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At least 523 records · Page 29

Neutron-induced fission cross section of {sup nat}Pb and {sup 209}Bi from threshold to 1 GeV: An improved parametrization

Neutron-induced fission cross sections for {sup nat}Pb and {sup 209}Bi were measured with a white-spectrum neutron source at the CERN Neutron Time-of-Flight (n{sub T}OF) facility. The experiment, using neutrons from threshold up to 1 GeV, provides the first results for these nuclei above 200 MeV. The cross sections were measured relative to {sup 235}U and {sup 238}U in a dedicated fission chamber with parallel plate avalanche counter detectors. Results are compared with previous experimental data. Upgraded parametrizations of the cross sections are presented, from threshold energy up to 1 GeV. The proposed new sets of fitting parameters improve former results along the whole energy range.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Threshold Properties of the K{Lambda} Photoproduction

We have investigated kaon photoproduction on a proton and a neutron near their production thresholds by utilizing an isobar model. The background term of the model is constructed from Feynman diagrams, while the resonance term is derived from the multipoles formalism. In the case of the {gamma}+p{yields}K{sup +}+{Lambda} channel we found that both pseudoscalar (PS) and pseudovector (PV) models are able to reproduce the available photoproduction data up to W = 50 MeV above the threshold. The hyperon resonance S{sub 01}(1800) is found to be important in improving the agreement between model calculation and experimental data. In the case of double polarization observables O{sub x}, and O{sub z}, our result is in agreement with the finding of Sandorfi et al. In the {gamma}+n{yields}K{sup 0}+{Lambda} channel we found that the difference between PS and PV models is sizable for future experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Light-induced hysteresis and recovery behaviors in photochemically activated solution-processed metal-oxide thin-film transistors

In this report, photo-induced hysteresis, threshold voltage (V{sub T}) shift, and recovery behaviors in photochemically activated solution-processed indium-gallium-zinc oxide (IGZO) thin-film transistors (TFTs) are investigated. It was observed that a white light illumination caused negative V{sub T} shift along with creation of clockwise hysteresis in electrical characteristics which can be attributed to photo-generated doubly ionized oxygen vacancies at the semiconductor/gate dielectric interface. More importantly, the photochemically activated IGZO TFTs showed much reduced overall V{sub T} shift compared to thermally annealed TFTs. Reduced number of donor-like interface states creation under light illumination and more facile neutralization of ionized oxygen vacancies by electron capture under positive gate potential are claimed to be the origin of the less V{sub T} shift in photochemically activated TFTs.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

THE CIRCUMGALACTIC MEDIUM OF MASSIVE GALAXIES AT z {approx} 3: A TEST FOR STELLAR FEEDBACK, GALACTIC OUTFLOWS, AND COLD STREAMS

We present new results on the kinematics, thermal and ionization state, and spatial distribution of metal-enriched gas in the circumgalactic medium (CGM) of massive galaxies at redshift {approx}3, using the Eris suite of cosmological hydrodynamic ''zoom-in'' simulations. The reference run adopts a blastwave scheme for supernova feedback that produces large-scale galactic outflows, a star formation recipe based on a high gas density threshold, metal-dependent radiative cooling, and a model for the diffusion of metals and thermal energy. The effect of the local UV radiation field is added in post-processing. The CGM (defined as all gas at R > 0.2 R{sub vir} = 10 kpc, where R{sub vir} is the virial radius) contains multiple phases having a wide range of physical conditions, with more than half of its heavy elements locked in a warm-hot component at T > 10{sup 5} K. Synthetic spectra, generated by drawing sightlines through the CGM, produce interstellar absorption-line strengths of Ly{alpha}, C II, C IV, Si II, and Si IV as a function of the galactocentric impact parameter (scaled to the virial radius) that are in broad agreement with those observed at high redshift by Steidel et al. The covering factor of absorbing material declines less rapidly with impact parameter for Ly{alpha} and C IV compared to C II, Si IV, and Si II, with Ly{alpha} remaining strong (W{sub Ly{alpha}} > 300 mA) to {approx}> 5 R{sub vir} = 250 kpc. Only about one third of all the gas within R{sub vir} is outflowing. The fraction of sightlines within one virial radius that intercept optically thick, N{sub H{sub I}}>10{sup 17.2} cm{sup -2} material is 27%, in agreement with recent observations by Rudie et al. Such optically thick absorption is shown to trace inflowing ''cold'' streams that penetrate deep inside the virial radius. The streams, enriched to metallicities above 0.01 solar by previous episodes of star formation in the main host and in nearby dwarfs, are the origin of strong (N{sub C{sub II}}>10{sup 13} cm{sup -2}) C II absorption with a covering factor of 22% within R{sub vir} and 10% within 2 R{sub vir}. Galactic outflows do not cause any substantial suppression of the cold accretion mode. The central galaxy is surrounded by a large O VI halo, with a typical column density N{sub O{sub VI}} {approx}> 10{sup 14} cm{sup -2} and a near unity covering factor maintained all the way out to 150 kpc. This matches the trends recently observed in star-forming galaxies at low redshift by Tumlinson et al. Our zoom-in simulations of this single system appear then to reproduce quantitatively the complex baryonic processes that determine the exchange of matter, energy, and metals between galaxies and their surroundings.

79 ASTRONOMY AND ASTROPHYSICS↗

Threshold photoelectron spectroscopy of unstable N-containing compounds: Resolution of ΔK subbands in HNCO{sup +} and vibrational resolution in NCO{sup +}

The threshold photoelectron spectra (TPES) of two unstable nitrogen-containing species, HNCO and NCO, were recorded utilizing vacuum ultraviolet synchrotron radiation. Both are intermediates in combustion processes and play a role in the removal of nitrogen oxides from exhaust gases. The rovibronic structure of the first band in the TPES of HNCO{sup +} was analyzed within the framework of an orbital ionization model, and the resolved structure of the origin band was assigned to ΔK subbands. An ionization energy of 11.602 ± 0.005 eV was determined and the vibrational structure of the cationic ground state was analyzed by a Franck-Condon fit. Low lying electronically excited states of HNCO{sup +} were also observed. In a second series of experiments, the NCO radical was generated by flash pyrolysis from chlorine isocyanate. The ionization energy to the X{sup +} {sup 3}Σ{sup −} ground state was determined to be 11.76 ± 0.02 eV, while for the a{sup +1}Δ state, a value of 12.93 ± 0.02 eV was obtained. Vibrational structure was observed for both states, and bands were assigned by Franck-Condon simulations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Modification of the {omega} meson properties in the nuclear medium

We have investigated the in-medium modifications of {omega} mesons in photoproduction experiments using the Crystal Barrel(CB)/TAPS detector system at the ELSA accelerator facility in Bonn. The {omega}-mesons were reconstructed using the {omega}{yields}{pi}{sup 0}{gamma} channel. In a first analysis of the data set on a Nb target, published by Trnka et al. [Phys. Rev. Lett. 94(2005) 192303], evidence for an in-medium mass shift of the {omega}-meson was deduced from the observed {omega} line shape. The extracted signal shape was, however, found to be sensitive to the background subtraction. For this reason a re-analysis of the same data set was initiated with the goal to reduce the background and to deduce the shape and the absolute magnitude of the background directly from the data. Here we present recent results from this re-analysis. The omega signal resulting after background subtraction has been compared to different scenarios of GiBUU transport model calculations for the full incident photon energy range (900-2200 MeV) and near the production threshold (900-1300 MeV).

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Examination of hot-carrier stress induced degradation on fin field-effect transistor

Degradation in fin field-effect transistor devices was investigated in detail under various hot-carrier stress conditions. The threshold voltage (V{sub TH}) shift, substrate current (I{sub B}), and subthreshold swing were extracted to determine the degradation of a device. The power-law time exponent of the V{sub TH} shift was largest at V{sub G} = 0.3 V{sub D}, indicating that the V{sub TH} shift was dominated by interface state generation. Although the strongest impact ionization occurred at V{sub G} = V{sub D}, the V{sub TH} shift was mainly caused by electron trapping resulting from a large gate leakage current.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Results of a Search for Sub-GeV Dark Matter Using 2013 LUX Data

The scattering of dark matter (DM) particles with sub-GeV masses off nuclei is difficult to detect using liquid xenon-based DM search instruments because the energy transfer during nuclear recoils is smaller than the typical detector threshold. However, the tree-level DM-nucleus scattering diagram can be accompanied by simultaneous emission of a Bremsstrahlung photon or a so-called "Migdal" electron. These provide an electron recoil component to the experimental signature at higher energies than the corresponding nuclear recoil. The presence of this signature allows liquid xenon detectors to use both the scintillation and the ionization signals in the analysis where the nuclear recoil signal would not be otherwise visible. In this work, we report constraints on spin-independent DM-nucleon scattering for DM particles with masses of 0.4-5 GeV/c$^2$ using 1.4$\times10^4$ kg$\cdot$day of search exposure from the 2013 data from the Large Underground Xenon (LUX) experiment for four different classes of mediators. Finally, this analysis extends the reach of liquid xenon-based DM search instruments to lower DM masses than has been achieved previously.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

TH-CD-201-12: Preliminary Evaluation of Organic Field Effect Transistors as Radiation Detectors

Purpose: To fabricate organic field effect transistors (OFETs) and evaluate their performance before and after exposure to ionizing radiation. To determine if OFETs have potential to function as radiation dosimeters. Methods: OFETs were fabricated on both Si/SiO{sub 2} wafers and flexible polymer substrates using standard processing techniques. Pentacene was used as the organic semiconductor material and the devices were fabricated in a bottom gate configuration. Devices were irradiated using an orthovoltage treatment unit (120 kVp x-rays). Threshold voltage values were measured with the devices in saturation mode and quantified as a function of cumulative dose. Current-voltage characteristics of the devices were measured using a Keithley 2614 SourceMeter SMU Instrument. The devices were connected to the reader but unpowered during irradiations. Results: Devices fabricated on Si/SiO2 wafers demonstrated excellent linearity (R{sup 2} > 0.997) with threshold voltages that ranged between 15 and 36 V. Devices fabricated on a flexible polymer substrate had substantially smaller threshold voltages (∼ 4 – 8 V) and slightly worse linearity (R{sup 2} > 0.98). The devices demonstrated excellent stability in I–V characteristics over a large number (>2000) cycles. Conclusion: OFETs have demonstrated excellent potential in radiation dosimetry applications. A key advantage of these devices is their composition, which can be substantially more tissue-equivalent at low photon energies relative to many other types of radiation detector. In addition, fabrication of organic electronics can employ techniques that are faster, simpler and cheaper than conventional silicon-based devices. These results support further development of organic electronic devices for radiation detection purposes. Funding Support, Disclosures, and Conflict of Interest: This work was funded by the Natural Sciences and Engineering Research Council of Canada.

60 APPLIED LIFE SCIENCES↗

The bond energy of UN + : Guided ion beam studies of the reactions of U + with N 2 and NO

In this work, a guided ion beam tandem mass spectrometer was used to study the reactions of U + with N 2 and NO. Reaction cross sections were measured over a wide range of energy for both systems. In each reaction, UN + is formed by an endothermic process, thereby enabling the direct measurement of the threshold energy and determination of the UN + bond dissociation energy. For the reaction of U + + N 2 , a threshold energy (E 0 ) of 4.02 ± 0.11 eV was measured, leading to D 0 (UN + ) = 5.73 ± 0.11 eV. The reaction of U + + NO yields UO + through an exothermic, barrierless process that proceeds with 94 ± 23% efficiency at the lowest energy. Analysis of the endothermic UN + cross section in this reaction provides E 0 = 0.72 ± 0.11 eV and, therefore, D 0 (UN + ) = 5.78 ± 0.11 eV. Averaging the values obtained from both reactions, we report D 0 (UN + ) = 5.76 ± 0.13 eV as our best value (uncertainty of two standard deviations). Combined with precise literature values for the ionization energies of U and UN, we also derive D 0 (UN) = 5.86 ± 0.13 eV. Both bond dissociation energies agree well with high-level theoretical treatments in the literature. The formation of UN + in reaction of U + with NO also exhibits a considerable increase in reaction probability above ~3 eV. Theory suggests that this may be consistent with the formation of UN + in excited quintet spin states, which we hypothesize are dynamically favored because the number of 5f electrons in reactants and products is conserved.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Velocity map imaging of O-atom products from UV photodissociation of the CH{sub 2}OO Criegee intermediate

UV excitation of jet-cooled CH{sub 2}OO X{sup 1}A′ to the excited B{sup 1}A′ electronic states results in dissociation to two spin-allowed product channels: H{sub 2}CO X{sup 1}A{sub 1} + O {sup 1}D and H{sub 2}CO a{sup 3}A″ + O {sup 3}P. In this study, the higher energy H{sub 2}CO a{sup 3}A″ + O {sup 3}P channel is characterized by velocity map imaging and UV action spectroscopy, in both cases utilizing 2 + 1 resonance enhanced multiphoton ionization detection of O {sup 3}P products, which complements a prior experimental study on the lower energy H{sub 2}CO X{sup 1}A{sub 1} + O {sup 1}D channel [Lehman et al., J. Chem. Phys. 139, 141103 (2013)]. Anisotropic angular distributions indicative of rapid dissociation are obtained at 330 and 350 nm, along with broad and unstructured total kinetic energy distributions that provide insight into the internal excitation of the H{sub 2}CO a{sup 3}A″ co-fragment. A harmonic normal mode analysis points to significant vibrational excitation of the CH{sub 2} wag and C–O stretch modes of the H{sub 2}CO a{sup 3}A″ fragment upon dissociation. At each UV wavelength, the termination of the kinetic energy distribution reveals the energetic threshold for the H{sub 2}CO a{sup 3}A″ + O {sup 3}P product channel of ca. 76 kcal mol{sup −1} (378 nm) and also establishes the dissociation energy from CH{sub 2}OO X{sup 1}A′ to H{sub 2}CO X{sup 1}A{sub 1} + O{sup 1}D products of D{sub 0} ≤ 49.0 ± 0.3 kcal mol{sup −1}, which is in accord with prior theoretical studies. The threshold for the H{sub 2}CO a{sup 3}A″ + O {sup 3}P channel is also evident as a more rapid falloff on the long wavelength side of the O {sup 3}P action spectrum as compared to the previously reported UV absorption spectrum for jet-cooled CH{sub 2}OO [Beames et al., J. Am. Chem. Soc. 134, 20045 (2012)]. Modeling suggests that the O {sup 3}P yield increases uniformly from 378 to 300 nm.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Modeling of radiation-induced charge trapping in MOS devices under ionizing irradiation

The numerical model of the radiation-induced charge trapping process in the oxide layer of a MOS device under ionizing irradiation is developed; the model includes carrier transport, hole capture by traps in different states, recombination of free electrons and trapped holes, kinetics of hydrogen ions which can be accumulated in the material during transistor manufacture, and accumulation and charging of interface states. Modeling of n-channel MOSFET behavior under 1 MeV photon irradiation is performed. The obtained dose dependences of the threshold voltage shift and its contributions from trapped holes and interface states are in good agreement with experimental data.

74 ATOMIC AND MOLECULAR PHYSICS↗

SU-F-T-276: Source Modeling and VMAT Quality Assurance Referring to the TrueBeam Representative Beam Data for Eclipse

Purpose: To study quality assurance (QA) of volumetric modulated arc therapy (VMAT) after the 6MV and 10MV photon beam source modeling, referring to the Varian TrueBeam representative beam data for Eclipse. Methods: The source model needs specific measured beam data, such as PDDs and profiles, diagonal profile, output factors (OFs), and MLC transmission factor (TF) and dosimetric leaf gap (DLG), et al. We downloaded the representative data from myVarian website, which includes TrueBeam 4MV-15MV photon beam data and 6MeV-22MeV electron beam data in w2CAD file format for use with Eclipse and in Excel spreadsheet format for use in data comparison. The beam data in W2CAD format can be imported into the Eclipse system and calibrated for use, as appropriate. We used PTW MP3 water tank to measure the beam data in some typical field sizes, and compared the measured data with the representative data. We found that the PDDs, profiles and OFs are similar. However according to some papers and our measurements, we decided that our MLC TF and DLG are 1.58 and 1.33 (6MV), 1.79 and 1.57 (10MV), respectively. After we had configured the anisotropic analytical algorithm (AAA) with the representative data in Eclipse, we also have done dosimetric verification for 88 VMAT plans. Results: The end-to-end test procedures of VMAT were performed for 6MV and 10MV energy modes. The NE Farmer ion chamber mean measurements showed 1.2% (6MV, 38 cases) and 1.2% (10MV, 50 cases) between measurement and calculation; the Sun Nuclear ArcCheck mean measurements demonstrated gamma pass rates are as followings: 98.9%, 93.2%, 61.0% for 6MV, and 98.9%, 91.9%, 59.5% for 10MV, using 3%/3mm, 2%/2mm, 1%/1mm, 10% threshold criteria, respectively. Conclusion: The representative data is applicable to our TrueBeam for the VMAT plan, though our MLC factors are a little different, and its patientspecific QA is good.

60 APPLIED LIFE SCIENCES↗

Long-term, non-invasive FTIR detection of low-dose ionizing radiation exposure

Non-invasive methods of detecting radiation exposure show promise to improve upon current approaches to biological dosimetry in ease, speed, and accuracy. Here we developed a pipeline that employs Fourier transform infrared (FTIR) spectroscopy in the mid-infrared spectrum to identify a signature of low dose ionizing radiation exposure in mouse ear pinnae over time. Mice exposed to 0.1 to 2 Gy total body irradiation were repeatedly measured by FTIR at the stratum corneum of the ear pinnae. We found significant discriminative power for all doses and time-points out to 90 days after exposure. Classification accuracy was maximized when testing 14 days after exposure (specificity > 0.9 with a sensitivity threshold of 0.9) and dropped by roughly 30% sensitivity at 90 days. Infrared frequencies point towards biological changes in DNA conformation, lipid oxidation and accumulation and shifts in protein secondary structure. Since only hundreds of samples were used to learn the highly discriminative signature, developing human-relevant diagnostic capabilities is likely feasible and this non-invasive procedure points toward rapid, non-invasive, and reagent-free biodosimetry applications at population scales.

61 RADIATION PROTECTION AND DOSIMETRY↗

Simulation of decelerating streamers in inhomogeneous atmosphere with implications for runaway electron generation

The dynamics of positive and negative streamers is numerically simulated in atmospheric pressure air in the range of parameters corresponding to the streamer deceleration and termination in the middle of the discharge gap. A detailed comparison with experiments in air at constant and variable density demonstrates good agreement between the 2D simulation results and the observations. It is shown that positive and negative streamers behave in radically different ways when decelerating and stopping. When the head potential drops, the negative streamer transits to the mode in which the propagation is due to the forward electron drift. In this case, the radius of the ionization wave front increases, whereas the electric field at the streamer head decreases further and the streamer stops. Its head diameter continues to increase due to the slow drift of free electrons in the residual under-breakdown field. On the contrary, the only advancement mechanism for a positive streamer with a decreasing head potential is a decrease in the effective radius of the ionization wave, leading to a local increase in the electric field. This mechanism makes it possible to compensate for the reduction in the efficiency of gas photoionization at small head diameters. A qualitative 1D model is suggested to describe streamer deceleration and stopping for different discharge polarities. Estimates show that, during positive streamer stopping, the local electric field at the streamer head can exceed the threshold corresponding to the transition of electrons to the runaway mode when the head potential (relative to the surrounding space) decreases to~1.2 kV in atmospheric pressure air. In this case, pulsed generation of a beam of runaway electrons directed into the channel of a stopping positive streamer can occur. The energy of the formed pulsed electron beam depends on the intensity of photoionization in front of the streamer head. This energy can vary from 700 V (when increasing the photoionization rate by a factor of 10 with respect to the value in atmospheric pressure air) to 2.6 kV (when decreasing the photoionization rate by a factor of 1000). It is possible that this behavior of decelerating positive streamers can explain the observed bursts of x-ray radiation during the streamer propagation in long air gaps.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Neutron Identification Capabilities in MicroBooNE Through the Application of Machine Learning with Blips

Neutrinos (ν) are subatomic particles first observed in 1956 by LANL physicists Clyde Cowan and Frederick Reines but first theorized by Wolfgang Pauli in 1930. Neutrinos are the least massive known particle and are classified as leptons with 3 flavors corresponding to their leptonic counterparts (electron, muon, and tau). We know that they are abundant, 65 billion neutrinos travel through your fingertip every second, and elusive, a single neutrino could fly through a lightyear of lead without interacting at all. Though, there is much still unknown and a better characterization of these “ghostly” particles can give us clues as to the matter/anti-matter asymmetry in the early universe and possible glimpses into new physics. To measure a particle that is extremely light and rarely interacting, physicists have developed an extremely sensitive detector known as a Liquid Argon Time Projection Chamber (LArTPC). The fiducial volume (or TPC) is bombarded with neutrinos, some of which interact with argon (Ar) atoms to produce particles that in turn excite and ionize the Ar. The products of these are free electrons which then drift through the TPC’s applied magnetic field towards a multi-plane wire readout system. The electrons’ charge is collected at this anode and the light from the initial interactions is collected by photomultiplier tubes (PMTs). In conjunction, these mechanisms allow LArTPCs to achieve millimeter spatial resolution and sub-MeV energy thresholds. The detector of interest in this study is the MicroBooNE Experiment at Fermilab. MicroBooNE is an above ground LArTPC with dimensions of approximately 10m × 2.5m × 2.3m, about the size of a school bus. Its purpose is to study neutrinos, so to improve rates of measured ν interactions, the detector is squarely in the path of the Booster Neutrino Beam (BNB) at Fermilab. A major challenge in neutrino studies is energy reconstruction, much of the neutrino’s original energy is lost in interactions that the detector is not sensitive to, often due to low-energy products. The initial goal of this analysis was to better identify neutrons, the main source of poor energy reconstruction in neutrino events. Because neutrons are neutral particles, like neutrinos, we can only directly measure the products of their interactions in LArTPCs. Most of these products are low-energy signals and while each one contributes a negligible amount of energy, collectively these signals make up most of the lost energy in each neutrino event. We define these signals as blips; point-like, isolated depositions of charge in the detector. Blips have MeV-scale energies and are the size of a single hit (charge deposition) or a cluster of a few hits on at least two wire planes. Blips are the principal detector features used to study low-energy physics; thus, they are the key to unlocking information not only about neutrons but gamma photons, supernova and solar neutrinos as well as helping us better identify certain particles. Therefore, this analysis strives to use blips for improved neutron identification (ID) and characterization.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Scaling law for direct current field emission-driven microscale gas breakdown

The effects of field emission on direct current breakdown in microscale gaps filled with an ambient neutral gas are studied numerically and analytically. Fundamental numerical experiments using the particle-in-cell/Monte Carlo collisions method are used to systematically quantify microscale ionization and space-charge enhancement of field emission. The numerical experiments are then used to validate a scaling law for the modified Paschen curve that bridges field emission-driven breakdown with the macroscale Paschen law. Analytical expressions are derived for the increase in cathode electric field, total steady state current density, and the ion-enhancement coefficient including a new breakdown criterion. It also includes the effect of all key parameters such as pressure, operating gas, and field-enhancement factor providing a better predictive capability than existing microscale breakdown models. The field-enhancement factor is shown to be the most sensitive parameter with its increase leading to a significant drop in the threshold breakdown electric field and also to a gradual merging with the Paschen law. The proposed scaling law is also shown to agree well with two independent sets of experimental data for microscale breakdown in air. The ability to accurately describe not just the breakdown voltage but the entire pre-breakdown process for given operating conditions makes the proposed model a suitable candidate for the design and analysis of electrostatic microscale devices.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Measurement of the (236)U(n,f) cross section from 170 MeV to 2 MeV at the CERN n_TOF Facility

The neutron-induced fission cross section of {sup 236}U was measured at the neutron Time-of-Flight (n-TOF) facility at CERN relative to the standard {sup 235}U(n,f) cross section for neutron energies ranging from above thermal to several MeV. The measurement, covering the full range simultaneously, was performed with a fast ionization chamber, taking advantage of the high resolution of the n-TOF spectrometer. The n-TOF results confirm that the first resonance at 5.45 eV is largely overestimated in some nuclear data libraries. The resonance triplet around 1.2 keV was measured with high resolution and resonance parameters were determined with good accuracy. Resonances at high energy have also been observed and characterized and different values for the cross section are provided for the region between 10 keV and the fission threshold. The present work indicates various shortcomings of the current nuclear data libraries in the subthreshold region and provides the basis for an accurate re-evaluation of the {sup 236}U(n,f) cross section, which is of great relevance for the development of emerging or innovative nuclear reactor technologies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗