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The 2022 magneto-optics roadmap

Abstract Magneto-optical (MO) effects, viz. magnetically induced changes in light intensity or polarization upon reflection from or transmission through a magnetic sample, were discovered over a century and a half ago. Initially they played a crucially relevant role in unveiling the fundamentals of electromagnetism and quantum mechanics. A more broad-based relevance and wide-spread use of MO methods, however, remained quite limited until the 1960s due to a lack of suitable, reliable and easy-to-operate light sources. The advent of Laser technology and the availability of other novel light sources led to an enormous expansion of MO measurement techniques and applications that continues to this day (see section 1). The here-assembled roadmap article is intended to provide a meaningful survey over many of the most relevant recent developments, advances, and emerging research directions in a rather condensed form, so that readers can easily access a significant overview about this very dynamic research field. While light source technology and other experimental developments were crucial in the establishment of today’s magneto-optics, progress also relies on an ever-increasing theoretical understanding of MO effects from a quantum mechanical perspective (see section 2), as well as using electromagnetic theory and modelling approaches (see section 3) to enable quantitatively reliable predictions for ever more complex materials, metamaterials, and device geometries. The latest advances in established MO methodologies and especially the utilization of the MO Kerr effect (MOKE) are presented in sections 4 (MOKE spectroscopy), 5 (higher order MOKE effects), 6 (MOKE microscopy), 8 (high sensitivity MOKE), 9 (generalized MO ellipsometry), and 20 (Cotton–Mouton effect in two-dimensional materials). In addition, MO effects are now being investigated and utilized in spectral ranges, to which they originally seemed completely foreign, as those of synchrotron radiation x-rays (see section 14 on three-dimensional magnetic characterization and section 16 on light beams carrying orbital angular momentum) and, very recently, the terahertz (THz) regime (see section 18 on THz MOKE and section 19 on THz ellipsometry for electron paramagnetic resonance detection). Magneto-optics also demonstrates its strength in a unique way when combined with femtosecond laser pulses (see section 10 on ultrafast MOKE and section 15 on magneto-optics using x-ray free electron lasers), facilitating the very active field of time-resolved MO spectroscopy that enables investigations of phenomena like spin relaxation of non-equilibrium photoexcited carriers, transient modifications of ferromagnetic order, and photo-induced dynamic phase transitions, to name a few. Recent progress in nanoscience and nanotechnology, which is intimately linked to the achieved impressive ability to reliably fabricate materials and functional structures at the nanoscale, now enables the exploitation of strongly enhanced MO effects induced by light–matter interaction at the nanoscale (see section 12 on magnetoplasmonics and section 13 on MO metasurfaces). MO effects are also at the very heart of powerful magnetic characterization techniques like Brillouin light scattering and time-resolved pump-probe measurements for the study of spin waves (see section 7), their interactions with acoustic waves (see section 11), and ultra-sensitive magnetic field sensing applications based on nitrogen-vacancy centres in diamond (see section 17). Despite our best attempt to represent the field of magneto-optics accurately and do justice to all its novel developments and its diversity, the research area is so extensive and active that there remains great latitude in deciding what to include in an article of this sort, which in turn means that some areas might not be adequately represented here. However, we feel that the 20 sections that form this 2022 magneto-optics roadmap article, each written by experts in the field and addressing a specific subject on only two pages, provide an accurate snapshot of where this research field stands today. Correspondingly, it should act as a valuable reference point and guideline for emerging research directions in modern magneto-optics, as well as illustrate the directions this research field might take in the foreseeable future.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Progress and Challenges for Memtransistors in Neuromorphic Circuits and Systems

Due to the increasing importance of artificial intelligence (AI), significant recent effort has been devoted to the development of neuromorphic circuits that seek to emulate the energy-efficient information processing of the brain. While non-volatile memory (NVM) based on resistive switches, phase-change memory, and magnetic tunnel junctions has shown potential for implementing neural networks, additional multi-terminal device concepts are required for more sophisticated bio-realistic functions. Of particular interest are memtransistors based on low-dimensional nanomaterials, which are capable of electrostatically tuning memory and learning behavior at the device level. Herein, a conceptual overview of the memtransistor is provided in the context of neuromorphic circuits. Recent progress is surveyed for memtransistors and related multi-terminal NVM devices including dual-gated floating-gate memories, dual-gated ferroelectric transistors, and dual-gated van der Waals heterojunctions. Further, the different materials systems and device architectures are classified based on the degree of control and relative tunability of synaptic behavior, with an emphasis on device concepts that harness the reduced dimensionality, weak electrostatic screening, and phase-changes properties of nanomaterials. Finally, strategies for achieving wafer-scale integration of memtransistors and multi-terminal NVM devices are delineated, with specific attention given to the materials challenges for practical neuromorphic circuits.

36 MATERIALS SCIENCE↗

Plasmasphere thermal structure as measured by ISEE-1 and DE-1

Characteristics of plasmaspheric ion thermal structure are presented from a statistical survey of low-energy of ion measurements made by the retarding ion mass spectrometer (RIMS) on the DE-1 satellite. Morning and evening results are compared to illustrate diurnal trends. Typical day side temperature range from about 4000 K in the inner plasmasphere to over 10,000 K in the outer plasmasphere, while corresponding evening side temperatures range from near 2000 K to over 10,000 K. Magnetic activity is found to affect the morning and evening sides somewhat differently. Temperatures are found to remain constant or increase with altitude along magnetic field lines, depending on local time and L shell. Thermal equilibrium between H(+) and He(+) prevails to a high degree throughout the plasmasphere. Ion temperatures from the Plasma Composition Experiment (PCE) on ISEE-1 are generally consistent with those from DE-1/RIMS, but are lower and tend to indicate more large scale structure on the day side.

Comfort, R. H.↗

The Aerial Regional-scale Environmental Survey (ARES) Mission to Mars

ARES is an exploration mission concept for an Aerial Regional-scale Environmental Survey of Mars designed to fly an instrumented platform over the surface of Mars at very low altitudes (1-3 km) for distances of hundreds to thousands of kilometers to obtain scientific data to address fundamental problems in Mars science. ARES helps to fill a gap in the scale and perspective of the Mars Exploration Program and addresses many key COMPLEX/MEPAG questions (e.g., nature and origin of crustal magnetic anomalies) not readily pursued in other parts of the exploration program. ARES supports the human exploration program through key environmental measurements and high-resolution contiguous data essential to reference mission design. Here we describe the major types of scientific goals, candidate instruments, and reference mission profiles.

Levine, J. S.↗

The Situational Awareness Sensor Suite for the ISS (SASSI): A Mission Concept to Investigate ISS Charging and Wake Effects

The complex interaction between the International Space Station (ISS) and the surrounding plasma environment often generates unpredictable environmental situations that affect operations. Examples of affected systems include extravehicular activity (EVA) safety, solar panel efficiency, and scientific instrument integrity. Models and heuristically‐derived best practices are well‐suited for routine operations, but when it comes to unusual or anomalous events or situations, especially those driven by space weather, there is no substitute for real‐time monitoring. Space environment data collected in real‐time (or near‐real time) can be used operationally for both real‐time alarms and data sources in assimilative models to predict environmental conditions important for operational planning. Fixed space weather instruments mounted to the ISS can be used for monitoring the ambient space environment, but knowing whether or not (or to what extent) the ISS affects the measurements themselves requires adequate space situational awareness (SSA) local to the ISS. This paper presents a mission concept to use a suite of plasma instruments mounted at the end of the ISS robotic arm to systematically explore the interaction between the Space Station structure and its surrounding environment. The Situational Awareness Sensor Suite for the ISS (SASSI) would be deployed and operated on the ISS Express Logistics Carrier (ELC) for long‐term "survey mode" observations and the Space Station Remote Manipulator System (SSRMS) for short‐term "campaign mode" observations. Specific areas of investigation include: 1) ISS frame and surface charging during perturbations of the local ISS space environment, 2) calibration of the ISS Floating Point Measurement Unit (FPMU), 3) long baseline measurements of ambient ionospheric electric potential structures, 4) electromotive force-induced currents within large structures moving through a magnetized plasma, and 5) wake‐induced ion waves in both electrostatic (i.e. particles) and electromagnetic modes. SASSI will advance the understanding of plasma‐boundary interaction phenomena, demonstrate a suite a sensors acting in concert to provide effective SSA, and validate and/or calibrate existing ISS space environment instruments and models.

Krause, L. Habash↗

Survey of Pancake-Shaped Warm Ion Distributions at Geosynchronous Orbit

It has been proposed that the electromagnetic proton cyclotron instability is a strong source of heating for the anisotropic warm ions observed at geosynchronous orbit. We present here the results of a statistical study of pancake-shaped warm ion distributions, using a one-year interval of data observed with the Los Alamos magnetospheric plasma analyzer (MPA) on the geosynchronous satellite 1994-084. Our results support previous findings that pancake-shaped warm ion distributions occur more frequently on the dayside of the magnetosphere and under magnetically quiet conditions. We also confirm that the electromagnetic proton cyclotron instability is operating and is constraining the hot proton temperature anisotropy. However, our results indicate that the pancake-shaped warm ion distributions observed at geosynchronous orbit are probably not generated by this instability but must be due to a different mechanism, possibly to heating by lower hybrid waves.

Ober, Daniel↗

Multiscale and multidimensional modeling of particle acceleration and transport in solar flares

Multi-messenger, multi-viewpoint, and time-resolved observations of solar flares are now providing unprecedented constraints on particle acceleration sites, energy conversion, and energy transport. The interpretation of current observations, including microwave imaging spectroscopy from EOVSA, hard x-ray (HXR) imaging from Solar Orbiter/STIX, gamma-ray diagnostics from Fermi, and in situ measurements from Parker Solar Probe and Solar Orbiter, collectively demands modeling frameworks that go beyond traditional spatially unresolved, one-zone models or single-mechanism descriptions. This review surveys multiscale and multidimensional modeling approaches, including kinetic, magnetohydrodynamic (MHD), and macroscopic particle models, that are being developed to meet the need. Kinetic simulations reveal that three-dimensional (3D) effects, including field-line chaos and self-generated turbulence, are essential for sustained power-law particle acceleration. MHD simulations now capture flux-rope eruptions, plasmoid-unstable current sheets, and turbulent flare regions in realistic magnetic topologies. Macroscopic models coupling MHD with energetic-particle models produce spatially resolved electron distributions and synthetic HXR and microwave emissions for direct comparison with observations. Despite these advances, outstanding challenges remain in bridging kinetic and global scales, improving MHD simulations and macroscopic particle models, and achieving quantitative model-observation closure.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Catalog of solar wind events identified from observations by ISTP spacecraft

The ISTP Science Planning and Operations Facility (SPOF), in collaboration with ISTP investigators, is developing a catalog of solar wind events and features. The catalog is primarily based on plasma and magnetic field observations from the WIND and IMP-8 spacecraft. Interplanetary events that may trigger magnetospheric activity are included as well as features of interest for using the solar wind as a plasma laboratory. Catalog coverage begins on September 8, 1992, the start of ISTP science data collection. The catalog is based on Key Parameter data sets (preliminary summary data at approximately 1 min time resolution produced quickly for survey purposes) and as such has limited citability in formal scientific work. Its primary intent is to serve as a reference for identifying candidate periods for further study, such as may be the focus of coordinated data analysis efforts during ISTP and/or IACG Science Campaigns. To facilitate access by members of the ISTP and wider space physics communities, the catalog will be available on the World Wide Web. The contents of the catalog will be described, and samples of catalog information will be presented.

Peredo, M.↗

Searching for Active Low-mass Stars in the CMa Star-forming Region: Multi-band Photometry with T80S

An exotic environment surrounds the young stellar groups associated with the Canis Major (CMa) OB1/R1 region, which probably was formed under feedback from at least three supernova events having occurred a few million years ago. We use astrometric data from the Gaia-DR2 to confirm the membership of the stars in CMa R1, based on proper motion and parallax, which revealed 514 new members and candidates. The mean age of 5 Myr estimated from the color–magnitude diagram characterizes the sources as likely pre-main-sequence candidates. In total, a sample of 694 stars detected with the T80-South telescope was analyzed according to different color–color diagrams, which were compared with theoretical colors from evolutionary models, aiming to reveal the objects that exhibit color excess due to accretion processes. Accretion and magnetic activity were also explored on the basis of empirical flux–flux relation, such as F {sub 660} and F {sub 861} that are related to Hα and Ca ii triplet emission, respectively. A low fraction (∼3 percent) of the sample have Hα excess and other colors expected for stars exhibiting chromospheric activity. The number of Class I and Class II objects, identified by the infrared (Wide-field Infrared Survey Explorer) colors, indicates a disk fraction of ∼6 percent, which is lower than that expected for stellar clusters with a similar age. Such a large sample of objects associated with CMa R1 without evidences of circumstellar accretion can be interpreted as a lack of disk-bearing stars, unusual for young star-forming regions. However, this may be explained as the result of supernova events.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Exploring beyond the planets - The Pioneer 10 and 11 missions

The Pioneer 10 and 11 missions are surveyed and illustrated with drawings, maps, graphs, and diagrams, with an emphasis on their present exploration of the outer heliosphere. The main goals of this exploration are examined (search for the heliospheric boundary, measurement of galactic cosmic radiation, and search for a trans-Neptunian planet); the ten scientific instruments carried by each spacecraft are characterized; and the results obtained so far with regard to the solar wind and interplanetary magnetic field, cosmic rays, and asteroid belt, Jupiter, and Saturn are summarized.

Dyal, P.↗

A Deep X-Ray Survey of Low Mass PMS Stars in NGC 2264

We have proposed to make a deep X-ray survey of a rotation- and proper-motion selected sample of young (3-15 Myr old), low-mass, pre-main sequence (PMS) stars in the populous star-forming region NGC 2264. These X-ray Multimirror Mission (XMM) data will be combined with an extensive set of rotation data for members of this cluster to allow us, for the first time, to probe the early evolution of magnetic dynamo activity for both fully convective stars and those stars found lower on their Hayashi tracks, which are developing radiative cores. We will use these data to study the interrelationship between rotation, interior structure, and coronal activity as a function of mass and age in the PMS and to define empirical constraints for theoretical models of angular momentum/dynamo evolution.

Patten, Brian M.↗

Reprocessing Models for the Optical Light Curves of Hypervariable Quasars from the Sloan Digital Sky Survey Reverberation Mapping Project

We explore reprocessing models for a sample of 17 hypervariable quasars, taken from the Sloan Digital Sky Survey Reverberation Mapping project, which all show coordinated optical luminosity hypervariability with amplitudes of factors ≳2 between 2014 and 2020. We develop and apply reprocessing models for quasar light curves in simple geometries that are likely to be representative of quasar inner environments. In addition to the commonly investigated thin-disk model, we include the thick-disk and hemisphere geometries. The thick-disk geometry could, for instance, represent a magnetically elevated disk, whereas the hemisphere model can be interpreted as a first-order approximation for any optically thick out-of-plane material caused by outflows/winds, warped/tilted disks, and so on. Of the 17 quasars in our sample, 11 are best-fitted by a hemisphere geometry, five are classified as thick disks, and both models fail for just one object. We highlight the successes and shortcomings of our thermal reprocessing models in case studies of four quasars that are representative of the sample. While reprocessing is unlikely to explain all of the variability that we observe in quasars, we present our classification scheme as a starting point for revealing the likely geometries of reprocessing for quasars in our sample and hypervariable quasars in general.

79 ASTRONOMY AND ASTROPHYSICS↗

FIP, FIT or MAD? Analysis of High Signal-to-Noise ASCA Spectra of Coronal Stars

ASCA (Advanced Satellite for Cosmology and Astrophysics) and EUVE (Extreme Ultraviolet Explorer) spectra of active late-type stars imply that Fe and other medium-Z elements may be 2-10 times less abundant in the coronae of these stars than in their photo-spheres (the MAD effect). These deficiencies may be related to the solar FIP (First Ionization Potential) effect, in which Fe and other low First Ionization Potential elements appear enriched in the solar corona over their photospheric values. The FIP effect is time variable. As part of this proposal, the K0-2 III star, 29 Draconis, was observed in X rays with the ASCA spacecraft in order to measure the coronal abundances of this star at three different stellar longitudes over its 31-day rotation cycle. The goal of the observations was to learn whether coronal abundances, and hence coronal magnetic structure, vary across the surface of 29 Draconis in phase with the motion of dark star-spots across its disk. A second task included in this project was a systematic reanalysis of 18-20 deep exposures of active coronal stars, which were extracted from the ASCA public archives. New thermal models were computed for each spectrum in order to derive coronal metal abundances for each star. The goal of this survey was to search for possible trends in coronal abundance with various stellar parameters such as rotation, chromospheric activity levels at ultraviolet and optical wavelengths, or evolutionary stage.

Simon, Theodore↗

Quantum Sensing and its Potential for Nuclear Safeguards

Quantum sensing has the potential to provide ultrasensitive measurements of physical phenomenon. Unlike quantum computing, quantum sensing is available now, though in general at research laboratories. A notable commercially-available quantum sensing device is the ubiquitous Superconducting Quantum Interference Device (SQUID), which can measure faint magnetic fields such as found in the human brain. Quantum sensing is used for direct measurement of environmental phenomenon, such as electromagnetic fields and accelerations, which then are used for certain applications. For example, quantum sensing of accelerations is useful for Position, Navigation, and Timing (PNT) applications. It is not clear, however, how quantum sensing can be useful for nuclear safeguards. This report provides first a background in quantum sensing, followed by a survey of potential safeguards utilizations of quantum sensing. Several potential safeguards applications are identified and explored.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A survey of actuator shaft sealing techniques for extended space missions

Actuators for control and articulation aboard Mariner spacecraft have employed output shaft seals to maintain an internal gaseous atmosphere. On future missions, considerably greater expected lifetimes, temperature ranges, and radiation exposures have led to a need to determine the limitations of the present O-ring output shaft seal and to examine other candidate seals. Seals suited both to dynamic and static sealing were examined for potential use in three specific actuator applications and the following candidate seals were selected: (a) O-ring seal, (b) chevron seal, (c) bellows seal (linear actuator only), (d) magnetic fluid seal (rotary actuators only) and as a backup seal to any of the foregoing, (e) the labyrinth seal.

Hotz, G. M.↗

Understanding flavin electronic structure and spectra

Abstract Flavins have emerged as central to electron bifurcation, signaling, and countless enzymatic reactions. In bifurcation, two electrons acquired as a pair are separated in coupled transfers wherein the energy of both is concentrated on one of the two. This enables organisms to drive demanding reactions based on abundant low‐grade chemical fuel. To enable incorporation of this and other flavin capabilities into designed materials and devices, it is essential to understand fundamental principles of flavin electronic structure that make flavins so reactive and tunable by interactions with protein. Emerging computational tools can now replicate spectra of flavins and are gaining capacity to explain reactivity at atomistic resolution, based on electronic structures. Such fundamental understanding can moreover be transferrable to other chemical systems. A variety of computational innovations have been critical in reproducing experimental properties of flavins including their electronic spectra, vibrational signatures, and nuclear magnetic resonance (NMR) chemical shifts. A computational toolbox for understanding flavin reactivity moreover must be able to treat all five oxidation and protonation states, in addition to excited states that participate in flavoprotein's light‐driven reactions. Therefore, we compare emerging hybrid strategies and their successes in replicating effects of hydrogen bonding, the surrounding dielectric, and local electrostatics. These contribute to the protein's ability to modulate flavin reactivity, so we conclude with a survey of methods for incorporating the effects of the protein residues explicitly, as well as local dynamics. Computation is poised to elucidate the factors that affect a bound flavin's ability to mediate stunningly diverse reactions, and make life possible. This article is categorized under: Structure and Mechanism > Computational Biochemistry and Biophysics Electronic Structure Theory > Combined QM/MM Methods Theoretical and Physical Chemistry > Spectroscopy

59 BASIC BIOLOGICAL SCIENCES↗

The Role of Evolutionary Age and Metallicity in the Formation of Classical BE Circumstellar Disks II. Assessing the True Nature of Candidate Disk Systems

Photometric 2-color diagram (2-CD) surveys of young cluster populations have been used to identify populations of B-type stars exhibiting excess Ha emission. The prevalence of these excess emitters, assumed to be "Be stars". has led to the establishment of links between the onset of disk formation in classical Be stars and cluster age and/or metallicity. We have obtained imaging polarization observations of six SMC and six LMC clusters whose candidate Be populations had been previously identified via 2-CDs. The interstellar polarization (ISP) associated with these data has been identified to facilitate an examination of the circumstellar environments of these candidate Be stars via their intrinsic polarization signatures, hence determine the true nature of these objects. We determined that the ISP associated with the SMC cluster NGC 330 was characterized by a modified Serkowski law with a lambda(sub max) of approx. 4500Angstroms, indicating the presence of smaller than average dust grains. The morphology of the ISP associated with the LMC cluster NGC 2100 suggests that its interstellar environment is characterized by a complex magnetic field. Our intrinsic polarization results confirm the suggestion of Wisniewski et al. that a substantial number of bona-fide classical Be stars are present in clusters of age 5-8 Myr. Hence, our data contradict recent assertions that the Be phenomenon develops in the second half of a B star's main sequence lifetime, i.e. no earlier than 10 Myr. These data imply that a significant number of B-type stars must emerge onto the zero-age-main-sequence rotating at near-critical rotation rates, although we can not rule out the possibility that these data instead reveal the presence of a sub-group of the Be phenomenon characterized by sub-critically rotating objects. Comparing the polarimetric properties of our dataset to a similar survey of Galactic classical Be stars, we find that the prevalence of polarimetric Balmer jump signatures decreases with metallicity. We speculate that these results might indicate that either it is more difficult to form large disk systems in low metallicity environments, or that the average disk temperature is higher in these low metallicity environments. We have characterized the polarimetric signatures of all candidate Be stars in our data sample and find approx. 25% are unlikely to arise from true classical Be star-disk systems. This detection of such a substantial number "contaminants" suggests one should proceed with caution when attempting to determine the role of evolutionary age and/or metallicity in the Be phenomenon purely via 2-CD results.

Wisniewski, J. P.↗

Observations of Earthward and tailward propagating flux rope plasmoids: Expanding the plasmoid model of geomagnetic substorms

A survey of Interplanetary Monitoring Platform (IMP 8) magnetometer data for plasmoid signatures during magnetospheric intervals from 1981 through 1983 found 16 plasmoids and 37 traveling compression regions as well as two earthward propagating flux ropes and 19 south-north bipolar lobe signatures. The properties of these relatively near-Earth plasmoids, traveling compression regions, and earthward propagating flux ropes and a qualitative model for their formation are presented. The plasmoids have estimated sizes, durations, magnetic field signatures, downtail velocities, and substorm associations very similar to those of the plasmoids identified in International Sun-Earth Explorer (ISEE) 3 deep-tail observations. The occurrence frequency of these near-Earth plasma sheet plasmoids is significantly smaller than that of plasmoids found in the mid- and deep tail with ISEE 3. The earthward propagating flux ropes are characterized by a south-north bipolar turning in the Geocentric Solar Magnetospheric (GSM) B(sub z) component, are localized near the noon-midnight meridional plane, and are strongly correlated with interplanetary magnetic field B(sub z) north and small isolated high latitude geomagnetic substorms. These events are also apparently very rare and/or spatially localized. We propose that these structures are 'proto-plasmoids,' i.e., plasmoids for which near-Earth magnetic reconnection stopped before all the closed plasma sheet field lines were reconnected. The proto-plasmoids are then 'trapped' inside closed magnetic field lines and propagate earthward owing to the effect of the distant X-line's earthward plasma flow. We suggest that the two different 'types' of plasmoids are due to the different energy states of the magnetosphere during periods of southward and northward interplanetary magnetic field.

Moldwin, Mark B.↗