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Present and future aerosol impacts on Arctic climate change in the GISS-E2.1 Earth system model

The Arctic is warming 2 to 3 times faster than the global average, partly due to changes in short-lived climate forcers (SLCFs) including aerosols. In order to study the effects of atmospheric aerosols in this warming, recent past (1990–2014) and future (2015–2050) simulations have been carried out using the GISS-E2.1 Earth system model to study the aerosol burdens and their radiative and climate impacts over the Arctic (>60°N), using anthropogenic emissions from the Eclipse V6b and the Coupled Model Intercomparison Project Phase 6 (CMIP6) databases, while global annual mean greenhouse gas concentrations were prescribed and kept fixed in all simulations. Results showed that the simulations have underestimated observed surface aerosol levels, in particular black carbon (BC) and sulfate (SO2−4), by more than 50 %, with the smallest biases calculated for the atmosphere-only simulations, where winds are nudged to reanalysis data. CMIP6 simulations performed slightly better in reproducing the observed surface aerosol concentrations and climate parameters, compared to the Eclipse simulations. In addition, simulations where atmosphere and ocean are fully coupled had slightly smaller biases in aerosol levels compared to atmosphere-only simulations without nudging. Arctic BC, organic aerosol (OA), and SO2−4 burdens decrease significantly in all simulations by 10 %–60 % following the reductions of 7 %–78 % in emission projections, with the Eclipse ensemble showing larger reductions in Arctic aerosol burdens compared to the CMIP6 ensemble. For the 2030–2050 period, the Eclipse ensemble simulated a radiative forcing due to aerosol–radiation interactions (RFARI) of −0.39 ± 0.01 W/sq. m, which is −0.08 W/sq. m larger than the 1990–2010 mean forcing (−0.32 W/sq. m), of which −0.24 ± 0.01 W/sq. m was attributed to the anthropogenic aerosols. The CMIP6 ensemble simulated a RFARI of −0.35 to −0.40 W/sq. m for the same period, which is −0.01 to −0.06 W/sq. m larger than the 1990–2010 mean forcing of −0.35 W/sq. m. The scenarios with little to no mitigation (worst-case scenarios) led to very small changes in the RFARI, while scenarios with medium to large emission mitigations led to increases in the negative RFARI, mainly due to the decrease in the positive BC forcing and the decrease in the negative SO2−4 forcing. The anthropogenic aerosols accounted for −0.24 to −0.26 W/sq. m of the net RFARI in 2030–2050 period, in Eclipse and CMIP6 ensembles, respectively. Finally, all simulations showed an increase in the Arctic surface air temperatures throughout the simulation period. By 2050, surface air temperatures are projected to increase by 2.4 to 2.6 °C in the Eclipse ensemble and 1.9 to 2.6 °C in the CMIP6 ensemble, compared to the 1990–2010 mean. Overall, results show that even the scenarios with largest emission reductions leads to similar impact on the future Arctic surface air temperatures and sea-ice extent compared to scenarios with smaller emission reductions, implying reductions of greenhouse emissions are still necessary to mitigate climate change.

Aerosols↗

Implications of Arctic Sea Ice Decline for the Earth System

Arctic sea ice decline has led to an amplification of surface warming and is projected to continue to decline from anthropogenic forcing, although the exact timing of ice-free summers is uncertain owing to large natural variability. Sea ice reductions affect surface heating patterns and the atmospheric pressure distribution, which may alter midlatitude extreme weather patterns. Increased light penetration and nutrient availability during spring from earlier ice breakup enhances primary production in the Arctic Ocean and its adjacent shelf seas. Ice-obligate marine mammals may be losers, whereas seasonally migrant species may be winners from rapid sea ice decline. Tundra greening is occurring across most of the Arctic, driven primarily by warming temperatures, and is displaying complex spatial patterns that are likely tied to other factors. Sea ice changes are affecting greenhouse gas exchanges as well as halogen chemistry in the Arctic. This review highlights the heterogeneous nature of Arctic change, which is vital for researchers to better understand.

Decline↗

Investigation of Benthic Foraminiferal Non-Traditional Stable Isotopes to Reconstruct Methane Fluxes in Sedimentary Environments

Methane (CH4) is an important greenhouse gas, with a global warming potential much higher than carbon dioxide (CO2) on a short time scale. Even if the residence time of CH4 in the atmosphere is relatively short (tens of years), one of the products of CH4 oxidation is CO2, a greenhouse gas with a much longer residence time in the atmosphere (tens to hundreds of years). CH4 has been proposed as one of the trigger mechanisms for rapid global climate change today and in the geological past. With regards to the geological past, numerous studies proposed the benthic foraminiferal carbon isotope ratio (Delta13C) as a tool to reconstruct the impact of marine CH4 on rapid climate changes; however, the investigation of modern benthic foraminiferal Delta13C have produced inconclusive results. CH4 has a distinctive hydrogen isotope (Delta(D)) and Delta13C signature compared to seawater, and sulfate reduction, often coupled to CH4 anaerobic oxidation in sediments, changes the sulfur isotope signature (Delta34S) of the remaining sulfate in porewater. Therefore, we hypothesize that the Delta(D) and Delta34S signature of infaunal benthic foraminiferal species can provide a complementary approach to Delta13C to study CH4 dynamics in sedimentary environments. Here, we present the preliminary results obtained analyzing Uvigerina peregrina Delta(D) and Delta34S from three different locations at Hydrate Ridge, offshore Oregon. Unfortunately, the lack of chemical data related to the moment of foraminiferal calcification makes difficult to build a robust relationship among the U. peregrina stable isotopes and the CH4 fluxes at the sampling sites. However, our results look very promising, as each site is characterized by a different Delta(D) and Delta34S signature. We emphasize that this study represents the first step in the development of new proxies (Delta(D)) and Delta34S), which may complement the more traditional benthic foraminiferal Delta13C values, to reconstruct marine CH4 fluxes in the geological past.

Borrelli, C.↗

Detectability of anthropogenic impacts on terrestrial carbon storage through space-based greenhouse gas observations

While changes in human activity and their impact on the terrestrial biosphere may be apparent in inventory and land-surface satellite data, reliably matching these changes to signals in atmospheric greenhouse gases remains challenging. The dominant signals in atmospheric carbon dioxide (CO2) are those of the seasonal and diurnal variability of the terrestrial biosphere. As a result, the historically large short-term change in anthropogenic fossil fuel emissions due to COVID-19 produced an atmospheric CO2 signal near the threshold of detectability of the current space-based observing system. Impacts of anthropogenic activity on terrestrial carbon storage are likewise expected to be difficult, if not impossible, to detect and validate with atmospheric observations. For example, many forest management projects involve reduction of wood removals that would otherwise be taken off site and decompose years later and are thus not reflected in immediate onsite carbon fluxes. Nevertheless, changes implemented over a jurisdictional scale, as opposed to individual projects, may be detectable. This presentation will analyze to what extent NASA’s Goddard Earth Observing System (GEOS)/Orbiting Carbon Observatory 2 (OCO-2) assimilated column CO2 (XCO2) product is able to detect anthropogenic changes to terrestrial carbon storage and the results of several simulation experiments meant to represent potential forest management scenarios. As examples, we consider past and future changes due to conversion in the Tropics to agricultural land use from slash-and-burn, e.g., from Reducing emissions from deforestation and forest degradation in developing countries (REDD+) efforts. This has the potential to inform what practices may be observable with current and future technology, e.g., Europe’s upcoming CO2 monitoring mission (CO2M), and where improvement is needed.

Brad Weir↗

Investigation of Bio-Regenerative Life Support and Trash-to-Gas Experiment on a 4-Month Mars Simulation Mission

Future crewed missions to other planets or deep space locations will require regenerative Life Support Systems (LSS) as well as recycling processes for mission waste. Constant resupply of many commodity materials will not be a sustainable option for deep space missions, nor will stowing trash on board a vehicle or at a lunar or Martian outpost. The habitable volume will decline as the volume of waste increases. A complete regenerative environmentally controlled life support system (ECLSS) on an extra-terrestrial outpost will likely include physico-chemical and biological technologies, such as bioreactors and greenhouse modules. Physico-chemical LSS do not enable food production and bio-regenerative LSS are not stable enough to be used alone in space. Mission waste that cannot be recycled into the bio-regenerative ECLSS can include excess food, food packaging, clothing, tape, urine and fecal waste. This waste will be sent to a system for converting the trash into high value products. Two crew members on a 120 day Mars analog simulation, in collaboration with Kennedy Space Centers (KSC) Trash to Gas (TtG) project investigated a semi-closed loop system that treated non-edible biomass and other logistical waste for volume reduction and conversion into useful commodities. The purpose of this study is to show how plant growth affects the amount of resources required by the habitat and how spent plant material can be recycled. Real-time data was sent to the reactor at KSC in Florida for replicating the analog mission waste for laboratory operation. This paper discusses the 120 day mission plant growth activity, logistical and plant waste management, power and water consumption effects of the plant and logistical waste, and potential energy conversion techniques using KSCs TtG technology.

Trash-to-Gas↗

Accounting for Static and Dynamic Open Water in the Modeling of SMAP Brightness Temperatures over Peatlands

Hydrological change in peatlands due to anthropogenic disturbance and global warming can release enormous amounts of greenhouse gas emissions. Passive microwave satellite observations are an opportunity to globally monitor these changes. Abundant static and dynamic open water surfaces in peatlands strongly affect observed brightness temperatures (Tb). Here, we account for these contributions in radiative transfer modeling using NASA's Goddard Earth Observing System Model version 5 (GEOS-5) static open water mask and, for the dynamic open water fraction, the simulated inundated area using a version of the GEOS-5 Catchment land surface model that has been modified for peatland areas (PEAT-CLSM). Modeled Tb is compared against two years of SMAP L-band Tb. Preliminary results indicate: (i) a bias reduction when including the static open water fraction in a simple RTM mixing model, and ii) significantly improved correlation between modeled and observed Tb when using land surface output from PEAT-CLSM instead of the operational CLSM.

passive microwave↗

Investigation of Bio-Regenerative Life Support and Trash-To-Gas Experiment on a 4 Month Mars Simulation Mission

Future crewed missions to other planets or deep space locations will require regenerative Life Support Systems (LSS) as well as recycling processes for mission waste. Constant resupply of many commodity materials will not be a sustainable option for deep space missions, nor will storing trash on board a vehicle or at a lunar or Martian outpost. The habitable volume will decline as the volume of waste increases. A complete regenerative environmentally controlled life support system (ECLSS) on an extra-terrestrial outpost will likely include physico-chemical and biological technologies, such as bioreactors and greenhouse modules. Physico-chemical LSS do not enable food production and bio-regenerative LSS are not stable enough to be used alone in space. Mission waste that cannot be recycled into the bio-regenerative ECLSS can include excess food, food packaging, clothing, tape, urine and fecal waste. This waste will be sent to a system for converting the trash into the high value products. Two crew members on a 120 day Mars analog simulation, in collaboration with Kennedy Space Centers (KSC) Trash to Gas (TtG) project investigated a semi-closed loop system that treated non-edible biomass and other logistical waste for volume reduction and conversion into useful commodities. The purposes of this study are to show the how plant growth affects the amount of resources required by the habitat and how spent plant material can be recycled. Real-time data was sent to the reactor at KSC in Florida for replicating the analog mission waste for laboratory operation. This paper discusses the 120 day mission plant growth activity, logistical and plant waste management, power and water consumption effects of the plant and logistical waste, and potential energy conversion techniques using KSCs TtG reactor technology.

trash to gas↗

Why Hasn't Earth Warmed as Much as Expected?

The observed increase in global mean surface temperature (GMST) over the industrial era is less than 40% of that expected from observed increases in long-lived greenhouse gases together with the best-estimate equilibrium climate sensitivity given by the 2007 Assessment Report of the Intergovernmental Panel on Climate Change (IPCC). Possible reasons for this warming discrepancy are systematically examined here. The warming discrepancy is found to be due mainly to some combination of two factors: the IPCC best estimate of climate sensitivity being too high and/or the greenhouse gas forcing being partially offset by forcing by increased concentrations of atmospheric aerosols; the increase in global heat content due to thermal disequilibrium accounts for less than 25% of the discrepancy, and cooling by natural temperature variation can account for only about 15 %. Current uncertainty in climate sensitivity is shown to preclude determining the amount of future fossil fuel CO2 emissions that would be compatible with any chosen maximum allowable increase in GMST; even the sign of such allowable future emissions is unconstrained. Resolving this situation, by empirical determination of the earth's climate sensitivity from the historical record over the industrial period or through use of climate models whose accuracy is evaluated by their performance over this period, is shown to require substantial reduction in the uncertainty of aerosol forcing over this period.

Schwartz, Stephen E.↗

Attribution of Trends and Variability in Surface Ozone over the United States

Concentrations of tropospheric ozone, a greenhouse gas and air pollutant, are impacted by changes in precursor emissions as well meteorology and influx from the stratosphere. Observations show a decreasing trend in summertime surface ozone at rural stations in the eastern United States, while some western stations show increasing trends, particularly in springtime. We use the Global Modeling Initiative (GMI) global chemical transport model to investigate the roles of precursor emission changes, meteorological variability, and stratosphere-troposphere exchange (STE) in explaining observed trends in surface ozone from rural sites in the United States from 1991-2010. The model's interannual variability shows significant correlations with observations from many of the surface sites. We also compare the simulated ozone to ozonesonde data for several locations with sufficiently long records. We compare a simulation with time-dependent precursor emissions, including emission reductions over the United States and Europe and increases over Asia, to a simulation with fixed emissions to quantify the impact of changing emissions on the surface trends. The simulation with varying emissions reproduces much of the east-west difference in summertime ozone over the U.S., although it generally underestimates the negative trend in the East. In contrast, the fixed-emission simulation shows increasing ozone at both eastern and western sites. We will discuss possible causes of this behavior, including long-range transport and STE.

ozone↗

MISTRAL: Concept and Analysis of Persistent Airborne Localization of GHG Emissions

In this study, we propose a concept for localizing and mitigating greenhouse gases and other emissions from areas of various sizes, using a multiscale, airborne localization fleet, supported by information from satellites. Our objective is a rapidly implementable capability for the reduction of atmospheric methane by empowering the communities in proximity to emissions to actively contribute to methane mitigation via fleet operations by local governments, first responders, and individuals . Fully autonomous operations are economically desirable and technically feasible now. However, the development of regulations for autonomous operations is in early stages. Since rapid impact is critical to reducing emissions, the concept starts with remotely controlled vehicles. As regulations for autonomous operations reach maturity, the concept can be easily transitioned from the remotely piloted to autonomous mode. We report on a preliminary system analysis of the concept. Localization of methane emissions from the Permian Basin oil and gas production site serves as the design reference mission; however, the airborne concept is applicable to a broad range of use cases, and we describe several in this analysis. We consider leveraging satellite and ground-based resources within the airborne concept of operations. The study analyses uninhabited aerial system localization operations under the most conservative assumptions on resources and available information. Even under these assumptions, the concept is shown to be viable for local community operations.

airborne methane localization↗

Simulation and Analysis of Technology and Operational Procedures to Reduce the Combined Effects of Emissions and Contrails

The development and evaluation of concepts and technology to support future air traffic management systems require a hierarchy of models ranging from real-time simulations to extensive field evaluations. Air traffic simulation models such as Airspace Concept Evaluation System, Center Tracon Automation System, Future Air traffic management Concept Evaluation Tool and others are used to design air traffic systems balancing the conflicting objectives of maximizing safety, meeting future demands for airports and airspace and increase efficiency of traffic flows in the presence of uncertain weather. The impact of aviation emissions and contrails on climate imposes another constraint on the design of aircraft and aviation operations. The understanding of the complex interaction between physical climate system, the carbon and other greenhouse gas emissions and aviation activity can be improved by the development of integrated assessment models that include emission and climate models together with air traffic simulations. The modeling of aircraft emissions and their interaction with each other to change the concentration levels of different gasses in the atmosphere and the resulting impact of the radiative forcing on the equilibrium of the Earth's atmosphere is complex and requires the use of coupled atmosphere-ocean general circulation models together with three-dimensional models of carbon cycle and chemistry of other non-CO2 greenhouse gases. These models are computationally intensive and unsuitable for studies involving the generation of multiple scenarios. Simple emission and climate models, based on the input-output relations of linear systems, capture the fundamental emission to climate impact behavior by careful selection of key variables and their dynamics. The impact of various greenhouse gases depends on the total concentration, effect per unit change in atmospheric concentration and the spatial distribution of the gas. All these quantities are influenced by the lifetime of the gas. The impact of a greenhouse gas depends on the interval of assessment, which may vary from a few decades to a few centuries. Climate metrics are aimed at providing a common scale to compare different greenhouse gases. If the metrics are to be used as a tool in developing and evaluating aviation operations, they should be transparent and easy to apply. Global Warming Potential and Aggregate Global Temperature Potential are some of the commonly used metrics. This paper integrates a national-level air traffic simulation and optimization capability with simple climate models and carbon cycle models, and climate metrics to assess the impact of aviation on climate. The capability brings together metrics, which are useful in aviation operations together with metrics used in climate studies. The capability can be used to make trade-offs between extra fuel cost and reduction in climate impact. There is considerable uncertainty in our understanding of the radiative forcing associated with emissions and contrails. The parameters in the simulation can be used to evaluate the effect of various uncertainties in emission models and contrails. It can also be used to evaluate the impact of different decision horizons. Alternatively, the optimization results from the simulation can be used as inputs to other tools that monetize global climate impacts like the FAA's Aviation Environmental Portfolio Management Tool for Impacts.

impact of aviation on the environment↗

Human influence on joint changes in temperature, rainfall and continental aridity

Despite the pervasive impact of drought on human and natural systems, the large-scale mechanisms conducive to regional drying remain poorly understood. Here we use a multivariate approach to identify two distinct externally forced fingerprints from multiple ensembles of Earth system model simulations. The leading fingerprint, F(M1)(x), is characterized by global warming, intensified wet–dry patterns and progressive large-scale continental aridification, largely driven by multidecadal increases in greenhouse gas (GHG) emissions. The second fingerprint, F(M2)(x), captures a pronounced interhemispheric temperature contrast, associated meridional shifts in the intertropical convergence zone and correlated anomalies in precipitation and aridity over California, the Sahel and India. F(M2)(x) exhibits nonlinear temporal behaviour: the intertropical convergence zone moves southwards before 1975 in response to increases in hemispherically asymmetric sulfate aerosol emissions, and it shifts northwards after 1975 due to reduced sulfur dioxide emissions and the GHG-induced warming of Northern Hemisphere landmasses. Both fingerprints are statistically identifiable in observations of joint changes in temperature, rainfall and aridity during 1950–2014. We show that the reliable simulation of these changes requires combined forcing by GHGs, direct and indirect effects of aerosols, and large volcanic eruptions. Our results suggest that GHG-induced aridification may be modulated regionally by future reductions in sulfate aerosol emissions.

Human influence↗

Requirements for an Advanced Low Earth Orbit (LEO) Sounder (ALS) for Improved Regional Weather Prediction and Monitoring of Greenhouse Gases

Hyperspectral infrared atmospheric sounders (e.g., the Atmospheric Infrared Sounder (AIRS) on Aqua and the Infrared Atmospheric Sounding Interferometer (IASI) on Met Op) provide highly accurate temperature and water vapor profiles in the lower to upper troposphere. These systems are vital operational components of our National Weather Prediction system and the AIRS has demonstrated over 6 hrs of forecast improvement on the 5 day operational forecast. Despite the success in the mid troposphere to lower stratosphere, a reduction in sensitivity and accuracy has been seen in these systems in the boundary layer over land. In this paper we demonstrate the potential improvement associated with higher spatial resolution (1 km vs currently 13.5 km) on the accuracy of boundary layer products with an added consequence of higher yield of cloud free scenes. This latter feature is related to the number of samples that can be assimilated and has also shown to have a significant impact on improving forecast accuracy. We also present a set of frequencies and resolutions that will improve vertical resolution of temperature and water vapor and trace gas species throughout the atmosphere. Development of an Advanced Low Earth Orbit (LEO) Sounder (ALS) with these improvements will improve weather forecast at the regional scale and of tropical storms and hurricanes. Improvements are also expected in the accuracy of the water vapor and cloud properties products, enhancing process studies and providing a better match to the resolution of future climate models. The improvements of technology required for the ALS are consistent with the current state of technology as demonstrated in NASA Instrument Incubator Program and NOAA's Hyperspectral Environmental Suite (HES) formulation phase development programs.

temperature↗

Impact of a Regional US Drought on Land and Atmospheric Carbon

The impacts of drought on regional land and atmospheric carbon are still poorly understood. Here we quantify the impact of a regional US drought on land carbon fluxes (Gross Primary Production, or GPP, and Net Biosphere Production, or NBP) and atmospheric carbon (CO2) by imposing an idealized 3-month meteorological drought in an ensemble of coupled land-atmosphere climate simulations. The imposed drought, applied to the lower Mississippi River Valley (~500,000 km (exp 2)), leads to a 23% GPP reduction in the drought area in the month immediately following the drought’s termination. The drought also caused GPP reductions in some remote areas through drought-induced impacts on remote meteorology, particularly the areas adjacent to the imposed drought. In the remote areas, the induced precipitation changes are responsible for most of the anomalous land productivity. The impact of the drought-induced meteorological anomalies on GPP is greater than that of the CO2 anomalies by at least an order of magnitude. While their impact on GPP is secondary, the drought-induced atmospheric CO2 anomalies near the land surface can be as large as 3.57ppm. The significant CO2 anomalies cover an area up to three times of that of the imposed drought, suggesting that atmospheric transport needs to be considered in the interpretation of drought-induced CO2 anomalies in the atmosphere. The imposed drought also leads to column-averaged CO2 increases of up to 0.78ppm, which is at the edge of the uncertainty from single soundings of current greenhouse gas (GHG) observing satellites.

Eunjee Lee↗

Adsorption and Processes in Spacecraft Environmental Control and Life Support Systems

The environmental control and life support system on a spacecraft must maintain a safe and comfortable environment in which the crew can live and work. The system's functions include supplying the crew with oxygen and water, as well as removing carbon dioxide, water vapor, and trace contaminants from cabin air. Although open-loop systems have been used in the past, logistics and safety factors of current and future missions in space make near-complete recycling of the cabin's air and water desirable. The recycling process may include separation and reduction of carbon dioxide, removal of trace gas-phase contaminants, recovery and purification of humidity condensate, purification and polishing of wastewater streams, and other processes. Several of these operations can be performed totally or in part by adsorption processes. Adsorption processes are frequently good candidates for separation and purification in space by virtue of such characteristics as gravity independence, high reliability, relatively high energy efficiency, design flexibility, technological maturity, and regenerability. For these reasons, adsorption has historically played a key role in life support on U.S. and Russian piloted spacecraft. This article focuses on three current spacecraft life support applications that often use adsorption technology: carbon dioxide separation from cabin air, gas-phase trace contaminant control, and potable water recovery from waste streams. In each application, adsorption technology has been selected for use on the International Space Station. The requirements, science, and hardware for each application are discussed. Eventually, human space exploration may lead to construction of planetary habitats. These habitats may have additional applications, such as control of greenhouse gas composition and purification of hydroponic solutions, and may have different requirements and resources available to them, such as gases present in the planetary atmosphere. Adsorption separation and purification processes may continue to fulfill environmental control and life support needs well into the future.

Dall-Bauman, Liese↗

Adsorption processes in spacecraft environmental control and life support systems

The environmental control and life support system on a spacecraft maintains a safe and comfortable environment in which the crew can live and work by supplying oxygen and water and by removing carbon dioxide, water vapor, and trace contaminants from cabin air. Although open-loop systems have been used successfully in the past for short-duration missions, the economics of current and future long-duration missions in space will make nearly complete recycling of air and water imperative. A variety of operations will be necessary to achieve the goal of nearly complete recycling. These include separation and reduction of carbon dioxide, removal of trace gas-phase contaminants, recovery and purification of humidity condensate, purification and polishing of wastewater streams, and others. Several of these can be performed totally or in part by adsorption processes. These processes are good candidates to perform separations and purifications in space due to their gravity independence, high reliability, relative high energy efficiency, design flexibility, technological maturity, and regenerative nature. For these reasons, adsorption has historically played a key role in life support on U.S. and Russian piloted spacecraft. Among the life support applications that can be achieved through use of adsorption technology are removal of trace contaminants and carbon dioxide from cabin air and recovery of potable water from waste streams. In each of these cases adsorption technology has been selected for use onboard the International Space Station. The requirements, science, and hardware for these applications are discussed. Human space exploration may eventually lead to construction of planetary habitats. These habitats may provide additional opportunities for use of adsorption processes, such as control of greenhouse gas composition, and may have different resources available to them, such as gases present in the planetary atmosphere. Separation and purification processes based on adsorption can be expected to continue to fulfill environmental control and life support needs on future missions.

Review, Tutorial↗

Adsorption Processes in Spacecraft Environmental Control and Life Support Systems

The environmental control and life support system on a spacecraft must maintain a safe and comfortable environment in which the crew can live and work. The system's functions include supplying the crew with oxygen and water as well as removing carbon dioxide, water vapor, and trace contaminants from cabin air. Although open-loop systems have been used in the past, logistics and safety factors of current and future missions in space make near-complete recycling of the cabin's air and water imperative. The recycling process may include separation and reduction of carbon dioxide, removal of trace gas-phase contaminants, recovery and purification of humidity condensate, purification and polishing of wastewater streams, and other processes. Several of these operations can be performed totally or in part by adsorption processes. These processes are frequently good candidates to perform separations and purifications in space due to their gravity independence, high reliability, relatively high energy efficiency, design flexibility, technological maturity, and regenerability. For these reasons, adsorption has historically played a key role in life support on U.S. and Russian piloted spacecraft. This article focuses on three current spacecraft life support applications that often use adsorption technology: gas-phase trace contaminant control, carbon dioxide removal from cabin air, and potable water recovery from waste streams. In each application, adsorption technology has been selected for use on the International Space Station. The requirements, science, and hardware for each of these applications are discussed. Eventually, human space exploration may lead to construction of planetary habitats. These habitats may provide additional opportunities for use of adsorption processes, such as control of greenhouse gas composition, and may have different requirements and resources available to them, such as gases present in the planetary atmosphere. Adsorption separation and purification processes can be expected to continue to fulfill environmental control and life support needs on future missions.

Bauman, Liese Dall↗

Sensitivity of wheat and rice to low levels of atmospheric ethylene

Ethylene (C2H4) gas is produced throughout the life cycle of plants and can accumulate in closed growth chambers to levels 100 times higher than in outside environments. Elevated atmospheric C2H4 can cause a variety of abnormal responses, but the sensitivity to elevated C2H4 is not well characterized. We evaluated the C2H4 sensitivity of wheat (Triticum aestivum L.) and rice (Oryza sativa L.) in five studies. The first three studies compared the effects of continuous C2H4 levels ranging from 0 to 1000 nmol mol-1 (ppb) in a growth chamber throughout the life cycle of the plants. A short-term 1000 nmol mol-1 treatment was included in which exposure was stopped at anthesis. Yield was reduced by 36% in wheat and 63% in rice at 50 nmol mol-1 and both species were virtually sterile when continuously exposed to 1000 nmol mol-1. However, the yield reductions were much less with exposure that stopped at anthesis, suggesting the detrimental effect of C2H4 on yield was greatest around the time of seed set. Two additional studies evaluated the differential sensitivity of two wheat cultivars (Super Dwarf and USU-Apogee) to 50 nmol mol-1 C2H4 at three CO2 levels [350, 1200, 5000 micromoles mol-1 (ppm)] in a greenhouse. Yield of USU-Apogee was not significantly reduced by C2H4 but the yield of Super Dwarf was reduced by 60%. Elevated CO2 did not influence the sensitivity to C2H4. A difference in the C2H4 sensitivity of USU-Apogee between greenhouse and growth chamber trials suggests that C2H4 sensitivity is dependent on the environment. Collectively, the data suggest that relatively low levels of C2H4 could induce anomalous plant responses by accumulation in greenhouses and growth chambers with inadequate ventilation. The data also suggest that C2H4 sensitivity can be reduced by both genetic and environmental manipulations. 2002 Crop Science Society of America.

NASA Discipline Life Sciences Technologies↗