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NASA NTRS1996

Composition and evolution of the atmosphere of Venus

The contract year started by analyzing Jovian atmospheric data acquired by the Galileo Probe Mass Spectrometer (GPMS). Two Venus hydrogen projects got underway as well. The first study strives to understand how to reconcile the standard treatment of the evolution of the H2O and HDO resevoirs on Venus over 4.5 Gyr in the presence of H and D escape and injection by comets. The second study is calculating the charge exchange contribution to hydrogen loss rates, using realistic models for exospheric H, H(+), D, D(+), and ion temperature from PV data. This report includes the following papers as attachments and supporting data: 'The Galileo Probe Mass Spectrometer: Composition of Jupiter's Atmosphere'; 'Chemical Composition Measurements of the Atmosphere of Jupiter with the Galileo Probe Mass Spectrometer'; 'Ion/Neutral Escape of Hydrogen and Deuterium: Evolution of Water'; 'Hydrogen and Deuterium in the Thermosphere of Venus: Solar Cycle Variations and Escape'; and 'Solar Cycle Variations in H(+) and D(+) Densities in the Venus Ionosphere: Implications for Escape'.

Donahue, Thomas↗

NASA NTRS1983

Control of the forebody vortex orientation by asymmetric air injection. Part A: Application to enhance departure/spin recovery of fighter aircraft and Part B: Details of the flow structure

A concept developed to provide powerful directional control effectiveness for a fighter aircraft at high angles of attack is described. The concept utilizes the energy concentrated in the strong forebody vortices (which form on slender bodies of high relative incidence) by controlling the lateral orientation of the vortices with respect to the body. The objective was to utilize the side force associated with asymmetric vortices, in a controlled manner, to enhance the ability of the fighter to recover from a departure from controlled flight. The results from water tunnel and wind tunnel experiments show that a small amount of tangential blowing along the forebody near the apex can effectively alter the forebody vortex system and generate large restoring yawing moments. Six degree of freedom digital simulation results show that this concept can substantially enhance recovery characteristics of fighter aircraft with long, slender forebodies. Also, the results of experiments which were conducted on a cone model are discussed where the principal test objective was to develop an understanding of the fluid mechanics involved in the process of vortex control. Knowledge gained in these more generic tests should allow the concept to be applied to a wider range of configurations.

Skow, A. M.↗

NASA NTRS2003

Jupiter System Data Analysis Program: Mechanisms, Manifestation, and Implications of Cryomagmatism on Europa

The objectives of the work completed under NASA Grant NAG5-8898 were (i) to document and characterize the low-albedo diffuse surfaces associated with triple bands and lenticulae, (ii) to determine their mechanisms of formation, and (iii) to assess the implications of these features for the resurfacing (in space and time) of the Europa and the nature of the Europan interior. The approach involved a combination of processing and analysis of Solid State Imaging data returned by the Galileo spacecraft during the primary and extended mission phases, together with numerical modeling of the physical processes interpreted to the observed features. We have modeled the formation of Europan triple explosive venting of cryoclastic material from bands and lenticulae halos by two processes: (i) a liquid layer in the Europan interior, and (ii) lag deposit formation by the thermal influence of subsurface cryomagmatic intrusions. We favor the latter hypothesis for explaining these features, and further suggest that a liquid water or brine intrusion is required to provide sufficient lateral heating of surface ice to explain the 25 km size of the largest features. (Solid ice diapirs, even under the most favorable conditions, become thermally exhausted before they heat significant lateral distances). We argue that water circulating in open fractures, or repeated cryomagmatic 'diking' events would provide sufficient thermal input to produce the observed features. Thus our work argues for the existence of a liquid beneath Europa's surface. Our results might most easily be explained by the presence of a continuous liquid layer (the putative Europan ocean); this would concur with the findings of the Galileo magnetometer team. However, we cannot rule out the possibility that discrete liquid pockets provide injections of fluid closer to the surface.

Fagents, Sarah A.↗

NASA NTRS1985

Film cooling on a convex wall: Heat transfer and hydrodynamic measurements for full and partial coverage

Turbine-blade cooling is an important issue for high-efficiency turbine engines, and discrete-hole injection is widely used as a cooling method. In the present study, detailed measurements were made of the heat transfer and hydrodynamics of a film-cooled flow on a convex wall, both for full and partial coverage. Two important parameters were altered: the blowing ratio, m, and the number of rows of injection holes. Three values of m were tested: m = 0.2, 0.4, and 0.6. In the blown region, m = 0.4 results in the lowest Stanton numbers of the three blowing ratios tested. This indicates that the value of m = 0.4 is near optimum on the convex wall from the point of view of cooling effect by injection. In the recovery region, Stanton numbers gradually approach the no injection values. Although the heat-transfer behavior during recovery from injection looks relatively complicated, the behavior of Stanton number can be explained in terms of two mechanisms: recovery from the thermal effect of injection and recovery from the turbulence augmentation. This interpretation of the data is supported by the hydrodynamic and temperture-profile measurements. For partial blowing cases, the data follow the full-coverage values inside the blown region. In the unblown region, both in the curved and in the flat plate, the effect of the number of blown rows is clearly seen. Hydrodynamic boundary-layer profiles were measured with the aid of a triple hot-water probe. Three mean-velocity components and six turbulence quantities were simultaneously measured, and inside the blown region strong three-dimensionality was observed.

Furuhama, K.↗

NASA NTRS1992

Rocket plume flowfield characterization using laser Rayleigh scattering

A Doppler-resolved laser Rayleigh scattering diagnostic was applied to a 111 N thrust, regenerative and fuel-film cooled, gaseous hydrogen/gaseous oxygen rocket engine. The axial and radial mean gas velocities were measured from the net Doppler shifts observed for two different scattering angles. Translational temperatures and number densities were estimated from the Doppler widths and scattered intensities, respectively, by assuming that water was the dominant scattering species in the exhaust. The experimental results are compared with theoretical predictions from a full Navier-Stokes code (RD/RPLUS) and the JANNAF Two-Dimensional Kinetics (TDK) and Standardized Plume Flowfield (SPF-II) codes. Discrepancies between the measured and predicted axial velocities, temperatures, and number densities are evident. Radial velocity measurements, however, show excellent agreement with predictions. The discrepancies are attributed primarily to inefficient mixing and combustion caused by the injection of excessive oxidizer along one side of the thrust chamber. Thrust and mass flow rate estimates obtained from the Rayleigh measurements show excellent agreement with the globally measured values.

Zupanc, Frank J.↗

NASA NTRS1992

Rocket plume flowfield characterization using laser Rayleigh scattering

Zupanc, Frank J.↗

NASA NTRS2012

Microchip Non-Aqueous Capillary Electrophoresis (MicronNACE) Method to Analyze Long-Chain Primary Amines

A protocol was developed as a first step in analyzing the complex organic aerosols present on Saturn's moon Titan, as well as the analogues of these aerosols (tholins) made on Earth. Labeling of primary amines using Pacific Blue succinimidyl ester is effected in ethanol with 25 mM triethylamine to maintain basic conditions. This reaction is allowed to equilibrate for at least one hour. Separation of the labeled primary amines is performed in ethanol with 1.05 M acetic acid, and 50 mM ammonium acetate in a commercial two-layer glass device with a standard crossmicrochannel measuring 50 microns wide by 20 microns deep. Injection potentials are optimized at 2 kV from the sample (negative) to the waste well (positive), with slight bias applied to the other two wells ( 0.4 and 0.8 V) to pinch the injection plug for the 30-s injection. Separation is performed at a potential of 5 kV along the channel, which has an effective separation distance of 7 cm. The use of ethanol in this method means that long-chain primary amines can be dissolved. Due to the low pH of the separation buffer, electro-osmotic flow (EOF) is minimized to allow for separation of both short-chain and longchain amines. As the freezing point of ethanol is much lower than water, this protocol can perform separations at temperatures lower than 0 C, which would not be possible in aqueous phase. This is of particular importance when considering in situ sampling of Titan aerosols, where unnecessary heating of the sample (even to room temperature) would lead to decomposition or unpredictable side reactions, which would make it difficult to characterize the sample appropriately.

Willis, Peter A.↗

NASA NTRSDate not supplied

Composition and Climate Impacts of Increasing Launches to Low Earth Orbit

We present simulations of an Earth system model in which launch vehicles inject gaseous and particulate combustion products into the stratosphere. We considered two plausible scenarios representative for the year 2050, one with 1000 launches per year and another with 10 times more, all of which assuming heavy lift (80 tons to low Earth orbit; LEO) launches using methane as a proxy for liquefied natural gas (LNG) fuel. An industry-standard plume flowfield model was used to predict emission of gaseous species including carbon monoxide, nitrogen oxides, and water vapor. Black carbon was introduced assuming vacuum emission equal 25% of equivalent kerosene engine. The gas emissions showed marginal or insignificant changes in atmospheric composition, while the black carbon emission was found to be the most influential component. Feedbacks involve tropopause and stratospheric warming, followed by a moistening of the stratosphere via tropospheric water vapor intrusions, together with a reduction in global albedo. The fact that LNG-fueled rockets could be a concern from aerosol emissions in our simulations, despite burning more efficiently than conventional fuels, underscores the need to better understand actual black carbon emissions from rocket engines in order to accurately predict the global impacts of launch vehicles on future climate.

Earth system model↗

NASA NTRS1977

Analysis of volatile organic compounds

An apparatus and method are described for reproducibly analyzing trace amounts of a large number of organic volatiles existing in a gas sample. Direct injection of the trapped volatiles into a cryogenic percolum provides a sharply defined plug. Applications of the method include: (1) analyzing the headspace gas of body fluids and comparing a profile of the organic volatiles with standard profiles for the detection and monitoring of disease; (2) analyzing the headspace gas of foods and beverages and comparing the profile with standard profiles to monitor and control flavor and aroma; and (3) analyses for determining the organic pollutants in air or water samples.

Zlatkis, A.↗

NASA NTRS1994

The gradient of meteorological and chemical variables across the tropopause

The downward transport of air through the tropopause can bring substantial amounts of ozone and reactive nitrogen into the upper troposphere. In this cold region of the atmosphere, O3 is particularly effective as a greenhouse gas. As part of the North Dakota Thunderstorm Project in June 1989, the NCAR Sabreliner made five flights through the tropopause. We measured ozone, nitric oxide (NO), total reactive nitrogen (NO(y)), carbon monoxide (CO), and water vapor (H2)), and took grab samples for hydrocarbon (HC) analysis. Hydrocarbons, CO, and H2O, species with sources primarily at the earth's surface, showed a strong concentration decrease with increasing altitude, while O3 and NO(y), species with a source in the stratosphere, showed a strong concentration increase with increasing altitude. Stratospheric concentrations of NO(x), NO(y), and H2O were all high relative to winter observations made during NASA's AASE. We suggest that midlatitude thunderstorms may inject wet, NO-rich air into the lower stratosphere. Calculation based on measured ratios of NO(x) and NO(y) to O3 yield a total flux of reactive nitrogen from the Northern Hemisphere stratosphere into the troposphere of 1 to 2 Tg(N) yr(exp -1) with about 8 percent in the form of NO(x). This value is higher than reported estimates of total stratospheric nitrogen fixation.

Dickerson, Russell R.↗

NASA NTRS1972

Mercury contamination study for flight system safety

The effects and prevention of possible mercury pollution from the failure of solar electric propulsion spacecraft using mercury propellant were studied from tankage loading of post launch trajector injection. During preflight operations and initial flight mode there is little danger of mercury pollution if proper safety precautions are taken. Any spillage on the loading, mating, transportation, or launch pad areas is obvious and can be removed by vacuum cleaning soil and chemical fixing. Mercury spilled on Cape Kennedy ground soil will be chemically complexed and retained by the sandstone subsoil. A cover layer of sand or gravel on spilled mercury which has settled to the bottom of a water body adjacent to the system operation will control and eliminate the formation of toxic organic mercurials. Mercury released into the earth's atmosphere through leakage of a fireball will be diffused to low concentration levels. However, gas phase reactions of mercury with ozone could cause a local ozone depletion and result in serious ecological hazards.

Gorzynski, C. S., Jr.↗

NASA NTRS2005

The Second SeaWiFS HPLC Analysis Round-Robin Experiment (SeaHARRE-2)

Eight international laboratories specializing in the determination of marine pigment concentrations using high performance liquid chromatography (HPLC) were intercompared using in situ samples and a variety of laboratory standards. The field samples were collected primarily from eutrophic waters, although mesotrophic waters were also sampled to create a dynamic range in chlorophyll concentration spanning approximately two orders of magnitude (0.3 25.8 mg m-3). The intercomparisons were used to establish the following: a) the uncertainties in quantitating individual pigments and higher-order variables (sums, ratios, and indices); b) an evaluation of spectrophotometric versus HPLC uncertainties in the determination of total chlorophyll a; and c) the reduction in uncertainties as a result of applying quality assurance (QA) procedures associated with extraction, separation, injection, degradation, detection, calibration, and reporting (particularly limits of detection and quantitation). In addition, the remote sensing requirements for the in situ determination of total chlorophyll a were investigated to determine whether or not the average uncertainty for this measurement is being satisfied. The culmination of the activity was a validation of the round-robin methodology plus the development of the requirements for validating an individual HPLC method. The validation process includes the measurements required to initially demonstrate a pigment is validated, and the measurements that must be made during sample analysis to confirm a method remains validated. The so-called performance-based metrics developed here describe a set of thresholds for a variety of easily-measured parameters with a corresponding set of performance categories. The aggregate set of performance parameters and categories establish a) the overall performance capability of the method, and b) whether or not the capability is consistent with the required accuracy objectives.

Source record↗

NASA NTRS2008

Cloud-Resolved Simulations of Lightning NOx in an Observed Hector Thunderstorm

Cloud chemistry simulations are being performed for a "Hector" storm observed on 16 November 2005 during the SCOUT-03lACTIVE campaigns based in Darwin, Australia. The primary objective of these simulations is to estimate the average production of NO per lightning flash during the storm. The 3-D WRF-AqChem model is being used for these calculations. This modeling package contains the WRF nonhydrostatic cloud-resolving model, online gas- and aqueous-phase chemistry, and a lightning algorithm (Barth et al., 2007). Early morning soundings of temperature, water vapor and winds are used to initialize the model. Surface heating of the Tiwi Islands is simulated in the model to induce convection. Observations from the Egrett, Falcon, Geophysica, and Dornier aircraft in air undisturbed by the storm are used to construct composite initial condition chemical profiles. Convective transport in the model is tested using tracer species such as CO and O3. Lightning flashes observed by the LINET network are input to the model and a lightning placement scheme is used to inject the resulting NO into the simulated cloud. Various scenarios of NO production per flash are used for cloud-to-ground and intracloud flashes in a series of simulations for the storm. Resulting NO, mixing ratios from each simulation are compared with upper tropospheric anvil observations (from the Geophysica and Egrett aircraft) to determine the best fit with the mean NOx at anvil altitudes, the profile shape, and the frequency distribution of NOx values. We will compare the results for lightning NO production from this tropical thunderstorm with similar analyses conducted for several midlatitude and subtropical convective events.

Pickering, Kenneth↗

NASA NTRS1987

Pick-up ions at Comet P/Halley's bow shock - Observations with the IIS spectrometer on Giotto

Gaseous material expanding from the nucleus of Comet Halley into space forms the neutral coma around the comet. Ionization in the solar UV radiation removes particles from the coma and injects them into the solar wind plasma. These freshly created ions are accelerated by the interplanetary electric field on cycloidal trajectories with gyrocenters moving with the speed of the magnetic field lines. In the solar wind frame of reference these particles move along the magnetic field lines with a fixed pitch angle. Pitch-angle scattering and energy diffusion reduce quickly the initial energy anisotropy which is associated with the narrow pick-up structures. First observations of heavy cometary pick-up ions (water group ions) at the bow shock are presented. The evolution of the distribution function in the vicinity of the shock and radial density profiles are discussed.

Wilken, B.↗

NASA NTRSDate not supplied

M2-SCREAM: A Stratospheric Composition Reanalysis of Aura MLS

Stratospheric composition and transport patterns are changing because of increasing greenhouse gas concentrations and declining levels of ozone depleting substances. Superimposed on forced trends are: dynamical variability at a range of time scales and unforeseen perturbations such as those resulting from injections of volcanic material and smoke from PyroCb events. Chemical reanalyses can be powerful tools for studying the composition of the stratosphere and disentangling forced responses from internal variability. This presentation introduces a new chemical reanalysis of stratospheric constituents developed and produced at NASA’s Global Modeling and Assimilation Office (GMAO) using the recently developed GMAO Constituent Data Assimilation System. Called the MERRA-2 Stratospheric Composition Reanalysis with Aura MLS (M2-SCREAM), this reanalysis consists of assimilated global three-dimensional fields of stratospheric ozone, water vapor, hydrogen chloride (HCl), nitric acid (HNO3) and nitrous oxide (N2O) mixing ratios and covers the period since the beginning of MLS observations in September 2004 to the present. M2-SCREAM assimilates version 4.2 MLS profiles of the five constituents alongside total ozone column from the Ozone Monitoring Instrument. The dynamics and tropospheric water vapor are constrained by assimilated meteorological fields from MERRA-2. The assimilated constituent fields and meteorology are provided to users at a 50-km horizontal resolution and a three-hourly frequency. Monthly analysis uncertainties and flags are also provided to the users. M2-SCREAM is an accurate and dynamically consistent high-resolution data record of the five constituents, all of which are of primary importance to stratospheric chemistry and transport studies. We will present a description of M2-SCREAM and selected results of a process-based evaluation of this product using independent data. As an illustration, we will discuss the perturbation to stratospheric composition from the eruption of Hunga Tonga–Hunga Ha'apai in January 2022 as seen in the reanalysis. We will also propose potential scientific applications of M2-SCREAM and outline plans for an upcoming comprehensive composition reanalysis that is being developed at NASA GMAO.

MERRA-2↗

NASA NTRS1997

Episodic Ocean-Induced CO2 Greenhouse on Mars: Implications for Fluvial Valley Formation

Pulses of CO2 injected into the martian atmosphere more recently than 4 Ga can place the atmosphere into a stable, higher pressure, warmer greenhouse state. One to two bar pulses of CO2 added to the atmosphere during the past several billion years are sufficient to raise global mean temperatures above 240 or 250 K for tens to hundreds of millions of years, even when accounting for CO2 condensation. Over time, the added CO2 is lost to carbonates, the atmosphere collapses and returns to its buffered state. A substantial amount of water could be transported during the greenhouse periods from the surface of a frozen body of water created by outflow channel discharges to higher elevations, despite global temperatures well below freezing. This water, precipitated as snow, could ultimately form fluvial valleys if deposition sites are associated with localized heat sources, such as magmatic intrusions or volcanoes. Thus, if outflow channel discharges were accompanied by the release of sufficient quantities of CO2, a limited hydrological cycle could have resulted that would have been capable of producing geomorphic change sufficient for fluvial erosion and valley formation. Glacial or periglacial landforms would also be a consequence of such a mechanism.

Gulick, V. C.↗

NASA NTRS2010

Computational Fluid Dynamics (CFD) Simulations of Jet Mixing in Tanks of Different Scales

For long-duration in-space storage of cryogenic propellants, an axial jet mixer is one concept for controlling tank pressure and reducing thermal stratification. Extensive ground-test data from the 1960s to the present exist for tank diameters of 10 ft or less. The design of axial jet mixers for tanks on the order of 30 ft diameter, such as those planned for the Ares V Earth Departure Stage (EDS) LH2 tank, will require scaling of available experimental data from much smaller tanks, as well designing for microgravity effects. This study will assess the ability for Computational Fluid Dynamics (CFD) to handle a change of scale of this magnitude by performing simulations of existing ground-based axial jet mixing experiments at two tank sizes differing by a factor of ten. Simulations of several axial jet configurations for an Ares V scale EDS LH2 tank during low Earth orbit (LEO) coast are evaluated and selected results are also presented. Data from jet mixing experiments performed in the 1960s by General Dynamics with water at two tank sizes (1 and 10 ft diameter) are used to evaluate CFD accuracy. Jet nozzle diameters ranged from 0.032 to 0.25 in. for the 1 ft diameter tank experiments and from 0.625 to 0.875 in. for the 10 ft diameter tank experiments. Thermally stratified layers were created in both tanks prior to turning on the jet mixer. Jet mixer efficiency was determined by monitoring the temperatures on thermocouple rakes in the tanks to time when the stratified layer was mixed out. Dye was frequently injected into the stratified tank and its penetration recorded. There were no velocities or turbulence quantities available in the experimental data. A commercially available, time accurate, multi-dimensional CFD code with free surface tracking (FLOW-3D from Flow Science, Inc.) is used for the simulations presented. Comparisons are made between computed temperatures at various axial locations in the tank at different times and those observed experimentally. The affect of various modeling parameters on the agreement obtained are assessed.

Breisacher, Kevin↗

NASA NTRS2011

The Development of a CO2 Test Capability in the NASA JSC ARCJet for Mars Reentry Simulation

The Atmospheric Reentry Materials and Structures Evaluation Facility (ARMSEF) located at NASA Johnson Space Center is used for simulating the extreme environment experienced upon reentry for the development and certification of thermal protection systems (TPS). The facility supports a large variety of programs and was heavily leveraged for the certification and operational support of the TPS for the Orbiter and, more recently, the development of the heat shield for CEV. This paper will provide more detail into the heritage of the facility. Unique attributes of the facility include a modular aerodynamically stabilized arc heater and independently controlled O2 and N2 for the test gases. When combining the O2 and N2 in a 23:77 mass ratio respectively the Earth s atmosphere is accurately simulated and via modification of this ratio the investigation of the effects of atomic oxygen on a material s response is possible. In the summer of 2010 a development effort was started to add CO2 as a third independently controlled test gas such that, when combined with N2, opens up the possibility of accurately simulating a Martian reentry environment. This paper will discuss the test facility, especially the arc heater, in more detail. Initial testing involved relatively low concentrations of CO2 combined with N2 for the primary purpose of gathering data to answer two pressing safety concerns. The first being the rate of production of carbon monoxide (CO) within the ejector vacuum system. The main concern was that CO can be flammable and possibly explosive at high enough concentrations and pressures. The hazard control during the development phase involved the use of injecting N2 inside the test chamber diffuser to dilute and reduce the concentration of any and all CO present. A residual gas analyzer (RGA) was used to determine the relative amount of CO in the exhaust gas and provide a conversion rate of CO2 to CO. This paper will discuss in more detail the results of the RGA data and the calculated conversion rate. The second safety concern addressed is the possible formation of hydrogen cyanide (HCN) and cyanide (CN). HCN would primarily be present in the cooling water while the CN would most probably condense onto the interior surfaces of the test chamber. Water samples and wipes of the test chamber surfaces were analyzed by an industrial hygienist for the presence of HCN and CN. His paper will discuss these results in more detail. Throughout this development effort measurements of the CO2:N2 flowfield were made with heat flux and pressure probes and with laser induced fluorescence (LIF) of the atomic oxygen. This paper will discuss these results

DelPapa, Steven V.↗