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How Do A-train Sensors Intercompare in the Retrieval of Above-cloud Aerosol Optical Depth? A Case Study-based Assessment

We intercompare the above-cloud aerosol optical depth (ACAOD) of biomass burning plumes retrieved from A-train sensors, i.e., Moderate Resolution Imaging Spectroradiometer (MODIS), Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), Polarization and Directionality of Earth Reflectances (POLDER), and Ozone Monitoring Instrument (OMI). These sensors have shown independent capabilities to retrieve aerosol loading above marine boundary layer clouds-a kind of situation often found over the southeast Atlantic Ocean during dry burning season. A systematic comparison reveals that all passive sensors and CALIOP-based research methods derive comparable ACAOD with differences mostly within 0.2 over homogeneous cloud fields. The 532 nm ACAOD retrieved by CALIOP operational algorithm is underestimated. The retrieved 1064 nm AOD however shows closer agreement with passive sensors. Given the different types of measurements processed with different algorithms, the reported close agreement between them is encouraging. Due to unavailability of direct measurements above cloud, the validation of satellite-based ACAOD remains an open challenge. The intersatellite comparison however can be useful for the relative evaluation and consistency check

Aerosol↗

New Approach to Monitor Transboundary Particulate Pollution over Northeast Asia

A new approach to more accurately monitor and evaluate transboundary particulate matter (PM) pollution is introduced based on aerosol optical products from Korea's Geostationary Ocean Color Imager (GOCI). The area studied is Northeast Asia (including eastern parts of China, the Korean peninsula and Japan), where GOCI has been monitoring since June 2010. The hourly multi-spectral aerosol optical data that were retrieved from GOCI sensor onboard geostationary satellite COMS (Communication, Ocean, and Meteorology Satellite) through the Yonsei aerosol retrieval algorithm were first presented and used in this study. The GOCI-retrieved aerosol optical data are integrated with estimated aerosol distributions from US EPA Models-3/CMAQ (Community Multi-scale Air Quality) v4.5.1 model simulations via data assimilation technique, thereby making the aerosol data spatially continuous and available even for cloud contamination cells. The assimilated aerosol optical data are utilized to provide quantitative estimates of transboundary PM pollution from China to the Korean peninsula and Japan. For the period of 1 April to 31 May, 2011 this analysis yields estimates that AOD as a proxy for PM2.5 or PM10 during long-range transport events increased by 117-265% compared to background average AOD (aerosol optical depth) at the four AERONET sites in Korea, and average AOD increases of 121% were found when averaged over the entire Korean peninsula. This paper demonstrates that the use of multi-spectral AOD retrievals from geostationary satellites can improve estimates of transboundary PM pollution. Such data will become more widely available later this decade when new sensors such as the GEMS (Geostationary Environment Monitoring Spectrometer) and GOCI-2 are scheduled to be launched.

Data Assimilation↗

TPSAS-NF1676L-34796-DND

The recently completed 2015-2017 EVS-2 mission NAAMES (The North Atlantic Aerosols and Marine Ecosystems Study) provides a unique set of airborne remote sensing and ship-based in situ measurements in a remote and under-sampled region of the Earth?s ocean. The NASA SABOR (Ship-Aircraft Bio-Optical Research) campaign was conducted during the summer of 2014, also in the Atlantic Ocean, out of the Chesapeake Bay and in the eastern coastal region of the United States. For both campaigns, the NASA GISS Research Scanning Polarimeter, a multi-angle, multi-spectral polarimeter measured the upwelling polarized radiances from aircraft. And for both campaigns, ship-based in situ measurements of the ocean were collected jointly with the aircraft measurements. We present results from the new RSP-MAPP (1) that is based on optimal estimation and that can retrieve simultaneous aerosol microphysical properties (including effective radius, single-scattering albedo, and real refractive index) and ocean color products using accurate radiative transfer, Mie calculations, and the DP (Detritus Plankton) series of accurate, numerically efficient ocean bio-optical models. The RSP-MAPP algorithm was applied to data collected during SABOR and NAAMES to retrieve aerosol microphysics and ocean products for all Aerosols-Above-Ocean (AAO) scenes. The RSP-MAPP products are compared against i) collocated aerosol extinction and backscatter profiles collected by the NASA LaRC airborne High Spectral Resolution Lidar (HSRL-1), including lidar depth profiles of the ocean diffuse attenuation coefficient and the hemispherical backscatter coefficient, and ii) collocated ship-based in situ measurements of the ocean.

Snorre Stamnes↗

Spaceborne lidar measurement accuracy - Simulation of aerosol, cloud, molecular density, and temperature retrievals

In connection with studies concerning the use of an orbiting optical radar (lidar) to conduct aerosol and cloud measurements, attention has been given to the accuracy with which lidar return signals could be measured. However, signal-measurement error is not the only source of error which can affect the accuracy of the derived information. Other error sources are the assumed molecular-density and atmospheric-transmission profiles, and the lidar calibration factor (which relates signal to backscatter coefficient). The present investigation has the objective to account for the effects of all these errors sources for several realistic combinations of lidar parameters, model atmospheres, and background lighting conditions. In addition, a procedure is tested and developed for measuring density and temperature profiles with the lidar, and for using the lidar-derived density profiles to improve aerosol retrievals.

Russell, P. B.↗

Principles in Remote Sensing of Aerosol from MODIS Over Land and Ocean

The well-calibrated spectral radiances measured by MODIS will be processed to retrieve daily aerosol properties that include optical thickness and mass loading over land and optical thickness, the mean particle size of the dominant mode and the ratio between aerosol modes over ocean. In addition, after launch, aerosol single scattering albedo will be calculated as an experimental product. The retrieval process over land is based on a dark target method that identifies appropriate targets in the mid-IR channels and uses an empirical relationship found between the mid-ER and the visible channels to estimate surface reflectance in the visible from the mid-HZ reflectance measured by satellite. The method employs new aerosol models for industrial, smoke and dust aerosol. The process for retrieving aerosol over the ocean makes use of the wide spectral band from 0.55-2.13 microns and a look-up table constructed from combinations of five accumulation modes and five coarse modes. Both the over land and over ocean algorithms have been validated with satellite and airborne radiance measurements. We estimate that MODIS will be able to measure aerosol optical thickness (t) to within 0.05 +/- 0.2t over land and to within 0.05 +/- 0.05t over ocean. Much of the earth's surface is located far from aerosol sources and experience very low aerosol optical thickness. Will the accuracy expected from MODIS retrievals be sufficient to measure the global aerosol direct and indirect forcing? We are attempting to answer this question using global model results and cloud climatology.

Remer, L. A.↗

Particle Shape, Size, and Composition from Satellites

The MISR Research Aerosol (RA) retrieval algorithm produces (A) aerosol amount (optical depth – AOD), (B) an aerosol size constraint (Angstrom Exponent) (C) fraction of non-spherical particles, and (D) particle light-absorption (SSA). Near the Camp fire source region the particles tend to be large (low Angstrom Exponent) and non-spherical particles, probably from burning in the town of Paradise. Aerosols are smaller and more spherical downwind, probably as the plume mixes with smoke from burning forest.

aerosol↗

Sensor Calibration Impacts on Dust Detection Based On MODIS And VIIRS Thermal Emissive Bands

Dust detection using remotely sensed measurements has been one of the challenging problems encountered by atmospheric scientists. MODerate Resolution Imaging Spectroradiometer (MODIS) on the Terra (T)and Aqua (A) platforms have been a versatile sensor for well over 21 and 18 years respectively and have been extremely useful in the retrieval of aerosol information over the entire globe. The MODIS radiances from the Level1B in general are expected to be within 5% accuracy in the reflective wavelengths and within 1% in the thermal emissive wavelengths. In this paper, we evaluate the sensitivity of previously developed dust detection technique based on thermal emissive wavelengths, which correspond to MODIS bands 20, 29, 31, and 32 respectively. The Thermal Emissive Dust Index (TEDI) performed very comparably to the traditional Aerosol Optical Thickness (AOT) retrievals by MODIS reflective channels. Since the MODIS Thermal Emissive Bands (TEB) are well calibrated on-orbit using a BlackBody (BB) source, the calibration of these long wave infrared bands is quite robust. As A-MODIS continues to perform well beyond its designed lifetime of 6 years, the instrument has undergone various levels of degradation during its mission time. As a consequence, it is imperative to check the impacts of calibration on the higher-level retrievals. In this paper, we rigorously analyze the sensitivity of TEDI due to the impact of calibration by the afore-mentioned TEB. The perturbation of the dominant (linear) calibration term demonstrated the following: first, there was a correlation in the sensitivity of the TEDI due to the uncertainty in the linear calibration term. Based on a perturbation in the linear calibration term for all aforementioned bands over a range of ± 5 % yielded the TEDI sensitivity to vary from approximately -3.2 % to about -3.6 %. When considering the uncertainty in each individual band significant changes were observed. The least change was observed for the perturbation in the calibration of band 20 with the TEDI sensitivity and the largest sensitivity in TEDI was observed in the perturbation of band 31 calibration. Thus, in the case of TEDI, noticeable sensitivity due to calibration uncertainty was observed in bands 29, 31, and 32, reiterating the importance of the TEB calibration in these bands. Also, the dust detection scheme based on A-MODIS was successfully transferred to the follow-on sensors such as Suomi (SNPP) and NOAA 20 (N20) VIIRS. The results presented in this paper would be extremely helpful in understanding impacts of calibration on the higher-level products for both current and future missions based on the MODIS heritage. Finally, the work also identifies the importance of radiometric fidelity in maintaining the accuracy of the dust detection. Results presented will show drastic improvement of the Saharan dust detection after the reduction of the electronic crosstalk in the 8.5 μm channel of T-MODIS.

Sriharsha Madhavan↗

Extending XBAER Algorithm to Aerosol and Cloud Condition

The retrieval of cloud optical properties for aerosol contaminated water cloud is challenging because of the complexity of physical processes in such situations. Conventionally, cloud optical data products are typically derived, ignoring the aerosol impacts on radiative transfer in the retrieval process. This is potentially a significant source of error. In this paper, the eXtensible Bremen Aerosol Retrieval (XBAER) algorithm has been optimized for the retrieval of aerosol/cloud properties for the aerosol contaminated cloud (ACC) scenarios. This version of XBAER delivers cloud optical thickness (COT) and cloud effective radius (CER) for ACCs and simultaneously retrieves aerosol optical thickness (AOT). The surface parameterization and aerosol types used in the standard XBAER algorithm have been adapted in this retrieval to account for the ACC conditions. Aerosol types in XBAER for the retrieval of ACC scenarios have been parameterized to comprise weak and strong absorptions. The comparisons of COT, CER, and AOT retrieved using this adapted XBAER algorithm and two new NASA algorithms show good agreements, especially for biomass burning aerosol. The correlation coefficients are >0.9 for AOT, ~0.8 for CER, and ~0.7 for COT. There is also a good agreement for dust plume contaminated cloud scene. The XBAER derived AOT values for dust aerosols are systematically smaller than the NASA retrieval, but both products have the same spatial distribution patterns. The comparison of COT retrieved using the adapted XBAER algorithm and that retrieved from ground-based microwave radiometer (MWR) measurements shows much better agreement for ACC conditions with high AOT.

satellite↗

AERONET Remotely Sensed Measurements and Retrievals of Biomass Burning Aerosol Optical Properties During the 2015 Indonesian Burning Season

An extreme biomass-burning event occurred in Indonesia from September through October 2015 due to severe drought conditions, partially caused by a major El Nino event, thereby allowing for significant burning of peatland that had been previously drained. This event had the highest sustained aerosol optical depths (AOD) ever monitored by the global Aerosol Robotic Network (AERONET). The newly developed AERONET Version 3 algorithms retain high AOD at the longer wavelengths when associated with high Angstrom Exponents (AEs), which thereby allowed for measurements of AOD at 675 nanometers as high as approximately 7, the upper limit of Sun photometry. Measured AEs at the highest monitored AOD levels were subsequently utilized to estimate instantaneous values of AOD at 550 nanometers in the range of 11 to 13, well beyond the upper measurement limit. Additionally, retrievals of complex refractive indices, size distributions, and single scattering albedos (SSA) were obtained at much higher AOD levels than possible from almucantar scans due to the ability to perform retrievals at smaller solar zenith angles with new hybrid sky radiance scans. For retrievals made at the highest AOD levels the fine mode volume median radii were approximately 0.25 to 0.30 microns, which are very large particles for biomass burning. Very high SSA values (approximately 0.975 from 440 to 1020 nanometers) are consistent with the domination by smoldering combustion of peat burning. Estimates of the percentage peat contribution to total biomass burning aerosol based on retrieved SSA and laboratory measured peat SSA were approximately 80-85 percent, in excellent agreement with independent estimates.

Eck, T. F.↗

Accuracy Assessment of Aqua-MODIS Aerosol Optical Depth Over Coastal Regions: Importance of Quality Flag and Sea Surface Wind Speed

Coastal regions around the globe are a major source for anthropogenic aerosols in the atmosphere, but the underlying surface characteristics are not favorable for the Moderate Resolution Imaging Spectroradiometer (MODIS) algorithms designed for retrieval of aerosols over dark land or open-ocean surfaces. Using data collected from 62 coastal stations worldwide from the Aerosol Robotic Network (AERONET) from approximately 2002-2010, accuracy assessments are made for coastal aerosol optical depth (AOD) retrieved from MODIS aboard Aqua satellite. It is found that coastal AODs (at 550 nm) characterized respectively by the MODIS Dark Land (hereafter Land) surface algorithm, the Open-Ocean (hereafter Ocean) algorithm, and AERONET all exhibit a log-normal distribution. After filtering by quality flags, the MODIS AODs respectively retrieved from the Land and Ocean algorithms are highly correlated with AERONET (with R(sup 2) is approximately equal to 0.8), but only the Land algorithm AODs fall within the expected error envelope greater than 66% of the time. Furthermore, the MODIS AODs from the Land algorithm, Ocean algorithm, and combined Land and Ocean product show statistically significant discrepancies from their respective counterparts from AERONET in terms of mean, probability density function, and cumulative density function, which suggest a need for future improvement in retrieval algorithms. Without filtering with quality flag, the MODIS Land and Ocean AOD dataset can be degraded by 30-50% in terms of mean bias. Overall, the MODIS Ocean algorithm overestimates the AERONET coastal AOD by 0.021 for AOD less than 0.25 and underestimates it by 0.029 for AOD greater than 0.25. This dichotomy is shown to be related to the ocean surface wind speed and cloud contamination effects on the satellite aerosol retrieval. The Modern Era Retrospective-Analysis for Research and Applications (MERRA) reveals that wind speeds over the global coastal region 25 (with a mean and median value of 2.94 meters per second and 2.66 meters per second, respectively) are often slower than 6 meters per second assumed in the MODIS Ocean algorithm. As a result of high correlation (R(sup 2) greater than 0.98) between the bias in binned MODIS AOD and the corresponding binned wind speed over the coastal sea surface, an empirical scheme for correcting the bias of AOD retrieved from the MODIS Ocean algorithm is formulated and is shown to be effective over the majority of the coastal AERONET stations, and hence can be used in future analysis of AOD trend and MODIS AOD data assimilation.

Anderson, J. C.↗

Validation of the aerosol optical property products derived by the GRASP/Component approach from multi-angular polarimetric observations

The multi-angle polarimetric satellite observations are helpful for improving the retrievals of aerosol parameters. However, practical applications of polarization technology are still limited because of complexity of measurement and interpretation of polarimetric observations. In this study, we analyze the performance of a new component approach developed in the frame of the Generalized Retrieval of Atmosphere and Surface Properties (GRASP) algorithm. In addition to aerosol optical properties including particle size distribution, non-sphericity and index of refraction that are commonly derived from multi-angle radiance and polarization measurements, the GRASP/Component approach also provides some information about aerosol composition. Specifically, in this approach aerosol is modeled as an internal mixture of several components with distinctly different chemical compositions and known refractive indices. The approach is intended not only to provide additional insight on aerosol composition but also to improve retrieval of basic aerosol optical properties. This study presents comprehensive validation and evaluation of Aerosol Optical Depth (AOD), Ångstrom exponent (AE), fine mode AOD (AODF), coarse mode AOD (AODC), and single scattering albedo (SSA) as retrieved by the GRASP/Component approach. The GRASP/Component products include aerosol retrievals using two different aerosol component mixing rules, i.e., Maxwell-Garnett (MG) effective medium approximation and a simple Volume- Weighted averaging (VW). The differences between the results obtained using these two assumptions are also discussed. The obtained results show that the aerosol optical property products of GRASP/Component approach have good agreement with the ground-based AERONET measurements, which is comparable to other PARASOL/ GRASP approaches. Specifically, the AOD retrieved by GRASP/Component approach show high correlation and nearly no bias both over land and ocean, as compared with AERONET. The more detailed aerosol properties such as AE, AODF, AODC and SSA also show one of the best comparisons with AERONET. These improvements can probably be attributed to the use of the additional physical constraints on spectral dependence of the complex refractive index and the reduction of total number of aerosol parameters directly retrieved in the GRASP/Component approach. In addition, the choice of mixing rules had no significant effect on optical retrievals. With the exception of SSA, the results obtained based on the MG mixing rule were found to be slightly better over those obtained using VW mixing rule, especially for bias.

Brent N Holben↗

Advanced Characterisation of Aerosol Size Properties from Measurements of Spectral Optical Depth Using the GRASP Algorithm

This study evaluates the potential of using aerosol optical depth (τ (sub a)) measurements to characterise the microphysical and optical properties of atmospheric aerosols. With this aim, we used the recently developed GRASP (Generalized Retrieval of Aerosol and Surface Properties) code for numerical testing of six different aerosol models with different aerosol loads. The direct numerical simulations (self-consistency tests) indicate that the GRASP-AOD retrieval provides modal aerosol optical depths (fine and coarse) to within 0.01 of the input values. The retrieval of the fine-mode radius, width and volume concentration are stable and precise if the real part of the refractive index is known. The coarse-mode properties are less accurate, but they are significantly improved when additional a priori information is available. The tests with random simulated errors show that the uncertainty in the bimodal log-normal size distribution parameters increases as the aerosol load decreases. Similarly, the reduction in the spectral range diminishes the stability of the retrieved parameters. In addition to these numerical studies, we used optical depth observations at eight AERONET locations to validate our results with the standard AERONET inversion products. We found that bimodal log-normal size distributions serve as useful input assumptions, especially when the measurements have inadequate spectral coverage and/or limited accuracy, such as moon photometry. Comparisons of the mode median radii between GRASP-AOD and AERONET indicate average differences of 0.013µm for the fine mode and typical values of 0.2–0.3µm for the coarse mode. The dominant mode (i.e. fine or coarse) indicates a 10 % difference in mode radii between the GRASP-AOD and AERONET inversions, and the average of the difference in volume concentration is around 17 % for both modes. The retrieved values of the fine-mode τ(sub a)(500) using GRASP-AOD are generally between those values obtained by the standard AERONET inversion and the values obtained by the AERONET spectral deconvolution algorithm (SDA), with differences typically lower than 0.02 between GRASP-AOD and both algorithms. Finally, we present some examples of application of GRASP-AOD inversion using moon photometry and the airborne PLASMA sun photometer during the ChArMEx summer 2013 campaign in the western Mediterranean.

Torres, Benjamin↗

Evidence of a Weakly Absorbing Intermediate Mode of Aerosols in AERONET Data from Saharan and Sahelian Sites

Accurate retrievals of aerosol size distribution are necessary to estimate aerosols' impact on climate and human health. The inversions of the Aerosol Robotic Network (AERONET) usually retrieve bimodal distributions. However, when the inversion is applied to Saharan and Sahelian dust, an additional mode of intermediate size between the coarse and fine modes is sometimes seen. This mode explains peculiarities in the behavior of the Angstrom exponent, along with the fine mode fraction retrieved using the spectral deconvolution algorithm, observed in a March 2006 dust storm. For this study, 15 AERONET sites in northern Africa and on the Atlantic are examined to determine the frequency and properties of the intermediate mode. The mode is observed most frequently at Ilorin in Nigeria. It is also observed at Capo Verde and multiple sites located within the Sahel but much less frequently at sites in the northern Sahara and the Canary Islands. The presence of the intermediate mode coincides with increases in Angstrom exponent, fine mode fraction, single-scattering albedo, and to a lesser extent percent sphericity. The Angstrom exponent decreases with increasing optical depth at most sites when the intermediate mode is present, but the fine mode fraction does not. Single-scattering albedo does not steadily decrease with fine mode fraction when the intermediate mode is present, as it does in typical mixtures of dust and biomass-burning aerosols. Continued investigation is needed to further define the intermediate mode's properties, determine why it differs from most Saharan dust, and identify its climate and health effects.

inversions↗

On Improving the Dust Lidar Ratios for Version 5 of CALIOP by Using Measurements with Source-tagged Model Results

Vertically resolved retrievals of aerosol backscatter and extinction have been available since 2006 from global measurements acquired by the space borne lidar CALIOP onboard the CALIPSO satellite. These retrievals depend crucially upon the ratio of extinction to backscatter (i.e., lidar ratio) which typically has to be assumed for the various aerosol species for an elastic backscatter lidar like CALIOP. For all CALIPSO data releases up until now (version 4.2), these lidar ratios have been taken as constant both spatially and temporally. However, it is well established that the aerosol lidar ratios can vary significantly regionally, seasonally, and also as a function of age and relative humidity. In particular, the dust lidar ratios show significant variation depending upon their source regions, which is related to the mineral composition of dust in that region. In this paper, we shall present a scheme to obtain the regionally and seasonally dependent lidar ratios of dust. In this scheme, which may be implemented in a forthcoming version of CALIOP aerosol extinction retrievals, we first derive lidar ratios of aerosol layers globally, classified as dust by CALIOP, by using the backscatter measurements constrained by collocated MODIS aerosol optical depths. Since this dust will frequently be a mixture of dust from various source regions, we obtain the corresponding regional contributions from the dust simulations using the GEOS model tagged to nine source regions. Finally, combining information from both measurements and models, we obtain the lidar ratios of dust corresponding to the nine source regions. The lidar ratio of the mixed dust anywhere can now be obtained from the tagged model fractions and the corresponding regional lidar ratio. We shall show the application of this scheme for various regions and seasons.

CALIPSO↗

An Airborne A-Band Spectrometer for Remote Sensing Of Aerosol and Cloud Optical Properties

Atmospheric remote sensing with the O2 A-band has a relatively long history, but most of these studies were attempting to estimate surface pressure or cloud-top pressure. Recent conceptual studies have demonstrated the potential of spaceborne high spectral resolution O2 A-band spectrometers for retrieval of aerosol and cloud optical properties. The physical rationale of this new approach is that information on the scattering properties of the atmosphere is embedded in the detailed line structure of the O2 A-band reflected radiance spectrum. The key to extracting this information is to measure the radiance spectrum at very high spectral resolution. Instrument performance requirement studies indicate that, in addition to high spectral resolution, the successful retrieval of aerosol and cloud properties from A-band radiance spectra will also require high radiometric accuracy, instrument stability, and high signal-to-noise measurements. To experimentally assess the capabilities of this promising new remote sensing application, the NASA Langley Research Center is developing an airborne high spectral resolution A-band spectrometer. The spectrometer uses a plane holographic grating with a folded Littrow geometry to achieve high spectral resolution (0.5 cm-1) and low stray light in a compact package. This instrument will be flown in a series of field campaigns beginning in 2001 to evaluate the overall feasibility of this new technique. Results from these campaigns should be particularly valuable for future spaceborne applications of A-band spectrometers for aerosol and cloud retrievals.

Pitts, Michael↗

Effect of Tropospheric Aerosols in Satellite-Based Trace Gas Retrieval

Scattering and absorption by tropospheric aerosol particles have an effect on the airmass factor (AMF), a fundamental quantity for trace gas concentration retrieval by inversion of satellite measurements. The interference effect depends on the aerosols micro-physical and optical properties as well as the relative distribution of the tropospheric trace gas and aerosol load. Quantifying the aerosol impact on trace gas retrieval requires a sensitivity study using radiative transfer calculations. In this presentation we will describe a recently initiated effort to characterize the aerosol-related error in trace gas retrievals when the presence of aerosol particles is not accounted in the inversion procedure. A general description of the project will be presented and preliminary results on aerosol effects on SO2 retrieved concentrations will be discussed.

Krotkov, Nickolay↗

Aerosol Optical Depths over Oceans: a View from MISR Retrievals and Collocated MAN and AERONET in Situ Observations

In this study, aerosol optical depths over oceans are analyzed from satellite and surface perspectives. Multiangle Imaging SpectroRadiometer (MISR) aerosol retrievals are investigated and validated primarily against Maritime Aerosol Network (MAN) observations. Furthermore, AErosol RObotic NETwork (AERONET) data from 19 island and coastal sites is incorporated in this study. The 270 MISRMAN comparison points scattered across all oceans were identified. MISR on average overestimates aerosol optical depths (AODs) by 0.04 as compared to MAN; the correlation coefficient and root-mean-square error are 0.95 and 0.06, respectively. A new screening procedure based on retrieval region characterization is proposed, which is capable of substantially reducing MISR retrieval biases. Over 1000 additional MISRAERONET comparison points are added to the analysis to confirm the validity of the method. The bias reduction is effective within all AOD ranges. Setting a clear flag fraction threshold to 0.6 reduces the bias to below 0.02, which is close to a typical ground-based measurement uncertainty. Twelve years of MISR data are analyzed with the new screening procedure. The average over ocean AOD is reduced by 0.03, from 0.15 to 0.12. The largest AOD decrease is observed in high latitudes of both hemispheres, regions with climatologically high cloud cover. It is postulated that the screening procedure eliminates spurious retrieval errors associated with cloud contamination and cloud adjacency effects. The proposed filtering method can be used for validating aerosol and chemical transport models.

AERONET↗

Validation of Long-Term Global Aerosol Climatology Project Optical Thickness Retrievals Using AERONET and MODIS Data

A comprehensive set of monthly mean aerosol optical thickness (AOT) data from coastal and island AErosol RObotic NETwork (AERONET) stations is used to evaluate Global Aerosol Climatology Project (GACP) retrievals for the period 1995-2009 during which contemporaneous GACP and AERONET data were available. To put the GACP performance in broader perspective, we also compare AERONET and MODerate resolution Imaging Spectroradiometer (MODIS) Aqua level-2 data for 2003-2009 using the same methodology. We find that a large mismatch in geographic coverage exists between the satellite and ground-based datasets, with very limited AERONET coverage of open-ocean areas. This is especially true of GACP because of the smaller number of AERONET stations at the early stages of the network development. Monthly mean AOTs from the two over-the-ocean satellite datasets are well-correlated with the ground-based values, the correlation coefficients being 0.81-0.85 for GACP and 0.74-0.79 for MODIS. Regression analyses demonstrate that the GACP mean AOTs are approximately 17%-27% lower than the AERONET values on average, while the MODIS mean AOTs are 5%-25% higher. The regression coefficients are highly dependent on the weighting assumptions (e.g., on the measure of aerosol variability) as well as on the set of AERONET stations used for comparison. Comparison of over-the-land and over-the-ocean MODIS monthly mean AOTs in the vicinity of coastal AERONET stations reveals a significant bias. This may indicate that aerosol amounts in coastal locations can differ significantly from those in adjacent open-ocean areas. Furthermore, the color of coastal waters and peculiarities of coastline meteorological conditions may introduce biases in the GACP AOT retrievals. We conclude that the GACP and MODIS over-the-ocean retrieval algorithms show similar ranges of discrepancy when compared to available coastal and island AERONET stations. The factors mentioned above may limit the performance of the validation procedure and cause us to caution against a direct extrapolation of the presented validation results to the entirety of the GACP dataset.

MODIS (radiometry)↗