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At least 451 records · Page 25

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DOE OSTI2022

Phonon‐Dominated Energy Transport in Purely Metallic Heterostructures

Abstract Ultrafast X‐ray diffraction is used to quantify the transport of energy in laser‐excited nanoscale gold–nickel (Au–Ni) bilayers. Electron transport and efficient electron–phonon coupling in Ni convert the laser‐deposited energy in the conduction electrons within a few picoseconds into a strong non‐equilibrium between hot Ni and cold Au phonons at the bilayer interface. Modeling of the subsequent equilibration dynamics within various two‐temperature models confirms that for ultrathin Au films, the thermal transport is dominated by phonons instead of conduction electrons because of the weak electron–phonon coupling in Au.

36 MATERIALS SCIENCE↗

DOE OSTI2019

CWDM transmit module for wavelength tuning and tracking

A photonic integrated circuit (PIC) includes a semiconductor substrate with a main bus waveguide disposed within the substrate. Two or more ring lasers are disposed within the substrate and are optically coupled to the main bus waveguide. The ring lasers have a wavelength control mechanism allowing change of a lasers emitted wavelength. A wavelength selective filter is optically coupled to the bus waveguide. A control circuit is electronically coupled to each wavelength control mechanism, and the wavelength selective filter. The control circuit in conjunction with the selective filter allows monitoring of a ring laser's wavelength on the main bus waveguide. Based on a determined wavelength, the control circuit may change a ring laser wavelength to a desired wavelength to achieve a desired wavelength spacing for each of the ring lasers. The PIC may be integrated as a coarse wave-length division multiplexing (CWDM) transmit module.

42 ENGINEERING↗

NASA NTRS1975

Development of a monolithic GaAs integrated optical transmitter

The paper discusses a program designed for the development of a GaAs IOC transmitter consisting of a monolithic surface laser whose output is coupled into patterned channel waveguides. Modulation and switching of the radiation occur in the waveguide circuit and are controlled separately. These structures are to be fabricated monolithically on a single semiconductor chip with each device amenable to integrated low-cost manufacture. The waveguide outputs of the IOC transmitter will be coupled to single mode optical fibers which form a transmission cable. The properties of the semiconductors (Ga,Al)As and (Ga,In)As permit performance of each of the basic functions included in the device considered. The concept of monolithic nondiscrete GaAs diode lasers is examined along with optical stripline channel waveguides and electro-optic channel waveguide modulators and switches.

Blum, F. A.↗

NASA NTRS2001

Laser Absorption Measurements of Equivalence Ratios Studied Along With Their Coupling to Pressure Fluctuations in Lean Premixed Prevaporized (LPP) Combustion

Concerns about damaging the Earth's ozone layer as a result of high levels of nitrogen oxides (known collectively as NOx) from high-altitude, high-speed aircraft have prompted the study of lean premixed prevaporized (LPP) combustion in aircraft engines. LPP combustion reduces NOx emissions principally by reducing the peak flame temperatures inside an engine. Recent advances in LPP technologies have realized exceptional reductions in pollutant emissions (single-digit ppm NOx for example). However, LPP combustion also presents major challenges: combustion instability and dynamic coupling effects between fluctuations in heat-release rate, dynamic pressure, and fuel pressure. These challenges are formidable and can literally shake an engine apart if uncontrolled. To better understand this phenomenon so that it can be controlled, we obtained real-time laser absorption measurements of the fuel vapor concentration (and equivalence ratio) simultaneously with the dynamic pressure, flame luminosity, and time-averaged gaseous emissions measurements in a research-type jet-A-fueled LPP combustor. The measurements were obtained in NASA Glenn Research Center's CE-5B optically accessible flame tube facility. The CE-5B facility provides inlet air temperatures and pressures similar to the actual operating conditions of real aircraft engines. The laser absorption measurements were performed using an infrared 3.39 micron HeNe laser in conjunction with a visible HeNe laser for liquid droplet scattering compensation.

Nguyen, Quang-Viet↗

NASA NTRS2000

Progress in Laser Based Carbon Nanotube Production and In-Situ Diagnostics at NASA/JSC

This paper focuses on the improvement of carbon nanotube production with the upgraded laser system operating at 60 Hz. The yield has increased by about five times with the new system, while the quality of the single wall nanotube (SWNT) is unchanged. Recent diagnostic data of spatial and temporal evolution of C2 in the laser ablation plume are obtained by imaging the plume area on a gated change coupled device. A three-laser setup is used to monitor nickel atoms in different parts of the plume by laser induced fluorescence (LIF). Measurements are made at different times after the ablating lasers. These results, along with the previous measurements of emission and LIF of C2 will be discussed. Our ultimate goal is to use these measurements to model the nanotube growth mechanism.

Arepalli, Sivaram↗

DOE OSTI2020

Understanding asymmetries using integrated simulations of capsule implosions in low gas-fill hohlraums at the National Ignition Facility

Current capsule implosions at the National Ignition Facility (NIF) using high-density-carbon ablators and laser energies close to 2 MJ have shown neutron yields in excess of 50 kJ. Improving on this performance requires understanding of the different degradation mechanisms. For many NIF implosions, nuclear diagnostic signatures have inferred residual hot-spot velocities that correlate with fuel areal density variations consistent with a low-order mode-1 asymmetry. A current working hypothesis attributes these asymmetries to a combination of beam to beam variations in the laser delivery and possibly coupling to target features, such as the diagnostic holes needed for x-ray imaging. Recently, a new source has been identified, thickness variation in the ablator shell. To gain better understanding and eventually mitigate the causes of <ρR> asymmetries, 3D integrated simulations using the actual delivered laser powers are needed. To capture the effect of the diagnostic holes (DHs) using direct numerical simulation would require significantly large computational resources. Instead, our 3D simulations make use of a subgrid model developed using highly-resolved 2D simulations that include several details of the DH engineering complexity. Simulations of NIF shots using hohlraums without DHs, to isolate the effect of beam-to-beam variations, reproduce fairly well the observed nuclear diagnostic signatures. Similarly, reasonable agreement between data and simulations is also obtained in the presence of diagnostic holes. To account for the remaining discrepancies a sensitivity study of ablator thickness variation showed that 1% thickness asymmetries are comparable in effect to 1% peak drive mode-1 asymmetries. Furthermore, this study identified sensitivity to variations in the imbedded doped layer (needed to shield the DT ice from the high energy x-rays generated in the hohlraum) thickness even when the inner and outer surface of the ablator are perfectly spherical.

radiation hydrodynamics↗

NASA NTRS1989

Monolithic Arrays of Grating-Surface-Emitting Diode Lasers and Quantum Well Modulators for Optical Communications

The electro-optic switching properties of injection-coupled coherent 2-D grating-surface-emitting laser arrays with multiple gain sections and quantum well active layers are discussed and demonstrated. Within such an array of injection-coupled grating-surface-emitting lasers, a single gain section can be operated as intra-cavity saturable loss element that can modulate the output of the entire array. Experimental results demonstrate efficient sub-nanosecond switching of high power grading-surface-emitting laser arrays by using only one gain section as an intra-cavity loss modulator.

Carlson, N. W.↗

DOE OSTI2024

Enhancement of harmonic generation by an intense driving laser with high-order waveguide modes in a high-pressure gas-filled hollow waveguide

High-order harmonics have been widely used as reliable tabletop coherent radiation sources recently, but their applications have often been limited by the available pulse energy. Here, we report that by using an overdriven intense laser in a long waveguide with high-pressure gas, phase matching can be achieved in three distinct “regimes”. In the third regime, favorable phase matching is achieved at near-axis positions to enhance harmonic yields. Our results are supported by a full theoretical analysis, and we demonstrate that coupling of the driving laser with the high-order waveguide modes (instead of the fundamental mode used in most prior experiments) is responsible for achieving phase matching. Furthermore, we establish that this phase matching (and harmonic enhancement) is robust, and a scaling relation is derived for the necessary waveguide and gas parameters, allowing our predictions to be tested immediately in any laboratory today.

Li, Baochang [Nanjing University of Science and Te↗

NASA NTRS1973

Crystal motion measurement by means of satellite techniques

A system for monitoring precursory crustal motions is presented. It involves a set of automated corner reflector stations tracked by means of a laser operating in the Geopause satellite. It is possible to range some three times during every Geopause pass to each of the sites in such an ensemble, weather permitting. One centimeter range data gathered during a quarter of a year can yield position component accuracies of the order of a couple of centimeters. A laser beam of a tenth of a milliradian in diameter would, illuminate a single station in such an array. A broader beam would generate reflections from several sites, yielding overlapping data. A chain or pattern of such overlapping regions can strengthen the solution for site positions. Pressure, temperature and humidity gauges can provide refraction correction data. Turnaround transponders interrogated by the Geopause radio tracking system can furnish corresponding data in excessively cloudy regions.

Siry, J. W.↗

NASA NTRS1976

Numerical optimization of gasdynamic lasers

A sophisticated numerical optimization procedure has been coupled to a detailed theoretical model of the carbon dioxide gasdynamic laser (GDL) for the purpose of systematically evaluating the performance of these systems. The integrated model was used to predict the performance of a wide variety of combustion-driven gasdynamic lasers and was then used to maximize the theoretical available specific energy of these lasers. Up to six design variables and three nonlinear constraints were used in these optimizations, although the method is not limited to this number. Results are presented to show the performance of typical lasers before and after optimization. Improvements approaching a factor of two in the available specific energy are found, suggesting that numerical optimization techniques are valuable in improving the design of gasdynamic lasers.

Saunders, R. C., III↗

NASA NTRS1985

High-power diode lasers for optical communications applications

High-power, single-mode, double-heterojunction AlGaAs diode lasers are being developed to meet source requirements for both fiber optic local area network and free space communications systems. An individual device, based on the channeled-substrate-planar (CSP) structure, has yielded single spatial and longitudinal mode outputs of up to 90 mW CW, and has maintained a single spatial mode to 150 mW CW. Phase-locked arrays of closely spaced index-guided lasers have been designed and fabricated with the aim of multiplying the outputs of the individual devices to even higher power levels in a stable, single-lobe, anastigmatic beam. The optical modes of the lasers in such arrays can couple together in such a way that they appear to be emanating from a single source, and can therefore be efficiently coupled into optical communications systems. This paper will review the state of high-power laser technology and discuss the communication system implications of these devices.

Carlin, D. B.↗

NASA NTRS2000

New Techniques to Test Spin-Gravity Coupling with Atomic Clock

Recent advances in laser technology have produced the opportunity to realize more stable and accurate atomic clocks, by laser excitation, manipulation and cooling of atoms. In this paper we will describe a new scheme based on the use of lasers with atomic clocks to increase the sensitivity of experimental search for a spin-gravity coupling.

atomic clocks↗

DOE OSTI2019

Investigation of a passively Q-switched Raman laser at 1176 nm with Nd{sup 3+}:YAG/Cr{sup 4+}:YAG/YAG composite crystal and a coupled cavity

To reduce the thermal lens effect and increase the efficiency, a composite crystal of Nd{sup 3+}:YAG/Cr{sup 4+}:YAG/YAG and a coupled cavity structure were employed in our passively Q-switched YVO{sub 4}-based Raman laser system. Both the simulation and the experiment results showed that the undoped YAG crystal bonded in the end-face of Cr{sup 4+}:YAG crystal can speed up the heat transfer of Cr{sup 4+}:YAG crystal and reduce the temperature difference between its side surfaces and the center significantly, and the coupled cavity structure can improve the laser performance, especially at high pump power. The maximum output power of Raman laser of 0.92 W at 1176 nm was obtained with an optical-to-optical efficiency of 11.51%. The corresponding repetition rate and the pulse width is 53.5 kHz and 3.22 ns, respectively.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

NASA NTRS1991

Experimental investigation of a unique airbreathing pulsed laser propulsion concept

Investigations were conducted into unique methods of converting pulsed laser energy into propulsive thrust across a flat impulse surface under atmospheric conditions. The propulsion experiments were performed with a 1-micron neodymium-glass laser at the Space Plasma Branch of the Naval Research Laboratory. Laser-induced impulse was measured dynamically by ballistic pendulums and statically using piezoelectric pressure transducers on a stationary impulse surface. The principal goal was to explore methods for increasing the impulse coupling performance of airbreathing laser-propulsion engines. A magnetohydrodynamic thrust augmentation effect was discovered when a tesla-level magnetic field was applied perpendicular to the impulse surface. The impulse coupling coefficient performance doubled and continued to improve with increasing laser-pulse energies. The resultant performance of 180 to 200 N-s/MJ was found to be comparable to that of the earliest afterburning turbojets.

Myrabo, L. N.↗

DOE OSTI2023

Analytic gradients for relativistic exact-two-component equation-of-motion coupled-cluster singles and doubles method

A first implementation of analytic gradients for spinor-based relativistic equation-of-motion coupled-cluster singles and doubles method using an exact two-component Hamiltonian augmented with atomic mean-field spin–orbit integrals is reported. To demonstrate its applicability, we present calculations of equilibrium structures and harmonic vibrational frequencies for the electronic ground and excited states of the radium mono-amide molecule (RaNH 2 ) and the radium mono-methoxide molecule (RaOCH 3 ). Spin–orbit coupling is shown to quench Jahn–Teller effects in the first excited state of RaOCH 3 , resulting in a C 3v equilibrium structure. Furthermore, the calculations also show that the radium atoms in these molecules serve as efficient optical cycling centers.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

Ultrafast-induced coherent acoustic phonons in the two-dimensional magnet CrSBr

Magnetism in two-dimensional (2D) van der Waals (vdW) crystals offers promising new directions for low-dimensional physics and devices. In this work, mega-electron volt (MeV) ultrafast electron diffraction was employed to investigate the ultrafast atomic dynamics of a novel, 2D vdW magnetic single-crystal CrSBr. Femtosecond (fs) optical pump pulses excited non-equilibrium atomic displacements shown to be coherent acoustic phonons (CAPs). Phonon frequencies were extracted by analyzing oscillations of different Bragg peak (BP) intensities and were determined to be GHz acoustic disturbances that propagated as strain waves. Phonon modes exhibit anisotropy with respect to the a and b crystal axes. Subharmonic phonon frequencies were also observed, and this provided a signature of nonlinear oscillatory coupling between the laser-induced pumping phonon frequency and secondary phonon frequencies. Thus, CrSBr was found to serve as a nonlinear phononic frequency converter. The ultrafast time dependence of the Bragg intensity was simulated by incorporating an oscillating deviation parameter ansatz into expressions for the dynamical scattering intensity yielded excellent modeling of the ultrafast structural dynamics of the photo-excited 2D crystal. Our work provides a foundation for exploring how fs light pulses can influence phonon dynamics in materials with strong spin-lattice coupling. These results suggest that CAPs can match the magnon frequencies and show the promise of CrSBr for use in optical-to-microwave transducers and phononic devices.

43 PARTICLE ACCELERATORS↗

DOE OSTI2023

Femtosecond Laser-Induced Nano-Joining of Volatile Tellurium Nanotube Memristor

Nanowire/nanotube memristor devices provide great potential for random-access high-density resistance storage. However, fabricating high-quality and stable memristors is still challenging. This paper reports multileveled resistance states of tellurium (Te) nanotube based on the clean-room free femtosecond laser nano-joining method. The temperature for the entire fabrication process was maintained below 190 °C. A femtosecond laser joining technique was used to form nanowire memristor units with enhanced properties. Femtosecond (fs) laser-irradiated silver-tellurium nanotube-silver structures resulted in plasmonic-enhanced optical joining with minimal local thermal effects. This produced a junction between the Te nanotube and the silver film substrate with enhanced electrical contacts. Noticeable changes in memristor behavior were observed after fs laser irradiation. Capacitor-coupled multilevel memristor behavior was observed. Compared to previous metal oxide nanowire-based memristors, the reported Te nanotube memristor system displayed a nearly two-order stronger current response. The research displays that the multileveled resistance state is rewritable with a negative bias.

42 ENGINEERING↗

NASA NTRS1985

Modelling of Laser-Enhanced Chemical Vapor Deposition

Research is directed at development of a detailed model of mass and heat transfer and chemical reaction in the pyrolysis of silane for the growth of thin amorphous silicon substrates incorporating laser heating of the gas phase above the film. The model will be the basis for evaluation of the relative importances of the decomposition of SiH4 in the vapor phase, mass transfer of the intermediate species, e.g., SiH2, and the evolution of hydrogen gas. Plans are also underway for developing a model for homogeneous nucleation of Si in the vapor phase to model the rate limitations observed at high gas-phase temperatures and high partial pressures of silane. Work was concentrated on an almost one-dimensional model for the coupling of the CO2 laser beam for heat transfer of the vapor phase with simple kinetic models for SiH4 decomposition and subsequent absorption of Si vapor on the substrate. Mass transfer in the vapor phase is assumed to be solely by diffusion. The role of convection in the vapor phase caused by the large changes in density in and around the center of the laser beam will be analyzed to evaluate the potential of microgravity experiments for increasing the uniformity of the film and the deposition rate.

Brown, R. A.↗