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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS2004

Rapid Measurements of Aerosol Ionic Composition and 3-10 nm Particle Size Distributions On The NASA P3 To Better Quantify Processes Affecting Aerosols Advected From East Asia

The Particle Into Liquid Sample (PILS) was deployed on the NASA P3 for airborne measurements of fine particle ionic chemical composition. The data have been quality assured and reside in the NASA data archive. We have analyzed our data to characterize the sources and atmospheric processing of fine aerosol particles advected from the region during the experiments. Fine particle water-soluble potassium was found to serve as a useful aerosol tracer for biomass smoke. Ratios of PILS potassium to sulfate are used as a means of estimating the percent contribution of biomass burning to fine particle mass in mixed plumes advecting from Asia. The high correlations between K+ and NO3(sup -) and NH4(sup +)' indicated that biomass burning was a significant source of these aerosol compounds in the region. It is noteworthy that the air mass containing the highest concentrations of fine particles recorded in all of ACE-Asia and TRACE-P appeared to be advecting from the Bejing/Tientsin urban region and also had the highest K(+), NO3(sup -) and NH4(sup +) concentrations of both studies. Based on K+/SO4(sup 2-) ratio's, we estimated that the plume was composed of approx. 60% biomass burning emissions, possibly from the use of bio-fuels in the urban regions.

Weber, Rodney J.↗
NASA NTRS2004

Biomass-Burning Aerosols in South East-Asia: Smoke Impact Assessment (BASE-ASIA)

Biomass burning has been a regular practice for land clearing and land conversion in many countries, especially those in Africa, South America, and Southeast Asia. However, the unique climatology of Southeast Asia is very different than that of Africa and South America, such that large-scale biomass burning causes smoke to interact extensively with clouds during the peak-burning season of March to April. Significant global sources of greenhouse gases (e.g., CO2, CH4), chemically active gases (e.g., NO, CO, HC, CH3Br), and atmospheric aerosols are produced by biomass burning processes. These gases influence the Earth- atmosphere system, impacting both global climate and tropospheric chemistry. Some aerosols can serve as cloud condensation nuclei, which play an important role in determining cloud lifetime and precipitation, hence, altering the earth s radiation and water budget. Analyses from satellite measurements reveal the reflected solar (emitted thermal) radiation from clouds due to smoke aerosols can be reduced (enhanced) by 100 (20) Watts per square meter over the month of March 2000. In addition, the reduction in cloud spectral reflectance is large enough to lead to significant errors in satellite retrievals of cloud properties (e.g., optical thickness and effective radius). The fresh water distribution in this region is highly dependent on monsoon rainfall; in fact, the predictability of the tropical climate system is much reduced during the boreal spring. Therefore, to accurately assess the impact of smoke aerosols in this region requires continuous observations from satellites, aircraft, ground-based networks and dedicated field experiments. BASE-ASIA initiative has been proposed and will be discussed.

Tsay, S.-C.↗
NASA NTRS2007

Continental Scale Aerosol Optical Properties Over East Asia as Measured by Aeronet and Comparison to Satellite and Modeled Results

The AERONET program has operated in E. Asia since 1995 providing time continuous and time averaged ground-based column-integrated aerosol optical properties in a variety of aerosol regimes In the last four years the distribution has greatly increased in Siberia, China, SE Asia and India in particular. Commensurate with that, significant improvement in data processing algorithms (Version 2.0) and access to ancillary data products through the WWW have become available to the scientific community. At this writing the following distribution represents E and S. Asia: 5 sites operate in Siberia (2 years), 1 in Mongolia (9 years), 3 in Korea (3 to 6 years), 3 in Japan (2 to 7 years), China 11 (6 to 0 years), Taiwan 4 (7 to 2 yrs), Viet Nam 2 (4 years), Thailand 2 to 5 (4 years), and Singapore 1 (4 months), India 1 to 3 (7 to 1 years), Pakistan 2 (1 year), and UAE 3 (3 years). An analysis of the aerosol optical depth at 500 nm using annual average quality assured AERONET data (pre 2006) was used to estimate the mean annual aerosol loading by continent, sub continent and ocean. The individual site data were assumed representative of regional aerosol loading and aggregated to the sub-continental, continental and oceanic areas and presented. This analysis will be updated with more recent data with particular emphasis on seasonal results for Asia and the addition of single scattering albedo retrievals. The ground based results will be compared to MODIS collection 5 results and model estimates for E. Asia using the AERONET Synergy Tool.

Holben, B. N.↗
NASA NTRS2013

Impact Assessment of Biomass Burning on Air Quality in Southeast and East Asia During BASE-ASIA

A synergy of numerical simulation, ground-based measurement and satellite observation was applied to evaluate the impact of biomass burning originating from Southeast Asia (SE Asia) within the framework of NASA's 2006 Biomass burning Aerosols in Southeast Asia: Smoke Impact Assessment (BASE-ASIA). Biomass burning emissions in the spring of 2006 peaked in MarcheApril when most intense biomass burning occurred in Myanmar, northern Thailand, Laos, and parts of Vietnam and Cambodia. Model performances were reasonably validated by comparing to both satellite and ground-based observations despite overestimation or underestimation occurring in specific regions due to high uncertainties of biomass burning emission. Chemical tracers of particulate K(+), OC concentrations, and OC/EC ratios showed distinct regional characteristics, suggesting biomass burning and local emission dominated the aerosol chemistry. CMAQ modeled aerosol chemical components were underestimated at most circumstances and the converted AOD values from CMAQ were biased low at about a factor of 2, probably due to the underestimation of biomass emissions. Scenario simulation indicated that the impact of biomass burning to the downwind regions spread over a large area via the Asian spring monsoon, which included Southern China, South China Sea, and Taiwan Strait. Comparison of AERONET aerosol optical properties with simulation at multi-sites clearly demonstrated the biomass burning impact via longrange transport. In the source region, the contribution from biomass burning to AOD was estimated to be over 56%. While in the downwind regions, the contribution was still significant within the range of 26%-62%.

biomass burning↗
NASA NTRS2005

Atmospheric Teleconnection over Eurasia Induced by Aerosol Radiative Forcing During Boreal Spring

The direct effects of aerosols on global and regional climate during boreal spring are investigated based on simulations using the NASA Global Modeling and Assimilation Office (GMAO) finite-volume general circulation model (fvGCM) with Microphyics of clouds in Relaxed Arakawa Schubert Scheme (McRAS). The aerosol loading are prescribed from three-dimensional monthly distribution of tropospheric aerosols viz., sulfate, black carbon, organic carbon, soil dust, and sea salt from output of the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The aerosol extinction coefficient, single scattering albedo, and asymmetric factor are computed as wavelength-dependent radiative forcing in the radiative transfer scheme of the fvGCM, and as a function of the aerosol loading and ambient relative humidity. We find that anomalous atmospheric heat sources induced by absorbing aerosols (dust and black carbon) excites a planetary scale teleconnection pattern in sea level pressure, temperature and geopotential height spanning North Africa through Eurasia to the North Pacific. Surface cooling due to direct effects of aerosols is found in the vicinity and downstream of the aerosol source regions, i.e., South Asia, East Asia, and northern and western Africa. Additionally, atmospheric heating is found in regions with large loading of dust (over Northern Africa, and Middle East), and black carbon (over South-East Asia). Paradoxically, the most pronounced feature in aerosol-induced surface temperature is an east-west dipole anomaly with strong cooling over the Caspian Sea, and warming over central and northeastern Asia, where aerosol concentration are low. Analyses of circulation anomalies show that the dipole anomaly is a part of an atmospheric teleconnection driven by atmospheric heating anomalies induced by absorbing aerosols in the source regions, but the influence was conveyed globally through barotropic energy dispersion and sustained by feedback processes associated with the regional circulations.

Kim, Maeng-Ki↗
NASA NTRS2006

Atmospheric Teleconnection over Eurasia Induced by Aerosol Radiative Forcing during Boreal Spring

The direct effects of aerosols on global and regional climate during boreal spring are investigated based on numerical simulations with the NASA Global Modeling and Assimilation Office finite-volume general circulation model (fvGCM) with Microphyics of Clouds with the Relaxed Arakawa Schubert Scheme (McRAS), using aerosol forcing functions derived from the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The authors find that anomalous atmospheric heat sources induced by absorbing aerosols (dust and black carbon) excite a planetary-scale teleconnection pattern in sea level pressure, temperature, and geopotential height spanning North Africa through Eurasia to the North Pacific. Surface cooling due to direct effects of aerosols is found in the vicinity and downstream of the aerosol source regions, that is, South Asia, East Asia, and northern and western Africa. Significant atmospheric heating is found in regions with large loading of dust (over northern Africa and the Middle East) and black carbon (over Southeast Asia). Paradoxically, the most pronounced feature in aerosol-induced surface temperature is an east west dipole anomaly with strong cooling over the Caspian Sea and warming over central and northeastern Asia, where aerosol concentrations are low. Analyses of circulation anomalies show that the dipole anomaly is a part of an atmospheric teleconnection pattern driven by atmospheric heating anomalies induced by absorbing aerosols in the source regions, but the influence was conveyed globally through barotropic energy dispersion and sustained by feedback processes associated with the regional circulations. The surface temperature signature associated with the aerosol-induced teleconnection bears striking resemblance to the spatial pattern of observed long-term trend in surface temperature over Eurasia. Additionally, the boreal spring wave train pattern is similar to that reported by Fukutomi et al. associated with the boreal summer precipitation seesaw between eastern and western Siberia. The results of this study raise the possibility that global aerosol forcing during boreal spring may play an important role in spawning atmospheric teleconnections that affect regional and global climates.

Kim, Maeng-Ki↗
DOE OSTI2022

Long-term trends in urban NO 2 concentrations and associated paediatric asthma incidence: estimates from global datasets

Combustion-related nitrogen dioxide (NO 2 ) air pollution is associated with paediatric asthma incidence. We aimed to estimate global surface NO 2 concentrations consistent with the Global Burden of Disease study for 1990-2019 at a 1 km resolution, and the concentrations and attributable paediatric asthma incidence trends in 13 189 cities from 2000 to 2019. We scaled an existing annual average NO 2 concentration dataset for 2010-12 from a land use regression model (based on 5220 NO 2 monitors in 58 countries and land use variables) to other years using NO 2 column densities from satellite and reanalysis datasets. We applied these concentrations in an epidemiologically derived concentration-response function with population and baseline asthma rates to estimate NO 2 -attributable paediatric asthma incidence. We estimated that 1.85 million (95% uncertainty interval [UI] 0.93-2.80 million) new paediatric asthma cases were attributable to NO 2 globally in 2019, two thirds of which occurred in urban areas (1.22 million cases; 95% UI 0.60-1.8 million). The proportion of paediatric asthma incidence that is attributable to NO 2 in urban areas declined from 19.8% (1.22 million attributable cases of 6.14 million total cases) in 2000 to 16.0% (1.24 million attributable cases of 7.73 million total cases) in 2019. Urban attributable fractions dropped in high-income countries (-41%), Latin America and the Caribbean (-16%), central Europe, eastern Europe, and central Asia (-13%), and southeast Asia, east Asia, and Oceania (-6%), and rose in south Asia (+23%), sub-Saharan Africa (+11%), and north Africa and the Middle East (+5%). The contribution of NO 2 concentrations, paediatric population size, and asthma incidence rates to the change in NO 2 -attributable paediatric asthma incidence differed regionally. Despite improvements in some regions, combustion-related NO 2 pollution continues to be an important contributor to paediatric asthma incidence globally, particularly in cities. Mitigating air pollution should be a crucial element of public health strategies for children.

60 APPLIED LIFE SCIENCES↗
DOE OSTI2023

Influence of Spatial Dipole Pattern in Asian Aerosol Changes on East Asian Summer Monsoon

Since China implemented the Air Pollution Prevention and Control Action Plan in 2013, the aerosol emissions in East Asia have been greatly reduced, while emissions in South Asia have continued to increase. This has led to a dipole pattern of aerosol emissions between South Asia and East Asia. Here, the East Asian summer monsoon (EASM) responses to the dipole changes in aerosol emissions during 2013–17 are investigated using the atmosphere model of Community Earth System Model version 2 (CESM2). We show that decreases in East Asian emissions alone lead to a positive aerosol effective radiative forcing (ERF) of 1.59 (±0.97) W m -2 over central-eastern China (25°–40°N, 105°–122.5°E), along with a 0.09 (±0.07)°C warming in summer during 2013–17. The warming intensified the land–sea thermal contrast and increased the rainfall by 0.32 (±0.16) mm day -1 . When considering both the emission reductions in East Asia and increases in South Asia, the ERF is increased to 3.39 (±0.89) W m -2 , along with an enhanced warming of 0.20 (±0.08)°C over central-eastern China, while the rainfall insignificant decreased by 0.07 (±0.16) mm day -1 . It is due to the westward shift of the strengthened western Pacific subtropical high, linked to the increase in black carbon in South Asia. Based on multiple EASM indices, the reductions in aerosol emissions from East Asia alone increased the EASM strength by almost 5%. Finally, considering the effect of the westward shift of WPSH, the dipole changes in emissions together increased the EASM by 5%–15% during 2013–17, revealing an important role of South Asian aerosols in changing the East Asian climate.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2011

A Critical Examination of Spatial Biases Between MODIS and MISR Aerosol Products - Application for Potential AERONET Deployment

AErosol RObotic NETwork (AERONET) data are the primary benchmark for evaluating satellite-retrieved aerosol properties. However, despite its extensive coverage, the representativeness of the AERONET data is rarely discussed. Indeed, many studies have shown that satellite retrieval biases have a significant degree of spatial correlation that may be problematic for higher-level processes or inverse-emissions-modeling studies. To consider these issues and evaluate relative performance in regions of few surface observations, cross-comparisons between the Aerosol Optical Depth (AOD) products of operational MODIS Collection 5.1 Dark Target (DT) and operational MODIS Collection 5.1 Deep Blue (DB) with MISR version 22 were conducted. Through such comparisons, we can observe coherent spatial features of the AOD bias while side-stepping the full analysis required for determining when or where either retrieval is more correct. We identify regions where MODIS to MISR AOD ratios were found to be above 1.4 and below 0.7. Regions where lower boundary condition uncertainty is likely to be a dominant factor include portions of Western North America, the Andes mountains, Saharan Africa, the Arabian Peninsula, and Central Asia. Similarly, microphysical biases may be an issue in South America, and specific parts of Southern Africa, India Asia, East Asia, and Indonesia. These results help identify high-priority locations for possible future deployments of both in situ and ground based remote sensing measurements. The Supplement includes a km1 file.

Shi, Y.↗
DOE OSTI2023

Influence of Spatial Dipole Pattern in Asian Aerosol Changes on East Asian Summer Monsoon

Since China implemented the Air Pollution Prevention and Control Action Plan in 2013, the aerosol emissions in East Asia have been greatly reduced, while emissions in South Asia have continued to increase. This has led to a dipole pattern of aerosol emissions between South Asia and East Asia. We report the East Asian summer monsoon (EASM) responses to the dipole changes in aerosol emissions during 2013–17 are investigated using the atmosphere model of Community Earth System Model version 2 (CESM2). We show that decreases in East Asian emissions alone lead to a positive aerosol effective radiative forcing (ERF) of 1.59 (±0.97) W m -2 over central-eastern China (25°–40°N, 105°–122.5°E), along with a 0.09 (±0.07)°C warming in summer during 2013–17. The warming intensified the land–sea thermal contrast and increased the rainfall by 0.32 (±0.16) mm day -1 . When considering both the emission reductions in East Asia and increases in South Asia, the ERF is increased to 3.39 (±0.89) W m -2 , along with an enhanced warming of 0.20 (±0.08)°C over central-eastern China, while the rainfall insignificant decreased by 0.07 (±0.16) mm day -1 . It is due to the westward shift of the strengthened western Pacific subtropical high, linked to the increase in black carbon in South Asia. Based on multiple EASM indices, the reductions in aerosol emissions from East Asia alone increased the EASM strength by almost 5%. Considering the effect of the westward shift of WPSH, the dipole changes in emissions together increased the EASM by 5%–15% during 2013–17, revealing an important role of South Asian aerosols in changing the East Asian climate.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2012

The Aerosol-Monsoon Climate System of Asia

In Asian monsoon countries such as China and India, human health and safety problems caused by air-pollution are worsening due to the increased loading of atmospheric pollutants stemming from rising energy demand associated with the rapid pace of industrialization and modernization. Meanwhile, uneven distribution of monsoon rain associated with flash flood or prolonged drought, has caused major loss of human lives, and damages in crop and properties with devastating societal impacts on Asian countries. Historically, air-pollution and monsoon research are treated as separate problems. However a growing number of recent studies have suggested that the two problems may be intrinsically intertwined and need to be studied jointly. Because of complexity of the dynamics of the monsoon systems, aerosol impacts on monsoons and vice versa must be studied and understood in the context of aerosol forcing in relationship to changes in fundamental driving forces of the monsoon climate system (e.g. sea surface temperature, land-sea contrast etc.) on time scales from intraseasonal variability (~weeks) to climate change (~ multi-decades). Indeed, because of the large contributions of aerosols to the global and regional energy balance of the atmosphere and earth surface, and possible effects of the microphysics of clouds and precipitation, a better understanding of the response to climate change in Asian monsoon regions requires that aerosols be considered as an integral component of a fully coupled aerosol-monsoon system on all time scales. In this paper, using observations and results from climate modeling, we will discuss the coherent variability of the coupled aerosol-monsoon climate system in South Asia and East Asia, including aerosol distribution and types, with respect to rainfall, moisture, winds, land-sea thermal contrast, heat sources and sink distributions in the atmosphere in seasonal, interannual to climate change time scales. We will show examples of how elevated absorbing aerosols (dust and black carbon) may interact with monsoon dynamics to produce feedback effects on the atmospheric water cycle, leading to in accelerated melting of snowpacks over the Himalayas and Tibetan Plateau, and subsequent changes in evolution of the pre-monsoon and peak monsoon rainfall, moisture and wind distributions in South Asia and East Asia.

Lau, William K. M.↗
NASA NTRS2005

NASA's East and Southeast Asia Initiatives: BASE-ASIA and EAST-AIRE

Airborne dust from northern China influences air quality and regional climate in Asia during springtime. However, with the economic growth in China, increased emission of particulate air pollutants from industrial and vehicular sources will not only impact the earth's radiation balance, but also adversely affect human health year round. In addition, both of dust and aerosol pollutants can be transported swiftly across the Pacific affecting North America within a few days. Asian dust and pollutant aerosols can be detected by their colored appearance using current Earth observing satellites (e.g., MODIS, SeaWiFS, TOMS, etc.) and by sunphotometers deployed on the surface of the earth. Biomass burning has been a regular practice for land clearing and conversion in many countries, especially those in Africa, South America, and Southeast Asia. However, the climatology of Southeast Asia is very different than that of Africa and South America, such that large-scale biomass burning causes smoke to interact extensively with clouds during the peak-burning season of March to April. Globally significant sources of greenhouse gases (eg., CO2, CH4), chemically active gases (e.g., NO, CO, HC, CH3Br), and atmospheric aerosols are produced by biomass burning. These gases influence the Earth-atmosphere system, impacting both global climate and tropospheric chemistry. Some aerosols can serve as cloud condensation nuclei, which play a role in determining cloud lifetime and precipitation, altering the earth's radiation and water budgets. Biomass burning also affects the biogeochemical cycling of nitrogen and carbon compounds; the hydrological cycle; land surface reflectivity and emissivity; and ecosystem biodiversity and stability. Two NASA initiatives, EAST-AIRE (East Asian Study of Tropospheric Aerosols: an International Regional Experiment) and BASE-ASIA (Biomass-burning Aerosols in South East-Asia: Smoke Impact Assessment) will be presented. The objectives of these initiatives is to develop a better understanding of the impacts of aerosols on regional-to-global climate, hydrological and carbon cycles, and tropospheric chemistry.

Tsay, S.↗
NASA NTRS2005

Effects of Aerosol on Atmospheric Dynamics and Hydrologic Processes during Boreal Spring and Summer

Global and regional climate impacts of present-day aerosol loading during boreal spring are investigated using the NASA finite volume General Circulation Model (fvGCM). Three-dimensional distributions of loadings of five species of tropospheric aerosols, i.e., sulfate, black carbon, organic carbon, soil dust, and sea salt are prescribed from outputs of the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The aerosol loadings are used to calculate the extinction coefficient, single scattering albedo, and asymmetric factor at eleven spectral wavelengths in the radiative transfer code. We find that aerosol-radiative forcing during boreal spring excites a wavetrain-like pattern in tropospheric temperature and geopotential height that emanates from Northern Africa, through Eurasia, to northeastern Pacific. Associated with the teleconnection is strong surface cooling over regions with large aerosol loading, i.e., China, India, and Africa. Low-to-mid tropospheric heating due to shortwave absorption is found in regions with large loading of dust (Northern Africa, and central East Asia), and black carbon (South and East Asia). In addition pronounced surface cooling is found over the Caspian Sea and warming over Eurasian and northeastern Asia, where aerosol loadings are relatively low. These warming and cooling are components of teleconnection pattern produced primarily by atmospheric heating from absorbing aerosols, i.e., dust from North Africa and.black carbon from South and East Asia. Effects of aerosols on atmospheric hydrologic cycle in the Asian monsoon region are also investigated. Results show that absorbing aerosols, i.e., black carbon and dust, induce large-scale upper-level heating anomaly over the Tibetan Plateau in April and May, ushering in an early onset of the Indian summer monsoon. Absorbing aerosols also enhance lower-level heating and anomalous ascent over northern India, intensifying the Indian monsoon. Overall, the aerosol-induced large-scale surface temperature cooling leads to a reduction of monsoon rainfall over the East Asia continent, and adjacent oceanic regions.

Lau, William K. M.↗
NASA NTRS2005

Effects of Aerosol on Atmospheric Dynamics and Hydrologic Processes During Boreal Spring and Summer

Global and regional climate impacts of present-day aerosol loading during boreal spring are investigated using the NASA finite volume General Circulation Model (fvGCM). Three-dimensional distributions of loadings of five species of tropospheric aerosols, i.e., sulfate, black carbon, organic carbon, soil dust, and sea salt are prescribed from outputs of the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The aerosol loadings are used to calculate the extinction coefficient, single scattering albedo, and asymmetric factor at eleven spectral wavelengths in the radiative transfer code. We find that aerosol-radiative forcing during boreal spring excites a wavetrain-like pattern in tropospheric temperature and geopotential height that emanates from Northern Africa, through Eurasia, to northeastern Pacific. Associated with the teleconnection is strong surface cooling over regions with large aerosol loading, i.e., China, India, and Africa. Low-to-mid tropospheric heating due to shortwave absorption is found in regions with large loading of dust (Northern Africa, and central East Asia), and black carbon (South and East Asia). In addition pronounced surface cooling is found over the Caspian Sea and warming over Eurasian and northeastern Asia, where aerosol loadings are relatively low. These warming and cooling are components of teleconnection pattern produced primarily by atmospheric heating from absorbing aerosols, i.e., dust from North Africa and black carbon from South and East Asia. Effects of aerosols on atmospheric hydrologic cycle in the Asian monsoon region are also investigated. Results show that absorbing aerosols, i.e., black carbon and dust, induce large-scale upper-level heating anomaly over the Tibetan Plateau in April and May, ushering in an early onset of the Indian summer monsoon. Absorbing aerosols also enhance lower-level heating and anomalous ascent over northern India, intensifying the Indian monsoon. Overall, the aerosol-induced large-scale surface tempera- cooling leads to a reduction of monsoon rainfall over the East Asia continent, and adjacent oceanic regions.

Lau, William K. M.↗