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NASA NTRS1995

Data Validation for Earth Probe-Total Ozone Mapping Spectrometer

This presentation represents the final report for the NASA grant project. The goal of this project was to provide scientific analysis to aid in validation fo data sets used in detection of long term global trends of total ozone. Ozone data from the Earth Probe Total Ozone Mapping Spectrometer instrument was compared for validation purposes with features in previous TOMS data. Atmospheric dynamic concepts were used in the analysis. The publications sponsored by the grant are listed along with abstracts.

Stanford, John L.↗
NASA NTRS1993

Ozone depletion at northern and southern latitudes derived from January 1979 to December 1991 Total Ozone Mapping Spectrometer data

An extended version of the Nimbus 7/TOMS ozone data set from the period January 1, 1979 to December 31, 1991 is presented. It is shown that the ozone-trend data indicate that regions of enhanced ozone depletion rates have formed at middle and high latitudes during recent years. The seasonal dependence and geographical extent of the enhanced ozone-depletion rates for the Northern and Southern hemispheres are examined. The variability of the long-term ozone trend determination is discussed via consideration of the differences among 11-, 12-, and 13-yr trend calculations. The effects of the Mount Pinatubo eruption and other volcanic eruptions on the TOMS equatorial zonal average ozone measurements, and its influence on long-term trend determinations are discussed. On the basis of a determination of the aerosol phase function using TOMS data, the effect of stratospheric aerosols on determination of ozone amounts from TOMS are shown to be less than 1 percent.

Herman, J. R.↗
NASA NTRS2000

Total Ozone Mapping Spectrometer (TOMS) Level-3 Data Products User's Guide

Data from the TOMS series of instruments span the time period from November 1978, through the present with about a one and a-half year gap from January 1994 through July 1996. A set of four parameters derived from the TOMS measurements have been archived in the form of daily global maps or Level-3 data products. These products are total column ozone, effective surface reflectivity, aerosol index, and erythermal ultraviolet estimated at the Earth surface. A common fixed grid of I degree latitude by 1.25 degree longitude cells over the entire globe is provided daily for each parameter. These data are archived at the Goddard Space Flight Center Distributed Active Archive Center (DAAQ in Hierarchical Data Format (HDF). They are also available in a character format through the TOMS web site at http://toms.gsfc.nasa.gov. The derivations of the parameters, the mapping algorithm, and the data formats are described. The trend uncertainty for individual TOMS instruments is about 1% decade, but additional uncertainty exists in the combined data record due to uncertainty in the relative calibrations of the various TOMS.

McPeters, Richard D.↗
NASA NTRS1997

Analysis, Repair, and Management of the Total Ozone Mapping Spectrometer Database

In the ensuing period we were able to demonstrate that the origin of these filamentous patterns resulted from the action of synoptic-scale vortical velocity field on the global-scale background gradient of ozone concentration in the meridional direction. Hyperbolic flow patterns between long-lived atmospheric vortices bring together air parcels from different latitudes, thus creating large gradients along the separatrices leaving the hyperbolic (stagnation) point. This result is further confirmed by the KL analysis of the ozone field in the equatorial region, where the background concentration gradient vanishes. The spectral slope in this region has been found to lie close to -1, in agreement with Batchelor's prediction. Another outcome of this result is that it at least provides indirect evidence about the kinetic energy spectrum of the atmospheric turbulence in the range of scales approximately 200 to 2000 km. Namely, Batchelor's analysis is based on the assumption that the velocity field is large-scale, that is the kinetic energy spectrum decays as O(k(sup -3)) or steeper. Since the scalar spectrum is confirmed, this also supports this form of the kinetic energy spectrum. The study of equatorial regions of TOMS data revealed the efficiency of the KL method is in detecting and separating a wave-like measurement artifact inherently present in the dataset due to the non-perfect correction for cross-track bias. Just two to three eigenfunctions represent the error, which makes it possible to enhance the data by reconstituting it from the data by eliminating the subspace of artifactual eigenfunctions. This represents a highly efficient means for achieving an improved rendering of the data. This has been implemented on the database. A wide range of techniques and algorithms have been developed for the repair and extension of the TOMS database.

Sirovich, Lawrence↗
NASA NTRS1987

Analysis and comparison of ozone maps obtained by TOMS and TOVS during the MAP/GLOBUS 1983 campaign

The Nimbus 7 TOMS (UV) and NOAA 7 and NOAA 8 TOVS (IR) data have been specially processed for the MAP/GLOBUS campaign (September 1983, over Europe). Comparison of the ozone results shows a general agreement but also some discrepancies due to clouds, emissivity of the surface, and latitude effects. The variability of the ozone field, closely linked to geopotential height field, may have induced a great change in total ozone along the balloon flights, but fortunately trajectories tend to lie parallel to the total ozone contours, so that the total ozone during each flight is nearly constant.

Muller, S.↗
NASA NTRS2014

Release 2 data products from the Ozone Mapping and Profiler Suite (OMPS) Limb Profiler

The OMPS Limb Profiler (LP) was launched on board the NASA Suomi National Polar-orbiting Partnership (SNPP) satellite in October 2011. OMPS-LP is a limb-scattering hyperspectral sensor that provides ozone profiling capability at 1.5 km vertical resolution from cloud top to 60 km altitude. The use of three parallel slits allows global coverage in approximately four days. We have recently completed a full reprocessing of all LP data products, designated as Release 2, that improves the accuracy and quality of these products. Level 1 gridded radiance (L1G) changes include intra-orbit and seasonal correction of variations in wavelength registration, revised static and intra-orbit tangent height adjustments, and simplified pixel selection from multiple images. Ozone profile retrieval changes include removal of the explicit aerosol correction, exclusion of channels contaminated by stratospheric OH emission, a revised instrument noise characterization, improved synthetic solar spectrum, improved pressure and temperature ancillary data, and a revised ozone climatology. Release 2 data products also include aerosol extinction coefficient profiles derived with the prelaunch retrieval algorithm. Our evaluation of OMPS LP Release 2 data quality is good. Zonal average ozone profile comparisons with Aura MLS data typically show good agreement, within 5-10% over the altitude range 20-50 km between 60 deg S and 60 deg N. The aerosol profiles agree well with concurrent satellite measurements such as CALIPSO and OSIRIS, and clearly detect exceptional events such as volcanic eruptions and the Chelyabinsk bolide in February 2013.

Limb scatter↗
NASA NTRS2004

Accuracy Assessments and Validation of an Expanded UV Irradiance Database from Satellite Total Ozone Mapping Spectrometer (TOMS)

The TOMS UV irradiance database (1978 to 2000) has been expanded to include 5 new products (noon irradiance at 305, 310, 324, and 380 nm, and noon erythemal-weighted irradiance), in addition to the existing erythemal daily exposure, which permit direct Comparisons with ground-based measurements from UV spectrometers. Sensitivity studies are conducted to estimate uncertainties of the new TOMS UV irradiance data due to algorithm apriori assumptions. Comparisons with Brewer spectrometers as well as filter radiometers are used to review of the sources of known errors. Inability to distinguish between snow and cloud cover using only TOMS data results in large errors in estimating surface UV using snow climatology. A correction is suggested for the case when the regional snow albedo is known from an independent source. The summer-time positive bias between TOMS UV estimations and Brewer measurements can be seen at all wavelengths. This suggests the difference is not related to ozone absorption effects. We emphasize that uncertainty of boundary layer UV aerosol absorption properties remains a major source of error in modeling UV irradiance in clear sky conditions. Neglecting aerosol absorption by the present TOMS algorithm results in a positive summertime bias in clear-sky UV estimations over many locations. Due to high aerosol variability the bias is strongly site dependent. Data from UV-shadow-band radiometer and well-calibrated CIMEL sun-sky radiometer are used to quantify the bias at NASA/GSFC site in Greenbelt, MD. Recommendations are given to enable potential users to better account for local conditions by combining standard TOMS UV data with ancillary ground measurements.

Krotkov, N. A.↗
NASA NTRS2012

Global Assimilation of EOS-Aura Data as a Means of Mapping Ozone Distribution in the Lower Stratosphere and Troposphere

Ozone in the lower stratosphere and the troposphere plays an important role in forcing the climate. However, the global ozone distribution in this region is not well known because of the sparse distribution of in-situ data and the poor sensitivity of satellite based observations to the lowermost of the atmosphere. The Ozone Monitoring Instrument (OMI) and Microwave Limb Sounder (MLS) instruments on EOS-Aura provide information on the total ozone column and the stratospheric ozone profile. This data has been assimilated into NASA s Global Earth Observing System, Version 5 (GEOS-5) data assimilation system (DAS). We will discuss the results of assimilating three years of OMI and MLS data into GEOS-5. This data was assimilated alongside meteorological observations from both conventional sources and satellite instruments. Previous studies have shown that combining observations from these instruments through the Trajectory Tropospheric Ozone Residual methodology (TTOR) or using data assimilation can yield useful, yet low biased, estimates of the tropospheric ozone budget. We show that the assimilated ozone fields in this updated version of GEOS-5 exhibit an excellent agreement with ozone sonde and High Resolution Dynamics Limb Sounder (HIRDLS) data in the lower stratosphere in terms of spatial and temporal variability as well as integrated ozone abundances. Good representation of small-scale vertical features follows from combining the MLS data with the assimilated meteorological fields. We then demonstrate how this information can be used to calculate the Stratosphere - Troposphere Exchange of ozone and its contribution to the tropospheric ozone column in GEOS-5. Evaluations of tropospheric ozone distributions from the assimilation will be made by comparisons with sonde and other in-situ observations.

Wargan, Krzysztof↗
NASA NTRS1999

Constructing Synoptic Maps of Stratospheric Column Ozone from HALOE, SAGE and Balloonsonde Data Using Potential Vorticity Isentropic Coordinate Transformations

In this study we utilize potential vorticity - isentropic (PVI) coordinate transformations as a means of combining ozone data from different sources to construct daily, synthetic three-dimensional ozone fields. This methodology has been used successfully to reconstruct ozone maps in particular regions from aircraft data over the period of the aircraft campaign. We expand this method to create high-resolution daily global maps of profile ozone data, particularly in the lower stratosphere, where high-resolution ozone data are sparse. Ozone climatologies in PVI-space are constructed from satellite-based SAGE II and UARS/HALOE data, both of which-use solar occultation techniques to make high vertical resolution ozone profile measurements, but with low spatial resolution. A climatology from ground-based balloonsonde data is also created. The climatologies are used to establish the relationship between ozone and dynamical variability, which is defined by the potential vorticity (in the form of equivalent latitude) and potential temperature fields. Once a PVI climatology has been created from data taken by one or more instruments, high-resolution daily profile ozone field estimates are constructed based solely on the PVI fields, which are available on a daily basis from NCEP analysis. These profile ozone maps could be used for a variety of applications, including use in conjunction with total ozone maps to create a daily tropospheric ozone product, as input to forecast models, or as a tool for validating independent ozone measurements when correlative data are not available. This technique is limited to regions where the ozone is a long-term tracer and the flow is adiabatic. We evaluate the internal consistency of the technique by transforming the ozone back to physical space and comparing to the original profiles. Biases in the long-term average of the differences are used to identify regions where the technique is consistently introducing errors. Initial results show the technique is useful in the lower stratosphere at most latitudes throughout the year,and in the winter hemisphere in the middle stratosphere. The results are problematic in the summer hemisphere middle stratosphere due to increased ozone photochemistry and weak PV gradients. Alternate techniques in these regions will be discussed. An additional limitation is the quality and resolution of the meteorological data.

Hollandsworth, Stacey M.↗
NASA NTRS2023

Using Regionalized Air Quality Model Performance and Bayesian Maximum Entropy Data Fusion to Map Global Surface Ozone Concentration and Associated Uncertainty

Estimates of ground-level ozone concentrations have been improved through data fusion of observations and atmospheric chemistry models. Our previous global ozone estimates for the Global Burden of Disease study corrected for bias uniformly across continents and then corrected near monitoring stations using the Bayesian Maximum Entropy (BME) framework for data fusion. Here, we use the Regionalized Air Quality Model Performance (RAMP) framework to correct model bias over a much larger spatial range than BME can, accounting for the spatial inhomogeneity of bias and nonlinearity as a function of modeled ozone. RAMP bias correction is applied to a composite of 9 global chemistry-climate models, based on the nearest set of monitors. These estimates are then fused with observations using BME, which matches observations at measurement stations, with the influence of observations declining with distance in space and time. We create global ozone maps for each year from 1990 to 2017 at fine spatial resolution. RAMP is shown to create unrealistic discontinuities due to the spatial clustering of ozone monitors, which we overcome by applying a weighting for RAMP based on the number of monitors nearby. Incorporating RAMP before BME has little effect on model performance near stations, but strongly increases R 2 by 0.15 at locations farther from stations, shown through a checkerboard cross-validation. Corrections to estimates differ based on location in space and time, confirming heterogeneity. We quantify the likelihood of exceeding selected ozone levels, finding that parts of the Middle East, India, and China are most likely to exceed 55 parts per billion (ppb) in 2017. About 96% of the global population was exposed to ozone levels above the World Health Organization guideline of 60 µg m −3 (30 ppb) in 2017. Our annual fine-resolution ozone estimates may be useful for several applications including epidemiology and assessments of impacts on health, agriculture, and ecosystems.

Ozone↗
NASA NTRS2000

Satellite Mapping of the Earth's Ozone and Sulfur Dioxide

The Total Ozone Mapping Spectrometer (TOMS) instruments are spatially-scanning UV spectrometers that have produced daily global images of total ozone over the last 21 years since the launch of the Nimbus 7 satellite. The instruments use a total ozone retrieval algorithm pioneered by J.V. Dave and C. L. Mateer for the Nimbus 4 Backscatter Ultraviolet (BUV) instrument, designed by D.F. Heath. The TOMS ozone maps have revealed the relations between total ozone and atmospheric dynamics, and shown the dramatic losses of ozone in the Antarctic ozone hole and the Northern hemisphere. The accepted long-term trends in global, regional, and local ozone are derived from data from the Nimbus 7 TOMS and three successive TOMS flights on Russian, Japanese, and American satellites. The next TOMS flight will be launched in 2000. The contiguous mapping design and fortuitous choice of TOMS wavelengths bands also permitted imaging of a second atmospheric gas, sulfur dioxide, which is transient due to its short lifetime. The importance of this measurement was first realized after the eruption of El Chichon volcano in 1982. The extreme range of sizes of volcanic eruptions and the 'associated danger require observations from a distant observing platform. The first quantitative time series of the input of sulfur dioxide by explosive volcanic eruptions into the atmosphere thus was developed from the TOMS missions. Finally, the Rayleigh and aerosol scattering spectral characteristic and reflectivity complete the four dominant pieces of information in the near UV albedo of the Earth. The four parameters are derived with a linear algorithm, the absorption coefficients of the gases, and effective paths computed from radiative transfer tables. Absorbing aerosol clouds (smoke, dust, volcanic ash) are readily identified by their deviation from a Rayleigh signature. The greatest shortcoming of the TOMS dataset is the 24 hour time resolution that is produced by the polar orbit of the satellite. Dynamic phenomena, such as upper air fronts that modulate total ozone and volcanic eruptions of sulfur dioxide and ash, cannot be adequately resolved. It is hoped that UV observations from geostationary satellites will soon be made to test the value of this unique information in weather forecasting and aviation safety.

Krueger, Arlin↗
NASA NTRS2000

Satellite Mapping of the Earth's Ozone and Sulfur Dioxide

The Total Ozone Mapping Spectrometer (TOMS) instruments are spatially-scanning UV spectrometers that have produced daily global images of total ozone over the last 21 years since the launch of the Nimbus 7 satellite. The instruments use a total ozone retrieval algorithm pioneered by J.V. Dave and C. L. Mateer for the Nimbus 4 Backscatter Ultraviolet (BUV) instrument, designed by D.F. Heath. The TOMS ozone maps have revealed the relations between total ozone and atmospheric dynamics, and shown the dramatic losses of ozone in the Antarctic ozone hole and the Northern hemisphere. The accepted long-term trends in global, regional, and local ozone are derived from data from the Nimbus 7 TOMS and three successive TOMS flights on Russian, Japanese, and American satellites. The next TOMS flight will be launched in 2000. The contiguous mapping design and fortuitous choice of TOMS wavelengths bands also permitted imaging of a second atmospheric gas, sulfur dioxide, which is transient due to its short lifetime. The importance of this measurement was first realized after the eruption of El Chichon volcano in 1982. The extreme range of sizes of volcanic eruptions and the associated danger require observations from a distant observing platform. The first quantitative time series of the input of sulfur dioxide by explosive volcanic eruptions into the atmosphere thus was developed from the TOMS missions. Finally, the Rayleigh and aerosol scattering spectral characteristic and reflectivity complete the four dominant pieces of information in the near UV albedo of the Earth. The four parameters are derived with a linear algorithm, the absorption coefficients of the gases, and effective paths computed from radiative transfer tables. Absorbing aerosol clouds (smoke, dust, volcanic ash) are readily identified by their deviation from a Rayleigh signature. The greatest shortcoming of the TOMS dataset is the 24 hour time resolution that is produced by the polar orbit of the satellite. Dynamic phenomena, such as upper air fronts that modulate total ozone and volcanic eruptions of sulfur dioxide and ash, cannot be adequately resolved. It is hoped that UV observations from geostationary satellites will soon be made to test the value of this unique information in weather forecasting and aviation safety.

Krueger, Arlin↗
NASA NTRS1988

Satellite maps of Antarctic total ozone

Satellite remote sensing techniques for ozone have made it possible to observe the detailed, daily horizontal structure of atmospheric ozone at all locations where sunlight is present. The Antarctic ozone 'hole' has been observed with the Total Ozone Mapping Spectrometer (TOMS) instrument since launch of Nimbus 7 in 1978. This feature is a continental-size ozone minimum found in the Antarctic winter and spring seasons which has generally deepened in recent years to levels in 1985 and 1987 far below the lowest values ever observed elsewhere. The minimum appears to be produced by atmospheric circulations, but the deepening almost certainly involves chemistry which is unique to cold, dark conditions.

Krueger, Arlin J.↗
NASA NTRS2014

Comparison of Spectral Radiance Calibration Techniques Used for Backscatter Ultraviolet Satellite Instruments

Methods for determining the absolute radiometric calibration sensitivities of backscatter ultraviolet (BUV) satellite instruments are compared as part of an effort to minimize pre-launch calibration errors. An internally illuminated integrating sphere source has been used for the Shuttle Solar BUV (SSBUV), Total Ozone Mapping Spectrometer (TOMS), Ozone Mapping Instrument (OMI), and Global Ozone Monitoring Experiment 2 (GOME-2) using standardized procedures traceable to national standards. These sphere-based sensitivities agree to within three percent [k equals 2] relative to calibrations performed using an external diffuser illuminated by standard irradiance sources, the customary radiance calibration method for BUV instruments. The uncertainty for these calibration techniques as implemented at the NASA Goddard Space Flight Centers Radiometric Calibration and Development Laboratory is shown to be 4 percent at 250nm [k equals 2] when using a single traceable calibration standard. Significant reduction in the uncertainty of nearly 1 percent is demonstrated when multiple calibration standards are used.

residual errors↗