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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 451 records · Page 25

Study of Applications of Radiological Data Fusion for Nuclear Security and Non-proliferation Applications

This report describes the radiological Scene Data Fusion (SDF) technology and the potential to apply the SDF technology to a variety of problems related to nuclear non-proliferation, radiological security, and other missions related to the national nuclear security agency and the US government, more broadly. The application space was conceived by both the authors of this report and the many scientists and stakeholders they interviewed. In order to successfully apply the SDF technology to the various applications, further research and development is often necessary and those R&D steps are also outlined herein.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Recent Advancements and Prospects of Chemical Heat Pumps for Temperature Amplification for Nuclear Process Heat Applications

The energy economy is continually evolving, particularly in terms of primary energy sources, their conversions to useful forms such as electricity and heat, and their utilization in different sectors, in response to socio-political factors. Because nuclear energy source is a clean and non-carbon-emitting energy source, it is crucial to consider its role in the evolution of the energy economy. Integrated Energy Systems (IES) are collaboratively controlled systems that can dynamically apportion thermal and/or electrical energy to promote the production of various energy products and have the potential to reduce greenhouse gas (GHG) emissions, improve energy efficiency, improve electrical grid dependability, and enhance energy economics. To realize the benefits of IES with the current reactor fleets, selection and development of a complimentary temperature upgrading technology are necessary for providing process heat and improving economics.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Survey of emerging nuclear data needs for nonproliferation applications with advanced reactors

Nuclear science plays a key role in non-proliferation activities supporting advanced reactor technologies. Nuclear data underpin predictions and interpretations of nuclear material behavior and signatures in reactor fuel production, use, transport, and storage. Advanced reactors provide new challenges compared to the current fleet of thermal fission reactors. This report consolidates reported nuclear data needs from representative workshops, conferences, and publications, identifying six themes for recommended future investments supporting non-proliferation and safeguards applications. While also identified as data needs, major fission product evaluations and (α,n) reactions were omitted as there are ongoing activities producing new data under NA22/Objective O. Each theme is summarized below with example data and association with the nonproliferation mission for advanced fuels and reactors.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Potential civil mission applications for space nuclear power systems

It is pointed out that the energy needs of spacecraft over the last 25 years have been met by photovoltaic arrays with batteries, primary fuel cells, and radioisotope thermoelectric generators (RTG). However, it might be difficult to satisfy energy requirements for the next generation of space missions with the currently used energy sources. Applications studies have emphasized the need for a lighter, cheaper, and more compact high-energy source than the scaling up of current technologies would permit. These requirements could be satisfied by a nuclear reactor power system. The joint NASA/DOD/DOE SP-100 program is to explore and evaluate this option. Critical elements of the technology are also to be developed, taking into account space reactor systems of the 100 kW class. The present paper is concerned with some of the civil mission categories and concepts which are enabled or significantly enhanced by the performance characteristics of a nuclear reactor energy system.

Ambrus, J. H.↗

Machine learning for fundamental spectroscopic and thermodynamic data of actinides and lanthanides

Accurately modeling optical spectra with absolute radiometric intensities is vital for nuclear forensics applications that depend on characterizing optical emissions from energetic nuclear phenomena. This requires precise knowledge of the individual atomic transition probabilities, known as Einstein A-coefficients, for each emission line. Obtaining these values theoretically or experimentally is often impractical due to the complex electronic structures and the number of transitions involved in atoms relevant to nuclear applications. In this study, we explore the use of machine learning to predict the Einstein A coefficients for atomic transitions. Seven models were evaluated that ranged from deep learning to decision tree algorithms, and found that gradient boosting performed best, specifically the Extreme Gradient Boosting (XGB) architecture, achieving a precision of 86% across transitions of 36 elements. Furthermore, the model was cross-validated using published transition probabilities reported in the literature and applied to estimate Pu plasma temperatures from a previous experiment conducted at Savannah River National Laboratory.

Atomic spectroscopy↗

Gas Turbine Energy Conversion Systems for Nuclear Power Plants Applicable to LiFTR Liquid Fluoride Thorium Reactor Technology

This panel plans to cover thermal energy and electric power production issues facing our nation and the world over the next decades, with relevant technologies ranging from near term to mid-and far term.Although the main focus will be on ground based plants to provide baseload electric power, energy conversion systems (ECS) for space are also included, with solar- or nuclear energy sources for output power levels ranging tens of Watts to kilo-Watts for unmanned spacecraft, and eventual mega-Watts for lunar outposts and planetary surface colonies. Implications of these technologies on future terrestrial energy systems, combined with advanced fracking, are touched upon.Thorium based reactors, and nuclear fusion along with suitable gas turbine energy conversion systems (ECS) will also be considered by the panelists. The characteristics of the above mentioned ECS will be described, both in terms of their overall energy utilization effectiveness and also with regard to climactic effects due to exhaust emissions.

Energy Conversion↗

Recent advances in chiral EFT based nuclear forces and their applications

During the past two decades, chiral effective field theory has evolved into a powerful tool to derive nuclear forces from first principles. Nearly all two-nucleon interactions have been worked out up to sixth order of chiral perturbation theory, while, with few exceptions, three-nucleon forces, which play a subtle, but crucial role in microscopic nuclear structure calculations, have been derived up to fifth order. We review the current status of these forces as well as their applications in nuclear many-body systems. While the ab initio description of light nuclei is generally very successful, we point out and analyze problems encountered with medium-mass nuclei. We also survey the construction of equations of state for symmetric nuclear matter and neutron-rich matter based on chiral forces. A focal point is the symmetry energy and its impact on neutron skins and systems of astrophysical relevance. The physics of neutron-rich systems, from nuclei to compact stars, is essentially determined by the density dependence of the symmetry energy. Here, we review the status of predictions in comparison with latest empirical constraints, with particular attention to those extracted from parity-violating electron scattering.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Contextually aware roadside radiation measurement testbed

Here we demonstrate a contextually aware multimodal roadside radiation measurement detection testbed for traffic monitoring applications in nuclear nonproliferation. Many variables in traffic such as vehicle or cargo size, mass, speed, shape, and distance of closest approach can have significant impacts on the radiation measured from a vehicle-transported radiation source. These factors can lead to uncertainties in the analysis of the radiation source, especially for lower-strength radiation sources of interest. Our testbed, known as the Multimodal Measurement System (MMS) uses non-radiation sensors including magnetometers, geophones, radiofrequency receivers, cameras, and LiDAR to extract contextual information about vehicles passing by the system. These contextual data can then be fused with data from radiation measurements to increase the system’s sensitivity and accuracy in nuclear threat detection applications. This work describes the instrumentation of the MMS and its data acquisition pipeline. Furthermore, we describe the pre-analysis performed on the raw multimodal data streams for data fusion, and the high-level machine learning analyses for detection and characterization. The variety of sensors within the MMS provides a valuable testbed that can be used to identify the combinations of contextual sensors that provide the greatest improvements to radiation source detection and characterization within the restrictions for various proliferation detection applications. The MMS is also modular so that additional combinations of sensors can be explored in the future.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Spectral Element Applications in Complex Nuclear Reactor Geometries: Tet-to-Hex Meshing

The spectral element code Nek5000 is an open-source, higher-order computational fluid dynamics code developed at Argonne National Laboratory. It is designed to solve incompressible Navier-Stokes equations, but it also has a low-Mach-number approximation feature available. Large eddy simulation is approached by explicit filtering of the velocity field (and other fields) to mimic the effect of dissipation due to the unresolved scale. The computational domain is decomposed into second-order hexahedral elements that conform to the boundaries. However, generating a high-quality pure-hexahedral mesh can be challenging for some problems. For simple geometries, traditional blocking methods can be used to decompose the domain into smaller blocks to generate a so-called structural mesh. A structural mesh can maintain good orthogonality but can have a highly skewed mesh to conform to the geometry, as well as unnecessary refinement in the far field. Moreover, for geometries with relative complexity, blocking the geometry becomes impossible. To address these issues, we adopted a let-to-hex strategy to generate a pure hexahedral mesh for Nek5000. First, we generate a pure tetrahedral mesh for the geometry; then we divide one tetrahedral element into four hexahedral elements. A pure tetrahedral mesh could be easily generated for complex geometries by using many current meshing codes. In this paper, we use the commercial codes ANSYS meshing and ANSYSICEM to generate the pure tetrahedral mesh and then convert it to a pure hexahedral mesh. Boundary layers are extruded in ANSYSICEM to maintain near-wall resolution.

ANSYS ICEM↗

Evaluation of subsurface transport processes of delayed gas signatures applicable to underground nuclear explosions

Radioactive gas signatures from underground nuclear explosions (UNEs) result from gas-migration processes occurring in the subsurface. The processes considered in this study either drive or retard upward migration of gases from the detonation cavity. The relative importance of these processes is evaluated by simulating subsurface transport in a dual-permeability medium for the multi-tracer Noble Gas Migration Experiment (NGME) originally intended to study some aspects of transport from a UNE. For this experiment, relevant driving processes include weak two-phase convection driven by the geothermal gradient, over pressuring of the detonation cavity, and barometric pumping while gas sorption, dissolution, radioactive decay, and usually diffusion represent retarding processes. From deterministic simulations we found that over-pressuring of the post-detonation chimney coupled with barometric pumping produced a synergistic effect amplifying the tracer-gas reaching the surface. Bounding simulations indicated that the sorption and dissolution of gases, tending to retard transport, were much smaller than anticipated by earlier laboratory studies. The NGME observations themselves show that differences in gas diffusivity have a larger effect on influencing upward transport than do the combined effects of tracer-gas sorption and dissolution, which is consistent with a Sobol’ sensitivity analysis. Both deterministic simulations and those considering parametric uncertainties of transport-related properties predict that the excess in concentration of SF 6 compared to 127 Xe as might be captured in small volumetric samples should be much smaller than the order-of-magnitude contrast found in the large-volume gas samples taken at the site. While extraction of large-volume subsurface gas samples is shown to be capable of distorting in situ gas compositions, the highly variable injection rate of SF 6 into the detonation cavity relative to that of 127 Xe at the start of the field experiment is the most likely explanation for the large difference in observed concentrations.

58 GEOSCIENCES↗

The effect of gamma ray irradiation on few layered MoSe2: A material for nuclear and space applications

In recent years, emerging two-dimensional (2D) materials, such as molybdenum diselenide (MoSe2), have been at the center of attention for many researchers. This is due to their unique and fascinating physicochemical properties that make them attractive in space and defense applications that include shielding harsh irradiation environments. In this study, we examined the effects of gamma (γ) rays at various doses on the structural, chemical, and optical properties of MoSe2 layers. After the samples were exposed to intense gamma radiation (from a 60Co source) with various exposure times to vary the total accumulated dosage (up to 100 kGy), Raman and photoluminescence spectroscopies were used to study and probe radiation-induced changes to the samples. When compared to pristine materials, very few changes in optical properties were typically observed, indicating good robustness with little sensitivity, even at relatively high doses of gamma radiation. The imaging using scanning electron microscopy revealed a number of nano-hillocks that were connected to substrate alterations. X-ray photoelectron spectroscopies revealed that Mo’s binding energies remained the same, but Se’s binding energies blueshifted. We associated this shift with the decrease in Se vacancies that occurred after irradiation as a result of Mo atoms creating adatoms next to Se atoms. When compared to pristine materials, very few changes in optical, chemical, and structural properties were typically observed. These findings highlight the inherent resilience of MoSe2 in hostile radioactive conditions, which spurs additional research into their optical, electrical, and structural characteristics as well as exploration for potential space, energy, and defense applications.

Materials Science↗

Normalizing Flows for Microscopic Many-Body Calculations: An Application to the Nuclear Equation of State

We report that normalizing flows are a class of machine learning models used to construct a complex distribution through a bijective mapping of a simple base distribution. We demonstrate that normalizing flows are particularly well suited as a Monte Carlo integration framework for quantum many-body calculations that require the repeated evaluation of high-dimensional integrals across smoothly varying integrands and integration regions. As an example, we consider the finite-temperature nuclear equation of state. An important advantage of normalizing flows is the ability to build highly expressive models of the target integrand, which we demonstrate enables precise evaluations of the nuclear free energy and its derivatives. Furthermore, we show that a normalizing flow model trained on one target integrand can be used to efficiently calculate related integrals when the temperature, density, or nuclear force is varied. This work will support future efforts to build microscopic equations of state for numerical simulations of supernovae and neutron star mergers that employ state-of-the-art nuclear forces and many-body methods.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

FAUST - Benchmark and Validation Framework [Slides]

This presentation discusses Python packages for nuclear data applications and for benchmarking. It also discusses the goals and objectives for FAUST which include providing input and output processing for different calculation codes, allowing for exchanging results between different applications and codes, running benchmarks and processing the results, automating and simplify plot and report generation, and providing a basis for developing applications useful for nuclear data evaluators. The presentation also discusses how the packages can be used both inside and outside LANL.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗