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DOE OSTI2026

Coupling of TIGRESS and EMMA with Auxiliary Array TIP at TRIUMF

The combination of a germanium detector array and recoil mass spectrometer allows for high-sensitivity experiments in nuclear structure and astrophysics by enabling high-energy-resolution -ray spectroscopy and reaction measurements of weak fusion-evaporation, transfer or radiative-capture reactions in the presence of dominant background reaction channels. The TIGRESS -ray spectrometer with an upgraded data acquisition system has been coupled with the EMMA mass spectrometer alongside a suite of auxiliary detectors housed within TIGRESS such as TIP. This paper reviews the unique combination of radioactive beams at TRIUMF with the capabilities of TIGRESS and EMMA in the context of fusion-evaporation with TIP and radiative-capture reactions without an auxiliary array.

A/Q identification↗

DOE OSTI2025

Investigation of the excited states of 114 Sn using the GRIFFIN spectrometer at TRIUMF

The semi-magic 110-122 Sn isotopes display signs of shape coexistence in their excited 0 + states, which, in contrast to the spherical 0+ ground states, are deformed. Here, this paper investigates the nuclear structure of 114 Sn using the competing β + decay and electron capture of a radioactive beam of 114 Sb produced at the TRIUMF-ISAC facility using the GRIFFIN spectrometer. This study will allow for an in-depth understanding of the excited 0 + states in 114 Sn, by focusing on their decay patterns. In the present experiment, transitions at 856.2-keV and 1405.0-keV, which were observed in an earlier β + decay study but not placed in the 114 Sn level scheme, have been Physics, assigned to the level scheme in connection to the 0$^+_3$ level at 2156.0-keV. Properly assigning these transitions refines the level scheme and enhances our understanding of the nuclear structure in 114 Sn.

GRIFFIN↗

DOE OSTI2022

Single neutron transfer on 23 Ne and its relevance for the pathway of nucleosynthesis in astrophysical X-ray bursts

We present new experimental measurements of resonance strengths in the astrophysical 23 Al($p, γ$) 24 Si reaction, constraining the pathway of nucleosynthesis beyond 22 Mg in X-ray burster scenarios. Specifically, we have performed the first measurement of the ($d, p$) reaction using a radioactive beam of 23 Ne to explore levels in 24 Ne, the mirror analog of 24 Si. Four strong single-particle states were observed and corresponding neutron spectroscopic factors were extracted with a precision of ~20%. Using these spectroscopic factors, together with mirror state identifications, we have reduced uncertainties in the strength of the key ℓ = 0 resonance at $E_r$ = 157 keV, in the astrophysical 23 Al($p, γ$) reaction, by a factor of 4. Our results show that the 22 Mg($p, γ$) 23 Al($p, γ$) pathway dominates over the competing 22 Mg($α, γ$) reaction in all but the most energetic X-ray burster events (T > 0.85 GK), significantly affecting energy production and the preservation of hydrogen fuel.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

Abrupt structural transition in exotic molybdenum isotopes unveils an isospin-symmetric island of inversion

Like electrons in atoms, protons and neutrons in nuclei occupy orbitals in a shell structure with energy gaps at magic numbers. Radioactive-beam experiments revealed the disappearance of magic numbers in some neutron-rich isotopes. In these nuclei, configurations involving particles excited across the shell gap gain correlation energy, becoming the ground state. Neutron-rich regions of the nuclear chart that exhibit this property are known as “Islands of Inversion”. Here we present the lifetime measurement of the first 2 + states in 84 Mo (N = Z) and 86 Mo (N = Z + 2) revealing an unexpected sharp structural change between them defining the edge of the region of deformation around 80 Zr. Similarly to the neutron-rich N = 40 Island of Inversion near 64 Cr where cross-shell excitations dominate, we identify this region as an Island of Inversion with symmetrical proton and neutron excitations that we term “Isospin-Symmetric Island of Inversion”. Three-nucleon forces are suggested to drive Mo isotope structural changes.

experimental nuclear physics↗

DOE OSTI2023

Constraining Nucleosythesis in Neutrino-Driven Winds Using the Impact of ({alpha}, xn) Reaction Rates

The lighter heavy elements of the first r-process peak, between strontium and silver, can be synthesized in the moderately neutron-rich neutrino-driven ejecta of either core-collapse supernovae or neutron star mergers via the weak r-process. This nucleosynthesis scenario exhibits uncertainties from the absence of experimental data from (alpha, xn) reactions on neutron-rich nuclei, which are currently based on statistical model estimates. We have performed a new impact study to identify the most important (alpha, xn) reactions that can affect the production of the lighter heavy elements under different astrophysical conditions using new, constrained (alpha, xn) reaction rates based on the Atomki-V2 alpha OMP. Our results show how when reducing the nuclear physics uncertainties, we can use abundance ratios to constrain the astrophysical conditions/environment. This can be achieved in the near future, when the key (alpha, xn) reaction rates will be measured experimentally in radioactive beam facilities.

Psaltis, Athanasios↗

DOE OSTI2024

Investigating nuclei produced in 9 Li + 11 B reaction

In this contribution, a preliminary analysis of the first part of the experiment S2012 conducted at the ISAC-II facility of Canada’s particle accelerator center TRIUMF in Vancouver will be presented. The experiment aims to study highly clustered structures of nuclei created in multi-nucleon transfer reactions of 9 Li radioactive beam on natural boron target ( 11 B and 10 B). The main objective of the experiment is to study exotic structures created in neutron-rich 16 C nucleus in the range of higher excitation energies. The analysis presented here probes the existence of exotic cluster configurations and the quality of detected results using the invariant mass techniques.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2025

Tritium targets for use in solenoidal spectrometers

Nucleon adding and removing reactions are an ideal probe to study the single-particle foundations of nuclear structure. For experiments far away from the valley of stability, one needs to use radioactive beams in inverse kinematics. To maintain excellent resolution, solenoidal spectrometers like HELIOS at Argonne National Laboratory (ANL), ISS at CERN or SOLARIS at the Facility for Rare Isotope Beams (FRIB) are used. Typically, deuterated plastic foils are the targets of choice. Depending on the energy deposited, these targets might degrade quickly in beam. The potential of using tritium-implanted targets in conjunction with the solenoidal spectrometers was realized for access to even more exotic nuclei with outstanding resolving power. While no tritiated polyethylene is commercially available at the moment, tritium-containing titanium targets have been produced in the past. Unfortunately the loading fraction of tritium for the latter was often very low and not reproducible. The progress in the production of tritium-containing targets is presented, including the characterization of the foils.

Müller-Gatermann, Claus↗

DOE OSTI2021

Unnuclear physics: Conformal symmetry in nuclear reactions

Significance Symmetry plays a key role in modern physics as a guiding principle for fundamental theories of nature. We use the nonrelativistic conformal symmetry to predict universal energy spectra of final states in reactions of quantum particles at vastly different length scales. Our work extends Georgi’s “unparticle” proposal to nonrelativistic spin-1/2 fermions in the unitary regime of strong interactions. These systems form so-called unparticles, which behave characteristically different from normal particles. They can be engineered with ultracold atoms and occur naturally in nuclear reactions with multiple neutrons—a situation we dub “unnuclear physics.” We present the general scenario of unnuclear physics, apply it to identify unnuclei in nuclear reactions, and highlight the opportunity to measure unnuclei at radioactive beam facilities.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2025

First on-line commissioning experiments at the St. Benedict facility

Nuclear beta decays provide an excellent probe of fundamental symmetries due to their mediation by the weak interaction. In particular, precise measurements of these decays provide constraints on the unitarity of the Cabbibo-Kobayashi-Maskawa (CKM) quark-mixing matrix. While superallowed pure Fermi decays currently set the most precise limits, the alternative suite of superallowed mixed mirror decays has been ill-studied. These nuclei can provide an important consistency check of calculation and measurement methods employed for the pure Fermi decays, more critically needed now in the wake of a 2.4σ deviation from unitarity of the CKM matrix. In order to remedy the gap in data for mirror decays, the Superallowed Transition Beta-Neutrino Decay Ion Coincidence Trap (St. Benedict) facility is being commissioned at the University of Notre Dame’s Nuclear Science Laboratory (NSL). In this paper, we present first results of the commissioning of the St. Benedict facility on-line at the TwinSol radioactive beam facility. The results of initial commissioning experiments involving the St. Benedict gas catcher, RF carpet, RFQ ion guide and RFQ cooler-buncher will be presented.

beta decay↗

DOE OSTI2022

Measurement of the Mo 100 ( α , x n ) cross section at weak r -process energies

Here, the weak r process in neutrino-driven winds following a core-collapse supernova is thought to contribute to the cosmic abundances of the first r-process peak elements between Se and Ag. Sensitivity studies have found that the early nucleosynthesis in the weak r process is primarily driven by (α, xn) reactions due to the high temperatures, and that current nuclear physics uncertainties in the (α, xn) rates result in significant uncertainties of the calculated abundances. The weak r-process path proceeds several nuclei away from stability where (α, xn) reaction cross sections have not yet been measured. In this paper we report the 100 Mo (α, xn) cross section (between 8.9 and 13.2 MeV in the center of mass, corresponding to 3.5–6.8 GK) in inverse kinematics using the Multi-Sampling Ionization Chamber (MUSIC) detector at the Argonne Tandem Linac Accelerator System (ATLAS) facility. With this first measurement of the 100 Mo (α, xn) cross section, we have demonstrated the ability of MUSIC to measure (α, xn) cross sections for A up to 100, therefore paving the way for further measurements with radioactive beams at ATLAS or the Facility for Rare Isotope Beams.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2025

Elastic scattering in the 12 N + 197 Au system at 𝐸 lab = 70 MeV

Halo structure is an interesting exotic configuration developed in some light weakly bound nuclei, where a valence particle orbits a nuclear core. Signatures of halo structure can be observed in the angular distributions of the elastic scattering induced by these nuclei at energies around the Coulomb barrier. There are some well-studied reactions with neutron-rich halo nuclei, such as 6 He and 11 Li . However, the information is scarce on the proton-rich side. Recent works confirm the halo structure in the 8B nuclei but still lack more experimental studies for other proton-halo candidates, such as 12 N and 17 F. In this work, we report experimental data for the elastic scattering of 12 N on 197 Au target at 𝐸 lab = 70 MeV. The 12 N is a proton-rich nucleus with proton separation energy 𝑆 𝑝 = 600 keV, which is higher than the 8 B (𝑆 𝑝 = 137 keV) and almost the same as the 17 F (𝑆 𝑝 = 601 keV). Data were obtained at the Cyclotron Institute of Texas A&M University where the 12 N radioactive beam was produced by the momentum achromatic recoil spectrometer. The calculation of the optical model was used to fit the measured angular distribution for the elastic scattering and to obtain the reaction cross section 𝜎 𝑅 . We also performed continuum discretized coupled-channel calculations to compare with the experimental data. The angular distribution of the elastic cross sections exhibits a suppression of the Fresnel peak. From the fitting of the optical model, we obtain the total reaction cross section, 𝜎 𝑅 = 1269 ± 41 mb. The agreement between the CDCC calculation and the experimental elastic scattering data is limited and the breakdown does not exhaust the measured 𝜎 𝑅 . The resulting reduced reaction cross section 𝜎 Red for 12 N + 197 Au is large and comparable to the one obtained for the 8 B + 208 Pb system. This suggests a strong decoupling of the valence proton from the core because of the low binding energy and a dynamic polarization effect. Here, more research is required to estimate the contribution of core excitation.

Elastic scattering reactions↗

DOE OSTI2021

Quasi-free scattering in inverse kinematics as a tool to unveil the structure of nuclei: A tribute to Mahir S. Hussein

Abstract Quasi-free scattering of electrons and protons has been extensively utilized in the past to study the single-particle structure of nuclei, clustering in light nuclei, and short-range correlated nucleon–nucleon pairs in nuclei. Recently, this approach has been applied in inverse kinematics using hydrogen targets. The characteristic features of this reaction and the experimental challenges and advantages of inverse-kinematics experiments are summarized. The applicability to radioactive beams opens a large research potential to study a variety of properties of neutron-to-proton asymmetric nuclei. Applications of quasi-free scattering in inverse kinematics and its potential are reviewed based on recent and ongoing research programs at different accelerator facilities worldwide.

Physics↗

DOE OSTI2022

Improving Fission Products at CARIBU: Near Field Detection (Q2/FY22 Quarterly Progress Report)

We continued our work on preparation for the upcoming branching ratio measurements. The CARIBU facility has not been delivering radioactive beams since January this year due to an issue with the magnet that is used for mass separation. The parts needed to be replaced to fix the issue has been since ordered, shipped from Germany, and installed at CARIBU. The CARIBU is now operational and the first experiments that are ran will be those that had to be cancelled in January due to the facility complications, and we are in a position to schedule our next sample collection. In the meantime, we have been continuing work on data analysis of fission product mass measurements in the Canadian Penning Trap. This analysis is now complete. We continue our outreach to recruit a graduate student who would be interested in working with us on this project. In the past month, we have a conversation with a potential student at UC Berkeley and Texas A&M. There students are still to decide if they would accept the offer to these graduate schools.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2023

Cubical moderators for the Neutron Target Demonstator (NTD)

Neutron capture cross sections of unstable isotopes are important for neutron induced nucleosynthesis as well as for technological applications. The traditional time-of-flight method reaches its limits once the necessary detection of the reaction products is hampered by the size (mass) of the sample. Several factors may limit the sample mass: The decay properties of radioactive isotopes interfere with the signals from the neutron capture or neutron-induced fission reactions; The limited range of charged reaction products requires a thin sample. In both cases, an increased neutron fluence at the sample position with ever improved neutron sources overcomes the lack of reaction rate. Reference proposed a combination of a radioactive beam facility, an ion storage ring and a spallation neutron source surrounded by neutron moderator. This idea is part of the LANSCE strategy to stay a worldwide leader for neutron induced research. Figure 1 shows a sketch of the proposed future setup.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2023

The St. Benedict Facility: Probing Fundamental Symmetries through Mixed Mirror $β$-Decays

Precise measurements of nuclear beta decays provide a unique insight into the Standard Model due to their connection to the electroweak interaction. These decays help constrain the unitarity or non-unitarity of the Cabibbo–Kobayashi–Maskawa (CKM) quark mixing matrix, and can uniquely probe the existence of exotic scalar or tensor currents. Of these decays, superallowed mixed mirror transitions have been the least well-studied, in part due to the absence of data on their Fermi to Gamow-Teller mixing ratios ($ρ$). At the Nuclear Science Laboratory (NSL) at the University of Notre Dame, the Superallowed Transition Beta-Neutrino Decay Ion Coincidence Trap (St. Benedict) is being constructed to determine the ρ for various mirror decays via a measurement of the beta–neutrino angular correlation parameter ($α_{βν}$) to a relative precision of 0.5%. In this work, we present an overview of the St. Benedict facility and the impact it will have on various Beyond the Standard Model studies, including an expanded sensitivity study of $ρ$ for various mirror nuclei accessible to the facility. A feasibility evaluation is also presented that indicates the measurement goals for many mirror nuclei, which are currently attainable in a week of radioactive beam delivery at the NSL.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2025

Low-metallicity Nova Explosions: A Site for Weak rp -process Nucleosynthesis

Classical novae are common cataclysmic events involving a binary system of a white dwarf and a main-sequence or red giant companion star. In metal-poor environments, these explosions produce ejecta differently from their solar counterparts due to the accretion of subsolar-metallicity material onto the white dwarf. In particular, it has been suggested that the nucleosynthesis flow in such low-metallicity nova explosions extends up to the Cu–Zn region, much beyond the expected endpoint, around Ca, predicted for solar-metallicity classical novae. This behavior resembles a weak rp-process, and such nuclear activity has never been observed in accreting white dwarf binaries with typical accretion flows. In this work, we study the characteristics of the weak rp-process for four nova models with metallicities Z = 2 × 10 −9 , 10 −7 , 2 × 10 −6 , and 2 × 10 −5 , and explore the impact of the nuclear physics uncertainties via a Monte Carlo sensitivity study. We identify nuclear reactions whose uncertainties affect the production of intermediate-mass nuclei under these conditions. These reactions and relevant nuclear quantities are targets for measurements at stable or radioactive beam facilities to reduce their rate uncertainties.

Classical novae↗

DOE OSTI2020

Two-neutron knockout as a probe of the composition of states in Mg 22 , Al 23 , and Si 24

Simpson and Tostevin proposed that the width and shape of exclusive parallel momentum distributions of the A - 2 residue in direct two-nucleon knockout reactions carry a measurable sensitivity to the nucleon single-particle configurations and their couplings within the wave functions of exotic nuclei. We further report here on the first benchmarks and use of this new spectroscopic tool. Exclusive parallel momentum distributions for states in the neutron-deficient nuclei Mg 22 , Al 23 , and Si 24 populated in such direct two-neutron removal reactions were extracted and compared to predictions combining eikonal reaction theory and shell-model calculations. For the well-known Mg 22 and Al 23 nuclei, measurements and calculations were found to agree, supporting the dependence of the parallel momentum distribution width on the angular momentum composition of the shell-model two-neutron amplitudes. In Si 24 , a level at 3439(9) keV, of relevance for the important Al 23 ( p , γ ) Si 24 astrophysical reaction rate, was confirmed to be the 2 2 + state, whereas the 4 1 + state, expected to be strongly populated in two-neutron knockout, was not observed. This puzzle is resolved by theoretical considerations of the Thomas-Ehrman shift, which also indicates that a previously reported 3471-keV state in Si 24 is, in fact, the ( 0 2 + ) level with one of the largest experimental mirror-energy shifts ever observed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2025

Performance evaluation of the SPES FEBIAD ion source

SPES (Selective Production of Exotic Species) is the Radioactive Ion Beam (RIB) facility that is currently in the installation phase at the Istituto Nazionale di Fisica Nucleare in the Laboratori Nazionali di Legnaro (LNL-INFN). The main purpose of the facility is to deliver neutron-rich radioactive beams with a range of mass between 60 and 160 amu produced as fission products originated within a Uranium Carbide (UC x ) target impinged by high energy protons (40–70 MeV). In the last few years, the SPES group and their collaborators have focused on multiple aspects: development of various ISOL targets, ion sources, a high-power beam dump, versatile Front-End designs, primary proton beam and RIB diagnostics, design of beam optic components, and remote target handling. The development and optimization of ionization sources represents one of the most important R&D activities. The collaboration between SPES and ISOLDE (CERN) groups has enabled the evaluation of the performances of a novel FEBIAD ion source taking advantage of the ISOLDE off-line Front-End. In this paper, the results of efficiency and transversal emittance measurements of the new SPES FEBIAD ion source are presented and discussed. Particular attention is dedicated to the description of the experimental setup and to the comparison of experimental data with simulation to promote the reproducibility of the experimental tests with other types of sources.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗