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At least 505 records · Page 28

Global Aerosol Climatology Project: An Update

This paper outlines the methodology of interpreting channe1 1 and 2 AVHRR (Advanced Very High Resolution Radiometer) radiance data over the oceans and describes a detailed analysis of the sensitivity of monthly averages of retrieved aerosol parameters to the assumptions made in different retrieval algorithms. The analysis is based on using real AVHRR data and exploiting accurate numerical techniques for computing single and multiple scattering and spectral absorption of light in the vertically inhomogeneous atmospheric-ocean system. We show that two-channel algorithms can be expected tp provide significantly more biased retrievals of the aerosol optical thickness than one-channel algorithms and that imperfect cloud screening and calibration uncertainties are by far the largest sources of errors in the retrieved aerosol parameters. Both underestimating and overestimating aerosol absorption as well as the potentially strong variability of the real part of the aerosol refractive index may lead to regional and/or seasonal biases in optical thickness retrievals. The Angstrom exponent appears to be the most invariant aerosol size characteristic and should be retrieved along with optical thickness as the second aerosol parameter.

Mishchenko, Michael I.↗

Microphysical modeling of cirrus. 1: Comparison with 1986 FIRE IFO measurements

We have used a one-dimensional model of cirrus formation to study the development of cirrus clouds during the 1986 First ISCCP (International Satellite Cloud Climatology Project) Regional Experiment (FIRE) intensive field observations (IFO). The cirrus model includes microphysical, dynamical, and radiative processes. Sulfate aerosols, solution drops, ice crystals, and water vapor are all treated as interactive elements in the model. Ice crystal size distributions are fully resolved based on calculations of homogeneous freezing nucleation, growth by water vapor deposition, evaporation, coagulation, and vertical transport. We have focused on the cirrus observed on November 1, 1986. Vertical wind speed for the one-dimensional simulation is taken from a mesoscale model simulation for the appropriate time period. The mesoscale model simulation suggested that strong upward motions over Wyoming and subsequent horizontal transport of upper level moisture were responsible for the cirrus observed over Wisconsin on this date. We assumed that our one-dimensional model could be used to represent a vertical column moving from Wyoming to Wisconsin over a period of several hours. Ice crystal nucleation occurs in our model in the 8 to 10-km region as a result of the strong updrafts (and cooling) early in the simulation. Growth, coagulation, and sedimentation of these ice crystals result in a broad cloud region (5-10 km thick) with an optical depth of 1-2 after a few hours, in agreement with the FIRE measurements. Comparison with aircraft microphysical measurements made over Wisconsin indicates that the simulation generated reasonable ice water content, but the predicted ice number densities are too low, especially for radii less than about 50 microns. Sensitivity tests suggest that better agreement between simulated and observed microphysical properties is achieved if the nucleation rate is higher or stronger vertical mixing (perhaps associated with multidimensional motions) is present.

Jensen, Eric J.↗

Transport of Aerosols from Asia and Their Radiative Effects Over the Western Pacific: A 3-D Model Study for ACE-Asia Experiment During Spring 2001

The Aerosol Characterization Experiment-Asia (ACE-Asia) took place in Spring 2001 in the East Asia-West Pacific Ocean. During the ACE-Asia intensive field operation period, high concentrations of dust and anthropogenic aerosols were observed over the Yellow Sea and the Sea of Japan, which were transported out from the Asian continent, with the plume often extending to 6-8 km altitude. The multi-component aerosols originated from Asia are expected to exert a significant radiative forcing over the Pacific region. We present here results from the Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model of aerosol transport and radiative forcing in the context of ACE-Asia. The model calculated aerosol concentrations, extinctions, optical thickness, size distributions, and vertical profiles are compared with the aircraft and ship measurements, and the distributions of aerosols are compared with satellite data. The model will be used to understand the origins of the aerosols observed in ACE-Asia, estimate the contributions from anthropogenic and natural aerosols to the total aerosol optical thickness, investigate the effects of humidification and clouds on aerosol properties, and assess the radiative forcing of Asian aerosols over the Pacific region and in the northern hemisphere.

Chin, Mian↗

Underestimation of Deep Convective Cloud Tops by Thermal Imagery

The most common method of ascertaining cloud heights from space is from thermal brightness temperatures. Deep cumulus clouds of high water content are expected to radiate as black bodies. Here, cloud tops are estimated from several sensors: GOES-8, the Moderate Resolution Imaging Spectroradiometer (MODIS), the Moderate resolution Imaging Sensor (MISR), and the Goddard Cloud Physics Lidar (CPL), all collected during the CRYSTAL Florida Area Cirrus Experiment (CRYSTAL-FACE). Thermally derived cloud tops are consistently approx. 1km too low compared with independent measurements, no matter how thick the clouds are, even when the finite optical extinctions near cloud top and in thin overlying cirrus are taken into account. The bias appears to get worse for the tallest clouds. Cloud material is often present 2 km or more above the apparent cloud top. This mysterious discrepancy appears to be satellite-independent.

Sherwood, Steven C.↗

Aerosol Source Plume Physical Characteristics from Space-based Multiangle Imaging

Models that assess aerosol effects on regional air quality and global climate parameterize aerosol sources in terms of amount, type, and injection height. The multiangle imaging spectroradiometer (MISR) aboard NASA's Terra satellite retrieves total column aerosol optical thickness (AOT), and aerosol type over cloud-free land and water. A stereo-matching algorithm automatically retrieves reflecting-layer altitude wherever clouds or aerosol plumes have discernable spatial contrast, with about 500-m accuracy, at 1.1-km horizontal resolution. Near-source biomass burning smoke, volcanic effluent, and desert dust plumes are observed routinely, providing information about aerosol amount, particle type, and injection height useful for modeling applications. Compared to background aerosols, the plumes sampled have higher AOT, contain particles having expected differences in Angstrom exponent, size, single-scattering albedo, and for volcanic plume and dust cloud cases, particle shape. As basic thermodynamics predicts, thin aerosol plumes lifted only by regional winds or less intense heat sources are confined to the boundary layer. However, when sources have sufficient buoyancy, the representative plumes studied tend to concentrate within discrete, high-elevation layers of local stability; the aerosol is not uniformly distributed up to a peak altitude, as is sometimes assumed in modeling. MISR-derived plume heights, along with meteorological profile data from other sources, make it possible to relate radiant energy flux observed by the moderate resolution imaging spectroradiometer (MODIS), also aboard the Terra spacecraft, to convective heat flux that plays a major role in buoyant plume dynamics. A MISR climatology of plume behavior based on these results is being developed.

aerosol plumes↗

Toward Unified Satellite Climatology of Aerosol Properties. 3. MODIS Versus MISR Versus AERONET

We use the full duration of collocated pixel-level MODIS-Terra and MISR aerosol optical thickness (AOT) retrievals and level 2 cloud-screened quality-assured AERONET measurements to evaluate the likely individual MODIS and MISR retrieval accuracies globally over oceans and land. We show that the use of quality-assured MODIS AOTs as opposed to the use of all MODIS AOTs has little effect on the resulting accuracy. The MODIS and MISR relative standard deviations (RSTDs) with respect to AERONET are remarkably stable over the entire measurement record and reveal nearly identical overall AOT performances of MODIS and MISR over the entire suite of AERONET sites. This result is used to evaluate the likely pixel-level MODIS and MISR performances on the global basis with respect to the (unknown) actual AOTs. For this purpose, we use only fully compatible MISR and MODIS aerosol pixels. We conclude that the likely RSTDs for this subset of MODIS and MISR AOTs are 73% over land and 30% over oceans. The average RSTDs for the combined [AOT(MODIS)+AOT(MISR)]/2 pixel-level product are close to 66% and 27%, respectively, which allows us to recommend this simple blend as a better alternative to the original MODIS and MISR data. These accuracy estimates still do not represent the totality of MISR and quality-assured MODIS pixel-level AOTs since an unaccounted for and potentially significant source of errors is imperfect cloud screening. Furthermore, many collocated pixels for which one of the datasets reports a retrieval, whereas the other one does not may also be problematic.

Mishchenko, Michael I.↗

Airborne High Spectral Resolution Lidar Aerosol Measurements during MILAGRO and TEXAQS/GOMACCS

Two1 field experiments conducted during 2006 provided opportunities to investigate the variability of aerosol properties near cities and the impacts of these aerosols on air quality and radiative transfer. The Megacity Initiative: Local and Global Research Observations (MILAGRO) /Megacity Aerosol Experiment in Mexico City (MAX-MEX)/Intercontinental Chemical Transport Experiment-B (INTEX-B) joint experiment conducted during March 2006 investigated the evolution and transport of pollution from Mexico City. The Texas Air Quality Study (TEXAQS)/Gulf of Mexico Atmospheric Composition and Climate Study (GoMACCS) (http://www.al.noaa.gov/2006/) conducted during August and September 2006 investigated climate and air quality in the Houston/Gulf of Mexico region. During both missions, the new NASA Langley airborne High Spectral Resolution Lidar (HSRL) was deployed on the NASA Langley B200 King Air aircraft and measured profiles of aerosol extinction, backscattering, and depolarization to: 1) characterize the spatial and vertical distributions of aerosols, 2) quantify aerosol extinction and optical thickness contributed by various aerosol types, 3) investigate aerosol variability near clouds, 4) evaluate model simulations of aerosol transport, and 5) assess aerosol optical properties derived from a combination of surface, airborne, and satellite measurements.

Ferrare, Richard↗

Theoretical quasar emission-line profiles. I - Curve-of-growth effects on observed profiles

Radiative transfer effects are examined in an investigation of the kinematics of quasar and Seyfert emission-line regions with pancake cloud geometries. Consideration is given only to the effects of limb brightening with the aspect angle of pancake clouds, assuming that all lines lie on a single portion of the curve of growth. This effect is coupled with several simple but plausible ensemble geometries and dynamics, and a number of theoretical emission-line profiles have been generated. It is shown that these profiles differ substantially depending on both the ensemble geometry and the portion of the curve of growth considered; for a given ensemble geometry, optically thick line profiles are different from optically thick profiles. It is shown that, for radiatively driven clouds, ensembles of clouds which have maximum velocities approaching the terminal velocity of the acceleration mechanism never produce acceptable profiles unless the cloud luminosity is a strongly decreasing function of radius.

Hubbard, E. N.↗

Relative alignment between magnetic fields and molecular gas structure in molecular clouds

Here, we compare the structure of synthetic dust polarization with synthetic molecular line emission from radiative transfer calculations using a three-dimensional, turbulent collapsing-cloud magnetohydrodynamics simulation. The histogram of relative orientation (HRO) technique and the projected Rayleigh statistic (PRS) are considered. In our trans-Alfvénic (more strongly magnetized) simulation, there is a transition to perpendicular alignment at densities above ~4 × 10 3 cm –3 . This transition is recovered in most of our synthetic observations of optically thin molecular tracers; however, for 12 CO it does not occur and the PRS remains in parallel alignment across the whole observer space. We calculate the physical depth of the optical depth τ = 1 surface and find that for 12 CO it is largely located in front of the cloud mid-plane, suggesting that 12 CO is too optically thick and instead mainly probes low-volume density gas. In our super-Alfvénic simulation, the magnetic field becomes significantly more tangled, and all observed tracers tend towards no preference for perpendicular or parallel alignment. An observable difference in alignment between optically thin and optically thick tracers may indicate the presence of a dynamically important magnetic field, though there is some degeneracy with viewing angle. We convolve our data with a Gaussian beam and compare it with HRO results of the Vela C molecular cloud. We find good agreement between these results and our sub-Alfvénic simulations when viewed with the magnetic field in the plane of the sky (especially when sensitivity limitations are considered), though the observations are also consistent with an intermediately inclined magnetic field.

79 ASTRONOMY AND ASTROPHYSICS↗

Modeled Impact of Cirrus Cloud Increases Along Aircraft Flight Paths

The potential impact of contrails and alterations in the lifetime of background cirrus due to subsonic airplane water and aerosol emissions has been investigated in a set of experiments using the GISS GCM connected to a q-flux ocean. Cirrus clouds at a height of 12-15km, with an optical thickness of 0.33, were input to the model "x" percentage of clear-sky occasions along subsonic aircraft flight paths, where x is varied from .05% to 6%. Two types of experiments were performed: one with the percentage cirrus cloud increase independent of flight density, as long as a certain minimum density was exceeded; the other with the percentage related to the density of fuel expenditure. The overall climate impact was similar with the two approaches, due to the feedbacks of the climate system. Fifty years were run for eight such experiments, with the following conclusions based on the stable results from years 30-50 for each. The experiments show that adding cirrus to the upper troposphere results in a stabilization of the atmosphere, which leads to some decrease in cloud cover at levels below the insertion altitude. Considering then the total effect on upper level cloud cover (above 5 km altitude), the equilibrium global mean temperature response shows that altering high level clouds by 1% changes the global mean temperature by 0.43C. The response is highly linear (linear correlation coefficient of 0.996) for high cloud cover changes between 0. 1% and 5%. The effect is amplified in the Northern Hemisphere, more so with greater cloud cover change. The temperature effect maximizes around 10 km (at greater than 40C warming with a 4.8% increase in upper level clouds), again more so with greater warming. The high cloud cover change shows the flight path influence most clearly with the smallest warming magnitudes; with greater warming, the model feedbacks introduce a strong tropical response. Similarly, the surface temperature response is dominated by the feedbacks, and shows little geographical relationship to the high cloud input. Considering whether these effects would be observable, changing upper level cloud cover by as little as 0.4% produces warming greater than 2 standard deviations in the Microwave Sounding Unit (MSU) channels 4, 2 and 2r, in flight path regions and in the subtropics. Despite the simplified nature of these experiments, the results emphasize the sensitivity of the modeled climate to high level cloud cover changes, and thus the potential ability of aircraft to influence climate by altering clouds in the upper troposphere.

Rind, David↗

Properties of multilayered cloud systems from satellite imagery

The spatial coherence method for obtaining fractional cloud cover from satellite imagery is extended to the case of multilayered cloud systems. Examples are presented in which simultaneous observations at 3.7 microns and 11 microns are used to solve a system of linear equations for the nonoverlapped fractional cover contributed by each of two layers. The retrieval relies on the assumption that the clouds reside in distinct, well-defined layers and are optically thick at the wavelengths of observation. Simultaneous observations at 3.7 microns and 11 microns of the separate layers indicate that the assumptions are generally valid. Owing to the reflection of solar radiation at 3.7 microns by low-level water clouds, the method is limited to nighttime observations.

Coakley, J. A., Jr.↗

Water vapor in Jupiter's atmosphere

High spectral resolution observations of Jupiter at 2.7 and 5 microns acquired from the Kuiper Airborne Observatory were used to infer the vertical distribution of H2O between 0.7 and 6 bars. The H2O mole fraction, qH2O, is saturated for P<2 bars, qH2O = 4x.000001 in the 2 to 4 bar range and it increases to 3x.00001 at 6 bars where T = 288 K. The base of the 5 micron line formation region is determined by pressure-induced H2 opacity. At this deepest accessible level, the O/H ratio in Jupiter is depleted by a factor of 50 with respect to the solar atmosphere. High spatial resolution Voyager IRIS spectra of Jupiter's North Tropical Zone, Equatorial Zone, and Hot Spots in the North and South Equatorial Belt were analyzed to determine the spatial variation of H2O across the planet. The column abundance of H2O above the 4 bar level is the same in the zones as in the SEB Hot Spots, about 20 cm-amgt. A cloud model for Jupiter's belts and zones was developed in order to fit the IRIS 5 micron spectra. An absorbing cloud located at 2 bars whose 5 micron optical thickness varies between 1 in the Hot Spots and 4 in the coldest zones satisfactorily matches the IRIS data.

Bjoraker, G. L.↗

Influence of Arctic Sea Ice Extent on Polar Cloud Fraction and Vertical Structure and Implications for Regional Climate

Recent satellite lidar measurements of cloud properties spanning a period of 5 years are used to examine a possible connection between Arctic sea ice amount and polar cloud fraction and vertical distribution. We find an anticorrelation between sea ice extent and cloud fraction with maximum cloudiness occurring over areas with little or no sea ice. We also find that over ice!free regions, there is greater low cloud frequency and average optical depth. Most of the optical depth increase is due to the presence of geometrically thicker clouds over water. In addition, our analysis indicates that over the last 5 years, October and March average polar cloud fraction has increased by about 7% and 10%, respectively, as year average sea ice extent has decreased by 5% 7%. The observed cloud changes are likely due to a number of effects including, but not limited to, the observed decrease in sea ice extent and thickness. Increasing cloud amount and changes in vertical distribution and optical properties have the potential to affect the radiative balance of the Arctic region by decreasing both the upwelling terrestrial longwave radiation and the downward shortwave solar radiation. Because longwave radiation dominates in the long polar winter, the overall effect of increasing low cloud cover is likely a warming of the Arctic and thus a positive climate feedback, possibly accelerating the melting of Arctic sea ice.

Palm, Stephen P.↗

The Influence of Arctic Sea Ice Extent on Polar Cloud Fraction and Vertical Structure and Implications for Regional Climate

Recent satellite lidar measurements of cloud properties spanning a period of five years are used to examine a possible connection between Arctic sea ice amount and polar cloud fraction and vertical distribution. We find an anti-correlation between sea ice extent and cloud fraction with maximum cloudiness occurring over areas with little or no sea ice. We also find that over ice free regions, there is greater low cloud frequency and average optical depth. Most of the optical depth increase is due to the presence of geometrically thicker clouds over water. In addition, our analysis indicates that over the last 5 years, October and March average polar cloud fraction has increased by about 7 and 10 percent, respectively, as year average sea ice extent has decreased by 5 to 7 percent. The observed cloud changes are likely due to a number of effects including, but not limited to, the observed decrease in sea ice extent and thickness. Increasing cloud amount and changes in vertical distribution and optical properties have the potential to affect the radiative balance of the Arctic region by decreasing both the upwelling terrestrial longwave radiation and the downward shortwave solar radiation. Since longwave radiation dominates in the long polar winter, the overall effect of increasing low cloud cover is likely a warming of the Arctic and thus a positive climate feedback, possibly accelerating the melting of Arctic sea ice.

Palm, Stephen P.↗

Cloud Features Detected by MODIS But Not by CloudSat and CALIOP

The ability to characterize the global cloud cover from space has been greatly enhanced by the availability of MODIS, CloudSat, and CALIOP data. The three sensors provide good complementary information about clouds. In this study, we investigated unexpected observations of certain types of clouds apparent in the MODIS data but not detected by CloudSat and CALIOP. Several examples are presented and generally these undetected clouds are geometrically thin, low-level clouds. In particular, they are located in the Arctic region and have optical thicknesses of less than 14, top height altitudes of below 2.5 km, and layer thickness of less than 1 km. CloudSat may miss such low-level clouds because of its coarse vertical resolution of about 500 m and it has limited sensitivity near the surface. Unexpectedly, CALIOP with a much higher vertical resolution of 30 m also misses these clouds and this is due to the cloud s geometrically thin nature and surface proximity.

Chan, Mark Aaron↗

Ultraviolet photometry of Venus: Scattering layer above the absorbing clouds

Experimental measurements by ultraviolet photometers aboard Venera-9 and -10 are presented, discussed, and compared with various theoretical models of the ultraviolet structure of the atmosphere of Venus. The model in best agreement with observation provides for a finely dispersed, 8 km thick Rayleigh scattering layer above the primary cloud cover. Dark contrast details are considered to be breaks or areas of lower optical thickness in the upper scattering layer.

Ksanfomaliti, L. V.↗

Using Observations of Deep Convective Systems to Constrain Atmospheric Column Absorption of Solar Radiation in the Optically Thick Limit

Atmospheric column absorption of solar radiation A(sub col) is a fundamental part of the Earth's energy cycle but is an extremely difficult quantity to measure directly. To investigate A(sub col), we have collocated satellite-surface observations for the optically thick Deep Convective Systems (DCS) at the Department of Energy Atmosphere Radiation Measurement (ARM) Tropical Western Pacific (TWP) and Southern Great Plains (SGP) sites during the period of March 2000 December 2004. The surface data were averaged over a 2-h interval centered at the time of the satellite overpass, and the satellite data were averaged within a 1 deg X 1 deg area centered on the ARM sites. In the DCS, cloud particle size is important for top-of-atmosphere (TOA) albedo and A(sub col) although the surface absorption is independent of cloud particle size. In this study, we find that the A(sub col) in the tropics is approximately 0.011 more than that in the middle latitudes. This difference, however, disappears, i.e., the A(sub col) values at both regions converge to the same value (approximately 0.27 of the total incoming solar radiation) in the optically thick limit (tau greater than 80). Comparing the observations with the NASA Langley modified Fu_Liou 2-stream radiative transfer model for optically thick cases, the difference between observed and model-calculated surface absorption, on average, is less than 0.01, but the model-calculated TOA albedo and A(sub col) differ by 0.01 to 0.04, depending primarily on the cloud particle size observation used. The model versus observation discrepancies found are smaller than many previous studies and are just within the estimated error bounds. We did not find evidence for a large cloud absorption anomaly for the optically thick limit of extensive ice cloud layers. A more modest cloud absorption difference of 0.01 to 0.04 cannot yet be ruled out. The remaining uncertainty could be reduced with additional cases, and by reducing the current uncertainty in cloud particle size.

Dong, Xiquan↗