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At least 451 records · Page 25

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DOE OSTI2024

Non-equilibrium plasma co-upcycling of waste plastics and CO 2 for carbon-negative oleochemicals

Mechanical recycling and chemical upcycling by thermochemical reactions have been the major approaches for recycling end-of-life plastics. Herein, we report an electrified approach to upcycle waste plastics into carbon-negative commodity chemicals using greenhouse gas CO 2 as the oxidant and additional carbon source. In this non-equilibrium plasma process, waste polyolefins were oxidatively depolymerized by plasma-activated CO 2 to produce oleochemicals and hydrocarbon chemicals in a single-step process at high reaction rates. In addition, a mixture of CO 2 and a small amount of O 2 was employed as plasma gases to selectively produce fatty alcohols from polyolefins. Based on this atmospheric pressure, non-solvent, and non-catalyst process, up to 97.6% of fatty alcohols could be produced within minutes. In this article, the co-conversion approach was demonstrated using common polyolefins and real-world mixed waste plastics to obtain comparable results. The techno-economic analysis estimates the internal rate of return to be 42.2% and 43.5% for the plasma-based conversion of waste plastics, depending on the plasma gas composition. Lifecycle assessment indicates the global warming potential is between −3.33 and −3.07 kg CO 2e per kg of plastic.

42 ENGINEERING↗

DOE OSTI2020

Latest Developments in PM Systems and Methods and their Application to WM Projects - 20364

How do you improve on an industry that is well established yet often misses the mark on key metrics demonstrating effective planning and execution of project scope, schedule and budget? With the increased complexity of DOE projects relative to either poorly kept records of what wastes are stored or the lack of specific knowledge relative to the waste concentrations/quantities, this is a question continually asked and investigated by many. In fact, in 2017, the GAO's report to Congress indicated that although the DOE has made some progress on its monitoring effectiveness and demonstrating progress criteria, these goals were not met and there needs to be more improvement and monitoring. This paper will offer some insights into the latest developments in project management methodologies and the possible application of these to waste management projects. Traditional data generated via a project schedule that utilizes critical path methodology (CPM) and additional earned value management (EVM) data needs to be accurate and enable the project manager to better understand the probability of project success. Although this data has readily been available on most large-scale projects, success as measured by various stakeholder groups including the client, project team, regulators, etc. is less than optimal. Therefore, an urgent need exists to explore how traditional project data (CPM and EVM) coupled with new methodologies allows for better planning and execution by the project team. Many new approaches/methodologies can even be used to predict the success of options prior to full implementation on the actual project. Three approaches/methodologies will be discussed: - Artificial Intelligence; - Change Management; - Blend of Traditional Management (Gantt chart) and Agile Methodologies. As market forces change, so will the direction of project management. The days of 'one size fits all' are no longer valid. A combination of predictive and adaptive approaches in the management of projects is essential to enable execution of project deliverables on time, under budget, and within the contractual scope. This paper is intended to provide the reader with insight to the close relationship of project management trends and business management trends, and to provoke critical thinking about what it means to align project management strategy with an environment of non-stop innovation. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2020

Distributed power generation via gasification of biomass and municipal solid waste: A review

The access to electricity has increased worldwide, growing from 60 million additional consumers per year in 2000-2012 to 100 million per year in 2012-2016. Despite this growth, approximately 675 million people will still lack access to electricity in 2030, indicating that electricity demand will continue to increase. Unfortunately, traditional large fossil power technologies based on coal, oil and natural gas lead to a major concern in tackling worldwide carbon dioxide emissions, and nuclear power remains unpopular due to public safety concerns. Distributed power generation utilizing CO 2 -neutral sources, such as gasification of biomass and municipal solid wastes (MSW), can play an important role in meeting the world energy demand in a sustainable way. Furthermore, this review focuses on the recent technology developments on seven power generation technologies (i.e. internal combustion engine, gas turbine, micro gas turbine, steam turbine, Stirling engine, organic rankine cycle generator, and fuel cell) suitable for distributed power applications with capability of independent operation using syngas derived from gasification of biomass and MSW. Technology selection guidelines is discussed based on criteria, including hardware modification required, size inflexibility, sensitivity to syngas contaminants, operational uncertainty, efficiency, lifetime, fast ramp up/down capability, controls and capital cost. Major challenges facing further development and commercialization of these power generation technologies are discussed.

09 BIOMASS FUELS↗

DOE OSTI2023

Application of Particle Accelerators to Mitigate Energy and Climate Change Problems Facing America

Reliable CO 2 -free baseload power is needed to address ever-increasing demands for electricity while minimizing adverse climate change. Diversified power supply provided by solar, wind, geothermal, and nuclear reactors can displace the use of fossil fuels. The United States (U.S.) is taking a new look at nuclear power as a source of electrical energy and the nuclear industry is proposing new approaches which may minimize capital costs. However, nuclear power comes with a variety of technical problems. Chief among those is managing the used fuel from nuclear reactors. No long-term, practicable solution to this problem is available. The lack of progress on a comprehensive waste management strategy restricts growth in the nuclear power industry and minimizes the role that nuclear energy may serve as part of a zero-carbon future (Bahr, 2021). According to the Nuclear Waste Policy Act of 1982, as amended, the U.S. Government has possession of the used reactor fuel and incurs large annual storage fees paid to utilities to store and safeguard the accumulated used fuel. In effect, short term on-site storage of nuclear waste is the current waste management plan. The amount of used reactor fuel in the U.S. is approximately 80,000 metric tons. While no geologic repository exists within the U.S., the potential site at Yucca Mountain, NV would accommodate 70,000 metric tons, which fails to meet current and future needs. Given the technical and political challenges associated with establishing a single geological storage site, it is necessary for the U.S. to implement technologies that improve the suitability of geological storage by reducing the volume and radiotoxicity of stored material. No extant technology meets this need. Accelerator driven waste burners have been proposed as a scalable method to process used nuclear fuel, however considerable technical challenges remain which impede commercialization. Innovations in design require investigation of novel materials, development of accurate models and simulations, and a comprehensive assessment of safety and performance. This proposal elaborates how LANL is uniquely positioned to make key contributions to this area of research.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

NASA NTRSDate not supplied

Hybrid Thermal Control System for Extreme Thermal Environments

NASA’s return to the moon brings about many challenges, including issues with survival on the Lunar surface. Marshall Space Flight Center (MSFC) has been developing a hybrid thermal control system that can be utilized for various surface assets that must survive in extreme lunar environments. This scalable system is targeted for human-rated systems and utilizes a combination of a- pumped fluid loop (PFL) and a loop heat pipe (LHP) with thermal control valve (TCV). Pumped fluid loops have a long history of use in human rated systems. They can collect large amounts of waste heat and transport it over long distances in rovers, habitats, and other systems. By utilizing a non-toxic working fluid in the habitable volume, the PFL is easily serviceable by the crew and does not pose a risk during any unexpected leaks or failures. The addition of a LHP for the exterior heat transport and rejection adds several benefits to the system for extreme environment survival. The quantity of LHP scan be tailored to optimize heat rejection for different systems and allows for larger adiative surfaces. By utilizing a TCV in combination with the LHP, there can be high heat transfer during the daytime with minimal heat transfer during the night. The TCV passively controls the amount of heat transfer through the LHP based on the environmental temperature. A prototype system has been tested in bench top and thermal vacuum conditions. Results are presented showing the feasibility of the system concept.

Thermal Control↗

NASA NTRS2023

Hybrid Thermal Control System for Extreme Thermal Environments

Thermal Control↗

NASA NTRS1982

ID slicing and the automated factory

The automation of the slicing system utilizing internal-diameter saws for the production of the silicon wafers used in solar arrays is discussed. It is argued that saw productivity can be increased by reducing silicon waste, decreasing usage of consumables, keeping the saw slicing, and increasing the cutting speed. Several machine enhancements utilizing automatic control are discussed. The need for record keeping to anticipate maintenance operations is noted, and a digital serial communication interface with the microprocessor-based saws is recommended. Distributed control of the manufacturing process is discussed in detail, and is recommended as a method for increasing productivity.

Lewandowski, T.↗

DOE OSTI2026

Waste-to-Energy Potential in Guam [Slides]

This report presents an overview of the potential applications and associated costs of implementing waste-to-energy technologies in Guam. It examines how these systems could contribute to the island’s energy portfolio by converting waste materials into usable power or heat.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2026

Treatment of Lagoon Dairy Manure Wastewater via Iron Electrocoagulation, Microfiltration, and Adsorption

Dairy manure wastewater generated by flushing barn cow waste contains nutrients, pathogens, and organic and inorganic contaminants. This study utilized a process consisting of iron electrocoagulation (Fe-EC), microfiltration (MF), and activated carbon (AC) adsorption to treat farm wastewater and explore the reclamation of clean water for irrigation and livestock consumption. Significant removal (>99.9%) of chemical oxygen demand (COD), total organic carbon (TOC), phosphorus (P), turbidity, and microorganisms, as well as ions including magnesium, calcium, sulfur, and silica was achieved by the combined EC-MF-AC process. Specifically, a charge loading of ∼37,500 C/L in a continuous-flow EC configuration, followed by MF, achieved more than 95% removal of TOC and COD. Characterization of produced flocs and foam via scanning-electron microscopy with energy-dispersal spectroscopy and Fourier transform infrared spectroscopy confirmed the removal of ions, including calcium, sulfur, and silica. A key finding was the electrocatalytic conversion of nitrogen species to ammonia gas through the intermediate reduction of nitrate/nitrite, which led to ∼60% total nitrogen (TN) removal. AC treatment further improved TN removal to ∼70%. The Fe-EC process also eradicated >99.9% of bacteria. Preliminary process cost assessment, based on recycled materials for EC electrodes, showed significant cost savings (∼2 times) compared to commercial electrodes.

Dutta, Swapnamoy [ORNL]↗

DOE OSTI2020

Preliminary Determination of the Impact of Alkaline Earth Metals on Crystalline Silicotitanate

Savannah River Remediation (SRR) recently deployed the Tank Closure Cesium Removal (TCCR) system which utilizes an ion exchange process to remove 137 Cs from tank waste supernate. In TCCR, salt solution is filtered and then passed through ion exchange columns containing crystalline silicotitanate (CST) media, commercially known as UOP IONSIV™ R9120-B, which is highly selective for removing cesium. The current process focuses on dissolving salt in Savannah River Site (SRS) Tank 10H, followed by processing in the TCCR skid located near the tank. Prior to processing each batch of waste generated in Tank 10H, the projected maximum cesium loading on the CST is determined using an in-tank batch contact equilibrium test. This involves placing a small amount (~0.1 g) of CST in a “teabag” device and submerging it in the tank waste for a period of 10 days. Results from those earlier teabag tests had indicated much lower cesium loading than predicted by the equilibrium sorption model (ZAM). There are numerous possible explanations for this result; however, based on the observed loadings of Ca (and other metals) on the CST from the teabag tests, it was hypothesized that competition from these other ions may be limiting the cesium loadings.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2022

Radiological Considerations Supporting the American Medical Isotope Producer Niowave

This report provides a summary of work performed by Savannah River National Laboratory (SRNL) during FY22 in support of Niowave, an American Medical Isotope Production (AMIP) facility. SRNL served in a technical support role, funded by NA-231, supporting Niowave in the beginning of non radiological functional testing of their airport facility in FY22. Through this agreement, SRNL provides Niowave access to subject matter experts (SMEs) for questions that may arise during the drafting of engineering plans, facility policies, and/or response procedures. This report summarizes discussions between SRNL and Niowave about guidance concerning issues with the floor of the hot cells, dispersible removable contamination (beta emitting fission product), hot cell operation specifically utilization of cameras or mirrors, and the process for removing contaminated waste from the hot cell. Lessons learned and other various resources provided to Niowave by SRNL during FY22 are referenced in this report. This work was funded through NNSA’s Office of Material Management and Minimization, Conversion Office (NA-231).

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2024

Tank Closure Cesium Removal Ion Exchange Column CST Characterization: SRNL-STI-2024-00072 (Rev.0) pdf

Savannah River Mission Completion (SRMC) recently suspended operation of the Tank Closure Cesium Removal (TCCR) system which utilized an ion exchange (IX) process to remove radioactive cesium from waste supernate. During the demonstration phase, a total of three batches of Tank 10H dissolved salt waste were processed through the original TCCR columns. Subsequently, dissolved salt waste from Tank 9H was processed through TCCR in a phase referred to as TCCR 1A with four new IX columns. All eight columns have now been moved to Interim Safe Storage (ISS). For each batch processed through the TCCR IX columns, SRNL performed a number of analyses on surface and variable depth samples as well as batch equilibrium contact tests (BECT) to determine equilibrium loadings of Cs on the crystalline silicotitanate (CST) IX media. The BECTs were performed by lowering “teabags” containing ~0.1 g of CST each into the tank for a period of at least 10 days. The teabags were then retrieved and sent to SRNL for digestion and analysis.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2023

Technical Feasibility of Recovering Critical Minerals from Oil and Gas Industry Produced Water

Economic recovery of critical minerals from solid and liquid streams produced from natural resource extraction operations including Oil and Gas production, Mining, geothermal, and other industries can help alleviate shortage of the minerals important to industry. It is important to develop techniques for extraction that can be utilized at large scale to be economically viable, and to minimize waste products that require special disposal procedures. NETL and Participant will collaborate to develop and evaluate at the lab-scale, a process to recover and concentrate critical minerals from oil and gas industry produced water using a combination of physical and chemical methods, so that it may be converted into a valuable product. This effort promotes a circular economy by converting a waste stream into marketable products.

02 PETROLEUM↗

NASA NTRS1974

General survey of solid-waste management

Potential ways of providing solid-waste management for a building complex serviced by a modular integrated utility system (MIUS) were explored. Literature surveys were conducted to investigate both conventional and unusual systems to serve this purpose. The advantages and disadvantages of the systems most compatible with MIUS are discussed.

Reese, T. G.↗

NASA NTRS1978

Disposal of radioactive iodine in space

The possibility of space disposal of iodine waste from nuclear power reactors is investigated. The space transportation system utilized relies upon the space shuttle, a liquid hydrogen/liquid oxygen orbit transfer vehicle, and a solid propellant final stage. The iodine is assumed to be in the form of either an iodide or an iodate, and calculations assume that the final destination is either solar orbit or solar system escape. It is concluded that space disposal of iodine is feasible.

Burns, R. E.↗

NASA NTRS2006

Vibroacoustic Analysis of Large Heat Rejection Radiators for Future Spacecraft

Spacecraft structures such as antennas, solar arrays and radiator panels significantly respond to high acoustic levels seen at lift-off. Some future spacecraft may utilize nuclear electric propulsion that require large radiator panels to reject waste heat. A vibroacoustic assessment was performed for two different radiator panel designs. Results from the analysis of the two designs using different analytical approaches are presented and discussed.

Larko, Jeffrey M.↗

NASA NTRS2018

Needs and Opportunities in the Development of Advanced Materials and Manufacturing Methods for Future Long-Duration Human Space Exploration

Weight, functionality, and sustainability are all critical concerns for future, long-duration, human exploration of space. Exploration missions will be mass-limited, since the amount of supplies and instruments that future astronauts will be able to take with them will be limited by launch vehicle and spacecraft mass and efficiency. Astronauts will need to have the capability to repair or replace worn-out or broke hardware and produce new components to be able to function for long periods at locations far-removed from Earth. Ultra-lightweight, multifunctional materials will be required to enable significant reductions in launch vehicle, spacecraft, and habitat mass in order to maximize payload. "Mass-less Exploration" concepts must be developed that will recycle materials and waste and convert available planetary materials into new feedstock materials and utilize in-space additive manufacturing to use these materials to produce the

composites↗

NASA NTRS2016

Thermal Stability Testing of Two-Phase Thermal Control Hardware for the Surface Water Ocean Topography Mission

The thermal architecture for the Surface Water Ocean Topography mission utilizes loop heat pipes and constant conductance heat pipes to transport waste heat (> 1000 Watts) from the instrument electronics to the radiator. The main thermal design risk is the ability to maintain a temporal stability of <0.05 Celsius per minute in a low earth orbit environment. The stringent thermal requirements are part of the overall error budget needed to meet the primary mission science objectives. A testbed was developed to simulate flight-like loads and environments in order to validate the thermal subsystem can meet the temporal stability requirements. Preliminary testing showed that the thermal control system can meet the stability requirement and that loop heat pipes are actually helping to maintain stability during transient sink temperature changes for this specific flight application and boundary conditions.

Somawardhana, Ruwan P.↗