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NASA NTRSDate not supplied

Analysis of Nonequilibrium Molecular Nitrogen Ultraviolet Radiation in Pure N2 Shockwaves

This paper presents an analysis of data previously reported from a test series in the Electric Arc Shock Tube Facility for incident shocks composed of pure Nitrogen. The present work focuses on the lowest velocity measured in the test (approximately 7 km/s) where molecular radiation is significant. Analysis of the spectral data with the NEQAIR radiative transport code obtains post-shock trends in temperature and number densities of the states of N2. The results suggest that chemical, and possibly thermal, equilibrium has not been obtained within the distance/time measured (about 5 cm/120 s). In the nonequilibrium region of the shock, differences between rotational temperatures of different species are observed, as well as differences between rotational and vibrational temperatures. Population of rotational states above the dissociation limit is observed to occur over a distance of several cm. Finally, these data suggest that predissociation strongly affects the C^3 Π_u state of N2, leading to a lower measured radiation than predicted. An effective average pre-dissociation rate is shown to produce reasonable agreement under quasi-steady state approximation.

Augustin Tibere Inglesse↗

NASA NTRSDate not supplied

Analysis of nonequilibrium molecular nitrogen ultraviolet radiation in pure N2 shockwaves

An analysis of data previously reported from a test series in the Electric Arc Shock Tube Facility for incident shocks composed of pure Nitrogen was performed. The present work focuses on the lowest velocity measured in the test (approximately 7 km/s) where molecular radiation is significant. Analysis of the spectral data with the NEQAIR radiative transport code obtains post-shock trends in temperature and number densities of the states of N2. The results suggest that chemical, and possibly thermal, equilibrium has not been obtained within the distance/time measured (about 5 cm/120 ms). In the nonequilibrium region of the shock, differences between rotational temperatures of different species are observed, as well as differences between rotational and vibrational temperatures. Population of rotational states above the dissociation limit is observed to occur over a distance of several cm. Finally, these data suggest that predissociation strongly affects the C^3 Π_u state of N2, leading to a lower measured radiation than predicted. An effective average pre-dissociation rate is shown to produce reasonable agreement under quasi-steady state approximation.

Augustin Tibere-Inglesse↗

NASA NTRSDate not supplied

Analysis of the Amplitude Response of a Two-Point and a Multi-Point Focused Laser Differential Interferometer

Experiments were performed with two different focused laser differential interferometer (FLDI) instruments to assess the relative amplitude response of each instrument to a traveling shockwave generated by a laser spark in air. The first FLDI instrument generated two slightly-separated measurement points, with each measurement point providing sensitivity to density fluctuations induced by the shockwave. By performing a cross-correlation between the signals obtained from each measurement point, the phase velocity of density fluctuations can be obtained. The second FLDI instrument generated a measurement line that was oriented parallel to the shockwave direction of travel with the resulting interference pattern sampled at multiple equally-spaced points along the line. As a result, this instrument provides density fluctuation measurement capability at multiple points simultaneously. When the measurement line is oriented parallel to the shockwave direction of travel, the phase velocity, rate of change of the phase velocity, and acceleration of density fluctuations traveling along each line can be obtained by performing a cross-correlation between points along the line. Numerical computations of the shockwave generated by the laser spark are used to simulate the response of each instrument and are compared to the experimental results. High-speed schlieren imaging has also been performed and is compared with the FLDI measurements and computational results.

Interferometry↗

DOE OSTI2020

Validation of the Mach Stem Triple Point

Among the more complex characteristics of an explosion’s shock front is the creation of the Mach stem and its triple point. The scientific footage of the US Atmospheric Nuclear Weapons Testing Program has a film that may show the locus of points formed by the triple point, allowing us to visually investigate the trajectory of these shockwaves. During a nuclear blast, once the X-ray diffusion process ends, an incident shockwave forms in all directions. When the incident shockwave contacts the ground, a reflected shockwave is created. The overall magnitude and impact of these two shockwaves are proportional to the increasing total pressure and temperature, allowing the disturbances to move faster than the local speed of sound.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

NASA NTRSDate not supplied

Analysis of the Amplitude Response of a Two-Point and a Two-Line/Multi-Point Focused Laser Differential Interferometer

Experiments were performed with two different focused laser differential interferometer (FLDI) instruments to assess the amplitude response of each instrument to a traveling shock-wave generated by a laser spark. The first FLDI instrument generated two measurement points, with each measurement point providing sensitivity to density fluctuations induced by the shockwave. By performing a cross-correlation between the signals obtained from each measurement point, the phase velocity of density fluctuations can be obtained. The second FLDI instrument generated two measurement lines that are oriented either parallel or orthogonal to the shockwave direction of travel with the resulting interference pattern sampled at multiple equally-spaced points along each line. As a result, this instrument provides density fluctuation measurement capability at multiple points simultaneously. When the measurement lines are oriented parallel to the shockwave direction of travel, the phase velocity, rate of change of the phase velocity, and acceleration of density fluctuations traveling along each line can be obtained by performing a cross-correlation between points along a single line. When the measurement lines are oriented orthogonal to the shockwave direction of travel, the spatially-varying phase velocity can be obtained by performing a cross-correlation between points at the same relative location on each measurement line. Computations of the shockwave generated by the laser spark are used to simulate the response of each instrument and are compared to the experimental results. High-speed Schlieren imaging has also been performed and is compared with the FLDI measurements and computational results.

Focused Laser Differential Interferometer↗

NASA NTRSDate not supplied

Analysis of the Amplitude Response of a Two-Point and a Multi-Point Focused Laser Differential Interferometer

Brett F. Bathel↗

DOE OSTI2020

Directional shock diode behavior through the interaction of geometric voids in engineered polymer assemblies

With the advent of additive manufacturing (AM) techniques, a new class of shockwave mitigation and structural supports has been realized through the hierarchical assembly of polymer materials. To date, there have been a limited number of studies investigating the role of structure on shockwave localization and whether AM offers a means to tailor shockwave behavior. Of particular interest is whether the mesoscopic structure can be tailored to achieve shockwave properties in one direction of impact vs the other. In this work, we illustrate directional response in engineered polymer foams. In situ time-resolved x-ray phase contrast imaging at the Advanced Photon Source was used to characterize these diode-like structures. This work offers a breakthrough in materials technology for the development of protective structures that require augmentation of shock in one direction while diminishing transmission in the opposite direction.

42 ENGINEERING↗

DOE OSTI2023

Investigation on the explosion dynamics of large-format lithium-ion pouch cells

Explosion is the most extreme case of thermal runaway of lithium-ion (Li-ion) batteries. In this study, explosion dynamics of large-format Li-ion cells are investigated experimentally and numerically. Overcharge-to-explosion tests are conducted on 40 Ah Li-ion cells with Li[Ni 0.8 Co 0.1 Mn 0.1 ]O 2 cathode. Based on the explosion physics, shockwave and detonation models are used to characterize the shock effect of the cell explosion and evaluate the explosion equivalent. Von Neumann peak is observed on the pressure curves, and the shockwave velocity is supersonic at this time; the unwrinkled spherical flame phenomenon observed in the experiment indicates that it is detonation. Additionally, a geometric model is established based on the real testing scenario, and the explosion behavior is numerically studied. The characteristics of the explosion dynamics process are interpreted and the propagation mechanism of the shockwave are revealed; the deflagration to detonation transition (DDT) phenomenon in this process is caused by the formation of “hot spots”, and the explosion of the cells eventually turns into stable combustion. Here this study fills the gap in the research on thermal runaway of Li-ion cells, especially in the extreme cases of fire and explosion, and provide useful guidance for battery safety.

42 ENGINEERING↗

DOE OSTI2023

Spontaneous shock waves in pulse-stimulated flocks of Quincke rollers

Active matter demonstrates complex spatiotemporal self-organization not accessible at equilibrium and the emergence of collective behavior. Fluids comprised of microscopic Quincke rollers represent a popular realization of synthetic active matter. Temporal activity modulations, realized by modulated external electric fields, represent an effective tool to expand the variety of accessible dynamic states in active ensembles. Here, we report on the emergence of shockwave patterns composed of coherently moving particles energized by a pulsed electric field. The shockwaves emerge spontaneously and move faster than the average particle speed. Combining experiments, theory, and simulations, we demonstrate that the shockwaves originate from intermittent spontaneous vortex cores due to a vortex meandering instability. They occur when the rollers’ translational and rotational decoherence times, regulated by the electric pulse durations, become comparable. The phenomenon does not rely on the presence of confinement, and multiple shock waves continuously arise and vanish in the system.

36 MATERIALS SCIENCE↗

DOE OSTI2021

Underwater plasma breakdown characteristics with respect to highly pressurized drilling applications

Deep earth drilling is a key technique to extract oil, gas, and geothermal heat from the earth. Many complex energy focusing methods have been explored as an alternative approach to reach these resources but most of them require high energy. However, by utilizing short time span liquid plasma discharges, energy focusing can be achieved within traditional drilling systems. These discharges induce a rapid expansion process and a resulting shockwave. It is believed that this focused energy will lower the required cutting force to progress through the rock. Lowering the required cutting force will allow for lower drill bit wear, quicker rate of penetration, and an overall cost savings of the project. Plasma breakdown characteristics at drilling relevant pressures, ranging from 1 to 350 atm, were studied. A resistance–capacitance circuit with an air gapped spark switch was utilized to generate pulsed plasma between the pressurized electrodes. It was found that the required breakdown voltage increases as the pressure increases. It was also found that a plasma channel formation and an associated breakdown may or may not occur between the electrodes at different pressures due to variation in required breakdown voltages. Breakdown time-lag in the dielectric medium (tap water, 780 μS cm –1 ) increased as the pressure was increased, which indicated a higher voltage drop at higher pressures (>100 atm). The plasma generated cavitation bubble with an associated shockwave occurred as pressures were increased. However, the bubble radius and the bubble duration decreased as the pressure was increased. The plasma generated shockwave speeds fall within the expected speed of sound in water. Lastly, preliminary rock cracking tests were performed on granite at high pressures (340 and 272 atm) and it was found that plasma is able to create cracks in the rock.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2025

Laser-driven flash x-ray radiography of a shocked metallic foil

Characterizing hydrodynamic instability evolution in millimeter-scale, high-Z foils is crucial for understanding complex phenomena in high-energy-density physics. Here, we demonstrate a proof-of-concept, laser-driven flash x-ray radiography platform tailored for two-dimensional linear density mapping in shocked high-Z foils. Using chromium (Cr) foils with internal shockwaves (∼100 μm width), our platform achieves a spatial resolution of 59.8 ± 1.4 μm by employing a broadband x-ray source extending into the hundreds of keV range. The setup combines a compound parabolic concentrator cone with a tantalum wire target, a magnetic field to deflect residual transmitted electrons, and a copper casing to shield the sides and rear of the image plate pack. By varying the delay of the short-pulse beam driving the flash x-ray source, we resolve shockwave dynamics, specifically the velocity, position, width, and density profile, within the Cr foil. Reported experimental results are consistent with the corresponding hydrodynamics and radiation transport simulations, which accurately reproduce the measured electron and x-ray source terms. These developments enable the conversion of shockwave radiographs into two-dimensional density maps, enhancing interpretability for hydrodynamic instability evolution applications and validating the simulation approach.

36 MATERIALS SCIENCE↗

DOE OSTI2025

An infrared on-shell action and its implications for soft charge fluctuations in asymptotically flat spacetimes

We study the infrared on-shell action of Einstein gravity in asymptotically flat spacetimes (AFSs), obtaining an effective, gauge-invariant boundary action for memory and shockwave spacetimes. We show that the phase space is in both cases parameterized by the leading soft variables in AFSs, thereby extending the equivalence between shockwave and soft commutators to spacetimes with non-vanishing Bondi mass. We then demonstrate that our on-shell action is equal to three quantities studied separately in the literature: (i) the soft supertranslation charge; (ii) the shockwave effective action, or equivalently the modular Hamiltonian; and (iii) the soft effective action. Finally, we compute the quantum fluctuations in the soft supertranslation charge and, assuming the supertranslation parameter may be promoted to an operator, we obtain an area law, consistent with earlier results showing that the modular Hamiltonian has such fluctuations.

asymptotically flat spacetimes↗

DOE OSTI2023

Shock physics and shadowgraphic measurements of laser-produced cerium plasmas

Shadowgraphic measurements are combined with theory on gas-dynamics to investigate the shock physics associated with nanosecond laser ablation of cerium metal targets. Time-resolved shadowgraphic imaging is performed to measure the propagation and attenuation of the laser-induced shockwave through air and argon atmospheres at various background pressures, where stronger shockwaves characterized by higher propagation velocities are observed for higher ablation laser irradiances and lower pressures. The Rankine-Hugoniot relations are also employed to estimate the pressure, temperature, density, and flow velocity of the shock-heated gas located immediately behind the shock front, predicting larger pressure ratios and higher temperatures for stronger laser-induced shockwaves.

42 ENGINEERING↗

DOE OSTI2020

Laser-Plasma Spatiotemporal Cyanide Spectroscopy and Applications

This article reports new measurements of laser-induced plasma hypersonic expansion measurements of diatomic molecular cyanide (CN). Focused, high-peak-power 1064 nm Q-switched radiation of the order of 1 TW/cm 2 generated optical breakdown plasma in a cell containing a 1:1 molar gas mixture of N 2 and CO 2 at a fixed pressure of 1.1 × 10 5 Pascal and in a 100 mL/min flow of the mixture. Line-of-sight (LOS) analysis of recorded molecular spectra indicated the outgoing shockwave at expansion speeds well in excess of Mach 5. Spectra of atomic carbon confirmed increased electron density near the shockwave, and, equally, molecular CN spectra revealed higher excitation temperature near the shockwave. Results were consistent with corresponding high-speed shadowgraphs obtained by visualization with an effective shutter speed of 5 nanoseconds. In addition, LOS analysis and the application of integral inversion techniques allow inferences about the spatiotemporal plasma distribution.

36 MATERIALS SCIENCE↗

DOE OSTI2023

On causality conditions in de Sitter spacetime

We carefully consider the Shapiro time delay due to black holes and shockwaves in de Sitter spacetime and study the implications for causality. We discuss how causality conditions of AdS and flat spacetime can be applied in de Sitter spacetime, using spatial shifts measured on the boundary to define 'fastest null geodesics' and taking into account the 'stretching' of the de Sitter Penrose diagram. We consider the propagation of a massless spin-1 field with a non-minimal coupling in a de Sitter shockwave background as an illustrative example. Here, we also briefly discuss connections to the average null energy condition.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Holographic probes of inner horizons

We study the inner horizons of rotating and charged black holes in anti-de Sitter space. These black holes have a classical analytic extension through the inner horizon to additional asymptotic regions. If this extension survives in the quantum theory, it requires particular analytic properties in a dual CFT, which give a prescription for calculating correlation functions for operators placed on any asymptotic boundary of the maximally extended spacetime. We show that for charged black holes in three or greater dimensions, and rotating black holes in four or greater dimensions, these analytic properties are inconsistent in the dual CFT, implying the absence of an analytic extension for quantum fields past the inner horizon. Thus, we find that strong cosmic censorship holds for all AdS black holes except rotating BTZ. To further study the latter case, we insert classical perturbations near the boundary at late times, producing shockwaves traveling along the inner horizon. We holographically compute CFT correlators in this background that probe a high energy scattering process near the inner horizon and argue that the shockwave does not destabilize the inner horizon violently enough to prevent signaling between different asymptotic regions of the Penrose diagram. This provides evidence that the rotating BTZ black hole does violate the strong cosmic censorship conjecture.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2023

Small $x$ physics beyond eikonal approximation: an effective Hamiltonian approach

Understanding the spin structure of hadrons in the small x regime is an important direction to unravel the spin puzzle in hadronic physics. To include spin degrees of freedom in the small x regime requires going beyond the usual eikonal approximation in high energy QCD. We developed an effective Hamiltonian approach to study spin related observables in the small x regime using the shockwave formalism. The small-x effective Hamiltonian incorporates both quark and gluon propagators in the background fields and the background field induced interaction vertices up to next-to-eikonal order. A novel feature of sub-eikonal interactions is the background gluon field induced gluon radiation inside the shockwave. Its relation to chromo-electrically polarized Wilson line correlator is established both in small x helicity evolution and in longitudinal double-spin asymmetry for gluon production.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Firewalls at exponentially late times

We consider a version of the typical state firewall setup recently reintroduced by Stanford and Yang, who found that wormholes may create firewalls. We examine a late-time scaling limit in JT gravity in which one can resum the expansion in the number of wormholes, and we use this to study the exact distribution of interior slices at times exponential in the entropy. We consider a thermofield double with and without early perturbations on a boundary. These perturbations can appear on interior slices as dangerous high energy shockwaves. For exponentially late times, wormholes tend to teleport the particles created by perturbations and render the interior more dangerous. In states with many perturbations separated by large times, the probability of a safe interior is exponentially small, even though these would be safe without wormholes. With perturbation, even in the safest state we conceive, the odds of encountering a shock are fifty-fifty. One interpretation of the phenomenon is that wormholes can change time-ordered contours into effective out-of-time-ordered folds, making shockwaves appear in unexpected places.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗