Search NASA⌕ Search

SEARCH · Search NASA

Results for “cloud aerosol interactions”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 451 records · Page 25
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

A meteorological overview of the ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) campaign over the southeastern Atlantic during 2016–2018: Part 1 – Climatology

In 2016–2018, the ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) project undertook 3-month-long deployments to the southeastern (SE) Atlantic Ocean using research aircraft to better understand the impact of biomass burning (BB) aerosol transport to the SE Atlantic Ocean on climate. In this (part 1 of the meteorological overview) paper, the climatological features at monthly timescales are investigated. The southern African easterly jet (AEJ-S), defined as the zonal easterlies over 600-700 hPa exceeding 6 m s-1 around 5-15°S, is a characteristic feature of the mid-level circulation over southern Africa that was also during the deployment months of August 2017, September 2016, and October 2018. Climatologically, the AEJ-S develops at lower altitudes (~3 km; 700 hPa) between 5-10° S in August, while it develops at around 4 km (~600 hPa) and further south (5-15 °S) in September and October, largely driven by the strong sensible heating over the African plateau. Notable meteorological anomalous characteristics during the 3 deployment months, compared to climatology (2000-2018), include the following: (1) during August 2017, the AEJ-S was weaker than the climatological mean, with an additional anomalous upper-level jet aloft (~6 km) around 10 °S. August 2017 was also drier over the SE Atlantic at 600-700 hPa than climatology, with a stronger Benguela low-level jet (LLJ) at 925-950 hPa along the Namibian coast of the SE Atlantic. Consistent with this, the southern Atlantic anticyclone was also stronger and closer to the coast than the August climatological mean. (2) During September 2016, the AEJ-S intensity was similar to the climatological mean, although the heat low and vertical motion over the land was slightly stronger compared to the September climatology. The LLJ and the large-scale southern Atlantic anticyclone were stronger than the climatological mean. (3) During October 2018, the AEJ-S was slightly weaker compared to the climatological mean, as was the LLJ and the southern Atlantic anticyclone. October 2018 was wetter over the Benguela coastal region at 600 hPa than the climatological mean. During all the deployment months, the sea surface temperatures (SST) over the SE Atlantic were warmer than the climatological means, but the monthly mean low cloud fraction was only noticeably reduced in August 2017. A weak August 2017 AEJ-S can explain low offshore black carbon (BC) mixing ratios within the European Centre for Medium-Range Weather Forecasts (ECMWF) Copernicus Atmosphere Monitoring Service (CAMS) reanalysis, although the BC peak altitude, at 2-3 km, is below that of the AEJ-S. The upper-level wave disturbance and the associated anomalous circulation also explain the weakening of AEJ-S through the reduction of the strength of the heat low over the land during August 2017.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2023

Spatially-Coordinated Airborne Data and Complementary Products for Aerosol, Gas, Cloud, and Meteorological Studies: the Nasa Activate Dataset

The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions, with applications extending from process-based studies to multi-scale model intercomparison and improvement as well as to remote-sensing algorithm assessments and advancements. ACTIVATE used two NASA Langley Research Center aircraft, a HU-25 Falcon and King Air, to conduct systematic and spatially coordinated flights over the northwest Atlantic Ocean, resulting in 162 joint flights and 17 other single-aircraft flights between 2020 and 2022 across all seasons. Data cover 574 and 592 cumulative flights hours for the HU-25 Falcon and King Air, respectively. The HU-25 Falcon conducted profiling at different level legs below, in, and just above boundary layer clouds (< 3 km) and obtained in situ measurements of trace gases, aerosol particles, clouds, and atmospheric state parameters. Under cloud-free conditions, the HU-25 Falcon similarly conducted profiling at different level legs within and immediately above the boundary layer. The King Air (the high-flying aircraft) flew at approximately ∼ 9 km and conducted remote sensing with a lidar and polarimeter while also launching dropsondes (785 in total). Collectively, simultaneous data from both aircraft help to characterize the same vertical column of the atmosphere. In addition to individual instrument files, data from the HU-25 Falcon aircraft are combined into “merge files” on the publicly available data archive that are created at different time resolutions of interest (e.g., 1, 5, 10, 15, 30, 60 s, or matching an individual data product's start and stop times). This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes. The data are publicly accessible through https://doi.org/10.5067/SUBORBITAL/ACTIVATE/DATA001 (ACTIVATE Science Team, 2020).

Aerosol Cloud meTeorology Interactions oVer the we↗
DOE OSTI2026

Corrected Moments in Antenna Coordinates (CMAC) Technical Report

Various corrections are needed in order to extract the best value of the measurements from the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) User Facility’s scanning precipitation radars. The Corrected Moments in Antenna Coordinates (CMAC) Value-Added Product provides an application chain for providing radar moments that are corrected for artifacts such as aliasing, attenuation, multi-trip echoes, and beam blockage. This technical report provides details on the entire process of correcting the ARM scanning precipitation radar data using CMAC. CMAC has been used at multiple ARM sites and ARM Mobile Facility deployments including the Tracking Aerosol Convection Interactions Experiment (TRACER), Cloud, Aerosol, and Complex Terrain Interactions (CACTI), and the Surface Atmosphere Integrated Laboratory (SAIL).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Assessing the vertical structure of Arctic aerosols using balloon-borne measurements

The rapidly warming Arctic is sensitive to perturbations in the surface energy budget, which can be caused by clouds and aerosols. However, the interactions between clouds and aerosols are poorly quantified in the Arctic, in part due to (1) limited observations of vertical structure of aerosols relative to clouds and (2) ground-based observations often being inadequate for assessing aerosol impacts on cloud formation in the characteristically stratified Arctic atmosphere. Here, we present a novel evaluation of Arctic aerosol vertical distributions using almost 3 years' worth of tethered balloon system (TBS) measurements spanning multiple seasons. The TBS was deployed at the U.S. Department of Energy Atmospheric Radiation Measurement Program's facility at Oliktok Point, Alaska. Aerosols were examined in tandem with atmospheric stability and ground-based remote sensing of cloud macrophysical properties to specifically address the representativeness of near-surface aerosols to those at cloud base. Based on a statistical analysis of the TBS profiles, ground-based aerosol number concentrations were unequal to those at cloud base 86 % of the time. Intermittent aerosol layers were observed 63 % of the time due to poorly mixed below-cloud environments, mostly found in the spring, causing a decoupling of the surface from the cloud layer. A uniform distribution of aerosol below cloud was observed only 14 % of the time due to a well-mixed below-cloud environment, mostly during the fall. The equivalent potential temperature profiles of the below-cloud environment reflected the aerosol profile 89 % of the time, whereby a mixed or stratified below-cloud environment was observed during a uniform or layered aerosol profile, respectively. In general, a combination of aerosol sources, thermodynamic structure, and wet removal processes from clouds and precipitation likely played a key role in establishing observed aerosol vertical structures. Results such as these could be used to improve future parameterizations of aerosols and their impacts on Arctic cloud formation and radiative properties.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

An attribution of the low single-scattering albedo of biomass burning aerosol over the southeastern Atlantic

Abstract. Aerosol over the remote southeastern Atlantic is some of the most sunlight-absorbing aerosol on the planet: the in situ free-tropospheric single-scattering albedo at the 530 nm wavelength (SSA530 nm) ranges from 0.83 to 0.89 within ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) aircraft flights from late August–September. Here we seek to explain the low SSA. The SSA depends strongly on the black carbon (BC) number fraction, which ranges from 0.15 to 0.4. Low organic aerosol (OA)-to-BC mass ratios of 8–14 and modified combustion efficiency values >0.975 point indirectly to the dry, flame-efficient combustion of primarily grass fuels, with back trajectories ending in the miombo woodlands of Angola. The youngest aerosol, aged 4–5 d since emission, occupied the top half of a 5 km thick plume sampled directly west of Angola with a vertically consistent BC:ΔCO (carbon monoxide) ratio, indicating a homogenization of the source emissions. The younger aerosol, transported more quickly off of the continent by stronger winds, overlaid older, slower-moving aerosol with a larger mean particle size and fraction of BC-containing particles. This is consistent with ongoing gas condensation and the coagulation of smaller non-BC particles upon the BC-containing particles. The particle volumes and OA:BC mass ratios of the older aerosol were smaller, attributed primarily to evaporation following fragmentation, instead of dilution or thermodynamics. The CLARIFY (CLoud–Aerosol–Radiation Interaction and Forcing: Year 2017) aircraft campaign sampled aerosols that had traveled further to reach the more remote Ascension Island. CLARIFY reported higher BC number fractions, lower OA:BC mass ratios, and lower SSA yet larger mass absorption coefficients compared to this study's. Values from one ORACLES 2017 flight, held midway to Ascension Island, are intermediate, confirming the long-range changes. Overall the data are most consistent with continuing oxidation through fragmentation releasing aerosols that subsequently enter the gas phase, reducing the OA mass, rather than evaporation through dilution or thermodynamics. The data support the following best fit: SSA530nm=0.801+0055⋅(OA:BC) (r=0.84). The fires of southern Africa emit approximately one-third of the world's carbon; the emitted aerosols are distinct from other regional smoke emissions, and their composition needs to be represented appropriately to realistically depict regional aerosol radiative effects.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2023

Overview and Statistical Analysis of Boundary Layer Clouds and Precipitation Over the Western North Atlantic Ocean

Due to their fast evolution and large natural variability in macro- and microphysical properties, the accurate representation of boundary layer clouds in current climate models remains a challenge. One of the regions with large intermodel spread in the Coupled Model Intercomparison Project Phase 6 ensemble is the western North Atlantic Ocean. Here, statistically representative in situ measurements can help to develop and constrain the parameterization of clouds in global models. To this end, we performed comprehensive measurements of boundary layer clouds, aerosol, trace gases, and radiation in the western North Atlantic Ocean during the NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) mission. In total, 174 research flights with 574 flight hours for cloud and precipitation measurements were performed with the HU-25 Falcon during three winter (February–March 2020, January–April 2021, and November 2021–March 2022) and three summer seasons (August–September 2020, May–June 2021, and May–June 2022). Here we present a statistical evaluation of 16 140 individual cloud events probed by the fast cloud droplet probe and the two-dimensional stereo cloud probe during 155 research flights in a representative and repetitive flight strategy allowing for robust statistical data analyses. We show that the vertical profiles of distributions of the liquid water content and the cloud droplet effective diameter (ED) increase with altitude in the marine boundary layer. Due to higher updraft speeds, higher cloud droplet number concentrations (N liquid ) were measured in winter compared to summer despite lower cloud condensation nucleus abundance. Flight cloud cover derived from statistical analysis of in situ data is reduced in summer and shows large variability. This seasonal contrast in cloud coverage is consistent with a dominance of a synoptic pattern in winter that favors conditions for the formation of stratiform clouds at the western edge of cyclones (post-cyclonic). In contrast, a dominant summer anticyclone is concomitant with the occurrence of shallow cumulus clouds and lower cloud coverage. The evaluation of boundary layer clouds and precipitation in the N liquid ED phase space sheds light on liquid, mixed-phase, and ice cloud properties and helps to categorize the cloud data. Ice and liquid precipitation, often masked in cloud statistics by a high abundance of liquid clouds, is often observed throughout the cloud. The ACTIVATE in situ cloud measurements provide a wealth of cloud information useful for assessing airborne and satellite remote-sensing products, for global climate and weather model evaluations, and for dedicated process studies that address precipitation and aerosol–cloud interactions.

Aerosol↗
NASA NTRS2021

Joint cloud water path and rainwater path retrievals from airborne ORACLES observations

This study presents a new algorithm that combines W-band reflectivity measurements from the Airborne Precipitation Radar – third generation (APR-3) passive radiometric cloud optical depth and effective radius retrievals from the Research Scanning Polarimeter (RSP) to estimate total liquid water path in warm clouds and identify the contributions from cloud water path (CWP) and rainwater path (RWP). The resulting CWP estimates are primarily determined by the optical depth input, although reflectivity measurements contribute ∼10 %–50 % of the uncertainty due to attenuation through the profile. Uncertainties in CWP estimates across all conditions are 25 % to 35 %, while RWP uncertainty estimates frequently exceed 100 %. Two-thirds of all radar-detected clouds observed during the ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) campaign that took place from 2016–2018 over the southeast Atlantic Ocean have CWP between 41 and 168 g/sq. m and almost all CWPs (99 %) between 6 to 445 g/sq. m. RWP, by contrast, typically makes up a much smaller fraction of total liquid water path (LWP), with more than 70 % of raining clouds having less than 10 g/sq. m of rainwater. In heavier warm rain (i.e., rain rate exceeding 40 mm/h or 1000 mm/d), however, RWP is observed to exceed 2500 g/sq. m. CWP (RWP) is found to be approximately 30 g/sq. m (7 g/sq. m) larger in unstable environments compared to stable environments. Surface precipitation is also more than twice as likely in unstable environments. Comparisons against in situ cloud microphysical probe data spanning the range of thermodynamic stability and meteorological conditions encountered across the southeast Atlantic basin demonstrate that the combined APR-3 and RSP dataset enable a robust joint cloud–precipitation retrieval algorithm to support future ORACLES precipitation susceptibility and cloud–aerosol–precipitation interaction studies.

algorithm↗
NASA NTRSDate not supplied

Distribution and Sources of Tropospheric Aerosols Over the Western North Atlantic During ACTIVATE (February-March 2020)

The Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) is a five-year (2019-2023) NASA Earth-Venture Suborbital-3 (EVS-3) mission to robustly characterize aerosol-cloud-meteorology interactions during February-June, with a focus on marine boundary layer clouds. This characterization requires understanding of aerosol composition, distribution, transport pathways, and sources. Here we use the GEOS-Chem chemical transport model driven by the MERRA-2 reanalysis to simulate tropospheric carbon monoxide (CO) and aerosols over the western North Atlantic Ocean (WNAO) during the first field deployment of ACTIVATE (February-March 2020). CO is used as a tracer to diagnose transport pathways for continental pollution outflow to the WNAO. The aerosol simulation represents all major aerosols including sulfate-nitrate-ammonium (SNA), mineral dust, sea salt, black and organic carbon aerosols. Model-simulated mixing ratios of SNA and organic carbon are compared with aircraft observations. We show that intensive aerosol mass measurements in the lower troposphere over the North American outflow region during ACTIVATE provide strong constraints on model aerosol wet scavenging. Comparisons of model aerosol extinctions with the airborne High Spectral Resolution Lidar-2 (HSRL-2) measurements indicate that the model generally captures continental outflow of aerosols and enhanced extinctions associated with sea salt. Simulated aerosol optical depths (AODs) and extinction vertical profiles are also compared with satellite retrievals from MODIS/Aqua and CALIOP/CALIPSO, respectively. CALIOP sometimes observes enhanced aerosol extinction at altitudes between ~1.5km and ~2.0km south of 32°N. The model reproduces this enhancement and attributes it to coarse-mode sea salt associated with high relative humidity. The relative contributions of continental and oceanic sources to the aerosol loading, AOD, and their distributions over the study domain will also be discussed.

aerosols↗
NASA NTRS2020

Saharan Dust Aerosols Change Deep Convective Cloud Prevalence, Possibly by Inhibiting Marine New Particle Formation

Deep convective clouds (DCCs) are important to global climate, atmospheric chemistry, and precipitation. Dust, a dominant aerosol type over the tropical North Atlantic, has potentially large microphysical impacts on DCCs over this region. However, dust effects are difficult to identify, being confounded by co-varying meteorology and other factors. Here, a method is developed to quantify DCC responses to dust and other aerosols at large spatial and temporal scales despite these uncertainties. Over 7 million tropical North Atlantic cloud, aerosol, and meteorological profiles from CloudSat satellite data and MERRA-2 reanalysis products are used to stratify cloud observations into meteorological regimes, objectively select a priori assumptions, and iteratively test uncertainty sensitivity. Dust is robustly associated with a 54% increase in DCC prevalence. However, marine aerosol proxy concentrations are five times more predictive of dust-associated increases in DCC prevalence than the dust itself, or any other aerosol or meteorological factor. Marine aerosols are also the most predictive factor for the even larger increases in DCC prevalence (61-87%) associated with enhanced dimethyl sulfide and combustion and sulfate aerosols. Dust-associated increases in DCC prevalence are smaller at high dust concentrations than at low concentrations. These observations suggest that not only is dust a comparatively ineffective CCN source, but it may also act as a condensation/coagulation sink for chemical precursors to CCN, reducing total CCN availability over large spatial scales by inhibiting new particle formation from marine emissions. These observations represent the first time this rocess, previously predicted by models, is supported and quantified by measurements.

Aerosol-cloud interactions↗
DOE OSTI2024

ARM Cloud and Precipitation Measurements and Science Group (CPMSG) 2024 Workshop Report

The mission of the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility is to improve the understanding and representation of cloud and aerosol processes and their interaction with the Earth's surface in Earth system models (ESMs) by providing comprehensive field observations and supporting advanced data analytics. The ARM Cloud and Precipitation Measurements and Science Group (CPMSG) was chartered in March 2019 to help improve the performance and scientific impact of ARM measurements of clouds and precipitation. The group aims to identify and address gaps in measurement capabilities, maximize the scientific impact of ARM data, and effectively serve the scientific community. To achieve these goals, the group includes experts in cloud and precipitation science, as well as representatives from ARM infrastructure, including instrument mentors, engineers, data quality officers, and data product translators. Prior to CPMSG, early discussions on cloud and precipitation measurements primarily focused on improving radar systems, but have since evolved to include a broader scope involving radiometers and other instruments. Since its formation, the CPMSG has gathered feedback using science traceability matrices. CPMSG aims to keep these as living documents to show the measurement needs, scientific drivers, roadblocks, maturity of measurements and retrievals, and pathways to model improvements. The group meets quarterly to discuss and prioritize measurement and operational improvements.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Ice Nucleating Particles, Aerosols and Clouds over the Higher Latitude Southern Ocean

Improved understanding of aerosol-cloud-precipitation interactions is a key goal of the DOE-ASR program. Ice Nucleating Particles (INPs) are rare aerosol particles that trigger ice formation in clouds. By doing so they may initiate precipitation in clouds, and this impacts cloud lifetime. Nowhere may the role of INPs be manifested so dramatically as in the Southern Ocean (SO). This vast region was the focus of the DOE-ARM MARCUS (Measurement of Aerosols, Radiation and CloUds over the Southern Oceans) and MICRE (Macquarie Island Cloud and Radiation Experiment) campaigns. In the SO, a deficit of INPs has been a leading hypothesis for why liquid clouds persist, which underlays the bias of global climate models in predicting excess shortwave radiation reaching the ocean surface between 55°S and Antarctica. In this study, we used the 6-month acquisition of INP data on four MARCUS cruises from Hobart, Tasmania, to Antarctica, and the single-location full annual INP cycle observed in MICRE, to gain a holistic, quantitative picture of the INP number concentrations as a function of temperature and their variability over SO latitudes from 43°S to Antarctica. Augmenting initial processing of filter collections of aerosol particles during MARCUS and MICRE, additional freezing studies following thermal treatment (to removes INPs associated with microbes) and peroxide treatment (to remove all organics), as well as ionic chemistry and total organic carbon analysis, were applied to samples to improve time and space resolution, and differentiate marine from terrestrial contributions. We also performed Next Generation Sequencing to determine that bacterial composition can tag periods of enhanced and degraded marine organic INPs and the relative lack of occurrence of land-sourced bio-particles. Through these and other analyses, INP data were categorized into representative source types (e.g., marine versus terrestrially-influenced). The products of our analyses are being used to parameterize ice formation for use in numerical modeling studies to determine if, and when, ocean-derived INPs control the microphysical composition and radiative balance of SO clouds in a manner not presently captured by global models. The specific objectives and approaches proposed were largely accomplished, including: 1) Additional and value-added chemical and biological analyses of archived samples of aerosols were completed to categorize and quantify INP types and concentrations over the SO. 2) Analyses were completed to place INP data in meteorological and aerosol context. 3) Sea spray aerosol INPs were demonstrated to dominate the SO region in all but episodic events. 4) New parameterizations for INP sources relevant to the SO were constructed. 5) Collaborative modeling studies demonstrating the crucial role of INPs in determining cloud radiative and precipitation properties were conducted with MARCUS and MICRE partners. Collaborative publication submissions in this regard ensued within the two year study. This work will advance the science of interactions of aerosols, clouds and precipitation, to improve their representation in regional and global climate models. Results have informed representation of primary ice crystal nucleation, give inference to the role of secondary processes, and improve investigations of aerosol influences on clouds via ice nucleation over SO high latitudes and similar vast ocean regions. Application will improve representation of such interactions for clouds in both regional and global climate models. The data base and analyses methods applied will continue to serve research studies in the future.

58 GEOSCIENCES↗
DOE OSTI2021

Observations of Clouds, Aerosols, Precipitation, and Surface Radiation over the Southern Ocean: An Overview of CAPRICORN, MARCUS, MICRE, and SOCRATES

Weather and climate models are challenged by uncertainties and biases in simulating Southern Ocean (SO) radiative fluxes that trace to a poor understanding of cloud, aerosol, precipitation, and radiative processes, and their interactions. Projects between 2016 and 2018 used in situ probes, radar, lidar, and other instruments to make comprehensive measurements of thermodynamics, surface radiation, cloud, precipitation, aerosol, cloud condensation nuclei (CCN), and ice nucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase clouds common to this pristine environment. Data including soundings were collected from the NSF–NCAR G-V aircraft flying north–south gradients south of Tasmania, at Macquarie Island, and on the R/V Investigator and RSV Aurora Australis. Synergistically these data characterize boundary layer and free troposphere environmental properties, and represent the most comprehensive data of this type available south of the oceanic polar front, in the cold sector of SO cyclones, and across seasons. Results show largely pristine environments with numerous small and few large aerosols above cloud, suggesting new particle formation and limited long-range transport from continents, high variability in CCN and cloud droplet concentrations, and ubiquitous supercooled water in thin, multilayered clouds, often with small-scale generating cells near cloud top. These observations demonstrate how cloud properties depend on aerosols while highlighting the importance of dynamics and turbulence that likely drive heterogeneity of cloud phase. Satellite retrievals confirmed low clouds were responsible for radiation biases. Furthermore, the combination of models and observations is examining how aerosols and meteorology couple to control SO water and energy budgets.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2022

Measurement report: Closure Analysis of Aerosol–cloud Composition in Tropical Maritime Warm Convection

Cloud droplet chemical composition is a key observable property that can aid understanding of how aerosols and clouds interact. As part of the Clouds, Aerosols and Monsoon Processes – Philippines Experiment (CAMP2Ex), three case studies were analyzed involving collocated airborne sampling of relevant clear and cloudy air masses associated with maritime warm convection. Two of the cases represented a polluted marine background, with signatures of transported East Asian regional pollution, aged over water for several days, while the third case comprised a major smoke transport event from Kalimantan fires. Sea salt was a dominant component of cloud droplet composition, in spite of fine particulate enhancement from regional anthropogenic sources. Furthermore, the proportion of sea salt was enhanced relative to sulfate in rainwater and may indicate both a propensity for sea salt to aid warm rain production and an increased collection efficiency of large sea salt particles by rain in subsaturated environments. Amongst cases, as precipitation became more significant, so too did the variability in the sea salt to (non-sea salt) sulfate ratio. Across cases, nitrate and ammonium were fractionally greater in cloud water than fine-mode aerosol particles; however, a strong covariability in cloud water nitrate and sea salt was suggestive of prior uptake of nitrate on large salt particles. A mass-based closure analysis of non-sea salt sulfate compared the cloud water air-equivalent mass concentration to the concentration of aerosol particles serving as cloud condensation nuclei for droplet activation. While sulfate found in cloud was generally constrained by the sub-cloud aerosol concentration, there was significant intra-cloud variability that was attributed to entrainment – causing evaporation of sulfate-containing droplets –and losses due to precipitation. In addition, precipitation tended to promote mesoscale variability in the sub-cloud aerosol through a combination of removal, convective downdrafts, and dynamically driven convergence. Physical mechanisms exerted such strong control over the cloud water compositional budget that it was not possible to isolate any signature of chemical production/loss using in-cloud observations. The cloud-free environment surrounding the non-precipitating smoke case indicated sulfate enhancement compared to convective mixing quantified by a stable gas tracer; however, this was not observed in the cloud water (either through use of ratios or the mass closure), perhaps implying that the warm convective cloud timescale was too short for chemical production to be a leading-order budgetary term and because precursors had already been predominantly exhausted. Closure of other species was truncated by incomplete characterization of coarse aerosol (e.g., it was found that only 10 %–50% of sea salt mass found in cloud was captured during clear-air sampling) and unmeasured gasphase abundances affecting closure of semi-volatile aerosol species (e.g., ammonium, nitrate and organic) and soluble volatile organic compound contributions to total organic carbon in cloud water.

Ewan Crosbie↗
NASA NTRS2005

A New Approach to using a Cloud-Resolving Model to Study the Interactions between Clouds, Precipitation and Aerosols

Numerical cloud models, which are based the non-hydrostatic equations of motion, have been extensively applied to cloud-scale and mesoscale processes during the past four decades. Because cloud-scale dynamics are treated explicitly, uncertainties stemming from convection that have to be parameterized in (hydrostatic) large-scale models are obviated, or at least mitigated, in cloud models. Global models will use the non-hydrostatic framework when their horizontal resolution becomes about 10 kilometers, the theoretical limit for the hydrostatic approximation. This juncture will be reached one to two decades from now. Over the past generation, voluminous datasets on atmospheric convection have been accumulated from radar, instrumented aircraft, satellites, and rawinsonde measurements in field campaigns, enabling the detailed evaluation of models. Improved numerical methods have resulted in more accurate and efficient dynamical cores in models. Improvements have been made in the parameterizations of microphysical processes, radiation, boundary-layer effects, and turbulence; however, microphysical parameterizations remain a major source of uncertainty in all classes of atmospheric models. In recent years, exponentially increasing computer power has extended cloud-resolving-model integrations from hours to months, the number of computational grid points from less than a thousand to close to ten million. Three-dimensional models are now more prevalent. Much attention is devoted to precipitating cloud systems where the crucial 1-kilometer scales are resolved in horizontal domains as large as 10,000 kilometers in two dimensions, and 1,000 x 1,000 square kilometers in three-dimensions. Cloud models now provide statistical information useful for developing more realistic physically-based parameterizations for climate models and numerical weather prediction models. A review of developments and applications of cloud models in the past, present and future will be presented in this talk. In particular, a new approach to using cloud-resolving models to study the interactions between clouds, precipitation and aerosols will be presented.

Tao, Wei-Kuo↗
NASA NTRS2005

A New Approach to Using a Cloud-resolving Model to Study the Interactions Between Clouds, Precipitation and Aerosols

Numerical cloud models, which are based the non-hydrostatic equations of motion, have been extensively applied to cloud-scale and mesoscale processes during the past four decades. Because cloud-scale dynamics are treated explicitly, uncertainties stemming from convection that have to be parameterized in (hydrostatic) large-scale models are obviated, or at least mitigated, in cloud models. Global models will use the non-hydrostatic framework when their horizontal resolution becomes about 10 km, the theoretical limit for the hydrostatic approximation. This juncture will be reached one to two decades from now. Over the past generation, voluminous datasets on atmospheric convection have been accumulated from radar, instrumented aircraft, satellites, and rawinsonde measurements in field campaigns, enabling the detailed evaluation of models. Improved numerical methods have resulted in more accurate and efficient dynamical cores in models. Improvements have been made in the parameterizations of microphysical processes, radiation, boundary-layer effects, and turbulence; however, microphysical parameterizations remain a major source of uncertainty in all classes of atmospheric models. In recent years, exponentially increasing computer power has extended cloud-resolving-model integrations from hours to months, the number of computational grid points from less than a thousand to close to ten million. Three-dimensional models are now more prevalent. Much attention is devoted to precipitating cloud systems where the crucial 1-km scales are resolved in horizontal domains as large as l0,OOO km in two-dimensions, and 1,OOO x 1,OOO km2 in three-dimensions. Cloud models now provide statistical information useful for developing more realistic physically-based parameterizations for climate models and numerical weather prediction models. A review of developments and applications of cloud models in the past, present and future will be presented in this talk. In particular, a new approach to using cloud-resolving models to study the interactions between clouds, precipitation and aerosols will be presented.

Tao, Wei-Kuo↗
NASA NTRS2005

A New Approach to using a Cloud-Resolving Model to Study the Interactions between Clouds, Precipitation and Aerosols

Numerical cloud models, which are based the non-hydrostatic equations of motion, have been extensively applied to cloud-scale and mesoscale processes during the past four decades. Because cloud-scale dynamics are treated explicitly, uncertainties stemming from convection that have to be parameterized in (hydrostatic) large-scale models are obviated, or at least mitigated, in cloud models. Global models will use the non-hydrostatic framework when their horizontal resolution becomes about 10 km, the theoretical limit for the hydrostatic approximation. This juncture will be reached one to two decades from now. Over the past generation, voluminous datasets on atmospheric convection have been accumulated from radar, instrumented aircraft, satellites, and rawinsonde measurements in field campaigns, enabling the detailed evaluation of models. Improved numerical methods have resulted in more accurate and efficient dynamical cores in models. Improvements have been made in the parameterizations of microphysical processes, radiation, boundary-layer effects, and turbulence; however, microphysical parameterizations remain a major source of uncertainty in all classes of atmospheric models. In recent years, exponentially increasing computer power has extended cloud-resolving-model integrations from hours to months, the number of computational grid points from less than a thousand to close to ten million. Three-dimensional models are now more prevalent. Much attention is devoted to precipitating cloud systems where the crucial 1-km scales are resolved in horizontal domains as large as 10,000 km in two-dimensions, and 1,000 x 1,000 square kilometers in three-dimensions. Cloud models now provide statistical information useful for developing more realistic physically-based parameterizations for climate models and numerical weather prediction models. A review of developments and applications of cloud models in the past, present and future will be presented in this talk. In particular, a new approach to using cloud-resolving models to study the interactions between clouds, precipitation and aerosols will be presented.

Tao, Wei-Kuo↗
NASA NTRS2022

Remote Sensing of Aerosol Water Fraction, Dry Size Distribution and Soluble Fraction Using Multi-Angle, Multi-Spectral Polarimetry

A framework to infer volume water fraction, soluble fraction and dry size distributions of fine-mode aerosol from multi-angle, multi-spectral polarimetry retrievals of column-averaged ambient aerosol properties is presented. The method is applied to observations of the Research Scanning Polarimeter (RSP) obtained during two NASA aircraft campaigns, namely the Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) and the Cloud, Aerosol, and Monsoon Processes Philippines Experiment (CAMP2Ex). All aerosol retrievals are statistically evaluated using in situ data. Volume water fraction is inferred from the retrieved ambient real part of the refractive index, assuming a dry refractive index of 1.54 and by applying a volume mixing rule to obtain the effective ambient refractive index. The uncertainties in inferred volume water fraction resulting from this simplified model are discussed and estimated to be lower than 0.2 and decreasing with increasing volume water fraction. The daily mean retrieved volume water fractions correlate well with the in situ values with a mean absolute difference of 0.09. Polarimeter-retrieved ambient effective radius for daily data is shown to increase as a function of volume water fraction as expected. Furthermore, the effective variance of the size distributions also increases with increasing effective radius, which we show is consistent with an external mixture of soluble and insoluble aerosol. The relative variations of effective radius and variance over an observation period are then used to estimate the soluble fraction of the aerosol. Daily results of soluble fraction correlate well with in situ-observed sulfate mass fraction with a correlation coefficient of 0.79. Subsequently, inferred water and soluble fractions are used to derive dry fine-mode size distributions from their ambient counterparts. While dry effective radii obtained in situ and from RSP show similar ranges, in situ values are generally substantially smaller during the ACTIVATE deployments, which may be due to biases in RSP retrievals or in the in situ observations, or both. Both RSP and in situ observations indicate the dominance of aerosol with low hygroscopicity during the ACTIVATE and CAMP2Ex campaigns. Furthermore, RSP indicates a high degree of external mixing of particles with low and high hygroscopicity. These retrievals of fine-mode water volume fraction and soluble fraction may be used for the evaluation of water uptake in atmospheric models. Furthermore, the framework allows us to estimate the variation in the concentration of fine-mode aerosol larger than a specific dry radius limit, which can be used as a proxy for the variation in cloud condensation nucleus concentrations. This framework may be applied to multi-angle, multi-spectral satellite data expected to be available in the near future.

Amount of water in particulate matter↗
NASA NTRS2010

A Global Modeling Study on Carbonaceous Aerosol Microphysical Characteristics and Radiative Effects

Recently, attention has been drawn towards black carbon aerosols as a short-term climate warming mitigation candidate. However the global and regional impacts of the direct, indirect and semi-direct aerosol effects are highly uncertain, due to the complex nature of aerosol evolution and the way that mixed, aged aerosols interact with clouds and radiation. A detailed aerosol microphysical scheme, MATRIX, embedded within the GISS climate model is used in this study to present a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative effects. Our best estimate for net direct and indirect aerosol radiative flux change between 1750 and 2000 is -0.56 W/m2. However, the direct and indirect aerosol effects are quite sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative flux change can vary between -0.32 to -0.75 W/m2 depending on these carbonaceous particle properties at emission. Taking into account internally mixed black carbon particles let us simulate correct aerosol absorption. Absorption of black carbon aerosols is amplified by sulfate and nitrate coatings and, even more strongly, by organic coatings. Black carbon mitigation scenarios generally showed reduced radiative fluxeswhen sources with a large proportion of black carbon, such as diesel, are reduced; however reducing sources with a larger organic carbon component as well, such as bio-fuels, does not necessarily lead to a reduction in positive radiative flux.

Bauer, S. E.↗