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At least 523 records · Page 29

Titan's aerosols. I - Laboratory investigations of shapes, size distributions, and aggregation of particles produced by UV photolysis of model Titan atmospheres

Experiments in which C2H2, C2H4, and HCN were photolyzed separately and as a mixture in UV light have been conducted in order to ascertain the physical properties of model Titan atmosphere aerosols. Aerosols formed from photolysis of C2H4 were physically similar to those formed from C2H2; protolysis of HCN rapidly generated particles that did not grow to sizes greater than 0.09 microns. While the formation of particles from C4H2 was observed within minutes, formation was slowed by a factor of 4 when C2H2 and HCN were added.

Scattergood, Thomas W.↗

Atmospheric science

The following types of experiments for a proposed Space Station Microgravity Particle Research Facility are described: (1) growth of liquid water drop populations; (2) coalescence; (3) drop breakup; (4) breakup of freezing drops; (5) ice nucleation for large aerosols or bacteria; (6) scavenging of gases, for example, SO2 oxidation; (7) phoretic forces, i.e., thermophoresis versus diffusiophoresis; (8) Rayleigh bursting of drops; (9) charge separation due to collisions of rimed and unrimed ice; (10) charged drop dynamics; (11) growth of particles in other planetary atmospheres; and (12) freezing and liquid-liquid evaporation. The required capabilities and desired hardware for the facility are detailed.

Hamill, Patrick↗

Spectral Polarization Distribution Models (PDMs) for NASA CLARREO Pathfinder’s Inter-Calibration Applications

Solar radiation scattered by Earth surfaces of various scene types such as oceans, deserts, tree leaves etc and atmospheric molecules and particles is polarized and the amount of polarization depends on the surface composition and particle physical properties. This can be a source of measurement errors in satellite data if a non-polarimetric radiometric sensor is sensitive to the polarization state of light. To obtain highly accurate spectral solar radiation data from the Earth-atmosphere system for the space-borne inter-calibration studies as proposed in NASA's Climate Absolute Radiance and Refractivity Observatory (CLARREO) mission and the CLARREO Pathfinder (CPF) mission, the spectral polarization state of the reflected solar light at the top of atmosphere (TOA) must be known with sufficient accuracy. The degree of polarization (DOP) and the angle of linear polarization (AOLP) of the light at the TOA as functions of incident and viewing geometry and scene type construct the Polarization Distribution Models (PDMs) for correction of polarization-induced error of satellite data. In this work, algorithms for modeling the spectral polarization state of reflected sunlight from various types of Earth, including oceans, deserts, vegetated land surfaces and these scene types with all kinds of clouds, are developed. By comparing the model results with the PARASOL satellite data, our numerical results demonstrate that the model can provide a reliable approach for making the spectral PDMs for wavelengths between 320 and 2300 nm for satellite inter-calibration applications as proposed in the CLARREO and the CLARREO CPF missions.

Sun, Wenbo↗

Combined Modeling of Acceleration, Transport, and Hydrodynamic Response in Solar Flares: The Numerical Model - 1

Acceleration and transport of high-energy particles and fluid dynamics of atmospheric plasma are interrelated aspects of solar flares, but for convenience and simplicity they were artificially separated in the past. We present here self consistently combined Fokker-Planck modeling of particles and hydrodynamic simulation of flare plasma. Energetic electrons are modeled with the Stanford unified code of acceleration, transport, and radiation, while plasma is modeled with the Naval Research Laboratory flux tube code. We calculated the collisional heating rate directly from the particle transport code, which is more accurate than those in previous studies based on approximate analytical solutions. We repeated the simulation of Mariska et al. with an injection of power law, downward-beamed electrons using the new heating rate. For this case, a -10% difference was found from their old result. We also used a more realistic spectrum of injected electrons provided by the stochastic acceleration model, which has a smooth transition from a quasi-thermal background at low energies to a non thermal tail at high energies. The inclusion of low-energy electrons results in relatively more heating in the corona (versus chromosphere) and thus a larger downward heat conduction flux. The interplay of electron heating, conduction, and radiative loss leads to stronger chromospheric evaporation than obtained in previous studies, which had a deficit in low-energy electrons due to an arbitrarily assumed low-energy cutoff. The energy and spatial distributions of energetic electrons and bremsstrahlung photons bear signatures of the changing density distribution caused by chromospheric evaporation. In particular, the density jump at the evaporation front gives rise to enhanced emission, which, in principle, can be imaged by X-ray telescopes. This model can be applied to investigate a variety of high-energy processes in solar, space, and astrophysical plasmas.

STOCHASTIC ACCELERATION MODEL↗

Absorption of visible radiation in atmosphere containing mixtures of absorbing and nonabsorbing particles

The presence of a strongly absorbing material, tentatively identified as graphitic carbon, or 'soot', is indicated by measurements of single-scattering albedo of tropospheric aerosols. Although theoretical calculations based on models of the ways in which soot may mix with other aerosol materials yield the single-scattering albedo values of 0.6, accounted for by a minimum 20% soot by volume, in urban regions and 0.8, yielded by 1-5% soot by volume, in rural settings, it is found that these same values can be produced by similar amounts of the iron oxide magnetite. Magnetite is shown to be indistinguishable from soot by optical measurements performed on bulk samples, and calculation of various mixtures of soot indicate the difficulty of determining aerosol composition by optical scattering techniques.

Ackerman, T. P.↗

Stellar Energetic Particle-driven Production of Biologically Relevant Molecules in Atmospheres of Young Earth-like Exoplanets Around Active G-K Stars

The chemistry of N2, CO2, CH4-rich atmospheres of terrestrial-type exoplanets around active G-K stars is a complex problem: the star's ionizing radiation in the form of X-ray and Extreme UV radiation and the precipitating energetic particles accelerated in coronal mass ejection driven shocks can drive complex chemistry in the exoplanetary atmosphere, and ignite the production of complex molecules (Airapetian et al., 2016). We developed a set of atmospheric models to simulate the formation of organic molecules that can be considered as atmospheric pre-biosignatures from exoplanets around active stars. The model has recently been extended to account for the production of ions, their role in the enhanced chemistry in the lower atmosphere, as well as the interaction of these ions with the aerosols. We applied the photochemical-collisional model to simulate the chemistry of a young terrestrial-type exoplanets resembling the Hadean Earth to highlight the creation of atmospheric pre-biosignatures, relevant greenhouse gases, and the presence of aerosols driven by stellar activity sources. We also discuss the impact of that modified atmospheric chemistry on the exoplanetary climate.

Guillaume Philippe Gronoff↗

Investigating the Martian Environment with the Mars Global Surveyor Thermal Emission Spectrometer

The Thermal Emission Spectrometer (TES) onboard Mars Global Surveyor (MGS) is being used to investigate the surface and atmosphere of Mars and the martian moons Phobos and Deimos. As such, it builds upon infrared observations obtained by previous spacecraft, e.g.. Mariner 9 and Viking Orbiters. The objectives of the TES experiment are: (1) determine and map surface minerals. rocks. and ices; (2) study the atmospheric dust composition. particle size, and spatial and temporal distribution; (3) investigate condensate clouds, CO2 and H2O, location. temperature, and height; (4) investigate polar cap deposits, e.g., growth, retreat, and energy balance; (5) measure the thermo-physical properties of surface materials; and (6) characterize the atmospheric structure and dynamics. The TES instrument is based upon a Michelson interferometer and collects data in the 1700-200 per cm region (about 6-50 micron at 5 or 10 per cm resolution. There are also broad-band bolometric (4.5100 microns and solar reflectance (0.3-2.7 microns) channels. The TES was designed to have a noise equivalent spectral radiance of 1.2 x l0(exp -8) per W per square cm per sr per cm corresponding to a signal-to-noise ratio of 490 at 1000 per cm (10 mm) for a 270 K scene and preflight data suggest a radiometric accuracy of about 1.2 x 10(exp -8) per W per square cm per sr per cm. In-flight observations indicate a small systematic calibration offset of about 1.2 x 10(exp -7) per W per square cm per sr per cm is present in the TES data. MGS achieved Mars orbital insertion September 11, 1997, and entered the initial aerobraking phase. MGS should have reached a circular orbit by early 1998. However, structural damage to one solar panel occurred during its deployment in the cruise phase and ultimately required an assessment of the extent of the damage and a much slower aerobraking period. This has delayed reaching the final circular orbit until March 1999. TES and the other MGS science instruments began operating just after orbital insertion and continued to obtain data until November 1998 when the TES was turned off to reduce power consumption on the spacecraft. TES data obtained during orbits 2 to 53 have previously been published and clearly illustrate the variety of scientific questions that can be addressed with them.

Roush, T. L.↗

Sky-Scanning Sun-Tracking Airborne Radiometer (3STAR): Instrument Design, Flight Testing, and Tracking Performance

The Sky-Scanning, Sun-Tracking Airborne Radiometer (3STAR) adapts commercial radiometer technology developed for the ocean color research community to airborne measurement of spectrally resolved solar irradiance and sky radiance. These atmospheric observations are used to derive aerosol optical depth (AOD), supporting localized AOD inputs for atmospheric correction of satellite and airborne data over terrestrial and aquatic (including optically dark) targets. The ability to regionally “tune” atmospheric correction schemes with relevant spatial AOD supports constraining atmospheric correction of remote sensing reflectance. Very wide dynamic range has been achieved for multi-channel band-pass-filter-radiometers originally designed for deployment into the water column. By actively tracking and directly pointing to the Sun, the light attenuation by aerosol particles in the atmospheric column can be quantified. These measurements improve knowledge of atmospheric constituents and the atmospheric corrections required to improve remote sensing capabilities for interpreting reflectance measurements from the Earth surface. 3STAR incorporates a custom Sun-tracking/sky-scanning pointing head, a Sun-tracking camera, and a commercially available, cylindrical, 19-channel radiometer tube assembly. An accurate and responsive mount and tracking system has been developed and certified to NASA and Naval Air Systems Command (NAVAIR) airworthiness standards for deployment into the aircraft slipstream. Ground and flight testing indicate typical tracking errors of less than 0.1 degrees, well within the field of view of the radiometer as required to minimize measurement uncertainty from alignment error. Preliminary AOD measurements compare to within 0.013 with 15 measurements from an Aerosol Robotic Network (AERONET) Cimel instrument at 500 nm wavelength and low solar angle.

Atmosphere↗

AEROICESTUDY-Colorado State University Ice Spectrometer

The dataset comprises measures, using Colorado State University's Ice Spectrometer (IS, an immersion freezing device with a range from 0 °C down to -26 to -29 °C) of atmospheric ice nucleating particle (INP) concentrations taken at ARM's Southern Great Plains (SGP) Site Guest Instrument Facility (GIF), in Lamont, Oklahoma, during the Aerosol-Ice Formation Closure Pilot Study (AEROICESTUDY). A filter sampler was mounted approximately 6 m above ground level atop the GIF rooftop platform. Single-use filter units open to the atmosphere fitted with pre-cleaned and pre-sterilized, 47-mm diameter Nuclepore polycarbonate filters were used. Filters were typically drawn for either a full day period (9AM-5PM CDT) or broken up into morning (9AM-12PM CDT) and afternoon (1PM-5PM CDT) periods. Additionally, 4 overnight filters were taken (6PM-8AM CDT). The volume of air filtered was typically between 3000 and 8000 standard liters for daily samples. After collection, filters were stored at -20 °C until processed. Initial processing to obtain spectra of INP number concentration active via the immersion freezing mechanism versus temperature was conducted using CSU's IS instrument (McCluskey et al., 2018). For measurement of INPs, collected aerosol particles were re-suspended in 8 mL of 0.1 µm-filtered deionized (DI) water. Aliquots of each suspension, and serial dilutions, were dispensed into trays which were fit into aluminum blocks in the IS. Samples were cooled at 0.33 °C per min and the freezing temperatures of wells recorded automatically. Cumulative INP concentrations were determined by first calculating the INPs per mL of suspension based on Vali (1971) and then converting to concentration per standard liter of air using the proportion of the total liquid sample dispensed and the air sample volumes. Two-tailed, 95% confidence intervals for binomial sampling were based on Equation 2 from Agresti and Coull (1998). Aliquots of suspensions from selected samples were also heat treated (95 °C for 20 min) to denature and deactiv

54 ENVIRONMENTAL SCIENCES↗

Transient particle acceleration associated with solar flares

Mechanisms that apply to solar flares are discussed, and their applicability to other astrophysical sites, where transient X-ray and gamma-ray bursts occur, is tested. Two different approaches are used to determine the characteristics of the charged particles, accelerated in association with solar flares: (1) measurement of the energy spectra and composition of charged particles observed in space and believed to be associated with a specific solar flare; and (2) recording of electromagnetic emissions in the visible, ultraviolet, soft X-ray, hard X-ray, and gamma-ray spectral regions, and also high-energy neutrons produced in the solar atmosphere by the particles accelerated in association with the solar flare. It is suggested that, at the present level of knowledge, regions where particle acceleration and interactions occur are unlikely to be specified.

Chupp, E. L.↗

Effect of meteoroid rotation on atmospheric entry heating and meteor beginning height

The beginning height of a meteor varies by approximately 10 km depending on the rotation state of a spherical meteoroid as long as the body sustains a temperature gradient. Such gradients build up in friable stony meteoroids larger than approximately 0.1 cm and in iron meteoroids that are approximately 1 cm or larger. The height where 100 microns or smaller zodiacal dust particles ablate is nearly independent of rotation. Stony particles in the 100 microns size range ablate near 120 km while both larger and smaller meteoroids penetrate deeper. All calculations were made with a nominal speed of 30 km/s and a zenithal distance equal to z(sub r) = 0 deg. Larger meteoroids cool their surface by conduction to the interior while smaller meteoroids decelerate significantly due to their large surface area to mass ratio so that the surface receives a lower energy flux. Some micro-meteoroids smaller than approximately 10 microns may escape abalation altogether at the nominal velocity. The effect of rotation on particle temperature during atmospheric flight is significant on meteoroids larger than 0.1 cm but may be negligible on micro-meteorites that are typically 10-50 microns in diameter.

Adolfsson, L. G.↗

Aeolian geomorphology from the global perspective

Any planet or satellite having a dynamic atmosphere and a solid surface has the potential for experiencing aeolian (wind) processes. A survey of the Solar System shows at least four planetary objects which potentially meet these criteria: Earth, Mars, Venus, and possibly Titan, the largest satellite of Saturn. While the basic process is the same among these four objects, the movement of particles by the atmosphere, the aeolian environment is drastically different. It ranges from the hot (730 K), dense atmosphere of Venus to the extremely cold desert (218 K) environment of Mars where the atmospheric surface pressure is only approximately 7.5 mb. In considering aeolian processes in the planetary perspective, all three terrestrial planets share some common areas of attention for research, especially in regard to wind erosion and dust storms. Relevant properties of planetary objects potentially subject to aeolian processes are given in tabular form.

Greeley, R.↗

The Pilatus Unmanned Aircraft System for Lower Atmospheric Research

This paper presents details of the University of Colorado (CU) "Pilatus" unmanned research aircraft, assembled to provide measurements of aerosols, radiation and thermodynamics in the lower troposphere. This aircraft has a wingspan of 3.2 m and a maximum take-off weight of 25 kg, and it is powered by an electric motor to reduce engine exhaust and concerns about carburetor icing. It carries instrumentation to make measurements of broadband up- and downwelling shortwave and longwave radiation, aerosol particle size distribution, atmospheric temperature, relative humidity and pressure and to collect video of flights for subsequent analysis of atmospheric conditions during flight. In order to make the shortwave radiation measurements, care was taken to carefully position a high-quality compact inertial measurement unit (IMU) and characterize the attitude of the aircraft and its orientation to the upward-looking radiation sensor. Using measurements from both of these sensors, a correction is applied to the raw radiometer measurements to correct for aircraft attitude and sensor tilt relative to the sun. The data acquisition system was designed from scratch based on a set of key driving requirements to accommodate the variety of sensors deployed. Initial test flights completed in Colorado provide promising results with measurements from the radiation sensors agreeing with those from a nearby surface site. Additionally, estimates of surface albedo from onboard sensors were consistent with local surface conditions, including melting snow and bright runway surface. Aerosol size distributions collected are internally consistent and have previously been shown to agree well with larger, surface-based instrumentation. Finally the atmospheric state measurements evolve as expected, with the near-surface atmosphere warming over time as the day goes on, and the atmospheric relative humidity decreasing with increased temperature. No directional bias on measured temperature, as might be expected due to uneven heating of the sensor housing over the course of a racetrack pattern, was detected. The results from these flights indicate that the CU Pilatus platform is capable of performing research-grade lower tropospheric measurement missions.

de Boer, Gijs↗

The upper atmosphere of Uranus

Voyager measurements of the upper atmosphere of Uranus are analyzed and developed. The upper atmosphere of Uranus is predominantly H2, with at most 10 percent He by volume, and the dominant constituent of the exosphere is H. The thermosphere is warm, with an asymptotic isothermal temperature of about 800 K. Atomic hydrogen at this temperature forms an extensive thermal corona and creates gas drag that severely limits the lifetime of small ring particles. The upper atmosphere emits copious amounts of UV radiation from pressures greater than 0.01 microbar. The depth of this emission level imposes a powerful constraint on permissible emission mechanisms. Electron excitation from a thin layer near the exobase appears to violate this constraint. Solar fluorescence is consistent with the observed trend in solar zenith-angle variation of the emissions and is absent from the night side of the planet. On Uranus, it accounts for the observed Lyman beta to H2 bands intensity ratio and an important fraction of the observed intensity (about 55 percent).

Strobel, Darrell F.↗

The neutral atmosphere temperature experiment

The AEROS Neutral Atmosphere Temperature Experiment (NATE) is designed to measure the kinetic temperature of molecular nitrogen in the thermosphere. A quadrupole mass spectrometer tuned to N2 measures the N2 density variation in a small spherical antechamber having a knife-edged orifice which is exposed to the atmosphere at the outer surface of the spacecraft. The changing density of N2 due to the spinning motion of the spacecraft permits determination of the velocity distribution of the N2 from which the temperature is calculated. An alternate mode of operation of the instrument allows measurement of the other gases in the atmosphere as well as N2 permitting determination of the neutral particle composition of the atmosphere.

Spencer, N. W.↗

Aerobraking in a dusty Martian atmosphere

The effects of dust particle impacts on the erosion of the heat shield were estimated for a 26 m diameter aerobraking vehicle entering the Mars atmosphere at 8.6 km/sec. An explicit Navier-Stokes code was used to compute the flow field about the vehicle for the actual Martian atmospheric composition at a speed of 7.5 km/sec. The deceleration and melting of the dust particles within the forebody shock-layer was computed for dust spherules having initial diameters from 3 to 10 microns. Two heat shield materials were considered: Shuttle tiles with glassy surfaces and a low-density ablator known as Avcoat.

Chang, I-Dee↗