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Corrections for the geometric distortion of the tube detectors on SANS instruments at ORNL

Small-angle neutron scattering instruments at the Oak Ridge National Laboratory's High Flux Isotope Reactor were upgraded in area detectors from the large, single volume crossed-wire detectors originally installed to staggered arrays of linear position-sensitive detectors (LPSDs). The specific geometry of the LPSD array requires that approaches to data reduction traditionally employed be modified. Here, two methods for correcting the geometric distortion produced by the LPSD array are presented and compared. The first method applies a correction derived from a detector sensitivity measurement performed using the same configuration as the samples are measured. In the second method, a solid angle correction is derived that can be applied to data collected in any instrument configuration during the data reduction process in conjunction with a detector sensitivity measurement collected at a sufficiently long camera length where the geometric distortions are negligible. Furthermore, both methods produce consistent results and yield a maximum deviation of corrected data from isotropic scattering samples of less than 5% for scattering angles up to a maximum of 35°. The results are broadly applicable to any SANS instrument employing LPSD array detectors, which will be increasingly common as instruments having higher incident flux are constructed at various neutron scattering facilities around the world.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

SU-C-201-03: Coded Aperture Gamma-Ray Imaging Using Pixelated Semiconductor Detectors

Purpose: Improved localization of gamma-ray emissions from radiotracers is essential to the progress of nuclear medicine. Polaris is a portable, room-temperature operated gamma-ray imaging spectrometer composed of two 3×3 arrays of thick CdZnTe (CZT) detectors, which detect gammas between 30keV and 3MeV with energy resolution of <1% FWHM at 662keV. Compton imaging is used to map out source distributions in 4-pi space; however, is only effective above 300keV where Compton scatter is dominant. This work extends imaging to photoelectric energies (<300keV) using coded aperture imaging (CAI), which is essential for localization of Tc-99m (140keV). Methods: CAI, similar to the pinhole camera, relies on an attenuating mask, with open/closed elements, placed between the source and position-sensitive detectors. Partial attenuation of the source results in a “shadow” or count distribution that closely matches a portion of the mask pattern. Ideally, each source direction corresponds to a unique count distribution. Using backprojection reconstruction, the source direction is determined within the field of view. The knowledge of 3D position of interaction results in improved image quality. Results: Using a single array of detectors, a coded aperture mask, and multiple Co-57 (122keV) point sources, image reconstruction is performed in real-time, on an event-by-event basis, resulting in images with an angular resolution of ∼6 degrees. Although material nonuniformities contribute to image degradation, the superposition of images from individual detectors results in improved SNR. CAI was integrated with Compton imaging for a seamless transition between energy regimes. Conclusion: For the first time, CAI has been applied to thick, 3D position sensitive CZT detectors. Real-time, combined CAI and Compton imaging is performed using two 3×3 detector arrays, resulting in a source distribution in space. This system has been commercialized by H3D, Inc. and is being acquired for various applications worldwide, including proton therapy imaging R&D.

60 APPLIED LIFE SCIENCES↗

LumaCam: a novel class of position-sensitive event mode particle detectors using scintillator screens

A new type of position-sensitive detectors is gaining attention in the neutron community. They are scintillator based detectors that detect the scintillation light on an individual photon basis via an image intensifier and a fast image sensor. Their readout operates in event mode i.e. it produces information about individual neutron interactions, reconstructed from the sensor data, thus enabling to achieve superior spatial and temporal resolutions compared to regular detectors. Although the development of current detectors is focused on neutrons, the concept is also applicable to the detection of other particles such as high-energy photons. This document provides a description on how these detectors are built, how they operate, and what their characteristics are. An example of a detector implementation based on a Timepix3 chip is described to illustrate the detector concept. This includes a detailed description of the algorithm that reconstructs the neutron interactions from the sensor data, one of the core components that sets it apart from established scintillator-based imaging detectors. Energy-resolved epithermal neutron radiography was performed at the ISIS EMMA beamline with this detector, illustrating some of the fundamental differences in the data that can be produced with the new type of detector compared to more established types of scintillator based neutron detectors. The term LumaCam is proposed to refer to this new class of position-sensitive event-mode detectors.

47 OTHER INSTRUMENTATION↗

Performance of position-sensitive resistive silicon detectors in the Forward Array Using Silicon Technology (FAUST)

The silicon telescopes of the Forward Array Using Silicon Technology (FAUST) have been recently upgraded with silicon detectors which use resistive charge-splitting to measure the position of charged particles. This is in addition to the measurement of the total energy that these charged particles deposit in the detector. The upgrade results in increased angular resolution with a much smaller number of signals than silicon strip detectors with similar resolution. Here, a novel method of calibration has been used to demonstrate the efficacy of these position-sensitive detectors, and the detectors have been used in a commissioning experiment.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Experimental energy resolution of a paracentric hemispherical deflector analyzer for different entry positions and bias

A specially designed hemispherical deflector analyzer (HDA) with 5-element input lens having a movable entry position R{sub 0} suitable for electron energy analysis in atomic collisions was constructed and tested. The energy resolution of the HDA was experimentally determined for three different entry positions R{sub 0}= 84, 100, 112 mm as a function of the nominal entry potential V(R{sub 0}) under pre-retardation conditions. The resolution for the (conventional) entry at the mean radius R{sub 0}= 100 mm was found to be a factor of 1.6-2 times worse than the resolution for the two (paracentric) positions R{sub 0}= 84 and 112 mm at particular values of V(R{sub 0}). These results provide the first experimental verification and a proof of principle of the utility of such a paracentric HDA, while demonstrating its advantages over the conventional HDA: greater dispersion with reduced angular aberrations resulting in better energy resolution without the use of any additional fringing field correction electrodes. Supporting simulations of the entire lens plus HDA spectrometer are also provided and mostly found to be within 20%-30% of experimental values. The paracentric HDA is expected to provide a lower cost and/or more compact alternative to the conventional HDA particularly useful in modern applications utilizing a position sensitive detector.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Indigenous design and development of multiPSD array for time of flight neutron spectrometer

Time of Flight neutron Spectrometer for inelastic neutron scattering studies is being commissioned at Dhruva reactor. Neutron pulse tagging is carried out using the Fermi chopper. Scattered neutrons at maximum possible scattered solid angle are needed to be detected along with the time information at detector. Precise and efficient detection system is essential for measurement of spatial and temporal distribution. Detection area is optimized to cover an angle of 70° in horizontal direction and 23° in vertical direction. Position sensitive detectors (PSDs) are designed with judicial use of precious {sup 3}He gas and a few PSDs with BF{sub 3} gas as suitable alternative for {sup 3}He gas. An array of vertically arranged 1 m long, 50 PSDs, covers the arc length of 2.5 m and detection area 2.5 m{sup 2}. The design of the BF{sub 3} PSDs is supported by investigations on the gas purity, fill gas pressure, drift region, drift field and neutron absorption in cathode wall. Design details and performance of the PSDs are presented in the paper.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A high sensitivity fiber optic macro-bend based gas flow rate transducer for low flow rates: Theory, working principle, and static calibration

A novel fiber optic macro-bend based gas flowmeter for low flow rates is presented. Theoretical analysis of the sensor working principle, design, and static calibration were performed. The measuring system consists of: an optical fiber, a light emitting diode (LED), a Quadrant position sensitive Detector (QD), and an analog electronic circuit for signal processing. The fiber tip undergoes a deflection in the flow, acting like a cantilever. The consequent displacement of light spot center is monitored by the QD generating four unbalanced photocurrents which are function of fiber tip position. The analog electronic circuit processes the photocurrents providing voltage signal proportional to light spot position. A circular target was placed on the fiber in order to increase the sensing surface. Sensor, tested in the measurement range up to 10 l min{sup -1}, shows a discrimination threshold of 2 l min{sup -1}, extremely low fluid dynamic resistance (0.17 Pa min l{sup -1}), and high sensitivity, also at low flow rates (i.e., 33 mV min l{sup -1} up to 4 l min{sup -1} and 98 mV min l{sup -1} from 4 l min{sup -1} up to 10 l min{sup -1}). Experimental results agree with the theoretical predictions. The high sensitivity, along with the reduced dimension and negligible pressure drop, makes the proposed transducer suitable for medical applications in neonatal ventilation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Momentum-imaging apparatus for the study of dissociative electron attachment dynamics

An ion-momentum spectrometer is used to study the dissociative dynamics of electron attachment to molecules. A skimmed, supersonic gas jet is crossed with a pulsed beam of low-energy electrons, and the resulting negative ions are extracted toward a time- and position-sensitive detector. Calculations of the momentum in three dimensions may be used to determine the angular dependence of dissociative attachment as well as the energetics of the reaction.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

CAMEA—A novel multiplexing analyzer for neutron spectroscopy

The analyzer detector system continuous angle multiple energy analysis will be installed on the cold-neutron triple-axis spectrometer RITA-2 at SINQ, PSI. CAMEA is optimized for efficiency in the horizontal scattering plane enabling rapid and detailed mapping of excitations. As a novelty the design employs a series of several sequential upward scattering analyzer arcs. Each arc is set to a different, fixed, final energy and scatters neutrons towards position sensitive detectors. Thus, neutrons with different final energies are recorded simultaneously over a large angular range. In a single data-acquisition many entire constant-energy lines in the horizontal scattering plane are recorded for a quasi-continuous angular coverage of about 60°. With a large combined coverage in energy and momentum, this will result in a very efficient spectrometer, which will be particularly suited for parametric studies under extreme conditions with restrictive sample environments (high field magnets or pressure cells) and for small samples of novel materials. In this paper we outline the concept and the specifications of the instrument currently under construction.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A new development on measurement and control software of SANS BATAN spectrometer (SMARTer) in Serpong, Indonesia

In 2005, the main computer for data acquisition and control system of Small-angle Neutron Scattering (SANS) BATAN Spectrometer (SMARTer) was replaced since it halted to operate the spectrometer. According to this replacement, the new software for data acquisition and control system has been developed in-house. Visual Basic programming language is used in developing the software. In the last two years, many developments have been made both in the hardware and also the software to conduct the experiment is more effective and efficient. Lately, the previous motor controller card (ISA Card) was replaced with the programmable motor controller card (PCI Card) for driving one motor of position sensitive detector (PSD), eight motors of four collimators, and six motors of six pinhole discs. This new control system software makes all motors can be moved simultaneously, then it reduces significantly the consuming time of setting up the instrument before running the experiment. Along with that development, the new data acquisition software under MS Windows operating system is also developed to drive a beam stopper in X-Y directions as well as to read the equipment status such as position of the collimators and PSD, to acquire neutron counts on monitor and PSD detectors, and also to manage 12 samples position automatically. A timer object which is set in one second to read the equipment status via serial port of the computer (RS232C), and general purpose interface board (GPIB) for reading the total counts of each pixel of the PSD from histogram memory was used in this new software. The experiment result displayed in real time on the main window, and the data is saved in the special format for further data reduction and analysis. The new software has been implemented and performed for experiment using a preset count or preset time mode for absolute scattering intensity method.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Radiological Shielding Design for the Neutron Backscattering Spectrometer EMU

In this paper we present modelling and design of compact radiation shielding required for operation of the EMU instrument, located at Australia's OPAL nuclear reactor. The acceptance criteria for the shielding design were (i) safety - dose rate ≤ 3 μSv/h at external surfaces of the instrument's experimental area, (ii) floor load limit < 20 tons/m{sup 2}, (iii) low cost and (iv) for maintenance purposes 'easy access' to components of the instruments. The EMU instrument is a cold neutron backscattering spectrometer designed to measure inelastic neutron scattering. Its distinctive feature is that it has a tight elastic energy transfer resolution, of about 1 μeV. The instrument provides unique opportunities to study diffusion in complex materials, e.g. water molecules in confinement, polymers or biological molecules, particularly in the Asia-Oceania region. EMU is the first instrument located on the CG3 neutron beam line of the OPAL Neutron Guide Hall (NGH). A pre-existing evacuated neutron guide of dimensions 200 mm (height) x 50 mm (width) feeds into the shared EMU/KOOKABURRA pre-monochromator bunker shielding assembly, and its bottom cross section will be intercepted ∼200 mm further in air by the highly orientated pyrolytic graphite (HOPG) EMU pre-monochromator (take-off angles from 125.4 deg. to 148 deg.). The bunker shielding assembly for EMU also contains a beryllium filter and Focusing Guide Section D (FGD, 170 mm (height) x 50 mm (width)). To accommodate the range of take-off angles Pb cylindrical shielding blocks of radius 140 mm and 500 mm height have been designed. These blocks will be located at the section of the bunker where the neutron beam will exit towards the experimental area and they will reside on top of a hollow steel base (sides 10 mm thick), on which they move by sliding and are integrated with the tertiary shutter. The experimental area is enclosed by a concrete wall of 2.5 m height and 300 mm thickness, shared with the KOOKABURRA instrument, Gyprock Plasterboard panels with viewing windows, a wall from the Out-of-Pile Bunker and the CG3 shielding. The neutron beam enters the experimental area via the tertiary shutter, into the Focusing Guide Section C (FGC), which has an entrance guide cross-section of 158 mm (height) x 79 mm (width) and exit guide cross-section of 149 mm (height) x 85 mm (width) and is of length 816 mm. The vacuum chamber of FGC will be connected to the vacuum chamber of the Background Chopper (BC, disc of outer radius 350 mm). Focusing Guide Section B (FGB) is aligned with FGC and its vacuum shared with the BC vacuum. The FGB has an exit guide cross section of 50 mm (height) x 49 mm (width) and is of length 4046 mm, which will focus the neutron beam vertically and horizontally towards the Al window entrance (0.82 mm thickness, labelled N16) of the Scattering Tank assembly (constructed from 20 mm - 40 mm thickness stainless steel and will be under vacuum < 1 x 10{sup -3} mbar). Inside the Scattering Tank there is another section of Focusing Guide (FGA), with an exit guide cross-section of 30 mm (height) 30 mm (width) and of length 417 mm. The neutron beam exiting the FGA will be reflected by the HOPG crystal pieces of the Graphite Chopper (GC) towards the Backscattering Monochromator (BM). The reflected neutron beam will first pass through the other Al window (0.82 mm thickness, labelled N17) of the Scattering Tank and then enter into a flight tube (steel of 10 mm thickness). The BM is formed in an 1800 mm spherical radius array of Si crystal elements (0.87 mm thickness) and is oscillated by the linear motor Doppler Drive. The neutron beam will be reflected back at 180 deg. from, and focussed by the BM to reenter the Scattering Tank through the N17 Al window. It will then pass through the GC (HOPG crystals are rotated out of the way) and will reach the scattering sample of interest to the instrument end user. Also, inside the Scattering Tank there will be {sup 3}He linear position-sensitive detectors, and Analyser Arrays formed in an 1800 mm radius spherical arrays of Si crystal elements (0.87 mm thickness) glued on aluminium support frames (10 mm thickness) and span ∼160 deg. arc.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

An instrument combining an electrospray ionization source and a velocity-map imaging spectrometer for studying delayed electron emission of polyanions

An instrument combining an electrospray ionization source and a velocity-map imaging (VMI) spectrometer has been developed in order to study the delayed electron emission of molecular anions and especially of polyanions. It operates at a high repetition rate (kHz) in order to increase the acquisition speed. The VMI spectrometer has been upgraded for nanosecond time resolution by gating the voltages applied on the position-sensitive detector. Kinetic energy release distribution of thermionic emission (without any contribution from direct detachment) can be recorded for well-defined delays after the nanosecond laser excitation. The capability of the instrument is demonstrated by recording photodetachment spectra of the benchmark C{sub 60}{sup −} anion and C{sub 84}{sup 2−} dianion.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Development and characterization of a multiple-coincidence ion-momentum imaging spectrometer

The design and performance of a high-resolution momentum-imaging spectrometer for ions which is optimized for experiments using synchrotron radiation is presented. High collection efficiency is achieved by a focusing electrostatic lens; a long drift tube improves mass resolution and a position-sensitive detector enables measurement of the transverse momentum of ions. The optimisation of the lens for particle momentum measurement at the highest resolution is described. We discuss the overall performance of the spectrometer and present examples demonstrating the momentum resolution for both kinetics and for angular measurements in molecular fragmentation for carbon monoxide and fullerenes. Examples are presented that confirm that complete space-time focussing is possible for a two-field three-dimensional imaging spectrometer.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A fiber-coupled displacement measuring interferometer for determination of the posture of a reflective surface

A fiber-coupled displacement measuring interferometer capable of determining of the posture of a reflective surface of a measuring mirror is proposed. The newly constructed instrument combines fiber-coupled displacement and angular measurement technologies. The proposed interferometer has advantages of both the fiber-coupled and the spatially beam-separated interferometer. A portable dual-position sensitive detector (PSD)-based unit within this proposed interferometer measures the parallelism of the two source beams to guide the fiber-coupling adjustment. The portable dual PSD-based unit measures not only the pitch and yaw of the retro-reflector but also measures the posture of the reflective surface. The experimental results of displacement calibration show that the deviations between the proposed interferometer and a reference one, Agilent 5530, at two different common beam directions are both less than ±35 nm, thus verifying the effectiveness of the beam parallelism measurement. The experimental results of angular calibration show that deviations of pitch and yaw with the auto-collimator (as a reference) are less than ±2 arc sec, thus proving the proposed interferometer’s effectiveness for determination of the posture of a reflective surface.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Experimental study for subcriticality measurement of fuel debris in the Fukushima Daiichi reactor - 14582

Fuel debris defueling in the Fukushima Daiichi reactors is planned. Furthermore, retrieved fuel debris will be packed and stored in casks for a long time. In these processes, from the viewpoint of criticality safety, the subcriticality of the fuel debris should be confirmed. Although there are some subcriticality measurement methods, the applicability of these methods to the fuel debris must be investigated because the elemental composition and shape of the fuel debris are unknown. In this study, we focus on the exponential experiment method which is able to measure a wide range of subcriticality. Basic experiments to validate the methods were carried out using Toshiba Nuclear Critical Assembly (NCA) and {sup 3}He Position Sensitive Detector (PSD). The decay curves of neutron flux distributions were measured by the PSD detector and fitted to a theoretical formula. The elemental compositions and neutron spectrum of the fuel debris have been estimated with a severe accident code and a Monte Carlo code. In the experiment, the neutron spectrum of the fuel debris was simulated in the NCA core. The porosity of the fuel debris was assumed to be 60%, which corresponds to be H/U=7.5 and Volume Ratio=1.5. In order to evaluate the effect of the uncertainty of the compositions on the measured subcriticality, a homogeneous region and a heterogeneous region were configured in an experimental core. These regions consisted of fuel rods with different UO{sub 2} enrichment zone or different gadolinia concentration zone in the axial direction. The effective multiplication factors deduced by the exponential experiment method were a range of 0.94 to 0.98. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Determination of the solid angle and response function of a hemispherical spectrograph with injection lens for Auger electrons emitted from long lived projectile states

We present SIMION 8.1 Monte Carlo type simulations of the response function and detection solid angle for long lived Auger states (lifetime τ ∼ 10{sup −9} − 10{sup −5} s) recorded by a hemispherical spectrograph with injection lens and position sensitive detector used for high resolution Auger spectroscopy of ion beams. Also included in these simulations for the first time are kinematic effects particular to Auger emission from fast moving projectile ions such as line broadening and solid angle limitations allowing for a more accurate and realistic line shape modeling. Our results are found to be in excellent agreement with measured electron line shapes of both long lived 1s2s2p{sup 4}P and prompt Auger projectile states formed by electron capture in collisions of 25.3 MeV F{sup 7+} with H{sub 2} and 12.0 MeV C{sup 4+} with Ne recorded at 0{sup ∘} to the beam direction. These results are important for the accurate evaluation of the 1s2s2p {sup 4}P/{sup 2}P ratio of K-Auger cross sections whose observed non-statistical production by electron capture into He-like ions, recently a field of interesting interpretations, awaits further resolution.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Investigation of Energy Selective Neutron Imaging at the PULSTAR Reactor

Neutron imaging is complementary to X-ray imaging where both are used to investigate the internal features of objects nondestructively. Historically, it only began three years after discovery of the neutron in 1932, however, neutron radiographs with reasonable quality were first made in the mid-fifties. Conventionally, the image is produced by placing the object between the neutron source and a two-dimensional position sensitive detector. The source commonly has a full energy spectrum (white beam) of thermal or cold neutrons to obtain high intensity in the sample and short exposure time. As a result, all neutron energies contribute to the obtained radiograph. Since the interaction of the neutron with matter is energy dependent, different energies produce different contrast on the radiographic image, hence, additional information about the object can be obtained. Neutron imaging that utilizes a narrow spectrum of energy instead of white beam is called energy selective neutron imaging. Many techniques have been explored to select a narrow band of neutron energy for the use in imaging such as the use velocity selectors, double crystal Monochromators, and time of flight techniques (at pulsed neutron sources). The PULSTAR reactor of North Carolina State University (1 MWth) currently has an operational neutron powder diffractometer (NPD) installed on beam tube no. 4, which was designed for neutron scattering experiments and can provide a monoenergetic beam of neutrons. The neutron energy could be selected by diffraction means using a Si bent perfect crystal as a Monochromator. In this work, an investigation of energy selective neutron imaging at the NPD is discussed in terms of the system performance and the ability of material discrimination on a test sample by observing the contrast variations of the neutron radiographs obtained using different neutron energies. Energy selective neutron imaging experiment was successfully tested at the PULSTAR reactor's NPD. Although, the uniform region is small and the exposure time is long in comparison with the NIF, both facilities exhibit similar spatial resolution which is a very important characteristic for any imaging facility. The contrast variation of neuron radiographs for the test sample obtained at different energies indicated a potential advantage for using energy selective neutron imaging over the white beam. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Elimination of ghosting artifacts from wavelength-shifting fiber neutron detectors

Misassignment of neutron position (ghosting) produces artifacts, which have been observed in wavelength-shifting (WLS) fiber detectors developed for time-of-flight (TOF) neutron powder diffraction. In position-sensitive detectors (PSDs) with WLS fiber encoding, thermal and cold neutrons interact with a monolithic 6LiF/ZnS:Ag scintillator screen, and scintillation photons are generated and transported through the crossed fibers to photomultipliers (PMTs). The neutron position is determined by photon counts in PMTs within a preset time window. Ghosting occurs when neutrons hit the group boundaries of two neighboring PMTs for x-position multiplexing, which is modeled as resulting from a long travel length (about 3-5 mm) of a small number of scintillation photons. This model is supported by the change observed in aperture images when the threshold number for photon-pulses was adjusted for a neutron event determination. When the threshold number of photon-pulses was set above 10 for each PMT, the ghost peaks in the aperture images and TOF spectra of powder diffraction were strongly suppressed or completely eliminated, and the intrinsic background levels of the WLS detectors were significantly reduced. Our result indicates that WLS fiber detector is a promising alternative for 3He PSDs for neutron scattering.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗