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At least 55 records · Page 3

On the particle-size distribution function of cometary dust

The characterization of the particle size distribution in cometary tails is considered. The particle-size related distribution function of the acceleration exerted on the cometary particle by solar radiation pressure used by Finson and Probstein (1968) is introduced, and distribution functions observed for the comets Arend-Roland 1957 III, Bennett 1970 II and Seki-Lines 1962 III are illustrated. It is pointed out that although the distribution functions have features in common, the rate of decrease of the distribution towards zero acceleration (large particles) is not well determined. An approximation for the size distribution in this range obtained from a photometric study of anomalous cometary tails is presented, and used to formulate an a priori distribution law which can be used to approximate all types of expected distributions by varying three key parameters.

Sekanina, Z.↗

Online submicron particle sizing by dynamic light scattering using autodilution

Efficient production of a wide range of commercial products based on submicron colloidal dispersions would benefit from instrumentation for online particle sizing, permitting real time monitoring and control of the particle size distribution. Recent advances in the technology of dynamic light scattering (DLS), especially improvements in algorithms for inversion of the intensity autocorrelation function, have made it ideally suited to the measurement of simple particle size distributions in the difficult submicron region. Crucial to the success of an online DSL based instrument is a simple mechanism for automatically sampling and diluting the starting concentrated sample suspension, yielding a final concentration which is optimal for the light scattering measurement. A proprietary method and apparatus was developed for performing this function, designed to be used with a DLS based particle sizing instrument. A PC/AT computer is used as a smart controller for the valves in the sampler diluter, as well as an input-output communicator, video display and data storage device. Quantitative results are presented for a latex suspension and an oil-in-water emulsion.

Nicoli, David F.↗

Radio occultation of Jupiter's ring - Bounds on optical depth and particle size and a comparison with infrared and optical results

A comparison of Voyager 1 data of the Jovian ring at radio, infrared and optical wavelengths suggests a population density that either falls more rapidly than the inverse square of the linear size, or is sharply bounded in maximum particle size. A fragmentation power law is used to estimate a minimum particle radius of 1-2 microns, and a specific model is developed which consists of a power law distribution of lossless or slightly absorbent Mie scatterers with a refractive index near 1.62, a power law index of -3.5, and a minimum particle size of 1.5 microns. The maximum particle radius is not critical, provided that it is greater than 4 microns, and the power law polydispersion of lossless or low absorbent Mie scatterers is consistent with previously reported observations as long as the parameter size minimum is 20 and the power index is about -3.5.

Tyler, G. L.↗

Comparison of Ice Cloud Particle Sizes Retrieved From Satellite Data Derived From In Situ Measurements

Cloud microphysical parameterizations have attracted a great deal of attention in recent years due to their effect on cloud radiative properties and cloud-related hydrological processes in large-scale models. The parameterization of cirrus particle size has been demonstrated as an indispensable component in the climate feedback analysis. Therefore, global-scale, long-term observations of cirrus particle sizes are required both as a basis of and as a validation of parameterizations for climate models. While there is a global scale, long-term survey of water cloud droplet sizes (Han et al. 1994), there is no comparable study for cirrus ice crystals. In this paper a near-global survey of cirrus ice crystal sizes is conducted using ISCCP satellite data analysis. The retrieval scheme uses phase functions based upon hexagonal crystals calculated by a ray tracing technique. The results show that global mean values of D(e) are about 60 micro-m. This study also investigates the possible reasons for the significant difference between satellite retrieved effective radii (approx. 60 micro-m) and aircraft measured particle sizes (approx. 200 micro-m) during the FIRE I IFO experiment. They are (1) vertical inhomogeneity of cirrus particle sizes; (2) lower limit of the instrument used in aircraft measurements; (3) different definitions of effective particle sizes; and (4) possible inappropriate phase functions used in satellite retrieval.

Han, Qingyuan↗

Effect of particle size on the chemisorption and decomposition of carbon monoxide by palladium and nickel clusters

The chemisorption of gases on well-defined, supported metal particles is a model for basic processes in heterogeneous catalysis. In this study, the chemisorption and decomposition of carbon monoxide on palladium and nickel particles was examined as a function of particle size. Particulate films with average particle sizes ranging from 1 to 10 nm were grown by vapor deposition on UHV-cleaved mica. Successive CO adsorption-desorption cycles resulted in the accumulation of carbon on the particles, which suppressed CO adsorption. The rate of carbon accumulation was strongly dependent on particle size and was higher for Ni than for Pd over the same size range. Carbon was removed from both metals by oxygen treatments at elevated temperatures. However, a mixture of CO and O2 was effective for monitoring the removal of carbon from palladium.

Doering, D. L.↗

Particle sizes in Comet Bennett /1970 II/

The particle size distribution in the coma and tail of Comet Bennett has been determined by several methods, each sensitive to a particular size range. It is confirmed that a minimum value of the particle density, size, and radiation pressure efficiency function exists at about .00003 to .00010 g/sq cm. The existence of such a cutoff is probably due to the decreasing radiation pressure efficiency for particles smaller than the wavelength of the light being scattered. An exact determination of this cutoff may allow identification of the particle type.

O'Dell, C. R.↗

Process for preparation of large-particle-size monodisperse latexes

Monodisperse latexes having a particle size in the range of 2 to 40 microns are prepared by seeded emulsion polymerization in microgravity. A reaction mixture containing smaller monodisperse latex seed particles, predetermined amounts of monomer, emulsifier, initiator, inhibitor and water is placed in a microgravity environment, and polymerization is initiated by heating. The reaction is allowed to continue until the seed particles grow to a predetermined size, and the resulting enlarged particles are then recovered. A plurality of particle-growing steps can be used to reach larger sizes within the stated range, with enlarge particles from the previous steps being used as seed particles for the succeeding steps. Microgravity enables preparation of particles in the stated size range by avoiding gravity related problems of creaming and settling, and flocculation induced by mechanical shear that have precluded their preparation in a normal gravity environment.

Vanderhoff, J. W.↗

Middle East Health and Air Quality Utilizing NASA EOS in the Saharan and Arabian Deserts to Examine Dust Particle Size and Mineralogy of Aerosols

Ground-based studies conducted in Iraq have revealed the presence of potential human pathogens in airborne dust. According to the Environmental Protection Agency (EPA), airborne particulate matter below 2.5micron (PM2.5) can cause long-term damage to the human respiratory system. NASA fs Earth Observing System (EOS) can be used to determine spectral characteristics of dust particles and dust particle sizes. Comparing dust particle size from the Sahara and Arabian Deserts gives insight into the composition and atmospheric transport characteristics of dust from each desert. With the use of NASA SeaWiFS DeepBlue Aerosol, dust particle sizes were estimated using Angstrom Exponent. Brightness Temperature Difference (BTD) equation was used to determine the area of the dust storm. The Moderate-resolution Imaging Spectroradiometer (MODIS) on Terra satellite was utilized in calculating BTD. Mineral composition of a dust storm that occurred 17 April 2008 near Baghdad was determined using imaging spectrometer data from the JPL Spectral Library and EO-1 Hyperion data. Mineralogy of this dust storm was subsequently compared to that of a dust storm that occurred over the Bodele Depression in the Sahara Desert on 7 June 2003.

Keeton, Tiffany↗

Development of a simplified optical technique for the simultaneous measurement of particle size distribution and velocity

Existing techniques were surveyed, an experimental procedure was developed, a laboratory test model was fabricated, limited data were recovered for proof of principle, and the relationship between particle size distribution and amplitude measurements was illustrated in an effort to develop a low cost, simplified optical technique for measuring particle size distributions and velocities in fluidized bed combustors and gasifiers. A He-Ne laser illuminated Rochi Rulings (range 10 to 500 lines per inch). Various samples of known particle size distributions were passed through the fringe pattern produced by the rulings. A photomultiplier tube converted light from the fringe volume to an electrical signal which was recorded using an oscilloscope and camera. The signal amplitudes were correlated against the known particle size distributions. The correlation holds true for various samples.

Smith, J. L.↗

Quantifying Uncertainty in Particle Size Distribution Parameters Inferred from SAGE III/ISS Extinction Spectra

Stratospheric aerosols play key roles in the chemistry and radiation balance of the atmosphere and are a key input parameter for global chemistry and climate models. The degree to which aerosols impact chemistry and radiation balance depends primarily on their microphysical properties such as particle size distribution (PSD). The PSD is a mathematical description of the relative abundance of different sized particles within a sampling volume. If the PSD is accurately known then other key modeling parameters (e.g., surface area density) can be derived. Occultation observations from orbital instruments such as SAGE III/ISS have been used to infer these PSD parameters by inverting the extinction coefficient spectra. However, past efforts failed to address two key issues with this methodology: 1. The measurement uncertainty was not accounted for; 2. They assumed the PSDs to be single-mode only, while “real-world” PSDs are predominantly bi-modal. Accounting for both issues in the retrieval will yield an expanded solution space to the inferred PSD parameters; the question is “by how much?” To address this knowledge gap, we propose to carry out a series of simulations and, for every valid SAGE III/ISS data point, determine the range of PSD parameters that yield extinction spectra that are indistinguishable from the SAGE III/ISS data, within the limits of the reported uncertainty. Further, we will expand the solution space, for the first time, to include bimodal distributions. The results of this work will advance Earth system modeling/prediction capability through identifying the uncertainty of PSD parameter estimates using SAGE III/ISS data. The key benefits of this study over previous studies are twofold: 1. we will provide PSD estimates that include bimodal distributions in the solution space, 2. we will provide an uncertainty estimate for these parameters. The results of this study may be used directly in current and future climate and chemistry models.

SAGE III/ISS↗

Particle Size Measurements from the 2018 Honeywell Uncertified Research Engine Test in the NASA Propulsion Systems Laboratory

The particle size measurements from the Honeywell Uncertified Research Engine Icing Test in the NASA Propulsion Systems Laboratory conducted in 2018 are presented. This work focuses on describing the experimental arrangement, the processing and analysis methods, and final results for select cases acquired during ice crystal cloud conditions. The measurements presented will include data acquired by two High Speed Imaging instruments located both upstream and downstream of the fan, in the engine bypass section. Experimental results demonstrate the expected downward shift in the particle size distribution as the cloud passes through the engine fan and the ice particles break-up. This work also demonstrates the feasibility of acquiring particle size distributions in the environment of a running engine.

Engine icing↗

Satellite derived cirrus particle size - Tropical clouds

The present study extends the earlier work of Wielicki et al. (1990) to examine several cases of tropical cirrus clouds. Particle effective radius is estimated and compared to other studies of cirrus clouds. Particle size and phase are estimated by comparing reflectance observations by the Landsat satellite with theoretical calculations for a range of possible water and ice particle sizes. An examination of effective particle radius for six cases of tropical cirrus clouds over the eastern Pacific Ocean found typical radii of 60 microns. This value is similar to that derived for a case of midlatitude cirrus during the FIRE experiment in October 1986. Particle size is found to increase with decreasing cloud optical depth.

Wielicki, Bruce A.↗

Particle size distributions in polar mesospheric clouds derived from solar mesosphere explorer measurements

Data from the visible and UV spectrometers on the Solar Mesosphere Explorer are used to derive the color ratios of the reflectance at 265, 296, and 393 nm of light scattered from polar mesospheric cloud particles. This analysis extends the spectral coverage into the visible region of the spectrum. The data reduction technique compared the cloud brightness to the brightness scattered from the background atmosphere at the same wavelength. The ratios determined in this way are independent of systematic errors in instrument radiometric calibration. The data are analyzed using theoretical determinations of the color ratios from the Mie theory of small particle scattering, assuming a lognormal distribution for the particle size dispersion. Here 'size' means the average radius of the sphere having the same ice volume. The present results confirm earlier findings that the effective sizes of polar mesospheric cloud particles are less than 70 nm. Still, there exists a small number of measurements which result in particle sizes of the order of 80 nm. Even for these large particle sizes the required vertical column content of water vapor does not exceed limits imposed by the available atmospheric water vapor concentrations.

Rusch, D. W.↗

Fluids and their Effect on Measurements on Lunar Soil Particle size Distribution

From the late 1960s until now, lunar soil particle size distributions have typically been determined by sieving sometimes dry, and at other times with fluids such as water or Freon. Laser diffraction instruments allow rapid assessment of particle size distribution, and eventually may replace sieve measurements. However, when measuring lunar soils with laser diffraction instruments, care must be taken in choosing a carrier fluid that is compatible with lunar material. Distilled water is the fluid of choice for laser diffraction measurements of substances when there is no concern about adverse effects of water on the material being measured. When we began our analyses of lunar soils using laser diffraction, our first measurements were made with distilled water. Although the medians that we measured were comparable to earlier sieve data, the means tended to be significantly larger than expected. The effect of water vapor on lunar soil has been studied extensively. The particles interact strongly with water vapor, and subsequent adsorptions of nitrogen showed that the specific surface area increased as much as threefold after exposure to moisture. It was observed that significant porosity had been generated by this exposure to water vapor. The possibility of other physical changes in the surfaces of the grains was not studied.

Cooper, B. L.↗

Martian particle size based on thermal inertia corrected for elevation-dependent atmospheric properties

Thermal inertia is commonly used to derive physical properties of the Martian surface. If the surface is composed of loosely consolidated grains, then the thermal conductivity derived from the inertia can theoretically be used to compute the particle size. However, one persistent difficulty associated with the interpretation of thermal inertia and the derivation of particle size from it has been the degree to which atmospheric properties affect both the radiation balance at the surface and the gas conductivity. These factors vary with atmospheric pressure so that derived thermal inertias and particle sizes are a function of elevation. By utilizing currently available thermal models and laboratory information, a fine component thermal inertia map was convolved with digital topography to produce particle size maps of the Martian surface corrected for these elevation-dependent effects. Such an approach is especially applicable for the highest elevations on Mars, where atmospheric back radiation and gas conductivity are low.

Bridges, N. T.↗

Saturn's rings - Particle size distributions for thin layer model

A model incorporating limited interaction between the incident energy and particles in the ring is considered which appears to be consistent with the multiple scattering process in Saturn's rings. The model allows for the small physical thickness of the rings and can be used to relate Voyager 1 observations of 3.6- and 13-cm wavelength microwave scatter from the rings to the ring particle size distribution function for particles with radii ranging from 0.001 to 20 m. This limited-scatter model yields solutions for particle size distribution functions for eight regions in the rings, which exhibit approximately inverse-cubic power-law behavior.

Zebker, H. A.↗

Coarsening Up: Expanding the Particle Size Distributions of Lunar Simulants to Encompass A Comprehensive Range of Regolith Granularity

Due to a paucity of lunar regolith samples, simulated granular materials (simulants) have been developed and deployed for a variety of engineering and research purposes in an attempt to meet the requirements for lunar exploration. Broadly speaking, these manufactured materials aim to replicate the compositional (i.e., mineralogy and chemistry) and physical (e.g., particle size distribution, particle shape) profiles of lunar soil samples collected during the Apollo missions. While creating a “near-perfect” lunar simulant is prohibitive due to the unique formative processes (i.e., meteorite impacts, solar wind implantation) and conditions (anhydrous, reducing environment and exposure to radiation on the surface over billions of years) encountered on the moon, certain granular properties of the regolith can be recreated with a high level of fidelity by leveraging contemporary technologies. A fundamental physical property and descriptor, grain size can be correlated between samples and replicated through processing; however, a holistic understanding of the particle size distribution of lunar regolith must be considered when creating analog materials. This study produces particle size distributions for Apollo 16 returned samples, incorporating the sieved out >1 cm coarse-grained fraction, in order to provide a more comprehensive characterization of surficial lunar regolith grain sizes for the development of highlands-type granular analog testing materials.

R. N. Kovtun↗