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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 523 records · Page 29
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Probing the electronic structure and spectroscopy of pyrrolyl and imidazolyl radicals using high-resolution photoelectron imaging of cryogenically cooled anions

High-resolution photoelectron imaging and photodetachment spectroscopy of cryogenically cooled pyrrolide and imidazolide anions are used to probe the electronic structure and spectroscopy of pyrrolyl and imidazolyl radicals. The high-resolution data allow the ground state vibronic structures of the two radicals to be completely resolved, yielding accurate electron affinities of 2.1433 ± 0.0008 eV and 2.6046 ± 0.0006 eV for pyrrolyl and imidazolyl radicals, respectively. Fundamental frequencies for eight vibrational modes of pyrrolyl and ten vibrational modes of imidazolyl are measured, including several nonsymmetric Franck–Condon-forbidden modes. Two electronic excited states are also observed for the two radicals, displaying diffuse spectral features in both systems. The observations of nonsymmetric vibrational modes in the ground states and the diffuse excited state features provide strong evidence for vibronic couplings between the ground state and the two close-by excited states. The 2-pyrrolide isomer is also observed as a minor species from the electrospray ionization source and the electron affinity of 2-pyrrolyl is measured to be 1.6690 ± 0.0030 eV along with five vibrational frequencies. Even though the HOMOs of both pyrrolide and imidazolide anions are p orbitals, photodetachment spectroscopy reveals completely different threshold behaviors for the two anions: a d-wave-dominated spectrum for pyrrolide and an s-wave-dominated spectrum for imidazolide. Furthermore, the current study provides a wealth of electronic and spectroscopic information, which is ideal to compare with more accurate vibronic coupling calculations for these two important radicals, as well as interesting information about the photodetachment dynamics of the two anions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

On the prospects of optical cycling in diatomic cations: effects of transition metals, spin–orbit couplings, and multiple bonds

Molecules with optical cycling centers (OCCs) are highly desirable in the context of fundamental studies as well as applications (e.g., quantum computing) because they can be effectively cooled to very low temperatures by repeated absorption and emission (hence, cycling). Charged species offer additional advantages for experimental control and manipulation. Here, we present a systematic computational study of a series of diatomic radical-cations made of a d-block metal and a p-block ligand, that are isoelectronic (in their valence shell) to the successfully laser-cooled neutral molecules. Using high-level electronic structure methods, we characterize state and transition properties of low-lying electronic states and compute Franck-Condon factors. The computed branching ratios and radiative lifetimes reveal that the electronic transitions analogous to those successfully used in the laser cooling of neutral molecules are less than optimal in the cations. We propose alternative transitions suitable for optical cycling and highlight trends that could assist future designs of OCCs in charged or neutral molecules.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2020

Ring-based electron cooler for EIC

An Electron Ion Collider (EIC) at Brookhaven National Laboratory (BNL) is being proposed as a new discovery machine for the nuclear physics and quantum chromodynamics. The hadron beam cooling plays an important role in the EIC machine to achieve its physics goals. The most challenging is cooling of protons at the highest energy in the EIC. In this paper, we present a possible design of a ring-based electron cooler for the high energy hadron beam cooling. In proposed approach, the electrons will cool the hadrons while being cooled themselves by radiation damping in the storage ring. For design of the cooler using storage ring approach several aspects becomes very important, including electron ring optics design, chromaticity correction, calculate the dynamic aperture, radiation damping, quantum excitation, and intrabeam scattering (IBS). In addition, such effects as beam-beam scattering (BBS) due to interaction of electrons with hadrons become of special concern. In this paper, we discuss and take into design all the effects above, as well as introduce generalized treatment of the BBS and 3-D quantum lifetime. A special feature of our design is an effective use of dispersion in the cooling section, both for the ions and electrons, to redistribute the cooling rate between the longitudinal and horizontal planes. Finally, the cooling performance is simulated for proton beam at the top energy of the EIC. Our conclusion is that such ring-based cooler could be a feasible approach to provide required parameters of hadron beam at the top energy of 275 GeV for the EIC.

43 PARTICLE ACCELERATORS↗
NASA NTRS1987

Solar EUV induced variations in the thermosphere

The effects of solar activity on the thermosphere are reviewed. The neutral total density, temperature, and electron density increase with solar activity, and their variations are fairly well correlated with variations in solar 10.7-cm flux. The electron temperature, by contrast, has a complex behavior with solar activity, depending on altitude and season, as increased heat input is balanced by increased cooling provided by the enhanced electron density. Also, individual neutral species do not all increase in step but are influenced by dissociation and dynamical processes. The increased ion drag at higher solar activities inhibits the neutral wind from increasing in the same proportion as the neutral temperatures and densities.

Hedin, A. E.↗
NASA NTRS2012

Radioisotope Stirling Engine Powered Airship for Low Altitude Operation on Venus

The feasibility of a Stirling engine powered airship for the near surface exploration of Venus was evaluated. The heat source for the Stirling engine was limited to 10 general purpose heat source (GPHS) blocks. The baseline airship utilized hydrogen as the lifting gas and the electronics and payload were enclosed in a cooled insulated pressure vessel to maintain the internal temperature at 320 K and 1 Bar pressure. The propulsion system consisted of an electric motor driving a propeller. An analysis was set up to size the airship that could operate near the Venus surface based on the available thermal power. The atmospheric conditions on Venus were modeled and used in the analysis. The analysis was an iterative process between sizing the airship to carry a specified payload and the power required to operate the electronics, payload and cooling system as well as provide power to the propulsion system to overcome the drag on the airship. A baseline configuration was determined that could meet the power requirements and operate near the Venus surface. From this baseline design additional trades were made to see how other factors affected the design such as the internal temperature of the payload chamber and the flight altitude. In addition other lifting methods were evaluated such as an evacuated chamber, heated atmospheric gas and augmented heated lifting gas. However none of these methods proved viable.

Colozza, Anthony J.↗
NASA NTRS2022

Exploration Extravehicular Mobility Unit (xEMU): Electron Beam Welding of the Portable Life Support System (PLSS) Ti-6Al-4V Backplate with Integrated Cooling Channels

The Exploration Extravehicular Mobility Unit (xEMU) is the first clean sheet redesign of the astronaut spacesuit in approximately 40 years. NASA Langley Research Center’s electron beam welding team, of which the author is a member, is leading the development of the weld technology required to manufacture the backplate component of the Portable Life Support System (PLSS). This backplate will provide both structural support and integral cooling for the life support systems, communications, and other electronics inside the spacesuit.

electron beam welding↗
DOE OSTI2023

Modeling the energetic tail of a dusty plasma's electron energy distribution and its effect on dust grain charge and behavior

A model for a weakly ionized dusty plasma is proposed in which UV or x-ray radiation continuously creates free electrons at high energy, which then cool through collisions with a cold neutral gas before recombining. The transition of a free electron from high energy at birth to low energy at demise implies that the electron energy distribution is not the simple Maxwellian of an isolated system in thermal equilibrium, but instead has a high-energy tail that depends on the recombination time. This tail can have a major effect on dust grain charging because the flux of tail electrons can be substantial even if the density of tail electrons is small. Detailed analytic and numerical calculations of dust grain charging show that situations exist in which a small high-energy tail dominates charge behavior. This implies that dust grain charge in terrestrial and space dusty plasmas may be significantly underestimated if a Maxwellian distribution is assumed and the non-thermal dynamics are neglected.

Physics↗
DOE OSTI2026

First DIII-D-West hybrid scenario similarity experiments for iter-relevant long-pulse operation

For the first time, similarity experiments between DIII-D and WEST were performed in the ITER "hybrid-like" regime during dedicated campaigns in April and May 2025. The matched parameters include elongation, triangularity, ion ∇B drift direction toward the X-point, qprofile, and core normalized physics quantities in terms of normalized pressure, normalized gyroradius, electron collisionality, ratio of ion to electron temperature, T i /T e . Core transport physics is explored with different aspect ratio (R/a) values (typically 3 at DIII-D and 5 on WEST). DIII-D explored high-beta conditions (electromagnetic effect) with low torque injection (~0 ± 0.5 N•m) using high heating power (up to 6 MW NBI and 2 MW ECRH powers), while scanning the heating mix (ion vs electron), beta, T i /T e , core radiation via controlled tungsten injection using the Laser Blow-Off system. WEST extended operation toward long-duration pulses using its actively cooled tungsten divertor, achieving dominated electron heating regimes with reduced tungsten contamination. Boron impurity injection were scanned on WEST to control edge conditions and core performance. It is found that core confinement improves-manifested by higher electron temperature, total energy content, neutron rate, and ion temperatureunder conditions of low separatrix density, consistent with previous observations [Bourdelle et al., Nucl. Fusion 63 (2023) 056021]. Conditions for Hmode access and for ion heating in electron-dominated regimes in both WEST and DIII-D will be discussed and compared. The ratio of the thermal energy confinement time (τ E ) to the volume-averaged electron-ion collisional heat exchange time (τ e-i ) is a key parameter to enhance ion heating and potentially facilitate H-mode access in electron-heated regimes. These first-of-a-kind coordinated DIII-D and WEST experiments provide a unique multi-machine dataset to validate predictive models and to optimize ITER hybrid-scenario performance under diverse core and edge conditions.

DIII-D↗
DOE OSTI2021

Quantization effects in semiconductor nanostructures and singlet fission in molecular chromophores for photovoltaics and solar fuels

Hot carriers in semiconductors are electrons and/or holes that have energies greater than carriers that reside at the top and bottom of the conduction and valence bands, respectively; the latter carriers are in equilibrium with the lattice and have a temperature equal to the lattice (ambient) temperature. Hot carriers are created in semiconductors upon the absorption of photons with energies greater than the bandgap. The excess energy above the bandgap energy is in the form of kinetic energy. The hot carriers can cool to the lattice temperature via electron–phonon scattering and establish separate Boltzmann distributions for electrons and holes at the band edges. Thus, upon cooling, the excess kinetic energy of the hot carriers is transformed into heat and is unavailable to be converted into electrical or chemical free energy in a solar photon-converting cell. This hot-carrier cooling process significantly limits the maximum possible power conversion efficiency (PCE) of the free energy of solar photons into electrical free energy or chemical free energy in chemical bonds of fuels. However, if hot-carrier cooling can be slowed such that the hot carriers can be extracted before cooling to create higher photovoltages, or utilized to create additional electron-hole pairs through carrier multiplication, then beneficial use can be made of the excess energy of hot carriers and the maximum thermodynamic PCE can be dramatically increased. Quantization effects in semiconductor nanostructures, unique properties of some bulk semiconductors, and exciton multiplication in both semiconductors and molecular chromophores that undergo singlet fission have shown a path forward for potential dramatic increases in the PCEs of solar photons into electricity and solar fuels. The status, history, and future promise of the science and technology of these future approaches for different types of photovoltaic cells and cells for solar fuels will be discussed.

14 SOLAR ENERGY↗
DOE OSTI2023

Integrated Traction Drive Thermal Management: Keystone Project 3

The presentation represents a report of accomplishments during FY 2022 and is prepared for 2022 DOE VTO Annual Merit Review. The project goal is facilitation of achieving DOE 2025 target of 33 kW/L system power density for an electric traction drive through support of other EDT consortium members in design and development of thermal management systems for their respective integrated drive concepts. Namely, identifying pathways enabling high-performance, compact, and reliable integrated electric drives. Specific objectives are: 1) Research and evaluation of motor-integrated power electronics packaging technologies and thermal management approaches. 2) Development of thermal management system and its sub-components to enable integrated electric drive DOE power density targets in collaboration with project partners. 3) Supporting activities of DOE's Electric Drive Technologies (EDT) consortium members, Oak Ridge National Laboratory (ORNL) and University of Wisconsin research teams in thermal management component design and thermal modeling of their integrated traction drives. 4) Identifying candidate driveline fluids suitable for direct cooling of traction-drive components and high-voltage power electronics and evaluate their convective cooling performance.

ADVANCED PROPULSION SYSTEMS↗
DOE OSTI2023

PCB-on-DBC GaN Power Module Design with High-Density Integration and Double-Sided Cooling

Lateral gallium nitride (GaN) high-electron-mobility transistors (HEMTs) present better electrical characteristics compared to silicon or silicon carbide devices such as high switching speed and low gate charge, but also present additional challenges on the module design. Here, this paper discusses a high-density GaN power module with double-sided cooling, low inductance, on-package decoupling capacitors, and integrated gate drivers. The GaN dies as well as the gate drive are sandwiched between the printed circuit board (PCB) and direct bonded copper (DBC) substrate to achieve compact loop and double-sided cooling effect. Design considerations and thermal performance are analyzed. A module assembly procedure is presented utilizing the layer-by-layer attachment process. Finally, a 2.7 cm x 1.8 cm half-bridge GaN power module is fabricated and tested, achieving a low power-loop inductance of 1.03 nH, and the overshoot voltage of the switching waveform is less than 5% under a 400-V/25-A double-pulse test. The thermal resistance is 0.32 K/W, verified by simulation and experimental results. The design and assembly process can be generalized and applied to high power applications to achieve high power density and high performance.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Atomic resolution scanning transmission electron microscopy at liquid helium temperatures for quantum materials

Fundamental quantum phenomena in condensed matter, ranging from correlated electron systems to quantum information processors, manifest their emergent characteristics and behaviors predominantly at low temperatures. This necessitates the use of liquid helium (LHe) cooling for experimental observation. Atomic resolution scanning transmission electron microscopy combined with LHe cooling (cryo-STEM) provides a powerful characterization technique to probe local atomic structural modulations and their coupling with charge, spin and orbital degrees-of-freedom in quantum materials. However, achieving atomic resolution in cryo-STEM is exceptionally challenging, primarily due to sample drifts arising from temperature changes and noises associated with LHe bubbling, turbulent gas flow, etc. In this work, we demonstrate atomic resolution cryo-STEM imaging at LHe temperatures using a commercial side-entry LHe cooling holder. Firstly, we examine STEM imaging performance as a function of He gas flow rate, identifying two primary noise sources: He-gas pulsing and He-gas bubbling. Secondly, we propose two strategies to achieve low noise conditions for atomic resolution STEM imaging: either by temporarily suppressing He gas flow rate using the needle valve or by acquiring images during the natural warming process. Lastly, we show the applications of image acquisition methods and image processing techniques in investigating structural phase transitions in Cr 2 Ge 2 Te 6 , CuIr 2 S 4 , and CrCl 3 . In conclusion, our findings represent an advance in the field of atomic resolution electron microscopy imaging for quantum materials and devices at LHe temperatures, which can be applied to other commercial side-entry LHe cooling TEM holders.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Transverse BBU Suppression with Feedback for Energy-Recovery Linacs

The Electron–Ion Collider (EIC) achieves its design luminosity by cooling the ion beam with a high-current electron beam generated in an energy-recovery linac (ERL). The baseline ERL lattice employs a BNL five-cell cavity that is frequency-scaled to 197 MHz, 591 MHz, and 1.773 GHz, raising concerns about multibunch beam-breakup (BBU) instabilities. Threshold currents for each frequency option are established with two independent BBU tracking codes, providing cross-validated operating margins that guide cavity selection. To further increase the current limit, we incorporate a digital transverse feedback (FB) system that targets the dominant higher-order modes (HOMs). Simulations show the FB raises the BBU threshold by roughly an order of magnitude: power-spectral-density analysis of the beam centroid at the linac exit confirms strong suppression of the aliased HOM peak, although some spectral growth appears at secondary frequencies. This combined study quantifies baseline BBU limits, demonstrates effective active mitigation, and charts a practical path toward robust, high-current operation of the EIC ERL.

Accelerator Physics↗
DOE OSTI2025

Conical intersections shed light on hot carrier cooling in quantum dots

Experimental observations of vibronic coherences in electronically excited colloidal semiconductor nanocrystals offer a window into the ultrafast dynamics of hot carrier cooling. In previous work, we showed that, in amine-passivated quantum dots (QDs), these coherences arise during relaxation through a cascade of conical intersections between electronically excited states. Here, in this work, we demonstrate the generality of this framework by application to QDs with surface-bound carboxylate ligands. A model involving a similar cascade of conical intersections accurately reproduces the frequencies of vibronic coherences observed with broadband multidimensional spectroscopy. The impact of ligands on the relaxation dynamics is attributed to two distinct mechanisms involving either electronic or vibrational coupling between the core and ligands. Compared to the amine-passivated QDs studied previously, the electronic coupling mechanism is less prominent in carboxylate-passivated QDs. Furthermore, comparison of acetate and formate ligands reveals that truncating the ligand alkyl chains alters the relaxation behavior predicted by the model.

14 SOLAR ENERGY↗
DOE OSTI2021

Plasma Muon Beam Cooling for HEP

Ionization cooling has the potential to shrink the phase space of a muon beam by a factor of 10⁶ within the muons’ short lifetime (2.2 µs) because the collision frequency in a cooling medium is extremely high compared to conventional beam cooling methods. It has been realized that ionization cooling inherently produces a plasma of free electrons inside the absorber material, and this plasma can have an important effect on the muon beam. In particular, under the right circumstances, it can both improve the rate of cooling and reduce the equilibrium emittance of the beam. This has the potential to improve the performance of muon facilities based on muon cooling; in particular a future muon collider. We describe how this project will integrate Plasma muon beam cooling into both the basic Helical Cooling Channel (HCC) and extreme Parametric-resonance Ionization Cooling (PIC) techniques. This potentially whole new approach to muon cooling has exciting prospects for significantly reduced muon beam emittance.

43 PARTICLE ACCELERATORS↗
NASA NTRS1992

Evaluation of the Benefits of High Temperature Electronics for Lunar Power Systems

A comparative evaluation is conducted of several approaches to the cooling of a lunar power system's power electronics, in view of the 400 K temperature of the 354-hour lunar day and lunar dust accumulation, which can contaminate power components and radiator surfaces. It is noted that, by raising the power electronics' baseplate temperature to 480 K, no thermal control system is required; the surface of the baseplate acts as its own, waste-heat-rejecting radiator, but the baseplate must be kept clean of lunar dust contamination.

Fay, Edgar H.↗
DOE OSTI2022

Dual Energy Electron Storage Ring Cooler Design for Relativistic Ion Beams

Collider experiments demand small beam emittances in order to achieve high luminosity. For light particles such as electrons, there exists a natural synchrotron radiation damping resulting in low emittance beams at equilibrium. In the case of heavy particle beams such as proton or ion beams, there is no significant synchrotron radiation damping effect and some cooling mechanism is needed to get to low emittance beams. A dual energy storage ring cooler is a novel concept proposed to cool hadron beams at higher energies. The design consists of two rings: a low energy ring and a high energy ring connected by the energy recovering linac (ERL) that provides the necessary energy difference. The low energy ring has an electron cooler where the cooling interaction takes place between the electron and hadron beams whereas electron beam going through the high energy ring undergoes synchrotron radiation damping. In this document, we present a possible design of a dual energy storage ring-based electron cooler for high energy proton beam cooling suitable for the Electron Ion Collider (EIC) to be built at Brookhaven National laboratory (BNL). A special feature of a dual energy storage ring cooler design is that the electron beam energy in the low energy section must be tuned to match the hadron beam velocity in the cooling section, and the electron beam energy in the high energy section is chosen to provide an adequate synchrotron radiation damping. In addition, the ring optics design is carried out considering chromaticity correction, dynamic aperture, momentum aperture, beam lifetime, radiation damping and the intrabeam scattering effect. Finally, the cooling performance is simulated for 275 GeV proton beams at the top energy of the EIC. In such a collider it is desirable to cool the hadron beams to balance the emittance growth rates due to intra-beam scattering (IBS) to maintain a high luminosity during the collision runs. In such a situation, a dual energy storage ring based cooler could be a practical approach to be used for hadron beam cooling.

Dhital, Bhawin↗