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Aerosol extensive and intensive properties vary throughout the world and remain one of the largest uncertainties in determining future climate both because of difficulties in their measurement and their modelled behaviors. Here we highlight the contributions of airborne sampling by the sunphotometer 4STAR (Spectrometers for Sky-Scanning Sun Tracking Atmospheric Research) from two different parts of the world; Korean peninsula and region during the KORUS-AQ experiment (KORean-US Air Quality in May-June 2016) and over the South East Atlantic during ORACLES (ObseRvations of CLouds above Aerosols and their intEractionS in August-September-October 2016, 2017, and 2018) field campaign. The high temporal and spatial resolution, afforded by airborne sampling during KORUS-AQ, are used to determine the variability of aerosol intensive and extensive properties, which is a metric than can be compared in between multiple different observations and models, even over varying surfaces and spanning multiple different aerosol emission sources. We show the consistency over spatial scales of the AOD (Aerosol Optical Depth), and the aerosol intensive properties (Angstrom exponent - AE, fine mode fraction - FMF) observed by 4STAR, GOCI (Geostationary Ocean Color Imager Yonsei aerosol retrieval v2), MERRA-2 reanalysis (Modern-Era Retrospective Analysis for Research and Applications, v2), and from airborne in situ aerosol optical measurements by LARGE (NASA Langley Aerosol Research Group Experiment). The majority of AODs due to fine mode aerosol is observed at altitudes lower than 2 km and is dependent on the prevailing meteorological conditions. AE and FMF are found to be more spatially variable than AOD during all of KORUS-AQ, even when accounting for potential sampling biases. This may indicate that microphysical processes like aerosol particle formation, growth, and coagulation impact the dominant aerosol size at shorter scales than their combined effect on the aerosol optical depth by the aerosol emission, transport, and removal. Averaging between measurements and model, the distance at which the correlation to itself is reduced by 15% is 65 km for AOD, and 22.7 km for AE. Vertically resolved measurement from an aircraft enable the direct measurements of aerosols overlying clouds. When aerosol overlie bright clouds, their radiative impact on the incident light can be either positive or negative. This difference in radiative impact promotes difficulties in remote sensing aerosol properties, which have shown biases in AOD retrievals when clouds are underneath. The AOD above clouds measured by 4STAR during ORACLES are used to build and improve upon the current Near-Real-Time MODACAERO algorithm for above cloud AOD from MODIS, into a continuity product for NASA EOS/SNPP/JPSS.