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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
NASA NTRS2013

Efficient 1.6 Micron Laser Source for Methane DIAL

Methane is a potent greenhouse gas and on a per molecule basis has a warming influence 72 times that of carbon dioxide over a 20 year horizon. Therefore, it is important to look at near term radiative effects due to methane to develop mitigation strategies to counteract global warming trends via ground and airborne based measurements systems. These systems require the development of a time-resolved DIAL capability using a narrow-line laser source allowing observation of atmospheric methane on local, regional and global scales. In this work, a demonstrated and efficient nonlinear conversion scheme meeting the performance requirements of a deployable methane DIAL system is presented. By combining a single frequency 1064 nm pump source and a seeded KTP OPO more than 5 mJ of 1.6 μm pulse energy is generated with conversion efficiencies in excess of 20%. Even without active cavity control instrument limited linewidths (50 pm) were achieved with an estimated spectral purity of ~95%. Tunable operation over 400 pm (limited by the tuning range of the seed laser) was also demonstrated. This source demonstrated the critical needs for a methane DIAL system motivating additional development of the technology.

Shuman, Timothy↗
NASA NTRS1981

Investigation of the CARS spectrum of water vapor

The dependence of the coherent anti-Stokes Raman (CARS) spectrum of water vapor on temperature has been measured and compared with CARS spectral model calculations to permit diagnostics of this important combustion product. Measurements have been made in a methane-air flame at 1700 K and in a heated cell, maintained at atmospheric pressure and temperatures between 310 K and 710 K. The agreement between measured and calculated spectra is very good. The importance of assumed Raman linewidth is shown to be critical to the calculation of spectral features near the band head of measured spectra.

Shirley, J. A.↗
NASA NTRS1992

Optical spectroscopy of Z Canis Majoris, V1057 Cygni, and FU Orionis - Accretion disks and signatures of disk winds

High resolution, high SNR optical spectra have been used to investigate the hypothesis that in outburst, FU Ori objects are self-luminous accretion disks whose light dominates at optical and near-IR wavelengths. Strong evidence has been found for linewidth versus wavelength correlation in good agreement with model predictions for Z CMa and V1057 Cyg, but not for FU Ori itself. Linewidth varies continuously with wavelength at optical wavelengths in the former two objects, In the case of FU Ori, it is argued that a combination of strong wind components to spectral lines, and surface gravity possibly being lower than that of supergiants, conceals the underlying linewidth versus wavelength relationship. A marginal correlation is found between linewidth and lower excitation potential in all three objects. Synthetic disk spectra are subtracted from observed spectral, and remarkably good fits are found for all three objects for wavelengths longer than about 5000 A.

Welty, Alan D.↗
NASA NTRS1988

Diode laser-pumped solid-state lasers

An evaluation is made of the consequences for solid-state lasers of novel diode laser-pumping technology. Diode laser-pumped neodymium lasers have operated at an electrical-to-optical efficiency of 10 percent in a single spatial mode, with linewidths of less than 10 kHz, and with a spectral power brightness sufficiently great to allow frequency extension by harmonic generation in nonlinear crystals; this has yielded green and blue sources of coherent radiation. Q-switched operation with kW peak powers and mode-locked operation with 10-picosec pulse widths have also been demonstrated. All-solid-state lasers at prices comparable to those of current flash-lamp-pumped laser systems are foreseen, as are power levels exceeding 1 kW, for coherent radar, global satellite sensing, and micromachining.

Byer, Robert L.↗
NASA NTRS1989

Linewidth measurements in the thermal infrared bands of (C-12)H3D at planetary atmospheric temperatures

Collision-broadened halfwidths of three lines in the nu3 fundamental band and of four lines in the nu6 fundamental band of (C-12)H3D have been measured at temperatures between 123 and 295 K using the Doppler-limited spectral resolution of a tunable diode laser spectrometer. Temperature dependence of the linewidths has been determined in self-broadening and in broadening by H2, He and N2.

Varanasi, Prasad↗
NASA NTRS2018

The Challenges of Measuring Methane from Space with a Lidar

The global and regional quantification of methane fluxes and identification of its sources and sinks has been highlighted as one of the goals of the NASA 2017 Earth Science Decadal Survey. Detecting methane from space and airborne platforms with an active (laser) remote sensing instrument presents several unique technology and measurement challenges. The instrument must have a single frequency, narrow-linewidth light source, and photon-sensitive detector at the right spectral region to make continuous measurements from orbit, day and night, all seasons and at all latitudes. It must have a high signal to noise ratio and must be relatively immune to biases from aerosol/cloud scattering, spectroscopic and meteorological data uncertainties, and instrument systematic errors. At Goddard Space Flight Center (GSFC), in collaboration with industry, we have developed an airborne instrument to measure methane. Our instrument is a nadir-viewing lidar that uses Integrated Path Differential Absorption (IPDA), to measure methane near 1.65 µm. We sample the absorption line using multiple wavelengths from a narrow linewidth laser source and a sensitive photodetector. This measurement approach provides maximum information content about the CH4 column, and minimizes biases in the XCH4 retrieval. In this paper, we will review our progress to date and discuss the technology challenges, options and tradeoffs to measure methane from space and airborne platforms.

airborne instruments↗
NASA NTRS1981

Anti-Stokes scattering as an XUV radiation source

Harris (1977) has shown that laser induced scattering from atoms stored in a metastable level may be used to produce an XUV radiation source with several unique properties, including narrow linewidth, tunability, linear polarization, picosecond pulsewidth, and relatively high peak spectral brightness. The present investigation provides a summary concerning the progress made on the use of this radiation source as a unique instrument for XUV spectroscopy, and as a possible flashlamp for a 200 A laser. Zych et al. (1978) demonstrated that the maximum spectral brightness of the source is that of a blackbody with a temperature of the metastable storage level. The peak count rate and peak spectral brightness of the anti-Stokes emission at 569 A are 17 times and 139 times greater than those of the 584 A resonance line. The anti-Stokes process was employed as an external source of radiation for high resolution spectroscopy of the 3p6 shell of potassium. Attention is also given to emission spectroscopy of lithium, metastable levels which are appropriate for storage, and a hollow cathode discharge.

Harris, S. E.↗
NASA NTRS1975

Measurements of SO2 absorption coefficients using a tunable dye laser

High-resolution measurements of SO2 absorption coefficients in the UV are presented in the wavelength interval between 2962 and 3011 A using a frequency-doubled dye laser as the radiation source. These measurements have application to pollution monitoring of SO2 using the differential absorption scattering (DAS) technique. The spectral resolution of the measurements was 0.2 A (determined by the linewidth of the dye laser) and the generated spectra exhibited considerable rotational structure on the (000) double prime to (060) prime, (070) prime, and (080) prime electronic-vibrational transitions. The latter transitions correspond to center wavelengths of 3001.8, 2981.0, and 2962 A, respectively. The laser measurements were obtained with a signal-processing technique which eliminated calibration procedures associated with conventional optical-absorption measurements. Using this technique, the statistical uncertainty associated with measured absorption coefficients has been reduced to less than plus or minus 2% with a wavelength uncertainty of the laser source of plus or minus 0.1 A.

Thompson, R. T., Jr.↗
NASA NTRS1983

Programmable, secondary frequency standard based infrared synthesizer using tunable lead-salt diode lasers

Quantum phase noise limited Lorentzian power spectral densities were achieved with tunable lead-salt diode lasers. Linewidths as narrow as 22 kHz were observed. A truly programmable infrared synthesizer was produced by frequency-offset-locking the tunable diode lasers to the combination of a stable CO2 (or CO) reference laser and a programmable microwave frequency synthesizer. Absolute frequency accuracy and reproducibility of about + or - 30 kHz (0.000001 kaysers) relative to the primary Cs frequency standard may now be obtained with this technique.

Freed, C.↗
NASA NTRS1986

Alexandrite laser source for atmospheric lidar measurements

During the past years, there has been a marked increase in interest in the applications of vibronic solid state lasers to meteorology and atmospheric physics. Two airborne lidar programs are now under development in France. The differential absorption lidar (DIAL) method with vibronic solid state lasers is very attractive for water vapor, temperature and pressure measurements. Alexandrite laser and titanium-sapphire are both suitable for these applications. However, only alexandrite rods are commercially available. The requirements on the laser source for airborne dial applications are two fold: (1) a restriction on laser linewidth and a requirement on stability and tunability with a good spectral purity; and (2) a requirement on the time separation between the two pulses. These constraints are summarized.

Pelon, J.↗
NASA NTRS1987

Titanium-doped sapphire laser research and design study

Three main topics were considered in this study: the fundamental laser parameters of titanium-doped sapphire, characterization of commercially grown material, and design of a tunable, narrow-linewidth laser. Fundamental parameters investigated included the gain cross section, upper-state lifetime as a function of temperature and the surface-damage threshold. Commercial material was found to vary widely in the level of absorption of the laser wavelength with the highest absorption in Czochralski-grown crystals. Several Yi:sapphire lasers were constructed, including a multimode laser with greater than 50mJ of output energy and a single-transverse-mode ring laser, whose spectral and temporal characteristics were completely characterized. A design for a narrow-linewidth (single-frequency) Ti:sapphire laser was developed, based on the results of the experimental work. The design involves the use of a single-frequency, quasi-cw master oscillator, employed as an injection source for a pulsed ring laser.

Moulton, Peter F.↗
NASA NTRS1973

Dye laser tuning with pellicles.

Thin nitrocellulose membranes (pellicles) are shown to exhibit properties which make them suitable for intracavity tuning elements in high-energy pulsed dye lasers. Uncoated pellicles of 2-micron and 8-micron thickness with surface figures of lambda/1 are shown to closely approximate the properties of low-finesse etalons with wide free spectral ranges. Pellicles of 8-micron thickness, coated on both surfaces with 50% reflectivity multilayer dielectrics, are shown to be effective as spectral narrowing elements with peak transmission greater than 80% and resultant laser linewidths of 0.57 nm full width at half-maximum.

Mumola, P. B.↗
NASA NTRS1997

Mid-Infrared Observations of the Galactic Center

Under this grant, Susan Stolovy completed her thesis work and performed an analysis of the galactic center. For her thesis Susan analyzed observations of the galactic center obtained with the KAO using the KEGS spectrograph, built at Cornell. These observations present a study of the distribution and kinematics of the atomic gas in the inner few parsecs of the Galaxy as traced by the forbidden [SiII] line at 34.814 microns. The integrated [SiII] emission peaks near Sgr A* and extends past the inner edge of the Circumnuclear Disk (CND), passing through a gap in the dense molecular material to the northwest. The [SiII] maps have a spatial resolution of 15" and a spectral resolution of 50 km/s. The spectra, which are characterized by broad linewidths of order 100 km/s, are kinematically consistent with the CND rotation to the southwest but not to the north. The northern extension may be experiencing shocks and is likely to be infalling along the Northern Arm. Observations of high [Sill]/ [OI] and [SiII]/dust continuum ratios support the conjecture that turbulent motions and shocks in the inner few parsecs of the Galaxy are destroying dust grains, thus elevating the abundance of atomic silicon.

Stolovy, Susan↗
NASA NTRS1984

Symmetry-dependent broadening parameters for methane

Experimental results for the pressure-broadened linewidths gamma of methane are presented and compared with theoretical results. A solar Fourier transform spectrometer with spectral resolving power of about one million was used together with a 6-m base length multitraversal absorption cell. Pressures were determined to an accuracy of + or - 0.2 Torr by means of a capacitance manometer. The pressuring gases were N2, H2, and He. Results are presented for numerical averages of all linewidths corresponding to a given tetrahedral symmetry for J = 0-6. For all cases studied, gamma(E) is found to be substantially less than gamma(A), and gamma(A) is found to be near to, but significantly smaller than, gamma(F). Relative inelastic cross sections calculated for argon scattering from methane are compared with relative pressure-broadened linewidths measured in several experiments involving methane and other gases.

Fox, K.↗
NASA NTRS1990

Electrooptic modulation methods for high sensitivity tunable diode laser spectroscopy

A CdTe phase modulator and low power RF sources have been used with Pb-salt tunable diode lasers operating near 8 microns to generate optical sidebands for high sensitivity absorption spectroscopy. Sweep averaged, first-derivative sample spectra of CH4 were acquired by wideband phase sensitive detection of the electrooptically (EO) generated carrier-sideband beat signal. EO generated beat signals were also used to frequency lock the TDL to spectral lines. This eliminates low frequency diode jitter, and avoids the excess laser linewidth broadening that accompanies TDL current modulation frequency locking methods.

Glenar, David A.↗
NASA NTRS1990

Active frequency stabilization of a 1.062-micron, Nd:GGG, diode-laser-pumped nonplanar ring oscillator to less than 3 Hz of relative linewidth

Results are presented on the frequency stabilization of two diode-laser-pumped ring lasers that are independently locked to the same high-finesse interferometer. The relative frequency stability is measured by locking the lasers one free spectral range apart and observing the heterodyne beat note. The resultant beat note width of 2.9 Hz is consistent with the theoretical system noise-limited linewidth and is approximately 20 times that expected for shot-noise-limited performance.

Day, T.↗
NASA NTRS1979

Optical feedback effects on the performance of Pb/1-x/Sn/x/Se semiconductor lasers

The effects of optical feedback on the performance of Pb(1-x)Sn(x)Se semiconductor lasers are reported. Experimental results are presented to demonstrate that uncontrolled optical feedback can occur from optics external to the laser cavity and that these external optical elements can result in the formation of a composite cavity. This composite cavity can sustain a number of narrow closely spaced emission modes with the spectral characteristics of these modes dependent upon the parameters of the cavity. With weak feedback, the spectral width of the amplitude envelope of the new lasing modes resembles that of the original laser mode with no optical feedback. With strongly coupled feedback the envelope of the external cavity modes substantially broadens the apparent linewidth of the laser. It is shown that these effects can be eliminated, and, moreover, they offer the potential for obtaining spectrally narrow single-mode emission from Pb-salt lasers through the use of carefully designed external cavities.

Harward, C. N.↗