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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
NASA NTRS1972

Pulsar rotation and dispersion measures and the galactic magnetic field.

Use of observations of pulsar polarization and pulse time of arrival at frequencies between 250 and 500 MHz to determine rotation and dispersion measures for 19 and 21 pulsars, respectively. These measurements have been used to calculate mean line-of-sight components of the magnetic field in the path to the pulsars. These and other observations show that there is probably no contribution to the observed rotation measure from the pulsar itself. Low-latitude, low-dispersion pulsars are observed to have strong field components, and a strong dependence of rotation-measure sign on galactic longitude has been found. The observations are consistent with a relatively uniform field of about 3.5 microgauss directed toward about l = 90 deg in the local region, but appear to be inconsistent with the helical model for the local field.

Manchester, R. N.↗
NASA NTRS1973

Recovery of nonferrous metals from scrap automobiles by magnetic fluid levitation.

Ferrofluids are colloidal dispersions of subdomain magnetic solids in carrier liquids. In the presence of a non-homogeneous magnetic field, ferrofluids exert a pressure on immersed nonmagnetic objects in the opposite sense of the field gradient. This pressure force can, when opposite to gravity, levitate objects of higher density than the ferrofluid. This levitation technique can be used to separate solids according to density. Its application to the separation of nonferrous metals from shredded automobiles has been demonstrated on a prototype of a full-scale separator. Its use to recover nonferrous metals from municipal solid wastes also seems practical.

Mir, L.↗
NASA NTRS1965

Magneto-gravity waves

Small amplitude low frequency waves in plasma of infinite conductivity under influence of constant external gravitational and magnetic fields

ATMOSPHERIC CONDUCTIVITY↗
NASA NTRS1980

Plasma waves in a relativistic, strongly anisotropic plasma propagated along a strong magnetic field

The dispersion properties of plasma waves in a relativistic homogeneous plasma propagated along a strong magnetic field are studied. It is shown that the non-damping plasma waves exist in the frequency range omega sub p or = omega or = omega sub L. The values of omega sub p and omega sub L are calculated for an arbitrary homogeneous relativistic function of the particle distribution. In the case of a power ultrarelativistic distribution, it is shown that, if the ultrarelativistic tail of the distribution drops very rapidly, slightly damping plasma waves are possible with the phase velocity (omega/K)c.

Onishchenko, O. G.↗
DOE OSTI2019

Influence of Particle Size on the Spin Pinning Effect in the fcc-FePt Nanoparticles

In this work, the Fe{sub 60}Pt{sub 40} nanoparticles were synthesized through the chemical reduction method by using the Fe(CO){sub 5} and the Pt(acac){sub 2} as the metallic precursor. The particle size of the synthesized FePt nanoparticles was controlled by adjusting the reaction conditions involving of the Fe(CO){sub 5}-injecting temperature and the soak time of reaction. The structure, morphology, and magnetic properties of the synthesized FePt nanoparticles were characterized by XRD, TEM, and vibrating sample magnetometer (VSM), respectively. The synthesized nanoparticles exhibit uniform size and good dispersity. The magnetization behaviors indicate that the nanoparticles present the core-shell magnetic structure including the ferromagnetic core part and the spin-disorder shell part. There exists a spin pinning effect of the shell part on the core part. The increase of particle size weakens the spin pinning effect.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2022

Spin dynamics and exchange interaction in orthoferrite TbFeO 3 with non-Kramers rare-earth ion

The low-temperature spin dynamics of the orthorhombic TbFeO 3 perovskite has been studied. It has been found that the inelastic neutron scattering (INS) spectrum of the investigated compound contains two modes corresponding to different sublattices. It is shown that the iron subsystem orders antiferromagnetically at T N =632 K and exhibits the high-energy magnon dispersion. The magnetic dynamics of this subsystem has been described within the linear spin wave theory and the in-plane and out-of-plane exchange anisotropy has been demonstrated. The approach proposed previously to describe the magnon dispersion in the TmFeO 3 compound has been used. Three levels of the nondispersive crystal electric field corresponding to Tb 3+ ions have been found in the energy region below 40 meV at about 17, 26, and 35 meV. The behavior of the magnetic correlation length of the terbium subsystem has been determined by studying the diffuse scattering at different temperatures. The evolution of this subsystem has been numerically described within the point charge model. In conclusion, it is shown that the numerical data agree satisfactorily with the experiment and with the general concept of the single-ion approximation applied to the rare-earth subsystem of orthorhombic perovskites.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Separation of Kondo lattice coherence from crystal electric field in CeIn 3 with Nd substitutions

The Ce m M n In 3m+2n (m=1,2;n=0,1) family has been one of the most studied families of heavy fermion compounds. This family has revealed many interesting low-temperature physics phenomena, like quantum critical points, heavy fermion superconductivity, and non-Fermi liquid behavior, when these materials are exposed to pressure, magnetic fields, and/or chemical substitution. In this work, we provide a thorough investigation of the Ce 1-x Nd x In 3 phase diagram through single crystal synthesis, x-ray diffraction, energy-dispersive spectroscopy, magnetic susceptibility, and electrical resistivity measurements. Previous electrical resistivity measurements on CeIn 3 reveal a broad maximum, T max ~50 K, which has been associated with the Kondo lattice coherence crossover and/or the crystal electric field depopulation effect as the 4f electrons condense from the high-energy quartet down to the ground state doublet. Our findings show that in the most disordered substitution region, x=0.4–0.5, these features disjoin to reveal two distinct broad humps in electrical resistivity measurements. Magnetic susceptibility and electrical resistivity data on Ce 1-x Nd x In 3 also reveal the antiferromagnetic ordering competition between CeIn 3 and NdIn 3 , where the T N of CeIn 3 is linearly suppressed to a critical concentration of x Nd ~0.6. This concentration is slightly lower than what was previously reported in nonmagnetically substituted Ce 1-x La x In 3 . Our magnetic susceptibility measurements and subsequent simulations show that in the CeIn 3 antiferromagnetic regime, x Nd ≤0.4, the Nd ions act as free paramagnets. The large magnitude of the associated paramagnetic response then masks the overlapping antiferromagnetic ordering signature of the Ce ions. Overall our study further sheds light on the underlying crystal electric field and Kondo lattice coherence interactions within the Ce m M n In 3m+2n family and could stimulate further studies of these systems via neutron diffraction or under applied pressure.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1981

Interacting vs. non-interacting single domain behavior in natural and synthetic samples

The disparity in response to high alternating field (AF) demagnetization for samples containing fine magnetic carriers is apparently related to the degree of interactions between those carriers. The presence of interaction fields between single domain (SD) grains can be tested by plotting isothermal remanence (IRM) acquisition vs. saturation remanence (SIRM) demagnetization. For the case of noninteracting SD grains, the two curves will be symmetrical. For the interacting SD case, the acquisition curve will be steepest at higher field, and the demagnetization curve steepest at lower fields, resulting in nonsymmetry. The point of intersection of the two curves approximates the remanent coercive force (H sub RC) field for all cases. Minor hysteresis loops and anhysteretic remanence (ARM) acquisition curves are also strongly influenced by interaction fields. Because of the difficulty in dispersing strongly magnetic grains, fine grained synthetic samples made with highly magnetic materials will not display equivalent AF stability to natural samples with fine, dispersed grains.

Cisowski, S.↗
DOE OSTI2018

Optical magnetism in planar metamaterial heterostructures

Harnessing artificial optical magnetism has previously required complex two- and three-dimensional structures, such as nanoparticle arrays and split-ring metamaterials. By contrast, planar structures, and in particular dielectric/metal multilayer metamaterials, have been generally considered non-magnetic. Although the hyperbolic and plasmonic properties of these systems have been extensively investigated, their assumed non-magnetic response limits their performance to transverse magnetic (TM) polarization. We propose and experimentally validate a mechanism for artificial magnetism in planar multilayer metamaterials. We also demonstrate that the magnetic properties of high-index dielectric/metal hyperbolic metamaterials can be anisotropic, leading to magnetic hyperbolic dispersion in certain frequency regimes. We show that such systems can support transverse electric polarized interface-bound waves, analogous to their TM counterparts, surface plasmon polaritons. Here, our results open a route for tailoring optical artificial magnetism in lithography-free layered systems and enable us to generalize the plasmonic and hyperbolic properties to encompass both linear polarizations.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2026

Collapse of Jahn-Teller phonons in La 1−x Sr x MnO 3 with weak magnetoresistance

Perovskite manganites are quantum materials exhibiting competing interactions inducing colossal magnetoresistance (CMR). The prevailing theory of CMR highlights the essential role of electron-phonon coupling (EPC), but mounting evidence suggests the underlying mechanism is more complicated. Here, we investigate phonons and spin-phonon coupling in ferromagnetic CMR manganites La 1−x Sr x MnO 3 (x=0.2,0.3) with relatively small CMR associated with melting of the magnetic order above room temperature. High-resolution neutron scattering experiments combined with density functional theory (DFT) show that the low-temperature ferromagnetic phase is conventional: neutron scattering from phonons agrees with DFT predictions and magnons follow sinusoidal dispersions. Fluctuating magnetic moments and low-energy phonons remain conventional in the high-temperature paramagnetic phase, indicating the Mn and La/Sr sublattices are not strongly perturbed by melting of ferromagnetism. In contrast, the Jahn–Teller-active optical oxygen vibrations collapse entirely above the Curie temperature, despite low CMR in these compositions, with some of the lost spectral weight reappearing as quasielastic scattering. We attribute this highly anomalous behavior to giant EPC in the charge and/or orbital channel. It drives cooperative diffusive motion of quasistatic carrier-trapping oxygen sublattice distortions once ferromagnetism disappears. We hypothesize the magnitude of magnetoresistance correlates with the rate of diffusion rather than with the strength of Jahn–Teller EPC.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Competing incommensurate spin fluctuations and magnetic excitations in infinite-layer nickelate superconductors

The recently discovered infinite-layer nickelates show great promise in helping to disentangle the various cooperative mechanisms responsible for high-temperature superconductivity. However, lack of antiferromagnetic order in the pristine nickelates presents a challenge for connecting the physics of the cuprates and nickelates. Here, by using a quantum many-body Green’s function-based approach to treat the electronic and magnetic structures, we unveil the presence of many two- and three-dimensional magnetic stripe instabilities that are shown to persist across the phase diagram of LaNiO 2 . Our analysis indicates that the magnetic properties of the infinite-layer nickelates are closer to those of the doped cuprates, which host a stripe ground state, rather than the undoped cuprates. The computed longitudinal-spin, transverse-spin, and charge spectra of LaNiO 2 are found to contain an admixture of contributions from localized and itinerant carriers. Theoretically obtained dispersion of magnetic excitations (spin-flip) is found to be in good accord with the results of recent resonant inelastic X-ray scattering experiments. Our study gives insight into the origin of strong magnetic competition in the infinite-layer nickelates and their relationship with the cuprates.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Magneto-optical Evidence of the Tilting Effect in Coupled Weyl Bands

Theories have revealed the universality of the band tilting effect in topological Weyl semimetals (WSMs) and its implications for the material physical properties. However, the experimental identification of tilted Weyl bands remains less explored. Here, we report the magneto-optical evidence of the tilting effect in WSM niobium phosphide. Specifically, we observe Landau level transitions with rich features that are well reproduced within a model of coupled tilted Weyl points. Our analysis indicates that the tilting effect relaxes the selection rules and leads to transitions that would otherwise be forbidden in the non-tilt case. Additionally, we observe unconventional interband transitions with flat and negative magnetic field dispersions, highlighting the importance of coupling between Weyl points. Our results not only emphasize the significance of the tilting effect in the optical responses of WSMs but also demonstrate magneto-optics as an effective tool for probing the tilting effect in electronic band structures.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
NASA NTRS1984

On the topological stability of magnetostatic equilibria

The topological stability of MHD equilibria is investigated by exploring the formal analogy, in the ideal MHD limit, between the topology of magnetic lines of force in coordinate space and the topology of integral surfaces of one- and two-dimensional Hamiltonian systems in phase space. It is demonstrated that in an astrophysical setting, symmetric magnetostatic equilibria satisfying the ideal MHD equations are exceptional. The principal result of the study is that previous infinitesimal perturbation theory calculations can be generalized to include finite-amplitude and symmetry-breaking effects. The effect of the ergodicity of perturbed symmetric equilibria on heat dispersal in magnetically dominated plasmas is discussed.

Tsinganos, K. C.↗
DOE OSTI2025

Understanding the Electronic Behavior of f-Element Intermetallics

Due to their partially filled f-orbitals, lanthanide and actinide intermetallic materials exhibit intriguing electronic, structural, and magnetic properties. These materials provide a unique platform to explore exotic magnetic and quantum phenomena that arise from their strongly correlated f-electrons, offering insights into f-electron behavior. Incorporating light elements such as boron and carbon can significantly impact the electronic, chemical, and physical properties of these materials, with varying influence between lanthanides and actinides due to the more localized f-electrons in lanthanides. In this work, lanthanide-based intermetallic single crystals containing light atoms were synthesized using the molten metal flux growth method. In this method, one or more low-melting metals such as aluminum, gallium, tin, and bismuth are used in excess as the reaction medium. This solution-state approach allows for lower reaction temperatures compared to solid-state reactions and enables the isolation of kinetic products rather than thermodynamically stable compounds. The synthesized crystals were analyzed using an extensive array of analytical and computational characterization techniques, including single crystal X-ray diffraction, scanning electron microscopy, energy-dispersive spectroscopy, magnetization measurements, and density functional theory calculations. These analyses provided detailed insights into the structural and magnetic properties of the synthesized materials.

37 - INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL C↗
DOE OSTI2024

Structural and Morphological Characteristics of Rare Earth Element-based MAX Phase and MXene

There has been a tremendous effort for the synthesis of crystalline MAX phases—a family of transition metal carbides and nitrides with a chemical formula of Mn+1AXn, where M is an early transition metal, A belongs to groups XIII – XVI in the periodic table, X is either C or N, and n can be in between 1 and 3. Furthermore, these materials have shown thermal and electrical conductance and have low density and high stiffness which open broad aspects of practical applications. Recently double transition metal MAX phases (M’ 2/3 M’’ 1/3 ) 2 AX - out-of-plane ordered, labeled as o-MAX and in-plane ordered, labeled as i-MAX, were reported. However, there are few reports on the synthesis and characterization of i-MAX and the corresponding MXenes. In this work, we synthesized Molybdenum-based rare earth containing i-MAX phase using arc melt technique. We then removed “A” element of i-MAX phase by acid treatment and sonication which resulted in two-dimensional (2D) transition metal carbides called MXenes. These MXenes offer high conductivity, hydrophilicity, magnetism, good dispersion ability in solvents, mechanical stability, and structural diversity with at least 100 stoichiometric MXene compositions and are recognized as multifunctional materials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2018

Thermal profile shaping and loss impacts of strain annealing on magnetic ribbon cores

We report the use of the advanced manufacturing technique of strain annealing for nanocomposite magnetic ribbons enables control of relative permeabilities and spatially dependent permeability profiles. Tuned permeability profiles enable enhanced control of the magnetic flux throughout magnetic cores, including the concentration or dispersion of the magnetic flux over specific regions. Due to the correlation between local core losses and temperature rises with the local magnetic flux, these profiles can be tuned at the component level for improved losses and reduced steady-state temperatures. We present analytical models for a number of assumed permeability profiles. This work shows significant reductions in the peak temperature rise with overall core losses impacted to a lesser extent. Controlled strain annealing profiles can also adjust the location of hotspots within a component for optimal cooling schemes. Finally, as a result, magnetic designs can have improved performance for a range of potential operating conditions.

36 MATERIALS SCIENCE↗