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At least 469 records · Page 26

Use of Collocated KWAJEX Satellite, Aircraft, and Ground Measurements for Understanding Ambiguities in TRMM Radiometer Rain Profile Algorithm

Coordinated ground, aircraft, and satellite observations are analyzed from the 1999 TRMM Kwajalein Atoll field experiment (KWAJEX) to better understand the relationships between cloud microphysical processes and microwave radiation intensities in the context of physical evaluation of the Level 2 TRMM radiometer rain profile algorithm and uncertainties with its assumed microphysics-radiation relationships. This talk focuses on the results of a multi-dataset analysis based on measurements from KWAJEX surface, air, and satellite platforms to test the hypothesis that uncertainties in the passive microwave radiometer algorithm (TMI 2a12 in the nomenclature of TRMM) are systematically coupled and correlated with the magnitudes of deviation of the assumed 3-dimensional microphysical properties from observed microphysical properties. Re-stated, this study focuses on identifying the weaknesses in the operational TRMM 2a12 radiometer algorithm based on observed microphysics and radiation data in terms of over-simplifications used in its theoretical microphysical underpinnings. The analysis makes use of a common transform coordinate system derived from the measuring capabilities of the aircraft radiometer used to survey the experimental study area, i.e., the 4-channel AMPR radiometer flown on the NASA DC-8 aircraft. Normalized emission and scattering indices derived from radiometer brightness temperatures at the four measuring frequencies enable a 2-dimensional coordinate system that facilities compositing of Kwajalein S-band ground radar reflectivities, ARMAR Ku-band aircraft radar reflectivities, TMI spacecraft radiometer brightness temperatures, PR Ku-band spacecraft radar reflectivities, bulk microphysical parameters derived from the aircraft-mounted cloud microphysics laser probes (including liquid/ice water contents, effective liquid/ice hydrometeor radii, and effective liquid/ice hydrometeor variances), and rainrates derived from any of the individual ground, aircraft, or satellite algorithms applied to the radar or radiometer measurements, or their combination. The results support the study's underlying hypothesis, particularly in context of ice phase processes, in that the cloud regions where the 2a12 algorithm's microphysical database most misrepresents the microphysical conditions as determined by the laser probes, are where retrieved surface rainrates are most erroneous relative to other reference rainrates as determined by ground and aircraft radar. In reaching these conclusions, TMI and PR brightness temperatures and reflectivities have been synthesized from the aircraft AMPR and ARMAR measurements with the analysis conducted in a composite framework to eliminate measurement noise associated with the case study approach and single element volumes obfuscated by heterogeneous beam filling effects. In diagnosing the performance of the 2a12 algorithm, weaknesses have been found in the cloud-radiation database used to provide microphysical guidance to the algorithm for upper cloud ice microphysics. It is also necessary to adjust a fractional convective rainfall factor within the algorithm somewhat arbitrarily to achieve satisfactory algorithm accuracy.

Smith, Eric A.↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-resolving Model Simulations

Cloud microphysics is inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, r d a U production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensembe1 (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e. pristine ice crystals (columnar and platelike), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and in the mid-latitude continent with different concentrations of CCN: a low "c1ean"concentration and a high "dirty" concentration. In addition, differences and similarities between bulk microphysics and spectral-bin microphysical schemes will be examined and discussed.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics is inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensembel (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e. pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and in the mid-latitude continent with different concentrations of CCN: a low "c1ean"concentration and a high "dirty" concentration. In addition, differences and similarities between bulk microphysics and spectral-bin microphysical schemes will be examined and discussed.

Tao, Wei-Kuo↗

Aerosol Models from the AERONET Database: Application to Surface Reflectance Validation Satellite Data

Aerosols play a critical role in radiative transfer within the atmosphere, and they have a significant impact on climate change. In this paper, we propose and implement a framework for developing an aerosol model using their microphysical properties. Such microphysical properties as the size distribution, the complex refractive index, and the percentage of sphericity are derived from the global AERosol RObotic NETwork (AERONET). These measurements, however, are typically retrieved when almucantar measurement procedures are performed (i.e., early mornings and late afternoons with clear sky) and might not have a temporal correspondence to a satellite overpass time, so a valid validation of satellite-derived products cannot be carried out. To address this problem of temporal inconsistency of satellite and ground-based measurements, we developed an approach to retrieve these microphysical properties (and the corresponding aerosol model) using the optical thickness at 440 nm, τ440, and the Ångström coefficient between 440 and 870 nm, α440–870. Such aerosol models were developed for 851 AERONET sites within the last 28 years. Obtained results suggest that empirically microphysical properties can be retrieved with uncertainties of up to 23 %. An exception is the imaginary part of the refractive index ni, for which the derived uncertainties reach up to 38 %. These specific parametric models of aerosol can be used for the studies when retrieval of microphysical properties is required as well as validation of satellite-derived products over land. Specifically, we demonstrate the usefulness of the aerosol models to validate surface reflectance records over land derived from optical remote sensing sensors. We then quantify the propagation of uncertainties in the surface reflectance due to uncertainties with the aerosol model retrieval that is used as a reference from radiative transfer simulations. Results indicate that individual aerosol microphysical properties can impact uncertainties in surface reflectance retrievals between 3.5 × 10(exp -5) to 1 × 10(exp -3) (in reflectance units). The overall impact of microphysical properties combined yields an overall uncertainty in surface reflectance <0.004 (in reflectance units). That corresponds, for example, to 1 to 3 % of the retrieved surface reflectance in the red spectral band (620–670 nm) by the Moderate Resolution Imaging Spectroradiometer (MODIS) instrument. These uncertainty values are well below the specification (0.005 + 0.05ρ; ρ is the retrieved surface reflectance) used for the MODIS atmospheric correction.

Jean-Claude Roger↗

Using Machine Learning to Predict Cloud Turbulent Entrainment–Mixing Processes

Different turbulent entrainment–mixing mechanisms between clouds and environment are essential to cloud–related processes; however, accurate representation of entrainment–mixing in weather/climate models still poses a challenge. This study exploits the use of machine learning (ML) to address this challenge. Four ML (Light Gradient Boosting Machine [LGB], eXtreme Gradient Boosting, Random Forest, and Support Vector Regression) are examined and compared. It is found that LGB performs best, and thus is selected to understand the impact of entrainment–mixing on microphysics using simulation data from Explicit Mixing Parcel Model. Compared with traditional parameterizations, the trained LGB provides more accurate microphysical properties (number concentration and cloud droplet spectral dispersion). The partial dependences of predicted microphysics on features exhibit a strong alignment with physical mechanisms and expectations, as determined by the interpreting method, thus overcoming the limitations of the “black box” scheme. The underlying mechanisms are that the smaller number concentration and larger spectral dispersion correspond to more inhomogeneous entrainment–mixing. Specifically, number concentration after entrainment–mixing is positively correlated with adiabatic number concentration and liquid water content affected by entrainment–mixing, and inversely correlated with adiabatic volume mean radius. Spectral dispersion after entrainment–mixing is negatively correlated with liquid water content affected by entrainment–mixing, turbulent dissipation rate and relative humidity of entrained air. Sensitivity analysis further suggests that number concentration is mainly determined by cloud microphysical properties whereas spectral dispersion is influenced by both cloud microphysical properties and environmental variables. The results indicate that the LGB scheme has the potential to enhance the representation of entrainment–mixing in weather/climate models.

54 ENVIRONMENTAL SCIENCES↗

A Model Intercomparison Study to Investigate Mixing Characteristics in Non‐Precipitating Stratocumulus Clouds

Recent aircraft observations of marine stratocumulus clouds consistently showed that cloud microphysical relationships vary with altitude, indicating inhomogeneous mixing characteristics near cloud top and homogeneous mixing characteristics in mid-levels of clouds. Here, we conduct model intercomparison of an idealized, non-precipitating stratocumulus cloud to evaluate model consistency and examine whether simulations can reproduce the observed mixing characteristics. The results show that eleven large-eddy simulations with various dynamics and microphysics schemes show good agreement on the thermodynamical, microphysical, and dynamical properties of the stratocumulus-topped boundary layer in a steady state. The inter-model spread in steady-state liquid water path is significantly reduced compared to previous model intercomparison studies. This improvement might be due to better models and more consistent initial conditions than those used decades ago. In addition, most simulations, including a low-dimensional simulation, capture inhomogeneous mixing characteristics near the cloud top and homogeneous mixing characteristics inside the cloud. Moreover, simulations using Lagrangian microphysics schemes agree better with the observed mixing characteristics compared with those using the bin microphysics schemes. Since most simulations do not fully resolve the entrainment process, the apparent mixing characteristics arise from the variations in the resolved cloud properties. Our results support the vertical circulation mixing hypothesis, which suggests that homogeneous mixing characteristics in mid-levels of clouds are due to the vertical circulation of entrainment-affected and diluted parcels from the cloud top moved to lower levels.

54 ENVIRONMENTAL SCIENCES↗

Cirrus cloud model parameterizations: Incorporating realistic ice particle generation

Recent cirrus cloud modeling studies have involved the application of a time-dependent, two dimensional Eulerian model, with generalized cloud microphysical parameterizations drawn from experimental findings. For computing the ice versus vapor phase changes, the ice mass content is linked to the maintenance of a relative humidity with respect to ice (RHI) of 105 percent; ice growth occurs both with regard to the introduction of new particles and the growth of existing particles. In a simplified cloud model designed to investigate the basic role of various physical processes in the growth and maintenance of cirrus clouds, these parametric relations are justifiable. In comparison, the one dimensional cloud microphysical model recently applied to evaluating the nucleation and growth of ice crystals in cirrus clouds explicitly treated populations of haze and cloud droplets, and ice crystals. Although these two modeling approaches are clearly incompatible, the goal of the present numerical study is to develop a parametric treatment of new ice particle generation, on the basis of detailed microphysical model findings, for incorporation into improved cirrus growth models. For example, the relation between temperature and the relative humidity required to generate ice crystals from ammonium sulfate haze droplets, whose probability of freezing through the homogeneous nucleation mode are a combined function of time and droplet molality, volume, and temperature. As an example of this approach, the results of cloud microphysical simulations are presented showing the rather narrow domain in the temperature/humidity field where new ice crystals can be generated. The microphysical simulations point out the need for detailed CCN studies at cirrus altitudes and haze droplet measurements within cirrus clouds, but also suggest that a relatively simple treatment of ice particle generation, which includes cloud chemistry, can be incorporated into cirrus cloud growth.

Sassen, Kenneth↗

The Estimation of Hydrometeor Profiles from Wideband Microwave Observations

Profiles of the microphysical properties of clouds and raincells are essential in many areas of atmospheric research and operational meteorology. In order to enhance the understanding of the nonlinear and underconstrained relationships between cloud and hydrometeor microphysical profiles and passive microwave brightness temperatures, estimations of cloud profiles for an anvil, a convective, and an updraft region of an oceanic squall were performed. The estimations relied on comparisons between radiative transfer calculations of incrementally estimated microphysical profiles and concurrent dual-altitude wideband brightness temperatures from the 22 February 1993 flight during TOGA-COARE. The wideband observations (10--220 GHz) are necessary for estimating cloud profiles reaching up to 20 km. The low frequencies enhance the rain and cloud water profiles, while the high frequencies are required to detail the higher altitude ice microphysics. A microphysical profile was estimated for each of the three regions of the storm. Each of the three estimated profiles produced calculated brightness temperatures within approximately 10 K of the observations. A majority, of the total iterative adjustment were to the estimated profile's frozen hydrometeor characteristics and were necessary to match the high frequency calculations with the observations. This indicates a need to validate cloud resolving models using high frequencies. Some difficulties matching the 37 GHz observation channels on the DC-8 and ER-2 aircrafts with the calculations simulated at the two aircraft heights (approximately 11 km and 20 km, respectively) were noted and potential causes presented.

Gail M Skofronick-Jackson↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e.,pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.A spectral-bin microphysical model is very expensive from a from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region using identical thermodynamic conditions but with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. Besides the initial differences in aerosol concentration, preliminary results indicate that the low CCN concentration case produces rainfall at the surface sooner than the high CCN case but has less cloud water mass aloft. Because the spectral-bin model explicitly calculates and allows for the examination of both the mass and number concentration of species in each size categor, a detailed analysis of the instantaneous size spectrum can be obtained for the two cases. It is shown that since the low CCN case produces fewer droplets, larger sized develop due to the greater condensational and collectional growth, leading to a broader size spectrum in comparison to the high CCN case.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitable affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distribution parameterized as spectral bin microphysics are needed to explicitly study the effect of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensembel (GCE) model. The formulation for the explicit spectral-bim microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e., pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), groupel and frozen drops/hall] Each type is described by a special size distribution function containing many categories (i.e., 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep cloud systems in the west Pacific warm pool region and in the mid-latitude using identical thermodynamic conditions but with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. Besides the initial differences in aerosol concentration, preliminary results indicate that the low CCN concentration case produces rainfall at the surface sooner than the high CCN case but has less cloud water mass aloft. Because the spectral-bim model explicitly calculates and allows for the examination of both the mass and number concentration of cpecies in each size category, a detailed analysis of the instantaneous size spectrum can be obtained for the two cases. It is shown that since the low CCN case produces fever droplets, larger size develop due to greater condencational and collectional growth, leading to a broader size spectrum in comparison to the high CCN case.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles (i.e., pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail). Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep cloud systems in the west Pacific warm pool region, in the sub-tropics (Florida) and in the mid-latitude using identical thermodynamic conditions but with different concentrations of CCN: a low 'clean' concentration and a high 'dirty' concentration.

Tao, Wei-Kuo↗

A Robust Multi-Scale Modeling System for the Study of Cloud and Precipitation Processes

During the past decade, numerical weather and global non-hydrostatic models have started using more complex microphysical schemes originally developed for high resolution cloud resolving models (CRMs) with 1-2 km or less horizontal resolutions. These microphysical schemes affect the dynamic through the release of latent heat (buoyancy loading and pressure gradient) the radiation through the cloud coverage (vertical distribution of cloud species), and surface processes through rainfall (both amount and intensity). Recently, several major improvements of ice microphysical processes (or schemes) have been developed for cloud-resolving model (Goddard Cumulus Ensemble, GCE, model) and regional scale (Weather Research and Forecast, WRF) model. These improvements include an improved 3-ICE (cloud ice, snow and graupel) scheme (Lang et al. 2010); a 4-ICE (cloud ice, snow, graupel and hail) scheme and a spectral bin microphysics scheme and two different two-moment microphysics schemes. The performance of these schemes has been evaluated by using observational data from TRMM and other major field campaigns. In this talk, we will present the high-resolution (1 km) GeE and WRF model simulations and compared the simulated model results with observation from recent field campaigns [i.e., midlatitude continental spring season (MC3E; 2010), high latitude cold-season (C3VP, 2007; GCPEx, 2012), and tropical oceanic (TWP-ICE, 2006)].

Tao, Wei-Kuo↗

LGM Paleoclimate Constraints Inform Cloud Parameterizations and Equilibrium Climate Sensitivity in CESM2

The Community Earth System Model version 2 (CESM2) simulates a high equilibrium climate sensitivity (ECS > 5°C) and a Last Glacial Maximum (LGM) that is substantially colder than proxy temperatures. In this study, we examine the role of cloud parameterizations in simulating the LGM cooling in CESM2. Through substituting different versions of cloud schemes in the atmosphere model, we attribute the excessive LGM cooling to the new CESM2 schemes of cloud microphysics and ice nucleation. Further exploration suggests that removing an inappropriate limiter on cloud ice number (NoNimax) and decreasing the time-step size (substepping) in cloud microphysics largely eliminate the excessive LGM cooling. NoNimax produces a more physically consistent treatment of mixed-phase clouds, which leads to an increase in cloud ice content and a weaker shortwave cloud feedback over mid-to-high latitudes and the Southern Hemisphere subtropics. Microphysical substepping further weakens the shortwave cloud feedback. Based on NoNimax and microphysical substepping, we have developed a paleoclimate-calibrated CESM2 (PaleoCalibr), which simulates well the observed twentieth century warming and spatial characteristics of key cloud and climate variables. PaleoCalibr has a lower ECS (∼4°C) and a 20% weaker aerosol-cloud interaction than CESM2. PaleoCalibr represents a physically more consistent treatment of cloud microphysics than CESM2 and is a valuable tool in climate change studies, especially when a large climate forcing is involved. Our study highlights the unique value of paleoclimate constraints in informing the cloud parameterizations and ultimately the future climate projection.

equilibrium climate sensitivity↗

Investigating Characteristic Droplet Size Distributions in Large Eddy Simulations of Stratocumulus Clouds

Cloud processes relevant to radiative and precipitation properties depend on the shape of the cloud droplet size distribution. Recent holographic observations revealed that cloud droplet populations do not have the same size distribution shapes throughout but form regions of characteristic distributions with similar microphysical properties. We investigate the existence and properties of these characteristic distributions within Large‐Eddy Simulations of stratocumulus clouds using Lagrangian and bin microphysics schemes. Distribution types are identified, revealing localized characteristic distributions that vary on the scale of the largest convective cell for simulations with bin microphysics. The results from the Lagrangian microphysics scheme hint at similar behavior. Compared to observations, the simulated clouds are much more uniform. Analysis of the LES results suggests a connection to the local entrainment rate, so the poorly resolved entrainment interface in LES may be a cause of the uniformity. The uniformity of the large‐scale forcing could also be a factor.

cloud droplet size distributions↗

Electrification Within Wintertime Stratiform Regions Sampled During the 2020/2022 NASA IMPACTS Field Campaign

Two nor'easter events—sampled during the NASA Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) field campaign—were examined to characterize the microphysics in relation to the underlying electrification processes within wintertime stratiform regions. A theoretical model was developed to determine whether accretion or diffusion growth regimes were preferential during periods of greatest electrification. Model simulation with electrification parameterization was used to provide supplemental context to the physical processes of in-cloud microphysics and electrification. The strongest electric fields (i.e., ∼80 V m −1 at 20 km) during the 2020 NASA IMPACTS deployment was associated with large non-rimed ice crystals colliding with each other. During the 29–30 January 2022 science flight, the NASA P-3 microphysical probe data demonstrated that non-inductive charging was possible off the coastline of Cape Cod, Massachusetts. Later in the science flight, when the NASA P-3 and ER-2 were coordinating with each other, measured electric fields consistently were less than 8 V m −1 and electrification was subdued owing to reduced concentrations of graupel and large ice hydrometeors. Altogether, the in-situ observations provide evidence for the non-riming collisional charging mechanism and demonstrates that graupel and supercooled liquid water may not be necessary for weak electrification within wintertime stratiform regions. Model output from simulation of both events suggested that the main synoptic snowbands were associated with elevated hydrometeor snow charge density and electric fields.

snowfall↗

Dual-Polarization Radar Fingerprints of Precipitation Physics: A Review

This article reviews how precipitation microphysics processes are observed in dual-polarization radar observations. These so-called “fingerprints” of precipitation processes are observed as vertical gradients in radar observables. Fingerprints of rain processes are first reviewed, followed by processes involving snow and ice. Then, emerging research is introduced, which includes more quantitative analysis of these dual-polarization radar fingerprints to obtain microphysics model parameters and microphysical process rates. New results based on a detailed rain shaft bin microphysical model are presented, and we conclude with an outlook of potentially fruitful future research directions.

precipitation↗

Comprehensive Analysis of the Relative Dispersion of Droplet-Size Distributions and Their Relationships to Key Physical Fog Processes Under Different Aerosol Conditions and Evolutionary Stages

The relative dispersion of cloud and fog droplets has significant impacts on aerosol indirect effects, radiative transfer, and microphysical processes. However, previous studies have been mostly concerned with clouds, with limited studies on fog, particularly those that examine the combined influences of all key physical processes and their roles during fog evolution. As such, this study aims to conduct a comprehensive investigation by examining the relationships between relative dispersion and other microphysical variables, as well as the underlying microphysical and dynamic processes, based on field fog campaigns in polluted and clean conditions. In polluted fog, droplet concentrations are higher, leading to smaller droplets and increased dispersion. The correlation between dispersion and droplet volume-mean radius is positive in the polluted fog, but shifts to negative in clean fog. Here, we attribute the difference to various microphysical processes like aerosol activation, condensation, collision-coalescence, and entrainment-mixing. In polluted fog, high aerosol concentrations, low supersaturations, and strong turbulence (entrainment-mixing) provide suitable conditions for the simultaneous occurrence of droplet condensation and aerosol activation, resulting in a positive correlation between dispersion and volume-mean radius, especially during the fog formation stage. In contrast, during the mature stage in clean fog, condensation is dominant with weak aerosol activation leading to a negative correlation between relative dispersion and volume-mean radius. The collision-coalescence process is more active in the mature stage, increasing radii and leading to the negative correlation between dispersion and volume-mean radius. This result sheds new light on understanding the relative dispersion and mechanisms in fog under different aerosol backgrounds.

54 ENVIRONMENTAL SCIENCES↗

Observations of anthropogenic cloud condensation nuclei

Cloud Condensation Nuclei (CCN) concentrations and spectral measurements obtained with the DRI instantaneous CCN spectrometer (Hudson, 1989) over the last few years are presented. The climatic importance of cloud microphysics has been pointed out. The particles which affect cloud microphysics are cloud condensation nuclei (CCN). The commonly-observed order of magnitude difference in cloud droplet concentrations between maritime and continental air masses (i.e., Squires, 1958) was determined to be caused by systematic differences in the concentrations of CCN between continental and maritime air masses (e.g., Twomey and Wojciechowski, 1969). Twomey (1977) first pointed out that cloud microphysics also affects the radiative properties of clouds. Thus continental and anthropogenic CCN could affect global temperature. Resolution of this Twomey effect requires answers to two questions - whether antropogenic CCN are a significant contribution to atmospheric CCN, and whether they are actually affecting cloud microphysics to an extent which is of climatic importance. The reasons for the contrast between continental and maritime CCN concentration are not understood. The question of the relative importance of anthropogenic CCN is addressed. These observations should shed light on this complex question although further research is being conducted in order to produce more quantitative answers. Accompanying CN measurements made with a TSI 3020 condensation nucleus (CN) counter are also presented.

Hudson, James G.↗