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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 433 records · Page 24
All sourcesNASA NTRSDOE OSTI
NASA NTRS1994

Radio occultation studies of the Venus atmosphere with the Magellan spacecraft. 2: Results from the October 1991 experiments

On October 5 and 6, 1991, three dual-frequency ingress radio occultation experiments were conducted at Venus during consecutive orbits of the Magellan spacecraft. The radio signals probed a region of the atmosphere near 65 deg N, with a solar zenith angle of 108 deg, reaching below 35 km at 3.6 cm, and below 34 km at 13 cm (above a mean radius of 6052 km). The high effective isotropic radiated power (EIRP) of the Magellan spacecraft and highly successful attitude maneuvers allowed these signals to probe deeper than any previous radio occultation experiment and also resulted in the most accurate thermal and sulfuric acid vapor abundance profiles ever obtained at Venus through radio occultation techniques. The performance of the spacecraft and the experiment design are discussed in an accompanying paper. Average electron density profiles retrieved from the data possess peaks between 2600 and 6000/cu cm, well below typical values of 10,000/cu cm retrieved in 1979 by Pioneer Venus at similar solar zenith angles. Other basic results include vertical profiles of temperature, pressure, and density in the neutral atmosphere, 13- and 3.6-cm absorpttivity, and H2SO4 (g) abundance below the main cloud layer. H2SO4 (g) becomes significant below 50 km, reaching peaks between 18 and 24 ppm near 39 km before dropping precipitously below 38 km. These sharp decreases confirm the thermal decomposition of sulfuric acid vapor below 39 km. Since the Venus atmosphere rotated approximately 10 deg between experiments, the data contain information about the horizontal variability of the atmosphere. All derived profiles exhibit significant variations from orbit to orbit, indicating the presence of dynamical processes between 33 and 200 km. In particular, the orbit-to-orbit variations in temperature and in H2SO4 (g) abundance appear to be correlated, suggesting that a common mechanism may be responsible for the observed spatial variations.

Jenkins, Jon M.↗
NASA NTRS2012

The Distribution of Snow Black Carbon observed in the Arctic and Compared to the GISS-PUCCINI Model

In this study, we evaluate the ability of the latest NASA GISS composition-climate model, GISS-E2- PUCCINI, to simulate the spatial distribution of snow BC (sBC) in the Arctic relative to present-day observations. Radiative forcing due to BC deposition onto Arctic snow and sea ice is also estimated. Two sets of model simulations are analyzed, where meteorology is linearly relaxed towards National Centers for Environmental Prediction (NCEP) and towards NASA Modern Era Reanalysis for Research and Applications (MERRA) reanalyses. Results indicate that the modeled concentrations of sBC are comparable with presentday observations in and around the Arctic Ocean, except for apparent underestimation at a few sites in the Russian Arctic. That said, the model has some biases in its simulated spatial distribution of BC deposition to the Arctic. The simulations from the two model runs are roughly equal, indicating that discrepancies between model and observations come from other sources. Underestimation of biomass burning emissions in Northern Eurasia may be the main cause of the low biases in the Russian Arctic. Comparisons of modeled aerosol BC (aBC) with long-term surface observations at Barrow, Alert, Zeppelin and Nord stations show significant underestimation in winter and spring concentrations in the Arctic (most significant in Alaska), although the simulated seasonality of aBC has been greatly improved relative to earlier model versions. This is consistent with simulated biases in vertical profiles of aBC, with underestimation in the lower and middle troposphere but overestimation in the upper troposphere and lower stratosphere, suggesting that the wet removal processes in the current model may be too weak or that vertical transport is too rapid, although the simulated BC lifetime seems reasonable. The combination of observations and modeling provides a comprehensive distribution of sBC over the Arctic. On the basis of this distribution, we estimate the decrease in snow and sea ice albedo and the resulting radiative forcing. We suggest that the albedo reduction due to BC deposition presents significant space-time variations, with highest mean reductions of 1.25% in the Russian Arctic, which are much larger than those in other Arctic regions (0.39% to 0.64 %). The averaged value over the Arctic north of 66degN is 0.4-0.6% during spring, leading to regional surface radiative forcings of 0.7, 1.1 and 1.0Wm(exp−2) in spring 2007, 2008 and 2009, respectively.

Dou, T.↗
NASA NTRS1992

Surface forcing of the infrared cooling profile over the Tibetan Plateau. I - Influence of relative longwave radiative heating at high altitude. II - Cooling-rate variation over large-scale plateau domain during summer monsoon transition

The role of the Tibetan Plateau on the behavior of the surface longwave radiation budget is investigated, and the behavior of the vertical profile of longwave cooling over the plateau, including its diurnal variation, is quantified. A medium spectral-resolution IR radiative transfer model utilizing a simple modification for applications in idealized complex (valley) terrain is developed for the investigation. An understanding of how surface and elevation biophysical factors, which are highly variable over the large-scale plateau domain, regulate the spatial distribution of clear-sky IR cooling during the transition phase of the summer monsoon, is described.

Smith, Eric A.↗
NASA NTRS1999

Nitrogen Species in the Post-Pinatubo Stratosphere: Model Analysis Utilizing UARS Measurements

We present an analysis of the impact of heterogeneous chemistry on the partitioning of nitrogen species measured by the Upper Atmosphere Research Satellite (UARS) instruments. The UARS measurements utilized include N2O, HNO3, and ClONO2 from the cryogenic limb array etalon spectrometer (CLAES), version 7 (v.7), and temperature, methane, ozone, H2O, HCl, NO and NO2 from the halogen occultation experiment (HALOE), version 18. The analysis is carried out for the UARS data obtained between January 1992 and September 1994 in the 100-to 1-mbar (approx. 17-47 km) altitude range and over 10 degrees latitude bins from 70 S to 70 N. The spatiotemporal evolution of aerosol surface area density (SAD) is adopted from analysis of the Stratospheric Aerosol and Gas Experiment (SAGE) II data. A diurnal steady state photochemical box model, constrained by the temperature, ozone, H2O, CH4, aerosol SAD, and columns of O2 and O3 above the point of interest, has been used as the main tool to analyze these data. Total inorganic nitrogen (NOy) is obtained by three different methods: (1) as a sum of the UARS-measured NO, NO2, HNO3, and ClONO2; (2) from the N2O-NOy correlation, and (3) from the CH4-NOy correlation. To validate our current understanding of stratospheric heterogeneous chemistry for post-Pinatubo conditions, the model-calculated monthly averaged NOx/NOy ratios and the NO, NO2, and HNO3 profiles are compared with the UARS-derived data. In general, the UARS-constrained box model captures the main features of nitrogen species partitioning in the post-Pinatubo years, such as recovery of NOx after the eruption, their seasonal variability and vertical profiles. However, the model underestimates the NO2 content, particularly in the 30- to 7-mbar (approx.23-32 km) range. Comparisons of the calculated temporal behavior of the partial columns of NO2 and HNO3 and ground-based measurements at 45 S and 45 N are also presented. Our analysis indicates that ground-based and HALOE v.18 measurements of the NO2 vertical columns are consistent within the range of their uncertainties and are systematically higher (up to 50%) than the model results at midlatitudes in both hemispheres. Reasonable agreement is obtained for HNO3 columns at 45 S, suggesting some problems with nitrogen species partitioning in the model. Outstanding uncertainties are discussed.

Danilin, Michael Y.↗
NASA NTRS1990

Measurements of CH4, N2O, CO, H2O, and O3 in the middle atmosphere by the Atmospheric Trace Molecule Spectroscopy Experiment on Spacelab 3

The volume mixing ratios of five minor gases (CH4, N2O, CO, H2O, and O3) have been retrieved through the middle atmosphere from the analysis of 0.01/cm resolution infrared solar occultation spectra recorded near 28 deg N and 48 deg S latitudes with the Atmospheric Trace Molecule Spectroscopy instrument, flow on board Spacelab 3 (April 30 through May 6, 1985). The results are in general agreement with reported measurements from ground-, balloon-, and satellite-based instruments for the same seasons. In detail, the vertical profiles of these gases show the effects of the upper and middle atmospheric transport patterns dominant during the season of these observations. The profiles inferred at different longitudes around 28 deg N suggest a near-uniform zonal distribution of these gases, for conditions corresponding to late spring. The sunrise occultation measurements point to a larger longitudinal variability in the vertical distribution of these gases at 48 deg S.

Gunson, M. R.↗
NASA NTRS1985

Nitric oxide profile from 7 to 32 km

An analysis is given of some results of the LIMS experiment, launched on the Nimbus 7 satellite on October 24, 1978 for the purpose of sounding the middle atmosphere composition and structure. One of the LIMS channels was centered spectrally in the 6 micron region to measure vertical profiles and the global distribution of NO2 mixing ratio. The data reveal that NO2 is highly variable with altitude, latitude, longitude and time. Steep latitudinal gradients are observed in high latitude winter ('the NO2 cliff') when a wave number one pattern exists in the geopotential height field. The daytime gradient under these conditions is less than that for the night. The summer hemisphere column amount is considerably greater (by a factor of about 2) than in the winter hemisphere. The largest mixing ratios occur at 4 mb at night (about 20 ppbv) and 9 mb in the day (about 7 ppbv) and the latitude region of the peak mixing ratio is skewed toward the Southern Hemisphere. The mixing ratio variability is greater at night (by a factor of about 2 to 3) than in the day and there are significant long-term changes revealed by mixing ratio time series analyses on a pressure vs time grid.

Matthews, W. A.↗
NASA NTRS1999

Nitrogen Species in the Post-Pinatubo Stratosphere: Model Analysis Utilizing UARS Measurements

We present an analysis of the impact of heterogeneous chemistry on the partitioning of nitrogen species measured by the Upper Atmosphere Research Satellite (UARS) instruments. The UARS measurements utilized include N2O, HNO3, and ClONO2 from the cryogenic limb array etalon spectrometer (CLAES), version 7 (v.7), and temperature, methane, ozone, H2O, HCl, NO and NO2 from the halogen occultation experiment (HALOE), version 18. The analysis is carried out for the UARS data obtained between January 1992 and September 1994 in the 100- to 1-mbar (approx. 17-47 km) altitude range and over 10 deg latitude bins from 70 deg S to 70 deg N. The spatiotemporal evolution of aerosol surface area density (SAD) is adopted from analysis of the Stratospheric Aerosol and Gas Experiment (SAGE) II data. A diurnal steady state photochemical box model, constrained by the temperature, ozone, H2O, CH4, aerosol SAD, and columns of O2 and O3 above the point of interest, has been used as the main tool to analyze these data. Total inorganic nitrogen (NOY) is obtained by three different methods: (1) as a sum of the UARS-measured NO, NO2, HNO3, and ClONO2; (2) from the N2O-NOY correlation; and (3) from the CH4-NOY correlation. To validate our current understanding of stratospheric heterogeneous chemistry for post-Pinatubo conditions, the model-calculated monthly averaged NO(x)/NO(y) ratios and the NO, NO2, and HNO3 profiles are compared with the UARS-derived data. In general, the UARS-constrained box model captures the main features of nitrogen species partitioning in the post-Pinatubo years, such as recovery of NO(x) after the eruption, their seasonal variability and vertical profiles. However, the model underestimates the NO2 content, particularly in the 30- to 7-mbar (approx. 23-32 km) range. Comparisons of the calculated temporal behavior of the partial columns of NO2 and HNO3 and ground-based measurements at 45 deg S and 45 deg N are also presented. Our analysis indicates that ground-based and HALOE v.18 measurements of the NO2 vertical columns are consistent within the range of their uncertainties and are systematically higher (up to 50%) than the model results at midlatitudes in both hemispheres. Reasonable agreement is obtained for HNO3 columns at 45 deg S, suggesting some problems with nitrogen species partitioning in the model. Outstanding uncertainties are discussed.

Danilin, Michael Y.↗
NASA NTRS1984

A measurement of stratospheric HO2 by ground-based millimeter-wave spectroscopy

Stratospheric perhydroxyl (HO2) was measured by using a sensitive mm-wave receiver to obtain spectroscopic line profiles of three rotational emission lines in the vicinity of 265.8 GHz. The observations were carried out over four days in September-October 1982 at Mauna Kea, Hawaii and yield good agreement with the column density and vertical distribution predicted above 35 km by three representative two-dimensional photochemical models employing JPL 82-57 reaction rates and chemistry. Contrasts between current theoretical predictions and previous observations by Anderson et al. (1981) are pointed out for HO2 in the 28 to 37-km range, along with the difficulty of joining the latter with the present measurements through a monotonically varying vertical profile for HO2. A possible explanation involving strong temporal and spatial variation in stratospheric water vapor content is suggested.

De Zafra, R. L.↗
NASA NTRS2000

Actinic Flux Calculations: A Model Sensitivity Study

calculate direct and diffuse surface irradiance and actinic flux (downwelling (2p) and total (4p)) for the reference model. Sensitivity analysis has shown that the accuracy of the radiative transfer flux calculations for a unit ETS (i.e. atmospheric transmittance) together with a numerical interpolation technique for the constituents' vertical profiles is better than 1% for SZA less than 70(sub o) and wavelengths longer than 310 nm. The differences increase for shorter wavelengths and larger SZA, due to the differences in pseudo-spherical correction techniques and vertical discretetization among the codes. Our sensitivity study includes variation of ozone cross-sections, ETS spectra and the effects of wavelength shifts between vacuum and air scales. We also investigate the effects of aerosols on the spectral flux components in the UV and visible spectral regions. The "aerosol correction factors" (ACFs) were calculated at discrete wavelengths and different SZAs for each flux component (direct, diffuse, reflected) and prescribed IPMMI aerosol parameters. Finally, the sensitivity study was extended to calculation of selected photolysis rates coefficients.

Krotkov, Nickolay A.↗
NASA NTRS2002

Overlap Properties of Clouds Generated by a Cloud Resolving Model

In order for General Circulation Models (GCMs), one of our most important tools to predict future climate, to correctly describe the propagation of solar and thermal radiation through the cloudy atmosphere a realistic description of the vertical distribution of cloud amount is needed. Actually, one needs not only the cloud amounts at different levels of the atmosphere, but also how these cloud amounts are related, in other words, how they overlap. Currently GCMs make some idealized assumptions about cloud overlap, for example that contiguous cloud layers overlap maximally and non-contiguous cloud layers overlap in a random fashion. Since there are difficulties in obtaining the vertical profile of cloud amount from observations, the realism of the overlap assumptions made in GCMs has not been yet rigorously investigated. Recently however, cloud observations from a relatively new type of ground radar have been used to examine the vertical distribution of cloudiness. These observations suggest that the GCM overlap assumptions are dubious. Our study uses cloud fields from sophisticated models dedicated to simulate cloud formation, maintenance, and dissipation called Cloud Resolving Models . These models are generally considered capable of producing realistic three-dimensional representation of cloudiness. Using numerous cloud fields produced by such a CRM we show that the degree of overlap between cloud layers is a function of their separation distance, and is in general described by a combination of the maximum and random overlap assumption, with random overlap dominating as separation distances increase. We show that it is possible to parameterize this behavior in a way that can eventually be incorporated in GCMs. Our results seem to have a significant resemblance to the results from the radar observations despite the completely different nature of the datasets. This consistency is encouraging and will promote development of new radiative transfer codes that will estimate the radiation effects of multi-layer cloud fields more accurately.

Oreopoulos, L.↗
NASA NTRS1989

Trends in ozone profile measurements

From an examination of the agreements and differences between different satellite instruments, it is difficult to believe that existing satellite instruments determine upper stratospheric ozone much better than 4 pct.; by extension, it probably would require at least a 4 pct. change to be reliably detected as a change. The best estimates of the vertical profiles of ozone change in the upper stratosphere between 1979 and 1986 are judged to be those given by the two SAGE satellite instruments. SAGE-2 minus SAGE-1 gives a much lower ozone reduction than that given by the archived Solar Backscatter UV data. The average SAGE profiles of ozone changes between 20 and 50 degs north and between 20 and 50 degs south are given. The SAGE-1 and SAGE-2 comparison gives an ozone reduction of about 4 pct. at 25 km over temperate latitudes. Five ground based Umkehr stations between 36 and 52 degs north, corrected for the effects of volcanic aerosols, report an ozone reduction between 1979 and 1987 at Umkehr layer 8 of 9 + or - 5 pct. The central estimate of upper stratospheric ozone reduction given by SAGE at 40 km is less than the central value estimated by the Umkehr method at layer 8.

Johnston, H.↗
NASA NTRS2020

Atmospheric Carbon Cycle Dynamics Over the Above Domain: an Integrated Analysis Using Aircraft Observations (Arctic-CA) and Model Simulations (GEOS)

The Arctic Carbon Atmospheric Profiles (Arctic-CAP) project conducted six airborne surveys of Alaska and northwestern Canada between April and November 2017 to capture the spatial and temporal gradients of northern high-latitude carbon dioxide (CO2), methane (CH4) and carbon monoxide (CO) as part of NASA's Arctic-Boreal Vulnerability Experiment (ABoVE). The Arctic-CAP sampling strategy involved acquiring vertical profiles of CO2, CH4 and CO from the surface to 5 km altitude at 25 sites around the ABoVE domain on a 4- to 6-week time interval. We observed vertical gradients of CO2, CH4 and CO that vary by eco-region and duration of the sampling period, which spanned the majority of the seasonal cycle. All Arctic-CAP measurements were compared to a global simulation using the Goddard Earth Observing System (GEOS) modeling system. Comparisons with GEOS simulations of atmospheric CO2, CH4 and CO highlight the potential of these multi-species observations to inform improvements in surface flux estimates and the representation of atmospheric transport. GEOS simulations provide estimates of the near surface average CO2 and CH4 enhancements that are well correlated with aircraft observations (R=0.74 and R=0.60 respectively), suggesting that GEOS has reasonable fidelity over this complex and heterogeneous region. This model-data comparison over the ABoVE domain reveals that while current state-of-the-art models and flux estimates are able to capture broadscale spatial and temporal patterns in near-surface CO2 and CH4 concentrations, more work is needed to resolve fine-scale flux features that are observed. The study also provides a framework for benchmarking a global model at regional scales, which is needed to use climate models as tools to investigate high-latitude carbon-climate feedbacks.

C Sweeney↗
NASA NTRSDate not supplied

An Overview of the NASA ADM-Aeolus Cal/Val Test Flight Campaign

Lidars are uniquely capable of collecting high precision and high spatio-temporal observations that have been used for atmospheric process studies from the ground, aircraft, and space for over 30 years. The Atmospheric Dynamics Mission Aeolus (ADM-Aeolus), the first-ever spaceborne Doppler wind lidar, was developed by the European Space Agency and launched in August 2018. The ADM-Aeolus Atmospheric Laser Doppler Instrument (ALADIN) observes profiles of the component of the wind vector and aerosol optical properties along the instrument’s line-of-sight direction on a global scale. Two airborne lidar systems have been developed at NASA Langley Research Center in recent years that collect measurements in support of several NASA Earth Science Division focus areas. The Doppler Aerosol WiNd (DAWN) lidar measures vertical profiles of horizontal wind speed and direction. The High Altitude Lidar Observatory (HALO) measure high resolution profiles of atmospheric water vapor (WV) and aerosol and cloud optical properties. Though new space-based missions with advanced capabilities such as Aeolus are continuously being conceived and developed, there are limitations in terms of spatial and vertical detail and measurement precision that can be accomplished from space, thus airborne remote sensing observations like those from DAWN and HALO are required to fill these observational gaps as well as to calibrate and validate space-based measurements. Over a two-week period in April 2019 during their Aeolus Cal/Val Test Flight campaign, NASA conducted five research flights over the Eastern Pacific Ocean with the DC-8 aircraft to 1) demonstrate the DAWN Doppler wind lidar, HALO high spectral resolution lidar aerosol/cloud measurement and differential absorption lidar WV measurement capabilities across a range of atmospheric conditions, 2) demonstrate Aeolus Cal/Val flight strategies and compare DAWN and HALO measurements with Aeolus to gain an initial perspective of Aeolus performance, and 3) demonstrate how atmospheric dynamic processes can be resolved and better understood through simultaneous observations of wind, WV, and aerosol profile observations, coupled with numerical model and other remote sensing observations. This paper provides a brief description of the DAWN and HALO instruments, discusses the synergistic observations collected across a wide range of atmospheric conditions sampled during the DC-8 flights, and a summary of the validation of DAWN, HALO, and Aeolus observations and comparisons.

Kristopher M. Bedka↗
NASA NTRS1974

Lidar measurements of stratospheric aerosols over Menlo Park, California, October 1972 - March 1974

During an 18-month period, 30 nighttime observations of stratospheric aerosols were made using a ground based ruby lidar located near the Pacific coast of central California (37.5 deg. N, 122.2 deg. W). Vertical profiles of the lidar scattering ratio and the particulate backscattering coefficient were obtained by reference to a layer of assumed negligible particulate content. An aerosol layer centered near 21 km was clearly evident in all observations, but its magnitude and vertical distribution varied considerably throughout the observation period. A reduction of particulate backscattering in the 23- to 30-km layer during late January 1973 appears to have been associated with the sudden stratospheric warming which occurred at that time.

Russell, P. B.↗
NASA NTRS2004

Trajectory Specification for High-Capacity Air Traffic Control

In the current air traffic management system, the fundamental limitation on airspace capacity is the cognitive ability of human air traffic controllers to maintain safe separation with high reliability. The doubling or tripling of airspace capacity that will be needed over the next couple of decades will require that tactical separation be at least partially automated. Standardized conflict-free four-dimensional trajectory assignment will be needed to accomplish that objective. A trajectory specification format based on the Extensible Markup Language is proposed for that purpose. This format can be used to downlink a trajectory request, which can then be checked on the ground for conflicts and approved or modified, if necessary, then uplinked as the assigned trajectory. The horizontal path is specified as a series of geodetic waypoints connected by great circles, and the great-circle segments are connected by turns of specified radius. Vertical profiles for climb and descent are specified as low-order polynomial functions of along-track position, which is itself specified as a function of time. Flight technical error tolerances in the along-track, cross-track, and vertical axes define a bounding space around the reference trajectory, and conformance will guarantee the required separation for a period of time known as the conflict time horizon. An important safety benefit of this regimen is that the traffic will be able to fly free of conflicts for at least several minutes even if all ground systems and the entire communication infrastructure fail. Periodic updates in the along-track axis will adjust for errors in the predicted along-track winds.

Paielli, Russell A.↗
DOE OSTI2026

3D Cloud Aerosol Precipitation Experiment at kennaook Cape Grim (3D-CAPE-k) Field Campaign Report

The objective of this campaign was to complement the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) User Facility’s Cloud And Precipitation Experiment at kennaook (CAPE-k) in northwest Tasmania by deploying scanning, fixed pointing angle, and in situ aerosol, cloud, and precipitation remote-sensing instruments during the last six months of the experiment. These instruments provided a three-dimensional (3D) context to the second ARM Mobile Facility (AMF2) vertically pointing observations collected at the kennaook Cape Grim (KCG) site and captured a portion of the life cycle of the clouds before and after the passage over the AMF2 vertical column. These 3D cloud measurements will be used in the near future to 1) investigate how the vertical profiles of aerosol and cloud properties are representative of the broader area and how these properties evolve during the portion of the cloud life cycle captured by the scanning instruments, 2) quantify how accurate the cloud fraction derived with assumptions from vertically pointing observations are compared with direct 3D cloud fraction measurements, 3) evaluate cloud fraction and liquid water path in the Australian Community Climate and Earth-System Simulator–Convective-scale (ACCESS-C) forecast model, and 4) evaluate aerosol and cloud products from the European Space Agency/Japanese Aerospace Exploration Agency (ESA/JAXA) Earth Cloud Aerosol Radiation Explorer (EarthCARE) mission using the scanning measurements, offering more chances of exact collocation, thereby complementing the statistical approach we are planning to employ with AMF2 observations for that same purpose.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1988

Emission of NO and deposition of O3 in a tropical forest system

Rates for emission of NO and deposition of O3 were measured at a tropical forest site in Reserve Adolfo Ducke, near Manaus, Brazil. Two independent techniques were used to determine the NO flux: (1) a soil enclosure method and (2) a method based on simultaneous observations of NO and O3 vertical profiles at night, when NO is irreversibly removed by reaction with O3. Results obtained using the two techniques agreed well, giving an average NO flux of 5.2 + or - 1.7 x 10 to the 10th molecules/sq cm per sec and an average vertical exchange coefficient of 2.2 x 10 to the 3rd cu cm/sec. Sources of NO from tropical forest soils may be important for global atmospheric chemistry. Rapid removal of O3 was observed in the lowest levels of the forest. The nocturnal deposition rate was estimated to be 5.6 + or - 2.5 x 10 to the 11th molecules/sq cm per sec through the 6-m level. The large deposition rate for O3 is consistent with the strong sink inferred from observations of ozone in the Amazon region.

Kaplan, W. A.↗
NASA NTRS2021

The Thermal Infrared Optical Depth of Mineral Dust Retrieved from Integrated CALIOP and IIR Observations

Recent studies reveal that a higher fraction of coarse mineral dust particles than that estimated by climate model simulations has been observed in the atmosphere, leading to a more significant positive (i.e., warming) longwave (LW) thermal infrared (TIR) direct radiative effect (DRE). However, the magnitude of this DRE remains highly uncertain because our understanding of the radiative properties, quantitatively represented by the optical depth of dust, especially information on the TIR, remains limited. This study presents a simple approach to retrieve the thermal infrared dust aerosol optical depth (DAODTIR) over oceans during nighttime using the observations from the Infrared Imaging Radiometer (IIR) and the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard CALIPSO. For each cloud-free dust-laden profile identified by the IIR-CALIOP observation, a Lookup-Table (LUT) of the 10.6 μm IIR band brightness temperatures difference (dBT) under different DAODTIR with respect to their dust-free BTs is constructed based on the CALIOP retrieved dust vertical profile and pre-assumed dust scattering properties using a fast radiative transfer model. Then the DAODTIR is retrieved by projecting the IIR-observed dBT on the LUT. Sensitivity studies show that the DAODTIR retrieval at 10.6 μm is more susceptible to the dust particle size distribution (PSD) assumption than dust refractive indices. To estimate the uncertainty caused by PSD assumption, two DAODTIR retrieval products, one based on the dust PSD from the AERONET at Cape Verde and the other on an in situ measured PSD from the recent Fennec campaign, are provided. The retrieval uncertainty is mainly contributed by the BT difference between the observation and simulation using auxiliary atmospheric data. The climatology of the retrieval from 2013 to 2019 shows confident spatiotemporal variations of DAODTIR with the global-averaged value of 0.006 and 0.008 based on different pre-assumed dust PSDs. Climatological results agree reasonably well with two independent DAODTIR retrieval products based on the Infrared Atmospheric Sounding Interferometer (IASI) over the active dust transport regions, such as North and Tropical Atlantic (r = 0.904 and 0.819) and Indian Ocean (r = 0.832). The seasonal and interannual variation is also well-compared (r = 0.758) with AERONET coarse-mode AOD at 97 selected sites. The synergic CALIOP observation allows the retrieved DAODTIR to directly compare with the extrapolated DAODTIR from DAOD in visible (i.e., 532 nm), which helps evaluate the observational constraints on DAODTIR. This study offers a unique prospect of collocating active lidar and passive IR observations for retrieving dust DAODTIR.

aerosol↗