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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 469 records · Page 26
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Magnetic field sensors for detection of trapped flux in superconducting radio frequency cavities

Superconducting radio-frequency (SRF) cavities are fundamental building block of modern particle accelerators. They operate at liquid helium temperatures 2-4 K to achieve very high quality factors 1e10-1e11. Trapping of magnetic flux within the superconductor is a significant contribution to the residual RF losses which limit the achievable quality factor. Suitable diagnostic tools are in high demand to understand the mechanisms of flux trapping in technical superconductors and the fundamental components of such diagnostic tool are magnetic field sensors. We have studied the performance of commercially available Hall probes, anisotropic magnetoresistive sensors and flux-gate magnetometers with respect to their sensitivity and capability to detect localized, low magnetic flux amplitudes, of the order of few tens of magnetic flux quantum at liquid helium temperature. Although Hall probes have the lowest magnetic field sensitivity (~96$ nV$/microT at 2 K), their physical dimensions are such that they have the ability to detect the lowest number of trapped vortices among the three type of sensors. Hall probes and anisotropic magnetoresistive sensors have been selected to be used in a setup to map regions of trapped flux on the surface of a single-cell SRF cavity.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Nanoscale Probing of Electrical Memory Effects in van der Waals Layered PdSe 2

Tunable electronic materials that can be switched between different impedance states are fundamental to the hardware elements for neuromorphic computing architectures. This “brain-like” computing paradigm uses highly paralleled and colocated data processing, leading to greatly improved energy efficiency and performance compared to traditional architectures in which data have to be frequently transferred between processor and memory. In this work, we use scanning microwave impedance microscopy for nanoscale electrical and electronic characterization of two-dimensional layered semiconductor PdSe 2 to probe neuromorphic properties. The local resolution of tens of nanometers reveals significant differences in electronic behavior between and within PdSe 2 nanosheets (NSs). In particular, we detected both n-type and p-type behaviors, although previous reports only point to ambipolar n-type dominating characteristics. Nanoscale capacitance–voltage curves and subsequent calculation of characteristic maps revealed a hysteretic behavior originating from the creation and erasure of Se vacancies as well as the switching of defect charge states. In addition, stacks consisting of two NSs show enhanced resistive and capacitive switching, which is attributed to trapped charge carriers at the interfaces between the stacked NSs. Stacking n- and p-type NSs results in a combined behavior that allows one to tune electrical characteristics. In conclusion, as local inhomogeneities of electrical and electronic behavior can have a significant impact on the overall device performance, the demonstrated nanoscale characterization and analysis will be applicable to a wide range of semiconducting materials.

2D material↗
DOE OSTI2023

Microstability of β ~ 1 tokamak equilibria

High-power-density tokamaks offer a potential solution to design cost-effective fusion devices. One way to achieve high power density is to operate at a high β value (the ratio of thermal to magnetic pressure), i.e. β~1 . However, a β~1 state may be unstable to various pressure- and current-driven instabilities or have unfavourable microstability properties. To explore these possibilities, we generate β~1 equilibria and investigate their stability. First, we demonstrate the generation of high-β equilibria with the computer code VMEC. We then analyse these equilibria to determine their stability against the infinite-n ideal-ballooning mode. We follow that by engaging in a detailed microstability study using the GS2 code, beginning with assessments of electrostatic ion-temperature-gradient and trapped election mode instabilities. We observe interesting behaviour for the high-β equilibria – stabilization of these modes through two distinct mechanisms – large negative local shear and reversal of electron precession drift. Finally, we perform electromagnetic gyrokinetic simulations and observe enhanced stability in the outer core of high-β equilibria and absence of kinetic ballooning modes in the negative-triangularity, high-β equilibria. The enhanced outer-core stability of high-β equilibria is different from their lower-β counterparts and offers an alternative, potentially favourable regime of tokamak operation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1979

Structure and properties of Jupiter's magnetoplasmadisc

Voyager 1 plasma-wave observations have revealed the existence of an earthlike continuum radiation trapped in Jupiter's magnetospheric cavity at frequencies below the solar-wind plasma frequency. This radiation serves as an accurate diagnostic of the local electron number density throughout most of Jupiter's outer magnetosphere and yields information regarding the gross configuration of the magnetoplasmadisk as well as its kinematical properties. Magnetic-field observations are used to construct radial profiles of plasma pressure, density, and temperature from 20-80 Jupiter radii in the early-morning plasma sheet, along with plasma-sheet crossings and estimated thicknesses. The study suggests that hot protons (about 10 keV) are the dominant constituents of the plasma sheet (average thickness about 4.2 Jupiter radii) out to 80 Jupiter radii, beyond which centrifugal effects take over and distort the sheet toward the rotational equator.

Barbosa, D. D.↗
NASA NTRS2019

Characteristics of Relativistic Microburst Intensity from SAMPEX Observations

Relativistic electron microbursts are an important electron loss process from the radiation belts into the atmosphere. These precipitation events have been shown to significantly impact the radiation belt fluxes and atmospheric chemistry. In this study we address a lack of knowledge about the relativistic microburst intensity using measurements of 21,746 microbursts from the Solar Anomalous Magnetospheric Particle Explorer (SAMPEX).We find that the relativistic microburst intensity increases as we move inward in L, with a higher proportion of low-intensity microbursts (<2,250 [MeV cu.cm sr s](exp −1)) in the 03–11 magnetic local time region. The mean microburst intensity increases by a factor of 1.7 as the geomagnetic activity level increases and the proportion of high-intensity relativistic microbursts (>2,250 [MeV cu.cm2 sr s](exp −1)) in the 03–11 magnetic local time region increases as geomagnetic activity increases, consistent with changes in the whistler mode chorus wave activity. Comparisons between relativistic microburst properties and trapped fluxes suggest that the microburst intensities are not limited by the trapped flux present alongside the scattering processes. However, microburst activity appears to correspond to the changing trapped flux; more microbursts occur when the trapped fluxes are enhancing, suggesting that microbursts are linked to processes causing the increased trapped fluxes. Finally, modeling of the impact of a published microburst spectra on a flux tube shows that microbursts are capable of depleting <500-keV electrons within 1 hr and depleting higher-energy electrons in 1–23 hr.

Douma, E.↗
DOE OSTI2018

Final Report - Impact of Microstructure on the Containment and Migration of CO 2 in Fractured Basalts

The overall objective of the project was to advance the scientific and technical understanding of fracture microstructure on the flow and mineralization of CO 2 injected into fractured basalt. The project combined bench-scale CO 2 -water-rock testing, geochemical characterization of rock cores, and advanced characterization of the evolution of fracture structure and carbon trapping mechanisms. A series of natural and artificial basalts were acquired and characterized for use in experiments. High pressure and high temperature experiments were performed in both batch modes and in flow-through systems. The dissolution of silicate minerals in the basalts was tracked, and the timing, identity and location of carbonate minerals that trap that added CO 2 were determined. A reactive transport model was developed that generated simulations that were consistent with the major trends in the experimental data. Novel X-ray computed tomography and nuclear magnetic resonance tools were developed as part of the project. The project found that the formation of carbonate minerals in basalts subjected to injection of CO 2 -rich aqueous solutions can be rapid and extensive. The mineral trapping rate and capacity of porous basalt is much greater than that of sandstone reservoirs. Geochemical gradients that develop upon the exposure of basalt to CO 2 -rich aqueous solutions lead to spatial localization of carbonate minerals in confined environments (e.g., narrow fractures, dead-end fractures, and vesicles). While carbonate minerals form in dead-end fractures, they do not form in ways that inhibit subsequent carbonation of the basalt.

58 GEOSCIENCES↗
DOE OSTI2015

PARTICLE TRAPPING AND STREAMING INSTABILITY IN VORTICES IN PROTOPLANETARY DISKS

We analyze the concentration of solid particles in vortices created and sustained by radial buoyancy in protoplanetary disks, e.g., baroclinic vortex growth. Besides the gas drag acting on particles, we also allow for back-reaction from dust onto the gas. This becomes important when the local dust-to-gas ratio approaches unity. In our two-dimensional, local, shearing sheet simulations, we see high concentrations of grains inside the vortices for a broad range of Stokes numbers, St. An initial dust-to-gas ratio of 1:100 can easily be reversed to 100:1 for St = 1.0. The increased dust-to-gas ratio triggers the streaming instability, thus counter-intuitively limiting the maximal achievable overdensities. We find that particle trapping inside vortices opens the possibility for gravity assisted planetesimal formation even for small particles (St = 0.01) and a low initial dust-to-gas ratio of 1:10{sup 4}, e.g., much smaller than in the previously studied magnetohydrodynamic zonal flow case.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Programmable interactions and emergent geometry in an array of atom clouds

Interactions govern the flow of information and the formation of correlations between constituents of many-body quantum systems, dictating phases of matter found in nature and forms of entanglement generated in the laboratory. Typical interactions decay with distance and thus produce a network of connectivity governed by geometry—such as the crystalline structure of a material or the trapping sites of atoms in a quantum simulator. However, many envisioned applications in quantum simulation and computation require more complex coupling graphs including non-local interactions, which feature in models of information scrambling in black hole, and mappings of hard optimization problems onto frustrated classical magnets. Here we describe the realization of programmable non-local interactions in an array of atomic ensembles within an optical cavity, in which photons carry information between atomic spins. By programming the distance dependence of the interactions, we access effective geometries for which the dimensionality, topology and metric are entirely distinct from the physical geometry of the array. As examples, we engineer an antiferromagnetic triangular ladder, a Möbius strip with sign-changing interactions and a treelike geometry inspired by concepts of quantum gravity. The tree graph constitutes a toy model of holographic duality, in which the quantum system lies on the boundary of a higher-dimensional geometry that emerges from measured correlations. Overall, our work provides broader prospects for simulating frustrated magnets and topological phases, investigating quantum optimization paradigms and engineering entangled resource states for sensing and computation.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2015

Optical and electron transport properties of rock-salt Sc{sub 1−x}Al{sub x}N

Epitaxial single-crystal Sc{sub 1−x}Al{sub x}N ternary alloy layers deposited by magnetron co-sputtering on MgO(001) substrates at 950 °C exhibit a solid solution rock-salt phase for x = 0–0.2 without decomposition. Optical absorption indicates a linear increase in the optical gap from 2.51 eV for ScN to 3.05 eV for Sc{sub 0.8}Al{sub 0.2}N and, after correction due to the Moss-Burstein shift, a direct X point interband transition energy E{sub g}(X) = 2.15 + 2.75 x (eV). Correspondingly, the direct transition at the zone center increases with Al concentration according to E{sub g}(Γ) = 3.80 + 1.45 x (eV), as determined from a feature in the reflection spectra. All layers are degenerate n-type semiconductors with a room temperature mobility that decreases from 22 to 6.7 to 0.83 cm{sup 2}/V s as x increases from 0 to 0.11 to 0.20. The corresponding carrier densities are 9.2 × 10{sup 20}, 7.9 × 10{sup 20}, and 0.95 × 10{sup 20 }cm{sup −3} as determined from Hall measurements and consistent with optical free carrier absorption below photon energies of 1 eV. Temperature dependent transport measurements indicate metallic conduction for ScN, but weak localization that leads to a resistivity minimum at 85 and 210 K for x = 0.051 and 0.15, respectively, and a negative temperature coefficient over the entire measured 4–300 K range for Sc{sub 0.8}Al{sub 0.2}N. The decreasing mobility is attributed to alloy scattering at randomly distributed Al atoms on cation sites, which also cause the weak localization. The carrier density is primarily due to unintentional F doping from the Sc target and decreases strongly for x > 0.15, which is attributed to trapping in defect states due to the deterioration of the crystalline quality, as evidenced by the x-ray diffraction peak width that exhibits a minimum of 0.14° for x = 0.11 but increases to 0.49° for x = 0.20. This is consistent with asymmetric x-ray diffraction analyses, indicating a relaxed lattice constant that decreases from 4.511 ± 0.005 to 4.411 ± 0.004 Å for x = 0–0.2, and a biaxial in-plane compressive strain that decreases from −1.1% to −0.2% as x increases from 0 to 0.11, which is attributed to the higher Al adatom mobility, but increases again to −1.8% for x = 0.20, as x approaches the critical composition for phase separation, which causes structural instability and a higher defect density.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Magnetism and Metal-Insulator Transition in Oxygen Deficient SrTiO 3

First-principles calculations to study the electronic and magnetic properties of bulk, oxygen-deficient SrTiO 3 (STO) under different doping conditions and densities have been conducted. The appearance of magnetism in oxygen-deficient STO is not determined solely by the presence of a single oxygen vacancy but by the density of free carriers and the relative proximity of the vacant sites. We find that while an isolated vacancy behaves as a nonmagnetic double donor, manipulation of the doping conditions allows the stability of a single-donor state, with emergent local moments coupled ferromagnetically by carriers in the conduction band. Strong local lattice distortions enhance the binding of this state. As a result, the energy of the in-gap local moment can be further tuned by orthorhombic strain. Consequently we find that the free-carrier density and strain are fundamental components to obtaining trapped spin-polarized electrons in oxygen-deficient STO, which may have important implications in the design of optical devices.

36 MATERIALS SCIENCE↗
NASA NTRS1972

Theory on the precipitation of magnetospheric electrons at the time of a sudden commencement.

At the time of a sudden commencement or even of a sudden impulse, very-low-frequency waves can be excited. In turn, the wave turbulence drives the pitch-angle diffusion of energetic electrons trapped in the magnetosphere, causing them to be precipitated into the lower ionosphere. The distribution of this precipitation as a function of geomagnetic latitude and local time is shown to be directly related to the characteristics of the magnetic disturbances.

Perona, G. E.↗
NASA NTRS1988

The global distribution, abundance, and stability of SO2 on Io

Voyager multispectral mosaics, earth-observed spectra, and photometric characterizations have been used to model and globally map the SO2 distribution and abundances, the bolometric hemispheric albedos, and the passive surface temperatures on Io. The SO2 is noted to be concentrated in the bright equatorial band, while being deficient in the region defined by Pele-type volcanic eruptions and the polar regions. The brightest, locally coldest areas correspond to SO2-rich regions, although many small patches occur elsewhere. These results are found to support the regional cold-trapping model for the surface and atmospheric SO2 of Fanale et al. (1982).

Mcewen, Alfred S.↗
NASA NTRS1985

Transient response to localized episodic heating in the tropics

It is generally recognized that equatorial disturbances in the lower stratosphere are excited by convective latent heat release associated with the Internal Tropical Convergence Zone (ITCZ). Recently, attention has also focused on tropical convection with regard to extratropical teleconnection patterns. Unlike equatorial waves which are trapped about the equator but propagate vertically, the latter extend well out of the tropics but are barotropic. They have been most widely discussed in connection with long-term climatological features. Both types of disturbances have been examined largely from the standpoint of steady monochromatic forcing, in the latter case zero frequency or time-mean heating. However, tropical convection as revealed by recent geostationary satellite imagery is anything but regular, surely not steady. Much of the heating variance is concentrated spatially within three localized convective centers: Indonesia, the Amazon, and the Congo. Convective activity within these regions undergoes an irregular evolution over the span of a couple of days. It involves a rather broad spectrum of spatial and temporal scales. The analysis of cloud brightness over the Eastern Atlantic and Africa suggests a characteristic time scale of 3-4 days and correlations scales in latitude and longitude of approximately 30 deg.

Salby, M. L.↗
DOE OSTI2015

Erosion products of plasma facing materials formed under ITER-like transient load and deuterium retention in them

Erosion of the plasma-facing materials in particular evaporation of the materials in a fusion reactor under intense transient events is one of the problems of the ITER. The current experimental data are insufficient to predict the properties of the erosion products, a significant part of which will be formed during transient events (edge-localized modes (ELMs) and disruptions). The paper concerns the experimental investigation of the graphite and tungsten erosion products deposited under pulsed plasma load at the QSPA-T: heat load on the target was 2.6 MJ/m{sup 2} with 0.5 ms pulse duration. The designed diagnostics for measuring the deposition rate made it possible to determine that the deposition of eroded material occurs during discharge, and the deposition rate is in the range (0.1–100) × 10{sup 19} at/(cm{sup 2} s), which is much higher than that for stationary processes. It is found that the relative atomic concentrations D/C and D/(W + C) in the erosion products deposited during the pulse process are on the same level as for the stationary processes. An exposure of erosion products to photonic energy densities typical of those expected at mitigated disruptions in the ITER (pulse duration of 0.5–1 ms, integral energy density of radiation of 0.1–0.5 MJ/m2) significantly decreases the concentration of trapped deuterium.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1976

The 2- to 12-min quasi-periodic variation of 50- to 1000-keV trapped electron fluxes

It was previously shown that trapped electron fluxes of energies in the range from 50 keV to 1 MeV observed in the afternoon magnetosphere during substorms frequently undergo periodic variations. High-resolution electron spectrometer data indicate that these electron variations are periodic in the range of about 2-12 min, correlated with magnetic field variations, organized by the local magnetic field, and dependent on pitch angle. The observations suggest that the electron variations are adiabatic. The study derives quantitative adiabatic expressions of particle flux variations in a model geomagnetic field perturbation to show that the observational features are consistent with effects arising from adiabatic modulation of trapped particle fluxes.

Lin, C. S.↗
NASA NTRS1989

Approximate angular distribution and spectra for geomagnetically trapped protons in low-earth orbit

The highly anisotropic nature of the radiation in the low-earth orbit has been ignored for most spacecraft shielding calculations made to date because the standard environmental models describe the omnidirectional flux only, because the varying attitude of the spacecraft in the environment is assumed to average out the effect and because of the added complexity of the calculation. The Space Station is planned to be stabilized with respect to the velocity vector and local vertical. Thus it will pass through the South Atlantic Anomaly where most of the radiation flux is encountered in much the same attitude on each pass. Any calculation including a complex shielding geometry should thus consider the angular distributuon of the incident radiation. An approximate trapped proton angular distribution is presented which includes both the 'pan caked' distribution relative to the magnetic field direction and the east-west effect which is energy dependent. This distribution is then used with a planar shielding geometry to obtain an estimate of the effect of the anisotropy on radiation dose rates in spacecraft.

Watts, J. W.↗
DOE OSTI2019

Coupled supercritical CO2 dissolution and water flow in pore-scale micromodels

Dissolution trapping is one of the most important mechanisms for geological carbon storage (GCS). Recent laboratory and field experiments have shown non-equilibrium dissolution of supercritical CO2 (scCO2) and coupled scCO2 dissolution and water flow, i.e., scCO2 dissolution at local pores/pore throats creating new water-flow paths, which in turn enhance dissolution by increased advection and interfacial area. However, the impacts of pore-scale characteristics on these coupled processes have not been investigated. In this study, imbibition and dissolution experiments were conducted under 40°C and 9?MPa using a homogeneous/isotropic hexagonal micromodel, two homogeneous elliptical micromodels with low or high anisotropy, and a heterogeneous sandstone-analog micromodel. The four micromodels, initially saturated with deionized (DI)-water, were drained by injecting scCO2 to establish a stable scCO2 saturation. DI water was then injected at different rates with logCa (the capillary number) ranging from -6.56 to -4.34. Results show that bypass of scCO2 by displacing water is the dominant mechanism contributing to the residual CO2 trapping, triggered by heterogeneity in pore characteristics or pore-scale scCO2-water distribution. Bypass can be enhanced by pore heterogeneity or reduced by increasing transverse permeability, resulting in relatively low (<2% of CO2 solubility) or high (9–13% of CO2 solubility) dissolved CO2 concentration in displacing water. The overall dissolution of residual scCO2 increases with decreasing Ca, and approaches to their solubility at low Ca value with sufficient residence time. This main trend is similar to a capillary desaturation curve that represents the relationship between the residual saturation and Ca. Spatially, dissolution initiates along the boundary of bypassed scCO2 cluster(s) in a non-equilibrium manner, and the coupling of water flow and dissolution occurs which fragments the bypassed scCO2 clusters and enhance scCO2 dissolution.

Chang, Chun↗
DOE OSTI2016

Helium trapping at erbium oxide precipitates in erbium hydride

The formation of He bubbles in erbium tritides is a significant process in the aging of these materials. Due to the long-standing uncertainty about the initial nucleation process of these bubbles, there is interest in mechanisms that can lead to the localization of He in erbium hydrides. Previous work has been unable to identify nucleation sites in homogeneous erbium hydride. This work builds on the experimental observation that erbium hydrides have nano- scale erbium oxide precipitates due to the high thermodynamic stability of erbium oxide and the ubiquitous presence of oxygen during materials processing. Fundamental DFT calculations indicate that the He is energetically favored in the oxide relative to the bulk hydride. Activation energies for the motion of He in the oxide and at the oxide-hydride interface indicate that trapping is kinetically feasible. A simple kinetic Monte Carlo model is developed that demonstrates the degree of trapping of He as a function of temperature and oxide fraction.

36 MATERIALS SCIENCE↗