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At least 469 records · Page 26
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Density Functional Theory Study of Controllable Optical Absorptions and Magneto-Optical Properties of Magnetic CrI 3 Nanoribbons: Implications for Compact 2D Magnetic Devices

A chromium triiodide (CrI 3 ) monolayer has an interesting ferromagnetic ground-state. In this work, we calculate band structures and magnetic moments of tensile-strained and bent zigzag CrI 3 nanoribbons with density functional theory. The edge iodine atoms form flat low-lying conduction bands and couple with chromium atoms ferromagnetically, while the non-edge iodine atoms weakly couple antiferromagnetically. Narrow CrI 3 nanoribbons have two locally stable magnetic moment orientations, namely out-of-plane and in-plane (along the nanoribbon periodic direction) configurations. This enables four magnetization states in CrI 3 nanoribbons, including two out-of-plane ones (up and down) and two in-plane ones (forward and backward along the nanoribbon periodical direction), increasing the operating controllability. Based on the one-dimensional Ising spin chain model, the spin correlation length of the narrow CrI 3 nanoribbon is estimated as about 10 Å at its estimated Curie temperature of 27 Kelvin, which is lower than the measured 45 Kelvin of the monolayer CrI 3 . The optical absorption and magneto-optical properties of CrI 3 nanoribbons are investigated with many-body perturbation GW-BSE (Bethe-Salpeter equation), including magnetic dichroism, Faraday and magneto-optical Kerr effects. Here, the low-energy dark excitons are mainly from transitions between electrons and holes with unlike spins and are non-Frenkel-like, while the bright excitons have mixed spin configurations. The intrinsic lifetime of excitons can be over one nanosecond, suitable for quantum information processes. Tensile strains and bending manifestly modulate the absorption spectra and magneto-optical properties of CrI 3 nanoribbons within a technologically important photon energy-range of ~1.0-2.0 eV. The CrI 3 nanoribbons can be used in 1D or 2D magnetic storage nanodevices, tunable magnetic optoelectronics, and spin-based quantum information controls.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Investigation on the Magnetocaloric Effect of the Pr{sub 7}Pd{sub 3} Compound

Magnetic transitional behaviors and the magnetocaloric effect of the intermetallic compound Pr{sub 7}Pd{sub 3} have been studied. A second-order metamagnetic transition between ferromagnetic and paramagnetic states was observed with a Curie temperature (T{sub C}) of 14.9 K. The paramagnetic Curie temperature (𝜃{sub p}) and the effective magnetic moment (μ{sub eff}) were investigated and determined to be 5.1 K and 3.43 μ{sub B}/Pr, respectively. A reversible magnetocaloric effect was observed in this compound originated from the magnetic phase transition. For a magnetic field change of 0–5 T, the maximum magnetic entropy change − ΔS{sub M} reached 5.5 J kg{sup − 1} K{sup − 1}, and the corresponding value of refrigerant capacity was estimated to be about 65 J kg{sup − 1} with no thermal and field hysteresis loss.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Nonlinear Magnetization Waves and Solitons in a Paramagnet with a Dipole Interaction

Based on a microscopic approach, we have derived equations for the local magnetization dynamics of a spin system coupled by a dipole–dipole interaction in a uniform magnetic field in the continuum approximation. Using the generalized method of multiple scales, we have found the corrections to the Larmor precession frequency of the magnetic moments due to the interparticle interaction, which lead to a broadening of spectral lines and the formation of satellites far from the Larmor frequency. We have derived nonlinear equations for the magnetization amplitude in higher expansion orders, which admit wave and soliton solutions. We have analyzed the influence of the nonsecular part of the dipole–dipole interaction on the stability of solitons and determined the conditions for their existence.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Intrinsic resonances and AC-dipole simulations of 3He in the AGS Booster

Polarized 3 He collisions are part of future RHIC physics programs and of the eRHIC project. The anomalous magnetic moment of 3 He (G=-4.184) is roughly three times greater than that of protons (G=1.793), a polarized species that is already used at the Collider-Accelerator complex at BNL. Because of the higher anomolous magnetic moment and possibly injecting into the AGS at rigidities beyond 7 T • m, 3 He may have to cross depolarizing intrinsic resonances while accelerating in the Booster. To overcome these strong intrinsic resonances we look to an AC-dipole, which will need to be installed in the Booster. An AC-dipole is a magnet that induces large betatron oscillations which forces the entire bunch to experience a stronger resonance and induce a spin flip of all particles. An artificial intrinsic resonance is created, with close proximity to the original intrinsic resonance, which requires simulations to gauge what magnet strength is required. Simulations have been performed using zgoubi regarding the resonances 0 + v y , 12 - v y , and 6 + v y and show that the AC-dipole is effective at overcoming these resonances. Benefits of avoiding the 0 + v y and crossing the 12 - v y and 6 + v y in the Booster presents the advantage of allowing injection above the 0 + v y in the AGS and minimizes the orbit distortions from the snakes.

43 PARTICLE ACCELERATORS↗
DOE OSTI2019

Effects of Oxygen Vacancy on the Magnetic Properties of Ni-Doped SnO{sub 2} Nanoparticles

We studied the ferromagnetism of Ni-doped SnO{sub 2} with and without oxygen vacancy (V{sub O}) by experiments and calculations. Sn{sub 0.96}Ni{sub 0.04}O{sub 2} nanocrystalline powder prepared by the sol-gel method exhibits room-temperature ferromagnetism, and the vacuum annealing reduces its saturation magnetizations. The density functional theory (DFT) calculations show that the doped Ni atom can introduce a local magnetic moment of about 2.0 μ{sub B} in SnO{sub 2} (110) surface, which is ascribed to the spin-polarization of Ni 3d and O 2p electrons. The type of preferential magnetic coupling of Ni-doped SnO{sub 2} (110) surface depends upon the distributions of Ni dopants, and ferromagnetic coupling is more favorable in most cases. Introduction of V{sub O} obviously weakens the ferromagnetic interaction of Ni-doped SnO{sub 2} (110) surface, which can give a reasonable explanation for our experimental observations.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2019

Geometric and Magnetic Structures of K 2 ReI 6 as an Antiferromagnetic Insulator with Ferromagnetic Spin-Canting Originated from Spin–Orbit Coupling

We present the results of a crystallographic analysis, magnetic characterization including neutron powder diffraction, and theoretical assessment of K 2 ReI 6 prepared using solvent reactions. K 2 ReI 6 crystallizes in the space group P 2 1 / n with an inversion center. Magnetic measurements of K 2 ReI 6 sample indicate dominant antiferromagnetic coupling with a Curie–Weiss temperature of θ W = –63.3(1) K, effective magnetic moment ~2.64 μ B /Re but show a weak ferromagnetism ordered at ~24 K. Neutron powder diffraction indicates long-range order of the Re spins below 24 K, with an ordered magnetic moment of 2.2(1) μ B /Re at 1.5 K. Therefore, a canted antiferromagnetic structure is concluded. The electronic structures using first-principles calculations suggest that the antiferromagnetic model of K 2 ReI 6 yields the lowest total energy and opens a band gap with ~1.0 eV width, which is consistent with the UV–vis–NIR optical measurements. After including the spin–orbit coupling (SOC) into the calculation, the band degeneracies slightly shift without influencing the band gap. Furthermore, the results imply that K 2 ReI 6 is an antiferromagnetic insulator with weak ferromagnetic spin-canting resulting from strong SOC-entangled ground state S = 3/2.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Neutrino electromagnetic properties and the weak mixing angle at the LHC Forward Physics Facility

The LHC produces an intense beam of highly energetic neutrinos of all three flavors in the forward direction, and the Forward Physics Facility (FPF) has been proposed to house a suite of experiments taking advantage of this opportunity. In this study, we investigate the FPF’s potential to probe the neutrino electromagnetic properties, including neutrino millicharge, magnetic moment, and charge radius. We find that, due to the large flux of tau neutrinos at the LHC, the FPF detectors will be able to provide more sensitive constraints on the tau neutrino magnetic moment and millicharge than previous measurements at DONUT, by searching for excess in low recoil energy electron scattering events. We also find that, by precisely measuring the rate of neutral current deep inelastic scattering events, the FPF detectors have the potential to obtain the strongest experimental bounds on the neutrino charge radius for the electron neutrino, and one of the leading bounds for the muon neutrino flavor. The same signature could also be used to measure the weak mixing angle, and we estimate that sin 2 θ W could be measured to about 3% precision at a scale Q ∼ 10 GeV , shedding new light on the longstanding NuTeV anomaly. Published by the American Physical Society 2025

Abraham, Roshan Mammen (ORCID:0000000346783808)↗
DOE OSTI2022

Eminuscent phase in frustrated magnets: a challenge to quantum spin liquids

A geometrically frustrated (GF) magnet consists of localised magnetic moments, spins, whose orientation cannot be arranged to simultaneously minimise their interaction energies. Such materials may host novel fascinating phases of matter, such as fluid-like states called quantum spin-liquids. GF magnets have, like all solid-state systems, randomly located impurities whose magnetic moments may “freeze” at low temperatures, making the system enter a spin-glass state. We analyse the available data for spin-glass transitions in GF materials and find a surprising trend: the glass-transition temperature grows with decreasing impurity concentration and reaches a finite value in the impurity-free limit at a previously unidentified, “hidden”, energy scale. We propose a scenario in which the interplay of interactions and entropy leads to a crossover in the permeability of the medium that assists glass freezing at low temperatures. This low-temperature, “eminuscent”, phase may obscure or even destroy the widely-sought spin-liquid states in rather clean systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Thermal Expansion in Fe{sub 2}MAl (M = Ti, V, Cr, Mn, Fe, Co, and Ni) Band Ferromagnets

The linear thermal expansion coefficients (LTEC) of semimetallic Fe{sub 2}MAl (M = Ti, V, Cr, Mn, Fe, Co, and Ni) alloys have been measured in the temperature range 80–900 K. The magnetic-fluctuation contribution to LTEC α{sub m,} {sub sf}(T) = α{sub m}(T) + α{sub sf}(T) consisting of negative “Stoner” α{sub m}(T) and positive “spin-fluctuation” α{sub sf}(T) contributions. The α{sub m}(T) contribution is assumed to be proportional to the square of the spontaneous magnetization. The α{sub sf}(T) contribution, as is the case in paramagnetic and ferromagnetic states, is due to the effects of inducing local magnetic moments by spin fluctuations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Magnetoresistance Hysteresis Evolution in the Granular Y–Ba–Cu–O High-Temperature Superconductor in a Wide Temperature Range

The temperature evolution of the magnetoresistance hysteresis in the granular YBa{sub 2}Cu{sub 3}O{sub 7-δ} high-temperature (T{sub C} ≈ 92 K) superconductor has been investigated. The measurements have been performed in the high-temperature region (78–90 K) and at the liquid helium temperature (4.2 K). The results obtained have been analyzed using the developed model of the behavior of transport properties of a granular high-temperature superconductor in an external magnetic field. Within the discussed model, the dissipation of the grain boundary subsystem is determined by the intergrain spacing-averaged effective field B{sub eff}, which is a superposition of external field H and the field induced by the magnetic moments of superconducting grains. Such a consideration yields the expression B{sub eff}(H) = H − 4πM(H) α for the effective field in the intergrain medium, where M(H) is the experimental hysteretic dependence of magnetization and α is the parameter of magnetic flux crowding in the intergrain medium. Here, the magnetoresistance is assumed to be proportional to the absolute value of the effective field: R(H) ~ |B{sub eff}(H)|. Analysis of the experimental R(H) and M(H) dependences obtained under the same conditions for the investigated high-temperature superconductor sample showed that in the high-temperature region this parameter is α ≈ 25. At the low temperature (4.2 K), we may state that the degree of flux crowding increases and the estimated α value is ~ 50. The estimates made are indicative of the strong effect of flux compression in the intergrain medium on the magnetotransport properties of the investigated granular high-temperature superconductor system. Possible reasons for a discrepancy between the developed model concepts and experimentally observed low-temperature R(H) hysteresis are analyzed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1979

Motions of charged particles in the magnetosphere under the influence of a time-varying large scale convection electric field

The motions of charged particles under the influence of the geomagnetic and electric fields are quite complex in the region of the inner magnetosphere. The Volland-Stern type large-scale convection electric field with gamma = 2 has been used successfully to predict both the plasmapause location and particle enhancements determined from Explorer 45 (S3-A) measurements. Recently introduced into the trajectory calculations of Ejiri et al. (1978) is a time dependence in this electric field based on the variation in Kp for actual magnetic storm conditions. The particle trajectories are computed as they change in this time-varying electric field. Several storm fronts of particles of different magnetic moments are allowed to be injected into the inner magnetosphere from L = 10 in the equatorial plane. The motions of these fronts are presented in a movie format. The local time of injection, the particle magnetic moments and the subsequent temporal history of the magnetospheric electric field play important roles in determining whether the injected particles are trapped within the ring current region or whether they are convected to regions outside the inner magnetosphere.

Smith, P. H.↗
DOE OSTI2017

Transformation of Structure, Electrical Conductivity, and Magnetism in AA'Fe 2 O 6-δ , A = Sr, Ca and A' = Sr

The ability to control electrical properties and magnetism by varying the crystal structure using the effect of the A-site cation in oxygen-deficient perovskites has been studied in AA’Fe 2 O 6-δ , where A=Sr, Ca and A’= Sr. The structure of Sr 2 Fe 2 O 6-δ , synthesized at 1250 °C in air, contains dimeric units of FeO 5 square-pyramids separated by FeO 6 octahedra. Here we show that this ordering scheme can be transformed by changing the A-site cations from Sr to Ca. This leads to a structure where layers of corner-sharing FeO 6 octahedra are separated by chains of FeO 4 tetrahedra. Through systematic variation of the A-site cations, we have determined the average ionic radius required for this conversion to be ~1.41 Å. We have demonstrated that the magnetic structure is also transformed. The Sr 2 compound has an incommensurate magnetic structure, where magnetic moments are in spin-density wave state, aligning perpendicular to the body diagonal of the unit cell. With the aid of neutron diffraction experiments at 10 K and 300 K, we have shown that the magnetic structure is converted into a long-range G-type antiferromagnetic system when one Sr is replaced by Ca. In this G-type ordering scheme, the magnetic moments align in the 001 direction, antiparallel to their nearest neighbors. We have also performed variable-temperature electrical conductivity studies on these materials in the temperature range 298 – 1073 K. These studies have revealed the transformation of charge transport properties, where the metallic behavior of the Sr 2 -compound is converted into semiconductivity in the CaSr-material. The trend of conductivity as a function of temperature is reversed upon changing the A-site cation. The conductivity of the Sr 2 compound shows a downturn, while the conductivity of the CaSr material increases as a function of temperature. We have also shown that the CaSr-compound exhibits temperature-dependent behavior typical of a mixed ionic-electronic conducting system.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2017

Probing new spin-independent interactions through precision spectroscopy in atoms with few electrons

The very high precision of current measurements and theory predictions of spectral lines in few-electron atoms allows us to efficiently probe the existence of exotic forces between electrons, neutrons and protons. We investigate here the sensitivity to new spin-independent interactions in transition frequencies (and their isotopic shifts) of hydrogen, helium and some heliumlike ions. We find that present data probe new regions of the force-carrier couplings to electrons and neutrons around the MeV mass range. We also find that, below few keV, the sensitivity to the electron coupling in precision spectroscopy of helium and positronium is comparable to that of the anomalous magnetic moment of the electron. Finally, we interpret our results in the dark-photon model where a new gauge boson is kinetically mixed with the photon. There, we show that helium transitions, combined with the anomalous magnetic moment of the electron, provide the strongest indirect bound from laboratory experiments above 100 keV.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Magnetic structure of A ≤ 10 nuclei using the Norfolk nuclear models with quantum Monte Carlo methods

Here we present quantum Monte Carlo calculations of magnetic moments, form factors, and densities of A ≤ 10 nuclei within a chiral effective field theory approach. We use the Norfolk two- and three-body chiral potentials and their consistent electromagnetic one- and two-nucleon current operators. We find that two-body contributions to the magnetic moment can be large (up to ≈ 33% in A = 9 systems). We study the model dependence of these observables and place particular emphasis on investigating their sensitivity to using different cutoffs to regulate the many-nucleon operators. Calculations of elastic magnetic form factors for A ≤ 10 nuclei show excellent agreement with the data out to momentum transfers q ≈ 3 fm -1 .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

The Fermilab Muon g-2 experiment: laser calibration system

The anomalous muon dipole magnetic moment can be measured (and calculated) with great precision thus providing insight on the Standard Model and new physics. Currently an experiment is under construction at Fermilab (U.S.A.) which is expected to measure the anomalous muon dipole magnetic moment with unprecedented precision. One of the improvements with respect to the previous experiments is expected to come from the laser calibration system which has been designed and constructed by the Italian part of the collaboration (INFN). Furthermore, an emphasis of this paper will be on the calibration system that is in the final stages of construction as well as the experiment which is expected to start data taking this year.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

Electronic and Magnetic States of Pr and Mn in the Pr{sub 1–x}Sr{sub x}MnO{sub 3} Films Studied by XANES and XMCD Spectroscopy

The spectral dependences of X-ray absorption near-edge spectroscopy (XANES) and X-ray magnetic circular dichroism (XMCD) and the field dependences of XMCD near the K edge of Mn and the L{sub 2,3} edges of Pr in the Pr{sub 0.8}Sr{sub 0.2}MnO{sub 3} and Pr{sub 0.6}Sr{sub 0.4}MnO{sub 3} films at T = 90 K are studied. The spectral dependences point to a mixed valence state of Mn and Pr in the films. It is found that, as compared to XANES, XMCD is more sensitive to the valence state of Pr{sup 4+}. The field dependences of XMCD point to ferromagnetic behavior of Mn ions and the Van Vleck paramagnetism of Pr ions, which makes a significant contribution to the total magnetization of the films. It is shown that as the Sr concentration increases, the XMCD intensity at the K edge of Mn increases, which indicates a growth of the total magnetic moment of the film due to an increase in the 4p–3d hybridization.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Measurement of vertical betatron oscillations using the straw tracking detectors for the E989 muon g-2 experiment at Fermilab.

The measurement of the anomalous magnetic moment of electrons and muons has been an important test of the Standard Model (SM) of particle physics over many decades. This is because it can be measured experimentally and calculated theoretically to a high precision. In particular the anomalous magnetic moment of the muon, a µ , is an ideal candidate for the search of new physics due to the combination of the muons large mass and relatively long lifetime. The current world’s most precise value of aµ was measured by the E821 experiment at the Brookhaven National laboratory (BNL). This achieved a precision of 540 ppb (463 ppb stat., 283 ppb syst.) and measured a ~ 3.5 σ deviation from the SM value [1]. This motivated a new experiment: the E989 muon g–2 experiment at the Fermi National Accelerator Laboratory (Fermilab) to confirm or reject this discrepancy. This experiment aims to gather a data sample 21 times larger than the BNL experiment and improve the determination of the systematic uncertainties by a factor of three and thereby achieve a fourfold increase in precision to 140 ppb [2]. If the aµ value were to remain unchanged, this improvement in precision would establish evidence for Beyond SM (BSM) physics with a significance of more than 7 standard deviations. The Fermilab experiment has the same methodology as the BNL experiment and reuses the experiment’s storage ring magnet. New, improved experimental apparatus has been introduced to reduce the systematic uncertainty on the a µ measurement. One such improvement is the addition of two straw tracking stations. These measure the trajectory of the positrons emitted from the (positive) muon decays which allows a detailed study of the spatial and temporal motion of the beam and critical crosschecks of the calorimeter data. This thesis describes in detail the design, construction and testing of the tracking detectors which were built at the University of Liverpool. A detailed study of the vertical motion of the beam is also presented. This study provides an important correction that must be applied to the data before a µ can be determined.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

Magnetism and Optical Property of Mn-Doped Monolayer CrSi{sub 2} by First-Principle Study

We investigate magnetism and optical properties of intrinsic and Mn-doped monolayer CrSi{sub 2} using the first-principle methods based on density functional theory. The results show that both monolayer CrSi{sub 2} sheets are metallic and ferromagnetic (FM) that hold promise in future 2D magnetic devices. In spite the slight reduction of the total magnetic moment of system after Mn doping in monolayer CrSi{sub 2}, the formation energies of ferromagnetic CrSi{sub 2} are also reduced. So, Mn doping in monolayer CrSi{sub 2} can have more promising applications in spintronics and magnetic storage. The optical properties of monolayer CrSi{sub 2}, including the absorption spectra, reflectivity, refractive index, loss function and dielectric function are also calculated. The intensity of reflectivity in far-infrared ranges is enhanced and real part n of refractive index decreases after Mn doping. The real part n of the refractive index is nearly constant (˜1) beyond 13 eV indicating that monolayer CrSi2 is vacuum like and fully transparent.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗