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DOE OSTI2026

Theoretical Study of High Harmonic Generation in Monolayer NbSe 2

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond time scales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including transition-metal dichalcogenides (TMDs). Among TMDs, bulk NbSe 2 exhibits charge density wave (CDW) order below 33 K and becomes superconducting below 7.3 K. Monolayer NbSe 2 also has superconducting and CDW behavior and is therefore interesting as a material whose different structural and electronic properties could be probed via HHG. Here, we predict the HHG response of the pristine 2H and CDW phases of monolayer NbSe 2 using real-time time-dependent density functional theory under the application of a simulated laser pulse excitation. We find that due to the lack of inversion symmetry in both monolayer phases, it is possible to excite even harmonics and that the even harmonics appear as the transverse components of the current response under excitations polarized along the zigzag direction of the monolayer, while odd harmonics arise from the longitudinal current response in all excitation directions. This suggests that the even and odd harmonic responses can be controlled via the polarization of the probing field, opening an avenue for potentially useful applications in optoelectronic devices.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Automatic detection of methane emissions in multispectral satellite imagery using a vision transformer

Curbing methane emissions is among the most effective actions that can be taken to slow down global warming. However, monitoring emissions remains challenging, as detection methods have a limited quantification completeness due to trade-offs that have to be made between coverage, resolution and detection accuracy. Here we show that deep learning can overcome the trade-off in terms of spectral resolution that comes with multi-spectral satellite data, resulting in a methane detection tool with global coverage and high temporal and spatial resolution. We compare our detections with airborne methane measurement campaigns, which suggests that our method can detect methane point sources in Sentinel-2 data down to plumes of 0.01 km 2 , corresponding to 200 to 300 kg CH 4 /h -1 sources. Our model shows an order of magnitude improvement over the state-of-the-art, providing a significant step towards the automated, high resolution detection of methane emissions at a global scale, every few days.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

Bringing weak transitions to light

Abstract Weak transitions between quantum states are of fundamental importance for a broad range of phenomena from analytical biochemistry to precision physics, but generally challenge experimental detection. Due to their small cross sections scaling with the absolute square of their transition matrix elements, spectroscopic measurements often fail in particular in the presence of competing background processes. Here we introduce a general concept to break this scaling law and enhance the transition probability by exploiting a stronger laser-coupled pathway to the same excited state. We demonstrate the concept experimentally by attosecond transient absorption spectroscopy in helium atoms. The quasi-forbidden transitions from the ground state 1s 2 to the weakly coupled doubly excited 2p3dandsp 2,4− states are boosted by an order of magnitude. Enhancing single-photon-suppressed transitions can find widespread applicability, from spectral diagnostics of complex molecules in life and chemical sciences to precision spectroscopy of weak transitions in metastable atomic nuclei in the search for new physics.

Science & Technology - Other Topics↗

DOE OSTI2026

Mapping the Perseus galaxy cluster with XRISM: Gas kinematic features and their implications for turbulence

We present extended gas kinematic maps of the Perseus cluster based on a combination of five new XRISM/Resolve pointings observed in 2025 with four performance verification datasets from 2024, totaling a net exposure of 745 ks. To date, Perseus remains the only cluster that has been extensively mapped out to ≃0.7 r 2500 by XRISM/Resolve, while simultaneously offering sufficient spatial resolution to resolve gaseous substructures driven by mergers and active galactic nucleus (AGN) feedback. Our observations cover multiple radial directions and a broad range of dynamical scales, enabling us to characterize the kinematic properties of the intracluster medium up to a scale of ∼500 kpc. In the measurements, we detected high-velocity dispersions (≃300km s −1 ) in the eastern region of the cluster that are spatially coincident with the extended X-ray surface brightness excess and correspond to a nonthermal pressure fraction of ≃7 − 13%. The velocity field outside the AGN-dominant region can be effectively described by a single, large-scale kinematic driver based on the velocity structure function, which statistically favors an energy injection scale of at least a few hundred kpc. The estimated turbulent dissipation energy is comparable to the gravitational potential energy released by a recent merger, implying a significant role of turbulent cascade in the merger energy conversion. In the bulk velocity field, we observed a dipole-like pattern along the east-west direction with an amplitude of ≃ ± 200 − 300 km s −1 , indicating rotational motions induced by the recent merger event. This feature constrains the viewing direction to ≃30° −50° relative to the normal of the merger plane. Our hydrodynamic simulations suggest that Perseus has experienced at least two energetic mergers since redshift z ∼ 1, the most recent of which is associated with the radio galaxy IC310, in agreement with recent SRG/eROSITA findings. This study showcases exciting scientific opportunities for future missions with high-resolution spectroscopic capabilities (e.g., HUBS, LEM, and NewAthena).

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2026

Improving EV Charger Resiliency for MW Charging Systems

In this paper, the resiliency of a megawatt-scale EV charging station is investigated. Fault detection and tolerance methodologies are presented, based on monitoring the voltage offsets in DABs and switch-level currents in three-phase inverters, with the goal of maintaining operation at rated power during single faults and at reduced power under multiple fault conditions. To validate the effectiveness of the proposed strategy, simulation results at the rated 1 MW power of the charging station are carried out, followed by controller hardware-in-the-loop (CHIL) experiments on a 250 kW section of the station. The results highlight the feasibility of the integrated fault-tolerant methods for resilient, high-power EV charging infrastructure.

Adib, Aswad [ORNL] (ORCID:000000020997056X)↗

DOE OSTI2025

Vertical column dual-comb spectroscopy to a TBS

Open-path dual-frequency-comb spectroscopy (DCS) is a broadband, high spectral resolution, and high precision method for measuring gas concentrations over kilometer-scale paths. It has been used for detection and quantification of emissions of pollutants, hazardous gasses, and greenhouse gasses (GHGs). DCS has been shown to measure trace-gas mixing ratios with 0.14%-0.4% agreement between instruments. To achieve high signal-to-noise ratios (SNRs) with DCS, comb light is targeted onto a retroreflector at the end of the measurement path, which returns the signal to a detector co-located with the launch signal. Installing the retroreflector on a mobile platform such as a balloon or unmanned aerial vehicle (UAV) extends the capabilities of DCS by enabling variable path lengths, greater mobility, and access to higher altitudes. Mobile-target DCS has many uses in plume and leak detection, emissions modeling, and planetary boundary layer (PBL) studies. It is a promising method for observing vertical distributions of GHGs and mixing processes in the PBL, which are difficult to measure but important for pollution and climate monitoring as well as for understanding transport of gasses through the atmosphere. Tethered balloons are an intriguing platform because they enable longer flight durations and higher altitudes than easily obtainable with a UAV and thus allow for column measurements up to and above the PBL. New measurements completed in October/November 2024 reach the highest altitudes above ground level yet achieved by mobile-target DCS. For these measurements, the retroreflector was mounted on a 7 m diameter tethered helium balloon. An actively tracking gimbal on the ground holds the DCS launch telescope and keeps the 5 cm beam pointed onto the retroreflector while the balloon is lifted, lowered, and moved by wind and turbulence.

atmosphere↗

NASA NTRS1971

The Nimbus image dissector camera system - An evaluation of its meteorological applications.

Brief description of the electronics and operation of the Nimbus image dissector camera system (IDCS). The geometry and distortions of the IDCS are compared to the conventional AVCS camera on board the operational ITOS and ESSA satellites. The unique scanning of the IDCS provides for little distortion of the image, making it feasible to use a strip grid for the IDCS received in real time by local APT stations. The dynamic range of the camera favors the white end (high reflectance) of the gray scale. Thus, the camera is good for detecting cloud structure and ice features through brightness changes. Examples of cloud features, ice, and snow-covered land are presented. Land features, on the other hand, show little contrast. The 2600 x 2600 km coverage by the IDCS is adequate for the early detection of weather systems which may affect the local area. An example of IDCS coverage obtained by an APT station in midlatitudes is presented.

Sabatini, R. R.↗

NASA NTRS1972

Measurements of electron detection efficiencies in solid state detectors.

Detailed laboratory measurement of the electron response of solid state detectors as a function of incident electron energy, detector depletion depth, and energy-loss discriminator threshold. These response functions were determined by exposing totally depleted silicon surface barrier detectors with depletion depths between 50 and 1000 microns to the beam from a magnetic beta-ray spectrometer. The data were extended to 5000 microns depletion depth using the results of previously published Monte Carlo electron calculations. When the electron counting efficiency of a given detector is plotted as a function of energy-loss threshold for various incident energies, the efficiency curves are bounded by a smooth envelope which represents the upper limit to the detection efficiency. These upper limit curves, which scale in a simple way, make it possible to easily estimate the electron sensitivity of solid-state detector systems.

Lupton, J. E.↗

NASA NTRS1974

Land use mapping and modelling for the Phoenix Quadrangle

The author has identified the following significant results. Changes in the land use in the Phoenix (1:250,000 scale) Quadrangle in Arizona have been mapped using only the images from ERTS-1, tending to verify the utility of a land use classification system proposed for use with ERTS images. Seasonal changes were studied on successive ERTS-1 images, particularly large scale color composite transparencies for August, October, February, and May, and this seasonal variation aided delineation of land use boundaries. Types of equipment used to aid interpretation included color additive viewer, a twenty-power magnifier, a density slicer, and a diazo copy machine. A Zoom Transfer Scope was used for scale and photogrammetric adjustments. Types of changes detected have been: (1) cropland or rangeland developed as new residential areas; (2) rangeland converted to new cropland or to new reservoirs; and (3) possibly new activity by the mining industries. A map of land use previously compiled from air photos was updated in this manner. ERTS-1 images complemented air photos: the photos gave detail on a one-shot basis; the ERTS-1 images provided currency and revealed seasonal variation in vegetation which aided interpretation of land use.

Place, J. L.↗

NASA NTRS1975

Interdisciplinary application and interpretation of EREP data within the Susquehanna River Basin

The author has identified the following significant results. It has become that lineaments seen on Skylab and ERTS images are not equally well defined, and that the clarity of definition of a particular lineament is recorded somewhat differently by different interpreters. In an effort to determine the extent of these variations, a semi-quantitative classification scheme was devised. In the field, along the crest of Bald Eagle Mountain in central Pennsylvania, statistical techniques borrowed from sedimentary petrography (point counting) were used to determine the existence and location of intensely fractured float rock. Verification of Skylab and ERTS detected lineaments on aerial photography at different scales indicated that the brecciated zones appear to occur at one margin of the 1 km zone of brecciation defined as a lineament. In the Lock Haven area, comparison of the film types from the SL4 S190A sensor revealed the black and white Pan X photography to be superior in quality for general interpretation to the black and white IR film. Also, the color positive film is better for interpretation than the color IR film.

Mcmurtry, G. J.↗

NASA NTRS1979

A search for X-ray emission from rich clusters, extended halos around clusters, and superclusters

The all-sky data base acquired with the HEAO A-2 experiment was searched for X-ray emission on a variety of metagalactic size scales which were either predicted or previously detected. Results in the 0.2-60 keV energy range are presented. The optically richest clusters, including those from which a microwave decrement were observed, appear to be relatively underluminous in X-rays. Observations of Abell 576 show its luminosity to be less than earlier estimates, and moreover less than the luminosity predicted from its microwave decrement, unless the intracluster gas is a factor of approximately 10 hotter than in typical clusters. Near SC0627 there are two X-ray sources, and the identification of the dominant source with SCO627 is probably incorrect. New spectral observations of Abell 401 and 2147, possible superclusters, reveal that they have typical cluster spectra with iron line emission.

Pravdo, S. H.↗

NASA NTRS1981

Observed dynamics of superclusters

Radial velocity measurements of two large, rich superclusters show evidence of a gravitational slowing of the Hubble flow within the superclusters. Models assuming spherically symmetric, noncrossing mass shells yield mass density estimates for the clusters ranging from less than one to several times the critical density, and preliminary counts of galaxies and Abell clusters indicate a density enhancement within the superclusters of 10-71 times the field mass density. The combination of these two results is found to favor an open universe, assuming a standard Friedmann cosmology. It is noted that all forms of mass that are clumped on the scale of superclusters, or smaller, will be detected by these measurements, including neutrinos sufficiently massive to significantly contribute to the cosmological density parameter.

Harms, R. J.↗

NASA NTRS1986

The brightness variations of Comet Halley at large heliocentric distances

The reasons for the intrinsic brightness variations of up to 500 percent on time scales as short as a few hours detected by Sekanina (1984) in Comet Halley between October 1982 and February 1984 are discussed. It is shown that solar wind-modulated electrostatic dust blowoff from the night side of the comet is consistent with the observed brightness variations. The variations coincide with the encounter of high-speed streams with the comet. The stream's propagation time to the comet and the sun's rotation during this transit were used to locate the stream origin on the coronal surface, and the results are shown.

Flammer, K. R.↗

NASA NTRS1986

Solar Doppler shifts - Sources of continuous spectra

Oscillation observations can be used to study nonoscillatory solar phenomena that exhibit Doppler shifts. The paper discusses several effects of these phenomena and their associated temporal and spatial power spectra: (1) they limit the signal-to-noise ratio and sometimes detectability of oscillation modes; (2) there is the potential for better understanding and/or detection of solar phenomena; (3) large-scale convection may spatially modulate oscillation modes, leading to a continuous background spectrum; and (4) in regions of the spectrum where the resolution to separate modes is lacking one can determine upper limits for the integrated effects of modes.

Duvall, T. L., Jr.↗

NASA NTRS1988

The detection and interpretation of long-term changes in ozone from space

Long-term measurements of backscattered ultraviolet radiances, now being acquired by orbiting monochromators, will provide the basis for seeking trends in atmospheric ozone. The unambiguous detection of ozone trends on decadal time scales demands a data set that is essentially free of instrument drifts. Periodic flights of an ultraviolet monochromator on the space shuttle will provide an independent means of evaluating the long-term stability of identical instruments operating on free-flying satellites. A successful calibration of the free-flying sensors using the shuttle instrument places strict demands on calibration repeatability from one flight to the next. In addition, spatial and temporal variability in cloud cover could pose further complications in carrying out these in-flight calibrations.

Frederick, John E.↗

NASA NTRS1989

The detection and interpretation of long-term changes in ozone from space

Frederick, John E.↗

NASA NTRS1990

Cometary activity in 2060 Chiron

Results of a 2-yr (1988-90) investigation of cometary activity in 2060 Chiron based on CCD photometry and spectroscopy are reported. The photometry observations include a new rotational light curve of Chiron, a newly refined rotation period, recent developments of its long-term photometric behavior and surface brightness profiles, a deep image of the coma of Chiron, and narrowband images at wavelengths ranging from 3200 to 6840 A. The spectroscopic data include moderate resolution CCD spectra (10-20 A FWHM). Major results include the detection of impulsive brightening on a time scale of hours, evidence for a secular change in the blue portion of the reflectivity spectrum of the nucleus, no evidence for Rayleigh scattering in the near ultraviolet, and an upper limit of the column density of CO(+) ions in the coma.

Luu, Jane X.↗

NASA NTRS1991

Images from Galileo of the Venus cloud deck

Images of Venus taken at 418 and 986 nm show that the morphology and motions of large-scale features change with depth in the cloud deck. Poleward meridional velocities, seen in both spectral regions, are much reduced in the NIR. In the south polar region the markings in the two wavelength bands are strongly anticorrelated. The images follow the changing state of the upper cloud layer downwind of the subsolar point, and the zonal flowfield shows a longitudinal periodicity that may be coupled to the formation of large-scale planetary waves. No optical lightning was detected.

Belton, Michael J. S.↗