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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Diffractive Imaging of Conical Intersections Amplified by Resonant Infrared Fields

The fate of virtually all photochemical reactions is determined by conical intersections. These are energetically degenerate regions of molecular potential energy surfaces that strongly couple electronic states, thereby enabling fast relaxation channels. Their direct spectroscopic detection relies on weak features that are often buried beneath stronger, less interesting contributions. For azobenzene photoisomerization, a textbook photochemical reaction, we demonstrate how a resonant infrared field can be employed during the conical intersection passage to significantly enhance its coherence signatures in time-resolved Xray diffraction while leaving the product yield intact. Furthermore, this transition-state amplification holds promise to bring signals of conical intersections above the detection threshold.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

On resistive interchange, double tearing, and resonant and non-resonant infernal modes in spherical tokamak negative central shear discharges

We examine the linear and nonlinear stability of a sequence of reversed shear NSTX equilibria with the same toroidal current density and pressure profile but with different toroidal field strengths. All equilibria have two q = 2 surfaces and have q > 1 everywhere. For this sequence, which all have β P ∼ 0.5, as the minimum value of q decreases below about 1.4, the localized resistive interchange criterion is strongly violated, and the unstable mode with toroidal mode number n=1 changes its dominant poloidal mode number m from a (m,n)=(2,1) double tearing mode to a non-resonant (1,1) infernal mode. This (1,1) mode nonlinearly flattens both the current density and the pressure near the magnetic axis. The higher-n unstable modes are all resistive infernal modes localized around the surface where q has a minimum and the magnetic shear vanishes. They generally saturate nonlinearly at low amplitude but can cause magnetic surface breakup near the axis.

Spitzer resistivity↗
DOE OSTI2024

Quasiparticle Poisoning of Superconducting Qubits from Resonant Absorption of Pair-Breaking Photons

The ideal superconductor provides a pristine environment for the delicate states of a quantum computer: because there is an energy gap to excitations, there are no spurious modes with which the qubits can interact, causing irreversible decay of the quantum state. As a practical matter, however, there exists a high density of excitations out of the superconducting ground state even at ultralow temperature; these are known as quasiparticles. Observed quasiparticle densities are of order 1 μ m - 3 , tens of orders of magnitude greater than the equilibrium density expected from theory. Nonequilibrium quasiparticles extract energy from the qubit mode and can induce dephasing. Here we show that a dominant mechanism for quasiparticle poisoning is direct absorption of high-energy photons at the qubit junction. We use a Josephson junction-based photon source to controllably dose qubit circuits with millimeter-wave radiation, and we use an interferometric quantum gate sequence to reconstruct the charge parity of the qubit. We find that the structure of the qubit itself acts as a resonant antenna for millimeter-wave radiation, providing an efficient path for photons to generate quasiparticles. A deep understanding of this physics will pave the way to realization of next-generation superconducting qubits that are robust against quasiparticle poisoning.

Liu, Chuan-Hong↗
DOE OSTI2020

Toward 1% single-photon anharmonicity with periodically poled lithium niobate microring resonators

The absence of the single-photon nonlinearity has been a major roadblock in developing quantum photonic circuits at optical frequencies. In this paper, we demonstrate a periodically poled thin film lithium niobate microring resonator (PPLNMR) that reaches 5,000,000%/W second-harmonic conversion efficiency—almost 20-fold enhancement over the state-of-the-art—by accessing its largest χ <#comment/> ( 2 ) tensor component d 33 via quasi-phase matching. The corresponding single-photon coupling rate g / 2 π <#comment/> is estimated to be 1.2 MHz, which is an important milestone as it approaches the dissipation rate κ <#comment/> / 2 π <#comment/> of best-available lithium niobate microresonators developed in the community. Using a figure of merit defined as g / κ <#comment/> , our device reaches a single-photon nonlinear anharmonicity approaching 1%. We show that, by further scaling of the device, it is possible to improve the single-photon anharmonicity to a regime where photon blockade effect can be manifested.

Lu, Juanjuan (ORCID:0000000319389119)↗
DOE OSTI2024

A Resolved Resonance Evaluation for 51 V with Resonance Parameter Covariance

In this presentation the 51 V evaluation in response to NCSP need is completed. Issues in connection to RR representation are addressed. Uncertainty and covariance information derived with the evaluation. Evaluation proposed and accepted for inclusion in ENDF/B-VIII.1 library.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Improved $^{95}\mathrm{Mo}$ neutron resonance parameters and astrophysical reaction rates

We report improved 95 Mo neutron resonance parameters and reaction rates are important for nuclear astrophysics, testing nuclear models, and nuclear criticality safety. However, despite many previous neutron-capture and total cross-section measurements on this nuclide, there still is much room for improvement as well as several discrepancies. For example, there are very few firm resonance spin and parity assignments; average resonance parameters are available only for each parity, the currently recommended astrophysical reaction rate results in disagreements between stellar models and meteoric isotopic anomalies, and there are substantial disagreements in the neutron-capture cross section at low energies important for nuclear criticality safety. To obtain an improved set of neutron resonance parameters and astrophysical reaction rates for 95 Mo. High-resolution neutron-capture and transmission data were measured at the Oak Ridge Electron Linear Accelerator (ORELA) using highly isotopically enriched 95 Mo samples. The neutron-capture apparatus, data reduction, and analysis were improved so that information contained in the γ-ray cascade following neutron capture were used to assign resonance J π values. Following this, simultaneous analysis of the new neutron-capture and transmission data was used to obtain resonance energies, gamma widths, and neutron widths and their uncertainties to a maximum energy of 10 keV. Accurate neutron-capture cross sections also were obtained for the unresolved resonance region to a maximum energy of 500 keV and, together with the new resonance parameters, used to calculate the astrophysical reaction rates in the temperature range from 5 to 30 keV. A vastly improved set of 95Mo neutron resonance parameters and an astrophysical reaction rate accurate to about 3% were obtained. Firm J π assignments were determined for 261 of the 314 observed resonances. This is a very large improvement over the previously published 32 firm J π assignments for 108 resonances. Also, the number of resonances having both firm J π assignments and Γ γ values was increased by almost a factor of 24—from 11 to 261. Neutron- and total-radiation-width distributions and average resonance spacings, average total radiation widths, and neutron strength functions were obtained for the six different s- and p-wave possibilities. Parameters for the lowest s-wave resonance, which is most important for criticality benchmarks, were obtained with high accuracy. Simple modification of the neutron-capture apparatus and expansion and improvement of data analysis techniques led to a large increase in firm J π assignments for 95 Mo neutron resonances. The resulting astrophysical reaction rate is 20%–30% larger than the currently recommended rate at s-process temperatures, which should lead to better agreement between stellar models and meteoric isotopic anomalies. The neutron-capture cross section at low energies is substantially larger than recommended in the latest evaluation, which is problematical for criticality benchmarks. The average resonance spacing as a function of spin and parity is significantly different from current models. The total-radiation-width distributions are significantly broader than predicted by theory and show significant departures from the expected Gaussian shapes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Correct Interpretations of ENDF-102 Definitions for Resonance Effects

My Uncle Willie circa 1600 wrote “What’s in a name; a rose by any other name would smell as sweet.” I fear in this case we have a somewhat similar problem in that we may be using the same word but are not using the same definition; specifically, the word Unresolved. The simplest physics definition as it applies to neutron resonances, is the energy point where we can no longer see/measure ALL – let me repeat that – ALL - of the individual resonances. That seems simple and clear, but the question is: how to represent resonances beyond this point in order to accurately reproduce the effects we have seen in measurements and expect/need to reproduce in our applications. We know there are more, unseen resonances, otherwise we wouldn’t say Unresolved. The ENDF approach is well defined in ENDF-102 and simple: for ENDF data the only way to represent Unresolved data is by using a theoretical model to define the distribution of resonances, including those that are too narrow to measure (i.e., are unresolved). It is important to note that in ENDF this is the one and only Unresolved model, e.g., there is no provision in ENDF to accurately define individually ALL resonances above the Resolved energy range – by ALL here I mean both those that we can measure and those that we cannot individually measure, but that theory and integral measurements tells us are present. An alternative approach, which would appear to be equally valid, would be to include the latest measured data as tabulated energy expendent data extending upwards in energy above the Resolved energy range. In this approach the evaluation would not include an ENDF style Unresolved energy range; it would only include a Resolved resonance region, followed by tabulated higher energy points, representing the resonances that could be measured beyond the Resolved range. But an important point to note: By listing these resonances above the resolved energy one admits that at least some resonances in this energy range are missing as Unresolved; i.e., they are too narrow or overlapping to measure. The purpose of this paper is to illustrate that the later approach, while done with good intentions, and appearing to be valid/adequate in plots, does not meet the need of our engineering applications. Why? As we will see below, of these two possible approaches, only the ENDF use of a model to statistically include the missing, i.e., unresolved, resonances, can meet our engineering needs to reproduce the integral effects we have measured and understand. Only with this statistical model can we predict and include in our calculated results the important effects of temperature (Doppler broadening), and energy integrals (self-shielding). Below I will first present results using two ENDF/B-VIII.1 evaluations, U235 and U238, that use the correct ENDF-102 definition of an Unresolved resonance region, using a statistical model to include the effects of resonances that theory predicts are present, but are too narrow to measure. These two evaluations reproduce the expected temperature (Doppler) and energy integral (self-shielding) effects that we expect. Next I will present results using one ENDF/B-VIII.1 evaluation, 26-Fe-56, that does not use an ENDF-102 Unresolved resonance region; instead above its Resolved energy range it lists many tabulated energy points, that look like measured data, but by definition, since they are included above the ENDF Resolved energy range there are missing Unresolved resonances, i.e., there are missing the resonances that are too narrow to resolve, i.e., are unresolved. My conclusion, and I hope yours, is that the below figures illustrate that this approach does not reproduce the temperature and energy integrals that we expect and need to accurately calculate results for our fission reactor calculations. As such this approach should not be used in ENDF formatted evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Noninvasive Near‐Field Spectroscopy of Single Subwavelength Complementary Resonators

Abstract Subwavelength metallic resonators provide a route to achieving strong light–matter coupling by means of tight confinement of resonant electromagnetic fields. Investigation of such resonators however often presents experimental difficulties, particularly at terahertz (THz) frequencies. A single subwavelength resonator interacts weakly with THz beams, making it difficult to probe it using far‐field methods, whereas arrays of resonators exhibit inter‐resonator coupling, which affect the resonator spectral signature and field confinement. Here, traditional far‐field THz spectroscopy is systematically compared with aperture‐type THz near‐field microscopy for investigating complementary THz resonators. While the far‐field method proves impractical for measuring single resonators, the near‐field technique gives high signal‐to‐noise spectral information, only achievable in the far‐field with resonator arrays. At the same time, the near‐field technique allows to analyze single resonators without significant interaction with the near‐field probe. Furthermore, the near‐field technique allows highly confined fields and surface waves to be mapped in space and time. This information gives invaluable insight into spectral response in resonator arrays. This near‐field microscopy and spectroscopy method enables investigations of strong light–matter coupling at THz frequencies in the single‐resonator regime.

Hale, Lucy L.↗
DOE OSTI2023

Laboratory electron screening in nuclear resonance reactions

Both nonresonant and resonance reaction data are subject to laboratory electron screening effects. For non resonant reactions, such effects are well documented and the measured cross sections can be corrected to find the unscreened ones. Frequently, the procedure and expression to calculate laboratory electron screening factors for nonresonant reactions are also applied to isolated narrow resonances, without much theoretical support or experimental evidence. Here, a simple model is applied to estimate electron screening factors, lengths, and potentials for narrow resonances. The corrections to the measured data result in an enhancement of the unscreened resonance strengths by less than 0.2%, contrary to published narrow-resonance screening correction factors, which predict a reduction of the unscreened strengths by up to 25%. Unless it can be proven otherwise, it is recommended that measured strengths of isolated narrow resonances not be corrected for laboratory electron screening. The prospects of investigating laboratory electron screening effects by measuring almost negligible differences in resonance strengths are not promising. Instead, the difference of the resonance energy for the unscreened and screened situation may be measurable. As an example, the case of the E r = 956-keV resonance in the 27 Al(p,γ) 28 Si reaction is discussed. It is also demonstrated that the claim of a previously reported detection of a resonance near 800 keV in the 176 Lu(p,n) 176 Hf reaction is incorrect.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

High-bandwidth density silicon photonic resonators for energy-efficient optical interconnects

The growth of artificial intelligence applications demands ever larger and more complex deep learning models, dominating today's—and tomorrow's—data center and high-performance computing systems. While traditional electronics are failing to keep pace with application demands, silicon photonic (SiPh) interconnects have emerged as a necessary technology to support these systems. SiPh-driven wavelength-division multiplexing (WDM) offers a particularly promising path toward supporting incredibly high-aggregate link bandwidth in a compact and efficient form factor. One of the basic building blocks of these integrated WDM interconnects is the SiPh resonator. Their inherent wavelength selectivity and compact footprint allow for efficient data transmission multiplexed across dozens of carrier wavelengths. Used as add-drop (AD) filters, SiPh resonators are critical to constructing integrated tunable wavelength-selective optical circuit switches as well as for demultiplexing the different carrier wavelengths toward independent wavelength-insensitive photodiodes in a dense wavelength-division multiplexing receiver. Resonators in the all-pass (AP) configuration are widespread as well, allowing for wavelength-selective modulation to drive aggregate link bandwidths far beyond the individual channel data rate. Unlike SiPh Mach–Zehnder modulators (MZM), resonant modulators can be driven using low, complementary metal-oxide-semiconductor drive voltages, allowing for tight co-integration between photonic integrated circuits, fabricated with larger process node technologies, and electronic integrated circuits, designed to exploit the advantages of the latest node. To push toward practical peta-scale interconnects, a comprehensive review of SiPh resonators is required, addressing bottlenecks and design constraints at both the architecture and device levels. We first describe the predominant integrated link architectures and identify their limits. We then discuss the device-level design considerations that can be made for both AD and AP configuration resonators to overcome the system level limits with novel resonator device designs. Analytical models and numerical simulation of resonators are validated by experimental measurement of devices fabricated in a commercial 300-mm foundry, showing a clear path toward volume manufacturing. The demonstrated resonant modulators and filters support the feasibility of increasing the aggregate bandwidth of resonator-driven SiPh interconnects into the peta-scale regime.

42 ENGINEERING↗
DOE OSTI2023

MEMS-tunable optical ring resonator

A microelectromechanical systems (MEMS)-tunable optical ring resonator is described herein. The ring resonator includes a resonator ring and a tuner ring, along with one or more springs. The springs may be internal or external, i.e., either within or outside the areal footprint of the resonator ring and the tuner ring. The one or more springs are configured to displace the tuner ring from the resonator ring by a desired gap based upon a desired resonant wavelength of the resonator ring. Tuning is implemented by applying a voltage to the ring resonator, with motion of the tuner ring causing a corresponding change in the effective index of the resonator ring. As the ring resonator is essentially a capacitive device, it draws very little power once tuning is achieved.

Wood, Michael↗
DOE OSTI2023

Anomalous Loss Reduction Below Two‐Level System Saturation in Aluminum Superconducting Resonators

Superconducting resonators are widely used in many applications such as qubit readout for quantum computing, and kinetic inductance detectors. These resonators are susceptible to numerous loss and noise mechanisms, especially the dissipation due to two-level systems (TLS) which become the dominant source of loss in the few-photon and low temperature regime. In this study, capacitively-coupled aluminum half-wavelength coplanar waveguide resonators are investigated. Surprisingly, the loss of the resonators is observed to decrease with a lowering temperature at low excitation powers and temperatures below the TLS saturation. This behavior is attributed to the reduction of the TLS resonant response bandwidth with decreasing temperature and power to below the detuning between the TLS and the resonant photon frequency in a discrete ensemble of TLS. When response bandwidths of TLS are smaller than their detunings from the resonance, the resonant response and thus the loss is reduced. At higher excitation powers, the loss follows a logarithmic power dependence, consistent with predictions from the generalized tunneling model (GTM). A model combining the discrete TLS ensemble with the GTM is proposed and matches the temperature and power dependence of the measured internal loss of the resonator with reasonable parameters.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗