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At least 505 records · Page 28

Scattering Properties of the Venusian Clouds Observed by the UV Imager on board Akatsuki

We analyze the albedo of Venus obtained from the UV Imager on board Akatsuki. A relative global mean albedo over phase angle is used in this study, and we confirm the glory feature at 283 and 365 nm in the data acquired in 2016 May. We successfully simulate the observation using a radiative transfer model. Our results show that cloud aerosols of r{sub eff}=1.26 μm and v{sub eff}=0.076 (mode 2) can explain the glory, consistent with a property of aerosols previously suggested by using the Venus Monitoring Camera on board Venus Express. We find that SO{sub 2} and the unknown UV absorber are necessary factors to explain the decreasing trend of the observed relative albedo at phase angles larger than 10°. We suggest a range of possible SO{sub 2} abundance from 80 to 400 ppbv at the cloud top level, depending on atmospheric conditions assumed.

79 ASTRONOMY AND ASTROPHYSICS↗

Ultraviolet radiation in the Arctic - The impact of potential ozone depletions and cloud effects

The combined effects of ozone depletions/redistributions and particulate clouds on atmospheric cheating/photolysis rates and UV radiation reaching the biosphere are investigated by means of an atmospheric radiation model. Consideration is given to four types of particulate clouds prevalent in the summertime Arctic: stratospheric aerosols, tropospheric aerosols (Arctic haze), cirrus clouds, and stratus clouds. The effects of ozone depletion and vertical redistributions of ozone are also examined. Stratus clouds are found to provide significant protection from UV radiation exposure, but while stratospheric aerosols imply increased UVB exposure, Arctic haze results in a decrease. A redistribution of ozone from the stratosphere to the troposphere tends to decrease UV exposure, but for low solar elevations an increase may occur. A 20-percent ozone depletion leads to about 0.4 K/d cooling in the lower stratosphere, while redistribution of ozone from the stratosphere to the troposphere implies a warming of about 0.015 K/d in the upper troposphere.

Tsay, Si-Chee↗

Near-global survey of effective droplet radii in liquid water clouds using ISCCP data

A global survey of cloud particle size variations can provide crucial constraints on how cloud processes determine cloud liquid water contents and their variation with temperature, and further, may indicate the magnitude of aerosol effects on clouds. A method, based on a complete radiative transfer model for Advanced Very High Resolution Radiometer (AVHRR)-measured radiances, is described for retrieving cloud particle radii in liquid water clouds from satellite data currently available from the International Satellite Cloud Climatology Project. Results of sensitivity tests and validation studies provide error estimates. AVHRR data from NOAA-9 and NOAA-10 have been analyzed for January, April, July and October in 1987 and 1988. The results of this first survey reveal systematic continental and maritime differences and hemispheric contrasts that are indicative of the effects of associated aerosol concentration differences: cloud droplet radii in continental water clouds are about 2-3 micrometers smaller than in marine clouds, and droplet radii are about 1 micrometer smaller in marine clouds of the Northern Hemisphere than in the Southern Hemisphere. The height dependencies of cloud droplet radii in continental and marine clouds are also consistent with differences in the vertical profiles of aerosol concentration. Significant seasonal and diurnal variations of effective droplet radii are also observed, particularly at lower latitudes. Variations of the relationship between cloud optical thickness and droplet radii may indicate variations in cloud microphysical regimes.

Han, Qingyan↗

Layered Model for Radiation-Induced Chemical Evolution of Icy Surface Composition and Dynamics on Kuiper Belt and Oort Cloud Bodies

The diversity of albedos and surface colors on observed Kuiper Belt and Inner Oort Cloud objects remains to be explained in terms of competition between primordial intrinsic versus exogenic drivers of surface and near-surface evolution. Earlier models have attempted without success to attribute this diversity to the relations between surface radiolysis from cosmic ray irradiation and gardening by meteoritic impacts. A more flexible approach considers the different depth-dependent radiation profiles produced by low-energy plasma, suprathermal, and maximally penetrating charged particles of the heliospheric and local interstellar radiation environment. Generally red objects of the dynamically cold (low inclination, circular orbit) Classical Kuiper Belt might be accounted for from erosive effects of plasma ions and reddening effects of high energy cosmic ray ions, while suprathermal keV-MeV ions could alternatively produce more color neutral surfaces. The deepest layer of more pristine ice can be brought to the surface from meter to kilometer depths by larger impact events and potentially by cryovolcanic activity. The bright surfaces of some larger objects, e.g. Eris, suggest ongoing resurfacing activity. Cycles of atmospheric formation and surface freezeout can further account for temporal variation as observed on Pluto. The diversity of causative processes must therefore be understood to account for observationally apparent diversities of the object surfaces.

Cooper, John F.↗

The Goddard Cumulus Ensemble Model: Model Description and Its Application for Studying the TOGA COARE and GATE Convective Systems

The Goddard Cumulus Ensemble (GCE) model was utilized in two and three dimensions in order to examine the behavior and response of simulated deep tropical cloud systems occurred in west Pacific warm pool region and Atlantic ocean. The periods chosen for simulation were convectively active period over the TOGA-COARE IFA (19-27 December 1992) and GATE (September 1 to 7, 1974). The TOGA COARE IFA period was also in the framework of the GEWEX Cloud System Study (GCSS) WG4 case 2. We will examine the differences between the microphysics (warm rain and ice processes, evaporation/sublimation and condensation/deposition), Q1 (Temperature) and Q2 (Water vapor) budgets between these two convective events occurred in different large-scale environments. The contribution of stratiform precipitation and its relationship to the vertical shear of the large-scale horizontal wind will also be examined. The results from GCSS model intercomparsion will be presented. The new improvements (i.e., microphysics, cloud radiation interaction, surface processes and numerical advection scheme) of the GCE model as well as their sensitivity to the model results will be discussed.

Tao, Wei-Kuo↗

Radiative feedback of polar stratospheric clouds on Antarctic temperatures

A one-dimensional time marching radiative transfer model has been used to investigate the potential effects of polar stratospheric clouds (PSCs) on winter and spring temperatures in the Antarctic lower stratosphere. High, middle, and low PSC amounts were specified from lidar backscatter profiles and were chosen to represent the likely range of PSC amounts present in the Antarctic region. The computed effects of the PSCs on temperatures depend strongly on the surface temperature and on the extent of tropospheric cloudiness, and range from a maximum increase of 6 K for a high amount of PSCs over a warm surface and clear troposphere to a maximum decrease of 2 K for a high amount of PSCs over a cold surface and a troposphere with high clouds. The average effect is unlikely to be more than a 1 or 2 K temperature change.

Rosenfeld, Joan E.↗

Detecting Super-Thin Clouds with Polarized Sunlight

We report a novel method for detecting cloud particles in the atmosphere. Solar radiation backscattered from clouds is studied with both satellite data and a radiative transfer model. A distinct feature is found in the angle of linear polarization of solar radiation that is backscattered from clouds. The dominant backscattered electric field from the clear-sky Earth-atmosphere system is nearly parallel to the Earth surface. However, when clouds are present, this electric field can rotate significantly away from the parallel direction. Model results demonstrate that this polarization feature can be used to detect super-thin cirrus clouds having an optical depth of only ~0.06 and super-thin liquid water clouds having an optical depth of only ~0.01. Such clouds are too thin to be sensed using any current passive satellite instruments.

Aerosols and particles↗

Chemistry of a polluted cloudy boundary layer

A one-dimensional photochemical model for cloud-topped boundary layers has been developed to include descriptions of gas- and aqueous-phase chemistry and the radiation field in and below the cloud. The model is applied to the accumulation of pollutants during a wintertime episode with low stratus over Bakersfield, CA. The mechanisms of sulfate production and the balance between the concentrations of acids and bases are examined. It is shown that most of the sulfate production may be explained by the Fe(III)-catalyzed autoxidation of S(IV). Another source of sulfate is the oxidation of SO2 by OH in both the gas and the aqueous phase. It is shown that the sulfate production in the model is controlled by the availability of NH3. It is suggested that this explains the balance observed between total concentration of acids and bases.

Jacob, Daniel J.↗

Simultaneous Retrieval of Aerosol and Cloud Properties During the MILAGRO Field Campaign

Estimation of Direct Climate Forcing (DCF) due to aerosols in cloudy areas has historically been a difficult task, mainly because of a lack of appropriate measurements. Recently, passive remote sensing instruments have been developed that have the potential to retrieve both cloud and aerosol properties using polarimetric, multiple view angle, and multi spectral observations, and therefore determine DCF from aerosols above clouds. One such instrument is the Research Scanning Polarimeter (RSP), an airborne prototype of a sensor on the NASA Glory satellite, which unfortunately failed to reach orbit during its launch in March of 2011. In the spring of 2006, the RSP was deployed on an aircraft based in Veracruz, Mexico, as part of the Megacity Initiative: Local and Global Research Observations (MILAGRO) field campaign. On 13 March, the RSP over flew an aerosol layer lofted above a low altitude marine stratocumulus cloud close to shore in the Gulf of Mexico. We investigate the feasibility of retrieving aerosol properties over clouds using these data. Our approach is to first determine cloud droplet size distribution using the angular location of the cloud bow and other features in the polarized reflectance. The selected cloud was then used in a multiple scattering radiative transfer model optimization to determine the aerosol optical properties and fine tune the cloud size distribution. In this scene, we were able to retrieve aerosol optical depth, the fine mode aerosol size distribution parameters and the cloud droplet size distribution parameters to a degree of accuracy required for climate modeling. This required assumptions about the aerosol vertical distribution and the optical properties of the coarse aerosol size mode. A sensitivity study was also performed to place this study in the context of future systematic scanning polarimeter observations, which found that the aerosol complex refractive index can also be observed accurately if the aerosol optical depth is larger than roughly 0.8 at a wavelength of (0.555 m).

Knobelspiesse, K.↗

Cloud feedback mechanisms and their representation in global climate models

Cloud feedback—the change in top-of-atmosphere radiative flux resulting from the cloud response to warming—constitutes by far the largest source of uncertainty in the climate response to CO 2 forcing simulated by global climate models (GCMs). In this paper, we review the main mechanisms for cloud feedbacks, and discuss their representation in climate models and the sources of intermodel spread. Global-mean cloud feedback in GCMs results from three main effects: (1) rising free-tropospheric clouds (a positive longwave effect); (2) decreasing tropical low cloud amount (a positive shortwave [SW] effect); (3) increasing high-latitude low cloud optical depth (a negative SW effect). These cloud responses simulated by GCMs are qualitatively supported by theory, high-resolution modeling, and observations. Rising high clouds are consistent with the fixed anvil temperature (FAT) hypothesis, whereby enhanced upper-tropospheric radiative cooling causes anvil cloud tops to remain at a nearly fixed temperature as the atmosphere warms. Tropical low cloud amount decreases are driven by a delicate balance between the effects of vertical turbulent fluxes, radiative cooling, large-scale subsidence, and lower-tropospheric stability on the boundary-layer moisture budget. High-latitude low cloud optical depth increases are dominated by phase changes in mixed-phase clouds. Finally, the causes of intermodel spread in cloud feedback are discussed, focusing particularly on the role of unresolved parameterized processes such as cloud microphysics, turbulence, and convection.

54 ENVIRONMENTAL SCIENCES↗

Fast and slow shifts of the zonal-mean intertropical convergence zone in response to an idealized anthropogenic aerosol

Previous modeling work showed that aerosol can affect the position of the tropical rain belt, i.e., the intertropical convergence zone (ITCZ). Yet it remains unclear which aspects of the aerosol impact are robust across models, and which are not. Here we present simulations with seven comprehensive atmosphere models that study the fast and slow impacts of an idealized anthropogenic aerosol on the zonal-mean ITCZ position. The fast impact, which results from aerosol atmospheric heating and land cooling before sea-surface temperature (SST) has time to respond, causes a northward ITCZ shift. Yet the fast impact is compensated locally by decreased evaporation over the ocean, and a clear northward shift is only found for an unrealistically large aerosol forcing. The local compensation implies that while models differ in atmospheric aerosol heating, this does not contribute to model differences in the ITCZ shift. The slow impact includes the aerosol impact on the ocean surface energy balance and is mediated by SST changes. The slow impact is an order of magnitude more effective than the fast impact and causes a clear southward ITCZ shift for realistic aerosol forcing. Models agree well on the slow ITCZ shift when perturbed with the same SST pattern. However, an energetic analysis suggests that the slow ITCZ shifts would be substantially more model-dependent in interactive-SST setups due to model differences in clear-sky radiative transfer and clouds. In conclusion, we also discuss implications for the representation of aerosol in climate models and attributions of recent observed ITCZ shifts to aerosol.

54 ENVIRONMENTAL SCIENCES↗

Ship‐Based Lidar Evaluation of Southern Ocean Low Clouds in the Storm‐Resolving General Circulation Model ICON and the ERA5 and MERRA‐2 Reanalyses

Global storm resolving models (GSRMs) represent the next generation of global climate models. One of them is a 5-km Icosahedral Nonhydrostatic Weather and Climate Model (ICON). Its high resolution means that parameterizations of convection and clouds, including subgrid-scale clouds, are omitted, relying on explicit simulation but necessarily utilizing microphysics and turbulence parameterizations. Standard-resolution (10–100 km) models, which use convection and cloud parameterizations, have substantial cloud biases over the Southern Ocean (SO), adversely affecting radiation and sea surface temperature. The SO is dominated by low clouds, which cannot be observed accurately from space due to overlapping clouds, attenuation, and ground clutter. We evaluated SO clouds in ICON and the ERA5 and MERRA-2 reanalyzes using approximately 2400 days of lidar observations and 2300 radiosonde profiles from 31 voyages and a Macquarie Island station during 2010–2021, compared to the model and reanalyzes using a ground-based lidar simulator. We found that ICON and the reanalyzes underestimate the total cloud fraction by about 10% and 20%, respectively. ICON and ERA5 overestimate the cloud occurrence peak at about 500 m, associated with underestimated lower tropospheric stability and overestimated lifting condensation level. The reanalyzes strongly underestimate fog and very low-level clouds, and MERRA-2 underestimates cloud occurrence at almost all heights. Outgoing shortwave radiation is overestimated in MERRA-2, implying a “too few, too bright” cloud problem. SO cloud and fog biases are a substantial issue in the analyzed model and reanalyzes and result in shortwave and longwave radiation biases.

Kuma, Peter [Stockholm Univ. (Sweden); Univ. of Ca↗

CERES Clouds and Radiative Swath (CRS) data in HDF. (CER_CRS_Terra-FM1-MODIS_Edition2A)

The Clouds and Radiative Swath (CRS) product contains one hour of instantaneous Clouds and the Earth's Radiant Energy System (CERES) data for a single scanner instrument. The CRS contains all of the CERES SSF product data. For each CERES footprint on the SSF the CRS also contains vertical flux profiles evaluated at four levels in the atmosphere: the surface, 500-, 70-, and 1-hPa. The CRS fluxes and cloud parameters are adjusted for consistency with a radiative transfer model and adjusted fluxes are evaluated at the four atmospheric levels for both clear-sky and total-sky. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2001-12-31] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Temporal_Resolution=1 hour; Temporal_Resolution_Range=Hourly - < Daily].

SHORTWAVE FILTERED RADIANCE↗

Simulations of Aerosol Microphysics in the NASA GEOS-5 Model

Aerosol-cloud-chemistry interactions have potentially large but uncertain impacts on Earth's climate. One path to addressing these uncertainties is to construct models that incorporate various components of the Earth system and to test these models against data. To that end, we have previously incorporated the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) module online in the NASA Goddard Earth Observing System model (GEOS-5). GEOS-5 provides a platform for Earth system modeling, incorporating atmospheric and ocean general circulation models, a land surface model, a data assimilation system, and treatments of atmospheric chemistry and hydrologic cycle. Including GOCART online in this framework has provided a path for interactive aerosol-climate studies; however, GOCART only tracks the mass of aerosols as external mixtures and does not include the detailed treatments of aerosol size distribution and composition (internal mixtures) needed for aerosol-cloud-chemistry-climate studies. To address that need we have incorporated the Community Aerosol and Radiation Model for Atmospheres (CARMA) online in GEOS-5. CARMA is a sectional aerosol-cloud microphysical model, capable of treating both aerosol size and composition explicitly be resolving the aerosol distribution into a variable number of size and composition groupings. Here we present first simulations of dust, sea salt, and smoke aerosols in GEOS-5 as treated by CARMA. These simulations are compared to available aerosol satellite, ground, and aircraft data and as well compared to the simulated distributions in our current GOCART based system.

Colarco, Peter↗

Final Report – Study of Shortwave Spectra in Fully 3D Environment. Synergy Between Scanning Radars and Spectral Radiation Measurements

ARM set out 20 years ago to “close” the radiation problem, that is, to improve radiation models to the point where they could routinely predict the observed spectral radiation fluxes knowing the optical properties of the surface and of gases, clouds and aerosols in the atmosphere. Only then could such radiation models form a proper springboard for global climate model (GCM) parameterizations of spectral radiation. Sustained efforts have more or less achieved that goal with regard to longwave radiation; ASR models now routinely predict ARM spectral longwave radiances to 1–2%. Similar efforts in the shortwave have achieved far less; the successes are mainly for carefully selected 1D stratiform cloud cases. Such cases amount, even with the most optimistic interpretation, to no more than 30% of all cases at SGP. The problem has not been lack of effort but lack of appropriate instruments.The new ARM stimulus-funded instruments, with their new capabilities, will dramatically improve this situation and once again make progress possible on the shortwave problem. The new shortwave spectrometers will provide a reliable, calibrated record including the near infrared – and for other climatic regimes than SGP. The new scanning radars will provide the 3D cloud view, making it possible to tackle fully 3D situations. Thus, our main theme for the project is the understanding and closure of the surface spectral shortwave radiation problem in fully 3D cloud situations by combining the new ARM scanning radars and shortwave spectrometers with the arsenal of radiative transfer tools.

54 ENVIRONMENTAL SCIENCES↗

Evaluating cloud feedbacks and rapid responses in the ACCESS model

A cloud feedback diagnostic package is implemented in the Australian Community Climate and Earth-System Simulator General Circulation Model, based on the methodology of “cloud radiative kernels.” Using separate increased sea surface temperature and CO 2 experiments, both the “rapid response” cloud contribution to forcing and temperature-mediated cloud feedbacks are analyzed. Under increased temperature and CO 2 changes, temperature-mediated cloud radiative feedback dominates over the rapid response in the final radiative response. Cloud feedback is positive in both long and short wave, with short wave dominating global values. Contributing most to this are low to mid-level clouds, of medium-to-high optical thickness. As a means of illustration of the methodology, a number of key parameters related to clouds, precipitation, and convection that are typically used in “tuning” in the model are modified. These changes result in substantial impacts on the model's current climate, but only modest changes to rapid response and feedbacks occur globally, regionally, and as a function of cloud optical thickness and height. This limited set of experiments shows that cloud adjustments and feedbacks in this model are robust under these changes, lending confidence that both model climate change projections and the conclusions of attribution studies are not overly sensitive to such parameterization tuning. Of course, a considerably larger set of experiments would be needed to demonstrate that feedbacks and rapid response are robust under the wider set of tuning adjustments commonly undertaken.

54 ENVIRONMENTAL SCIENCES↗

Cloud Adjustments From Large-Scale Smoke–Circulation Interactions Strongly Modulate the Southeastern Atlantic Stratocumulus-to-Cumulus Transition

Smoke from southern Africa blankets the southeastern Atlantic Ocean from June to October, producing strong and competing aerosol radiative effects. Smoke effects on the transition between overcast stratocumulus and scattered cumulus clouds are investigated along a Lagrangian (air-mass-following) trajectory in regional climate and large eddy simulation models. Results are compared with observations from three recent field campaigns that took place in August 2017: ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES), CLouds and Aerosol Radiative Impacts and Forcing: Year 2017 (CLARIFY), and Layered Atlantic Smoke Interactions with Clouds (LASIC). The case study is set up around the joint ORACLES–CLARIFY flight that took place near Ascension Island on 18 August 2017. Smoke sampled upstream on an ORACLES flight on 15 August 2017 likely entrained into the marine boundary layer later sampled during the joint flight. The case is first simulated with the WRF-CAM5 regional climate model in three distinct setups: (1) FireOn, in which smoke emissions and any resulting smoke–cloud–radiation interactions are included; (2) FireOff, in which no smoke emissions are included; (3) RadOff, in which smoke emissions and their microphysical effects are included but aerosol does not interact directly with radiation. Over the course of the Lagrangian trajectory, differences in free tropospheric thermodynamic properties between FireOn and FireOff are nearly identical to those between FireOn and RadOff, showing that aerosol–radiation interactions are primarily responsible for the free tropospheric effects. These effects are non-intuitive: in addition to the expected heating within the core of the smoke plume, there is also a “banding” effect of cooler temperature (∼1–2 K) and greatly enhanced moisture (>2 g kg−1) at the plume top. This banding effect is caused by a vertical displacement of the former continental boundary layer in the free troposphere in the FireOn simulation resulting from anomalous diabatic heating due to smoke absorption of sunlight that manifests primarily as a few hundred meters per day reduction in large-scale subsidence over the ocean. A large eddy simulation (LES) is then forced with free tropospheric fields taken from the outputs for the WRF-CAM5 FireOn and FireOff runs. Cases are run by selectively perturbing one variable (e.g., aerosol number concentration, temperature, moisture, vertical velocity) at a time to better understand the contributions from different indirect (microphysical), “large-scale” semi-direct (above-cloud thermodynamic and subsidence changes), and “local” semi-direct (below-cloud smoke absorption) effects. Despite a more than 5-fold increase in cloud droplet number concentration when including smoke aerosol concentrations, minimal differences in cloud fraction evolution are simulated by the LES when comparing the base case with a perturbed aerosol case with identical thermodynamic and dynamic forcings. A factor of 2 decrease in background free tropospheric aerosol concentrations from the FireOff simulation shifts the cloud evolution from a classical entrainment-driven “deepening–warming” transition to trade cumulus to a precipitation-driven “drizzle-depletion” transition to open cells, however. The thermodynamic and dynamic changes caused by the WRF-simulated large-scale adjustments to smoke diabatic heating strongly influence cloud evolution in terms of both the rate of deepening (especially for changes in the inversion temperature jump and in subsidence) and in cloud fraction on the final day of the simulation (especially for the moisture “banding” effect). Such large-scale semi-direct effects would not have been possible to simulate using a small-domain LES model alone.

southeast Atlantic Ocean↗

How Consistent are Recent Variations in the Tropical Energy and Water Cycle Resolved by Satellite Measurements?

One notable aspect of Earth's climate is that although the planet appears to be very close to radiative balance at top-of-atmosphere (TOA), the atmosphere itself and underlying surface are not. Profound exchanges of energy between the atmosphere and oceans, land and cryosphere occur over a range of time scales. Recent evidence from broadband satellite measurements suggests that even these TOA fluxes contain some detectable variations. Our ability to measure and reconstruct radiative fluxes at the surface and at the top of atmosphere is improving rapidly. One question is 'How consistent, physically, are these diverse remotely-sensed data sets'? The answer is of crucial importance to understanding climate processes, improving physical models, and improving remote sensing algorithms. In this work we will evaluate two recently released estimates of radiative fluxes, focusing primarily on surface estimates. The International Satellite Cloud Climatology Project 'FD' radiative flux profiles are available from mid-1983 to near present and have been constructed by driving the radiative transfer physics from the Goddard Institute for Space Studies (GISS) global model with ISCCP clouds and TOVS (TIROS Operational Vertical Sounder)thermodynamic profiles. Full and clear sky SW and LW fluxes are produced. A similar product from the NASA/GEWEX Surface Radiation Budget Project using different radiative flux codes and thermodynamics from the NASA/Goddard Earth Observing System (GEOS-1) assimilation model makes a similar calculation of surface fluxes. However this data set currently extends only through 1995. We also employ precipitation measurements from the Global Precipitation Climatology Project (GPCP) and the Tropical Rainfall Measuring Mission (TRMM). Finally, ocean evaporation estimates from the Special Sensor Microwave Imager (SSM/I) are considered as well as derived evaporation from the NCAR/NCEP Reanalysis. Additional information is included in the original extended abstract.

Robertson, F. R.↗