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At least 55 records · Page 3

Studies of radiative effects for polar stratospheric clouds

Data from the Antarctic Ozone Experiment of 1987 are used to model the radiative effects of polar stratospheric clouds. Heating and cooling rates are examined, showing that the heating and/or cooling rates within a polar stratospheric cloud depend on particle size, composition, optical depth of the cloud, solar angle, and temperature profile. The rates for an optically thin Type I cloud are too small to drive vertical motions in the stratosphere, while optically thin Type II clouds cause a stratospheric cooling.

Kinne, S.↗

Albedo enhancement and perturbation of radiation balance due to stratospheric aerosols

The effect of stratospheric aerosols on the earth's monthly zonal radiation balance is investigated using a model layer consisting of 75% H2SO4, which is the primary constituent of the background aerosol layer. The reduction in solar energy absorbed by the earth-atmosphere system is determined through the albedo sensitivity, defined here as the change in albedo per unit mid-visible optical depth of the aerosol layer. The optically thin approximation is used in conjunction with the Henyey-Greenstein phase function for scattering to simplify computations. Satellite derived planetary albedos are used as the frame of reference about which the change in albedo is computed. An infrared radiative transfer model is used to estimate the increased greenhouse effect attributed to the aerosol layer. The infrared heating tends to compensate for the albedo effect in altering the radiation balance. The results indicate that the dominant influence of the thin model stratospheric aerosol layer is an increased reflection of solar energy all over the globe except for the polar-winter region, but the change in the radiation balance is seen to be uniform and small equatorwards of 50%.

HARSHVARDHAN↗

Perturbation of the zonal radiation balance by a stratospheric aerosol layer

The effect of stratospheric aerosols on the earth's monthly zonal radiation balance is investigated using a model layer consisting of 75% H2SO4, the primary constituent of the background aerosol layer. The reduction in solar energy absorbed by the earth-atmosphere system is determined through the albedo sensitivity, and the optically thin approximation is used in conjunction with the Henyey-Greenstein phase function for scattering. An infrared radiative transfer model is used to estimate the increased greenhouse effect from the aerosol layer, and the infrared heating compensates for the albedo effect in altering the radiation balance. The results indicate that the dominant influence of the thin model stratospheric aerosol layer is an increased reflection of solar energy all over the globe except for the polar-winter region, but the change in the radiation balance is uniform and small equatorward of 50 deg.

Harshvardhan, MR.↗

Radiative feedback of polar stratospheric clouds on Antarctic temperatures

A one-dimensional time marching radiative transfer model has been used to investigate the potential effects of polar stratospheric clouds (PSCs) on winter and spring temperatures in the Antarctic lower stratosphere. High, middle, and low PSC amounts were specified from lidar backscatter profiles and were chosen to represent the likely range of PSC amounts present in the Antarctic region. The computed effects of the PSCs on temperatures depend strongly on the surface temperature and on the extent of tropospheric cloudiness, and range from a maximum increase of 6 K for a high amount of PSCs over a warm surface and clear troposphere to a maximum decrease of 2 K for a high amount of PSCs over a cold surface and a troposphere with high clouds. The average effect is unlikely to be more than a 1 or 2 K temperature change.

Rosenfeld, Joan E.↗

The 200- to 300-nm radiation field in the stratosphere - Comparison of models with observation

The SABE 1 experiment (Herman and Mentall, 1982) measured the direct and scattered solar radiation at wavelengths between 190 and 320 nm from a balloon floating at 40 km altitude. We use state of the art radiative transfer models together with cross sections and solar flux data commonly used in modeling of the stratosphere to calculate the direct and scattered radiation at 40 km. The comparison between theory and experiment made by Herman and Mentall (1982) is extended. Significant discrepancies in the ratio of the scattered to direct flux not discussed in their work were found in the Schumann-Runge band and above 280 nm. Possible reasons for the differences are discussed.

Kylling, A.↗

A computation of the stratospheric diabatic circulation using an accurate radiative transfer model

The global diabatic circulation is computed for the months of January, April, July and October over the altitude region 100 to 0.1 mb using an accurate troposphere-stratosphere radiative transfer model, SBUV and SME ozone data, and NMC temperatures. There is high correlation between the level of wave activity and the local departure of the atmosphere from radiative equilibrium. An excess in the globally averaged net stratospheric heating from 40 to 50 km is computed for all months, and a deficit from 50 to 60 km is computed during solstice. A 20 percent uniform reduction in ozone from 40 to 50 km, or a temperature perturbation with an increase of 5 K at 1 mb, will bring the atmosphere into global radiative equilibrium without significant impact on the diabatic circulation. In the transitional months of April and October, the net heating in the fall hemispheres are very similar, while substantial differences exist between the spring hemispheres.

Rosenfield, Joan E.↗

Radiative properties of the background stratospheric aerosols and implications for perturbed conditions

A series of Mie scattering calculations has been performed to define the wavelength-dependent, single scattering properties of aerosols present in the stratosphere during July 1979. Additional radiative transfer computations were conducted to assess the impact of aerosols on the earth's radiation budget. For these purposes, an extensive set of measurements of aerosol characteristics that were obtained in Alaska from aircraft and satellite platforms was used. At that time, the optical depth was too small for aerosols to significantly impact earth's climate. But the optical depth of the stratospheric aerosol layer has been large enough during some volcanically perturbed periods for the aerosols to have caused a noticeable warming of the stratosphere and cooling of the troposphere.

Pollack, J. R.↗

Stratospheric Aerosol--Observations, Processes, and Impact on Climate

Interest in stratospheric aerosol and its role in climate have increased over the last decade due to the observed increase in stratospheric aerosol since 2000 and the potential for changes in the sulfur cycle induced by climate change. This review provides an overview about the advances in stratospheric aerosol research since the last comprehensive assessment of stratospheric aerosol was published in 2006. A crucial development since 2006 is the substantial improvement in the agreement between in situ and space-based inferences of stratospheric aerosol properties during volcanically quiescent periods. Furthermore, new measurement systems and techniques, both in situ and space based, have been developed for measuring physical aerosol properties with greater accuracy and for characterizing aerosol composition. However, these changes induce challenges to constructing a long-term stratospheric aerosol climatology. Currently, changes in stratospheric aerosol levels less than 20% cannot be confidently quantified. The volcanic signals tend to mask any nonvolcanically driven change, making them difficult to understand. While the role of carbonyl sulfide as a substantial and relatively constant source of stratospheric sulfur has been confirmed by new observations and model simulations, large uncertainties remain with respect to the contribution from anthropogenic sulfur dioxide emissions. New evidence has been provided that stratospheric aerosol can also contain small amounts of nonsulfatematter such as black carbon and organics. Chemistry-climate models have substantially increased in quantity and sophistication. In many models the implementation of stratospheric aerosol processes is coupled to radiation and/or stratospheric chemistry modules to account for relevant feedback processes.

Kresmer, Stefanie↗

A Three-Wave Model of the Stratosphere with Coupled Dynamics, Radiation and Photochemistry

A zonal mean chemistry transport model (2-D CTM) coupled with a semi-spectral dynamical model is used to simulate the distributions of trace gases in the present day atmosphere. The zonal-mean and eddy equations for the velocity and the geopotential height are solved in the semi-spectral dynamical model. The residual mean circulation is derived from these dynamical variables and used to advect the chemical species in the 2- D CTM. Based on a linearized wave transport equation, the eddy diffusion coefficients for chemical tracers are expressed in terms of the amplitude, frequency and growth rate of dynamical waves; local chemical loss rates; and a time constant parameterizing small scale mixing. The contributions to eddy flux are from the time varying wave amplitude (transient eddy), chemical reactions (chemical eddy) and small scale mixing. In spite of the high truncation in the dynamical module (only three longest waves are resolved), the model has simulated many observed characteristics of stratospheric dynamics and distribution of chemical species including ozone. Compared with the values commonly used in 2-D CTMs, the eddy diffusion coefficients for chemical species calculated in this model are smaller, especially in the subtropics. It is also found that the chemical eddy diffusion has only a small effects in determining the distribution of most slow species, including ozone in the stratosphere.

Shia, Run-Lie↗

A simple method to compute the change in earth-atmosphere radiative balance due to a stratospheric aerosol layer

A computer code was developed in terms of a three-layer model for the earth-atmosphere system, using a two-stream approximation for the troposphere and stratosphere. The analysis was limited to variable atmosphere loading by solar radiation over an unperturbed section of the atmosphere. The scattering atmosphere above a Lambertian ground layer was considered in order to derive the planar albedo and the spherical albedo. Attention was given to the influence of the aerosol optical thickness in the stratosphere, the single scattering albedo and asymmetry factor, and the sublayer albedo. Calculations were performed of the zonal albedo and the planetary radiation balance, taking into account a stratospheric aerosol layer containing H2SO4 droplets and volcanic ash. The resulting ground temperature disturbance was computed using a Budyko (1969) climate model. Local decreases in the albedo in the summer were observed in high latitudes, implying a heating effect of the aerosol. An accompanying energy loss of 23-27 W/sq m was projected, which translates to surface temperature decreases of either 1.1 and 0.45 C, respectively, for background and volcanic aerosols.

Lenoble, J.↗

Stratospheric aerosol properties and their effects on infrared radiation.

This paper presents a stratospheric aerosol model and infers its effects on terrestrial radiation. Composition of the aerosol is assumed to be concentrated sulfuric acid. An appropriate size distribution has been determined from available size distribution measurements of other investigators. Aerosols composed of concentrated sulfuric acid emit energy in the atmospheric window region of the infrared spectrum, 8-13 microns. Laboratory measurements of optical constant data obtained at room temperature are presented for 75 and 90% aqueous sulfuric acid. Calculations of an aerosol extinction coefficient are then performed by using the above data. Effects of changes in aerosol phase and temperature are discussed but not resolved.

Remsberg, E. E.↗

Solar UV radiation variations and their stratospheric and climatic effects

Nimbus-7 SBUV measurements of the short-term solar UV variations caused by solar rotation and active-region evolution have determined the amplitude and wavelength dependence for the active-region component of solar UV variations. Intermediate-term variations lasting several months are associated with rounds of major new active regions. The UV flux stays near the peak value during the current solar cycle variation for more than two years and peaks about two years later than the sunspot number. Nimbus-7 measurements have observed the concurrent stratospheric ozone variations caused by solar UV variations. There is now no doubt that solar UV variations are an important cause of short- and long-term stratospheric variations, but the strength of the coupling to the troposphere and to climate has not yet been proven.

Donnelly, R. F.↗