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At least 469 records · Page 26

Data for Magnetic Anisotropy due to Localized Structural Defects in Strained Yttrium Iron Garnet Thin Films

This dataset contains electron microscopy, magnetic, and X-ray diffraction characterization data for YIG/YSGG thin films associated with the manuscript "Magnetic anisotropy due to localized structural defects in strained yttrium iron garnet thin films". Characterizations include: scanning electron nano diffraction (SEND, or 4D-STEM), dark field transmission electron microscopy (DF-TEM), energy dispersive X-ray spectroscopy (EDS), ferrimagnetic resonance (FMR), superconducting quantum interference device (SQUID), scanning transmission electron microscopy (STEM), X-ray diffraction (XRD).

Electron microscopy↗

Quantum-enhanced phase imaging without coincidence counting

Quantitative phase imaging provides a way to image transparent objects, such as biological cells, and measure their thickness. We report on a phase-imaging method that achieves twice the phase shift and approximately 1.7 times the spatial resolution of an equivalent spatially and temporally coherent classical quantitative phase-imaging system by using quantum interference between successive spontaneous parametric downconversion events in a nonlinear crystal. Furthermore, our method is approximately 1000 times faster than imaging the parametric downconversion photons in coincidence, which requires measurement times on the order of tens of hours. Our method may be useful for imaging sensitive transparent objects that require low illumination intensities at near-infrared and longer illumination wavelengths, such as photosensitive biological samples.

47 OTHER INSTRUMENTATION↗

Non-Invasive Functional-Brain-Imaging with an OPM-based Magnetoencephalography System

A non-invasive functional-brain-imaging system based on optically-pumped-magnetometers (OPM) is presented. The OPM-based magnetoencephalography (MEG) system features 20 OPM channels conforming to the subject’s scalp. We have conducted two MEG experiments on three subjects: assessment of somatosensory evoked magnetic field (SEF) and auditory evoked magnetic field (AEF) using our OPM-based MEG system and a commercial MEG system based on superconducting quantum interference devices (SQUIDs). We cross validated the robustness of our system by calculating the distance between the location of the equivalent current dipole (ECD) yielded by our OPM-based MEG system and the ECD location calculated by the commercial SQUID-based MEG system. We achieved sub-centimeter accuracy for both SEF and AEF responses in all three subjects. Due to the proximity (12 mm) of the OPM channels to the scalp, it is anticipated that future OPM-based MEG systems will offer enhanced spatial resolution as they will capture finer spatial features compared to traditional MEG systems employing SQUIDs.

60 APPLIED LIFE SCIENCES↗

Magnetic relaxometry as applied to sensitive cancer detection and localization

Abstract Here we describe superparamagnetic relaxometry (SPMR), a technology that utilizes highly sensitive magnetic sensors and superparamagnetic nanoparticles for cancer detection. Using SPMR, we sensitively and specifically detect nanoparticles conjugated to biomarkers for various types of cancer. SPMR offers high contrast In SPMR measurements, a brief magnetizing pulse is used to align superparamagnetic nanoparticles of a discrete size. Following the pulse, an array of superconducting quantum interference detectors (SQUID) sensors detect the decaying magnetization field. NP size is chosen so that, when bound, the induced field decays in seconds. They are functionalized with specific biomarkers and incubated with cancer cells As a result, superparamagnetic NPs developed here have small size dispersion. Cell incubation studies measure specificity for different cell lines and antibodies with very high contrast.

59 BASIC BIOLOGICAL SCIENCES↗

Accelerated microwave-assisted synthesis and in situ X-ray scattering of tungsten-substituted vanadium dioxide (V 1-x W x O 2 )

Vanadium dioxide (VO 2 ) has been widely studied due to its metal-insulator phase transition at 68°C, below which it is a semiconducting monoclinic phase, P2 1 /c, and above it is a metallic tetragonal phase, P4 2 /mnm. Substituting vanadium with transition metals allows transition temperature tunability. An accelerated microwave-assisted synthesis for VO 2 and 5d tungsten substituted VO 2 presented herein decreased synthesis time by three orders of magnitude while maintaining phase purity, particle size, and transition character. Tungsten substitution amount was determined using inductively coupled plasma-optical emission spectroscopy. Differential scanning calorimetry, superconducting quantum interference device measurements, and in-situ heating and cooling experiments monitored through synchrotron x-ray diffraction (XRD) confirmed the transition temperature decreased with increased tungsten substitution. Scanning electron microscopy analyzed through the line-intercept method produced an average particle size of 3 – 5 μm. Average structure and local structure phase purity was determined through Rietveld analysis of synchrotron XRD and least-squares refinement of pair-distribution function data.

36 MATERIALS SCIENCE↗

Synthesis and behavior of bulk iron nitride soft magnets via high-pressure spark plasma sintering

Abstract In this study, dense bulk iron nitrides (Fe x N) were synthesized for the first time ever using spark plasma sintering (SPS) of Fe x N powders. The Fe 4 N phase of iron nitride in particular has significant potential to serve as a new soft magnetic material in both transformer and inductor cores and electrical machines. The density of SPSed Fe x N increased with SPS temperature and pressure. The microstructure of the consolidated bulk Fe x N was characterized with X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM), and superconducting quantum interference device (SQUID) magnetometry. XRD revealed a primary phase of Fe 4 N with secondary phases of Fe 3 N and metallic iron. Finite element analysis (FEA) was also applied to investigate and explain localized heating and temperature distribution during SPS. The effects of processing on interface bonding formation and phase evolution were investigated and discussed in detail to provide insight into fundamental phenomena and microstructural evolution in SPSed Fe x N. Graphic abstract

36 MATERIALS SCIENCE↗

SQUID Noise Measurements for CDMS Detectors

The Cryogenic Dark Matter Search is the second iteration of SuperCDMS dark matter experiments with an increase in sensitivity to low mass dark matter particles. The experiment uses germanium and silicon crystals which are capable of detecting both the charges and phonon signals produced from dark matter interactions. Detectors are housed in towers which are then housed in a cryogenics system able to cool down to 15 mK. The experiment will be installed in an underground lab in Sudbury, Ontario in order to shield from cosmic rays and background radiation. SQUIDs are an acronym for superconducting quantum interference devices that are capable of detecting extremely small magnetic fields. A typical dark matter nuclear recoil interaction can be detected by a TES (transition edge sensor). SQUIDs are then used to read out and amplify the signals generated by the TES. It is essential that these SQUIDS add negligible noise to the intrinsic noise of the TES to be able to distinguish the internal circuit noise from a true dark matter interaction signal. The noise was measured while varying several parameters. Both an Agilent and an SRS785 spectrum analyzer were used. Furthermore, an amplifier which amplified the signal 10x was tested. The Agilent machine produced more noticeably greater noise in the region from 100-1000 Hz, whereas the SRS785 did not. Next, the amplifier was tested and the signal generated was analyzed in comparison to the original signal. The amplifier did not produce any noticeable additional noise over the intrinsic noise of the SQUID. Further work includes testing to see if detectors with higher voltage sources can also be used with negligible noise.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Identifying Muons for Neutrino Oscillation and Cross Section Experiments

Neutrinos ($\nu$) are interesting for many reasons; they are the only fundamental fermions which are electrically neutral; their mass is orders of magnitude smaller than the lightest charged lepton, the electron; and their solely weak interactions make them an excellent probe of the weak nuclear force. However, one of the most interesting aspects of neutrinos is that, unlike their charged lepton partners, neutrino mass and flavor eigenstates are not the same. All leptons possess 'lepton flavor', a property which is conserved in neutrino interactions. However, because of the difference in the mass and weak eigenstates of neutrinos, a quantum-interference effect is seen in the time evolution of neutrinos. This results in energy and distance dependent oscillations of the neutrino's lepton flavor called 'neutrino oscillations'. The MINOS experiment (Main Injector Neutrino Oscillation Search) was designed to measure the neutrino oscillation parameters, $\Delta m^2_{32}$ and $sin^2(2\theta_{32})$. MINOS is composed of two detectors located on a 'beam' of v[subscript mu]s. The MINOS Near Detector is located at Fermilab, and the Far Detector is located at the Soudan Mine in Minnesota, 734 km after the Near Detector. The MINER$\nu$A experiment (Main Injector Neutrino Experiment for $\nu$ - A) is a neutrino experiment placed directly in front of the MINOS Near Detector. MINER$\nu$s goal is to make precision measurements of neutrino cross sections. This will help with uncertainties in oscillation measurements, such as MINOS' at low energy. Although lepton flavor is conserved in neutrino interactions, the final state lepton can be a charged lepton ('charged current' interactions) or a neutrino ('neutral current' interactions) of a particular flavor. The identification of charged current $\nu_\mu$ interactions through the identification of a muon in the final state is a critical component to both neutrino oscillation and cross section measurements; neutral current events are a background to the oscillation signal bec! ause the properties of the incoming neutrino cannot be determined. Such identification is particularly difficult and important for low-energy neutrino events. In this thesis, we will discuss improvements to the MINOS charged current identification at low energies, studies to estimate the effect of the neutral current background on the measurement of the oscillation parameters, and the aspects of muon identification which are similar for the MINOS and MINER$\nu$A experiments. In 2010, the MINOS experiment released a measurement of the oscillation parameters based on $7.32x10^{20}$ POT. The results were $\Delta m^2_{32} = 2.32^{+.012}_{-0.08} x 10^3 eV^2$, and $sin^2(2\theta_{32}) > 0.90(90%,C.L.)$. This is the best measurement of the oscillation parameter, $\Delta m^2_{32}$, and a competitive measurement of $sin^2(2\theta_{32})$. The improvements to the charged current event selection helped MINOS observe a complete oscillation in neutrino energy.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Developing Quantum Levitation of ICF Capsules Coated with MgB 2 Thin Films

Current inertial confinement fusion (ICF) capsule support technologies create implosion perturbations which reduce fusion yield, driving the search for new support paradigms. Quantum levitation of the capsule will eliminate the requirement of a physical support structure, increasing fusion yield. The application of an external magnetic field to a capsule coated with a superconducting film can provide the necessary conditions for levitation. Magnesium diboride (MgB 2 ) is an attractive option for ICF applications as it has a high reported superconducting transition temperature of 39 K and is a low Z compound. This project is part of an ongoing effort which seeks to coat ICF capsules with a thin layer of superconducting MgB 2 . This project studied the synthesis of MgB 2 and diffusion/reaction kinetics of B/Mg/B m ultilayer thin films. These films were sputter deposited on flat glassy carbon substrates. Films were annealed in a tube furnace at temperatures between 400 °C and 650 °C for a total of 29 hours with film characterization done at predetermined intervals. At each interval, superconducting properties of the samples were evaluated with superconducting quantum interference device (SQUID) magnetometry, while Rutherford backscattering (RBS) with 2 MeV 4 He + ions was done to determine the composition and depth profile of the films. Scanning electron microscopy (SEM) and atomic force microscopy (AFM) were used to characterize surface morphology. Superconducting behavior was observed in thin films annealed at and above 450 °C. Formation of superconducting MgB 2 at 450 °C h as not been previously reported below 500 °C. The surface of the samples annealed at 500 °C and below was smooth with a measured roughness of ~3 nm. After 29 hours of annealing time, the 450 °C sample had a transition temperature of 27.3 K. The highest transition temperature measured was 30.9 K and was associated with a sample annealed for 29 hours at 650 °C. Transition temperatures were weakly positively correlated with annealing temperature and showed dependence on initial structural quality and oxygen contamination. Current research is attempting to synthesize superconducting MgB 2 coatings on spherical Si beads with the findings of this study. Future efforts are focused on the construction and testing of a levitation apparatus.

36 MATERIALS SCIENCE↗

Cationic Ordering and Its Influence on the Magnetic Properties of Co-Rich Cobalt Ferrite Thin Films Prepared by Reactive Solid Phase Epitaxy on Nb-Doped SrTiO 3 (001)

Here, we present the (element-specific) magnetic properties and cation ordering for ultrathin Co-rich cobalt ferrite films. Two Co-rich Co x Fe 3-x O 4 films with different stoichiometry (x=1.1 and x=1.4) have been formed by reactive solid phase epitaxy due to post-deposition annealing from epitaxial CoO/Fe 3 O 4 bilayers deposited before on Nb-doped SrTiO 3 (001). The electronic structure, stoichiometry and homogeneity of the cation distribution of the resulting cobalt ferrite films were verified by angle-resolved hard X-ray photoelectron spectroscopy. From X-ray magnetic circular dichroism measurements, the occupancies of the different sublattices were determined using charge-transfer multiplet calculations. For both ferrite films, a partially inverse spinel structure is found with increased amount of Co 3+ cations in the low-spin state on octahedral sites for the Co 1.4 Fe 1.6 O 4 film. These findings concur with the results obtained by superconducting quantum interference device measurements. Further, the latter measurements revealed the presence of an additional soft magnetic phase probably due to cobalt ferrite islands emerging from the surface, as suggested by atomic force microscope measurements.

36 MATERIALS SCIENCE↗

Structure-Related Electronic and Magnetic Properties in Ultrathin Epitaxial Ni x Fe 3–x O 4 Films on MgO(001)

Off-stoichiometric Ni x Fe 3–x O 4 ultrathin films (x < 2.1) with varying Ni content x and thickness 16 (±2) nm were grown on MgO(001) by reactive molecular beam epitaxy. Synchrotron-based high-resolution X-ray diffraction measurements reveal vertical compressive strain for all films, resulting from a lateral pseudomorphic adaption of the film to the substrate lattice without any strain relaxation. Complete crystallinity with smooth interfaces and surfaces is obtained independent of the Ni content x. For x < 1 an expected successive conversion from Fe 3 O 4 to NiFe 2 O 4 is observed, whereas local transformation into NiO structures is observed for films with Ni content x > 1. However, angle-resolved hard X-ray photoelectron spectroscopy measurements indicate homogeneous cationic distributions without strictly separated phases independent of the Ni content, while X-ray absorption spectroscopy shows that also for x > 1, not all Fe 2+ cations are substituted by Ni 2+ cations. The ferrimagnetic behavior, as observed by superconducting quantum interference device magnetometry, is characterized by decreasing saturation magnetization due to the formation of antiferromagnetic NiO parts.

36 MATERIALS SCIENCE↗

Influence of Resonances on the Noise Performance of SQUID Susceptometers

Scanning Superconducting Quantum Interference Device (SQUID) Susceptometry simultaneously images the local magnetic fields and susceptibilities above a sample with sub-micron spatial resolution. Further development of this technique requires a thorough understanding of the current, voltage, and flux ( I V Φ ) characteristics of scanning SQUID susceptometers. These sensors often have striking anomalies in their current–voltage characteristics, which we believe to be due to electromagnetic resonances. The effect of these resonances on the performance of these SQUIDs is unknown. To explore the origin and impact of the resonances, we develop a model that qualitatively reproduces the experimentally-determined I V Φ characteristics of our scanning SQUID susceptometers. We use this model to calculate the noise characteristics of SQUIDs of different designs. We find that the calculated ultimate flux noise is better in susceptometers with damping resistors that diminish the resonances than in susceptometers without damping resistors. Such calculations will enable the optimization of the signal-to-noise characteristics of scanning SQUID susceptometers.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Germanium coated microbridge and method

A superconducting microbridge is provided for use in superconducting quantum interference devices wherein a pair of spaced layers of superconductive material are connected by a weak link bridge to establish an electrical junction. The superconductive layers and bridge are coated with a semiconductor material shunting the bridge at room temperatures to prevent the destruction of the device by minute electrical currents while the coating acts as a dielectric permitting normal electrical behavior of the microbridge at cryogenic temperatures.

Holderman, L. B.↗

Biomagnetic instrumentation and measurement

The instruments and techniques of biomagnetic measurement have progressed greatly in the past 15 years and are now of a quality appropriate to clinical applications. The paper reports on recent developments in the design and application of SQUID (Superconducting Quantum Interference Device) magnetometers to biomagnetic measurement. The discussion covers biomagnetic field levels, magnetocardiography, magnetic susceptibility plethysmography, ambient noise and sensor types, principles of operation of a SQUID magnetometer, and laboratory techniques. Of the many promising applications of noninvasive biomagnetic measurement, magnetocardiography is the most advanced and the most likely to find clinical application in the near future.

Iufer, E. J.↗

Improved LEEM ranges over four decades

Low-energy electron magnetometer is suitable for terrestrial and aerial applications. Electron beam strikes tantalum collector plates in device, amplifying current and converting it to frequency. Current difference increases with beam deflection, providing measure of local field strength. LEEM operation requires no liquid helium unlike superconducting quantum interference device. LEEM sensitivity compares favorably with that of optical absorption magnetometers, and microsecond response range makes analyzing fast magnetic transients and signatures possible.

Singh, J. J.↗

Space applications of superconductivity - Low frequency superconducting sensors

Although this paper deals with several low-frequency instruments and devices, most of the discussion relates to SQUID (Superconducting QUantum Interference Device) magnetometers and gradiometers, since these are perceived as the instruments with the greatest potential for space applications. The discussion covers SQUID for magnetic field measurements; present state of the art of SQUID technology; ultimate potential performance; applications to magnetic measurements in space; SQUID galvanometers, voltage and current sensors, and wide-band amplifiers; magnetic shielding, and superconducting dc transformer. SQUIDS are superior to all other magnetic sensors in sensitivity, frequency response, range, and linearity. It is suggested that SQUID instruments, both magnetometers and gradiometers, would be valuable in studies of the dynamics of interplanetary and planetary fields. SQUID gradiometers are useful for detection and mapping of magnetic anomalies at short to moderate ranges.

Zimmerman, J. E.↗

Three-Axis Superconducting Gravity Gradiometer

Gravity gradients measured even on accelerating platforms. Three-axis superconducting gravity gradiometer based on flux quantization and Meissner effect in superconductors and employs superconducting quantum interference device as amplifier. Incorporates several magnetically levitated proof masses. Gradiometer design integrates accelerometers for operation in differential mode. Principal use in commercial instruments for measurement of Earth-gravity gradients in geo-physical surveying and exploration for oil.

Paik, Ho Jung↗

SQUID readout and ultra-low magnetic fields for Gravity Probe-B (GP-B)

The superconducting readout system to be used for resolving 0.001 arcsec changes in the gyroscope spin direction in the Relativity Gyroscope (GP-B) experiment is described. This system couples the London magnetic moment flux of the spinning gyro to a low noise superconducting quantum interference device (SQUID) detector. Resolution limits and noise performance of the detection system are discussed, and improvements obtained and expected with advanced SQUIDs are presented. Also described is the novel use of superconducting magnetic shielding techniques to obtain a 250 dB attenuation of the earth's magnetic field at the location of the gyroscopes. In this approach, expanded superconducting foil shields are coupled with fixed cylindrical superconducting shields and special geometric considerations to obtain the extremely high attenuation factor required. With these shielding techniques, it appears that the 0.5-Gauss earth field (which appears to the gyroscopes as an ac field at the satellite roll rate) can be reduced to the 10 to the -13th G level required by the experiment. Recent results concerning improvements in the performance of the superconducting foil techniques obtained with the use of a new computer-controlled cooling system are presented.

Lockhart, James M.↗