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Characterizing Density and Complexity of Imported Cargos

X-ray inspection systems are used to detect radiological and nuclear threats in imported cargo. In order to better understand performance of these systems, system imaging capabilities and the characteristics of imported cargo need to be determined. This project involved calculation of the modulation transfer function as a metric of system imaging performance and a study of the density and inhomogeneity of imported cargos, which have been shown to correlate with human analysts, threat detection performance.

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Cooperation on Improved Isotopic Identification and Analysis Software for Portable, Electrically Cooled High-Resolution Gamma Spectrometry Systems Final Report

Under a 2006 agreement between the Department of Energy (DOE) of the United States of America and the Institut de Radioprotection et de Sûreté Nucléaire (IRSN) of France, the National Nuclear Security Administration (NNSA) within DOE and IRSN initiated a collaboration to improve isotopic identification and analysis of nuclear material [i.e., plutonium (Pu) and uranium (U)]. The specific aim of the collaborative project was to develop new versions of two types of isotopic identification and analysis software: (1) the fixed-energy response-function analysis for multiple energies (FRAM) codes and (2) multi-group analysis (MGA) codes. The project is entitled Action Sheet 4 – Cooperation on Improved Isotopic Identification and Analysis Software for Portable, Electrically Cooled, High-Resolution Gamma Spectrometry Systems (Action Sheet 4). FRAM and MGA/U235HI are software codes used to analyze isotopic ratios of U and Pu. FRAM is an application that uses parameter sets for the analysis of U or Pu. MGA and U235HI are two separate applications that analyze Pu or U, respectively. They have traditionally been used by safeguards practitioners to analyze gamma spectra acquired with high-resolution gamma spectrometry (HRGS) systems that are cooled by liquid nitrogen. However, it was discovered that these analysis programs were not as accurate when used on spectra acquired with a newer generation of more portable, electrically cooled HRGS (ECHRGS) systems. In response to this need, DOE/NNSA and IRSN collaborated to update the FRAM and U235HI codes to improve their performance with newer ECHRGS systems. Lawrence Livermore National Laboratory (LLNL) and Los Alamos National Laboratory (LANL) performed this work for DOE/NNSA.

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Safeguards Technology Development Program 3rd Quarter FY 2018 Report

LLNL will evaluate the performance of a stilbene-based scintillation detector array for IAEA neutron multiplicity counting (NMC) applications. This effort will combine newly developed modeling methodologies and recently acquired high-efficiency stilbene detector units to quantitatively compare the prototype system performance with the conventional He-3 counters and liquid scintillator alternatives.

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Risk-Informed Safety Margins Characterization (RISMC) Pathway Technical Program Plan

Safety is central to the design, licensing, operation, and economics of nuclear power plants (NPPs). As the current Light Water Reactor (LWR) NPPs age beyond 60 years, there are possibilities for increased frequency of systems, structures, and components (SSCs) degradations or failures that initiate safety-significant events, reduce existing accident mitigation capabilities, or create new failure modes. Plant designers commonly “over-design” portions of NPPs and provide robustness in the form of redundant and diverse engineered safety features to ensure that, even in the case of well-beyond design basis scenarios, public health and safety will be protected with a very high degree of assurance. This form of defense-in-depth is a reasoned response to uncertainties and is often referred to generically as “safety margin.” Historically, specific safety margin provisions have been formulated, primarily based on “engineering judgment.” The ability to better characterize (i.e., describe and quantify) safety margin is important to improved decision making about LWR design and long-term operation. A systematic approach to characterizing safety margins and the subsequent risk informed margins management options represents a vital input to the licensee and regulatory analysis and decision making that will be involved. In addition, as research and development (R&D) in the LWRS Program and other collaborative efforts yield new data and improved scientific understanding of physical processes that govern the aging and degradation of plant SSCs (and concurrently support technological advances in nuclear reactor fuels and plant instrumentation and control systems), needs and opportunities to better optimize plant safety, economics, and performance will become known. The purpose of the Risk-Informed Safety Margins Characterization (RISMC) Pathway R&D is to support plant decisions for risk-informed margins management with the aim to improve economics, reliability, and sustain safety of current NPPs over periods of extended plant operations. The goals of the RISMC Pathway are twofold: (1) develop and demonstrate a risk-assessment method that is coupled to safety margin quantification that can be used by NPP decision makers as part of risk-informed margin management strategies; (2) create an advanced RISMC Toolkit that enables more accurate representation of NPP safety margins. The methods and tools provided by RISMC are essential to a comprehensive and integrated risk-informed margin management approach that supports effective preservation of margin for both active and passive SSCs.

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Defining and Characterizing Methods, Tools, and Computing Resources to Support Pseudo Exhaustive Testability of Software Based I&C Devices

Under the Department of Energy’s Light Water Reactor Sustainability Program, within the Plant Modernization research pathway, the Digital I&C Qualification Project is identifying new methods that would be beneficial in qualifying digital I&C systems and devices for safety-related usage. One such method that would be useful in qualifying field components such as sensors and actuators is the concept of testability. The Nuclear Regulatory Commission (NRC) considers testability to be one of two design attributes sufficient to eliminate consideration of software-based or software logic-based common cause failure (the other being diversity). The NRC defines acceptable “testability” as follows: Testability – A system is sufficiently simple such that every possible combination of inputs and every possible sequence of device states are tested and all outputs are verified for every case (100% tested). [NUREG 0800, Chapter 7, Branch Technical Position (BTP) 7-19] This qualification method has never proven to be practical in view of the very large number of combinations of inputs and sequences of device states for a typical I&C device. However, many of these combinations are not unique in the sense that they represent the same state space or in that that they represent state space that would not affect the critical design basis functions of the device. Therefore, the state space of interest might possibly be reduced to a manageable dimension through such analysis. This project focuses on a representative I&C device similar in design, function, and complexity to the types of devices that would likely be deployed in nuclear power plants as digital or software based sensors and actuators (e.g. Smart Sensors). Analysis will be conducted to determine the feasibility of testing this device in a manner consistent with the NRC definition. This report describes acceptable test methods, needed tools (existing or new), and computing resources, all based on engineering and computer science principles. This information will then be used in a later phase of this project to develop a test specification for I&C device testability that can be used in a future phase of this project to demonstrate digital qualification with respect to common cause failure. Following that, testing will be conducted and the results analyzed to determine if the methods employed are sufficient to eliminate consideration of software common cause failure in accordance with the concept of testability.

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FY 2018 Summary Report on Industrial and Regulatory Engagement Activities

The Plant Modernization Pathway of the Light Water Reactor Sustainability (LWRS) Program conducts a vigorous engagement strategy with the U.S. nuclear power industry, including the nuclear operating companies, major support organizations, the Nuclear Regulatory Commission (NRC), and suppliers. The goal of this engagement strategy is to develop a shared vision and common understanding across the nuclear industry of the need for plant modernization, the performance improvement that can be attained, and the opportunities for collaboration to enact this vision. In FY 2018, the vision, strategy, and project work was communicated to a number of key organizations, including the major industry support organizations, and a number of important industry conferences that are attended by leaders in nuclear plant modernization. This report presents the specific engagement activities that occurred in FY 2018 to promote awareness and participation by the nuclear power industry in the activities of the Plant Modernization Pathway.

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Self-powered Wireless Dual-mode Langasite Sensor for Pressure/Temperature Monitoring of Nuclear Reactors

Safety issues in nuclear power plants are of extreme importance. Numerous sensors are used within nuclear power plants for sensing and monitoring of its critical operation parameters. As currently implemented, during massive losses of power across the plant in accidents, the backup batteries for the monitoring sensors will ultimately be drained and can cease to operate. The overall objective of this NEUP project is to develop a novel self-powered wireless hybrid sensor which can accurately monitor both pressure and temperature using a single device, even in the extreme harsh environments of severe nuclear accidents, without the requirement of external electricity. At Virginia Tech side, a heat pipe assisted thermoelectric generator (TEG) energy harvester and associated power management and data transmission circuits were developed. The energy harvester can produce electrical power continuously, even in loss of plant and external power situations, providing power for important data transmission for accident diagnosis. The self-powered sensing system could be integrated directly onto key nuclear components including pipes, pump housings, heat exchangers, reactor vessels, and shielding structures inside and outside of the reactor core. Two TEG based energy harvesters which can work in relatively low (50-250 ºC) and high temperature ranges (250-350 ºC) were established and tested. In the prototypes, heat pipes were introduced to reduce the heat resistances of the device at the hot and cold ends. The power output of the heat pipe assisted TEG module is 2.22 W, which is 6 times more than one using an aluminum rod. In-lab tests showed that these devices canmeet the requirement to power the sensors and circuit during normal and off-normal conditions.Amodel was then built to analyze the thermal network in the energy harvester, and was used to optimize its performance and reduce its geometry size. The design and testing of the vibrational energy harvester were completed. The harvester, has shown to effectively increase the vibrational potential of the main coolant pump, though it has been shown that thermal energy has a much higher potential for the powering of sensors. In this project, a self-start charger circuit for the energy harvester was designed to regulate and manage the power. An energy storage element was incorporated into the energy harvesting module for sensors and wireless transceivers in an off-normal situation. The signal conditioning and wireless communication electronic circuits were developed and tested in the lab. An important consideration for an energy harvester within a nuclear power plant is the level of radiation it will encounter during operation. The two main sources of radiation in a nuclear power plant are gamma and neutron radiation. Aradiation experiment was conducted in the Westinghouse Electric Company during which the prototypes were placed in a 106 rad radiation environment to test their ability to operate in the extreme environment. The results showed that this level of radiation had little effect on the performance of the TEGmaterial and heat pipe heat exchanging system. Its influence on the circuit was still under research, however the need for more development on radiation hardened electronics is needed. Pressure measurement based on piezoelectric crystal resonators has advantages over the commercially available methods like capacitive, electromagnetic, optical, potentiometric, and piezo resistive strain gauges. Since the output of piezoelectric based sensors are digital in format, it has a very high resolution, high accuracy, and long-term stability. Quartz is one of the commonly used piezoelectric material in digital pressure sensors design. This material is elastic in nature, providing high stability, high repeatability, high elasticity, repeatable mechanical behavior for many cycles of operation, and is free of hysteresis. The quartz resonator has a high Q, which means that very high vibration can be driven with the very low electric power. Langasite (LGS) is a new promising piezoelectric material that combines the advantageous properties of quartz with a better performance at high temperatures. LGS will not undergo any phase transitions up to its melting temperature of 1473 C, and hence, the application of Langasite in measuring pressure at high temperatures is promising. In this project, the design and fabrication of the piezo oscillator crystal for temperature and pressure measurement has been completed. The entire sensor has been fabricated and tested to see its sensitivity to temperature and pressure changes. The design and optimization of the radiation shielding systems that can effective protect the duel-mode Langasite sensor inside reactor core were demonstrated. To maximize the radiation shielding effectiveness, different types of materials are investigated based upon recent developments of radiation shielding systems including aluminum + Boron carbide and bismuth borosilicate glass B2O3 in addition to tungsten/B4C. New materials based upon metatheses is included as potential shielding to mitigate neutron fluencies. The radiation shielding effectiveness of selected composites are evaluated within a broader neutron spectrum from thermal, epithermal, fast (1 MeV) and 15 MeV neutrons. Performance analysis was also conducted to evaluate the effects of selected composite systems.Aconceptual design was also proposed for the packaging and integration of the radiation shielding system with the sensor, and its applicability within the reactor core was discussed. At end of the project, all components necessary for a complete sensing and monitoring system, including a langasite sensor, electrodes, the TEG harvester, an energy storage device, and power management and transmission electronics were integrated to demonstrate feasibility in powering the sensor. Finally, integration of each component into a full package, and a full demonstration were done.

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Addressing Nuclear I&C Modernization Through Application of Techniques Employed in Other Industries

This research focuses on presenting advancements that have been made by non-nuclear I&C OT vendors and potential savings that could be realized by their optimized nuclear industry application. To promote understanding and to bound the initial scope for this effort, a pilot vendor and an associated pilot implementation were chosen as an integrated, presentation example for illustration. This integrated example is unique in that a utility in the United States (Duke Energy) engaged a traditional non-nuclear vendor (Honeywell Process Solutions) to install a non-safety, Distributed Control System (DCS) in four of its nuclear units. Duke Energy is currently exploring performing a “technology refresh” of these installed systems as part of a program to address digital obsolescence. This research presents techniques developed by distributed control system vendors to enable such upgrades and potential methods to employ them in a nuclear industry context. The objectives of such an effort are to minimize the utility cost both to refresh the systems and to put the systems into a repeatable refresh cycle for future obsolescence management. This will enable the utility to maximize the benefits of expanded use of their DCS as part of a larger plant strategy to eliminate obsolete I&C systems, reduce Operating and Maintenance (O&M) costs, and improve operational performance through digitalization.

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Modeling and Simulation - Introducing hardware-in-the-loop capabilities to the Human Systems Simulation Laboratory

The DOE Office of Nuclear Energy (DOE-NE) cybersecurity program would like to expand the use of the Human Systems Simulation Laboratory to include capabilities for cybersecurity research and development. Specifically, the introduction of hardware-in-the-loop (HITL) simulation of nuclear power plant architecture into the HSSL will enable researchers and nuclear utilities the ability to identify impacts generated by sophisticated hostile cyber adversaries to identify the consequences of simulated potential attack vectors, and to develop solutions for detecting or preventing these cyber attacks.

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REALIZATION OF A AUTOMATED T-WAY COMBINATORIAL TESTING APPROACH FOR A SOFTWARE BASED EMBEDDED DIGITAL DEVICE

Under the Department of Energy’s Light Water Reactor Sustainability Program, within the Plant Modernization research pathway, the Digital I&C Qualification Project is identifying new methods that would be beneficial in qualifying digital I&C systems and devices for safety-related usage. One such method that would be useful in qualifying field components such as sensors and actuators is the concept of testability. The Nuclear Regulatory Commission (NRC) considers testability to be one of two design attributes sufficient to eliminate consideration of software-based or software logic-based common cause failure (the other being diversity). The NRC defines acceptable “testability” as follows: Testability – A system is sufficiently simple such that every possible combination of inputs and every possible sequence of device states are tested and all outputs are verified for every case (100% tested). [NUREG 0800, Chapter 7, Branch Technical Position (BTP) 7-19] This qualification method has never proven to be practical in view of the very large number of combinations of inputs and sequences of device states for a typical I&C device. However, many of these combinations are not unique in the sense that they represent the same state space or in that that they represent state space that would not affect the critical design basis functions of the device. Therefore, the state space of interest might possibly be reduced to a manageable dimension through such analysis. This project will focus on a representative I&C device similar in design, function, and complexity to the types of devices that would likely be deployed in nuclear power plants as digital or software based sensors and actuators (e.g. Smart Sensors). Analysis will be conducted to determine the feasibility of testing this device in a manner consistent with the NRC definition. This report describes the development of test process for Bounded Exhaustive Testing with respect to Combinatorial Test (CT) methods. The report describes the candidate Device Under Test SW – the VCU smart sensor, conceptual experimental methods for stated test objectives, description of the process, tools, resources, and computing. This information will be used to fully develop a detailed test plan (based on statistical measure needs) and test environment for conducting an I&C device testability demonstration study. The future planed experimental study of this project is to demonstrate digital qualification via Bounded Exhaustive Testability with respect to Common Cause Failure.

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Experiments at TA-55 have used optical pyrometry to measure temperatures of shocked plutonium on the 40mm gun

Researchers at LANL, along with collaborators from MSTS, have worked for more than a decade to develop and implement an optical pyrometry method to measure the temperature of metals shocked to the high pressures and temperatures. Because traditional shock wave measurements only provide information on the mechanical state of the material, temperature measurements are required to validate and improve equation-of-state (EOS) models for materials. The conditions sampled are complex; commenserate with those found in planetary impacts, and accressed by conventional and nuclear weapons. Optical pyrometry is currently the best available method for inferring the temperature of shocked metals, by careful measurement of the calibrated radiance emitted by a surface at finite temperature. These measurements are difficult often complicated by the short time scales associated with shock wave experiments (<1 µs) coupled with the many sources of non-thermal light (impact flash, fracture light, etc.) that pollutes the radiant light measured from the sample.

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Design of Microwave Resonant Cavity Transducer. Development of sensor performance model of microwave cavity flow meter for advanced reactor high temperature fluids

High-temperature fluid reactors, such as molten salt cooled reactors (MSCR) and sodium fast reactors (SFR), are a promising advanced reactor option. Measurement of high-temperature fluid process variables, in particular the flow inside the pressure vessel, is a challenging task because of harsh environment, which includes high radiation, high temperature, and contact with highly corrosive coolant fluid. We are investigating a microwave cavity-based transducer for high-temperature fluid flow sensing. This sensor is a hollow metallic cylindrical cavity, which can be fabricated from stainless steel, and as such is expected to be resilient to radiation, high temperature and corrosive environment of MSCR and SFR. The principle of sensing consists of making one wall of the cylindrical cavity flexible enough so that dynamic pressure, which is proportional to fluid velocity, will cause membrane deflection. A cavity is characterized by its resonant frequencies. Membrane deflection causes cavity volume change, which leads to a shift in the resonant frequency. Feasibility of the flow sensor is evaluated with signal sensitivity using COMSOL computer simulations. A right cylinder geometry stainless steel cavity with dimeter of 0.8in was investigated. We choose membrane thickness of 10mil, so that corrosion anticipated to proceed at the rate of 1mil/year in liquid sodium would affect no more than 10% of the membrane. Using the properties of liquid sodium fluid, and stainless-steel material property values at 500oC, we calculate frequency shift for a range of values of fluid velocity from 0.5m/s to 2m/s. Results of computer simulations indicate measurable sensitivity to flow for this cavity design. Following these simulations, we have developed a preliminary design for fabrication of a transducer operating in microwave K-band for proof-of-principle tests.

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Electroanalytical Sensors for Liquid Fueled Fluoride Molten Salt Reactor

ThorCon is developing a thermal thorium / uranium molten salt fueled reactor that uses a fuel salt consisting of NaF - BeF 2 - ThF 4 - UF 4 - UF 3 , which uses 19.75% enriched uranium. It is not a breeder reactor but requires regular additions of fissile material. On-site fuel processing is limited to adding make-up fuel, and adding beryllium to maintain redox balance in the fuel salt. The fluoride salt is an excellent flux that will strip the protective oxygen away from all metal surfaces it contacts. In order to protect the metal surfaces in the primary loop, no free fluorine is allowed. Maintaining a ratio of UF 4 to UF 3 provides a chemical buffer that can absorb any free fluorine released during the fission process before it can harm the structure. Periodic additions of metallic beryllium to the fuel salt will react with UF 4 to form BeF 2 and UF 3 , which will maintain the desired UF 4 /UF 3 ratio. A means to measure the UF 4 /UF 3 ratio is important to maintain the fuel salt in a non-corrosive state and could also provide additional insight into the corrosion behavior and chemical constitution of the system. A promising measurement technique is based on electrochemistry.

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Towards a New Supply Chain Cybersecurity Risk Analysis Technique

Supply chain cyber-attacks, such as the SolarWinds Orion attack, are occurring with greater frequency. These attacks compromise a digital device before it is sent to customers, bypassing traditional security controls to remain persistent and undetected in operational environments. While supply chain attacks are prevalent, methods for analyzing the risk of these attacks are currently unavailable. This paper proposes new supply chain cyber-attack difficulty and risk metrics to evaluate the relative risk of an attack throughout the supply chain lifecycle. Difficulty metrics for each stakeholder in a digital device’s supply chain (e.g., hardware manufacturing, firmware development, software development, storage, and distribution entities) are calculated using scores from cybersecurity maturity questionnaires in a Bayesian Network leaky Noisy-MAX model. These difficulty metrics are then used to calculate an overall supply chain cyber-attack risk. Vulnerability and recoverability metrics are also proposed to evaluate the relative stakeholder influence in the attack risk. These proposed relative risk metrics enable continuous supply chain monitoring, provide decision-makers with information necessary for improved supplier selection, and help drive improvements in the cybersecurity posture of the stakeholders in their supply chain.

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Analysis of Microwave Resonant Cavity Transducer Degradation Mechanisms

We are investigating a microwave resonant cavity transducer for flow sensing in the vessel of a high temperature fluid advanced reactor (AR), such as a molten salt cooled reactor (MSCR) or a sodium fast reactor (SFR). This transducer is a hollow metallic cylindrical cavity, with the flat wall of the cylinder flexible enough to undergo microscopic deflection due to dynamic fluid pressure. Membrane deflection leads to a shift in the resonant frequency, which can be detected with a spectrum analyzer. Because the transducer is intended for immersion in a high temperature corrosive fluid, understanding of material degradation is crucial for estimation of transducer performance lifetime, and development of measurement interpretation algorithms. We conducted a preliminary computational investigation of relevant damage mechanisms of a stainless steel 316 cylindrical resonator in FLiBe salt. The two main damage mechanisms, creep and corrosion, were modeled using multiphysics COMSOL software. Degradation was modeled for a temperature range 500°C to 700°C. Coupling of the damage mechanisms was not considered. These models predict significant inelastic deformation at most temperatures due to creep, and qualitatively predict chromium depletion both along the liquid/solid interface and along the grain boundaries. An algorithmic approach for compensation of these degradation effects during fluid flow measurements will be developed in the future work.

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Development of Optical Fiber-Based Sensors for Nuclear Microreactor Structural Health Monitoring

This report provides an experimental assessment of two different optical fiber–based acoustic sensors that are being investigated for application in nuclear microreactors to enhance structural health monitoring capabilities. Optical fibers are resilient in high-temperature and high-radiation environments, have a small sensor footprint, are immune to electromagnetic interference, and are capable of spatially distributed sensing. The two sensors investigated here are (1) Fabry–Pérot Cavities (FPCs) between two copper-coated fibers, embedded in nickel capillary tubes and (2) type-I fiber Bragg grating (FBG) arrays contained within metal capillary tubes. These sensors can be interrogated using low-coherence interferometry or swept wavelength interferometry, respectively, to measure the resonant frequencies of the components or systems to which these sensors are bonded. The FPC developed herein has been subjected to temperatures up to nearly 800°C while tack-welded to a tubular test specimen. Even at the highest temperatures, the measured resonant frequencies compared well with those obtained using an accelerometer that was bonded to an unheated portion of the specimen. The FBG array was tested in multiple bonding configurations to a tubular test specimen, all at room temperature, with the understanding that high temperature (i.e., type II) FBGs could be used to obtain similar data at high temperatures; the FBG array data were validated with noncontact laser vibrometry, which is being used at Los Alamos National Laboratory to relate acoustic signatures to component stresses and/or structural defects. The goal of this work is to identify the most promising techniques that are also compatible with operation in a microreactor environment.

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