLWFA), a novel laser wakefield acceleration concept based on the recently demonstrated “flying focus” technology, offers a new paradigm in laser-plasma acceleration that could advance the progress toward a TeV linear accelerator using a single-stage system without guiding structures. The recently proposed NSF OPAL laser facility could be the transformative technology that enables this grand challenge in laser-plasma acceleration. We review the viable parameter space for DLWFA based on the scaling of its performance with laser and plasma parameters, and we compare that performance to traditional laser wakefield acceleration. These scalings indicate the necessity for ultrashort, high-energy laser architectures such as NSF OPAL to achieve groundbreaking electron energies using DLWFA. Initial results from MTW-OPAL, the platform for the 6-J DLWFA demonstration experiment, show a tight, round focal spot over a distance of 3.7 mm. New particle-in-cell simulations of that platform indicate that using hydrogen for DLWFA reduces the amount of laser light that is distorted due to refraction at ionization fronts. An experimental path, and the computational and technical design work along that path, from the current status of the field to a single-stage, 100-GeV electron beam via DLWFA on NSF OPAL is outlined. Progress along that path is presented.

Shaw, J. L. [University of Rochester, NY (United S↗

Laser aircraft

The concept of a laser-powered aircraft is discussed. Laser flight would be completely compatible with existing airports and air-traffic control, with the airplane using kerosene only power, up to a cruising altitude of 9 km where the laser satellite would lock on and beam laser energy to it. Two major components make up the laser turbofan, a heat exchanger for converting laser radiation into thermal energy, and conventional turbomachinery. The laser power satellite would put out 42 Mw using a solar-powered thermal engine to generate electrical power for the closed-cycle supersonic electric discharge CO laser, whose radiators, heat exchangers, supersonic diffuser, and ducting will amount to 85% of the total subsystem mass. Relay satellites will be used to intercept the beam from the laser satellite, correct outgoing beam aberrations, and direct the beam to the next target. A 300-airplane fleet with transcontinental range is projected to save enough kerosene to equal the energy content of the entire system, including power and relay satellites, in one year.

Hertzberg, A.↗

Ultraviolet lasers. Citations from the International Aerospace Abstracts data base

Reports cited from the international literature describe various aspects of ultraviolet lasers including laser output, far ultraviolet radiation, electron pumping, optical pumping, and laser materials. Gas lasers, pulsed lasers, dye lasers, CO2 lasers, xenon fluoride lasers, and transversely excited atmospheric (TEA) lasers are considered. This updated bibliography contains 283 citations, 66 of which are new additions to the previous edition.

Mauk, S. C.↗

Tunable diode lasers for 3-30 micron infrared operation

The tunable diode laser is now widely used in high resolution infrared spectroscopy studies, taking into account laboratory and industrial applications. The present investigation is concerned with advances related to laser performance and reliability. The advances are the result of improvements in materials and device technologies. Reliability data for broad-area Pb(1-x)Sn(x)Se lasers are considered along with performance improvements in stripe-geometry lasers, laser performance at wavelengths above 25 microns, and laser performance at wavelengths below 4 microns. Attention is given to tunable Pb-salt infrared diode lasers, mesa-stripe geometry lasers of Pb(1-x)Sn(x)Se and PbS(1-x)Se(x), and long wavelength diode laser emission observed in both Pb(1-x)Sn(x)Te and Pb(1-x)Sn(x)Se.

Linden, K. J.↗

Laser production and heating of plasma for MHD application

Experiments have been made on the production and heating of plasmas by the absorption of laser radiation. These experiments were performed to ascertain the feasibility of using laser-produced or laser-heated plasmas as the input for a magnetohydrodynamic (MHD) generator. Such a system would have a broad application as a laser-to-electricity energy converter for space power transmission. Experiments with a 100-J-pulsed CO2 laser were conducted to investigate the breakdown of argon gas by a high-intensity laser beam, the parameters (electron density and temperature) of the plasma produced, and the formation and propagation of laser-supported detonation (LSD) waves. Experiments were also carried out using a 1-J-pulsed CO2 laser to heat the plasma produced in a shock tube. The shock-tube hydrogen plasma reached electron densities of approximately 10 to the 17th/cu cm and electron temperatures of approximately 1 eV. Absorption of the CO2 laser beam by the plasma was measured, and up to approximately 100 percent absorption was observed. Measurements with a small MHD generator showed that the energy extraction efficiency could be very large with values up to 56 percent being measured.

Jalufka, N. W.↗

Comparison of electrically driven lasers for space power transmission

High-power lasers in space could provide power for a variety of future missions such as spacecraft electric power requirements and laser propulsion. This study investigates four electrically pumped laser systems, all scaled to 1-MW laser output, that could provide power to spacecraft. The four laser systems are krypton fluoride, copper vapor, laser diode array, and carbon dioxide. Each system was powered by a large solar photovoltaic array which, in turn, provided power for the appropriate laser power conditioning subsystem. Each system was block-diagrammed, and the power and efficiency were found for each subsystem block component. The copper vapor system had the lowest system efficiency (6 percent). The CO2 laser was found to be the most readily scalable but has the disadvantage of long laser wavelength.

Deyoung, R. J.↗

Magnetically switched power supply system for lasers

A laser power supply system is described in which separate pulses are utilized to avalanche ionize the gas within the laser and then produce a sustained discharge to cause the gas to emit light energy. A pulsed voltage source is used to charge a storage device such as a distributed capacitance. A transmission line or other suitable electrical conductor connects the storage device to the laser. A saturable inductor switch is coupled in the transmission line for containing the energy within the storage device until the voltage level across the storage device reaches a predetermined level, which level is less than that required to avalanche ionize the gas. An avalanche ionization pulse generating circuit is coupled to the laser for generating a high voltage pulse of sufficient amplitude to avalanche ionize the laser gas. Once the laser gas is avalanche ionized, the energy within the storage device is discharged through the saturable inductor switch into the laser to provide the sustained discharge. The avalanche ionization generating circuit may include a separate voltage source which is connected across the laser or may be in the form of a voltage multiplier circuit connected between the storage device and the laser.

Pacala, Thomas J.↗

Development in tunable solid state lasers with high spectral purity, high efficiency and long lifetime for differential absorption lidar

The paper presents a review of tunable vibronic solid state lasers for DIAL measurements and provides new experimental results for tunable Ti:sapphire lasers, materials development, and spectral bandwidth narrowing through injection control. Pulsed injection control of a Ti:sapphire laser with a 2.5-pm narrow band pulsed dye laser and with another Ti:sapphire laser is demonstrated with nearly complete energy extraction, indicating homogeneous line broadening. The status of tunable solid state lasers in the 1.6-2.3 micron range for DIAL measurements of trace gases, and development trends for lasers with reduced cryogenic cooling needs, are included. The effects of laser gain on optical damage, energy extraction, and amplified spontaneous emission are indicated for several tunable lasers.

Hess, R. V.↗

Direct solar-pumped iodine laser amplifier

The optimum conditions of a solar pumped iodine laser are found in this research for the case of a continuous wave operation and a pulsed operation. The optimum product of the pressure(p) inside the laser tube and the tube diameter(d) was pd=40 approx. 50 torr-cm on the contrary to the case of a high intensity flashlamp pumped iodine laser where the optimum value of the product is known to be pd=150 torr-cm. The pressure-diameter product is less than 1/3 of that of the high power iodine laser. During the research period, various laser materials were also studied for solar pumping. Among the laser materials, Nd:YAG is found to have the lowest laser threshold pumping intensity of about 200 solar constant. The Rhodamine 6G was also tested as the solar pumped laser material. The threshold pumping power was measured to be about 20,000 solar constant. The amplification experiment for a continuously pumped iodine laser amplifier was performed using Vortek solar simulator and the amplification factors were measured for single pass amplification and triple pass amplification of the 15 cm long amplifier tube. The amplification of 5 was obtained for the triple pass amplification.

Han, Kwang S.↗

An investigation of a mathematical model of an optically pumped Ti(3+):Al2O3 laser system

During the last several years, solid state lasers were developed that have the potential for meeting rigorous performance requirements for space-based remote sensing of the atmosphere. In order to design a stable and efficient laser and to understand the effect on laser output of changes in the physical and design parameters, an understanding of the development of the dynamical processes of the laser is necessary. Typically, the dynamical processes in a laser system are investigated via rate equations describing the evolution of the occupancy in the electronic levels and of the photon density in the laser cavity. There are two approaches to this type of study. Most often, for the sake of simplicity, the spatial variations of the dynamic variables in the laser system are disregarded and the mathematical model consists of a system of first order nonlinear ordinary differential equations (ODE). The second approach is to take into account both spatial and temporal variations in the dynamic variables in the laser cavity. The resulting model consists of a first order semilinear system of partial differential equations (PDE). The model which was studied was studied was generic in the sense that it was a four-level laser system, but the parameters used in the numerical study were specific to Titanium-doped sapphire. For simplicity, a constant, spatially uniform pumping scheme was considered. In addition, a simplification of the model was made so that it treats a single lasing wavelength with a narrow bandwidth. The purpose was to investigate both versions of the mathematical model and to determine whether the numerical solutions are similar both qualitatively and quantitatively. The systems of ordinary differential equations were solved numerically using a Runge-Kutta-Fehlberg algorithm which was very efficient for typical values of the physical parameters. A numerical scheme, based on the Modified Euler method, for computing solutions to the system of partial differential equations was developed and implemented. The PDE model was solved numerically at the expense of greatly increased computer time.

Roberts, Lila F.↗

Injection-seeded operation of a Q-switched Cr,Tm,Ho:YAG laser

Single-frequency Tm,Ho:YAG lasers operating near 2 microns are attractive sources for several applications including eye-safe laser radar (lidar) and pumping of AgGaSe2 parametric oscillators for efficient generation of longer wavelengths. As part of a program to develop a coherent lidar system using Tm,Ho:YAG lasers, a diode laser-pumped tunable CW single-longitudinal-mode (SLM) Cr:Tm:Ho:YAG laser and a flashlamp-pumped single-transverse-mode Q-switched Cr,Tm,Ho:YAG laser were developed. The CW laser was used to injection-seed the flashlamp-pumped laser, resulting in SLM Q-switched output. Operational characteristics of the CW and Q-switched lasers and injection-seeding results are reported.

Henderson, Sammy W.↗

Scientific applications of frequency-stabilized laser technology in space

A synoptic investigation of the uses of frequency-stabilized lasers for scientific applications in space is presented. It begins by summarizing properties of lasers, characterizing their frequency stability, and describing limitations and techniques to achieve certain levels of frequency stability. Limits to precision set by laser frequency stability for various kinds of measurements are investigated and compared with other sources of error. These other sources include photon-counting statistics, scattered laser light, fluctuations in laser power, and intensity distribution across the beam, propagation effects, mechanical and thermal noise, and radiation pressure. Methods are explored to improve the sensitivity of laser-based interferometric and range-rate measurements. Several specific types of science experiments that rely on highly precise measurements made with lasers are analyzed, and anticipated errors and overall performance are discussed. Qualitative descriptions are given of a number of other possible science applications involving frequency-stabilized lasers and related laser technology in space. These applications will warrant more careful analysis as technology develops.

Schumaker, Bonny L.↗

KrF laser-induced OH fluorescence imaging in a supersonic combustion tunnel

Planar fluorescence images of OH in a continuous-flow, electrical-resistively heated, high enthalpy, hydrogen-air combustion tunnel, induced by a tunable KrF laser, were recorded. These images were compared to previously recorded fluorescence images induced by a doubled-dye laser under similar conditions. Images induced by the doubled-dye laser system demonstrated a severe distortion caused by absorption and fluorescence trapping. By contrast, images of the fluorescence induced by the tunable KrF laser retained the symmetry properties of the flow. Based on signal-to-noise ratio measurements the yield of the fluorescence induced by the doubled-dye laser is larger than the fluorescence yield induced by the KrF laser. The measurements in the present facility of OH fluorescence induced by the KrF laser were limited by the photon-statistical noise. Based 2 on this result, doubled-dye laser systems are recommended for OH imaging in small and OH lean (less than 10 exp 15/cu cm) facilities. KrF lasers should be selected otherwise.

Quagliaroli, T. M.↗

Spectral performance of monolithic holmium and thulium lasers

Fabry-Perot resonators have been used to demonstrate single-mode lasing of holmium and neodymium YAG. The previous demonstration in the holmium laser required TE cooling the crystal to -15 C in order to achieve threshold. The present study extends that result, demonstrating +25 C operation in a 1-mm thick plano/plano resonator. The experimental configuration of lasing both the holmium and thulium lasers used a 500-mW diode laser which was collimated, circularized, and focused into a beam radius of 60 microns. The single-frequency lasing spectrum of the holmium laser is shown. By adjusting the mirror reflectivity, the ability to control the laser's wavelength is demonstrated. This laser operated with 11 mW of optical power, a 57-percent slope efficiency, and 120-mW threshold vs absorbed diode power laser for the 60-micron beam radius. The thulium laser operated very efficiently at room temperature, but on seven longitudinal modes. The Tm:TAG laser exhibits typical characteristics of spatial hole burning not seen in the Ho:Tm:YAG for flat/flat resonators.

Storm, Mark E.↗

Modeling of high efficiency solar cells under laser pulse for power beaming applications

Solar cells have been used to convert sunlight to electrical energy for many years and also offer great potential for non-solar energy conversion applications. Their greatly improved performance under monochromatic light compared to sunlight, makes them suitable as photovoltaic (PV) receivers in laser power beaming applications. Laser beamed power to a PV array receiver could provide power to satellites, an orbital transfer vehicle, or a lunar base. Gallium arsenide (GaAs) and indium phosphide (InP) solar cells have calculated efficiencies of more than 50 percent under continuous illumination at the optimum wavelength. Currently high power free-electron lasers are being developed which operate in pulsed conditions. Understanding cell behavior under a laser pulse is important in the selection of the solar cell material and the laser. An experiment by NAsA lewis and JPL at the AVLIS laser facility in Livermore, CA presented experimental data on cell performance under pulsed laser illumination. Reference 5 contains an overview of technical issues concerning the use of solar cells for laser power conversion, written before the experiments were performed. As the experimental results showed, the actual effects of pulsed operation are more complicated. Reference 6 discusses simulations of the output of GaAs concentrator solar cells under pulsed laser illumination. The present paper continues this work, and compares the output of Si and GaAs solar cells.

Jain, Raj K.↗