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At least 433 records · Page 24
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Estimation of Fission Product Transport Parameters for Cesium in the AGR-3/4 TRISO Fuel Experiment

A one-dimensional (1D) finite-element model of fission product transport in the AGR-3/4 experiment has been developed using the Multiphysics Object Oriented Simulation Environment (MOOSE) framework and implemented in the fuel performance code, BISON. The model resolves capsule-specific geometries, materials, and temperature histories and simulates radial migration of fission products from the fuel compact through the inner ring, outer ring, and into the sink ring. Model parameters governing diffusion and sorption were estimated for key fission products – cesium (Cs), and europium (Eu) – by simultaneously fitting modeled isotopic concentration profiles and total ring inventories to a post-irradiation experimental measurement. These data include gamma scanning, liquid scintillation for Sr-90, radial deconsolidation leach-burn-leach analysis, tomographic reconstructions, and destructive physical sampling. A mortar-based interfacial sorption framework was implemented to enforce physically consistent mass transfer and flux conservation across gas gaps. Two classes of parameter sets were derived: a least-squares best-fit, and a safety-oriented conservative-fit, what applies strong penalties for underprediction of sink inventories. Across all twelve capsules, the model successfully reproduces the dominant radial transport trends for Cs, Sr, with decreasing concentrations from the compact outward through successive rings. Cs behavior is captured most consistently, while strontium predictions reveal systematic trade-offs between compact accuracy and conservative sink-ring bounding. The results demonstrate that sink ring weighted calibration provides conservative, safety relevant bounds on low temperature fission product transport, but at the cost of underpredicting compact inventories for Sr isotopes. These discrepancies highlight the need for additional physics, including fast-slow diffusion model, incorporating trapping mechanism in the transport behavior. Overall, this work establishes a robust, capsule-specific modeling framework for AGR-3/4 fission product transport and provides a defensible basis for parameter selection in source-term and fuel performance analyses for high temperature gas-cooled reactors.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

Measuring Neutron Polarisation in Deuteron Photo-disintegration with the CLAS Start Counter [Thesis]

Deuteron photo-disintegration (γd → γp) is a reaction that represents the simplest case in which nuclear and hadron physics models can be tested. Despite this, associated polarization analyses are limited in terms of angular coverage and energy ranges, especially in observables related to the recoil neutron. This is largely due to a lack in dedicated polarimetry equipment, and represents a roadblock in global progress to understand high-energy phenomena such as hexaquarks, and quark-gluon degrees of freedom. To address this problem, this PhD thesis pioneers a new methodology for the parasitic measurement of nucleon polarization using kinematic reconstruction of (spin-dependent) nucleon-nucleus scattering of reaction products, prior to their detection in large acceptance particle detector apparatus. Following this novel approach, which requires no dedicated polarimeter, a determination of the double polarization observable, $C^n_{x'}$, from deuteron photo-disintegration is presented, using Jefferson Lab’s CLAS detector. The analysis utilizes the (n,p) charge exchange reaction in CLAS’s "start counter" (plastic scintillator) to determine the final state neutron polarizations. The results present the first ever data for this observable above 0.7 GeV (photon beam energy) and significantly extend the angular range of the world data set. This new data is largely statistically consistent with the previous measurement of $C^n_{x'}$ by Bashkanov et al . in the overlapping energy range of 0.4-0.7 GeV. It is planned for the statistical accuracy of the presented result to be increased by the inclusion of additional data. The analysis herein serves as a key proof of concept for future applications, including a recommended similar analysis to be implemented with data from the more modern CLAS12 detector. This paves the way for a plethora of additional analyses using existing data sets that would provide crucial new constraints for hadron and nuclear physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2026

Detector architecture and data flow of the CMS HGCAL Phase-2 Endcap Calorimeter Upgrade

The CMS High Granularity Calorimeter (HGCAL) is the Phase-2 endcap calorimeter upgrade for the High-Luminosity Large Hadron Collider, designed to provide precise spatial, energy, and timing measurements in a high-radiation, high-pileup environment. This work presents an overview of the HGCAL assembly process, detector architecture, and end-to-end data flow. The data flow goes from signal generation in silicon sensors and scintillator tiles through front-end electronics, optical transmission, and back-end data acquisition. The study highlights how the integrated detector, electronics, and readout systems enable efficient event reconstruction and support the physics objectives of the HL-LHC.

Osei Boakye, Prince [Grambling State U.]↗
DOE OSTI2026

NOvA in 10 Minutes

NOvA is a long-baseline neutrino oscillation experiment that utilizes the NuMI beamline at Fermilab. The experiment consists of two functionally identical, segmented liquid scintillator detectors. A 300-ton near detector sits at Fermilab, while a 14-kiloton far detector is located 810 km away in Ash River, Minnesota. Both are situated 14.6 mrad off the beam axis to peak the neutrino energy spectrum near the first oscillation maximum. NOvA measures muon neutrino disappearance and electron neutrino appearance in both neutrino and antineutrino beam modes, providing sensitivity to the neutrino mass ordering, the octant of the atmospheric mixing angle \theta_{23}, and the CP-violating phase \delta_{CP}. In this talk, I will give a concise overview of the NOvA experiment and its detectors, followed by highlights from recent oscillation analyses. I will also highlight notable cross-section measurements at the near detector. Finally, I will briefly introduce ongoing analyses beyond the standard three-flavor oscillation framework, including searches for sterile neutrinos and non-standard interactions, as well as exotic signatures such as magnetic monopoles, light dark matter, neutrino magnetic moments, and cosmic-ray muon studies.

Khanam, Aklima [Syracuse U. (main)] (ORCID:0009000↗
DOE OSTI2024

Understanding the temperature and humidity dependence of the SiPM characteristics

A miniature version of the ICAL experiment at the India-based Neutrino Observatory, the mini-ICALis in operation at the IICHEP, Madurai. The commissioning work of a Cosmic Muon Veto detector (CMVD)on top of the mini-ICAL is continued using extruded plastic scintillators with embeddedWLS fibers and the SiPM as a photo-transducer. The CMVD is being built to study thefeasibility of a cosmic muon veto for a shallow-depth neutrino experiment. The SiPM is calibratedusing an ultrafast LED driver andthe same calibration techniques will be used during the data taking period with a simplified LED in thesame readout PCB. An experimental setup wasdesigned to characterise the SiPMs in a temperature controlled environment. The readout electronicsinvolves trans-impedance amplifiers and a voltage followers of combined gain 1.24 mV/$\mu$A and adigital storage oscilloscope for the data collection with a minimal distortion of SiPM signal.Various characteristics of the Hamamatsu SiPM (S13360-2050VE), e.g. signal shape, optically correlatedand uncorrelated noise, recovery time etc were studied as a function of $V_{ov}$, number of photoelectrons,the ambient temperature and the humidity. This paper will cover the details of those results.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

A review of NEST models for liquid xenon and an exhaustive comparison with other approaches

This paper discusses the microphysical simulation of interactions in liquid xenon, the active detector medium in many leading rare-event searches for new physics, and describes experimental observables useful for understanding detector performance. The scintillation and ionization yield distributions for signal and background are presented using the Noble Element Simulation Technique (NEST), a toolkit based on experimental data and simple empirical formulas, which mimic previous microphysics modeling but are guided by data. The NEST models for light and charge production as a function of the particle type, energy, and electric field are reviewed, along with models for energy resolution and final pulse areas. NEST is compared with other models or sets of models and validated against real data, with several specific examples drawn from XENON, ZEPLIN, LUX, LZ, PandaX, and table-top experiments used for calibrations.

WIMPs↗
DOE OSTI2026

Operation of a Modular 3D-Pixelated Liquid Argon Time-Projection Chamber in a Neutrino Beam

The 2x2 Demonstrator, a prototype for the Deep Underground Neutrino Experiment (DUNE) liquid argon (LAr) Near Detector, was exposed to the Neutrinos from the Main Injector (NuMI) neutrino beam at Fermi National Accelerator Laboratory (Fermilab). This detector is a prototype of a new modular design for a liquid argon time-projection chamber (LArTPC), comprising a two-by-two array of four modules, each further segmented into two optically isolated LArTPCs. The 2x2 Demonstrator features a number of pioneering technologies, including a low-profile resistive field shell to establish drift fields, native 3D ionization pixelated imaging, and a high-coverage dielectric light readout system. The 2.4-tonne active mass detector is flanked upstream and downstream by supplemental solid-scintillator tracking planes, repurposed from the MINERvA experiment, which track ionizing particles exiting the argon volume. The antineutrino beam data collected by the detector over a 4.5 day period in 2024 include over 30,000 neutrino interactions in the LAr active volume—the first neutrino interactions reported by a DUNE detector prototype. During its physics-quality run, the 2x2 Demonstrator operated at a nominal drift field of 500 V/cm and maintained good LAr purity, with a stable electron lifetime of approximately 1.25 ms. This paper describes the detector and supporting systems, summarizes the installation and commissioning, and presents the initial validation of collected NuMI beam and off-beam self-triggers. In addition, it highlights observed interactions in the detector volume, including candidate muon antineutrino events.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

Limits on the Low-energy Electron Antineutrino Flux from the Brightest Gamma-Ray Burst of All Time

The electron antineutrino flux limits are presented for the brightest gamma-ray burst (GRB) of all time, GRB221009A, over a range of 1.8–200 MeV using the Kamioka Liquid Scintillator Antineutrino Detector. Using multiple time windows ranging from minutes to days surrounding the event to search for electron antineutrinos coincident with the GRB, we set an upper limit on the flux under the assumption of several power-law neutrino source spectra, with power-law indices ranging from 1.5 to 3 in steps of 0.5. No excess was observed in any time windows ranging from seconds to days around the event trigger time T 0 . For a power-law index of 2 and a time window of T 0 ± 500 s, a flux upper limit of 2.34 × 10 9 cm −2 was calculated. The limits are compared to the results presented by IceCube.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Spectral Properties of Globally Distributed ENA Fluxes across Diverse Regions of the Heliosphere

This study analyzes energetic neutral atom (ENA) spectral properties across distinct regions of globally distributed flux (GDF) sky maps, using Interstellar Boundary Explorer data from a full solar cycle, corrected for time dispersion. By time-shifting the data to the heliosheath using GDF source distances from D. B. Reisenfeld et al., we achieve a more accurate representation of heliosheath GDF energy spectra. We quantify ENA spectral characteristics, heliosheath line-of-sight-integrated proton pressure, and heliosheath proton temperature, comparing these to solar wind properties at 1 au and interplanetary scintillation-derived solar wind data. Our findings show that the spectral index is generally anticorrelated with heliosheath proton temperature and pressure, except in the central tail, where a partial positive correlation is observed. The lowest spectral index values occur when high-latitude heliosheath regions are dominated by fast solar wind from polar coronal holes. The south pole exhibits the flattest energy spectra due to plasma heating from both fast solar wind and a late-2014 pressure pulse. The central tail shows shorter variability (5–6 yr) for spectral index and heliosheath proton temperature, while proton pressure follows the 11 yr solar cycle. Most spectral shapes exhibit a “knee” distribution, peaking during solar maximum, with an “ankle” shape observed only at the south pole during solar cycle transitions. Asymmetry in proton pressure in the lobes is driven by the draping effect of the local interstellar magnetic field. This study provides insights into the energetic properties of GDF across the heliosphere, enhancing our understanding of the heliospheric environment.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

A Unified Model of Cosmic-Ray Propagation and Radio Extreme Scattering Events from Intermittent Interstellar Structures

Intermittent magnetic structures are a plausible candidate for explaining cosmic-ray (CR) diffusion rates derived from observed CR energy spectra. Independently, studies of extreme scattering events (ESEs) of radio quasars and pulsar scintillation have hinted that very straight, large aspect ratio magnetic current sheets may be responsible for the localized large scattering of radio waves. The required shortest axis of the typical structures producing ESEs is of the same scale (∼au) as the gyroradii of ∼GeV CRs. In this Letter, we propose that the same magnetic/density sheets can produce large scattering of both CRs and radio waves. We demonstrate that the geometry and volume-filling factor of the sheets derived from quasar ESEs can explain the observed mean free path of GeV CRs without introducing free parameters. The model places constraints on the sheet geometry, such as straightness and large aspect ratio, and assumes that the statistics of the sheets are similar throughout the Galactic volume. We therefore discuss observational tests of the sheet model, which includes observations of echoes in pulsars and fast radio bursts, gravitationally lensed quasars, the distribution of ESE durations, and spatial correlations between ESE events and rotation measure fluctuations. Such tests will be enabled by upcoming wide-field radio instruments, including the Canadian Hydrogen Observatory and Radio-transient Detector and Deep Synoptic Array 2000 Antennas.

Kempski, Philipp [Princeton Univ., NJ (United Stat↗
DOE OSTI2025

MATHUSLA: An External Long-Lived Particle Detector to Maximize the Discovery Potential of the HL-LHC

We present the current status of the MATHUSLA (MAssive Timing Hodoscope for Ultra-Stable neutraL pArticles) long-lived particle (LLP) detector at the HL-LHC, covering the design, fabrication and installation at CERN Point 5. MATHUSLA40 is a 40 m-scale detector with an air-filled decay volume that is instrumented with scintillator tracking detectors, to be located near CMS. Its large size, close proximity to the CMS interaction point and about 100 m of rock shielding from LHC backgrounds allows it to detect LLP production rates and lifetimes that are one to two orders of magnitude beyond the ultimate reach of the LHC main detectors. This provides unique sensitivity to many LLP signals that are highly theoretically motivated, due to their connection to the hierarchy problem, the nature of dark matter, and baryogenesis. Data taking is projected to commence with the start of HL-LHC operations. We summarize the new 40m design for the detector that was recently presented in the MATHUSLA Conceptual Design Report, alongside new realistic background and signal simulations that demonstrate high efficiency for the main target LLP signals in a background-free HL-LHC search. We argue that MATHUSLA's uniquely robust expansion of the HL-LHC physics reach is a crucial ingredient in CERN's mission to search for new physics and characterize the Higgs boson with precision.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

Timing-Based Search for Magnetic Monopoles with the NOvA Detector on the Surface

We report a search for a magnetic monopole component of the cosmic-ray flux in a 2743-live-day exposure of the NOvA experiment's Far Detector, a 14 kt segmented liquid scintillator detector designed primarily to observe GeV-scale electron neutrinos. No events consistent with monopoles were observed, setting an upper limit on the flux of $8\times 10^{-16}~\mathrm{cm^{-2}s^{-1}sr^{-1}}$ at 90% C.L. for monopole speed $6\times 10^{-4} < β< 5\times 10^{-3}$ and mass greater than $10^{9}$ GeV. Because of NOvA's small overburden of 3 meters-water equivalent, this constraint covers a previously unexplored low-mass region.

Abubakar, S. [Erciyes U.]↗
DOE OSTI2025

A New Measurement of the Neutron Electric Form Factor with the Super Bigbite Spectrometer Apparatus

Protons and neutrons, collectively known as nucleons, make up the nuclei at the core of atoms which form our world. The nucleon has been under intensive study for over 100 years, and yet we still do not fully understand the internal dynamics which govern properties like its spin or its mass-which contributes to almost all of the visible mass in the universe. These dynamics are governed by quantum chromodynamics(QCD), the predictions of which are experimentally tested at high energy accelerator facilities such as Jefferson Lab. TheGEN-II experiment (E12-09-016) is one such experiment. GEN-II is part of the Super Bigbite Spectrometer (SBS) experimental form factor pro gramme taking place in Hall A at Jefferson Lab, which aims to make precision measurements of the nucleon electromagnetic form factors(EMFFs)at record high values of squared four momentum transfer ¿2. EMFFs describe the electric and magnetic moment distributions within the nucleon. They can be measured through elastic electron scattering off the nucleon, and describe the recoil response of the target nucleon at a given energy scale. GEN-II is a double polarized semi-exclusive beam target asymmetry (BTA) experiment, seeking to measure the electric form factor of the neutron,¿¿ ¿,at three new values of squared four-momentum transfer¿2 =2.92,6.74and9.82GeV². The latter two points being at record high ¿2. The form factor is determined through measuring the BTA of quasielliptical scattering of a neutron from a polarized nuclear target. The experiment utilized the CEBAF accelerator to produce longitudinally polarized electrons up to ~85% polarization, which were scattered off neutrons within a novel polarized helium-3 (³He) target. This new polarized ³He target was employed by building on the technology of its precursors which existed in similar preceding experiments. This target was designed to operate at the high luminosities typical of Hall A, and reached a record breaking combination of polarization and beam intensity known as figure of merit, three times larger than those predecessors. The SBS collaboration designed and constructed two brand new high acceptance spectrometers for these experiments, an electron arm named Bigbite (BB) and a hadron arm named Super Bigbite. Both spectrometers featured a large acceptance EM dipole magnet, and complementary detector systems. The electron arm contained gaseous electronmultipliers(GEMs) which were used for high precision tracking of the scattered electrons, a heavy gas cherenkov (GRINCH) which was used for PID between electrons and pions, a plastic i ii scintillator timing hodoscope to provide high resolution timing of the start of events, and a pair of EM calorimeters (BBCal) which provided energy measurements of detected particles, and provided the experimental trigger. The hadron arm also contained a system of GEMs which will be utilized for future SBS experiments, and a hadron calorimeter designed to provide position, timing and energy measurements of the recoiling nucleon. The calibration of all detector subsystems, beam and target data is discussed, with a focus on novel timing calibrations to the hodoscope and hadron calorimeter. An analysis of selecting quasielliptical events and suppressing background contributions from a number of sources which contaminate the final event sample is given. The largest irreducible backgrounds are found to be from misidentified protons, timing accidentals and inelastic events. The physical asymmetry is measured and used to extract a value for the form factor ratio ¿¿ ¿/¿¿ ¿. High precision ¿2 data for ¿¿ ¿ is used to then extract ¿¿ ¿. This work finds at ¿2 = 2.92 GeV2 that ¿¿ ¿ = 0.0129+0.0019 -0.0020. This result is in statistical agreement with existing fits to world data, and predictions from the constituent quark model and Dyson–Schwinger equations, in this region of ¿2.

Penman, Gary [Univ. of Glasgow, Scotland (United K↗
DOE OSTI2024

Search for New Physics with the Compact Muon Solenoid Experiment and QIS-enabled Technology

Understanding the fundamental nature of dark matter (DM)---its cosmological origin, constituents, and interactions---is one of the most important questions in fundamental science today. In this thesis, I present two novel and highly complementary approaches to cover the gaps in sensitivity of current DM searches. The searches are enabled by a first-of-its-kind reconstruction technique to search for hidden-sector particles using the Compact Muon Solenoid (CMS) and by new advances in quantum sensing technology to search for axions and hidden-sector DM. In the first part of this thesis, I present a search for long-lived hidden sector particles, predicted by many extensions of the SM, using a novel technique to reconstruct decays of long-lived particles (LLPs) in the CMS muon detector. The innovative LLP reconstruction technique is sensitive to a broad range of LLP decays and to LLP masses below GeV. The search yields competitive sensitivity for proper lifetime 0.1--1000 m with the full Run 2 dataset recorded at the LHC between 2016--2018 at $\sqrt{s} = 13~$TeV. To extend the physics reach of this novel muon detector shower (MDS) signature, I present the model-independence of MDS and the reinterpretation of the search to a large number of LLP models, demonstrating its complementarity with proposed and existing dedicated LLP experiments. Finally, I present a new dedicated MDS trigger that improves the trigger efficiency by at least an order of magnitude and was deployed in 2022, at the start of Run 3 of the LHC operations. In the second part of the thesis, I present for the first time, the use of a novel quantum sensor, the low-noise and single-photon sensitive superconducting nanowire single photon detectors (SNSPDs), to directly detect dark matter. The low detection threshold and ultra-low dark count rate of SNSPDs can close the gap in DM discovery reach due to the current limitations in detector sensitivity. I will present my work on the development and characterization of SNSPDs for two entirely new experiments to directly detect axions via absorption and hidden-sector DM via electron scattering. The search for axions employs a novel broadband reflector technique with the Broadband Reflector Experiment for Axion Detection (BREAD). A unique parabolic mirror is then used to focus axion-converted photons to the SNSPDs, extending the reach to axion masses of 0.04--1 eV. On the other hand, by coupling the SNSPDs with gallium arsenide, a bright cryogenic scintillator well matched to SNSPD detection, a prototype sensing system can be built as a basis of new direct DM detection experiments capable of extending the discovery to DM masses as low as 1 MeV.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Implementation of a Time-domain Cosmic-ray-muon Tagger for the NEXUS Low-background Cryogenic Facility

Quantifying the effects of radiation on the operation of qubits both as quantum information systems as well as particle detectors has emerged as a pressing issue in quantum science in recent years. We present an overview of the design, operation, and deployment of a 90-$\mathrm{in}^2$ three-panel muon detector for use in the NEXUS experimental facility at Fermilab to temporally isolate correlated errors in qubits and determine if they possess an astrophysical origin. Constructed with three scintillator-attached PMTs read out with NIM modules in a triply-coincident logic scheme, we measure a surface-level muon luminosity of 9.7425 muons per second---consistent with an average surface-level cosmic-ray flux of approximately one muon per square centimeter per minute. Integrating the NIM modules with an MCC 128 DAQ HAT and Raspberry Pi, a Python script records exactly when a muon struck the detector and writes a timestamp to a log file for follow-up cross referencing. This experiment will broadly contribute to further studies aimed at understanding the source and mitigation of information loss in qubits.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Road to PROSPECT-II

The Precision Reactor Oscillation and SPECTrum (PROSPECT) experiment is based in a segmented liquid scintillator antineutrino detector situated approximately 7 meters from the highly enriched High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory. Its main goal is to investigate short-baseline antineutrino oscillations. The first phase of data collection, known as PROSPECT-I, was held from 2018 to 2019 and was used for several high-precision analyses, including multiple measurements of the $^{235}U$ antineutrino spectrum and searches for $eV$-scale sterile antineutrino oscillations. The collaboration is now preparing for the second phase, PROSPECT-II, which features an upgraded detector design. This advancement will enhance sensitivity and statistical power, allowing for a broader range of analyses beyond those achieved in PROSPECT-I. As we transition into this new phase, new questions have arisen concerning background simulation and its potential differences from those conducted during the initial phase of the experiment. Moreover, it is essential to ascertain, through simulations, the positive effects that an improved detector could have on the study of oscillations. This information is crucial for justifying the proposed enhancements, and I will cover all of this in the talk.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

MAIA: A new detector concept for a 10 TeV muon collider

Muon colliders offer a compelling opportunity to explore the TeV scale and conduct precision tests of the Standard Model, all within a relatively compact geographical footprint. This paper introduces a new detector concept, MAIA (Muon Accelerator Instrumented Apparatus), optimized for $\sqrt{s}=10$ TeV $\mu\mu$ collisions. The detector features an all-silicon tracker immersed in a 5T solenoid field. High-granularity silicon-tungsten and iron-scintillator calorimeters surrounding the solenoid capture high-energy electronic and hadronic showers, respectively, and support particle-flow reconstruction. The outermost subsystem comprises an air-gap muon spectrometer, which enables standalone track reconstruction for high-momentum muons. The performance of the MAIA detector is evaluated in terms of differential particle reconstruction efficiencies and resolutions. Beam-induced background (BIB) simulations generated in FLUKA are overlaid with single particle gun samples to assess detector reconstruction capabilities under realistic experimental conditions. Even with BIB, reconstruction efficiencies exceed 95% for energetic tracks, photons, and neutrons in the central region of the detector. This paper outlines promising avenues of future work, including forward region optimization and opportunities for enhanced flavor/boosted object tagging, and addresses the technological assumptions needed to achieve the desired detector performance.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Multiaxis sensing system for detection of airborne molecules and radionuclides

Various technologies presented herein relate to a method and equipment for detecting both airborne radioisotope and molecular effluent gases. Multi-Axis Sensing can be conducted by utilizing a pressurized MOF sorbent, such as a scintillating Metal-Organic Frameworks (S-MOFs). These MOFs are crystalline nanoporous materials that have synthetic versatility that allow adjustment of pore size, chemical environment, and luminescence properties. A method for detecting an analyte in a fluid sample is provided that comprises: loading a sorbent with a sample fluid, wherein the sorbent comprises a MOF material; pressurizing the sample fluid to increase the fluid in the sorbent thereby making a pressurized sorbent; and detecting ionizing radiation or a chemical property of the analyte in the pressurized sorbent.

Allendorf, Mark D.↗